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Pulsedlaserdiode Intermittently Pumped 213211 Acoustooptic Qswitched TM Lu AGLaser
Pulsedlaserdiode Intermittently Pumped 213211 Acoustooptic Qswitched TM Lu AGLaser
(Received October 17, 2019 : revised January 16, 2020 : accepted April 10, 2020)
The heat distribution in crystals in a 2-µm acousto-optic Q-switched Tm:LuAG laser pumped by
pulsed-laser-diode (pulsed-LD) intermittent-pumping technology was analyzed using COMSOL software.
The thermal lensing effect of the Tm:LuAG crystal can be mitigated by pulsed-LD intermittent-pumping
techniques. An experimental setup using this kind of approach achieved maximum output energy of 8.31
mJ, minimum pulse width of 101.9 ns, and highest peak power of 81.55 kW, reached at a Q-switched
repetition rate of 200 Hz. It offers significant improvement of performance of the output laser beam,
compared to pulsed-LD double-ended pumping technology at the same repetition rate.
- 238 -
Pulsed-laser-diode Intermittently Pumped 2-µm Acousto-optic Q-switched … - Ya Wen et al. 239
Parameter Value
Laser Diode 1 and Laser Diode 2 emission
788
wavelength (nm)
Cooling temperature (℃) 15
Room temperature (℃) 22
-2 -1
Heat-transfer coefficient of air (W cm K ) 5 × 10-5
-1
Absorption coefficient of 3 at.% Tm:LuAG (cm ) 4.36
FIG. 3. The illustration of double-ended bonding Tm:LuAG
crystal model double-ended pumped by pulsed LD. Pump-beam waist (µm) 400
Crystal radius (mm) 1.5
The beam of pumping light incident upon the bonding Tm:LuAG crystal length (mm) 25
surface of the rod has a Gaussian intensity distribution Poisson ratio 0.3
Thermo-optical coefficient (dn/dT) (℃-1) 6 × 10-6
r r , a, t 2
I r , a, t I 0 exp 2 G t . (1) Refractive index of Tm:LuAG 1.81
2 -1 -1
Heat conductivity of Tm:LuAG (W cm K ) 7.94 × 10-2
Thermal-expansion coefficient (℃-1) 7.1 × 10-6
The pumping light incident upon the other bonding
surface of the rod has its own Gaussian distribution
G t square2ft , T 1 2 , (2)
r r , L a, t 2
I r , L a, t I 0 exp 2 G t , (3)
2
T1 Tw , r b 0 z L 2a , (7) T2 Tw , r b 0 z L 2a , (12)
T1 T2
k hT1 hTe z 0, (8) k hT2 hTe z 0, (13)
z z
T1 T2
k hT1 hTe z L 2a , (9) k hT2 hTe z L 2a , (14)
z z
and and
T1 T0 , t 0, 0 z L 2a , (10) T2 r , z , t t T1 r , z , . (15)
where is the crystal density, c is the specific heat In the case when the repetition frequency is 100 Hz,
capacity of the crystal, h is the heat-transfer coefficient, k pulse width is 5 ms, the pulse is pumped for 10 s, and the
is the thermal conductivity of the crystal, Tw is the water- single-ended single-pulse energy takes values of 25, 55,
cooling temperature, Te is the initial temperature of the 75, 100, 125, and 150 mJ, the center temperatures in the
crystal, and T0 is room temperature. bonding surfaces of the double-end-bonded Tm:LuAG crystal
The heat-transfer equation, boundary conditions, and initial double-end-pumped by a pulsed LD are shown in Fig. 5.
conditions of the Tm:LuAG crystal in temperature-fall period In another case where the repetition frequency is 100 Hz,
are, respectively, the pulse width is 5 ms, the pulse is pumping for 10 s, and
the single-ended single-pulse energy takes values of 25, 55, With the increase of pump energy, due to the crystal being
75, 100, 125, and 150 mJ, the center temperatures in the intermittently pumped, the crystal is heated more evenly
bonding surfaces of the double-end-bonded Tm:LuAG crystal and the crystal temperature is changed smoothly. This
intermittently pumped by a pulsed LD are shown in Fig. 6. intermittent-pumping technology can be applied to pump
It is obvious from Figs. 5 and 6 that the temperatures in with larger energy, and the greater the pump energy, the
the bonding surfaces of the double-end-bonded Tm:LuAG more significant the improvement that can be achieved. It is
crystal gradually decrease along the radius outward, and beneficial to alleviate the thermal-lens effect of the crystal,
the temperatures at the edge of the crystal are constant,
which are 15°C, the same as the water-cooling temperature.
