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Fisher information universally identifies quantum resources

Kok Chuan Tan,∗ Varun Narasimhachar, and Bartosz Regula


School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Republic of Singapore

We show that both the classical as well as the quantum definitions of the Fisher information faithfully identify
resourceful quantum states in general quantum resource theories, in the sense that they can always distinguish
between states with and without a given resource. This shows that all quantum resources confer an advantage
in metrology, and establishes the Fisher information as a universal tool to probe the resourcefulness of quantum
states. We provide bounds on the extent of this advantage, as well as a simple criterion to test whether different
resources are useful for the estimation of unitarily encoded parameters. Finally, we extend the results to show
that the Fisher information is also able to identify the dynamical resourcefulness of quantum operations.
arXiv:2104.01763v1 [quant-ph] 5 Apr 2021

Introduction — The Fisher information (FI) plays an impor- of general quantum resources, and in which settings different
tant foundational role in quantum information science. In notions of quantumness can provide tangible practical advan-
quantum metrology and sensing, it determines the ultimate tages.
limits of precision of our measurement devices via the well In this work, we show that the FI universally characterizes
known quantum Cramér-Rao bound [1–3]. Existing applica- the resources of quantum states, regardless of the specific re-
tions include interferometry [4–6], magnetometry [7, 8], ther- source in consideration, in that it is able to identify every
mometry [9, 10], quantum illumination [11–13], displacement resourceful state in general quantum resource theories. An
sensing [14, 15], among others. Crucially, such applications immediate implication of this result is that quantum resources
exploit the use of well-studied nonclassical quantum properties are always useful for quantum metrology, since there always
such as coherence [16, 17], entanglement [18, 19], and neg- exists some metrological problem where a resourceful probe
ative quasiprobabilities [20, 21] in order to demonstrate the outperforms a probe which does not possess a given resource.
intrinsic superiority of quantum measurement devices over This also implies that the FI can be used as a generic tool to
classical ones. FI has also been used to study nonclassical fea- probe the resources of any system. We then establish theoret-
tures of quantum systems such as quantum coherence [22, 23] ical bounds on the advantages provided by a given quantum
and entanglement [24, 25]. states by relating the FI to the robustness measure of the given
Traditionally, different notions of nonclassicality in quan- resource. We additionally provide a simple criterion for test-
tum mechanics have been studied independently. As such, ing whether a given resource is useful for unitary parameter
the theoretical tools and quantities that were developed in the estimation. Finally, we also show that the FI can identify the
past typically probe a single nonclassical feature at a time. resources of quantum operations in general resource theories.
However, recent developments have made tremendous strides
in providing a unified framework to study not only several Preliminaries — We first define what a general quantum re-
disparate notions of nonclassicality [26–28], but also more source theory means in our context. Let S be the state space
general resources of quantum systems [29, 30]. This has led that describes a quantum system. A quantum resource theory
to the discovery of physical tasks and operational quantities is composed of a well-defined set of free quantum states F
that are relevant in not just one particular resource theory, — depending on the setting, these can be understood as the
but also in general settings. This motivates us to consider classical states, or the states without the given resource. Such
quantities that are universally applicable in the sense that they states are accompanied by some set of free quantum operations
maintain a physically meaningful interpretation while being O. In order to account for as many possible formulations of
able to identify every state which is considered “nonclassi- quantum resources as possible, only a minimal set of assump-
cal” or “resourceful” within the physical constraints of the tions are imposed on the sets F and O. The set of free states
given resource theory [31–39]. An example of such quantities F is assumed to be some closed and convex, but otherwise ar-
would be the class of robustness measures [40], which are well- bitrary subset of the state space S. The physical interpretation
defined quantifiers of any quantum resource that find use in of the assumption of convexity is that if one statistically mixes
quantifying the operational advantages of resources in channel two free states together, the output will remain free. Given a
discrimination tasks [34, 36, 41]. Not all meaningful quanti- well-defined set F , we assume that O is some set of quantum
ties can identify all resource states of interest — for instance, maps that satisfies Φ(𝜎) ∈ F if 𝜎 ∈ F and Φ ∈ O. These
in the theory of quantum entanglement, there exist important very minimal assumptions made on F and O maximizes the
tasks such as distillation or quantum teleportation for which generality of the subsequent results.
certain classes of entangled states are useless [18, 42], and so
We now define the FI. In a typical scenario, there are two
quantities based on such tasks fail to faithfully characterize
types of FI considered in quantum information. The first type
entanglement as a resource. This raises the questions of which
is the FI one obtains from the classical post-processing of
tasks and quantities can be considered as universal witnesses
statistical data. This data is typically obtained from the mea-
surement output of a fixed measurement setup. We will refer
to this as the classical FI (CFI), and denote it as 𝐹𝐶 .
∗ bbtankc@gmail.com The second type of FI is the maximum CFI one can obtain
2

