Professional Documents
Culture Documents
3 Tie Liu
4 Department of Physics and Jiujiang Research Institute,
5 Xiamen University,
6 Xiamen 361005, China
7
d
8 Zhimin Yang *
ite
9 Department of Physics and Jiujiang Research Institute,
10 Xiamen University,
11
ed
Xiamen 361005, China
12 E-mail: zhiminyoung@hotmail.com
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13
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15 by using a thermoelectric generator, a new model of a combined system is established, where the
16 ot
thermoelectric generator is attached on the backside of the thermophotovoltaic converter to harvest the
17
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heat produced in the thermophotovoltaic converter. The effects of the voltage output of the
18 thermophotovoltaic converter, band gap energy of the thermophotovoltaic converter, dimensionless current
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19 of the thermoelectric generator, and emitter temperature on the performance of the combined system are
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20 examined numerically. It is found that the performance of the thermophotovoltaic converter can be
21 enhanced by using the thermoelectric generator. The percentage increment of the maximum power output
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22 density is larger than that of the maximum efficiency. There are optimally working regions of the converter
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23 voltage, dimensionless current, and band gap energy. The elevated emitter temperature results in the
24 increase of the power output density of the combined system. However, there is an optimal emitter
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25 temperature that yields the maximum efficiency of the combined system. Moreover, the thermoelectric
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26 generator is not suitable to harvest the heat produced in the thermophotovoltaic converter when the emitter
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28
*
Corresponding author.
32 1. Introduction
33 A thermophotovoltaic (TPV) converter is a new type of photovoltaic (PV) converter that directly converts
34 heat into electricity [1]. Main advantages of TPV converters are high efficiency, with no moving parts, and
35 scalability [2]. TPV converters are promising alternative to conventional thermoelectric and thermionic
36 converters due to their high efficiency (~25% in the current state of the art devices [2, 3]). Generally, TPV
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37 converters consist of two main components: an emitter that converts the heat supplied by outer heat
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38 sources into spectrally selective thermal emission and a PV cell that produces the electrical power [4].
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39 Various heat sources, such as waste heats [5], fossil fuels [6], radioisotopes [7], and solar energy [8], are
40 available.
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41 The performance of the TPV converter is governed by many parameters, including the materials of
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42 the emitter and the PV cell and the geometry structure of the TPV converter. Wang et al. [9] reported that
43 the internal quantum efficiency of GaInAsSb/GaSb is ~90% at 1.6 µm under a lower temperature of 525ºC.
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44 Nam et al. [10] analyzed the solar thermophotovoltaic system with 2D tantalum photonic crystals (Ta PhCs)
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45 absorbers and emitters, and the absorber-to-electrical solar thermophotovoltaic efficiency is as high
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46 as~10%. Bernardi et al. [11] analyzed the performances of a nano-gap thermophotovoltaic converter in
47
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which several losses including the radiative, electrical, and thermal losses are considered.
48 However, the emitter should be operated at a high temperature to obtain the high power output density
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49 [12]. This may increase the PV cell temperature and degrade the efficiency significantly [13]. Therefore, it
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50 is important to reduce the temperature of PV cell in the TPV. If the heat released from the PV cell can be
51 exploited to generate additional electricity, the efficiency of energy conversion can be enhanced.
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52 Thermoelectric generators (TEGs) are widely used to harvest the waste heat [14-18]. Combining the PV
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53 cell and the TEG together as a combined system is a common approach to harvest the heat produced in the
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54 PV cell. Many hybrid systems consisting of the PV cell and the TEG have been reported. For example,
55
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Sark [19] theoretically predicted the efficiency enhancement of 8-23% for the PV-TEG combined system.
56 Dallan et al. [20] reported that the power output of the PV cell can be increased up to 39% by using the
57 TEG. However, Lin et al. [21] found that the efficiency of the PV cell alone is generally higher than that of
58 the PV-TEG combined system. Based on the above studies, the TPV-TEG combined system should be
59 assessed because the conversion efficiency of the TPV may be improved by using the TEG. Qiu et al. [22]
60 designed a prototype cascading GaSb TPV and TEG and found that the TEG can be used to improve the
61 efficiency of the TPV-TEG system. Besides, researches on TPV-TEG combined systems are rarely reported
62 [23]. Therefore, it is of great significance to assess and optimize the performance of the TPV-TEG system.
