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Brazilian Journal

of Chemical ISSN 0104-6632


Printed in Brazil
Engineering
Vol. 21, No. 02 pp. 275 - 284, April - June 2004

A STUDY OF A WIRE-PLATE ELECTROSTATIC


PRECIPITATOR OPERATING IN THE REMOVAL
OF POLYDISPERSED PARTICLES
S. W. Nóbrega1, M. C. R. Falaguasta2 and J. R. Coury2*
1
Departamento de Engenharia Química, Universidade Federal de Alagoas,
Phone +(55) (82) 214-1280, Fax +(55) (82) 214-1625, Campus A. C. Simões,
BR 104, km 14, 57072-970, Maceió - AL, Brazil.
E-mail: swn@ctec.ufal.br
2
Departamento de Engenharia Química, Universidade Federal de São Carlos,
Phone +(55) (16) 260-8264, Fax +(55) (16) 260-8266, Rodovia Washington
Luís, km 235, Cx. P. 676, CEP 13560-970, São Carlos - SP, Brazil.
E-mail: jcoury@power.ufscar.br

(Received: February 13, 2003 ; Accepted: October 7, 2003)

Abstract - Performance of a wire-plate electrostatic precipitator in the removal of particles with a wide
particle size distribution was evaluated. The experimental rig utilized consisted of a set of three precipitators
whose dimensions could be varied. It was observed that precipitator performance increased with an increase
in the gap between the collecting plates, which resulted in a substantial increase in energy consumption per
volume of cleaned gas. The grade efficiency predicted by correlations from the literature did not match the
experimental measurements, and a new correlation is proposed.
Keywords: electrostatic precipitator, gas cleaning, particle collection.

INTRODUCTION used a mathematical model to show that the wider


precipitators do not function as well. Navarrete et al.
The electrostatic precipitator is widely employed (1997), however, verified that precipitators with
in the control of particles emissions in different wider ducts were more efficient in the removal of
industrial processes. In this equipment, the particles high resistivity materials.
in the gaseous current are electrically charged and The performance of electrostatic precipitators is, in
separated from the gas under the influence of an general, evaluated under different electric operational
electric field. conditions, which is perhaps what leads to the different
Project and operation parameters have a big conclusions observed in the literature. The complexity
influence on the performance of a precipitator. of the phenomenon is poorly addressed in the models
Although a great deal of research has been done on available for predicting collection efficiency,
the influence of these parameters, contradictory particularly in the submicron particle size range.
conclusions are often reported. The objective of this work was to study the
The shape of the precipitator has considerable performance of the electrostatic precipitator in the
influence on its performance. Many researchers (e.g. removal of a particulate with a wide range of sizes,
Leonard et al., 1980; Petersen, 1981; Riehle and under different operational conditions and to
Löffler, 1992a) discuss this influence, but the compare the results for collection efficiency with
conclusions are contradictory. Chang and Bai (2000) predictions by available theoretical models.

*To whom correspondence should be addressed


276 S. W. Nóbrega, M. C. R. Falaguasta and J. R. Coury

Collection Efficiency Co b v
C(x, y) exp(X ') (5)
In the literature there are several correlations for 2 SD p x
prediction of collection efficiency in electrostatic
precipitators. However, their use has been limited by with
empirical constants that are difficult to estimate as
well by their complexity in some cases (Zhao and 2
§ wx ·
Pfeffer, 1996). v¨ y  ¸
v ¹
The classic model for collection efficiency, X'  © (6)
known as the Deutsch equation, Equation 1, is still 4Dp x
frequently used to predict the performance of
precipitators due to its simplicity (Riehle, 1997). In where y and x are the axial and traverse distances in
this model it is assumed that the profile for respect to the gas flow, respectively.
concentration of particles in any traverse section of From the definition of collection efficiency, it
the duct is uniform. follows that
§  w th A · §  w th L NE ·
¨ ¸ ¨
vos
¸ §  Pe( [ De)2 ·
Kdpi 1 e © Q ¹ 1 e © ¹ (1) 0.5 ¨ ¸
§ Pe · 1 ¨ 4De ¸
Kdpi 1 ¨ ¸ ³ e© ¹ d[ (7)
In this equation, wth is the theoretical migration © 4SDe ¹ 0

velocity, which is obtained from the use of balance


equations on a particle, assuming Stokes law, and is where the Pèclet, Pe, and Deutsche, De, numbers are
given by given by

