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PHYSICAL REVIEW B 104, 115420 (2021)

Topological Magnus responses in two- and three-dimensional systems

Sanjib Kumar Das ,1,*,† Tanay Nag ,2,*,‡ and Snehasish Nandy3,§
1
IFW Dresden and Würzburg-Dresden Cluster of Excellence ct.qmat, Helmholtzstr. 20, 01069 Dresden, Germany
2
Institute für Theorie der Statistischen Physik, RWTH Aachen University, 52056 Aachen, Germany
3
Department of Physics, University of Virginia, Charlottesville, Virginia 22904, USA

(Received 26 April 2021; revised 22 August 2021; accepted 9 September 2021; published 17 September 2021)

Recently, time-reversal symmetric but inversion broken systems with nontrivial Berry curvature in the
presence of a built-in electric field have been proposed to exhibit a new type of linear Hall effect in ballistic
regime, namely, the Magnus Hall effect. The transverse current here is caused by the Magnus velocity that is
proportional to the built-in electric field enabling us to examine the Magnus responses, in particular, Magnus
Hall conductivity and Magnus Nernst conductivity, with chemical potential. Starting with two-dimensional (2D)
topological systems, we find that warping induced asymmetry in both the Fermi surface and Berry curvature can
in general enhance the Magnus response for monolayer graphene and surface states of topological insulator.
The strain alone is only responsible for Magnus valley responses in monolayer graphene, while warping
leads to finite Magnus response there. Interestingly, on the other hand, strain can change the Fermi surface
character substantially that further results in distinct behavior of Magnus transport coefficients as we observe
in bilayer graphene. These responses there remain almost insensitive to warping unlike the case of monolayer
graphene. Going beyond 2D systems, we also investigate the Magnus responses in three-dimensional multi-Weyl
semimetals (mWSMs) to probe the effect of tilt and anisotropic nonlinear energy dispersion. Remarkably,
Magnus responses can only survive for the WSMs with chiral tilt. In particular, our study indicates that the
chiral (achiral) tilt engenders Magnus (Magnus valley) responses. Therefore, Magnus responses can be used as
a tool to distinguish between the untilted and tilted WSMs in experiments. In addition, we find that the Magnus
Hall responses get suppressed with increasing the nonlinearity associated with the band touching around the
multi-Weyl node.

DOI: 10.1103/PhysRevB.104.115420

I. INTRODUCTION symmetry [13–21]. Very recently, the same systems (TRS


invariant but inversion broken) with a built-in electric field at
The family of Hall effects have revolutionized the solid
zero magnetic field are found to exhibit a new type of a linear
state physics in the context of novel electronic states and elec-
response, namely the Magnus Hall effect (MHE) [22]. The
tron dynamics [1–3]. Starting from the Lorentz force mediated
MHE is originated from the Magnus velocity of electron that
classical Hall effect and quantum Hall effect, various new
is perpendicular to the BC and the built-in electric field. Along
types of Hall effect such as anomalous Hall effect, spin Hall
with the prediction of MHE, it has also been proposed that the
effect, thermal Hall effect, etc. have been discovered over the
Magnus Nernst effect (MNE) and Magnus thermal Hall effect
years [1–11]. Among them, the Berry curvature (BC) induced
can also appear in these systems in the presence of an applied
Hall effects, taking place without external magnetic field, have
thermal gradient [23].
drawn tremendous attention to both theorists and experimen-
It has been proposed that the two-dimensional (2D) tran-
talists [4–10,12]. For time reversal symmetry (TRS) broken
sition metal dichalcogenides MX2 (M = Mo, W and X = S,
systems, the BC takes the form (k) = −(−k) leading to
Se, Te) [14,24–26], monolayer (ML) graphene on hBN, bi-
a finite total BC for the occupied states. By contrast, in TRS
layer (BL) graphene with applied perpendicular electric field
invariant systems, BC follows (k) = −(−k) giving rise to [27–29], heterostructures [30], and surfaces of topological
zero total BC [12], that further causes the intrinsic anomalous insulator (TI) [31] are the possible candidates to investigate
Hall effect to vanish. Interestingly, it has been theoretically the MHE and MNE for their TRS invariant and inversion bro-
proposed and experimentally verified that, unlike the linear ken nature. The MHE has been theoretically studied recently
anomalous Hall effect, the nonlinear anomalous Hall effect in graphene and transition metal dichalcogenides using the
can survive in TRS invariant systems with broken inversion low-energy model without warping (except bilayer graphene
where trigonal warping is considered) and strain [22,23].
On the other hand, it has been shown that, without spin-
*
Both authors contributed equally to this work. orbit coupling and tilting of the Dirac cone, the BC dipole

