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(2015) Modeling Cavitation in A Rapidly Changing Pressure Field - Application To
(2015) Modeling Cavitation in A Rapidly Changing Pressure Field - Application To
Ultrasonics Sonochemistry
journal homepage: www.elsevier.com/locate/ultson
a r t i c l e i n f o a b s t r a c t
Article history: Ultrasonic horn transducers are frequently used in applications of acoustic cavitation in liquids. It has
Received 14 October 2013 been observed that if the horn tip is sufficiently small and driven at high amplitude, cavitation is very
Received in revised form 8 May 2014 strong, and the tip can be covered entirely by the gas/vapor phase for longer time intervals. A peculiar
Accepted 16 May 2014
dynamics of the attached cavity can emerge with expansion and collapse at a self-generated frequency
Available online 22 May 2014
in the subharmonic range, i.e. below the acoustic driving frequency. The term ‘‘acoustic supercavitation’’
was proposed for this type of cavitation Žnidarčič et al. (2014) [1].
Keywords:
We tested several established hydrodynamic cavitation models on this problem, but none of them was
Cavitation
Ultrasonic horn
able to correctly predict the flow features. As a specific characteristic of such acoustic cavitation problems
Rayleigh–Plesset equation lies in the rapidly changing driving pressures, we present an improved approach to cavitation modeling,
CFD which does not neglect the second derivatives in the Rayleigh–Plesset equation. Comparison with mea-
Acoustic supercavitation surements of acoustic supercavitation at an ultrasonic horn of 20 kHz frequency revealed a good agree-
ment in terms of cavity dynamics, cavity volume and emitted pressure pulsations.
The newly developed cavitation model is particularly suited for simulation of cavitating flow in highly
fluctuating driving pressure fields.
Ó 2014 Elsevier B.V. All rights reserved.
1. Introduction engineering applications. Most of the codes treat the two phase
flow as a single vapor–liquid phase mixture flow. An exception is
Cavitation occurs in very different situations and is denoted as for example a numerical study of cavitating flow in the nozzle per-
the process of a breakdown of a homogeneous liquid medium formed by Alajbegovic et al. [3], where each phase was separately
under very low pressures and a consequent collapse of vapor bub- modeled.
bles when the pressure is elevated. In liquid flows, this phase In the simplest approach it is assumed that the flow is seeded
change is generally due to local high velocities which induce low by cavitation nuclei. Usually a simplified Rayleigh–Plesset equa-
pressures. The liquid medium is then ‘‘broken’’ at one or several tion is used to determine the change in bubble size and conse-
points and ‘‘voids’’ appear, whose shape depends strongly on the quently the mixture density in each computational cell. The
structure of the flow. However, cavitation can also occur in a static advantage of this formulation is that it follows, to some part, a
or nearly static liquid. When an oscillating pressure field is applied physical law. However one neglects the hydrodynamics of the
over the free surface of a liquid contained in a reservoir, cavitation vapor phase and overpredicts the vapor volume fraction – espe-
bubbles may appear within the liquid bulk if the oscillation ampli- cially in cases of cloud cavitation. This approach was first intro-
tude is large enough. This type of cavitation is known as acoustic duced by Kubota et al. [4] who used the linear part in the
cavitation [2]. Rayleigh–Plesset equation to describe the evolution of bubble
Numerical simulation of cavitating flows and specifically the radius as a function of the surrounding pressure.
development of phase change models has received enormous A different approach was proposed by several authors [5–13] in
attention from researchers during the last years. Early studies, that form of essentially the same transport equation models. In their
primarily utilized the potential flow theory, are still widely used in approach volume or mass fraction of liquid (and vapor) phase is
convected. This method has the advantage that it can take into
account the time influence on the mass transfer phenomena
⇑ Corresponding author. Tel.: +386 31203044.
through empirical laws for the source term. One clear advantage
E-mail address: matevz.dular@fs.uni-lj.si (M. Dular).
http://dx.doi.org/10.1016/j.ultsonch.2014.05.011
1350-4177/Ó 2014 Elsevier B.V. All rights reserved.