63 In this study, a combined system composed of the TPV and the TEG is proposed. The performance of
64 the combined system is numerically assessed and optimized. The effects of the converter voltage, band gap
65 energy of the TPV, dimensionless current, and emitter temperature on the performance of the TPV-TEG
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66
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combined system are discussed.
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67 2. Model description
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68 The schematic diagram of the TPV-TEG combined system is depicted in Fig. 1, in which the TPV is
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69 mainly composed of the emitter and the PV cell with a back surface reflector. The emitter converts the
70 supplied heat into thermal radiation impinging on the PV cell. The electric energy and thermal energy are
71
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generated from the PV cell. The thermal energy is rejected to the environment. The TEG is placed at the
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72 back side of the PV cell to collect the heat rejected from the PV cell. Assuming that the system is insulated
73 from two sides, one-dimensional heat transfer is considered. In Fig. 1, qn is the net heat flow from the
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74 emitter to the PV cell, q1 is the heat flow from the PV cell to the hot side of the TEG, q2 is the heat flow
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75 from the cold side of the TEG to the ambient, Te , Tc , T1 , T2 , and T0 are the temperatures of the
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76 emitter, PV cell, hot and cold side of the TEG, and environment, respectively. It should be pointed out that
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77 there exist thermal contact resistances between the TPV and the TEG, which are dependent on the filled
78 material. These thermal contact resistances will alter the performance of the combined system. The higher
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79 the thermal conductivity of the filled material is, the smaller the thermal contact resistance and the better
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80 the performance of the combined system. In the design of the TPV-TEG combined system, the materials
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81 with high thermal conductivities are adopted as far as possible to fill the interface between the TPV and the
82 TEG so that the effects of these thermal contact resistances are assumed to be negligible [24, 25].
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83
84 The energy flow of the TPV converter is shown in Fig. 1. The thermal emission from the emitter
85 impinges on the surface of the PV cell. The PV cell absorbs the incident photons with energy higher than
86 the band gap energy to generate electron-hole pair. The radiative recombination of electron-hole pairs
87 comes from spontaneous emission of the PV cell. The non-absorbed photons are reflected by the back
88 surface reflector and re-absorbed by the emitter. It is assumed that the areas of the emitter and the PV cell
∞ E3 ∞ E3
2p
∫0 exp [ E / ( K BTe ) ] − 1
dE − Fec ∫
Eg exp
( E − eVc ) / ( K BTc ) − 1
dE
90 qn = 3 2 Ae , (1)
hc A g Fec2 Eg E3
− e
Ac 1 − g Fcc ∫
0 exp [ E / ( K BTe ) ] − 1
dE
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91 and the current density generated in the TPV converter can be expressed as
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Ae ∞ E2 ∞ E2
Fec ∫ dE − (1 − Fcc ) ∫ dE
[ B e ] ( E − eVc ) / ( K BTc ) − 1
ed
Eg exp E / ( K T ) − 1
2p e Ac
Eg exp
92 ic = 3 2 , (2)
hc ∞ E2
−n (1 − g ) ∫
2
dE
py
Eg exp
( E − eVc ) / ( K BTc ) − 1
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93 where Ac and Ae are the areas of the PV cell and emitter, Eg is the band gap energy of the PV cell, e
94 is the elementary charge, c is the speed of light, h is the Planck constant, K B is the Boltzmann
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95 constant, Fec is the emitter-cell view factor, Fcc is the cell-cell view factor, Vc is the voltage output, n
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96 is the refractive index of the PV cell, and g is the reflectivity. The power output of the TPV converter can
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97 be obtained as
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Ae ∞ E2 ∞ E2
Fec ∫ dE − (1 − Fcc ) ∫ dE
98 2p e Ac [ B e ]
Eg exp E / ( K T ) − 1 Eg exp
( E − eVc ) / ( K BTc ) − 1
Pc = Vc ic Ac = Vc 3 2 Ac . (3)
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hc ∞ E2
−n (1 − g ) ∫
2
dE
Eg exp
( E − eVc ) / ( K BTc ) − 1
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99 The thermoelectric generator consists of large numbers of n-and p-type semiconductor legs connected
100
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electrically in series and thermally in parallel, as shown in Fig. 1. The heat flows through the hot and cold
101 sides of the TEG can be expressed as [27]
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103 and
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107 conductance, N is the couple number of the thermoelectric elements, α p and α n are the Seebeck
108 coefficients of the p- and n-type semiconductors, κ p and κ n are the thermal conductivities of the p- and
109 n-type semiconductors, rp and rn are the electrical resistivities of the p- and n-type semiconductors, and
110 An and ln are the cross-sectional area and length of thermoelectric elements. R and K can be
111 expressed as (
R = N rp + (r r κ ) κ )l Ap and (
K = N κp + (κ κ r ) )
rp Ap l p when the
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p n n p p p n n
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112 geometric configuration of the thermoelectric device is optimal and ln An = ( l p Ap ) κ n rp (κ r ) [28].
