You are on page 1of 11

PHYSICAL REVIEW B 71, 184508 共2005兲

Dynamics and thermal instability of magnetic flux in type-II superconductors


B. Ya. Shapiro,1,* I. Shapiro,1 B. Rosenstein,2 and F. Bass1
1Department of Physics, Bar Ilan University, Ramat Gan 52100, Israel
2Department of Electrophysics, National Chiao Tung University, Hsinchu, Taiwan, Republic of China.
共Received 8 June 2004; revised manuscript received 17 November 2004; published 17 May 2005兲

In recent experiments, trapped magnetic flux is initially generated by abrupt laser heating of a strip of a
type-II superconducting film subjected to a weak magnetic field. We study herein the nonequilibrium penetra-
tion of the flux into the Meissner state area. Effects of the heat dissipation and transport on the motion and
stability of the interface between the magnetic flux and flux-free domains are considered. It is shown that the
magnetic induction and the temperature have the form of a shock wave moving with constant velocity as large
as that corresponding to the depairing current. In the vicinity of the front, superconductivity is suppressed by
strong screening currents. The front velocity is determined by the Joule heat caused by the electric current in
the normal domain at the flux front. The stability of the shock wave solution is investigated both analytically
and numerically. For sufficiently small heat diffusion constant a finger shaped thermal instability is found.

DOI: 10.1103/PhysRevB.71.184508 PACS number共s兲: 74.20.De, 74.25.Ha, 74.25.Qt

I. INTRODUCTION initially fills the normal domain. Recovery of superconduc-


The dynamics of magnetic flux penetration into a type-II tivity occurs in two stages. Once the short pulse is over, the
superconductor and its instabilities have been studied by a strip cools and the flux nucleates into a dense system of
variety of techniques over the years, 共see Ref. 1, and refer- Abrikosov vortices. The characteristic time of that stage is
ences therein兲. Magneto-optics experiments2 demonstrate microscopic, of order of the Ginzburg-Landau 共GL兲 relax-
that in a wide range of situations there exists a well-defined ation time 共appearing in the time dependent GL equations兲
interface 共front兲 between the magnetic flux penetrating into tGL ⬃ 10−10 s. This process has been studied by us some time
the sample and the flux-free Meissner state. Improvements to ago11 and we do not address this stage in the present paper
since it was shown that no instability is originated at this
these magneto-optical techniques have revealed a wide class
stage.
of instabilities, including magnetic macroturbulence3,4 and a
On the larger 共mesoscopic兲 time scale the rapidly created
dendritic instability.5 The instability of the magnetic flux and vortices are pushed into the superconducting part of the
flux avalanches are observed both in anisotropic high tem- sample. The fluxons move very fast with velocities of order
perature superconductor4 and in an isotropic material like of 105 cm/ s 共in YBCO兲.10 The flux flow currents, J, in this
Nb.5 case are much higher than the critical current Jc typical for
Traditionally there are three possible scenarios in which the thermodynamic Bean model critical state, but smaller
the instabilities could arise. The standard thermomagnetic 共although not much smaller兲 than the depairing current Jd:
instabilities appear when the critical vortex state6 is per- Jd ⬎ J Ⰷ Jc. Just after the vortex nucleation stage the mag-
turbed locally by the heat released by a moving vortex. This netic flux forms a rapidly moving front. This highly nonequi-
dissipation leads to the thermal softening of the vortex sys- librium relaxation dynamics is very different from the essen-
tem which in turn is responsible for the instability.1 In this tially adiabatic dynamics of the critical state discussed
case the instability develops around a well defined thermo- earlier. The front line shape is not always stable: sometimes
dynamically stable Bean state. There is no moving front in it dynamically develops dendriticlike structures.12
this case. A different type of thermal instability, namely the The existence of the sharp and typically straight front can
thermal overheating instability of the steady flux-antiflux be in principle understood in the framework of the theory of
front, was considered theoretically by some of us.7 In this nonlinear magnetic flux diffusion.13,14 Geshkenbein et al.
case the excess heat released at the front is caused by vortex- considered the flux diffusion in the creep regime, while Sha-
antivortex annihilation. Yet another type of instability occurs piro et al.14 considered the flux flow regime. In both cases
in strongly anisotropic superconductors.8,9 In this case the the temperature gradient effects were neglected and no insta-
stationary vortex-antivortex interface is destroyed by the bility of the front was predicted, namely, it was shown that
Thomas-Kelvin instability. corrugation of the front line is unfavorable. The front veloc-
Recently, a type of flux instability was observed experi- ity under these assumptions decreases with time.14 However,
mentally. In these experiments superconductivity was locally corrugation of the front is typically caused by thermal
destroyed in a completely nonadiabatic fashion by a femto- effects,1 hence, one expects that in the case of fast dynamics
second laser pulse.10 The pulse clearly forces the system out of the front, these effects are even more important.
of thermal equilibrium. The superconductivity is destroyed In the present paper we study both numerically and ana-
inside a narrow strip of a YBCO film subjected to a magnetic lytically the dynamics of the nonadiabatically created mag-
field perpendicular to the film. The field does not exceed the netic flux in sufficiently thick 共thickness larger than the mag-
first critical field Hc1, so that initially fluxons cannot pen- netic penetration length兲 superconducting films. In particular,
etrate the rest of the sample. Therefore the magnetic flux effects of dissipation and the heat transport on the motion

1098-0121/2005/71共18兲/184508共11兲/$23.00 184508-1 ©2005 The American Physical Society


B. YA. SHAPIRO, I. SHAPIRO, B. ROSENSTEIN, AND F. BASS PHYSICAL REVIEW B 71, 184508 共2005兲

and stability of the flux front are considered. It is shown that resistivity, one obtains R = 共4␲ / ␾20兲D f . The electric current
the Joule heat released at the flux front can produce front density in turn is equal to Ji = 共c / 4␲兲␧ijⵜ jB. The flux diffu-
propagation at constant velocity inside the type-II supercon- sion equation then takes the form