s.k.das@ifw-dresden.de becomes substantially large in the presence of strain and warp-

tnag@physik.rwth-aachen.de ing for graphene [29]. Motivated by the BC dipole induced
§
sn5jm@virginia.edu nonlinear anomalous Hall effect in TRS invariant systems,

2469-9950/2021/104(11)/115420(15) 115420-1 ©2021 American Physical Society


DAS, NAG, AND NANDY PHYSICAL REVIEW B 104, 115420 (2021)

our interest here is to investigate Magnus transport in the II. FORMALISM OF MAGNUS TRANSPORT
presence of strain and warping for the above proposed suitable
In this section, we derive the general expression for MH,
candidates.
MN conductivities in both diffusive and ballistic regimes
Turning to the field of three-dimensional (3D) topological
systems, Weyl semimetals (WSMs), considered to be a 3D using the Boltzmann transport equation. To begin with, we
analog of graphene, have been studied extensively for their consider mesoscopic systems of electronic transport in a Hall
intriguing properties and anomalous response functions. The bar device without applying any external magnetic field. In
gap closing points, guaranteed by some crystalline symme- this setup, the source and the drain are kept at different electro-
tries, in WSMs are referred to as Weyl nodes with topological static potential energy with the gate voltages given by Us and
charge n = 1 [32–38]. There exists two Weyl nodes of op- Ud , respectively. Their difference U = Us − Ud introduces
posite chiralities for the TRS broken WSM, while inversion a built-in electric field E in = ∇ rU/e (−e is the electronic
broken WSM exhibits at least four Weyl nodes [39,40]. The charge) in the device with a slowly varying electric potential
WSMs can also be classified as type I and type II. In the case energy U (r) along the length of the sample.
of type-I WSM, the Fermi surface is always pointlike irrespec- Now in the presence of external electric field E and temper-
tive of the tilting of the node. On the other hand, in type-II ature gradient ∇T applied between the source and drain, the
WSM finite electron and hole pockets appear at the Fermi charge current J and thermal current Q from linear response
level as a result of finite tilting of the energy spectra [41–43]. theory can be written as
Moreover, it has been recently found that n > 1 multi-WSM Ja = σab Eb + αab (−∇b T ),
(mWSM) shows nonlinear band touching [44,45]. The WSMs
are shown to exhibit many intriguing transport properties, Qa = ᾱab Eb + κab (−∇b T ), (1)
originated by chiral anomaly, such as negative longitudinal where a and b are spatial indices running over x, y, z. Here σ ,
magnetoresistance and planar Hall effect [46–59]. Tilting of α, and κ are different conductivity tensors.
energy dispersion and nonlinearity of band touching further The phenomenological Boltzmann transport equation can
decorate the transport signatures [60–64]. This motivates us be written as [65,66]
to extend our investigation of MHE to 3D topological systems  
considering a generic mWSM Hamiltonian. ∂
+ ṙ · ∇r + k̇ · ∇k fk,r,t = Icoll { fk,r,t }, (2)
In this work, we first capture intriguing Fermi surface phe- ∂t
nomena in the presence of strain and warping by examining
where the right side Icoll { fk,r,t } is the collision integral which
MHE and MNE in a ballistic regime for 2D topological sys-
incorporates the effects of electron correlations and impu-
tems, such as ML, BL graphene, and surface states of TIs. We
rity scattering. The electron distribution function is denoted
find that, in strained ML graphene without warping, the total
by fk,r,t . Now under the relaxation time approximation the
valley integrated Magnus responses are zero as the contribu-
steady-state Boltzmann equation can be written as
tions coming from the individual valley exactly cancel each
other. The valley polarized contribution thus leads to the Mag- f0 − fk
(ṙ · ∇r + k̇ · ∇k ) fk = , (3)
nus valley Hall, Magnus valley Nernst effects. Interestingly, τ (k)
warping induces valley integrated finite Magnus responses as
the asymmetries in Fermi surface and BC result in unequal where τ (k) is the scattering time. Note that, in this work, we
valley polarized contributions. The magnitude of the Magnus ignore the momentum dependence of τ (k) for simplifying the
responses are enhanced with the increasing warping parame- calculations and assume it to be a constant. The equilibrium
ter. The same is observed for the surface states of TI in the distribution function f0 in the absence of applied electric
presence of hexagonal warping. On the other hand, for BL field E and temperature gradient ∇ r T is given by the Fermi
graphene, the Magnus transport coefficients are substantially function,
modified depending on the positive and negative values of 1
strain, while warping does not affect the Magnus transport. Fi- f0 (k, r) = , (4)
1 + eβ[ (k,r)−μ]
nally, going beyond 2D systems, we study Magnus responses
in 3D WSMs to examine the effect of tilt and anisotropic where β = 1/(kB T ), (k, r) = k + U (r), with k and μ are
nonlinear dispersion. We find that the MHE is identically zero the energy dispersion and chemical potential, respectively.
for each Weyl node without tilt. Remarkably, chiral (achiral) The motion of the wave packet inside the Hall bar is described
tilt causes finite MH and MN conductivities to generate from by the semiclassical equations of motion [12,67]
individual Weyl nodes resulting in Magnus (Magnus Valley) h̄ṙ = ∇k + [∇rU + eE] × , (5)
k
responses. Moreover, our study indicates that the topological
charge associated with Weyl node imprints its effect on the h̄k̇ = −∇rU − eE. (6)
Magnus transport properties.
The rest of the paper is organized as follows. In Sec. II, we The first, second, and third term in the right hand side of
derive the general expressions of MH and MN conductivities Eq. (5) respectively represent the band velocity, Magnus ve-
in both ballistic and diffusive regimes. Following which, in locity VMagnus = ∇rU × , and anomalous velocity Vano =
Sec. III we have calculated the Magnus transport responses in E × . The Magnus velocity Vmagnus can be thought of as a
the presence of strain and warping (tilt and nonlinearity) for quantum analog of the classical Magnus effect.
different 2D (3D) topological systems, respectively. Finally, Now, to calculate MH and MN conductivities, we apply the
we summarize our results and discuss possible future direc- electric field and temperature gradient along the x direction.
tions in Sec. IV. Assuming the length of the sample is along the x axis, we