over all possible quantum measurements. This is typically using any resourceless state 𝜎 ∈ F . Since the excess FI can
called the quantum FI (QFI), and will here be denoted 𝐹𝑄 . By only be attributed to the given resource, the state 𝜌 must be
definition, we see that the CFI is a simple lower bound to the resourceful.
QFI. Upon first inspection, one may expect, since the QFI con-
Suppose we have a quantum channel Φ 𝜃 that depends on tains more information about the metrological utility of the
some real parameter 𝜃, and we would like to estimate 𝜃. In quantum state than the CFI, that 𝑁 𝑄 performs better than
order to do this, we pass a state 𝜌, called a probe, through the 𝑁𝐶 at identifying nonclassicality. This is in fact incorrect.
quantum channel Φ 𝜃 and then perform a quantum measure- To see this, recall that the QFI is the CFI optimized over
ment (positive operator–valued measure)Í 𝑀 = {𝑀𝑖 }, where all possible quantum measurements. Suppose 𝑀 ★ is the op-
𝑀𝑖 are positive operators such that 𝑖 𝑀𝑖 = 11. This results timal measurement. This implies that for any channel Φ 𝜃 ,
in the measurement statistics 𝑃(𝑖 | 𝜃) = Tr[Φ 𝜃 (𝜌) 𝑀𝑖 ]. The it is always possible to find a measurement 𝑀 ★ such that
maximum information about 𝜃 that we can obtain from the 𝑁𝐶 (𝜌 | 𝑀 ★) ≥ 𝑁 𝑄 (𝜌). In general, we therefore see that the
statistics 𝑃(𝑖 | 𝜃) is quantified by the CFI, which is given gap between resourceful and free states is larger using the CFI
by [43, 44]: compared to the QFI, i.e., the CFI is able to identify more states
 2 as resourceful. Indeed, there exist scenarios where 𝑁 𝑄 wit-
Õ 𝜕 log 𝑃(𝑖 | 𝜃) nesses strictly fewer states than 𝑁𝐶 . This is further discussed
𝐹𝐶 (𝜌 | Φ 𝜃 , 𝑀) ≔ 𝑃(𝑖 | 𝜃) . (1)
𝑖
𝜕𝜃 in the Supplemental Material [47].
In the following Theorem, we show that both the classical
In most cases, the quantum channel is fixed, so we can and the quantum versions of the FI can be used to identify
suppress the dependence on Φ 𝜃 and use the simplified notation general quantum resources.
𝐹𝐶 (𝜌 | 𝑀) instead. A similar notation will also be employed
for the QFI 𝐹𝑄 . Theorem 1. There exists a parameter estimation problem with
In general, the FI is to be evaluated with respect to some quantum channel Φ 𝜃 and measurement 𝑀 such that 𝑁𝐶 (𝜌 |
given value of 𝜃. Since the QFI 𝐹𝑄 (𝜌) is just the CFI maxi- 𝑀) > 0 and 𝑁 𝑄 (𝜌) > 0 if and only if 𝜌 ∉ F .
mized over all possible measurements 𝑀, the former depends
only on the state 𝜌 and the quantum channel Φ 𝜃 , and we have Proof. We will first prove the statement for 𝑁𝐶 .
𝐹𝐶 (𝜌 | 𝑀) ≤ 𝐹𝑄 (𝜌). Formally, the QFI is given by the It is immediately clear that if 𝑁𝐶 (𝜌 | 𝑀) > 0 or 𝑁 𝑄 (𝜌) > 0
expression for any parameter estimation problem,then 𝜌 must be resource-
ful, which proves the “only if" direction.
𝐹𝑄 (𝜌) ≔ Tr(𝜌 𝜃 𝐷 2𝜃 ), (2) To prove the converse direction, we use a result from
where 𝐷 𝜃 is the symmetric logarithmic derivative [45, 46], Ref. [34], which states that if 𝜌 is resourceful, then there ex-
𝜕
satisfying the equation 𝜕𝜃 𝜌 𝜃 = {𝜌 𝜃 , 𝐷 𝜃 }/2. ists a pair of quantum channels {𝐴0 , 𝐴1 } and POVM {𝜋 0 , 𝜋 1 }
such that 𝑝 succ (𝜌) > max 𝜎 ∈F 𝑝 succ (𝜎), where 𝑝 succ (𝜌) ≔
1 1
Nonclassicality from the FI — We will now establish our main 2 Tr[ 𝐴0 (𝜌)𝜋 0 ] + 2 Tr[ 𝐴1 (𝜌)𝜋 1 ].
result, which is that the FI can reveal general quantum re- Let {𝐴0 , 𝐴1 } and POVMs {𝜋 0 , 𝜋 1 } be any such channel
sources. In order to do this, we need to demonstrate that for satisfying the above condition. We also introduce some state
any resourceful state 𝜌 ∉ F , there always exists a metrological 𝜎0 ≠ 𝜌 which will be specified later.
problem represented by some quantum channel Φ 𝜃 together We now consider the following series of quantum channels
with some measurement 𝑀, where the resulting FI correctly acting on some arbitary state 𝜏:
identifies 𝜌 to possess some resources.
Suppose we would like to witness the resources of a state 1
Λ1 (𝜏) = 𝜏 ⊗ 11 ⊗ [𝜃 |0ih0| + (1 − 𝜃) |1ih1|] (5)
via the CFI. One way to go about doing this is to consider the 2
quantity:
𝑁𝐶 (𝜌 | 𝑀) ≔ 𝐹𝐶 (𝜌 | 𝑀) − max 𝐹𝐶 (𝜎 | 𝑀), (3) 1
𝜎 ∈F Λ2 ◦ Λ1 (𝜏) = 𝜏 ⊗ 11 ⊗ 𝜃 |0ih0|
2 (6)
where 𝐹𝐶 (𝜌 | 𝑀) is the CFI obtained by performing the mea- 1
surement 𝑀 on the state Φ 𝜃 (𝜌), and the maximization is over + 𝜎0 ⊗ 11 ⊗ (1 − 𝜃) |1ih1|
2
F , the set of free states in any given resource theory. 𝑁𝐶 then
quantifies the minimum quantum advantage of a nonclassical
state 𝜌 over all possible classical states for a given metrological 1
problem. Λ3 ◦ Λ2 ◦ Λ1 (𝜏) = 𝐴0 (𝜏) ⊗ |0ih0| ⊗ 𝜃 |0ih0|
2
We can also consider a similar definition using the QFI: 1
+ 𝐴1 (𝜏) ⊗ |1ih1| ⊗ 𝜃 |0ih0|
2 (7)
𝑁 𝑄 (𝜌) ≔ 𝐹𝑄 (𝜌) − max 𝐹𝑄 (𝜎). (4) 1
𝜎 ∈F + 𝐴0 (𝜎0 ) ⊗ |0ih0| ⊗ (1 − 𝜃) |1ih1|
2
We see that if 𝑁 𝑄 (𝜌) > 0 or 𝑁𝐶 (𝜌 | 𝑀) > 0, then the FI 1
+ 𝐴1 (𝜎0 ) ⊗ |1ih1| ⊗ (1 − 𝜃) |1ih1|
that is obtained using 𝜌 exceeds that which can be obtained 2
3

from a given state 𝜌 over all resourceless states? To this end,


an even stronger statement can be proven which quantitatively
Λ4 ◦ Λ3 ◦ Λ2 ◦ Λ1 (𝜏) =
relates the quantum advantage 𝑁𝐶 and an important resource
{Tr[Λ3 ◦ Λ2 ◦ Λ1 (𝜏)𝜋 0 ⊗ |0ih0| ⊗ 11] quantifier — the (generalized) robustness measure [40], which
+ Tr[Λ3 ◦ Λ2 ◦ Λ1 (𝜏)𝜋 1 ⊗ |1ih1| ⊗ 11]} |0ih0| (8) we denote 𝑅(𝜌).
{Tr[Λ3 ◦ Λ2 ◦ Λ1 (𝜏)𝜋 0 ⊗ |1ih1| ⊗ 11] So far, we have considered 𝑁𝐶 given some fixed parame-
ter estimation problem with encoding Φ 𝜃 and measurement
+ Tr[Λ3 ◦ Λ2 ◦ Λ1 (𝜏)𝜋 1 ⊗ |0ih0| ⊗ 11]} |1ih1|
𝑀. As a measure of the extent of the quantum advantage, it
Finally, we perform the projection 𝑃0 ≔ |0ih0| and 𝑃1 ≔ is reasonable to consider the maximum nonclassical advan-
|1ih1| to obtain the statistics tage one may obtain over all such encodings and measure-
ments. Since the Fisher information can be scaled via a simple
𝑃(0 | 𝜃) = 𝜃 𝑝 succ (𝜏) + (1 − 𝜃) 𝑝 succ (𝜎0 ) (9) reparametrization 𝜃 → 𝑘𝜃, we are also motivated to normal-
ize the type of encoding channels over the set of free states.
and 𝑃(1 | 𝜃) = 1 − 𝑃(0 | 𝜃). In light of these considerations, we can define the following
Since 𝑃(𝑖 | 𝜃), 𝑖 ∈ {0, 1} is obtained from a series of quantity:
quantum maps followed by a projection on 𝜏, we see that this
fits into the basic form 𝑃(𝑖 | 𝜃) = Tr[Φ 𝜃 (𝜏) 𝑀𝑖 ]. Suppose we 𝑁𝐶max (𝜌) ≔ max 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀), (12)
would like to estimate the parameter 𝜃. We can then use Eq. 1 Φ 𝜃 ∈P, 𝑀
to evaluate the classical information of the statistics.
One may verify that where P is the set of all parameter estimation problems sat-
2 isfying max 𝜎 ∈F 𝐹𝐶 (𝜎 | Φ 𝜃 , 𝑀) ≤ 1. It can be shown that
𝑁𝐶max is a resource monotone, which we elaborate further upon

