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D r. L j u b i s a P e r i c, A u t h o r
COUPLED TENSORS OF
PIEZOELECTRIC
MATERIALS STATE
AND APPLICATIONS
Published 2005 in Switzerland by MPI
430 pages, Copyright © by MPI
All international distribution rights exclusively reserved for MPI
CONTENTS
List of Symbols
1. INTRODUCTION …………………………..……………...…….……...………….…………...1
9. CONCLUSION …………………………………………………..……………………...…….353
L i t e r a t u r e .………………………………………………...……………………...………...361
TθθD = c12D S rr + c11D Sθθ + c13D S zz − h31 Dz , TθθE = c12E S rr + c11E Sθθ + c13E S zz − e31 E z ,
TzzE = c13E (S rr + Sθθ ) + c33E S zz − e33 E z ,
T = c ( S rr + Sθθ ) + c S zz − h33 Dz ,
D D D
zz 13 33
DzE = e31 (S rr + Sθθ ) + e33 S zz + ε 33S E z .
E zD = −h31 ( S rr + Sθθ ) − h33 S zz + Dz / ε 33S .
∑ F jD v Dj + V D I = ∑ F jE v Ej + I EV ,
j =1 j =1
n = 2, 3, 4, ... , k .
Then follows:
n −1 n −1 n −1 n −1
V
z +
D
nn ∑z D
in
vi +
D
∑z D
nj
v +
D
j ∑∑ z D
ij
viD v jD
Zp = = n = 2, 3, 4, ... , k .
i =1 j =1 i =1 j =1
n −1 n −1 n −1 n −1
,
∑z ∑z ∑∑ z
I
z nnE + E
in
vi E + E
nj
v jE + E
ij
v jE viE
i =1 j =1 i =1 j =1
D E
z ijD , z njD , z nn , z ijE , z njE and z nn - internal mechanical and electric impedances, transfer functions of system (black box).
Comparison of derived formula by computer simulation using software package MATLAB, with analogous
characteristic obtained by experimental measuring on Automatic Network Analyzer HP4194A, shows results at
least 50% better than all known results published until now in scientific literature available to me.
Formula is applicable on: 1D, 2D, and 3D oscillating models of piezoelectric ceramic bodies, whose number of surfaces
S n [m ] may extend to infinity (n →∝). Also, it can join different assumed oscillation models (any combination of: 1D, 2D,
2
and 3D model) of the same piezoceramic specimen loaded under equal conditions in the same period of time.
7
1 – Case: n = 2 - 1D model (transversal oscillation of the: circular plate, circular-ring plate,
rectangular plate etc; or longitudinal oscillation of a: free beam, cantilever, cylinder, circular-ring
cylinder, circular-ring sectional cylinder, etc.):
F1D v1D + V D I = F1E v1E + I EV ,
V ( z11D v1D + z12D v2D + z13D )v1D + ( z 21D v1D + z 22D v2D + z 23D )v2D + z31D v1D + z32D v2D + z33D
Zp = = .
I ( z11E v1E + z12E v2E + z13E )v1E + ( z 21E v1E + z 22E v2E + z 23E )v2E + z31E v1E + z32E v2E + z33E
3 – Case: n = 4 - 3D model (3D oscillation of the: circular plate, circular-ring plate, rectangular plate,
free beam, cantilever, cylinder, circular-ring cylinder, circular-ring sectional cylinder, etc.):
F1D v1D + F2D v 2D + F3D v3D + V D I = F1E v1E + F2E v 2E + F3E v3E + I EV ,
V (z11Dv1D + z12Dv2D + z13Dv3D + z14D)v1D +(z21Dv1D + z22Dv2D + z23Dv3D + z24D)v2D +(z31Dv1D + z32Dv2D + z33Dv3D + z34D)v3D + z41Dv1D + z42Dv2D + z43Dv3D + z44D
Zp = = E E E E E E E E E E E E E E E E E E E E E E E E E E E E E E E .