p n
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113 The material properties of n-and p-type semiconductors are dependent on the temperature and are given by
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114 [29-31]
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α = α p − (−α n ) = ( 44448 + 1861.2Tm − 1.981Tm2 ) × 10−9 V/K
115 rp = rn = ( 5112 + 163.4Tm + 0.6279Tm2 ) × 10−10 W m , (6)
κ p = κ n = ( 62605 − 277.7Tm + 0.4131Tm2 ) × 10−4 W/ ( m K )
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116 where Tm = (T1 + T2 ) 2 .
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117 In addition, the heat q1 absorbed from the TPV converter to the hot side of the TEG and the heat q2
118 released from the cold side of the TEG to the environment are assumed to be irreversible, which can be
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121 and
123 where k1 and A1 are the heat transfer coefficient and area between the PV cell and the hot side of the
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124 TEG, and k2 and A2 are the heat transfer coefficient and area between the cold side of the TEG and the
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125 environment.
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126 Based on Eqs. (4) and (5), the power output of the TEG is given by
128 where ig = α I g K is the dimensionless current and Z = α 2 KR is the figure of merit. Moreover, the
129 TEG should be operated in the region of 0 < ig < (T1 − T2 ) Z to ensure the TEG operation normally.
130 Based on the energy conservation law and Fig. 1, the energy balance equations of the hot and cold
131 sides of the TEG as well as the PV cell are
134 and
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−1
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135 ln κ pκ n rn
qn* − Pc* − k L (1 − a ) (Tc − T0 ) = a l p + κp + ig T1 − ig 2 2Z + (T1 − T2 ) , (12)
(κ κ ) κ κ
n p p n
rp
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136 where a = At Ae , k L is the heat leakage coefficient, and At = N ( An + Ap ) is the total area of the TEG.
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137 Finally, the power output and efficiency of the combined system can be calculated by
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−1
138 ln κ pκ n rn
P = Pg + Pc = At l p + κp + (T1 − T2 ) ig − ig2 Z + Vc ic Ac (13)
(κ r ) κ
n p p rn
rp ot
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139 and
−1
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ln κ pκ n rn
140 a lp + κp + (T1 − T2 ) ig − ig2 Z + Vc ic
Pg + Pc (κ r ) κ
n p p rn
rp , (14)
η=
sc
=
qn qn*
nu
142
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144 In the following discussion, the numerical study is implemented to evaluate and optimize the performance
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145 of the TPV-TEG combined system based on the parameters listed as follows [33]: Fec = 1 , Fcc = 0 , n = 3.5 ,
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147 T0 = 300 K . The values of these parameters are kept constant unless mentioned specially.