A. Žnidarčič et al. / Ultrasonics Sonochemistry 22 (2015) 482–492 483
of models from this family comes from the convective character of cloud or streamer is not appropriate. Likewise, hydrodynamic
the equation that allows modeling of the impact of inertial forces models can fail to accurately reproduce acoustically driven cavita-
on cavities like elongation, detachment and drift of bubbles. tion due to the high frequency of the pressure fields. In the follow-
Another way to model cavitation processes is by the so called ing we focus on a peculiar case which appears somehow
barotropic state law that links the density of vapor–liquid mixture intermediate between hydrodynamic and acoustic cavitation,
to the local static pressure. The model was proposed by Delannoy & namely a large cavity attached to an ultrasonic horn tip and col-
Kueny [14] and later widely used by others [15–18]. The results lapsing with its self-generated subharmonic cycle frequency
obtained with the barotropic cavitation model show very good cor- (‘‘acoustic supercavitation’’). Here we report that several standard
relation to the experiments but past simulations lacked robustness hydrodynamic codes were not able to reproduce the experimental
of numerical algorithms, which resulted in numerical instability observations, but that a suitable extension of the vapor source
and sometimes in poor convergence. term removes the deficiencies and leads to a convincing simulation
All of the mentioned models were developed and compared result by the new code.
with experiments on hydrodynamic cavitation, where very rapid
driving pressure changes are unlikely to occur. This is quite differ-
ent in acoustic cavitation, where bubble growth and collapse are 2. Problem statement and conventional simulation
driven by ultrasound (>20 kHz) and the driving pressure switches
from positive to negative values periodically in a matter of micro- Ultrasonic horn transducers are frequently used in applications
seconds. Additionally to the faster excitation pressure time scales, like ultrasonic homogenization, sonochemical reactions, milling,
other essential differences occur for acoustically driven as com- emulsification, spraying and cell disruption (the applications of
pared to hydrodynamically driven cavitation: bubbles can show acoustic cavitation go even further – for example water purifica-
longer life time in terms of collapse cycles (up to hundreds), and tion, surface cleaning and lithotripsy). They are operated typically
they are re-circulated. Both leads, together with acoustic bubble– in the frequency range up to about 50 kHz and have tip diameters
bubble interaction, to characteristic structure formation [19–21]. from some mm to several cm. It has been observed that if the horn
Furthermore, the bubble distribution acts back on the driving pres- tip is sufficiently small and driven at high amplitude, cavitation is
sure wave by acoustic impedance change of the two phase medium very strong, and the tip can be covered entirely by the gas/vapor
– a phenomenon that typically does not play a role in hydrody- phase for longer time intervals. In Fig. 1 an acoustic horn emitter
namic cavitation problems. For these reasons, the models for of small diameter (3 mm) and oscillation amplitude of 164 lm at
numerical simulation of acoustic cavitation are rather distinct from 20 kHz is shown for several representative cycles. A large single
the hydrodynamic codes mentioned above. They traditionally split cavity of a large extension occurs at the tip, while a cloud of indi-
into ‘‘continuum models’’ and ‘‘particle models’’. The former focus vidual bubbles is seen below. In this condition, the horn tip is
on the acoustic wave propagation in bubbly (cavitating) liquids working most of the time against gas and only in short intervals
and couple the gas/vapor resp. bubble density, which is given by against liquid. The large attached cavity is undergoing a character-
a continuous field variable in space and time, to the acoustic pres- istic ‘‘mushroom’’ shape oscillation with strong collapse. It is gen-
sure amplitude [19,22–26]. The latter resolve the bubble popula- erating its own oscillation frequency which is smaller than the
tion into individual bubbles (‘‘particles’’) and focus on their driving and thus falls into the subharmonic range of the excitation
dynamics, motion and re-distribution driven by the sound wave frequency f0 (for instance somewhere between f0/6 and f0/4). The
and acoustic forces [27,28]. Recently, also hybrid forms and combi- subharmonic acoustic emission generated by the large bubble
nations of the two model types have been proposed [29–31]. Nev- can be even more pronounced in an acoustic power spectrum than
ertheless, the development of simulation codes of acoustic the primary wave [33].