𝜕𝑃 (0| 𝜃)
𝜕𝜃
𝐹𝐶 (𝜏 | 𝑀) = . (10) in the Supplemental Material [47].
𝑃(0 | 𝜃) (1 − 𝑃(0 | 𝜃))
Theorem 2. In any resource theory, there exists a parameter
Evaluating near the vicinity of 𝜃 = 0, the resulting FI is
estimation task Φ 𝜃 such that
[ 𝑝 succ (𝜏) − 𝑝 succ (𝜎0 )] 2
𝐹𝐶 (𝜏 | 𝑀) = . (11) 𝑅(𝜌) 2 ≤ 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀) ≤ 𝑅(𝜌) 2 + 2𝑅(𝜌), (13)
𝑝 succ (𝜎0 ) (1 − 𝑝 succ (𝜎0 ))
Recall that so far, the state 𝜎0 is not yet specified. We now In particular, 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀) > 0 iff 𝜌 ∉ F , and
choose it such that it satisfies 𝑝 succ (𝜎0 ) = min 𝜎 ∈F 𝑝 succ (𝜎). 𝑁𝐶max (𝜌) ≥ 𝑅(𝜌) 2 is a computable lower bound for any re-
This means that the numerator is a monotonically increasing source.
function of 𝑝 succ (𝜏). We also see that the denominator does not
depend on the state 𝜏. Together with the fact that 𝑝 succ (𝜌) > Theorem 2 provides a computable lower bound on the quan-
𝑝 succ (𝜎) for every 𝜎 ∈ F , we must have 𝐹𝐶 (𝜌 | 𝑀) > tum advantage that can be extracted. We stress that the robust-
max 𝜎 ∈F 𝐹𝐶 (𝜎 | 𝑀) and 𝑁𝐶 (𝜌 | 𝑀) > 0 if 𝜌 is nonclassical. ness 𝑅(𝜌) can always be computed as a convex optimization
This shows the existence of at least one parameter estimation problem. In many cases, such as the resource theories of co-
problem where 𝑁𝐶 (𝜌 | 𝑀) > 0 if 𝜌 is nonclassical. For herence [48], multi-level coherence [49], and magic [50–53],
the special case where 𝑝 succ (𝜎0 ) = 0, then Eq. 10 becomes it becomes an efficiently computable semidefinite program,
𝐹𝐶 (𝜏 | 𝑀) = 𝑝 succ (𝜏)/𝜃 instead and a similar conclusion while in many theories including entanglement [40, 54, 55]
is reached. This is sufficient to prove both directions of the and multi-level entanglement [56] it can be computed analyt-
statement for 𝑁𝐶 . ically for all pure states. Furthermore, in the class of affine
The equivalent statement for 𝑁 𝑄 comes from the observa- resource theories [57, 58], which includes theories such as co-
tion that the quantum map Λ4 ◦ Λ3 ◦ Λ2 ◦ Λ1 maps any input herence and imaginarity [59, 60], the lower bound of Thm. 2
state to a diagonal state, and that the measurement 𝑀 is also is tight, in the sense that there always exists a task such that
diagonal. We then use the fact that for diagonal states, the 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀) = 𝑅(𝜌) 2 .
QFI is saturated by a measurement in the diagonal basis [1].
Taking this quantitative relationship further, it is natural
This is sufficient to show that 𝐹𝐶 (𝜌 | 𝑀) − max 𝜎 ∈F 𝐹𝐶 (𝜎 |
to ask whether there is also an upper bound on the quantum
𝑀) = 𝐹𝑄 (𝜌) − max 𝜎 ∈F 𝐹𝑄 (𝜎) = 𝑁 𝑄 (𝜌 > 0), which proves
advantage that a resource state affords in estimation tasks.
the required statement. 
Indeed, this is possible in the case where the decoding mea-
Theorem 1 establishes that 𝑁𝐶 and 𝑁 𝑄 are both able to surement has a binary outcome:
identify any resourceful state in general quantum resource
theories. Both of the quantities therefore constitute faithful Theorem 3. For any parameter estimation task with en-
resource witnesses of direct physical relevance. This result coding channel family Φ 𝜃 and two-outcome measurement
also demonstrates the existence of a metrological advantage 𝑀 ≡ (𝑃, 11 − 𝑃), let 𝑟 ≔ 𝐹𝐶 (𝜌 | 𝑀) < ∞ and
for any nonclassical state.
However, one can also be interested in understanding this 𝜕Tr𝑃Φ 𝜃 (𝜌)
𝜔 := . (14)
advantage precisely: how much advantage can be extracted 𝜕𝜃
𝜃=0
4

Then, To see that 𝑠∗ in indeed an upper bound, we use the fact that
𝐹𝑄 (𝜎) ≤ 4Δ2𝜎 𝐺 where Δ2𝜎 𝐺 is the variance of 𝐺 given the
[𝑅𝑆 (𝜌) + 1] −2 𝜔2 state 𝜎. We then observe that 𝑋 𝐴𝐵 = 𝜎 ⊗ 𝜎 where 𝜎 ∈ F is a
𝑁𝐶 (𝜌 | 𝑀) ≤ 𝑟 −
max Tr[𝑃 Φ0 (𝜏)] (1 − Tr[𝑃 Φ0 (𝜏)]) feasible solution. Finally, we observe that 2Tr[(𝐺 𝐴 ⊗ 11 𝐵 −11 𝐴 ⊗
𝜏 ∈F
𝐺 𝐵 ) 2 𝜎 ⊗ 𝜎] = 4Δ2𝜎 𝐺 so we must have 𝑠∗ ≥ max 𝜎 ∈F 𝐹𝑄 (𝜎)
4𝜔2 as required. 
≤𝑟− , (15)
[𝑅𝑆 (𝜌) + 1] 2
The convex optimization in Theorem 4 provides a direct
where 𝑅𝑆 (𝜌) is the standard robustness of 𝜌 with respect to method of testing of whether the particular parameter estima-
F [40]. tion problem generated by 𝐺 will benefit from a given quantum
resource. Note that this is a sufficient condition, so failure of
𝑅𝑆 is another operationally significant resource measure the test does not necessarily imply the resource is not useful
closely related to 𝑅, and like the latter, admits efficient SDP for this encoding. We also highlight that the criterion is based
formulations in many resource theories. Thus, given any par- on the QFI-based quantity, 𝑁 𝑄 , but it also applies to the CFI
ticular parameter estimation task with a two-outcome measure- case as well, since if 𝑁 𝑄 (𝜌) > 0, then we are guaranteed
ment, we have an efficiently computable upper bound to the some measurement 𝑀 for which 𝑁𝐶 (𝜌 | 𝑀) > 𝑁 𝑄 (𝜌) > 0.
quantum advantage 𝑁𝐶 of any given resource state. The bound A similar sufficient condition can be obtained for non-unitary
in the first line is less computationally feasible but tighter. encoding channels, in terms of their unitary dilation.
We note here that the parameter 𝜔 scales with the energy We illustrate Theorem 4 with a simple worked example.
cost of applying the given family of encoding channels on 𝜌, Consider a qubit system, with the free set F = {|0ih0|} being
with finer 𝜃-resolution costing more energy. We expand on this a trivial set with only a single element. Let 𝐺 = 𝜎𝑧 , the Pauli
connection in [47], together with a proof of Theorem 3; there matrix in the 𝑧 direction. In this case, the feasible set only
we also discuss why we suspect the upper bound (15) cannot be has one state 𝑋 𝐴𝐵 = |0ih0| ⊗ |0ih0|, from which we can verify
made independent of the estimation task in general. Finding 𝑠∗ = 0. Since (𝜆max − 𝜆min ) 2 = 4, from Theorem 4, there must
upper bounds for the case of more general measurements is exist some state 𝜌 ∉ F such that 𝑁𝐶 (𝜌) > 0. One can repeat
left for future work. the same argument for the case where F = {|1ih1|}. Since
the FI is convex [2], 𝜌 must outperform any convex mixture of
Quantum resources for unitary encodings — We now consider
|0ih0| and |1ih1|, i.e. any incoherent quantum state. This is one
the important special case where the quantum channel Φ 𝜃 is a
way to verify that quantum coherence is a useful nonclassical
unitary encoding channel Φ 𝜃 (𝜌) = 𝑈 𝜃 𝜌𝑈 †𝜃 and 𝑈 𝜃 ≔ 𝑒 −𝑖 𝜃𝐺 .
resource for the unitary encoding generated by 𝐺 = 𝜎𝑧 .
Here, 𝐺 is some Hermitian operator specifying the unitary
evolution, and is called the generator of the unitary encoding. Identifying nonclassical operations — Thus far, we have con-
Given any unitary encoding generated by the Hermitian op- sidered the use of the FI to identify general resources in quan-
erator 𝐺, one may be interested to know whether the parameter tum states. Recall that every quantum resource theory is also
estimation problem corresponding to 𝐺 is benefited by having accompanied by some set of free quantum operations O. Just
nonclassical states in a given quantum resource theory. The as any resourceful state can be defined as a state that is not in
following result establishes a simple criterion for determining the set of free states F , we can similarly define a resourceful
whether 𝐺 reveals nonclassicality. operation as any quantum channel not in the set O [62, 63]. It
Theorem 4. Consider any Hermitian generator 𝐺 and convex turns out that the FI can also universally distinguish operations
set of free states F . Let 𝑠∗ be an optimal solution to the convex with and without a given resource.
optimization problem Theorem 5. For any set of free operations O and quantum map
Ξ ∉ O, there exists a quantum trajectory 𝜌 𝜃 on an extended
maximize 2Tr[(𝐺 𝐴 ⊗ 11𝐵 − 11 𝐴 ⊗ 𝐺 𝐵 ) 2 𝑋 𝐴𝐵 ] Hilbert space such that the map 11 ⊗ Ξ satisfies
𝑋 ≥0
subject to Tr 𝐴 𝑋 𝐴𝐵 = Tr𝐵 𝑋 𝐴𝐵 = 𝜎 ∈ F . 𝐹𝐶 [11 ⊗ Ξ(𝜌 𝜃 ) | 𝑀] > max 𝐹𝐶 [11 ⊗ Ω(𝜌 𝜃 ) | 𝑀] (16)
Ω∈F