冋 册 冋 册
ductor. Heating of the front by the moving magnetic flux is
essential. We found that for certain voltage–current charac- 4␲ ⳵ B ⳵ ⳵B ⳵ ⳵B
= R + R . 共5兲
teristics of the superconductor in its resistive state, the mag- c2 ⳵ t ⳵ x ⳵x ⳵y ⳵y
netic induction penetrating a flux-free superconductor forms
a sharp front. Strong superconducting currents in the vicinity The function R共B , T兲 will be phenomenologically defined in
of the front suppress superconductivity in this area and create the next subsection. In the normal state the same equation
a normal domain at the front. The interface moves with con- applies with the normal state resistivity.
stant velocity which is completely determined by the Joule Now we turn to the heat transport equation, identical to
heat released in the normal domain at the leading edge of the the conventional normal state heat balance equation
front. The straight front line shows an instability with respect ⳵T
to local temperature fluctuations. In fact an excessive local C = Dⵜ2T + J · E共B,T兲 − ␥C共T − T0兲. 共6兲
⳵t
temperature at the front leads to excessive Joule heat re-
leased there and in turn increases the local front velocity in Here C is the heat capacity and D is the heat diffusion con-
the area of the fluctuation. The hydrodynamical tangential stant, T0 is the temperature of the cooling liquid with ␥
instability of the flux front destroys the flat front. Numerical = 1 / tr being the heat relaxation constant, when tr the heat
simulation of the exact set of nonlinear equations allows us relaxation time. The first term on the right hand side is the
to study the evolution of the instability and demonstrates the heat conduction, the second is the Joule heat, and the third
emergence and development of the corrugated interface. describes the heat exchange between the slab and the cooling
liquid. The Joule heat term consists of two different contri-
II. MODEL AND BASIC EQUATIONS butions. In the mixed state it is dominated by the motion of
the magnetic flux, while in the normal metal when the super-
A. Hydrodynamics of the vortex matter conductivity is suppressed by the currents, one has usual
(for the slab geometry) Ohmic resistance losses.
Let us consider a typical experimental situation 共see Ref. In the geometry we consider 共see Fig. 3兲, the dependence
12兲, when a relatively thick 共with thickness larger than mag- of both the temperature and the magnetic induction on z can
netic penetration depth ␭兲 type-II superconducting film is be neglected. The magnetic induction is independent of z,
subjected to a weak external magnetic field 共B ⬍ Bc1兲. The since thickness of the thick film 共slab兲 in the z direction is
magnetic induction B therefore has only a z component Bz assumed to be larger than the magnetic penetration length ␭,
⬅ B and all dependencies on the z coordinate can be ne- while the temperature is uniform in the z direction, despite
glected. The two dimensional vortex systems is described by the presence of the last term, since the thermal diffusion
the magnetic induction B共r , t兲 and the temperature profile length is typically much larger than the film’s thickness. The
T共r , t兲, where r = 共x , y兲 is a two dimensional vector. To derive detailed argumentation is presented in Ref. 15.
the hydrodynamic equations one starts from the continuity
equation for the fluxon density n共r , t兲 = 兺a␦关r − ra共t兲兴 and the B. Resistivity at high currents
flux current Ii共r , t兲 = 兺avai 共t兲␦关r − ra共t兲兴. Here i = x , y and a As a rule, the nonlinear resistivity R共J , B , T兲
= 1 , …N labels the fluxons. The continuity equation ⬅ E共J , B , T兲 / J in the mixed state of a type-II superconductor
⳵n is a complicated function of magnetic field, current and tem-
= − ⵜ iI i 共1兲 perature, see Fig. 1. In this work we will be interested mainly
⳵t in resistivity at currents much larger than the critical current
supplemented by the constituent relation Jc, when the pinned vortices are released. The vortex resis-
tivity grows quickly above Jc either exponentially or as a
Ii共r,t兲 = D f 共r,t兲ⵜin共r,t兲 共2兲 power R ⬀ J␮ with large ␮. In this relatively low current re-
leads to the flux diffusion equation gime the dependence of the resistivity on magnetic induction
B is very smooth 共roughly linear兲. However, when the cur-
⳵ n共r,t兲 rent approaches the depairing current Jd the power ␮ be-
= − ⵜi关D f 共r,t兲ⵜin共r,t兲兴. 共3兲 comes smaller and resistivity strongly depends on B.
⳵t
Recently detailed measurements of the I–V characteristics
Since n共r , t兲 = B共r , t兲 / ␾0, where ␾0 is the unit flux, the Max- of Nb films at high current density of order 106 A / cm2 were
well equation performed.16 Near the depairing current it has the form


1 ⳵B
c ⳵t
= ␧ijⵜiE j 共4兲 R共B,T兲 = Rn共T兲 冋 J
Jd共T,B兲
册 ␮
. 共7兲

leads to the identification Ei = 共c / ␾0兲␧ijD f 共r , t兲ⵜ jn共r , t兲, Here Rn共T兲 is the normal state resistivity. The dependence of
while ␧ij is the antisymmetric tensor. Since in the mixed state the depairing current Jd on magnetic field and temperature16
of the type-II superconductor E = RJ, where R共B , T兲 is the can be fitted well by the following form:

184508-2
DYNAMICS AND THERMAL INSTABILITY OF… PHYSICAL REVIEW B 71, 184508 共2005兲

FIG. 3. The geometry of the problem. The dashed area contains


the flux that penetrated the sample during the initial period in which
FIG. 1. Schematic plot of the nonlinear resistivity of a type-II superconductivity was destroyed in a narrow strip around x = 0. The
superconductor in the mixed state as a function of current. The arrows marked with v indicate the direction of the flux front mo-
resistivity is zero below the critical current Jc, exponentially small tion. The direction of the magnetic field B is perpendicular to the xy
in the flux creep regime just above Jc and evolves into a power plane.
function in the flux flow regime. At the depairing current it merges
with the Ohmic normal state resistivity.
above Bc1 共see Ref. 17兲 in which the power law is clearly