Qf w th .s
p ECu Pe (8)
w th (2) Dp
3SPd p

To calculate migration velocity, Riehle (1997) w th .L NE


De (9)
suggests using the Cochet equation (Equation 3) for vo .s
estimation of the saturation charge of the particles,
Qpf. The electric field, still according to Riehle, can Equation 7 is therefore the theoretical model of
be estimated by the ratio of applied potential to the Zhibin and Guoquan (1994) for collection efficiency
distance of the wire from the plate (s). in electrostatic precipitators.
ª § · º
2 ¨
«§ · ¸ »
«¨1  2O ¸  ¨ 2 ¸ ¨ H r  1 ¸ » SH d 2 E
§ · (3)
Qf
p
MATERIALS AND METHODS
«¨ d p ¸ ¨ 2O ¸ © H r  2 ¹ » o p
«© ¹ ¨1 »
«¬ © d p ¸¹ »¼
Experimental Setup

Attempting to avoid the assumption of a constant The experimental system used in this study
concentration profile in the Deutsch model, several consisted of three electrostatic precipitators of the
other researchers suggested new models that consider wire-plate type, whose main dimensions are given in
the diffusivity of the particle in the flowing gas. Table 1. A schematic view of one of the three
Zhibin and Guoquan (1994) included the effect of modules is shown in Figure 1.
diffusion in their development of an analytic model Each precipitator consisted of a rectangular box
for collection efficiency in which the equation of built of acrylic and PVC, with the lateral walls
bidimensional transport of the particles as a function covered by grounded copper plates. These plates
of concentration (Equation 4) was analytically constituted the collection electrodes. The discharge
solved. Equation 5 gives the solution presented by electrodes were stainless steel wires, stretched
the authors. halfway and orthogonal between the collecting
plates. The distance between the electrodes (2c)
w 2C wC wC could be varied for each precipitator, according to
Dp 2
 vo w th (4)
wy wx wy the values presented in Table 1.

Brazilian Journal of Chemical Engineering


A Study of a Wire-Plate Electrostatic Precipitator 277

Table 1: Main dimensions of the precipitators utilized.

Precipitator
01 02 03
2s (cm) 10 15 20
2c (cm) 3.3; 5.0; 10.0 5.0; 7.5; 15.0 6.6; 10.0; 20.0
2rSE (mm) 0.5 0.5 0.5
LNE (cm) 60 60 60
hNE (cm) 30 30 30

high-voltage
supply

blower

sampling sampling port


powder
port
feed
(a)
2s

hNE
2c
2rSE LNE

(b)
Figure 1: (a) Scheme of a module of the experimental unit; (b) Shape of the precipitator

100

90

80

70
Accum. fraction (%)

60

50

40

30

20

10

0
0.1 1 10 100
dp (Pm)

Figure 2: Size distribution of the particulate matter utilized.

Brazilian Journal of Chemical Engineering Vol. 21, No. 02, pp. 275 - 284, April - June 2004
278 S. W. Nóbrega, M. C. R. Falaguasta and J. R. Coury