From Fig. 5, when the double-end bonded Tm:LuAG
crystal double-end pumped by the pulsed LD has a
quasi-thermal-equilibrium state, the maximum temperature
of the crystal increases with increasing pump energy, and
its locations move from 6.7 and 13.4 mm to 6.9 and 13.1
mm respectively, with maximum temperatures 293.47 to
321.51 K. From Fig. 6, the double-end-bonded Tm:LuAG
crystal double-end-intermittently-pumped by the pulsed LD
has a quasi-thermal-equilibrium state, and the maximum
temperatures of the crystal also increase with increasing
pump energy. Its locations of maximum temperatures move
from 6.2 and 13.1 mm to 6.5 and 12.8 mm respectively,
and the highest temperatures are 288.71 to 309.41 K.
Figure 7 shows that the intermittent-pumping method can
alleviate the maximum temperatures in the crystal, and make FIG. 7. Tm:LuAG-crystal temperature versus input energy
the temperature distribution of the crystal more uniform. curve.
because the crystal is evenly heated, which makes the laser Laser output spectra are measured by a spectrometer
more stable. (AQ6375, Co. YOKOGAWA) with wavelength range 1.2~
2.4 µm. A pulse-width detector (PCI-3TE-12, VIGO) with
wavelength range 2~12 µm is used to detect the pulse width
III. EXPERIMENTAL SETUP of the pulsed laser. The average output power is measured
by a power meter (F150A-BB-26, Ophir). A beam-quality
The experimental configuration of the acousto-optic analyzer (Pyrocam-III Co. Spiricon, Duma Optronics) is
Q-switched Tm:LuAG laser double-end-intermittently-pumped used to measure the spot pattern of the output laser and the
by pulsed LDs is shown in Fig. 8. beam quality.
Two fiber-coupled pulsed lasers (LD1 and LD2) with In order that the acousto-optical Q-switched Tm:LuAG
emission wavelength of 788 nm are utilized as the pump laser could be intermittently double-end-pumped by pulsed
source. When the repetition frequency is 100 Hz and the LDs, an external triggering device is used to control the
pulse width is 5 ms, the maximum single-pulse energies of output time sequence of the two diode lasers. The Tm:LuAG
LD1 and LD2 are 91.8 and 93.8 mJ respectively. The crystals are intermittently pumped without changing the
diameter and numerical aperture of the fiber core are 400 optimal operating frequency of each laser medium; the
µm and 0.22 respectively. Two diode beams are collimated output of the laser can be optimized better when the
and focused into the doped part of the Tm:LuAG crystal repetition frequency increases exponentially.
by lenses with a focal length of 75 mm. The Tm:LuAG
laser crystal is rod crystal with a diameter of 3 mm and
a length of 25 mm. The doping concentration of Tm3+ is IV. EXPERIMENTAL RESULTS AND ANALYSIS
3 at.%, and the length of the doping part is 15 mm. Both
end faces are coated with antireflective film near 788 nm First, an experimental study of the Q-switched Tm:LuAG
and 2.0~2.1 µm, and the side faces of the crystal are laser double-end-pumped by pulsed LDs was carried out.
polished. The Tm:LuAG crystal is wrapped in indium foil In this experiment, the LD repetition frequency was 100
and put in a water-cooled copper apparatus, the tempe- Hz and the duty ratio 50%, and the output energy and
rature of which is maintained at 289 K. The input mirror pulse width were measured when the Q-switched repeat
M1 is a flat mirror coated with high reflection at 2.0~2.1 frequency was 100 and 200 Hz respectively.
µm (R > 99.5%) and high antireflection at 788 nm (R < As shown in Fig. 9, when the pumping energy was 52.2
0.5%). The 45° mirror M2 is coated for high reflection at mJ and the repetition frequency was 100 Hz, the single-
2.0~2.1 µm (R > 99.5%) and high antireflection at 788 nm pulse energy was 13.7 mJ, the slope efficiency was 40.61%,
(R < 0.5%). The output coupler M3, coated for high antire- the pulse width was 291.5 ns, and the peak power was
flection at 788 nm and 5% transmittance at 2.0~2.1 µm, is 46.99 kW; when the repetition frequency was 200 Hz, the
a plane-concave mirror with radius of curvature 150 mm. single-pulse energy was 5.51 mJ, the slope efficiency was
A Gooch acousto-optic switch (QS041-10M-HI8) is 15.68%, the pulse width was 367.7 ns, and the peak power
composed of a acousto-optic Q head and driver power. The was 14.98 kW.
