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High-Fidelity Transport of Trapped-Ion Qubits in a Multi-Layer Array

Deviprasath Palani, Florian Hasse, Philip Kiefer, Frederick


Boeckling, Jan-Philipp Schroeder, Ulrich Warring, Tobias Schaetz
Albert-Ludwigs-Universitaet Freiburg, Physikalisches Institut Hermann-Herder-Strasse 3, Freiburg 79104, Germany
(Dated: May 11, 2023)
A variety of physical platforms are investigated for quantum control of many particles, and tech-
niques are extended to access multiple dimensions. Here, we present our experimental study of
shuttling single Mg+ ions within a scalable trap-array architecture that contains up to thirteen
trapping sites in a three-dimensional arrangement. We shuttle ions from a dedicated loading hub
to multiple sites with a success rate of larger than 0.99999. In a prototype application, we demon-
strate the preservation of the coherence of superposition states of a hyperfine qubit during inter-site
shuttling. Our findings highlight the potential of these techniques for use in future large-scale
arXiv:2305.05741v1 [quant-ph] 9 May 2023

architectures.

Developments toward larger-scale quantum technol- 150 quanta for a single shuttle operation. In addition,
ogy are driven by conceived performance advantages for we preserve coherence of the electronic degree of free-
quantum information processing, experimental simula- dom despite shuttling ions through four sites of an array
tion, and metrology applications [1–3]. Experimental re- spanning a triangular-pyramidal configuration.
search pursues two common objectives in multiple eli- Our custom-designed ultra-high vacuum chamber
gible platforms: (i) improving manipulation techniques hosts the radio-frequency (rf) surface-electrode trap, fea-
towards near-unity fidelity, and (ii) fostering architec- turing an array of individual trapping sites, fine-tuned by
tures with global and local control capabilities. Trapped 30 discrete control electrodes [16], see Fig. 1. We employ
atomic ions naturally feature reproducible qubits and laser beams aligned parallel to the chip surface from five
demonstrate notable performance qualities, approach- different laser sources for ablation loading [33, 34] and
ing operational fidelities for all required tasks at a level manipulation [35] of 24 Mg+ and 25 Mg+ (with hyperfine
of 0.9999 for ensembles of few-ions in linear arrange- structure) in a quantization field |Bquant | ' 10.9 mT [36].
ments [4–9]. Integration of these features into suffi- We find average storage duration (1/e time) of single
ciently extendable architectures is investigated in several ions to be ' 15 minutes. Currently, storage is limited
ways, e.g., following bottom-up approaches of quantum by background gas collisions, consistent with the resid-
charged-coupled devices (QCCD) [10, 11], ion-photon ual gas pressure of our chamber at ' 10−9 Pa. We im-
networks [12, 13], and trapped-ion arrays [14–17] or top- age the fluorescence light of trapped ions either on an
down approaches [18–20]. The QCCD, on the one hand, electron-multiplying charge-coupled device camera or a
builds on ion qubits stored in memory regions, being photo-multiplier tube (PMT). Our experimental control
shuttled along dedicated ion-guides to interaction re- hardware is software interfaced by Python, and we con-
gions for logic operations, e.g., to build up many-qubit trol parameters, record data, and perform data analysis
entanglement [21]. Required shuttling routines are per- routines in a JupyterLab environment.
formed, mitigating ion-loss [22] while being optimized for The trap chip is fabricated by Sandia National Labora-
speed [23–25] within interlinked 1D trapping arrays. On tories [16]. A high-power frequency generator provides a
the other hand, the array of individually trapped ions power of ' 26 dBm oscillating at ΩRF /(2π) ' 52.4 MHz
features trapping sites at sufficiently small distances that to a helical resonator that amplifies the trapping volt-
allow for directly exploiting the Coulomb interaction at age with a loaded quality factor of ' 20. The three-
long range. This may allow evolving the quantum sys- dimensional trapping landscape of the array is gener-
tem as a whole, even in higher dimensions. For example, ated by a common rf potential applied to two optimally
multidimensional entanglement is envisioned to be con- shaped electrodes [16]. We estimate a rf voltage am-
ceived by engineered and tunable inter-site interactions – plitude of URF ' 200 V (zero-to-peak). In Fig. 1, we
required methods are established in one [26–28] and two show two calculated equipotential surfaces of the cor-
dimensions [16, 29–31]. The latter is anticipated to per- responding pseudo-potential Φrf for 24 Mg+ at 0.5 meV
mit addressing currently intractable open questions of and 4 meV, respectively. In this pure rf configuration
interest via experimental quantum simulations [31, 32]. (all other electrodes are electrically grounded), we create
Combining the advantages of QCCD and multidimen- seven distinct trapping regions featuring 13 sites, each
sional array architectures may turn out beneficial for fu- site is highlighted by disks in the overlay of Fig 1. The
ture quantum applications. regions are mutually separated by the 0.5 meV potential
In this Letter, we present high-fidelity shuttling of sin- barrier, but overall enclosed by the 4 meV potential bar-
gle Mg+ between different sites of our multi-layer (2d+) rier. In the following, we focus on three in-plane (the
trap-array. The success rate for shuttling through locally xy plane, parallel to the surface) sites and one out-of-
controlled transfer channels is larger than 0.99999. We plane site: The three sites, labelled T0 , T1 and T2 , form
observe an excess motional mode heating smaller than a 40 µm equilateral triangle at z ' 40 µm. The site TH
2