Let 𝜆max , 𝜆min denote the largest and smallest eigenvalues for some 𝜃.
of the generator 𝐺 resepectively. If (𝜆max − 𝜆min ) 2 > 𝑠∗ , then
𝑁 𝑄 (𝜌) > 0 for some 𝜌. A full discussion of the proof can be found in [47]. The-
orem 5 demonstrates that the FI plays a foundational role not
Proof. One may immediately verify that the objective function just in the study of nonclassicality in states, but also in the
2Tr[(𝐺 𝐴 ⊗ 11 𝐵 − 11 𝐴 ⊗ 𝐺 𝐵 ) 2 𝑋 𝐴𝐵 ] is linear and that the feasible study of the resources of quantum channels.
set is convex, so 𝑠∗ is the solution to a convex optimization
problem. Conclusion — Many quantities traditionally used to study the
To prove the statement, we just need to show that 𝑠∗ upper nonclassical features of quantum mechanics are typically rele-
bounds max 𝜎 ∈F 𝐹𝑄 (𝜎). In general, for any generator 𝐺 the vant only when considering specific notions of nonclassicality.
maximum achievable QFI can be verified to be (𝜆max − 𝜆min ) 2 However, quantum advantages in different tasks rely on a broad
[61], so if (𝜆max − 𝜆min ) 2 > 𝑠∗ ≥ max 𝜎 ∈F 𝐹𝑄 (𝜎), we neces- range of quantum phenomena, motivating the study of phys-
sarily have 𝑁 𝑄 (𝜌) > 0. ical quantities which can be used to identify all reasonable
5

quantum resources. To this end, we showed that two Fisher resourceful states. For the case of estimation problems with
information (FI)-based quantities 𝑁𝐶 and 𝑁 𝑄 , defined through binary outcomes, we also provided an upper bound, in terms
the classical and quantum variants of the FI, respectively, are of a related quantity called the standard robustness. The spe-
examples of such universally relevant operational quantities. cial case of unitary encodings was also considered, where we
This implies that every quantum resource can provide a quan- provided a simple criterion to test whether a given quantum re-
tum advantage in some parameter estimation problem. In this source provides an advantage for a unitary encoding generated
sense, any feasible notion of nonclassicality objectively al- by a Hermitian operator 𝐺. Finally, we showed that not only
ways provides a quantum advantage in metrology, although it does the FI universally identify resources of quantum states, it
remains subjective as to whether such applications are relevant also universally witnesses resourceful quantum operations in
to the interests of an experimentalist. We also highlight that, every resource theory. These results solidify the central role
while the focus of this work is on identifying (detecting) gen- that the FI plays in the study of quantum resources.
eral quantum resources, it is also possible to construct resource
measures — also called resource monotones — using 𝑁𝐶 and
𝑁 𝑄 . This is discussed in greater detail in the Supplemental Acknowledgments — K.C.T. and B.R. acknowledge support by
Material [47]. the NTU Presidential Postdoctoral Fellowship program funded
We then provided a lower bound on the maximum extent by Nanyang Technological University. V.N. acknowledges
of this quantum advantage in terms of the generalized robust- support from the Lee Kuan Yew Endowment Fund (Postdoc-
ness measure [34, 36, 40], which also universally identifies toral Fellowship).

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SUPPLEMENTAL MATERIAL estimation task Φ 𝜃 such that

𝑅(𝜌) 2 ≤ 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀) ≤ 𝑅(𝜌) 2 + 2𝑅(𝜌), (18)


In this Supplemental Material, we provide detailed technical
proofs of several theorems in the main text, as well as addi- In particular, 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀) > 0 iff 𝜌 ∉ F , and 𝑁𝐶max (𝜌) ≥
tional discussions comparing classical and quantum Fisher 𝑅(𝜌) 2 is a computable lower bound for any resource.
information, as well as how the Fisher information may be Furthermore, if the resource theory is affine — that is, the
used to construct nonclassicality measures in general resource set F is the intersection of some affine subspace with the set
theories. of density matrices — then 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀) = 𝑅(𝜌) 2 .
Proof. We will use the fact that the robustness can be written
as [64, 65]

A. Proof of Theorem 2 𝑅(𝜌) = sup { Tr(𝑊 𝜌) − 1 | 𝑊 ≥ 0, Tr(𝑊𝜎) ≤ 1 ∀𝜎 ∈ F } ,


(19)
and let 𝑊 ≠ 0 be any feasible solution to the above optimisa-
We employ the (generalized) robustness measure 𝑅 [40], tion. As shown in [34, Thm. 2], there exists a channel discrimi-
given by nation task with 𝑑 channels {Λ𝑖 } (in fact, unitary channels) and
a POVM 𝑁 = {𝑁𝑖 } such that the probability of successfully
discriminating the channels with uniform prior probability for
 
𝜌 + 𝜆𝜔
𝑅(𝜌) = inf 𝜆
∈F , (17) any input state 𝜏 is
1+𝜆
Õ1 Tr(𝑊𝜏)
𝑝 succ (𝜏) ≔ Tr(Λ𝑖 (𝜏)𝑁𝑖 ) = . (20)
where the optimization is over all quantum states 𝜔. 𝑑 Tr𝑊
𝑖
The result below is a slight extension of the statement of
Thm. 2 from the main text. We then define 𝜎0 ≔ argmin 𝜎 ∈F Tr(𝑊𝜎).
We will first assume that 𝑝 succ (𝜎0 ) > 0, so that Tr(𝑊𝜎0 ) >
0. Noticing that Tr𝑊 ≥ Tr(𝑊𝜎0 ), we then define the channel
Theorem. In any resource theory, there exists a parameter Φ 𝜃 as

!
Õ1 p
A 𝜃 (𝜏) ≔ Λ𝑖 (𝜏) ⊗ |𝑖ih𝑖| ⊗ Tr(𝑊𝜎0 ) (Tr𝑊 − Tr(𝑊𝜎0 )) 𝜃 |0ih0|
𝑖
𝑑
!
Õ1 p
+ Λ𝑖 (𝜎0 ) ⊗ |𝑖ih𝑖| ⊗ (1 − Tr(𝑊𝜎0 ) (Tr𝑊 − Tr(𝑊𝜎0 )) 𝜃) |1ih1| , (21)
𝑖
𝑑
" #! " #!
Õ Õ
Φ 𝜃 (𝜏) ≔Tr A 𝜃 (𝜏) 𝑁𝑖 ⊗ |𝑖ih𝑖| ⊗ 11 |0ih0| + Tr A 𝜃 (𝜏) 𝑁𝑖 ⊗ | 𝑗ih 𝑗 | ⊗ 11 |1ih1|
𝑖 𝑖≠ 𝑗

where, without loss of generality, we have taken 𝜃 small enough so that A 𝜃 and Φ 𝜃 are valid CPTP maps. Performing the mea-
7

surement 𝑀 = {|0ih0| , |1ih1|}, we then obtain the statistics where we note that the terms inside the outer brackets are
p always non-negative. This gives
𝑃(0 | 𝜃) = 𝜃 Tr(𝑊𝜎0 ) (Tr𝑊 − Tr(𝑊𝜎0 )) 𝑝 succ (𝜏)
 p  𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀)
+ 1 − 𝜃 Tr(𝑊𝜎0 ) (Tr𝑊 − Tr(𝑊𝜎0 )) 𝑝 succ (𝜎0 ),
= [𝑅(𝜌) + 1 − Tr(𝑊 ★𝜎0 )] 2 − [1 − Tr(𝑊 ★ 𝜎0 )] 2
𝑃(1 | 𝜃) = 1 − 𝑃(0|𝜃). = 𝑅(𝜌) + 1 − Tr(𝑊 ★ 𝜎0 ) − 1 + Tr(𝑊 ★𝜎0 )
 
(29)
(22)
× 𝑅(𝜌) + 1 − Tr(𝑊 ★𝜎0 ) + 1 − Tr(𝑊 ★ 𝜎0 )
 
We can then use Eq. (1) to compute the classical information
of the statistics. One may verify that = 𝑅(𝜌) 𝑅(𝜌) + 2(1 − Tr(𝑊 ★ 𝜎0 )) .
 