Q-switching crystal is a quartz crystal with a 2-cm light After increase of the repetition frequency, the single-pulse
diameter and 46-mm length; its RF power is 50 W. The energy decreased and the pulse widened. This is because as
Q-switch apparatus is cooled by a water-cooling machine. the repetition frequency increases, the accumulation time of
The total cavity length is 175 mm. particles at the energy level of the laser working substance
is reduced, and the accumulated number of particles is
limited, causing a widened output pulse, because the period
during which the photon oscillates in the cavity increases
if a Q-switched apparatus is used.
As shown in Fig. 10, when the pumping energy was
56.27 mJ and the repetition frequency was 100 Hz, the
maximum single-pulse energy was 16.3 mJ, the slope
efficiency was 35%, the pulse width was 142 ns, and the
peak power was 114.79 kW. When the repetition frequency
was 200 Hz, the maximum single-pulse energy was 8.31
mJ, the slope efficiency was 19.06%, the pulse width was
101.9 ns, and the peak power was 81.55 kW. However, at
the same repetition frequency, the larger the pumping light
energy, the narrower the pulse width of the laser output;
FIG. 8. The experimental configuration of the acousto-optic this phenomenon indicates that the number of inverted
Q-switched Tm:LuAG laser double-end-intermittently-pumped particles increases with higher pumping power supplied to
by pulsed LDs. the laser working substance in a limited time.
244 Current Optics and Photonics, Vol. 4, No. 3, June 2020
(a) (b)
FIG. 9. Output energy (a) and pulse width (b) varying with the input energy of a Tm:LuAG Q-switched laser double-end-pumped by
pulsed LDs, at repetition frequencies of 100 and 200 Hz.
(a) (b)
FIG. 10. Output energy (a) and pulse width (b) versus input energy of a Tm:LuAG Q-switched laser double-end-intermittently-pumped
by pulsed LDs, at repetition frequencies of 100 and 200 Hz.
The comparison of the experimental results of the pulsed- subjected to energy and the number of upper-energy particles
LD intermittent-pumping technology and the pulsed-LD accumulates and then is released, but not completely released.
double-end-pumping technology is shown in Table 2. When the B face is subjected to energy, the particles
According to the simulation results, by adopting pulsed- generated earlier and newly generated particles at the upper
LD intermittent-pumping technology, after increasing the energy level of the laser working substance are accumulated
repetition frequency the single-pulse energy is reduced and together, over and over again. Adopting the method of
a narrow pulse width is obtained at the same time. This pulsed-LD intermittent pumping, the maximum temperature
is because each end-face absorbs energy alternately. As at the maximum pump energy of 55 mJ was 295.47 K,
shown in Fig. 3, when the energy reaches surface A, A is while the maximum temperature was 300.1 K when adopting
Pulsed-laser-diode Intermittently Pumped 2-µm Acousto-optic Q-switched … - Ya Wen et al. 245
the method of pulsed-LD double-ended pumping. The The output wavelength of 2023.65 nm was detected by
intermittent-pumping technique mitigates the thermal-lens a spectrometer, as shown in Fig. 13. The spectrometer
effect of the crystal, so that narrow pulse width and high
peak power output can still be obtained after the repetition
frequency increases.
Figure 11 shows that, adopting the method of pulsed-LD
intermittent pumping, the maximum peak power obtained at
a repetition frequency of 200 Hz was 81.55 kW, while the
maximum peak power was only 14.98 kW when adopting
the method of pulsed-LD double-ended pumping.
Figure 12 shows the pulse sequence and narrowest pulse
width at the 100-Hz repetition frequency of the power
supply and 200-Hz Q-switched laser output.
(a)
(b)
FIG. 12. (a) Pulsed-LD intermittent-pumping sequence and
Q-switched repetition-frequency sequence; (b) the narrowest
pulse width of the Tm:LuAG laser. FIG. 15. Beam quality of the output laser.
246 Current Optics and Photonics, Vol. 4, No. 3, June 2020
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15. Z. Zhou, X. Huang, X. Guan, J. Lan, B. Xu, H. Xu, Z.
This work is supported by the Education Department of Cai, P. Liu, D. Yan, X. Xu, J. Zhang, M. Lei, and J. Xu,
Jilin Province in China, grant no. JJKH20181102KJ, and “Continuous-wave and passively Q-switched Tm3+-doped
the Science and Technology Department Project of Jilin LuAG ceramic lasers,” Opt. Mater. Express 7, 3441-3447
Province, grant no. 20180101033JC. (2017).
16. Q. Song, X. Xu, Z. Zhou, Z. Xu, B. Xu, D. Li, P. Liu, J.
Xu, and K. Lebbou, “Laser operation in a Tm:LuAG crystal
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