Jd共T,B兲 = Jd0⌬ 冋 册
Bc2共T兲
B
␯/␮
. 共8兲
seen, but ␮ = 2, ␯ = 2. The corresponding data on high Tc
superconductors are not yet available for fields below Bc1, to
our knowledge, and therefore we treat the powers as phe-
The upper critical field depends on temperature as Bc2共T兲 nomenological parameters 共see also Refs. 14 and 18兲. An
= Bc2共0兲⌬, where we assumed that dimensionless tempera- additional difference between the conventional and the high
ture ␪ = T / Tc is not far from 1, namely ⌬ ⬅ 1 − ␪ is small. Tc materials is that the normal state conductivity in high Tc
When the current exceeds Jd共B , T兲, the electric field is cuprates is linear 共“strange metal”兲.
continuous, the resistivity saturates at its’ normal value
R共B , T兲 = Rn共T兲. The derivative of R appearing in the nonlin- C. Boundary and initial conditions
ear flux diffusion Eq. 共5兲 is discontinuous. We fitted the I–V
curves of Nb and obtained ␮ = 1.5 with temperature indepen- In a typical experiment12 the heat of the laser beam sup-
dent Rn. For Nb at fields of the order of Bc1 we obtain the presses superconductivity in a narrow strip of width l divid-
best fit ␯ = 1.3. The values of other material parameters are: ing the sample into two equal superconducting parts of
Bc2共0兲 = 4.43 T, Rn = 9.9 ␮⍀ cm and Tc = 8.6 K. These were length Lx on both sides of the irradiated strip. Magnetic flux
measured directly. The obtain the best fit for the constant promptly fills the normal area and forms a nonequilibrium
Jd0 = 9.2· 106 A / cm2. See Fig. 2 for a sample of data taken at vortex strip state. Subsequently the laser is switched off and
T = 7.8 K, ␪ = 0.9. sample is cooled 共see Fig. 3兲. The set of Eqs. 共5兲 and 共6兲
Of course the exponents depend on material and weakly must be supplemented by the initial and boundary conditions
depend on field for larger magnetic fields. The power law in the center of the sample and on the sample’s edges. The
however generally holds. Examples include YBCO well initial temperature is assumed to be homogeneous

T共x,y,t = 0兲 = T0 , 共9兲

where T0 is the temperature of the cooling liquid. Magnetic


field fills the irradiated area of width l and magnetic flux of
magnitude

⌽ = 2lLyB0 = 冕 B共x,y,t兲dxdy 共10兲

is assumed to be trapped in superconductor and conserved.


Here Ly is width of the sample. The boundary conditions for
temperature are

T共x = ± Lx,y = ± Ly,t兲 = T0 . 共11兲


FIG. 2. A fit of the resistivity dependence on the current density
of Ref. 16 to the model resistivity Eqs. 共7兲,共8兲 with exponents ␯ An alternative boundary condition for the magnetic induction
= 1.3, ␮ = 1.5. Magnetic field is 20 mT 共circles兲, 30 mT 共stars兲 and which we consider independently is fixed magnetic field at
40 mT 共squares兲. the center B共x = 0兲 = B0, while B共x = ± Lx兲 = 0.

184508-3
B. YA. SHAPIRO, I. SHAPIRO, B. ROSENSTEIN, AND F. BASS PHYSICAL REVIEW B 71, 184508 共2005兲

D. Basic equations in terms of dimensionless quantities III. STRAIGHT FLUX FRONT FOR ␮ = 0
Dimensionless coordinate, time, and magnetic induction A. Asymptotics in the superconducting phase
are defined using natural units of length x* = cRn共T = Tc兲
When the boundary conditions are independent of y 共see
⬅ cRn, magnetic field B* = 冑4␲CTc and time
notations in Fig. 3兲, the front is straight and the problem

t* = 4␲Rn 冉 4␲RnJd0
B*
冊冋 册

Bc2共0兲
B*

共12兲
becomes one dimensional. We start with a case when the
resistivity depends only on magnetic induction. Hence, now
we consider ␮ = 0, returning to the general case in Sec. IV A.
as follows: In addition we initially solve a simplified set dropping the
relaxation term ⌫ = 0 and diffusion ␬ = 0. This assumption
x → x/x* ; t → t/t* ; b = B/B* . 共13兲 will be supported a posteriori by calculating the terms’ ef-
For the free electron gas B is * fects and comparing with the numerical solution.
Looking for a solution of Eqs. 共15兲 and 共16兲 in the form
␭ 2k Fv F
B* ⬇ Hc1 , 共14兲 b = bs共X兲, ⌬ = ⌬s共X兲, 共22兲
c␰
where X = x − Vt is the distance from the interface and V is the
where ␭, kF, vF, and ␰ are the London penetration length, interface velocity, one obtains

冋冉 冊 册
Fermi momentum, Fermi velocity, and the coherence length

respectively. dbs d bs dbs
−V = , 共23兲
Using the scaled variables, the set of nonlinear coupled dX dX ⌬s dX
equations in the superconducting state 关J ⬍ Jd共B , T兲兴 reads
⳵b ⳵
= ␳
⳵t ⳵x ⳵x
⳵b
+ 冉 冊 冉 冊


⳵y ⳵y
⳵b
, 共15兲
V
d⌬s
dX
= PJ . 共24兲

Here the Joule power density is PJ = ␳ j2. Let us first investi-


⳵␪ gate the asymptotics of bs共X兲 in the vicinity of the front X
= ␬ⵜ2␪ + ␳ j2 − ⌫共␪ − ␪0兲, 共16兲 → 0. In the cold superconductor, the magnetic field vanishes.
⳵t
Therefore formally 共ignoring formation of the very narrow
where the dimensionless resistivity and the electric current normal region near the front which will be discussed in the
density are next subsection兲 we look at the magnetic field bs共X兲 as a

冉 冊冉 冊 冑冉 冊 冉 冊
power with coefficient dependent on velocity only for X
␯ ␮
R n共 ␪ 兲 b j ⳵b 2
⳵b 2
⬍ 0:
␳= ; j= + 共17兲
Rn ⌬ ⌬ ⳵x ⳵y
bs共X兲 = A共V兲兩X兩␣ . 共25兲
and ␪0 = T0 / Tc. The unit of current density is cB / 4␲x . The * *
The temperature is assumed to be of the form
flux diffusion equation does not contain parameters, while
the heat transfer equation has two: the dimensionless tem- ⌬s共X兲 = ⌬s0 − ⌬s1共V兲兩X兩␤ . 共26兲
perature diffusion constant ␬ and the relaxation coefficient ⌫:
Substituting the Ansatz Eqs. 共25兲 and 共26兲 into Eqs. 共23兲 and
Dt* 共24兲, one obtains on the superconducting side of the front
␬ = *2 , ⌫ = ␥t* . 共18兲 共X ⬍ 0兲:
Cx
−␯
In the region in which superconductivity is suppressed by VA␣兩X兩␣−1 = A␯+1⌬s0 ␣关共␯ + 1兲␣ − 1兴兩X兩共␯+1兲␣−2 , 共27兲
the superconducting current J exceeding the depairing cur-

rent value Jd共B , T兲, the normal state resistivity becomes R A2+␯␣兩X兩2␣−2+␣␯ = ⌬s1␤⌬s0 V兩X兩␤−1 , 共28兲
= Rn共T兲. In this case the basic equations are
which is satisfied for
⳵b ⳵
=
⳵t ⳵x
␳n
⳵b
⳵x
+冉 冊 冉 冊