 2
𝜕
𝑃(0 | 𝜃) Since Tr(𝑊 ★ 𝜎0 ) ∈ [0, 1], we thus see that
𝜕𝜃
𝐹𝐶 (𝜏 | Φ 𝜃 , 𝑀) = . (23)
𝑃(0 | 𝜃) (1 − 𝑃(0 | 𝜃)) 𝑅(𝜌) 2 ≤ 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀) ≤ 𝑅(𝜌) [𝑅(𝜌) + 2]. (30)
Evaluating near the vicinity of 𝜃 = 0, the resulting Fisher In the special case of affine resource theories, one can always
information is then choose an optimal 𝑊 ★ satisfying Tr(𝑊 ★ 𝜎) = 1 ∀𝜎 ∈ F [58],
𝐹𝐶 (𝜏 | Φ 𝜃 , 𝑀) which gives 𝑁𝐶 (𝜌|Φ 𝜃 , 𝑀) = 𝑅(𝜌) 2 .

[Tr(𝑊𝜎0 ) (Tr𝑊 − Tr(𝑊𝜎0 ))] [ 𝑝 succ (𝜏) − 𝑝 succ (𝜎0 )] 2
=
𝑝 succ (𝜎0 ) (1 − 𝑝 succ (𝜎0 )) Remark. We have seen in the proof that the lower bound
h i2 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀) ≥ 𝑅(𝜌) 2 can be tight. Note that there also
𝜎0 )
[Tr(𝑊𝜎0 ) (Tr𝑊 − Tr(𝑊𝜎0 ))] Tr(𝑊 𝜏)−Tr(𝑊 Tr𝑊 exist cases in which the upper bound is tight, in the sense that
=   𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀) = 𝑅(𝜌) 2 + 2𝑅(𝜌). This includes the resource
Tr(𝑊 𝜎0 ) Tr(𝑊 𝜎0 )
Tr𝑊 1 − Tr𝑊 theory of entanglement where, for a 𝑑 × 𝑑-dimensional pure
state 𝜌, the optimal witness 𝑊 ★ is simply 𝑊 ★ = 𝑑 |Ψ+ ihΨ+ |
= [Tr(𝑊𝜏) − Tr(𝑊𝜎0 )] 2 . + 1 Í ★
with |Ψ i = √ 𝑖 |𝑖𝑖i [54, 55], which satisfies Tr(𝑊 𝜎0 ) = 0.
(24) 𝑑
In the case that 𝑝 succ (𝜎0 ) = 0, we can make an analo- We also remark that the degenerate case 𝑅(𝜌) = ∞, which
gous choice of channels A 𝜃 , Φ 𝜃 but replacing the constant we have considered for completeness, can only occur when the
p
Tr(𝑊𝜎0 ) (Tr𝑊 − Tr(𝑊𝜎0 )) with Tr𝑊. This then gives the support of 𝜌 is not contained in the support of any state in F .
statistics In particular, as long as there exists at least one full-rank state
𝜎 ∈ F , we always have 𝑅(𝜌) < ∞.
𝑃(0 | 𝜃) = 𝜃Tr𝑊 𝑝 succ (𝜏)
(25)
𝑃(1 | 𝜃) = 1 − 𝜃Tr𝑊 𝑝 succ (𝜏).
B. Proof of Theorem 3
Taking 𝜃 to 0, this gives
Here, we employ the standard robustness [40]
𝐹𝐶 (𝜏 | Φ 𝜃 , 𝑀) = [Tr𝑊 𝑝 succ (𝜏)] 2
 
𝜌 + 𝜆𝜎
= [Tr(𝑊𝜏)] 2 (26) 𝑅𝑆 (𝜌) = inf 𝜆 ∈ F, 𝜎 ∈ F . (31)
2 1+𝜆
= [Tr(𝑊𝜏) − Tr(𝑊𝜎0 )]
Theorem. For any parameter estimation task with encod-
analogously to the case 𝑝 succ (𝜎0 ) > 0. ing channel family Φ 𝜃 and two-outcome measurement 𝑀 ≡
Noticing that 𝐹𝐶 (𝜎 | Φ 𝜃 , 𝑀) ≤ 1 for any 𝜎 ∈ F , we have (𝑃, 11 − 𝑃), let 𝑟 ≔ 𝐹𝐶 (𝜌 | 𝑀) < ∞ and
that Φ 𝜃 ∈ P, and so

𝜕Tr[𝑃 Φ 𝜃 (𝜌)]
𝑁𝐶max (𝜌) ≥ 𝑁𝐶 (𝜌|Φ 𝜃 , 𝑀) 𝜔 := . (32)
𝜕𝜃
𝜃=0
= [Tr(𝑊 𝜌) − Tr(𝑊𝜎0 )] 2 − max [Tr(𝑊𝜎) − Tr(𝑊𝜎0 )] 2 .
𝜎 ∈F
Then,
(27)
In the degenerate case 𝑅(𝜌) = ∞, Tr(𝑊 𝜌) can be made ar- [𝑅𝑆 (𝜌) + 1] −2 𝜔2
bitrarily large, so we see that 𝑁𝐶max (𝜌) = ∞. Assuming then 𝑁𝐶 (𝜌 | 𝑀) ≤ 𝑟 −
max Tr[𝑃 Φ0 (𝜏)] (1 − Tr[𝑃 Φ0 (𝜏)])
that 𝑅(𝜌) < ∞, there must exist an optimal choice 𝑊 ★ such 𝜏 ∈F
that Tr(𝑊 ★ 𝜌) − 1 = 𝑅(𝜌); for such a choice, there must then [𝑅𝑆 (𝜌) + 1] −2 𝜔2
exist 𝜎 ∈ F such that Tr(𝑊 ★𝜎) = 1, since otherwise we ≤𝑟−  ,
could rescale 𝑊 ★ to obtain a higher value of the robustness, max Tr[𝑃 Φ0 (𝜏)] 1 − min Tr[𝑃 Φ0 (𝜂)]
contradicting its optimality. With this choice of 𝑊, we obtain 𝜏 ∈F 𝜂 ∈F
(33)
𝐹𝐶 (𝜌 | Φ 𝜃 , 𝑀) = [𝑅(𝜌) + 1 − Tr(𝑊 ★𝜎0 )] 2 ,
(28) where 𝑅𝑆 (𝜌) is the standard robustness of 𝜌 with respect to
max 𝐹𝐶 (𝜎 | Φ 𝜃 , 𝑀) = [1 − Tr(𝑊 ★𝜎0 )] 2 , F.
𝜎 ∈F
8