148 By combining Eqs. (10)-(12), Tc , T1 , and T2 can be solved so that η and P can be obtained.
149 Figure 2 shows three-dimensional graphs of the (a) efficiency η , (b) power output density P* = P / Ac ,
150 temperatures of the (c) PV cell as well as the (d) hot and (e) cold sides of the TEG varying with the
151 converter voltage Vc and the dimensionless current ig . As seen in Fig. 2(a) and (b), there are optimal Vc
152 and ig that yield the maximum η and P* , respectively. For the TPV, both the power output density and
153 efficiency initially increase and then reach, respectively, the maximum values with the increase of the
154 converter voltage, because the decrease of the current density due to the increase of the radiative
155 recombination is less than the increase of the converter voltage. The radiative recombination becomes
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156 significant when the converter voltage is further increased, leading to the evident decrease of the current
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157 density. Therefore, the power output density and efficiency of the TPV are decreased at a high converter
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158 voltage. For the TEG, the power generated due to the heat conductance is larger than the Joule heat at a low
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159 ig . When the TEG is operated at the case of a high ig , the Joule heat becomes significant. Thus, the power
160 output density of the TEG is decreased at a high ig . As a result, the maximum η and P* occur. Figs. 2(c)
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161 and (d) display the same trend. The Tc and T1 initially decrease and then increase with the increase of
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162 Vc for a fixed ig , while they decrease linearly as ig increases for a given Vc . In Fig. 2(e), T2 first
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163 decreases and then increases as ig and Vc increase. These trends can be explained as follows: the increase
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164 of Vc leads to an increase in the power output density of the TPV, causing the decrease of the heat
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165 released from the TPV. The power output density of the TPV reduces with the further increase of Vc after
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166 reaching a maximum value, which results in the increase of the heat released from the TPV. As a result, Tc ,
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167 T1 , and T2 first decrease and then increase with the increase of Vc for a fixed ig . When Vc is fixed,
168 the Joule heat is increased with the increase of ig . According to Eqs. (10) and (11), the heat absorbed q1
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169 from the TPV is reduced, while the heat released q2 from the cold side of the TEG is increased. When ig
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170 is small, the heat conductance is dominant. Therefore, Tc and T1 are decreased significantly, while T2
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171 decreases slightly. When ig is large, q1 decreases, while q2 increases due to the significant increase of
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172 the Joule heat. Thus, Tc and T1 decrease, while T2 increases slightly. Therefore, ig and Vc should
174
175 Based on Fig. 2, ig can be optimized for each Vc and then η and P* versus the converter
176 voltage can be plotted in Fig. 3(a). Similarly, η and P* versus ig are shown in Fig. 3 (b), where Vc
177 has been optimized. Fig. 3 shows that there are optimal converter voltages and dimensionless currents
178 corresponding to the maximum η and P* , while the optimal values at the maximum η and P* are
179 different because the net heat flow qn is a function of the converter voltage and the temperatures of the
180 emitter and PV cell. Therefore, there are optimally working regions of the converter voltage and
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181 dimensionless current for given parameters ( Eg , Te , and a ) , which can be expressed as
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182 Vc ,η ≥ Vc ≥ Vc , p (15)
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183 and
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184 ig , p ≥ ig ≥ ig ,η . (16)
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185 Moreover, it can be seen from Fig.3 that the optimally working regions of the converter voltage and the
186 dimensionless current are relatively narrow.
187
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188 In order to compare the performances of the TPV converter and the TPV-TEG combined system, the
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189 efficiencies and power output densities of the TPV converter and the TPV-TEG combined system versus
190 the band gap energy Eg are shown in Fig. 4, where Vc and ig have been optimized. Fig. 4 shows that
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191 the maximum power output density of the combined system is 3.30 W m -2 , which is 1.04 times larger
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192 than that (3.18 W m-2) of the TPV converter. The maximum efficiency of the combined system is 37.3%,
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193 which is 1.02 times of the maximum efficiency (36.7%) of the TPV converter. Fig. 4 indicates that the
194 performance of the combined system can be enhanced by using the TEG.
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195 Moreover, it is observed from Fig. 4 that there is an optimally working region of the band gap energy
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198 Equation (17) shows that the band gap energy of the optimally working region is relatively broad. Many
199 suitable semiconductor materials, such as InAs (0.35eV), PbS (0.37eV), and GaInAs (0.477eV), can be
200 selected.