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TOPOLOGICAL MAGNUS RESPONSES IN TWO- AND … PHYSICAL REVIEW B 104, 115420 (2021)

have U (r) = U (x), (k, r) = k + U (x), and E in = 1e ∂U∂x(x) x̂. and T /L = −∇x T . The MH and MN coefficients in the
Since we consider U (x) is slowly varying, the electron wave ballistic regime can be obtained as [22,23]
packets traveling inside the sample still have well-defined

momentum k. Considering the velocity of an incident electron e2
(vx , vy ), transit time through the electric field region becomes σ =− U dk z ∂ f0 , (13)
h̄ vx >0
t = L/vx , where L is the device length along x direction. For 
e
vy = 0, the center of the wave packet receives a transverse α= U dk z ( k − μ)∂ f0 . (14)
shift (in y direction), followed by Magnus velocity propor- h̄T vx >0

tional to ∇xU z , while traversing the junction due to the


built-in electric field E in . Now the charge and thermal currents Similar to the diffusive regime, the Magnus transport coeffi-
can be written as cients in the ballistic regime also obey the Mott relation and
 the Wiedemann-Franz law.
{J(x), Q(x)} = dk ṙ{−e, [ (k, x) − μ]} f (k, x). (7) We would now like to add a few comments on Magnus re-
sponses. It is clear from Eqs. (9) and (10) as well as Eqs. (13)
and (14) that the MHE and MNE are purely determined by
Combining Eqs. (3), (5), and (6), the nonequilibrium dis-
Fermi surface properties as they incorporate the ∂ f0 factor. In
tribution function f up to linear order in the bias fields can be
order to obtain finite Magnus responses, the systems should
written as
have an asymmetric Fermi surface. In addition, the system
 