cavitation with sufficient predictive power is still ongoing; see It was suggested by the present authors [1] to term the
e.g. [32]. observed phenomenon of attached cavities partly covering the full
Yet, the standard acoustic cavitation model approaches prove horn tip as ‘‘acoustic supercavitation’’. This reflects the conjecture
inefficient in cases were acoustic cavitation resembles the hydro- that not the sound field in terms of acoustic (negative) pressure in
dynamic one – with large coherent gas/vapor structures. Then the bulk liquid is responsible for nucleation, but the rapid motion
the notion of ‘‘bubbly liquid’’ or individually acting bubbles in a of the transducer surface.
484 A. Žnidarčič et al. / Ultrasonics Sonochemistry 22 (2015) 482–492
Fig. 1. Two cycles of the oscillation of a large cavity at an ultrasonic horn tip of 3 mm diameter in water (acoustic frequency 20 kHz, recording at 100,000 frames/s (only every
2nd image is shown), exposure 1 ls, sequence row by row from top left). Conditions are the same as for the case A in Table 1.
Fig. 2. Simulation of cavitation on an ultrasonic horn by the original Schnerr–Sauer model [12]. The boundary conditions correspond to the sequence shown in Fig. 1.
Table 1 the Rayleigh solution (Eq. (1)). As already mentioned this is not
Source terms of some commonly used cavitation models. appropriate in the case of rapidly changing pressure fields, and hence
Authors Source terms we propose to replace it with the equation of bubble growth velocity
Kunz et al. [5] 2C prod: ql minf0;p1 pv g based on the simplified Rayleigh–Plesset equation derived in the fol-
Sprod: ¼ ql u21 t1
C q a2 ð1al Þ
lowing section.
Sdest: ¼ dest: v t1l
Merkle [6] 2C q minf0;p p ga
Sprod: ¼ prod: lq q u2 t11 v l
v l 1
2C prod: maxf0;p1 pv gð1al Þ
3.2. Simplyfing the Rayleigh–Plesset equation
Sdest: ¼ ql u21 t1
pffiffi qffiffiffiffiffiffiffiffiffiffiffiffiffiffi
Singhal et al. [9] Sprod: ¼ C prod: rk l v 23 jp1qpjð1
qq fv fg Þ
qffiffiffiffiffiffiffiffiffiffiffiffiffiffi
l
The general Rayleigh–Plesset equation can be written as [2]:
pffiffi
Sdest: ¼ C dest: rk l l 23 jp1qpjfv
qq 3c
l
qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi pv ðT 1 Þ p1 p ðT b Þ pv ðT 1 Þ pg0 R0
Frobenious et al. [10] n0
Sprod: ¼ C prod: 1þ4=3n 3 4pR
2 2 jp1 pv j
3 ql þ v þ
0 pR qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ql ql ql R
n0
Sdest: ¼ C dest: 1þ4=3n pR3 4pR 2 2 jp1 pv j
3 ql
|fflfflfflfflfflfflfflfflfflffl{zfflfflfflfflfflfflfflfflffl
ffl} |fflfflfflfflfflfflfflfflfflfflfflfflffl{zfflfflfflfflfflfflfflfflfflfflfflfflffl} |fflfflfflfflfflfflffl
ffl{zfflfflfflfflfflfflfflffl}
0
qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi 1 2 3
Zwart et al. [11] 3a ð1a Þq
Sprod: ¼ C prod: nuc R v v 23 jp1qpv j 2
2
3a a q
qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffil d R
3 dR 2r 4l dR
Sdest: ¼ C dest: nucR v v 23 jp1qpv j ¼R 2þ þ ð4Þ
qffiffiffiffiffiffiffiffiffiffiffiffiffiffi
l
2 d q lR
dtffl} |fflfflfflfflffl{zfflfflfflfflffl} |{z} ql R dt
Schnerr and Sauer [12] qq
Sprod: ¼ ql v 3að1 aÞ 2 jp1 pj |fflffl{zffl |fflfflffl{zfflfflffl}
R 3 ql 4
m
q ffiffiffiffiffiffiffiffiffiffiffiffiffiffi 5 6 7
qq
Sprod: ¼ ql v 3að1
R
aÞ 2 jp1 pj
3 q
Dauby et al. [13]
m
could be drawn for all cases. Hence, only results at 70 W power Table 2
(990 W/cm2 power density), 164 lm oscillation amplitude at Maximum size of the attached cavitation structure and cavitation oscillation
frequency for different fluid parameters.