⳵y
␳n
⳵b
⳵y
, 共19兲 ␣ = 1/␯ ; ␤ = 2/␯; 共29兲

A共V兲 = ⌬s0共␯V兲1/␯ ; ⌬s1共V兲 = 21 ⌬s0


2
共␯V兲2/␯ . 共30兲
⳵␪
= ␬ⵜ2␪ + ␳n j2 − ⌫共␪ − ␪0兲, 共20兲 The electric current j = ⳵bs / ⳵X formally diverges as
⳵t 兩X兩1/␯−1 at the front for ␯ ⬎ 1. Of course the divergence is
where the dimensionless normal state resistance is defined by intercepted by the phase transition into the normal state cre-
ating the “hot” region of presumably small width wn deter-
c 2t * mined by the condition that the depairing current is reached
␳ n共 ␪ 兲 = R n共 ␪ 兲 . 共21兲
4␲x*2 j共X = − wn兲 = jd = ⌬s0V共␯Vwn兲1/␯−1 . 共31兲
In the following section we solve these equations both ana- There is also dissipation in the superconducting part of a
lytically and numerically. larger width ws. The expression for the Joule heat term

184508-4
DYNAMICS AND THERMAL INSTABILITY OF… PHYSICAL REVIEW B 71, 184508 共2005兲

caused by the magnetic flux motion everywhere, not neces-


sarily close to the front interface, diverges at the front as 关see
Eq. 共25兲兴 PJ ⬀ 兩X兩2/␯−1 for ␯ ⬎ 2 only. Its integral, however,
always converges.
To determine V , wn, and other characteristics of the front
motion we need the solution in the normal domain. This and
its matching with the asymptotics in the superconductor is
considered next.

B. Solution in normal domain for the temperature


independent resistivity
In the normal domain we assume first we assume for sim- FIG. 4. The magnetic induction profile at the front. Three dif-
plicity that ␳n共T兲 = const in addition to the previously used ferent regions, the mixed, the normal domain and the Meissner state
simplification ␬ = ⌫ = 0. The nonlinear wave Ansatz are presented. Here wn is the width of the normal domain in which
superconductivity is suppressed by the high current, indicated by
b = bn共X兲, ⌬ = ⌬n共X兲 共32兲 the hatched area at the leading edge of the front.
will be initially used to find the current density jn
= 共dbn / dX兲. Substitution of Eq. 共32兲 into the normal state j2d ⌬s0
2

Eqs. 共19兲 and 共20兲 leads to the following set in terms of the ⌬⬘共− wn兲 = = 共␯Vwn兲2/␯ . 共39兲
V ␯wn
front variable X = x − Vt:
The only solution of the set of three algebraic Eqs. 共31兲,
djn 共38兲, and 共39兲 is very simple
− Vjn = ␳n , 共33兲

冉 冊
dX
⌬0
关1 + 冑1 + 4⌬0/␯兴 ⬇
jd jd
V= 1+ , 共40兲
d⌬n 2⌬0 ⌬0 ␯
V = ␳n j2n . 共34兲
dX
⌬0
The first equation has a solution wn ⬇ , 共41兲
␯ jd

jn共X兲 = jn0exp − 冋 册 冉 冊 XV
␳n
⬇ jn0 1 −
XV
␳n
. 共35兲
⌬s0 ⬇ ⌬0 −
⌬20
. 共42兲

The approximate form is generally valid since 共兩X 兩 V / ␳n兲
⬍ 共wnV / ␳n兲 Ⰶ 1 as will be justified a posteriori. Then the The front velocity is determined by the Joule heat released in
heat transfer equation and the boundary condition ⌬n共X = 0兲 the normal domain Eq. 共37兲
= ⌬0 gives

再 冋 册 冎
␳ n j d⌬ 0
⌶n = ␳n j2nwn = 共43兲
␳n jn0
2
2XV 2
jn0 ␯
⌬n共X兲 = ⌬0 − exp − − 1 ⬇ ⌬ 0 + X.
2V2 ␳n V as
共36兲
␯⌶n
In this region most of the heat is released V= . 共44兲
␳n⌬20

⌶n ⬅ 冕 0

−wn
␳ n共 ␪ 兲 冉 冊
⳵ bn
⳵X
2
dX ⬇ ␳n j2nwn . 共37兲 We will use this simple relation in numerical simulation de-
scribed in the next subsection.
As we discuss later, the numerical results demonstrate that
We will use this result later. the width of the normal domain wn 共hatched area in Fig. 4兲 is
much smaller than the width of the superconducting domain
C. Matching solutions on the superconductor-normal interface ws in which the current is significant. When ␬ and ⌫ are
and the flux front velocity nonzero only numerical analysis is possible. The results 共see
The current, temperature, and the temperature gradient are later兲 show that for reasonable values of ␬ and ⌫ the corre-
all continuous on the superconductor-normal interface lo- sponding terms in the heat transfer equation are qualitatively
cated at X = −wn. Consequently the current on the normal side insignificant. Of course in this case we cannot assume the
approaches the same depairing current as that on the super- simple form of Eq. 共22兲.
conducting side, see Eq. 共31兲. The temperature matching
conditions are
D. The macroscopic description of the normal domain
j 2w n Since the normal domain is very narrow, it is more con-
⌬共− wn兲 = ⌬0 − d = ⌬s0 , 共38兲
V venient to avoid explicit matching in simulations treating

184508-5
B. YA. SHAPIRO, I. SHAPIRO, B. ROSENSTEIN, AND F. BASS PHYSICAL REVIEW B 71, 184508 共2005兲

instead the heat release phenomenologically. In this approach


the width of the normal domain is considered to be smaller
than any other relevant scale and the normal part of the Joule
heat term in the heat diffusion Eq. 共16兲 is replaced by a delta
function. This is equivalent to boundary condition on the
front in which the normal domain contribution ⌶n calculated
in Eq. 共43兲 is added. The fine structure of the front is ignored
in such an approach but it still provides a simple relation
between the temperature difference between the Meissner
domain and the mixed state domain 关␪兴,
⌶n
V⯝ . 共45兲
关␪兴
This is obtained by integration of the heat transfer Eq. 共16兲 in
the vicinity of the front.
The temperature jump at the front 关␪兴 however cannot be
calculated in the framework of such a simple phenomeno-
logical theory and has to be obtained from the microscopic
theory 关see Eq. 共44兲兴. This allows us to relate the temperature
jump across the front to the microscopic parameters of the
problem
␳n⌬20
关␪兴 = , 共46兲

where resistivity of the normal domain ␳n is a parameter the
microscopic model. This relation significantly simplifies the
numerical simulation in which appearance of a singular
shock wave naturally increases complexity. The simulation
will go beyond the limit ␬ = ⌫ = 0 treated analytically earlier.