Proof. For a given arbitrary two-outcome estimation task where 𝜌˜ ≡ Tr𝐶 (𝜌 𝐴 ⊗ |𝜓ih𝜓| 𝐵 ) is 𝜃-independent, and
[Φ 𝜃 , 𝑀 ≡ (𝑃, 11 − 𝑃)] and probe state 𝜏, define
𝐺 𝜌 = Tr𝐶 [𝜌 𝐴 ⊗ |𝜓ih𝜓| 𝐵 , 𝐻 𝐴𝐵 ] (41)
𝑝 𝜏 (𝜃) := Tr [𝑃 Φ 𝜃 (𝜏)] . (34) generates the action of Φ 𝜃 in the neighbourhood of 𝜃 = 0. We
thus have
as a function of the real parameter 𝜃. We then observe that
𝜕Tr[𝑃 Φ 𝜃 (𝜌)] 
𝜔= = Tr 𝑖𝑃 𝐺 𝜌 . (42)
𝑝¤2𝜏 (0) 𝜕𝜃
𝜃=0
𝐹𝐶 (𝜏 | Φ 𝜃 , 𝑀) = , (35)
𝑝 𝜏 (0) [1 − 𝑝 𝜏 (0)] Since 𝐻 is the Hamiltonian generating the encoding operation
where a dot above denotes the derivative wrt 𝜃. For brevity, on 𝜌, we see that 𝜔 is a measure of the order of magnitude of
we will omit the argument 0 for 𝑝 𝜏 and 𝑝¤ 𝜏 in the remainder, the energy used in executing the encoding on the support of
explicating only nonzero arguments where they occur. We first 𝜌 measured by 𝑃. In particular, the same encoding channel
note that family can be implemented at a finer resolution by using a
Hamiltonian 𝐻 ′ = 𝑐𝐻 (corresponding to 𝜔 ′ = 𝑐𝜔) for 𝑐 > 1.
𝑝¤2𝜎 Remark (more general bounds). Can we make the bound even
max 𝐹𝐶 (𝜎 | Φ 𝜃 , 𝑀) = max
𝜎 ∈F 𝜎 ∈F 𝑝 𝜎 (1 − 𝑝 𝜎 ) more task-independent than in Theorem 3? Unfortunately, this
max 𝑝¤2𝜎 is unlikely: while convex-geometric properties such as robust-
𝜎 ∈F
≥ (36) ness measures help upper-bound linear functionals like 𝑝 𝜏 for
max 𝑝 𝜏 (1 − 𝑝 𝜏 ) a resource state in terms of the maximum value attained in the
𝜏 ∈F
convex free set F , the nonlinear 𝑝 𝜏 (1 − 𝑝 𝜏 ) appears to have
We will now lower-bound the numerator. To this end, con- no such task-independent bounds. A possible recourse might
sider the task of discriminating between the two channels (oc- be to use convex-geometric bounds on each of the two factors
curring with equal probabilities) Λ0 := 𝑀 ◦ Φ0 and Λ1 := in the denominator in the last expression in (33); however, the
𝑀 ◦ Φ 𝛿 for some small 𝛿 > 0, where 𝑀 is co-opted to denote resulting bound turns out to be worse than the 0.25 of the main
the channel 𝑀 ( 𝑋) := Tr (𝑃𝑋) |0ih0| + [1 − Tr (𝑃𝑋)] |1ih1|. theorem. On the other hand, by eschewing generality and con-
Using a probe state 𝜏, the game reduces to that of distinguish- sidering tasks where the performance of 𝜌 necessarily “costs”
ing the states at least 𝜔, we prevent 𝑝 𝜌 (1 − 𝑝 𝜌 ) from getting vanishingly
small and helping 𝜌 attain arbitrarily high FI at a fixed energy
𝑝 𝜏 (𝑘𝛿) |0ih0| + [1 − 𝑝 𝜏 (𝑘𝛿)] |1ih1| , cost.
𝑘 ∈ {0, 1}. By the Haelstrom bound, the “bias” or “gain”
that the best distinguishing strategy achieves over a random C. Proof of Theorem 5
guess (what [36] denotes by variants of the notation 𝑝 gain ) is
proportional to 𝛿 | 𝑝¤ 𝜏 | for small 𝛿. Now we invoke [36, Thm.
Theorem. For any set of free operations O and quantum map
7], which puts an upper bound on the gain of a given resource
Ξ ∉ O, there exists a quantum trajectory 𝜌 𝜃 on an extended
state relative to that achieved by the free states:
Hilbert space such that the map 11 ⊗ Ξ satisfies
𝑝 gain (𝜌) 𝐹𝐶 [11 ⊗ Ξ(𝜌 𝜃 ) | 𝑀] > max 𝐹𝐶 [11 ⊗ Ω(𝜌 𝜃 ) | 𝑀] (43)
≤ 𝑅𝑆 (𝜌) + 1. (37) Ω∈F
max 𝑝 gain (𝜎)
𝜎 ∈F
for some 𝜃.
By the above observation relating 𝑝 gain to 𝑝¤ 𝜏 , it follows that Proof. We will use the fact that for any set of free operations
O and quantum channel Ξ ∉ O, there exists some collection
𝑝¤2𝜌 𝜔2 of states and probabilities {𝑝 𝑖 , 𝜌𝑖 }, as well as POVMs {𝜋 𝑗 }
max 𝑝¤2𝜎 ≥ = . (38)
Í that 𝑝 succ (Ξ) > maxΩ∈O 𝑝 succ (Ω), where 𝑝 succ (Ξ) ≔
such
2
𝜎 ∈F [𝑅𝑆 (𝜌) + 1] [𝑅𝑆 (𝜌) + 1] 2
𝑖 𝑝 𝑖 Tr[ 11 ⊗ Ξ(𝜌 𝑖 )𝜋 𝑖 ](Ref. [34]).
The result of the theorem in the main text then follows by noting Consider the following input state:
that max 𝑝 𝜏 (1 − 𝑝 𝜏 ) ≤ 0.25, together with Eq. (36).  Õ
𝜏 ∈F 𝜌𝜃 ≔ 𝜌𝑖 ⊗ 𝑝 𝑖 |𝑖ih𝑖| ⊗ [𝜃 |0ih0| + (1 − 𝜃) |1ih1|]. (44)
𝑖
Remark (𝜔 as an energy scale). To understand the significance
of the parameter 𝜔, let us consider an encoding channel family For some Ω0 ∈ O, we consider the following series of quantum
given explicitly through its Stinespring dilation, as maps that depends on the map Ξ:

Φ 𝜃 ( 𝜌) = Tr𝐶 𝑒 −𝑖 𝜃 𝐻 𝐴𝐵 (𝜌 𝐴 ⊗ |𝜓ih𝜓| 𝐵 ) 𝑒 𝑖 𝜃 𝐻 𝐴𝐵 , (39)


 
Λ1 (𝜌 𝜃 ) (45)
where 𝐻 𝐴𝐵 is Hermitian, 𝐶 is some subsystem of 𝐴𝐵, and |𝜓i
Õ
≔𝜃 11 ⊗ Ξ(𝜌𝑖 ) ⊗ 𝑝 𝑖 |𝑖ih𝑖| ⊗ |0ih0| (46)
can be made 𝜃-independent as above without loss of generality. 𝑖
For a small 𝜃, we have Õ
+ (1 − 𝜃) 11 ⊗ Ω0 (𝜌𝑖 ) ⊗ 𝑝 𝑖 |𝑖ih𝑖| ⊗ |1ih1| . (47)
Φ 𝜃 ( 𝜌) ≈ 𝜌˜ + 𝑖𝜃𝐺 𝜌 , (40) 𝑖
9