[ (k, r) − μ] must possess finite BC. Moreover, the condition vx > 0 hap-
f = f0 + vx τ eEx + ∇x T ∂ f 0 . (8) pens to be very important while summing the BC over the
T
Brillouin zone. Combining all these, the active momentum
Considering U as a slowly varying function of x, ∂U/∂x = modes kv , over the Fermi surface k = μ, for which vx > 0
U/L, one can obtain f to be spatially independent. To be would contribute to Magnus transport. The remaining mo-
precise, using Eq. (8) in Eq. (7) and comparing with Eq. (1), mentum modes k − kv become inert in this ballistic transport
the MH conductivity σ is found to be [23] and BC for these momentum modes do not determine the
 transport. These transports thus allow us to scan different
e2 τ U Fermi surfaces by tuning μ and get the idea about angular
σ =− dk z vx ∂ f0 . (9)
h̄ L distribution of BC within a given Fermi surface.
The Magnus responses can be regarded as an effective
Similarly, the MN conductivity α is given by [23] second order transport as the built-in electric field U and ex-
 ternal bias both come into calculation of currents. However, in
ekB τ U
α= dk z vx β( k − μ) ∂ f0 , (10) terms of the external bias field, it is still a linear response phe-
h̄ L nomena. The BC dipole induced second order transport [13],
where we have neglected the contributions coming from the given by Di j = dk di j δ( k − μ) with di j = vi (k) j (k), is
band velocity. Interestingly, as discussed above these Magnus primarily different from Magnus transport for which the tilt-
responses are dependent on the built-in electric field. ing of the Dirac cone is no longer important to obtain a finite
Considering the limit μ  β1 in Eqs. (9) and (10), the response. Depending upon the mirror symmetries present in
Wiedemann-Franz law and Mott relation allow us to compute the systems, one can find symmetry permitted components
MN conductivity α and Magnus thermal Hall (MTH) conduc- of nonlinear transport coefficients where di j becomes an even
tivity κ alternatively [65,68,69]: function of k [17,70,71]. By contrast, quantized nonlinear re-
sponse, namely circular photogalvanic effect, can be observed
π 2 kB2 T ∂σ π 2 kB2 T for mirror symmetry broken noncentrosymmetric systems
α=− , κ= σ. (11) [72,73].
3e ∂μ 3e2
Regarding the symmetry requirements to observe Magnus
Having discussed above the diffusive limit, we shall now ballistic transport, we note that the presence of crystalline
illustrate the Magnus responses in the ballistic regime. In this symmetries such as in-plane C2 and out-of-plane mirror can
regime, the mean free time between two collisions is infinite generate clean MH responses, nullifying other trivial linear
τ → ∞, i.e., essentially no collision occurs in the transport transverse signals [74]. Using these crystalline symmetries,
direction inside the length L along the x direction of the Hall it is also possible to categorize nonlinear anomalous Hall
bar. Therefore, the right hand side of the Boltzmann transport and Magnus Hall effects in different classes of material, in
equation given in Eq. (2) vanishes in the ballistic regime. In which time-reversal symmetry is preserved but inversion is
this setup, the carriers from the source with only positive ve- broken. To be more precise, the noncentrosymmetric point
locity vx > 0 are allowed in region 0 < x < L. Now the ansatz groups containing {C2z , C4z , C6z , S4z } symmetry operations
for the nonequilibrium distribution function is the following: force the BC to become zero, and as a consequence both MH
 conductivity and nonlinear Hall conductivity both vanish in
−μ∂ f0 − (k,r)−μ T ∂ f0 for vx > 0, these systems. Following the above analysis, crystallographic
f (k, r) = T
0 for vx < 0. point groups {C1 , C1h , C1v , C2 , C2v , C3 , C3h , C3v , D3h , D3 } (2D
(12) transition metal dichalcogenides such as WTe2 , MoS2 ) and
Comparing Eq. (8) and Eq. (12), one can identify the scatter- {O, T, Th } (particularly for 3D) allowing nonzero local BC can
ing length vx τ with the device length L so that −eLEx = μ lead to both MHE and nonlinear Hall effect in general [13,74].