20 kHz, are shown (comparison between experimental results at
30 and 50 W and simulations are given in Fig. 9). The main goal Case Fluid Temp. Saturation Viscosity Surf. Mean Max.
of this part of the study is to investigate the fluid parameters, which ten. freq. vol.
(°C) (%) (Pas) (N/m) (Hz) (mm3)
could influence or explain the peculiar (slow) dynamics of cavita-
tion on the small ultrasonic horn. We tested the influence of: A H2O 23 100 0.00093 0.072 5058 8.97
B H2O 23 50 0.00093 0.072 5085 8.58
C H2O + SDS 23 100 0.00093 0.05 5095 8.95
- Presence of gas in the liquid. Degassing the water could reduce D C2H6O2 23 100 0.0169 0.048 5074 8.63
or suppress bubble nucleation. E H2O 45 100 0.0006 0.069 5074 8.87
- Viscosity. It could influence the intensity of the turbulence and
consequently also cavitation inception, as the pressure can
locally drop below vapor pressure inside the eddies. Further-
more, damping of the sound wave and the bubble oscillation the maximum size of the attached cavitation and its mean oscilla-
is increased with viscosity. tion frequencies are listed according to fluid parameters.
- Surface tension. It could influence the critical amplitude of As can be deducted from Fig. 3 and Table 2, both the typical
acoustic pressure at which cavitation nuclei begin to rapidly attached cavity oscillation frequency and the maximum volume
grow into bubbles. of the cavity are almost unaffected by the fluid parameters. From
- Temperature. The increase of temperature leads to increase of the diagrams in Fig. 3 one can see that the evolution of the cavita-
vapor pressure and by this to the conditions more prone to cav- tion volume changes only slightly, with more obvious changes in
itation. There will also be indirect changes of viscosity, surface the evolutions of the pressure. This is probably related to different
tension and density due to the variation of the temperature attenuation of the signal [1].
(the experiments were conducted in a way to minimize these, One can conclude, on the basis of these experiments, that terms
indirect, effects). 2, 3, 6 and 7 in the Rayleigh–Plesset equation (Eq. (4)) can be
neglected in the new cavitation model, namely temperature,
The main results of the experimental campaign are shown in (non-condensable) gas pressure, surface tension, and viscosity.
Fig. 3, which presents the attached cavity size and pressure evolu- The only relevant additional part appears to be the second deriva-
tions in time for different fluid parameters, and in Table 2 where tive (4) representing the inertial terms.
Fig. 3. Evolution of the size of attached cavitation and pressure for different fluid parameters.
A. Žnidarčič et al. / Ultrasonics Sonochemistry 22 (2015) 482–492 487
Its relevance also becomes clear if we remember that the driv- 3.4. Model constants
ing frequency of the horn (in the present case) lies at 20 kHz. From
a numerical point of view this means that the time step has to be Like the original model [36], the present approach requires the
considerably shorter than 105 s. As a consequence the accelera- input of nuclei number density n0 and the initial nuclei size R0 –
tion (term 4) cannot be disregarded, as the bubble will still be the two values define the initial local vapor volume fraction in
accelerating its growth velocity during such a short time interval Eq.(3). According to the recommendations in [12,38,39] n0 was
(it takes 104 s or less to reach a stationary growth) [36]. set to n0 = 1012 1/m3. The size of the nuclei could be determined
With the before mentioned considerations, we obtain the sim- from close inspection of images just prior to the cavity growth
plified Rayleigh–Plesset equation, which can be used to obtain (for example the first frame in Fig. 1) – it was set to R0 = 25 lm.
the source term of the new model: Predictions of simulations proved immune against reasonable var-
2 iation of the n0 and R0 values.