Particulate collection area (A/Q), for three values of applied


electric field. All the curves show an identical
The particulate material used in the experimental behavior: efficiency reaches a minimum in the
tests was a phosphatic concentrate with an electric vicinity of the 1 Pm size range. Efficiency in the
resistivity of 8.3˜108 Wm, a dielectric constant of removal of larger particles is well understood and the
6.5 and a density of 3.0 ˜10 3 kg/m3. The size electric force created by the precipitator is reliably
correlated with removal forces. Some comprehensive
analysis of this powder was obtained utilizing an
reviews on the subject can be found in the literature
equipment, the Malvern Mastersizer, which
(Oglesby and Nichols, 1978; Parker, 1997).
determines the particle size distribution by laser
Conversely, efficiency in the submicron range does
diffraction. The size distribution of the powder
not have a clear theoretical description and is still
utilized in this work is shown in Figure 2.
poorly understood. In this size range, the effects of
turbulent diffusion and of discontinuity of the
Experimental Tests
flowing medium can prevail.
Figure 3 also shows that an increase in the width
The methodology used in the tests consisted in
of the duct increased particles removal, especially for
initially setting up the experimental system with the
the electric field of low intensity. The fact that wider
levels of the variables to be tested: the blower was
precipitators function better is known as the "non-
started and the air flow rate adjusted so that the gas
Deutschian" phenomenon (Chang and Bai, 2000).
velocity inside the precipitator reached the required
Riehle and Löffler (1992b) attribute this behavior to
value.
the fact that the electric field increases in proximity
The test was then started with the feeding of the
to the collection plates with the increase in the width
particulate matter. After reaching the steady state
of the duct, intensifying the collection of particles.
(approximately five minutes), the powder concentration
Although the results show that wider precipitators
was measured at the entrance of the system by
function better, it is important to observe that the
isokinetic sampling. Soon after, a new sampling was
costs of installation and operation for these
taken as the matter left the precipitator to obtain the
precipitators are higher than those for narrower
concentration of particles at the exit of the system.
ducts. This is because the increased width of the duct
The grade efficiency of collection (Kdpi) for each
requires a proportional increase in the electric
test was obtained from the size analysis of the
potential to maintain the same electric field.
particulate matter retained in the filters used in the
Consequently, it is necessary to utilize a high-voltage
samplings. The particulate matter sampled from the
source of larger capacity, increasing the initial cost
precipitator was re-dispersed in a solution (deionized
of installation. Regarding the cost of operation, the
water plus dispersant agent) utilizing an ultrasonic
power consumed by unit of flow rate of treated gas
bath. The suspension was then put in a Malvern
increases with the width of the duct, as can be
Mastersizer, where size was analyzed.
observed in Figure 4, where the values in percentage
From the results obtained in these analyses,
represent the increase in consumption of electricity.
together with the particle concentrations at the
Therefore, an increase in the width of the duct might
entrance and exit of the system, grade efficiency was
not be economically viable, especially when the
calculated with the use of the following equation
specific collection area (A/Q) is small.
Another form of evaluating the influence of
§ cS 'dSpi · distance between the collection plates (2s) is by
Kdpi (%) ¨1  ¸100 (10) comparing precipitator performance for different
¨ c E 'd Epi ¸
© ¹ duct widths with the same consumption of electricity
power per unit of treated gas flow rate. The results
obtained in these tests are presented in Figure 5.
RESULTS AND DISCUSSION Observing the behavior of these curves, it can be
observed that for the same amount of power
Influence of Duct Width on Precipitator consumed, performance of the precipitators improves
Performance as the distance between the plates decreases. This is
due to the fact that the increase in duct width
Figure 3 shows the experimental results of the requires more energy to increase the migration
performance of two precipitators with different velocity of the particles in order to compensate for
widths 2s, operating with the same specific the increase in the distance to be traveled.
Brazilian Journal of Chemical Engineering
A Study of a Wire-Plate Electrostatic Precipitator 279

100

90

80

Kdpi (%)
70

E = 3 kV/cm
60
2s = 0.10 m
2s = 0.20 m
50
0.1 1 10

dp (Pm)
100

90

80

Kdpi (%)
70

E = 4 kV/cm
60
2s = 0.10 m
2s = 0.20 m
50
0.1 1 10
dp (Pm)
100

90

80

Kdpi (%)
70

60 E = 5 kV/cm
2s = 0.10 m
2s = 0.20 m
50
0.1 1 10
dp (Pm)
Figure 3: Influence of 2s on collection efficiency: A/Q = 12 s/m; s/2c = 0.5

Brazilian Journal of Chemical Engineering Vol. 21, No. 02, pp. 275 - 284, April - June 2004
280 S. W. Nóbrega, M. C. R. Falaguasta and J. R. Coury

1800
22%
2s = 0.10 m
1600
2s = 0.20 m
1400

1200

Pelet (W/m /s)


1000

3
800 50%

600

400 199%

200

0
3 4 5
E (kV/cm)
Figure 4: Power consumption per unit of gas flow rate: A/Q = 12 s/m; S/2c = 0.5.
100

Kdpi (%) 90

80

70

60

50
3
P = 100 Watts/m /s
40
2s = 0.10 m
30 2s = 0.15 m
2s = 0.20 m
20
0.1 1 10

dp (Pm)

100

95
Kdpi (%)
90

85

80
3
P = 300 Watts/m /s
75
2s = 0.15 m
2s = 0.20 m
70
0.1 1 10

dp (Pm)
Figure 5: Influence of the distance between the plates on efficiency for precipitators
with the same power consumption per unit of gas flow rate.