E. Numerical solution for magnetic flux conserving boundary


conditions
The set of the scaled one dimensional Eqs. 共15兲 and 共16兲
for resistivity in the form of Eq. 共17兲 in the superconducting
domain was solved numerically using the Euler method. The
normal domain was not directly simulated and matched. In-
stead we used the phenomenological relations described in
the previous subsection to set the boundary condition on the
front. Parameters describing the, numerical “experiment”
were chosen to be: ␮ = 0, ␯ = 5, ⌫ = 0, and ␬ in the range
0.01–0.1. Size of the system is Lx / x* = 200. The boundary
conditions are: the total flux ⌽ / 共B*x*2兲 in the range 0.5–2.5, FIG. 5. The evolution of the magnetic induction for the flux
temperature of the cold superconductor ␪0 = 0.7: conserving boundary condition. The value of the Joule heat released
in the normal domain ⌶n was kept fixed at ⌶n = 0.5. The curves
␪共x = − 200兲 = ␪共x = 200兲 = ␪0 . 共47兲 correspond 共from left to right兲 to six different times with intervals
The normal phase was not simulated since it can be inte- of ⌬t between them. 共a兲 The flux ⌽ = 0.5 and the heat diffusion
constant ␬ = 0.1, ⌬t = 2.5 t*. 共b兲 ⌽ = 0.5, ␬ = 0.01, ⌬t = 2.5 t*. 共c兲
grated analytically. The transition to the normal state at de-
⌽ = 2.4, ␬ = 0.05, ⌬t = 5 t*.
pairing current was taken into account by holding constant
the normal domain Joule heat dissipation ⌶n for values in the is constant and is plotted as a function of ⌶n in Fig. 6 for
range 5 · 10−2–2. ⌽ = 2.4 and ␬ = 0.05. The temperature front moves together
The results of the numerical solution are presented in with the flux front velocity. The data are presented for the
Figs. 5–7. The evolution of the magnetic induction is pre- same times as for the magnetic induction. It demonstrates
sented in Fig. 5 for the following values of the flux and heat that the front interface velocity V is linearly dependent on
diffusion constant: 共a兲 ⌽ = 0.5, ␬ = 0.1, 共b兲 ⌽ = 0.5, ␬ = 0.01, ⌶n. The dependence of ⌽ is negligible. The results closely
and 共c兲 ⌽ = 2.4, ␬ = 0.05. The value of ⌶n was kept fixed at follow Eq. 共44兲 obtained analytically for ␬ = 0 and confirms
⌶n = 0.5. Different curves represent successive times with in- the general physical picture proposed in the previous section
tervals of ⌬t = 2.5t* between them. Velocity of the sharp front that the velocity of the shock wave is universal in a sense

184508-6
DYNAMICS AND THERMAL INSTABILITY OF… PHYSICAL REVIEW B 71, 184508 共2005兲

that it depends only the heat released in the normal domain.


The simulation reveals that the evolution is qualitatively the
same for other values of the parameters.
The dynamics of the temperature distribution ␪共x , t兲 is
presented in Fig. 7 and has a form of a thermal shock wave.
Two sets of parameters were simulated: 共a兲 ⌽ = 0.5, ␬ = 0.1,
and 共b兲 ⌽ = 0.5, ␬ = 0.01. The maximum of temperature ␪ in
this wave is reached at the interface between the supercon-
ducting and normal domains in the vicinity of the magnetic
flux front. As we discussed in the previous section, the cur-
rent is maximal in the normal domain which is narrow. We
found in all the cases studied that the Joule heat released in
the mixed state domain 共see Fig. 4兲 does not exceed 1% of
that in the normal domain. Note a curious feature of Fig. 7
that all the curves intersect at a certain point.

IV. GENERALIZATIONS: THE ␮ Å 0 RESISTIVITY AND


FIG. 6. Front velocity as a function of the Joule heat released in THE CONSTANT MAGNETIC FIELD BOUNDARY
the normal domain ⌶n. Here the flux is ⌽ = 2.4, the heat diffusion CONDITION
constant is ␬ = 0.05. Squares correspond to the simulated values of A. More general I–V ␮ Å 0
⌶n, while the straight line is the analytical result.
Although in real samples resistance in the resistive mixed
state might be a more complicated function than it was as-
sumed earlier, the model representation in the form of Eqs.
共7兲 and 共8兲 with arbitrary critical exponents ␯ and ␮ is a
robust and experimentally justified way to treat the problem.
In such a case the main conclusions obtained for resistance
with ␮ = 0, remain valid for some special relations between
the critical exponents only.
Assuming bs and ⌬s in the vicinity of the front 共X → 0兲 in
the form of the Eqs. 共25兲 and 共26兲 one obtains asymptotically
for A共V兲 and ␣:

␣=
␮+1
␯+␮
; A共V兲 = ⌬s0V1/共␯+␮兲 冉 冊␮+1
␮+␯
−共␮+1兲/共␮+␯兲
.