I (z11v1 + z12v2 + z13v3 + z14)v1 +(z21v1 + z22v2 + z23v3 + z24)v2 +(z31v1 + z32v2 + z33v3 + z34)v3 + z41v1 + z42v2 + z43v3 + z44
kg
For PZT8 circular plate with dimensions: 2a 2 = 50 [mm] , 2h = 3[mm] , ρ = 7600[ ] , whose coefficients are:
m3
c11E = 13,7 ⋅ 1010 [ N / m 2 ], c12E = 6,97 ⋅1010 , c13E = 7,16 ⋅1010 , c33E = 12,4 ⋅1010 , h31 = −7,8 ⋅10 8 [V / m], h33 = 26,9 ⋅10 8 [V / m],
D
c11 = 14 ⋅ 1010 [ N / m 2 ], c12D = 7,28 ⋅1010 , c13D = 6,08 ⋅1010 , c33D = 16,1 ⋅1010 , e31 = −4 [C / m 2 ], e33 = 13,8 , ε 33S / ε 0 = 582,
D
z F1
I D
v3 F D
v1D
⎧F1D ⎫ ⎡ z11D z14D ⎤⎧v1D ⎫
3
- v2D v3D z12D z13D
⎪ D⎪ ⎢ D D ⎥⎪ D ⎪
⎪F2 ⎪ ⎢ z21 ⎥⎪v2 ⎪.
+ 3D model D D
D z22 z23 z24
⎨ D⎬ = ⎢ D
V
D ⎥⎨ D ⎬
a D D
2h
F2 F3 D D
Black Box
⎪F3 ⎪ ⎢ z31 z32 z33 z34 ⎪v3 ⎪
r
D ⎥⎪
D
v1D
F1
⎪⎩V D ⎪⎭ ⎣⎢ z41
D D
z42 D
z43 z44 ⎦⎥⎩ I ⎪⎭
VD
v2D F
D I
a) 2 b)
E
z F1
I
E
v3E F E
v1E
3
- v2E v3E ⎧F1E ⎫ ⎡ z11E z12E z13E z14E ⎤⎧v1E ⎫
+ 3D model ⎪ E⎪ ⎢ E E ⎥⎪ E ⎪
⎪F2 ⎪ ⎢ z21 ⎥⎪v2 ⎪.
E E
V a E z22 z23 z24
⎨ E⎬= ⎢ E
E
2h
E ⎥⎨ E ⎬
F2 F3
Black Box E E
⎪F3 ⎪ ⎢ z31 z32 z33 z34 ⎪v3 ⎪
r
E ⎥⎪
F1
v1E V E
⎪⎩ I E ⎪⎭ ⎢⎣ z41
E E
z42 E
z43 z44 ⎥⎦⎩ V ⎪⎭
v2 FE E I
c) 2 d)
8
Formula provides following simulated characteristic of electric impedance model, which is
compared with analogous, obtained by measuring on Automatic Network Analyzer HP4194A:
9
Zp
Circular plate: PZT 8, 2a=50, 2h=3, h/a=0,06
R1
Experiment
R2 T1
Model
R3
R4
f
Knowing values of resonant frequencies is an initial condition during design of piezoceramic elements.
From the picture above one may see that by this formula one may determine several exact positions of
radial resonant modes R1, R2, R3 and R4, and transversal mode T1, which are the most frequently used
in technical practice and application.
4 – Case: n = 5 - 3D model (rectangular plate, free beam, etc.):
F1D v1D + F2D v 2D + F3D v3D + F4D v 4D + V D I = F1E v1E + F2E v 2E + F3E v3E + F4E v 4E + I EV ,
V (zDv D + zDv D + zDv D + zDv D + zD )v D +...+ (z41Dv1D + z42Dv2D + z43Dv3D + z44Dv4D + z45D )v4D + z51Dv1D + z52Dv2D + z53Dv3D + z54Dv4D + z55D
Zp = = 11E 1 E 12E 2 E 13E 3E 14E 4E 15E 1E .
I (z11v1 + z12v2 + z13v3 + z14v4 + z15)v1 +...+ (z41E v1E + z42E v2E + z43E v3E + z44E v4E + z45E )v4E + z51Ev1E + z52E v2E + z53E v3E + z54E v4E + z55E
F1D v1D + F2D v 2D + F3D v3D + F4D v 4D + F5D v5D + V D I = F1E v1E + F2E v 2E + F3E v3E + F4E v 4E + F5E v5E + I EV ,
V (zDvD + zDvD + zDvD + zDvD + zDvD + zD)vD +...+(z51Dv1D + z52Dv2D + z53Dv3D + z54Dv4D + z55Dv5D + z56D)v6D + z61Dv1D + z62Dv2D + z63Dv3D + z64Dv4D + z65Dv5D + z66D
Zp = = 11E 1 D 12E 2 E 13E 3 E 14E 4E 15E 5E 16E 1E .