accuracy of 10 ns. In this work, we use six dedicated


control potential configurations Φc , designated and cali-
brated for ion loading ΦHL and storage ΦH in TH , as well
as, single-ion storage in one of the three lower lying sites:
Φ0 , Φ1 , and Φ2 . Moreover, we calibrated ΦPyramid , to
initialize the pyramid, i.e., single ions in all four sites, re-
spectively. Note that the total trapping potential is given
by Φrf + Φc (here, ignoring stray potential contribution),
and we describe our routine to find such configurations
in [38].
To shuttle single ions, we switch between initial and fi-
nal Φc with variable timings tplayback of 0.1 to 1 ms. For
example, to shuttle the ion from TH to T1 , we choose
initially Φc = ΦH and switch to Φc = Φ1 . During play-
back of the corresponding waveform comprised by a lin-
ear ramp, a transfer channel between TH and T1 is estab-
lished, and the ion is shuttled. To reverse this process, we
shift back to Φc = ΦH . In this way, we can engineer arbi-
trary inter- and intra-regional shuttling, while we focus
here on demonstrations of inter-regional shuttling.
For loading ions, we use an ablation laser with a wave-
length of 1030 nm, a repetition rate of 1.5 kHz, a pulse
width of 1.4 ns, and a maximal pulse energy of 93 µJ. The
FIG. 1. Illustration of our trap-array archeticture. In the
background, we show a schematic of the two radio-frequency beam is focused by a 150 mm focal length lens onto a Mg
and 30 control electrodes used for the generation and fine con- wire with 0.4(1) mm diameter inside the vacuum cham-
trol of our trapping landscape. Overall, we create 13 discrete ber, mounted at a distance of ' 10 mm from TH . We
trapping sites marked by disks in the overlay. We depict cal- tune the pulse energy by a variable neutral density filter
culated pseudo-potential equipotential surfaces for 0.5 meV and estimate the beam waist on the target to be smaller
(red, high opacity), mutually separating seven regions with than 1/10 of the diameter of the wire. A photo-ionization
single or multiple sites, and 4 meV (red, low opacity). To ef- beam near 285 nm is tuned to selectively ionize 24 Mg or
fectively open and close inter-regional ion transport channels, 25
Mg. We pass the beam near TH with a waist of 30 µm
we switch between dedicated control potentials. We highlight and a power of ' 1 mW.
four sites that define a unit cell of a 2d+ lattice in the shape of
Three additional laser beams from a common laser
a triangular pyramid (dashed lines). The inset shows a false-
color fluorescence image of four single ions at T0 , T1 , T2 , and source are tuned to address a S1/2 to P3/2 cycling tran-
TH , respectively. Ions are observed at a 16◦ angle relative to sition with natural line width Γ/(2π) ' 42 MHz: Two
the surface normal, and their positions are adjusted by local for Doppler cooling [35], detuned by −8 Γ and −Γ/2, and
control fields. one tuned close to resonance for detection. Optionally,
we use two additional laser beams from another source
tuned to address dedicated S1/2 -P1/2 transitions for im-
(hub) is situated at the center of our array, but is elevated proved state preparation in 25 Mg+ via optical pump-
to z ' 53 µm. In combination, all four sites define a unit ing. Laser frequencies of both sources are stabilized via
cell in the shape of a triangular pyramid. For our exper- a wavemeter and/or Doppler-free saturation absorption
imental parameters, we find mode frequencies ω/(2π) of spectroscopy. All five laser beams (for global ion ma-
4 to 7 MHz of single ions in sites T0 , T1 , and T2 and of nipulation) are superimposed, aligned with Bquant , and
1 to 3 MHz in TH . polarized to yield σ + polarization. We align these beams
A metal sheet mounted ' 7 mm above the chip sur- with waists ' 30 µm at TH . This results in significantly
face is biased to apply a global electric field to compen- lower beam intensities at sites T0 , T1 , and T2 , which we
sate stray fields along the z-axis. In addition, we use estimate at 25 %, 30 %, and 15 %, respectively. Option-
30 control electrodes (integrated in the chip) for local ally, we apply local AC Stark shifts [35] via a dedicated
fine-tuning of trapping conditions. For example, we ap- laser beam detuned by ' +1000 Γ from the S1/2 -P3/2
ply local stray field compensation and tuning of local transition. This far-detuned beam is focused at T1 with
potential curvatures, i.e., mode frequencies and orien- a waist of ' 10 µm.
tations. Control voltages are supplied by a 36-channel Using 25 Mg+ , we span a qubit by the hyper-
arbitrary waveform generator (AWG) [37] with outputs fine ground states S1/2 , F = 3, mF = +1 ≡ |↓i and