共48兲

The electric current now behaves as

j ⬀ 兩X兩共1−␯兲/共␮+␯兲 共49兲

and still diverges for ␯ ⬎ 1. This condition is independent of


␮, although the power in Eq. 共49兲 depends on ␮. In the case
␯ ⬍ 1 there is no normal domain and one can neglect the
Joule heat. Hence, the temperature gradients are small and it
suffices to consider the flux dynamics described by Eq. 共15兲
with temperature fixed at ␪0. Looking for an exact solution in
a form

b = b1t−␣ f共␨兲, 共50兲

where ␨ = b2x / t␤, we obtain for b1 and f共␨兲 共see Refs. 7 and
19兲, under the flux conservation law boundary condition ⌽
FIG. 7. The evolution of the temperature profile for the flux = 兰dxb共x , t兲:
conserving boundary condition. The value of the Joule heat released
in the normal domain. ⌶n was kept fixed at ⌶n = 0.5. The curves ␣ = ␤ = 1/共2␮ + 2 + ␯兲; b1 = ⌽共␮+2兲/共2␮+2+␯兲;
correspond to six different times with intervals of ⌬t = 2.5 t* be-
tween them. 共a兲 The flux ⌽ = 0.5 and heat diffusion constant is ␬
= 0.1. 共b兲 ⌽ = 0.5, ␬ = 0.01. b2 = ⌽−共␯+␮兲/共2␮+2+␯兲 ,

184508-7
B. YA. SHAPIRO, I. SHAPIRO, B. ROSENSTEIN, AND F. BASS PHYSICAL REVIEW B 71, 184508 共2005兲

f共␨兲 = 再冉 冊冉
␮+␯
␮+2
冊 1
2␮ + 2 + ␯
1/共␮+1兲
␨共f␮+2兲/共␮+1兲

冋 冉 冊 册冎
⫻ 1−

␨f
共␮+2 共Ⲑ␮+1兲 共1+␮ 共Ⲑ␮+␯兲
, 共51兲

␨−共2
f
␮+␯+2 Ⲑ共␮+␯兲
= 冉 冊
␮ + 1 ␮ + ␯ 共共␮+1 Ⲑ共␮+␯兲
␮+2 ␮+2
1
关2 + 2␮ + ␯兴1/共␯+␮兲

⫻B 冋 2 + 2␮ + ␯ ␮ + 1
␮+␯ ␮+2
, , 册 共52兲

where B is the beta function. The flux front moves with


velocity V f 共t兲 = dx f / dt⬀ t␤−1 decaying with time. In the ab-
sence of the excessive heat released at the flux front the flux
front in this case is completely stable.

B. Constant magnetic field


In certain cases similar phenomena will occur when flux
is not conserved. Examples include narrow stripes, fields
larger than Hc1, etc. This does not mean that the effect dis-
appears since magnetic flux generally forms a thermomag-
netic shock wave. The main prerequisite is a phase transition
from superconductor to normal metal resulting in a sharp
flux front. This case was studied numerically for constant
magnetic field 共in units of B*兲 b = 0.05 and parameters ␯ = 5,
␬ = 0.05, ⌫ = 0, and ⌶ = 0.5. The profile of the magnetic field
and the temperature shock waves are presented in Figs. FIG. 8. Magnetic field at x = 0 is constant. The curves corre-
8共a兲,8共b兲, where different curves correspond 共from left to spond to six different times from left to right with intervals of ⌬t
right兲 to various times: t = 0, 5, 10, 15… 共in the t* units兲. It is = 5 t* between them. Joule heat released at the front ⌶ = 0.5. 共a兲 The
important to note that, when the simulation was done for magnetic induction evolution and 共b兲 the temperature shock wave.
different ⌶, the dependence was linear like for the constant
flux in Fig. 6. This is consistent with our analytic result pre- ⳵␩ ⳵ ␪n ⳵ ␩ ⳵ 2b n ⳵ bn ⳵␨
dicting that the front velocity is governed solely by the Joule = ␳n共␪n兲ⵜ2␩ + ␳1 + ␳1 2 ␨ + ␳1 ,
heat released in the normal domain. Other features are also ⳵t ⳵x ⳵x ⳵x ⳵x ⳵x
independent of boundary conditions. 共54兲

V. INSTABILITY OF THE STRAIGHT FRONT


A. Linear stability analysis for ␬ = ⌫ = 0
⳵␨
⳵t
= 2 ␳ n共 ␪ n兲
⳵ bn ⳵ ␩
⳵x ⳵x
冉 冊
+ ␳1
⳵ bn
⳵x
2
␨. 共55兲

The dependence of the front velocity on the Joule heat


released near the interface can lead to an instability of the Due to translation invariance of these eigenvalue equations
straight front. Perturbations like a slight spatial distribution in time and the direction along the front y one represents ␩ , ␨
of the sample parameters 共resistance, for example兲 can trig- in a form
ger the front instability. Keeping the normal resistivity in the
form ␳n = ␳0 + ␳1␪共x , t兲 we look for a solution of the corru-
gated front in the normal domain as ␩ = ␩共x兲exp共⍀t + ky y兲; ␨ = ␨共X兲exp共⍀t + ky y兲. 共56兲

b = bn共x − Vt兲 + ␩共x,y,t兲,


Then the eigenvalue equations become one dimensional
␪ = ␪n共x − Vt兲 + ␨共x,y,t兲. 共53兲
The leading order solution ␤n and ␪n for the set of basic Eqs.
共15兲 and 共16兲 for ␳1 = 0 were obtained in Sec. III, while cor-
rections to the first order in ␳1 will not be required in the
L̂ 冋册 冋册


=⍀


, 共57兲

stability analysis. The first order terms in perturbations ␩ and


␨ are where

184508-8
DYNAMICS AND THERMAL INSTABILITY OF… PHYSICAL REVIEW B 71, 184508 共2005兲

First of all the instability can develop when the characteristic


time t0 ⯝ 1 / 共␳1 j2d兲 is smaller than the characteristic time of
the heat absorption in the sample tr ⬇ ⌫−1. In addition the
heat diffusion along the y axis can also affect the unstable
fluctuations. In the latter case the requirement is: ut0 ⬎ 冑␬t0.
These two requirements allow us to determine the critical
共58兲 velocity of the fluctuation for the onset of the instability
Let us first consider the simpler case of conventional super- u ⬎ uc = min兵⌫wn, jd冑␬␳1其. 共63兲
conductors for which ␳1 = 0. Substituting Eqs. 共35兲,共36兲 into
Eqs. 共54兲 and 共55兲 one obtains 关replacing 共⳵ / ⳵X兲 → ikX兴: In metals and alloys the normal state resistivity practically
does not depend on temperature in the relevant temperature
range. This means that ␳1 = 0 and consequently no instability
is expected.
共59兲 The threshold in the fluctuation velocity uc 共which is pro-
portional to the Joule heat released in the front兲 means that
only a large temperature fluctuation can provide Joule heat-
The matrix L̂0 has one stable ⍀1 = −␳0共kX2 + k2y 兲 and one mar- ing necessary to destroy the planar front. Physically large
ginal ⍀2 = 0 eigenvalues. This eigenvalue is highly degener- amplitude fluctuations of the temperature at the front are
ate: any temperature deviation ␨ for ␩ = 0 belongs to this nonuniform because they are caused by the spatial distribu-
subspace: L̂0关 0␨ 兴 = 0. Strictly speaking the marginal eigen- tion of the impurities in the sample locally increasing resis-
value ⍀2 calls for investigation beyond the linear stability tivity and hence the Joule heat and velocity of the fluctua-
analysis. However, we believe it is stable and, in any case, tions in the front. Numerical simulations support this
addition of the ␳1 term to resistivity removes the marginality scenario.
and the degeneracy. To find the corrected eigenvalue ⍀2, one In order to study the development of the instability for
has to diagonalize on the corresponding subspace the opera- arbitrary ␬, the set of the Eqs. 共15兲,共16兲 have been solved
tor numerically. The Joule heat power ⌶n released in the normal