I (z11v1 + z12v2 + z13v3 + z14v4 + z15v5 + z16)v1 +...+(z51Ev1E + z52Ev2E + z53Ev3E + z54Ev4E + z55Ev5E + z56E )v6E + z61Ev1E + z62Ev2E + z63Ev3E + z64Ev4E + z65Ev5E + z66E
…, etc.
10
2h
v1 Black Box
F3 F4
a2
F2
v2 U0
I
v3 F
3
a) b)
Figure 8.121. – 3D model of circular-ring plate
It may be seen that circular-ring plate may be observed as black box device with five
variable parameters (five input-output values). First group of values (usually used as input –
leading of electric energy on plate coatings from electric generator of alternate voltage) is
electric voltage U 0 and electric current strength I. Remained four groups of values conform to
cylindric surfaces - r = a1 (surface force F1 and velocity v1 ), r = a 2 (surface force F2 and
velocity v 2 ), and plane mutually opposite surfaces z = − h (surface force F3 and velocity v3 ), and
z = h (surface force F4 and velocity v4).
Oscillations of circular-ring plate are excited by leading of alternate difference of electric
potential 2U 0 e iω t on surfaces z = ± h. Plate oscillations, i.e., vibration of particles, have radial-
r r r
transversal character of motion, that is s = u (r , t ) r0 + w( z , t )k .
Equations of piezoelectric effect, which are used in this analysis and procedure of derivation is
identical with procedure in item 8.5.2♣, expressions (8.271) ÷ (8.275).
Partial differential equations of oscillation of circular-ring plate:
⎛ ∂ 2 u 1 ∂u u ⎞ ∂ 2u
⎜
c ⎜ 2 +
D
− ⎟ =ρ 2 ,
⎝ ∂r r ∂r r 2 ⎟⎠ ∂t
11
(8.321)
∂2w ∂2w
D
c33 =ρ
∂z 2 ∂t 2
♣
8.5.1. 3D model of oscillations of circular plate
11
r I
view(-15,50) f view(160,30) r
) ) ) )
Figure 8.122. – Componential displacement u = u ( f , r ) Figure 8.123. – Componential displacement u = u (r , I )
) prog209 ) prog210
u u
I a1 / a 2
view(160,30) f view(-120,30) f
) ) ) )
Figure 8.124. – Componential displacement u = u ( f , I ) Fig. 8.125. – Component. Displacement u = u ( f , a1 / a 2 )
) prog211 ) prog212
u u
2h I
view(150,60) f view(70,30) 2h
) ) ) )
Figure 8.126. – Componential displacement u = u ( f , 2h) Figure 8.127. – Componential displacement u = u ( I , 2h)
) prog213
u
I
r
view(120,60) 2h a1 / a 2
12
) prog214
u
view(80,50)
) ) ) )
Figure 8.128. – Componential displacement u = u (r , 2h) Fig. 8.129. – Component. Displacement u = u ( I , a1 / a 2 )
) prog216
w
z=b
view(160,30) f
) ) ) )
Figure 8.130. – Componential displacement w = w( f , z ) Figure 8.131. – Componential displacement w = w( f , I )
) prog216 ) prog217
w w
z =b/2
I a1 / a 2
view(160,30) f view(-120,30) f
) ) ) )
Figure 8.132. – Componential displacement w = w( f , I ) Fig. 8.133. – Component. Displacement w = w( f , a 1 / a 2 )
) prog218 ) prog219
w w
f = 5 ⋅ 105
I z
a1 / a 2
view(160,30) z view(50,60)
) ) ) )
Figure 8.134. – Componential displacement w = w( z , I ) Fig. 8.135. – Component. Displacement w = w( z , a1 / a 2 )
) prog219
w
13
) prog220
w
f = 4 ⋅ 105
view(110,30) a1 / a 2
) ) ) )
Fif. 8.136. – Component. Displacement w = w( z , a1 / a 2 ) Fif. 8.137. – Component. Displacement w = w( I , a1 / a2 )
) prog300 ) prog301
Ez Ez
f f
view(110,50) view(110,50)
) ) ) )