connected via low-pass filters with cut-off frequencies S1/2 , F = 2, mF = 0 ≡ |↑i coupled via a first-order field-
ωlowpass /(2π) ' 7 kHz. The AWG is integrated into our independent transition ωqubit /(2π) ' 1762.974 MHz at
data acquisition system for real-time playback of wave- |Bquant | [36]. We can coherently manipulate all S1/2 hy-
forms within our experimental sequences with a timing perfine states via microwaves. We currently prepare
3

TABLE I. Quality of roundtrips from TH to all sites, follow-


ing similar protocols as illustrated in Fig. 3a. We list fluores-
cence changes, upper bound estimates of mode heating per
roundtrip, and maximal slew rates required for the playback
of waveforms.
Visited ∆Fluo. per Mode heating Slew rate
site round trip(%) (quanta/roundtrip) (V/ms)
T0 -8.7(6) /287 <4
T1 -2.1(6) /84 <3
T2 -5.9(6) /197 <3

about 1.2 s. If a single ion is detected, step 3 is engaged:


The AWG is triggered to switch to ΦH and the ion is
FIG. 2. Automated loading of single ions at the hub for continuously Doppler cooled. If the loading attempt is
subsequent redistribution within the unit cell. (Inset) A single unsuccessful, the program repeats steps 1 and 2. In case
loading attempt is comprised by the following sequence: 1) ten subsequent loading attempts are unsuccessful, the
Ablation (red, five to ten pulses), photo-ionization (yellow), automated loading sequence is terminated, and we man-
and cooling lasers (blue), as well as control potentials, are ually adjust relevant parameters, e.g., re-tuning of ΦHL .
engaged for loading in TH , 2) cooling laser remains on during During about 180 days, we attempt 973 loading bursts,
a triggered snapshot of our camera, the image is analyzed for and we find a probability of about ' 0.4 to be successful
the presence of a single ion, and 3) a successfully loaded ion is after the first burst. Typically, we carefully check rele-
kept Doppler cooled. Typically, we use about five to ten laser
vant experimental parameters once per week. For loading
ablation pulses in a single loading attempt. The histogram
shows the accumulated 973 attempts of ' 180 days of data of multiple ions, we adapt the sequence to fill dedicated
taking. sites. For example, for filling all four sites of the pyramid
(see inset of Fig. 1), we repeat steps 1 and 2 until we load
four ions into TH and switch control potentials from ΦHL
qubit states with a fidelity of 90(2)% and find a coherence to ΦPyramid .
time τcoh ' 6 ms for equal superposition states of |↓i and To benchmark the shuttling fidelity of single ions, we
|↑i. State preparation fidelity and coherence duration study relocation roundtrips with 24 Mg+ . The experimen-
are likely to be limited by stray currents in rf electrodes. tal sequence (Fig. 3a) comprises initialization and detec-
Further, we measure static magnetic-field gradients of tion at TH with interleaved shuttling roundtrips to T1
' 0.013 T/m near TH . at a distance of dH,1 ' 25 µm. We measure the change
An objective, collecting fluorescence light from the of average fluorescence rate due to a shuttling roundtrip
ions, is mounted at an angle of ' 16◦ regarding the z- in comparison to reference histograms taken for the ion
axis and projects tilted image planes onto our camera remaining at TH . In Fig. 3b, we show corresponding data
chip. We can spatially resolve individually trapped ions for 11,000 repetitions. In this way, we calculate an up-
with a resolution of 0.32(1) µm per pixel. The inset of per bound for the motional heating of 84 quanta per