L̂␨␨ = ␳1 冉 冊
⳵ bn
⳵X
2
. 共60兲
domain at the front has the following model form:
⌶ n共 ␪ 兲 ␳ n共 ␪ 兲
⬅ = 1 + ␣关␪共x,y,t兲 − ␪0兴, 共64兲
The derivative is nearly constant in the normal domain, see ⌶n0 ␳0
Eq. 共35兲: where initial temperature is perturbed in the region 0 ⬍ x

L̂␨␨ = ␳1 jn0
2
冋 册
exp −
2XV
␳n
⬇ ␳1 j2d . 共61兲
⬍ 5 , 4 ⬍ y ⬍ 5, 共temperature fluctuation ␪共x , y , t = 0兲 = 0.88兲,
while outside this region ␪共x , y , t = 0兲 = ␪0 = 0.7. We chose ␣
= 14.5, ␬ = 0.05 and 2.5. Physically this kind of fluctuation
Consequently represents a local variation of the normal state resistivity
共proportional to ⌶n兲 when the front of the shock wave passes
⍀2 = ␳1 j2d , 共62兲 an inhomogeneity.
The evolution of a small fluctuation in two opposite limits
which demonstrates the instability for any wave vector.
is presented in Fig. 9. For small ␬, Fig. 9共a兲, an unstable
The physical reason for the instability is the positive feed-
pattern of the magnetic induction develops. It should be
back between temperature fluctuation at the front increasing
noted that the flux front line lost its stability essentially im-
in its turn both the Joule power at the front and its velocity.
mediately after the temperature fluctuation affected the sys-
In fact, it is the well known hydrodynamics tangential
tem. For finite ␬ we observe that most of the ␬ = 0 unstable
instability20 of the flux front which is responsible for the
modes are diffused away and do not develop into an insta-
front instability. Indeed, in this case warmer segments of the
bility of the system. For large ␬, Fig. 9共b兲, a similar pertur-
front move faster and can destroy the flat front line.
bation relaxes into a straight line front and disappears in
accord with the stability analysis.
B. Stability in the general case: Numerical simulation
If the normal resistivity of the sample is temperature de- VI. DISCUSSION
pendent and ␬ = ⌫ = 0, then the normal domain in the front
shows instability with respect to small temperature fluctua- To summarize, we considered the formation and stability
tions with arbitrary wave vector. In this case the normal do- of the shock waves in the vortex matter under extreme con-
main in the front shows instability with respect to small tem- ditions of the fast flux expansion into the Meissner state. In
perature fluctuations with arbitrary wave vectors. The this case very strong screening currents significantly exceed-
dispersion appears for the nonzero heat diffusion coefficient. ing the critical current Jc flow in the mixed state. For such
In fact, however, these small fluctuations cannot destroy the strong currents the vortex matter resistivity R has a form R
straight line front. It becomes unstable due to large amplitude ⬀ B␯J␮. We predict that when ␯ ⬎ 1 both the moving flux and
fluctuations. Let us consider the evolution of the instability. the temperature profile form a sharp singular shock waves.