201
202
203 In order to further examine the effect of the emitter temperature on the performance of the combined
204 system, the maximum efficiency and the power output density of the combined system and the TPV under
205 different emitter temperatures are calculated and listed in Tab.1 for a = 0.8 , where Eg , Vc , and ig have
206 been optimized. As seen in Tab. 1, the maximum power output density monotonously increases when the
207 emitter temperature ranges from 1100 K to 1900K, while there is a maximum efficiency occurring at
Te = 1500 K . In addition, the percentage increment [(ηmax − ηmax,c ) ηmax,c ] × 100% of the maximum
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208
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209 efficiency of the combined system with respect to the TPV is, respectively, 1.63% and 2.98% at
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210 Te = 1300 K and Te = 1700 K . The percentage increment [( Pmax
*
− Pmax,
*
c ) Pmax,c ] × 100% of the maximum
*
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211 power output density of the combined system with respect to the TPV is, respectively, 3.77% and 4.42% at
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212 Te = 1300 K and Te = 1700 K . The optimally working region of the band gap energy is broadened as the
213 emitter temperature increases. Moreover, there is an optimally working region of the emitter temperature,
214
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but the PV cell temperature is as high as 500 K at Te = 1500 K . According to Eq. (9), the properties of the
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215 thermoelectric materials depend on their temperatures and the optimal temperature of the thermoelectric
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216 materials is around 470 K. Thus, the TPV-TEG combined system should be operated in the region of
218
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219 4. Conclusions
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220 The combined system consisting of the TPV and the TEG has been established and its performances are
221 assessed numerically. There are optimally working regions of the converter voltage, dimensionless current,
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222 and band gap energy in the combined system. The optimally working regions of the converter voltage and
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223 dimensionless current are narrow. The percentage increment of the maximum power output density is
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224 larger than that of the maximum efficiency. The percentage increments of the maximum power output
225
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density and efficiency of the combined system with respect to the TPV are 3.77% and 1.63% at
226 Te = 1300 K . When the emitter temperature is increased, the extreme value of the maximum efficiency
227 occurs at Te = 1500 K and the maximum power output density monotonously increases. The percentage
228 increments of the maximum power output density and efficiency of the combined system with respect to
229 the TPV are 4.42% and 2.98% at Te = 1700 K . Moreover, the elevated emitter temperature leads to the
d
e =elementary charge (C)
ite
Eg =band gap energy of the PV cell (eV)
Fcc =cell-cell view factor
Fec =emitter-cell view factor
ed
h =Planck constant (J s)
ic =current density of the PV cell (A/m2)
ig
py
=dimensionless current of the TEG
Ig =electric current of the TEG (A)
k1 =heat transfer coefficient between the PV cell and the hot side of the TEG (W/(K m2))
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k2 =heat transfer coefficient between the cold side of the TEG and the environment (W/(K
m2))
k L = heat leakage coefficient (W/(K m2))
K = thermal conductance (W/K) ot
K B = Boltzmann constant (J/K)
l = length of thermoelectric element (m)
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n = refractive index of the PV cell
N = couple number of the thermoelectric elements
P = output power (W)
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r = electrical resistivity ( Ωm )
R = electrical resistance ( Ω )
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η = efficiency
κ = thermal conductivities (W/(m K))
g = reflectivity
ce
Subscripts
c = TPV converter
Ac
e = emitter
g = thermoelectric generator
n = n-type semiconductor
p = p-type semiconductor
Acronyms
TPV = thermophotovoltaic
TEG = thermoelectric generator
232
10
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307 [30] Ahiska, R., and Ahiska, K., 2010, “New method for investigation of parameters of real thermoelectric
nu
310 Circular Thermoelectric Skutterudite Couple Using Compression Technology,” ASME J. Energy Resour.
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314 [33] Datas, A., and Algora, C., 2013, “Global optimization of solar thermophotovoltaic systems,” Prog.
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318
319
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322 Fig. 2. Three-dimensional graphs of the (a) efficiency η , (b) power output density P* , and temperatures
323 of the (c) PV cell as well as the (d) hot- and (e) cold-sides of the TEG varying with the converter voltage
Fig. 3. The efficiency η and the power output density P* versus (a) the converter voltage and (b) the
d
325
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326 dimensionless current for a = 0.8 , Te = 1300 K , and Eg = 0.40 eV , where ig and Vc have been
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327 optimized, respectively.
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328 Fig. 4. The efficiency and the power output density versus the band gap energy Eg for a = 0.8 and
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329 Te = 1300 K , where Vc and ig have been optimized, Eg , p is the optimal band gap energy at the
330 *
maximum power output density Pmax of the combined system, and Eg ,η is the optimal band gap energy
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331 at the maximum efficiency ηmax of the combined system.
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332
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337
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338 Fig. 1
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340
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341 Fig. 2a
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342
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344
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345 Fig. 2b
346
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348
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349 Fig.2c
350
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351
352
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353 Fig. 2d
354
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356
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357 Fig.2e
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359
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360 Fig.3a
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364 Fig. 3b
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366
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367 Fig. 4
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369 Table 1
Te ( K ) ηmax ηmax,c Eg ,η Tc ,η *
Pmax *
Pmax,c Eg , p Tc , p
(eV) (eV)
(K ) (W m -2 ) (W m -2 ) (K )
d
1500 0.382 0.373 0.588 403 5.64 5.39 0.358 500
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1700 0.380 0.369 0.700 455 8.51 8.15 0.448 588
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1900 0.370 0.357 0.814 523 11.7 11.3 0.560 680
370
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