Fig. 1 shows a false-color image of recorded fluorescence round trip, estimated for the lowest-frequency mode at
light of four 24 Mg+ forming a fully filled unit cell. Ion 2π 1 MHz, to get a conservative bound. Note, that exci-
positions are altered from the ideal triangular-pyramidal tations are more-likely to be unevenly distributed on all
locations by less than 5 µm – considering a correction for three modes, and details depend on the evolution of mode
the tilted perspective. Alternatively, we collect photon orientations regarding rf field lines along shuttling tra-
count histograms with the PMT, and estimate motional jectories. While we assume in the following that excita-
mode excitation [39] or electronic-state populations [35]. tions are non-coherent (thermal) for our shuttling speeds
In most of our experiments presented here, we utilize dH,1 /tplayback ' 0.25 m/s, we attribute excess heating
an automated single-ion loading sequence. We study its to a rf noise heating mechanism and digital sampling
repeatability with data taken over the course of about noise [22, 40]. We summarize corresponding shuttling re-
180 days (see Fig. 2). We choose a pulse energy of the sults to all sites in Tab. I, and emphasize that motional-
ablation laser of ' 30 µJ. The automated sequence, il- heating rates per shuttling roundtrip are < 300 quanta.
lustrated in the inset of Fig. 2, comprises three steps. The average ion storage duration, currently, limits us to
Step 1: Control voltages are set to ΦHL , cooling and ' 100, 000 consecutive shuttling sequences, yielding an
photo-ionization beams are on, while a burst of about estimate for a shuttling failure rate of lower than 10−5 .
five to ten ablation pulses is fired. Step 2: The program To study the effects of shuttling on the electronic de-
captures a single camera frame with 500 ms integration grees of freedom, we probe the coherence of qubit su-
duration, and analyzes the image to identify the pres- perposition states in 25 Mg+ for multiple ion relocation
ence of a single ion at TH . Steps 1 and 2 take in total scenarios. All sequences are comprised of three steps, see
4

FIG. 3. Quality of shuttling single ions from TH to T1 and


back (roundtrip). We enable transport by playback of wave-
forms between fine-tuned control potential configurations ΦH FIG. 4. Coherent manipulation of qubit states in 25 Mg+ with
and Φ1 within 0.1 ms. During reference experiments, we fix multiple relocations. a) In three single-ion sequences, we ini-
the control potential configuration to ΦH . In a), we illustrate tialize I) |↓i-|↑i superposition and probe coherences with anal-
transport (squares) and reference (discs) sequences that I) ini- ysis pulses before D) detection in TH . In the first and second
tialize and D) detect 24 Mg+ at TH . Here, we execute 11,000 sequences, we probe single relocation roundtrips to T1 (discs)
repetitions of shuttling without ion loss. In b), we show cor- and apply optional local AC Stark shifts (squares). In the
responding photon count histograms (reference: disks joined third sequence, we study the effect of multiple subsequent
by black line) and find a fluorescence change of −2.1(6) % relocation roundtrips to all sites (diamonds). In b), we com-
due to shuttling. We summarize relocation results to all sites pare the resulting P↓ for all sequences as a function of analysis
in Table I, and find that mode heating due to shuttling is phase ϕ. Model fits result anticipated phase shifts and probed
< 300 quanta per round trip. coherence amplitudes are consistent with background effects.