Brazilian Journal of Chemical Engineering


A Study of a Wire-Plate Electrostatic Precipitator 281

Therefore, analyzing the influence of duct width the center of the precipitator duct and increases moving
(2s) on the performance of the precipitator, it becomes towards the collection plates, which seems quite
evident that an increase in this parameter generally reasonably in agreement with the experimental data
causes a higher energy consumption without, however, obtained by Schmid and Umhauer (1998) and shown in
resulting in a significant improvement in precipitator Figure 7. Riehle and Löffler (1993) also depicted this
performance. behavior in a number of photographs taken from inside a
wire-plate precipitator.
Comparison Between Theoretical Models and
Experimental Data on Grade Collection Efficiency v1.5 yCo b
C(x, y) exp(X ') (11)
Figure 6 compares values for grade collection wx SD p x
efficiency, obtained experimentally with predictions
by the models of Deutsch and Zhibin and Guoquan, where X' is given by Equation 6.
Equations 1 and 7, respectively. As can be seen in The equation for collection efficiency is given in
these figures, those correlations did not represent this case by
well the experimental data.
An alternative proposal to the solution given by Pe
Zhibin and Guoquan is shown in Equation 11, which is ª Pe 2º
1 «¬  4De [ De »¼
also a solution to Equation 4. In this new equation, it is Kdpi 1 S ³0 [e d[ (12)
assumed that the concentration of particles is smaller at De1.5

100

90

80

Kdpi (%) 70

60

50

40

30 (a)
20
Experimental
10 Deutsch (Eq. 1)
Zhibin-Guoquan (Eq. 7)
0
0.1 1 10
dp (Pm)
100

90

80
Kdpi (%)
70

60

50

40

30
(b)
20
Experimental
10 Deutsch (Eq. 1)
Zhibin-Guoquan (Eq. 7)
0
0.1 1 10
dp (Pm)
Figure 6: Comparison between theoretical models and experimental data for collection efficiency
2s = 0.20; s/2c = 1 (a) vo = 1.5 m/s and E = 5 kV/cm; (b) vo = 1.0 m/s and E = 3 kV/cm.
Brazilian Journal of Chemical Engineering Vol. 21, No. 02, pp. 275 - 284, April - June 2004
282 S. W. Nóbrega, M. C. R. Falaguasta and J. R. Coury

0.6
rd
after the 3 electrode
th
0.5 after the 4 electrode
th
after the 5 electrode
th
after the 6 electrode
0.4

0.3

JN/JN,0 0.2

0.1

0.0
0 20 40 60 80 100
y (mm)

Figure 7: Profile of particle flow in consecutive crossections of the precipitator for V = -45 kV,
vo = 1.0 m/s, dp = 1.0 Pm, 2s = 0.2 m, from Schmid and Umhauer (1998)

The value to be attributed to the diffusion (1988), is in agreement with the tendencies observed.
coefficient, Dp, was a matter of concern. No reliable
theoretical correlation is currently available and the 2x107
Dp (m2/s) (13)
one used by Zhibin and Guoquan (1994), in which dp
Dp was independent of particle size, did not seem
reasonable. For simplicity, Dp was assumed to be for dp in meters.
inversely proportional to particle size, and the A comparison between experimental results and
proportionality constant was obtain from the experiment. the new correlation (Equation 12) in presented in
The resulting expression is shown in Equation 13. The Figures 8, 9 and 10. It can be observed that the
values obtained for the range of particle diameters model represents the experimental behavior well,
between 0.1 and 10 Pm varied between 0.01 and 3 responding satisfactorily to the changes in the
m2/s, which according to Cooperman apud Licht operational conditions and precipitator shape.

100

95

90

Kdp (%) 85
i

80

75

70

65

60
2s = 0.10 m: eq 12 experim.
55 2s = 0.15 m: eq 12 experim.
2s = 0.20 m: eq 12 experim.
50
0.1 1 10
dp (Pm)

Figure 8: Comparison between theoretical prediction (Equation 12) and experimental


data for grade collection efficiency. E = 4 kV/cm, vo = 1.5 m/s and s/2c = 1.0.