Fif. 8.274. – Electric field E z = E z ( f , Z 1 / Z 2 ) Fif. 8.275. – Electric field E z = E z ( f , Z 3 / Z 4 )
100 70
prog200 1D Mason-ov
90 realizovani transverzalni model
R2 3D model R2 T1
T1 60 R1 realizovani
80 3D model
70 50
R1
60
Z ul [dB]
40
Z ul [dB]
50
R3 30 R3
40
R4
30 R4
20
20
10
10
0 0
0 1 2 3 4 5 6 0 1 2 3 4 5 6
5 5
f [Hz] x 10 f [Hz] x 10
Figure 8.276. - Electric impedance Z ul = Z ul ( f ) Figure 8.277. - Electric impedance Z ul = Z ul ( f )
70 70
2D radijalni model
3D model 3D Brissaudov T1
60 R1 R2 T1 60 R1 R2
model
realizovani
3D model
50 50
40 40
Zul [dB]
Zul [dB]
30 30
R4
R4
20 20
10 10
0 0
0 1 2 3 4 5 5 6 0 1 2 3 4 5 5
6
f [Hz] x 10 f [Hz] x 10
♣
8.5.4. Second approach to the problem of 3D oscillations of circularring plate.
15
70 70
Z1=Z2=Z3=Z4=400 Rayl Z1=Z2=Z3=Z4=400 Rayl
R2 T1 R2 T1
60 R1 60 R1
Z1=Z2=Z3=400 Rayl Z1=3 MRayl
Z4=5 MRayl Z2=Z3=Z4=400 Rayl
50 50
Z1=Z2=400 Rayl Z1=Z2=3 MRayl
Z3=Z4=5 MRayl Z3=Z4=400 Rayl
40 40
Z ul [dB]
Zul [dB]
30 R3 30 R3
R4 R4
20 20
10 10
0 0
0 1 2 3 4 5 5
6 0 1 2 3 4 5 5 6
f [Hz] x 10 f [Hz] x 10
In order to further represent capabilities of proposed 3D model on Figure 8.282. and 8.283.,
dependence of electric impedance in function of frequency f and thickness of the ring 2h is presented.
16
prog201 prog201
Zul
Z ul
2h 2h
f f
view(-20,60) view(-160,60)
Figure 8.282. - Electric impedance Z ul = Z ul ( f , 2h) Figure 8.283. - Electric impedance Z ul = Z ul ( f , 2h)
prog202
prog202
Z ul
Z ul
a1
a1
a2
a2
a1 / a2
view(-80,60) f view(110,60) f a1 / a2
view(110,60) f
view(-80,60) f
Figure 8.284. - Electric impedance Z ul = Z ul ( f , a1 / a 2 ) Figure 8.285. - Electric impedance Z ul = Z ul ( f , a1 / a 2 )
17
As expected, one may see (Figure 8.284. and Figure 8.285) that change of radius ratio has
the greatest influence on state of radial resonant modes, thereat one may notice an interesting
phenomenon that first radial resonant mode moves to lower frequencies, while other radial
resonant modes tend to higher frequencies, and thereat considerably affect the transversal resonant
mode. This influence of internal radius on resonant frequency of transversal oscillations was not
analyzed till now in the field of modelling of piezoceramic circular-ring plates and ultrasonic
sandwich transducers. Similarly to the previous case, alteration of area size of metalized surface
due to the alteration of internal radius generates alteration of its capacitance, and by itself also
change of level value of input electric impedance.
Results from previous analysis can be presented more clearly through diagrams of spatial
states of input electric impedance Z ul in function of frequency and applied external load (applied
acoustic impedance) Z 3 and Z 4 . Spatial diagrams of input electric impedance presented on Figure
8.286. and 8.287 conform to the input electric impedance from Figure 8.280., while spatial
diagrams of input electric impedance presented on Figure 8.288. and 8.289 conform to the input
electric impedance from Figure 8.281. On these Figures are clearly noticed values of external
(acoustic) loads at which some resonant modes disappear.