Fig.4a. Step 1: We Doppler cool, and initialize an equal sponding reference sequences of 5(4)◦ , 44(3)◦ , and 4(4)◦ ,
superposition of |↓i and |↑i with a microwave π/2 pulse respectively. Relative shifts arise from the magnetic-field
at TH . Step 2: We implement this step in three differ- gradients and are, in particular, in agreement with the
ent versions for direct comparison: i) Ion is shuttled to anticipate AC-stark shift of 2π 2.21(6) kHz applied during
T1 and back, ii) ion is shuttled to T1 , and we apply a scenario ii). We conclude that dephasing contributions
calibrated AC stark shift with the far-detuned beam for due to ion shuttling are below our resolution, while rel-
50 µs before shuttling it back, iii) we engage multiple sub- ative phase shifts can be accounted for via appropriate
sequent shuttling roundtrips from TH to all sites. Note, bookkeeping.
versions i) and ii) span a total duration of 0.25 ms and iii) To summarize, in approximately 90 % of the attempts,
spans 0.6 ms, i.e, 24 to 10 times shorter than τcoh . Step 3: we load and confirm the presence of single ions within
Before fluorescence detection at TH , we use an analysis 6 seconds at any site on demand. Simultaneous deter-
π/2 pulse of variable phase ϕ, relative to the initial π/2 ministic loading of four sites with single ions is enabled
pulse, to probe the qubit coherence. We analyze photon by mutual Coulomb repulsion. Alternative loading meth-
count histograms to estimate the population probability ods, e.g., using a pre-cooled atom source [41, 42] may be
P↓ of state |↓i, and plot data points as a function of ϕ beneficial in refilling arrays even more efficiently. Af-
in Fig. 4b. Each data point is an average of 1,000 repe- ter loading, a single ion is shuttled to four sites and
titions. Using sinusoidal model fits, we extract the con- back for more than 100,000 repetitions (limited by back-
trast and phase offsets. We compare our findings to the ground gas pressure) with a mean energy gain of be-
results of dedicated reference sequences, in which a single low 150 quanta per trip within a single trip duration of
ion remains at TH : The contrasts are 82(1) %, 85(2) %, 0.1 ms. Tuning of experimental parameters can enable
and 82(3) %, respectively, while for the reference on av- even non-adiabatic shuttling entailing moderate motional
erage 83(1) % – coherence rates are consistent with the heating [23, 24, 40]. Previously, we showed the prepara-
reference. Further, we find phase offsets relative to corre- tion of quantum mechanical ground states in single and
5

multiple sites [39], control of motional parameters [16], tecture, with its tunable long-range interactions, holds
and tunable inter-site interactions via engineered phonon potential for future exploitation. By combining it with
couplings [29, 30] in two dimensions. On the one hand, the exceptional operational fidelities of single and few
establishing phonon couplings between arbitrary sites in ions systems, we may be able to initialize and further
our 2d+ array permits accessing quantum simulations explore multi-dimensional, fiducial entangled states.
extended in size and dimension [43]. On the other hand,
exploiting two-to-three times smaller distances d (inter-
action strength ∝ 1/d3 ) and ancilla ions (boosting inter- ACKNOWLEDGMENTS
actions by additional electric charges), coupling rates can
significantly exceed current decoherence rates. Technical The trap chip was designed together with R. Schmied
limitations such as electric-field noise and background in cooperation with the NIST ion storage group and
gas pressure can be mitigated by surface treatment meth- produced by Sandia National Laboratories. This work
ods [44] and cryogenic environments [45]. Finally, we sub- was supported by the Deutsche Forschungsgemeinschaft
stantially extend, here, our toolbox by shuttling qubits (DFG) (Grant No. SCHA 973/6-3) and the Georg H.
within our array, while preserving coherence. Thus, we Endress foundation. We thank Joern Denter, Kambiz
demonstrate prototype features of a 2d+ QCCD that can Mahboubi, Fraenk Grossman, and their teams for tech-
be upgraded with existing tools [21, 46–48]. Our archi- nical support.