2
pv ðT 1 Þ p1 d R 3 dR
¼R þ ð5Þ
ql dt
2 2 dt
4. Numerical simulation
where q is the fluid density, ~ u is the flow velocity vector, ~ug is the
grid velocity of the moving mesh, C is the diffusion coefficient
and S/ is the source term of / A is used to represent the boundary
of the control volume V.
The equations were combined with the newly developed cavita-
tion model, described in the previous section. In addition, also
equations of state, which describe the relation between the pres-
sure and the liquid and vapor densities and the relations for the
volume fraction and the mixture (liquid–vapor) density and viscos-
ity, had to be introduced.
The flow in the vicinity of the horn is clearly turbulent (the Rey-
nolds number based on the horn diameter and maximal flow veloc-
ity lies in the range of 15,000), hence a k–e realizable model [43]
was used, as it offers better accuracy in areas, which are specific
for the flow around an ultrasonic horn (development of cylindrical
jets, boundary layers under the influence of adverse pressure gra-
dient, flow detachment and recirculation). The boundary layer
influence on flow development was considered with the use of
enhanced wall functions [44].
Fig. 5. Sequence showing a simulation of cavitation on an ultrasonic horn with the new cavitation model for 164 lm horn oscillation amplitude at a frequency of 20 kHz (test
A from Table 2).
A. Žnidarčič et al. / Ultrasonics Sonochemistry 22 (2015) 482–492 489
size remains almost constant for another 50 ls. The main cavity
collapse occurs roughly 180 ls after the start of the cycle. A brief
rebound follows, where a toroidally shaped cloud forms for about
20 ls (probably due to a strong toroidal vortex beneath the tip).
During each cavitation period (about 200 ls or 5 kHz) the tip of
the horn advances and retracts about 4 times (at 20 kHz). The same
periodicity and the dynamics could also be observed during the
experiments.
A comparison between the measured and predicted cavity vol-
ume is given in Fig. 6.
It is evident that the simulation accurately predicts the dynam-
ics of the cavity volume. Some discrepancies do exist though – pos-
Fig. 6. Comparison between the predicted and measured attached cavity volumes sibly due to the inability of the simulation to capture the single
for 164 lm horn oscillation amplitude at a frequency of 20 kHz (case A from small bubble jetting (seen in Fig. 1) when the cavity is the largest
Table 2).
(the volume of the single bubbles are considered in experiment
but not in simulation). One can also observe a rebound of the cavity
just before the end of the second period in Fig. 6.
The small oscillations superimposed to the main volume oscil-
lations, well visible during the time when the size of the cavity is
close to its maximum, can be attributed to the movement of the
tip of the horn, as their period of 50 ls corresponds to the
20 kHz driving frequency. Their amplitude of approximately
1 mm3 is roughly equal to the moving volume of the horn
(V ¼ h pr 2 ¼ 164 lm p ð1:5 mmÞ2 ¼ 1:15 mm3 ). In the experi-
mental curve this moving volume does not appear as it could not
be resolved from the images.
The measured and predicted pressure evolutions at the position
indicated below and during the same time frame are shown in
Fig. 7.