184508-9
B. YA. SHAPIRO, I. SHAPIRO, B. ROSENSTEIN, AND F. BASS PHYSICAL REVIEW B 71, 184508 共2005兲

ity of the sample. The flux front velocity has the form for
␮ = 0 共in dimensional units兲 is V = 关cRnJd0 / 共1 − T0 / Tc兲B*兴
⫻关B* / Bc2共0兲兴␯ . Taking for example material parameters of
the optimally doped YBCO, Jd0 = 108 A / cm2, Rn
= 2 · 10−6 ⍀ cm, C = 1 J / cm3 K,21 one obtains for the flux
front velocity V ⬇ 105 cm/ s, which is in a good agreement
with experimental data.12 Note, however, that the value
strongly depends on the exponents ␮ and ␯. The width of the
normal stripe is 0.5 ␮m.
The type of the voltage–current characteristic therefore is
the decisive factor determining the flux front stability in
type-II superconductors. The instability is developed when
the voltage–current characteristics of the uniform supercon-
ductor in its resistive state provides sufficient screening cur-
rents at the moving flux front interface. The physical reason
for the instability is very similar to a well known hydrody-
namic instability,20 when different layers of the liquid move
with different and parallel velocities. In fact it is the positive
feedback between excessive local temperature at the front
and Joule heat released there that leads to instability. The
hydrodynamic tangential instability of the flux front destroys
the flat front. The instability develops for the fluctuation ve-
FIG. 9. Evolution of the magnetic flux front pattern for different locities exceeding the critical value U ⬎ Uc = min兵关cB*共1
values of the heat diffusion constant. The perturbation is triggered − T0 / Tc兲 / 4␲␯Jd0tr兴 , 共Jd0 / C兲冑D兩共dRn / dT兲兩Tc其, where D is the
by the temperature inhomogeneity specified in Eq. 共64兲. 共a兲 Small heat diffusion constant and tr is the heat absorption time.
heat diffusion constant ␬ = 0.05. Development of the avalanche in- Taking D = 30 J / 共cm s K兲 and tr = 10−11 s, one estimates the
stability. Five snapshots 共intervals of ⌬t = 0.05 t*兲 of a finger shaped
two velocities as 5 · 106 cm/ s and 2.6· 105 cm/ s.
instability in magnetic induction are shown from left to right. 共b兲
Large heat diffusion constant ␬ = 2.5. Evolution of the magnetic flux
The avalanche-type instability appears when the moving
pattern. The five snapshots 共intervals of ⌬t = 0.125 t*兲 show that the flux front enters the area in which locally the normal resis-
initial small fluctuation dissipates away. tivity is large. The experimental observation of the fast flux
dynamics in YBCO has been carried out by Leiderer et al.12
Strong screening currents in the vortex matter approaching The velocity of the front indeed has the universal character
the depairing current Jd cause destruction of superconductiv- on the advanced stage of the instability and does not depend
ity. An area of material adjacent to the interface between the on initial magnetic gradients. The dendrite velocity in the
Meissner state and the mixed state of the size 共returning to later stages of disintegration of the front are expected to be
dimensional units兲 Wn = 关cB*共1 − T0 / Tc兲 / 4␲␯Jd0兴 becomes of order of Uc. This instability is not expected to arise in
normal. Here B* = 冑4␲CTc, C is the heat capacity and T0 is materials like Nb since 兩dRn / dT兩Tc is negligibly small and Uc
temperature of the cool superconductor. The stable vanishes.
superconductor-normal interface is formed due to combined
effect of the nonlinear magnetic flux dynamics and thermal
ACKNOWLEDGMENTS
effects. The condition ␯ ⬎ 1 is independent on ␮ and has the
following physical meaning. It is well known that above the We are grateful to D. Kessler, Y. Yeshurun, Y. Rabin, A,
critical current resistivity is proportional to the number of Shaulov, and H. H. Wen for discussions and V. Vinokur for
vortices 共the flux flow Bardeen-Stephen formula兲, R ⬀ B共 ␯ his criticism. This work was supported by The Israel Science
= 1兲. The condition for formation of the normal domain is Foundation, ESF Program “Cosmology in the Laboratory.”
therefore that the dependence on magnetic induction at cur- We are also grateful to the Binational Israel-USA and
rents close to the depairing currents is stronger than linear. Germany-Israel Foundations for support and to the Inter-
As was shown in Sec. II B for Nb, this happens at least for University Computational Center for providing Cray J932
small fields. supercomputer facilities. B.R. acknowledges Albert Einstein
The interface moves with constant velocity, which is Minerva Center for Theoretical Physics in Weizmann Insti-
completely determined by the Joule heat released in the tute and NSC grant ROC94-2112-M009-024 of R.O.C. and
normal domain at the front and hence on the normal resistiv- the hospitality of Bar Ilan University.

184508-10
DYNAMICS AND THERMAL INSTABILITY OF… PHYSICAL REVIEW B 71, 184508 共2005兲

*Author to whom correspondence should be addressed. 757 共2000兲; U. Bolz, D. Schmidt, B. Biehler, B.-U. Runge, R. G.
1 R. G. Mints and A. I. Rahmanov, Rev. Mod. Phys. 53, 551 Mints, K. Numssen, H. Kinder, and P. Leiderer, Physica C 388-
共1981兲; A. V. Gurevich, R. G. Mints, and A. I. Rahmanov, The 389, 715 共2003兲.
Physics of Composite Superconductors 共Begell House, NY, 11
I. Shapiro, E. Pechenik, and B. Ya. Shapiro, Phys. Rev. B 63,
1997兲. 184520 共2001兲.
2 L. A. Dorosinskii, M. V. Indenbom, V. I. Nikitenko, Yu. A. Os- 12 U. Bolz, B. Biehler, D. Schmidt, B. U. Runge, and P. Leiderer,

sipyan, A. A. Polanskii, and V. K. Vlasko-Vlasov, Physica C Europhys. Lett. 64, 517-523 共2003兲.
203, 149 共1992兲. 13
V. M. Vinokur, M. V. Feigelman, and V. B. Geshkenbein, Phys.
3
V. K. Vlasko-Vlasov, V. I. Nikitenko, A. A. Polyanskii, G. M. Rev. Lett. 67, 915 共1991兲.
Crabtree, U. Welp, and B. W. Veal, Physica C 222, 361 共1994兲. 14
F. Bass, B. Ya. Shapiro, I. Shapiro, and M. Shvartser, Physica C
4 M. E. Gaevski, T. H. Johansen, Yu. Galperin, H. Bratsberg, A. V. 297, 269 共1998兲; 297, 269 共1998兲.
Bobyl, D. V. Shautsev, and S. F. Karmarenko, Appl. Phys. Lett. 15
F. Bass, B. Ya. Shapiro, and M. Shvartser, Phys. Rev. Lett. 80,
71, 3147 共1997兲. 2441 共1998兲; I. Aranson, A. Gurevich, and V. Vinokur, ibid. 87,
5 C. A. Duran, P. L. Gammel, R. E. Miller, and D. J. Bishop, Phys. 067003 共2001兲.
Rev. B 52, 75 共1995兲. 16 C. Villard, C. Peroz, and A. Sulpice, J. Low Temp. Phys. 131,
6
C. P. Poole, H. A. Farrah, and R. J. Creswick, Superconductivity 957 共2003兲.
共Academic Press, San Diego, 1995兲. 17
B. Kalisky, G. Koren, A. Shaulov, Y. Yeshurun, and R. P. Hue-
7 F. Bass, B. Ya. Shapiro, and M. Shvartser, Phys. Rev. Lett. 80, bener 共unpublished兲.
2441 共1998兲. 18 L. Burlachkov, D. Giller, and R. Prozorov, Phys. Rev. B 58,
8
A. Gurevich, Phys. Rev. B 46, 3638 共1992兲. 15067 共1998兲.
9 L. M. Fisher, P. E. Goa, M. Baziljevich, T. H. Johansen, A. L. 19 D. Zwillinger, Handbook of Differential Equations, 3rd ed. 共Aca-

Rakhmanov, and V. A. Yampol’skii, Phys. Rev. Lett. 87, 247005 demic Press, Boston, 1997兲, p. 424.
共2001兲. 20
L. D. Landau and E. M. Lifshitz, Fluid Mechanics, Course of
10
P. Leiderer, J. Boneberg, P. Brull, V. Bujok, and S. Herminghaus, Theoretical Physics Vol. 6 共Pergamon Press, New York, 1980兲.
Phys. Rev. Lett. 71, 2646 共1993兲; U. Bolz, J. Eisenmenger, J. 21 M. Aravind and P. C. W. Fung, Meas. Sci. Technol. 10, 979

Schiessling, B.-U. Runge, and P. Leiderer, Physica B 284-288, 共1999兲.

184508-11

You might also like