Brazilian Journal of Chemical Engineering


A Study of a Wire-Plate Electrostatic Precipitator 283

100

95

90

Kdpi (%) 85

80

75

70

65

60 vo = 0.5 m/s: eq 12 experim.


vo = 1.0 m/s: eq 12 experim.
55
vo = 1.5 m/s: eq 12 experim.
50
0.1 1 10
dp (Pm)

Figure 9: Comparison between theoretical prediction (Equation 12) and experimental


data for grade collection efficiency. E = 5 kV/cm, 2s = 0.2 m and s/2c = 1.0.

100

90

80
Kdpi (%)
70

60

50

40

30
Ep = 3 kV/cm: eq 12 experim.
20 Ep = 4 kV/cm: eq 12 experim.
Ep = 5 kV/cm: eq 12 experim.
10
0.1 1 10
dp (Pm)

Figure 10: Comparison between theoretical prediction (Equation 12) and experimental
data for grade collection efficiency. vo=1.5 m/s, 2s = 0.2 m and s/2c = 1.0.

CONCLUSIONS NOMENCLATURE

The experimental evidence presented here in has A Total collecting area, m2


shown that an increase in duct width (2s) resulted in 2c Distance between two discharge electrodes, m
an increase in collection efficiency, but also in a ce Mass concentration of particles at the
larger consumption of energy. entrance, kg/m3
The models of Deutsch and Zhibin and Guoquan
cs Mass concentration of particles at the exit,
(1994) did not predict precipitator efficiency in the
submicron particle size range. A new correlation kg/m3
(Equation 12), which represented the experimental Cu Cunningham slip correction factor,
behavior very well for different operational dimensionless
conditions, is proposed. De Deutsch number, dimensionless

Brazilian Journal of Chemical Engineering Vol. 21, No. 02, pp. 275 - 284, April - June 2004
284 S. W. Nóbrega, M. C. R. Falaguasta and J. R. Coury

dp Particle diameter, m Marcel Dekker, New York (1988).


Dp Particle diffusivity, m2/s Navarrete, B. and Cañadas, L., Cortés, V., Salvador,
E Electric field, V/m L., Galindo, J., Influence of Plate Spacing and
Ash Resistivity on the Efficiency of Electrostatic
LNE Length of the collecting plate, m
Precipitators, Journal of Electrostatics, vol. 39,
Pe Pèclet number, dimensionless pp. 65-81 (1997).
Q Gas volumetric flow rate, m3/s Oglesby, S. and Nichols, G.B., Electrostatic
Qpf Particle saturation charge, C Precipitation, Pollution Engineering and
s Distance between the discharge and Technology, Marcel Dekker, New York, NY
collecting electrodes, m (1978).
2s Duct width, m Parker, K.R., Applied Electrostatic Precipitation,
Blackie Academic & Professional, New York,
vo Gas velocity, m/s
NY (1997).
wth Migration velocity, m/s Petersen, H.H., New Trends in Electrostatic
'dpiE Fraction of particles with diameter dpi at the Precipitation: Wide Duct Spacing, Precharging,
entrance of the system, % Pulse Energization, IEEE Transactions on
'dpiS Fraction of particles with diameter dpi at the Industry Applications, vol. IA–17, no. 5, pp. 496-
exit of the system, % 501 (1981).
Riehle, C., Basic and Theoretical Operation of ESPs.
Ho Permittivity of the vacuum, 8.86 ˜10 12 x 10-12
In: Parker, K.R., ed., Applied Electrostatic
As/Vm Precipitation, Chap.3, pp. 25–88, Blackie
Hr Dielectric constant of the particles, Academic & Professional, New York, NY (1997).
dimensionless Riehle, C. and Löffler, F., Electrical Similarity
Kdpi Grade efficiency, % Concerning Particle Transport in Electrostatic
O Mean free path of the ions, m Precipitators, Journal of Electrostatics, vol. 29,
pp. 147-165 (1992a).
P Gas viscosity, Ns/m2 Riehle, C. and Löffler, F., The Effective Migration
Rate in Electrostatic Precipitators, Aerosol
Science and Technology, vol. 16, pp. 1-14
ACKNOWLEDGEMENTS (1992b).
Riehle, C. and Löffler, F., Reflections on Similarity
The authors would like to thank CAPES and Laws Concerning Particle Transport in Electrical
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this work possible. 201-208 (1993).
Schmid, H.J. and Umhauer, H., In-situ Measurement
of Local Particle Fluxes in a Laboratory-scaled
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Brazilian Journal of Chemical Engineering

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