Transversal (crossing) mode of oscillation disappears with increase of external load in
direction of polarization axis across thickness of circular-ring plate (Figure 8.286. and Figure
8.287). Radial mode of oscillation disappears with increase of acoustic load Z 1 and Z 2 in radial
direction on cylindric surfaces of circular-ring plate (Figure 8.288. and Figure 8.289). However,
since it is about coupled tensors of state, these influences are not isolated (independent), but also
the resonant modes are coupled. From Figure 8.286. and 8.287. One may see that changes at
transversal resonant mode also affect changes of the third and fourth radial mode of oscillation,
which are closest to the transversal mode, and at high external loads they also affect changes of
distant radial resonant mode of oscillation.
prog203 prog203
Z ul Z ul
Z3 = Z4
Z3 = Z4
f f
view(110,40) view(-115,40)
Fig. 8.286. - Electric impedance Z ul = Z ul ( f , Z 3 = Z 4 ) Fig. 8.287. - Electric impedance Z ul = Z ul ( f , Z 3 = Z 4 )
prog204
Z ul
18
prog204
Z ul
Z1 = Z 2
Z1 = Z 2
f
view(110,40) view(-120,30)
Fig. 8.288. - Electric impedance Z ul = Z ul ( f , Z 1 = Z 2 ) Fig. 8.289. - Electric impedance Z ul = Z ul ( f , Z 1 = Z 2 )
Mutual arrangement of radial and transversal resonant modes of oscillation depend of
relation between internal and external radius, as well as of thickness of the piezoceramic circular-
ring plate itself (figures 8.282, 8.283, 8.284, and 8.285). For definite concrete dimensions of
piezoceramic circular-ring plate resonant modes of oscillation may be very close, and analyzed
mechanical external load caused by acoustic impedances, can generate, besides intensity decrease
of resonant modes, also their frequency shift. So, for example, at circular-ring plate with small
external diameter and greater height, cylindric lateral surfaces become dominant, and lateral
external radial loads (acoustic impedances) have significant influence on radial resonant modes of
oscillation. In these cases, disappearing of radial modes with increase of external load can generate
frequency shift of transversal mode of oscillation because of their very significant mutual coupling
(coupled tensors of piezoelectric material state).
♣
8.5.4. Second approach to the problem of 3D oscillations of circular-ring plate.
19
so in space. Other programmes used in this dissertation are similar, and they are not presented because of
volume and complexity of exposed matter. Dependence of electric impedance of frequency, for
piezoceramic circular-ring plates and circular plates, is experimentally measured by automatic network
analyzer HP4194A♣, and comparative results are presented on Figures 8.291, 8.293, 8.295, 8.297, 8.299,
8.301.
On Figure 8.290. is presented characteristic of modulus of input electric impedance, simulated
numerically on computer in function of frequency, for PZT8 piezoceramic circular-ring plate with
dimensions 2a1 = 4 [mm], 2a 2 = 10 [ mm], and 2h = 2 [mm]. It is assumed that oscillation is
performed in air without additional external loading.
On Figure 8.291. is presented comparison of quoted numerically simulated and measured
experimental dependence of modulus of input electric impedance.
From Figure 8.290. and 8.291. one may see that forms and calculated values of input electric
impedances, as well as calculated values of resonant and antiresonant frequency of oscillation for circular-ring
piezoceramic plate, are very close to the correspondent experimentally obtained results, as for the first radial
mode of oscillation R1, as well as for the first transversal (crossing) mode of oscillation T1.
80 80
model prog205
T1 eksperiment
70 R2 70 R2 T1
R1 R1 model
60 60
50 50
Zul [dB]
Zul [dB]
40 40
30 30
R3 R3
20 20
10 10
0 0
0 2 4 6 8 10 12 14 16 18 0 2 4 6 8 10 12 14 16 18
f [Hz] x 10
5 f [Hz] x 10 5
Figure 8.290. - Electric impedance Z ul = Z ul ( f ) Figure 8.291. - Electric impedance Z ul = Z ul ( f )
♣
Network Impedance Analyzer.