Here, the map Λ1 performs the map 11 ⊗ Ξ on 𝜌𝑖 when the last Proposition 1. There exist resource theories and unitary en-
qubit is in the state |0i and performs some other operations codings of the form 𝑈 𝜃 = 𝑒 −𝑖 𝜃𝐺 where 𝑁𝐶 (𝜌 | 𝑀) identifies
11 ⊗ Ω0 where Ω0 ∈ O when the last qubit is in the state |1i. a strictly greater number of nonclassical states than 𝑁 𝑄 (𝜌).
We then consider the quantum map
This can be shown by considering an explicit example. As
mentioned above, recall that single parameter estimation prob-
Λ2 ◦ Λ1 (𝜌 𝜃 ) (48) lem, the set of nonclassical states identified by 𝑁𝐶 is at least as
≔ Tr{Λ1 (𝜌 𝜃 )𝜋 𝑖 ⊗ |𝑖ih𝑖| ⊗ 11} |0ih0| (49) large as the set identified by 𝑁 𝑄 . It therefore suffices to demon-
strate that there is at least one plausible set of classical states
+ Tr{Λ1 (𝜌 𝜃 )𝜋 𝑖 ⊗ ( 11 − |𝑖ih𝑖|) ⊗ 11} |1ih1| . (50) F where 𝑁 𝑄 (𝜌) = 0 for every unitary encoding 𝑈 𝜃 = 𝑒 −𝑖 𝜃𝐺 ,
but there exists Hermitian generator 𝐺 and measurement 𝑀
We then perform the projection 𝑃0 ≔ |0ih0| and 𝑃1 ≔ |1ih1|
where 𝑁𝐶 (𝜌 | 𝑀) > 0.
to obtain the statistics
To do this, let us consider an artificial but plausible resource
𝑃(0 | 𝜃) = 𝜃 𝑝 succ (Ξ) + (1 − 𝜃) 𝑝 succ (Ω0 ) (51) theory with free states F . Consider a qubit system where F is
some strict convex subset of the Bloch sphere.
and We define the subset F ≔
Conv ({|𝜙, 𝜃i | 𝜃 ∈ [𝜋/2, 3𝜋/2]}), where |𝜙, 𝜃i ≔
𝑃(1 | 𝜃) = 1 − 𝑃(0 | 𝜃). (52) cos(𝜃/2) |0i + 𝑒 𝑖 𝜙 sin(𝜃/2) |1i. This is just the lower
hemisphere of the Bloch sphere, inclusive of the 𝑥-𝑦 plane.
We can absorb the maps Λ1 , Λ2 and measurements 𝑃0 , 𝑃1 Since this is the convex hull over a set of pure states, it is also
and represent it as a single generalized measurement 𝑀 = a strict convex subset of the Bloch sphere, which makes it a
{𝑀𝑖 }. One may then verify that plausible set of classical states to consider for some resource
theory based on the assumptions made in the main text.
(0| 𝜃) 2
( 𝜕𝑃𝜕𝜃 ) Consider now the set of all possible unitary encodings 𝑈 𝜃 =
𝐹𝐶 [11 ⊗ Ξ(𝜌 𝜃 ) | 𝑀] = . (53) 𝑒 −𝑖𝜇𝐺 . Since the set of Pauli matrices {11, 𝜎𝑥 , 𝜎𝑦 , 𝜎𝑧 } spans
𝑃(0 | 𝜃) (1 − 𝑃(0 | 𝜃))
the operator space, we see that every Hermitian generator 𝐺
Similar to Theorem 1, evaluating near the vicinity of 𝜃 = 0, can be written as 𝑟 0 11 + 𝑟®.® 𝜎 , where 𝜎® = 𝜎𝑥 , 𝜎𝑦 , 𝜎𝑧 ) is the
the resulting Fisher information is vector of Pauli matrices. Since 𝑒 −𝑖𝜇𝑟0 11 just adds a global
phase, it does not affect any measurement statistics, so we
[ 𝑝 succ (Ξ) − 𝑝 succ (Ω0 )] 2 can just consider a Hermitian generator of the type 𝐺 = 𝑟®.® 𝜎.
𝐹𝐶 [11 ⊗ Ξ(𝜌 𝜃 ) | 𝑀] = . (54)
𝑝 succ (Ω0 ) (1 − 𝑝 succ (Ω0 )) Without any loss in generality, we can also normalize 𝐺 such
that | 𝑟®| = 1. This means that 𝐺 = 𝑟®.®𝜎 is a Pauli matrix pointing
The quantum map Ω0 is not yet specified. We choose it such in the direction 𝑟®. To summarize, this means that every unitary
that it satisfies 𝑝 succ (Ω0 ) = minΩ∈O 𝑝 succ (Ω). This means that encoding on the Bloch sphere is equivalent to a rotation about
𝐹𝐶 [11 ⊗ Ξ(𝜌 𝜃 ) | 𝑀] is a monotonically increasing function of an axis 𝑟®.
𝑝 succ (Ξ). Together with the fact that 𝑝 succ (Ξ) > 𝑝 succ (Ω) for For 𝐺 = 𝜎𝑧 , it is known that every pure state lying
every Ω ∈ O, we must have 𝑖 𝜙
√ on the 𝑥-𝑦
plane, i.e. every state of the form (|0i+𝑒 |1i)/ 2, maximizes
the quantum Fisher information. We see that these states lie on
𝐹𝐶 [11 ⊗ Ξ(𝜌 𝜃 ) | 𝑀] > max 𝐹𝐶 [11 ⊗ Ω(𝜌 𝜃 ) | 𝑀] (55)
Ω∈F a greater circle on the Bloch sphere. The problem of finding
𝐺 = 𝑟®.® 𝜎 such that 𝑁 𝑄 (𝜌) > 0 for some 𝜌 therefore boils down
in the vicinity 𝜃 = 0. This shows the existence of at least to finding a greater circle on the Bloch sphere which does not
one quantum trajectory 𝜌 𝜃 where 𝐹𝐶 [11 ⊗ Ξ(𝜌 𝜃 ) | 𝑀] > intersect the set of classical states F . If the greater sphere in-
maxΩ∈F 𝐹𝐶 [11 ⊗ Ω(𝜌 𝜃 ) | 𝑀] for some value of 𝜃.  tersects F , then there exists a classical state which maximizes
the quantum Fisher information, which necessarily means that
𝑁 𝑄 (𝜌) ≯ 0. However, we see that it is impossible to draw a
D. Comparison between classical and quantum Fisher greater circle without intersecting the lower hemisphere. 𝑁 𝑄
information for resource identification is therefore unable to identify any nonclassical state outside of
F over the set of unitary encodings.
In the main text, we make a distinction between classical Let us consider 𝐺 = 𝜎𝑦 /2 and POVMs 𝑀0 = |0ih0| +
and quantum Fisher information and defined corresponding |1ih1| /2 and 𝑀1 = |1ih1| /2. First, we note that 𝐺 generates
resource witnesses 𝑁𝐶 and 𝑁 𝑄 . In was also discussed in a rotation about the 𝑦-axis. Any component along the 𝑦 axis
the main text that the classical Fisher information is at least as therefore does not contain any information about this rotation.
good as the quantum Fisher information at identifying resource It therefore suffices to optimize the classical Fisher information
states. This is because for any parametrized channel Φ 𝜃 , in over the 𝑧-𝑥 plane. One can then verify that the resulting
the sense that it is always possible to find a measurement 𝑀 ★ classical Fisher information for any input state |𝜙 = 0, 𝜃i ≔
such that 𝑁𝐶 (𝜌 | 𝑀 ★) ≥ 𝑁 𝑄 (𝜌). In fact, there exist situations cos(𝜃/2) |0i + sin(𝜃/2) |1i is given by 𝐹𝐶 (|𝜙, 𝜃ih𝜙, 𝜃| | 𝑀) =
where 𝑁𝐶 is a strictly better resource identifier than 𝑁 𝑄 . This 2 cos2 (𝜃/2)/(3 + cos 𝜃). Over the top hemisphere, this is
is summarized by the following statement: maximized by the state |0i, and 𝐹𝐶 (|0ih0| | 𝑀) = 1/2. Over
10

the bottom
√ hemisphere, this is maximized by |+i ≔ (|0i + property. Recall that
|1i)/ 2, for which 𝐹𝐶 (|+ih+| | 𝑀) = 1/3. We therefore have
𝑁𝐶 (|0ih0| | 𝑀) = 1/2 − 1/3 = 1/6. This shows that there 𝑁𝐶max (𝜌) ≔ max 𝑁𝐶 (𝜌 | Φ 𝜃 , 𝑀), (56)
Φ 𝜃 ∈P, 𝑀
exists some 𝐺 and measurement 𝑀 such that 𝑁𝐶 (𝜌 | 𝑀) > 0
for some 𝜌. Thus demonstrates that 𝑁𝐶 identifies strictly more where P is the set of all parameter estimation problems satis-
nonclassical states than 𝑁 𝑄 over all possible unitary encodings fying max 𝜎 ∈F 𝐹𝐶 (𝜎 | Φ 𝜃 , 𝑀) ≤ 1.
and resource theories. The following theorem shows that the above quantity is a
resource monotone in general resource theories.