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7

SUPPLEMENTAL MATERIAL: HIGH-FIDELITY


TRANSPORT OF TRAPPED-ION QUBITS IN A
MULTI-LAYER ARRAY

We show a schematic of our trap architecture with the


30 control electrodes in Fig. 5; the metal sheet is not
shown. Using the AWG, we apply voltages correspond-
ing to individual Φc to all electrodes (31 in total), and
list values in Table II. To establish shuttling of single ions
from TH to all sites, we perform dedicated calibration se-
quences with single 24 Mg ions and optimize Φc for fixed
rf drive parameters. The procedure comprises two steps:
Step 1, for shuttling an ion, we linearly ramp between
two control potential configurations used for ion storage
at two different sites (TH and the site of choice). Step 2,
by comparing the collected photon count histograms, we
fine-tune individual sets of control potentials to opti-
mize/reduce the overall slew rate needed. Thereby, mini-
mizing the fluorescence loss due to relocation. We ensure
the success of operations via camera images. In Table I of
the main text, we list the maximum slew rates required
for the playbacks. For a single relocation, we play back
FIG. 5. Schematic of the central region of our rf surface waveforms between dedicated fine-tuned control poten-
electrode trap. We show the two rf electrodes and labels of tial configurations with minimized slew rates in a time
all 30 control electrodes. period of 0.1 ms.
8

TABLE II. Voltages (V) applied to electrodes for dedicated


ΦC . Our AWG has a discretization limit at 3 × 10−4 V (for
each channel), and provides voltages in the range of [-10,10] V.
Electrodes Φ0 Φ1 Φ2 ΦH ΦHL ΦPyramid
el1 0.0959 0.0959 0.0959 0.0959 -0.0038 0.0959
el2 -0.1676 -0.1676 -0.1676 -0.1676 0.1484 -0.1676
el3 -0.2760 -0.2760 -0.2760 -0.2760 -0.1484 -0.2760
el4 0.2328 0.2328 0.2328 0.2328 0.1484 0.2328
el5 -0.1246 -0.1246 -0.1246 -0.0246 0.0870 -0.1246
el6 0.1520 0.1520 0.1520 0.1520 -0.1484 0.1520
el7 -0.5683 -0.5683 -0.5683 -0.5683 -0.1484 -0.5683
el8 0.3005 0.3005 0.3005 0.3005 -0.0094 0.3005
el9 -0.4945 -0.4945 -0.4945 -0.4945 -0.1484 -0.4945
el10 -0.4502 -0.4502 -0.4502 -0.4502 -0.0641 -0.4502
el11 0.7980 0.7980 0.7980 0.7980 0.1484 0.7980
el12 0.1130 0.1130 0.1130 0.1130 0.1484 0.1130
el13 0.0327 0.0327 0.0327 0.0327 0.1484 0.0327
el14 -0.1239 -0.3239 -0.1239 -0.1239 0.1484 -0.3239
el15 0.0007 0.0007 0.0007 0.0007 -0.0387 0.0007
el16 0.6000 0.6000 0.6000 0.6000 -0.1484 0.6000
el17 0.0064 0.0064 0.0064 0.0064 -0.1484 0.0064
el18 -0.6718 -0.6718 -0.6718 -0.6718 -0.1484 -0.6718
el19 -0.3833 -0.3833 -0.3833 -0.3833 -0.1484 -0.3833
el20 -0.0137 -0.0137 -0.0137 -0.0137 -0.1484 -0.0137
el21 0.1892 -0.1108 -0.1108 -0.1108 -0.1484 0.1892
el22 -0.1364 -0.1364 -0.1364 -0.1364 0.0671 -0.1364
el23 0.5604 0.5604 0.2604 0.5604 0.1484 0.2604
el24 -0.1949 -0.1949 -0.1949 -0.1949 -0.1111 -0.1949
el25 0.4670 0.4670 0.4670 0.4670 -0.1484 0.4670
el26 -0.4358 -0.4358 -0.4358 -0.4358 0.0103 -0.4358
el27 0.1844 0.1844 0.1844 0.1844 0.1484 0.1844
el28 0.3901 0.3901 0.3901 0.3901 0.1484 0.3901
el29 -0.6760 -0.6760 -0.6760 -0.6760 -0.1484 -0.6760
el30 -0.6392 -0.6392 -0.6392 -0.6392 -0.1484 -0.6392
Metal sheet -3.5000 -3.5000 -3.5000 -3.5000 -2.7000 -3.5000

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