At every cavity collapse a pressure wave is emitted and
Fig. 7. Comparison between the predicted and measured pressure for 164 lm horn recorded by a hydrophone (or a monitor in the simulation) posi-
oscillation amplitude at a frequency of 20 kHz (case A from Table 2).
tioned at a distance of 7 mm from the tip of the horn. It reaches
a peak amplitude of about 4 bar, and peak negative amplitude of
ultrasonic horn powers 30 and 50 W) are given more briefly in 1 bar. It is evident that the frequency of the pressure peaks is cor-
Fig. 9. rectly predicted. The peak pressure amplitude seems to be slightly
Fig. 5 shows the prediction of the cavitation structure beneath overpredicted. This could be a result of the choice of the water
the tip of the horn. The instants shown correspond to the ones in compressibility model and the fact that in the simulation we are
Fig. 1. not considering the influence of inclusion of small single bubbles
As in the experiment (Fig. 1) the cavity firstly grows and forms a on attenuation of the pressure wave (these can be nicely seen in
characteristic ‘‘mushroom’’ shape (between 40 and 80 ls). The Fig. 1). Furthermore, contributions of non-condensable gas in the
maximum volume is achieved about 100 ls after the start of the cavity – not considered in the simulations – might damp the acous-
growth. The cavity then contracts at the outer rim, while its axial tic emissions during its collapse.
Fig. 8. Time averaged experimental (left) and predicted (right) velocity profiles in the vicinity of the tip of the horn for 164 lm horn oscillation amplitude at a frequency of
20 kHz (case A from Table 2).
490 A. Žnidarčič et al. / Ultrasonics Sonochemistry 22 (2015) 482–492
Fig. 9. Measured and predicted characteristic values of attached cavitation bubble oscillation frequency, maximal volume of the cavity and maximal recorded pressure for
cases (A)–(E) (Table 2) and at 30 W (F) and 50 W (G) power. The ‘‘original’’ model is Schnerr–Sauer from [12].
Finally also the mean measured and predicted velocity fields quency, its maximal volume and the maximal recorded pressure
were compared (Fig. 8). For the case of the measured profile a for all cases (A–E in Table 2 and additional two for the same fluid
method based on the advection diffusion equation [45,46], which properties as in test A but at a reduced power 30 W (test F) and
couples the velocity field with the field of concentrations of a pas- 50 W (test G)).
sive tracer (in the present case cavitation bubbles), was used. One When one compares the quantitative agreement between the
needs to bear in mind that the measurement gives the velocity of measurements and simulations (Fig. 9) an obvious improvement
the vapor phase while the simulation considers a velocity in a can be seen when the new cavitation model is employed. Results
mixed fluid – these can differ significantly [47]. obtained with existing models (results obtained by the original
The periodical movement of the horn creates a flow away from Schnerr–Sauer model [12] are shown for comparison in Fig. 9)
the tip (downwards) near the axis of the horn. As the flow looses poorly predict the characteristic parameters of cavitation in our
momentum it turns radially outwards, and then upwards. One case. Without the acceleration term, the existing model is unable
can observe a significant toroidal vortex which forms beneath to predict the slow cavitation dynamics – the cavity always follows
the outer rim of the tip of the horn. We believe that it is this vortex the driving frequency (20 kHz). As a consequence the attached cav-
that initiates the rebound of the cavity at the end of its period ity does not grow to its correct size (its maximal size is in average
(Fig. 5, frame at 180 ls). The velocity fields (measured (left) and 30% too small compared to the experiment) and implodes at a sig-
predicted (right)) qualitatively agree reasonably. The very clear nificantly lower aggressiveness (about 1 bar pressure wave instead
vorticity shown in the simulation is less pronounced in the exper- of 4 bar was continuously predicted).
imental results – it can be seen a bit closer to the face of the horn With the new model the values significantly improve. The char-
but somewhat further away from its center. The qualitative and acteristic cavitation frequency is very accurately predicted – the
quantitative deviations probably origin from the different veloci- average discrepancy lies at only 1%. The maximal cavitation vol-
ties of vapor (experiment) and liquid/vapor mixture (simulation). ume is predicted at somewhat worse accuracy (within 5%). Finally
In Fig. 9 we present comparisons of measured and predicted about 7% prediction accuracy was achieved for the maximal
values of characteristic attached cavitation bubble oscillation fre- recorded pressure at 7 mm distance from the tip of the horn.
A. Žnidarčič et al. / Ultrasonics Sonochemistry 22 (2015) 482–492 491
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