E. General resource measures based on Fisher information Theorem. In any quantum resource theory with resource
states F and free operations O, the quantity 𝑁𝐶max (𝜌) is a re-
The main text focused on the use of Fisher information to source measure in the sense that it satisfies: (i) 𝑁𝐶max (𝜌) ≥ 0
identify resource states in general resource theories. Here, we for every state 𝜌 and 𝑁𝐶max (𝜌) > 0 iff 𝜌 is nonclassical.
provide addition discussion on how Fisher information based (ii) 𝑁𝐶max monotonically decreases under free operations, i.e.
measures can be used to measure the resourcefulness of a 𝑁𝐶max [Φ(𝜌)] ≤ 𝑁𝐶max (𝜌) for any Φ (iii) 𝑁𝐶max is a convex
Í ∈ O. max
max
function of state, i.e. 𝑁𝐶 [𝜌] ≤ 𝑖 𝑝 𝑖 𝑁𝐶 (𝜌𝑖 ).
quantum state, again, within the context of general resource
theories.
Proof. To prove the first property, we first see that from The-
A fundamental property of a resource quantifiers is that they
orem 1, there must exist Φ 𝜃 and 𝑀 s.t. 𝑁𝐶 (𝜌 | 𝜙 𝜃 , 𝑀) > 0
should be convex functions of state. If a resource quantifier is
if 𝜌 is nonclassical, hence 𝑁𝐶max (𝜌) > 0 if 𝜌 is nonclassical.
not convex, we face a problematic situation where preparing a
Conversely, if 𝑁𝐶max (𝜌) > 0 then 𝑁𝐶max (𝜌) > 0 for some Φ 𝜃
simple statistical mixture of states, which is a classical process,
and 𝑀, so the state must be nonclassical. We also see that if
can increase the amount of quantum resource in the system. In
𝜎 ∈ F is classical, then the identity encoding Φ 𝜃 = 11 will
the following proposition we establish that the quantities 𝑁𝐶
reach 𝑁𝐶max (𝜎) = 0 which is the maximum for a classical state.
and 𝑁 𝑄 are convex functions, so they avoid this complication.
Second, we show that 𝑁𝐶max (𝜌) always monotonically de-
creases under quantum operations. Suppose Φ′ ∈ O is a free
Proposition 2. Both Í 𝑁𝐶 (𝜌 | 𝑀) and 𝑁 𝑄 (𝜌)Íare convex func- operation, and let Φ∗𝜃 , 𝑀 ∗ be optimal for the state Φ′ (𝜌) such
tions of state, i.e. 𝑝 𝑖 𝑁𝐶 (𝜌𝑖 | 𝑀) ≥ 𝑁𝐶 ( 𝑖 𝑝 𝑖 Í
𝑖Í 𝜌𝑖 | 𝑀) and
that 𝑁𝐶max [Φ′ (𝜌)] = 𝑁𝐶 [Φ′ (𝜌) | Φ∗𝜃 , 𝑀 ∗ ]. We have the fol-
𝑖 𝑝 𝑖 𝑁 𝑄 (𝜌 𝑖 ) ≥ 𝑁𝐶 ( 𝑖 𝑝 𝑖 𝜌 𝑖 ), where 𝑝 𝑖 ≥ 0 and 𝑖 𝑝 𝑖 = 1.
Í
lowing chain of inequalities:
Proof. This property follows from the convexity of 𝐹𝐶 and
𝐹𝑄 [1, 2]. 𝑁𝐶max (𝜌) (57)
We first consider 𝑁𝐶 . From the definition 𝑁𝐶 (𝜌 | 𝑀) ≔
 
𝐹𝐶 (𝜌 | 𝑀) − max 𝜎 ∈F 𝐹𝐶 (𝜎 | 𝑀), we see that the second = max 𝐹𝐶 (𝜌 | Φ 𝜃 , 𝑀) − max 𝐹𝐶 (𝜎 | Φ 𝜃 , 𝑀) (58)
Φ 𝜃 ∈P, 𝑀 𝜎 ∈F
term max 𝜎 ∈F 𝐹𝐶 (𝜎 | 𝑀) does not depend on the input state,
so if 𝐹𝐶 (𝜌 | 𝑀) is convex, so is 𝑁𝐶 (𝜌 | 𝑀). ≥ 𝐹𝐶 (𝜌 | Φ∗𝜃 ◦ Φ′ , 𝑀 ∗ ) − max 𝐹𝐶 (𝜎 | Φ∗𝜃 ◦ Φ′ , 𝑀 ∗ ) (59)
𝜎 ∈F
Consider two states 𝜌 and 𝜎, with statistics 𝑃𝜌 (𝑖 | = 𝐹𝐶 [Φ′ (𝜌) | Φ∗𝜃 , 𝑀 ∗ ] − max 𝐹𝐶 [Φ′ (𝜎) | Φ∗𝜃 , 𝑀 ∗ ] (60)
𝜃) = Tr[Φ 𝜃 (𝜌) 𝑀𝑖 ] and 𝑃 𝜎 (𝑖 | 𝜃) = Tr[Φ 𝜃 (𝜎) 𝑀𝑖 ]. The 𝜎 ∈F
convex combination 𝑝𝜌 + (1 − 𝑝)𝜎 leads to the statistics ≥ 𝐹𝐶 [Φ′ (𝜌) | Φ∗𝜃 , 𝑀 ∗ ] − max 𝐹𝐶 [𝜎 | Φ∗𝜃 , 𝑀 ∗ ] (61)
𝑃 𝑝𝜌+(1− 𝑝)) 𝜎 (𝑖 | 𝜃) = 𝑝𝑃𝜌 (𝑖 | 𝜃) + (1 − 𝑝)𝑃 𝜎 (𝑖 | 𝜃), where 𝜎 ∈F
𝑝 ∈ [0, 1]. We see that this is just the convex combina- = 𝑁𝐶max [Φ′ (𝜌)]. (62)
tion of two distributions 𝑃𝜌 (𝑖 | 𝜃) and 𝑃 𝜎 (𝑖 | 𝜃). It is
known that the classical Fisher information 𝐹𝐶 is convex The first inequality above comes from the fact that Φ∗𝜃 ◦Φ′ , 𝑀 ∗
function over classical probability distributions so we have is in general suboptimal for the state 𝜌. The second inequality
𝑝𝐹𝐶 (𝜌 | 𝑀) + (1 − 𝑝)𝐹𝐶 (𝜎 | 𝑀) ≥ 𝐹𝐶 ( 𝑝𝜌 + (1 − 𝑝)𝜎 | 𝑀). comes from the fact that Φ′ ∈ O is a free operation, so Φ′ (𝜎) ∈
This shows that 𝐹𝐶 (𝜌 | 𝑀) is convex so 𝑁𝐶 is also a convex F for every 𝜎 ∈ F .
function of state. Finally,Íwe show that it is a convex function of state. Sup-
Similarly, 𝐹𝑄 (𝜌) is known to be a convex function of state pose 𝜌 = 𝑖 𝑝 𝑖 𝜌𝑖 , and let Φ∗𝜃 , 𝑀 ∗ and Φ∗𝜃,𝑖 , 𝑀𝑖∗ be the optimal
so 𝑁 𝑄 (𝜌) must also be convex. channel encodings and measurements for 𝜌 and 𝜌𝑖 respectively.
 We then have

In general resource theories, a function of state is considered 𝑁𝐶max (𝜌) = 𝑁𝐶 (𝜌 | Φ∗𝜃 , 𝑀 ∗ ) (63)
Õ
a resource measure only when it monotonically decreases un- ≤ 𝑝 𝑖 𝑁𝐶 (𝜌𝑖 | Φ∗𝜃 , 𝑀 ∗ ) (64)
der some set of “free" quantum operations O. The exact nature 𝑖
of O varies depending on the resource theory under consider- Õ
ation, but they share one thing in common: they always map ≤ 𝑝 𝑖 𝑁𝐶 (𝜌𝑖 | Φ∗𝜃,𝑖 , 𝑀𝑖∗ ) (65)
𝑖
a classical state to another classical state, i.e. if Φ ∈ O, then Õ
Φ(𝜎) ∈ F for every 𝜎 ∈ F . We will discuss the construction = 𝑝 𝑖 𝑁𝐶max (𝜌𝑖 ), (66)
𝑁𝐶max based on 𝑁𝐶 that naturally satisfies this monotonicity 𝑖
11

where the first inequality comes from the convexity of 𝑁𝐶 where P is the set of all parameter estimation problems satisfy-
(Proposition 2) and the second inequality comes from the sub- ing max 𝜎 ∈F 𝐹𝑄 (𝜎 | Φ 𝜃 ) ≤ 1. It can also be shown that 𝑁 𝑄max

optimality of Φ∗𝜃 , 𝑀 ∗ for the state 𝜌𝑖 . also monotonically decreases under free operations, following
 largely identical arguments as 𝑁𝐶max .
We have shown that 𝑁𝐶max is a resource monotone. One may
also consider the quantum Fisher information based measure
max
𝑁𝑄 (𝜌) ≔ max 𝑁 𝑄 (𝜌 | Φ 𝜃 ), (67)
Φ 𝜃 ∈P

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