20
80 80
model prog205 eksperiment
70 70 model
60 R2 T1 60 R2 T1
50 R1 R4 50 R4
R1
Zul [dB]
Zul [dB]
40 40
30 30
20 R3 20 R3
R5 R5
10 10
0 0
0 1 2 3 4 5 6 7 8 0 1 2 3 4 5 6 7 8
5
f [Hz] x 10 f [Hz] x 10 5
80 80
60 60 R2
R2
R3 R3
R1 R1
50 50
T1 T1
Zul [dB]
Zul [dB]
40 40
30 30
20 20
10 10
0 0
0 0.5 1 1.5 2 2.5 3 3.5 4 4.5 5 0 0.5 1 1.5 2 2.5 3 3.5 4 4.5 5
f [Hz] 5
x 10 f [Hz] x 10 5
First radial mode R1 and first transversal mode T1 are the most often-used modes of oscillation at
piezoelectric transducers in practical application. Adopted and analyzed model, as one may see, predicts
with very good accuracy these modes of oscillation at different types of piezoceramic circular-ring
specimens. Transversal mode of oscillation T1 is most frequently used at ultrasonic high frequency
21
transducers. However, there is often need in practice for use of transducers at lower frequencies.
Obtaining of lower operating resonant frequencies is possible to realize by application of Langevin’s
sandwich transducer, or simple piezoceramic circular-ring plate (or circular plate), which oscillates in
its first radial mode R1. At first radial resonant mode R1 a considerable stressing in transversal (crossing)
direction exists because of the elastic coupling and high interaction between coupled tensors of state of
piezoelectric materials. Analysis of the cited transversal oscillation of circular-ring piezoceramic plate is
enabled by proposed 3D model, and it may be broadened on cylindric piezoceramic bodies in shape of
circular plates. Adopted 3D model considers mutual coupling of transversal and radial oscillations, and
thereby is possible to determine optimal geometry of circular-ring plate or circular plate, in order to
obtain increased displacement in transversal direction during oscillation in region of the first radial mode.
60 60
R1
model prog206 (a) eksperiment T1
T1 model
50 50 R1
R2 R2
40 40
Zul [dB]
Zul [dB]
30 30
20 20
10 10
0 0
0 1 2 3 4 5 6 7 8 9 10 0 1 2 3 4 5 6 7 8 9 10
f [Hz] x 10
5
f [Hz] x 105
Figure 8.296. - Electric impedance Z ul = Z ul ( f ) Figure 8.297. - Electric impedance Z ul = Z ul ( f )
On Figure 8.296. is presented characteristic of modulus of input electric impedance, simulated
numerically on computer in function of frequency, for PZT8 piezoceramic circular plate with
dimensions 2a 2 = 50 [mm], and 2h = 3 [mm]. It is assumed that oscillation is performed in air without
additional external loading. On Figure 8.297. is presented comparison of numerically simulated and
experimentally measured dependence of modulus of input electric impedance.
On Figure 8.298. is presented characteristic of modulus of input electric impedance, simulated
numerically on computer in function of frequency, for PZT4 piezoceramic circular plate with
dimensions 2a 2 = 20 [mm], i 2h = 5 [mm]. It is assumed that oscillation is performed in air without
additional external loading. On Figure 8.299. is presented comparison of numerically simulated and
experimentally measured dependence of modulus of input electric impedance.
22
80 80
prog206 R1 T1
R2 R1 eksperiment T1
70 70
model
R2
60 model 60
50 50
Zul [dB]
Zul [dB]
40 40
30 30
20 20
10 10
0 0
0 0.5 1 1.5 2 2.5 3 3.5 4 4.5 5 0 0.5 1 1.5 2 2.5 3 3.5 4 4.5 5
f [Hz] 5 f [Hz] x 10 5
x 10
Figure 8.298. - Electric impedance Z ul = Z ul ( f ) Figure 8.299. - Electric impedance Z ul = Z ul ( f )
40 40
30 30
R4 R4
20 20
10 10
0 0
0 0.5 1 1.5 2 2.5 3 3.5 4 4.5 5 0 0.5 1 1.5 2 2.5 3 3.5 4 4.5 5
f [Hz] x 10
5 f [Hz] x 10 5
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