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DAS, NAG, AND NANDY PHYSICAL REVIEW B 104, 115420 (2021)

We would also like to point out that at least one symmetry be written as [29]
between TRS and inversion symmetry has to be broken in g
the system. Although the previous studies only concentrate H0ML (k) = σz + ζ v1 kx σx + v2 ky σy , (15)
on TR invariant and inversion symmetry broken systems, 2
one can in principle get Magnus responses even in the absence where v1 and v2 = v1 are two strain-dependent Fermi veloci-
of TRS as long as the active momentum modes over the ties along x and y directions, respectively, g is the gap (also
Fermi surface have finite BC. This further motivates us to called Semenoff mass), ζ is the valley index, and σ ’s represent
study TRS broken topological systems in addition to the TRS Pauli matrices incorporating sublattice degrees of freedom. To
invariant topological systems. Since the strain, warping, and introduce the warping effect in the system, we add trigonal
tilt can modify the Fermi surface significantly as well as the warping terms, proportional to k 2 , in the Hamiltonian (15).
BC distribution accordingly, the Magnus responses can show Even though the magnitude of the warping term is smaller
interesting behavior which we discuss in the next section. compared to the leading order term in k, it plays a crucial role
It is important to note that along with Magnus Hall current, in MH responses. Now the complete Hamiltonian for the ML
there exists a trivial transverse current (regular Hall current) graphene in the presence of both uniaxial strain and trigonal
that arises from the transverse velocity anisotropy of the Fermi warping reads as [29]
surface: vx >0 dk vy (k) δ( k − μ). However, according to the
g
symmetry analysis given above, in the presence of certain mir- HML (k) = σz + ζ v1 kx σx + v2 ky σy + 2ζ λ3 kx ky σy
ror symmetry (specifically, mirror plane perpendicular to the 2
 
current direction) combined with time reversal symmetry, the + λ1 ky2 − λ2 kx2 σx = Nk · σ, (16)
trivial transverse current can be shown to vanish leaving a fi-
nite MH current [22,74]. In addition to the trivial Hall current, with Nk = {N1k , N2k , N3k } = {ζ v1 kx + (λ1 ky2 − λ2 kx2 ), v2 ky

linear anomalous Hall current induced by the nontrivial BC + 2ζ λ3 kx ky , 2g } and σ = {σ1 , σ2 , σ3 }. Here, λ1 , λ2 , and λ3 are
can appear simultaneously with MHE in time-reversal broken the warping terms. The energy dispersion of the Hamiltonian
systems. However, in contrast to MHE, linear anomalous Hall for ζ = ±1 valley is given by
response is not a Fermi surface phenomenon and, therefore,
does not depend on the derivative of the Fermi function. These E ML (k) = |Nk | = ± N1k
2 + N2 + N2 ,
2k 3k
(17)
two effects can be distinguished by looking at their chemical
potential dependencies in experiments. We will discuss these where +(−) represents a conduction (valence) band. The
issues elaborately in Sec. III D. warping results in nonlinearity and strain causes anisotropy
in the dispersion. The BC reads as
 k 
Nk · ∂N
∂kb
× ∂N k
∂kc
a (k) = abc ,
III. RESULTS (18)
4|Nk |3
In this section, we discuss the effect of strain and warping
on MH and MN conductivities in inversion symmetry broken where abc is the usual Levi-Civita symbol.
but TRS invariant 2D topological systems, namely for ML, BL Since ML graphene is a two-dimensional system, only the
graphene, and surface states of TI. We extend our analysis in z component of the BC is nonzero. Using Eq. (18), the BC
3D topological systems WSMs, breaking either TRS or inver- for strained ML graphene (ζ = ±1) given in Eq. (16) can be
sion symmetry, to investigate the effect of tilt and nonlinearity calculated as
on MHE and MNE. At the outset, we note that we will often
z (k, ζ )
ML
refer to MH and MN conductivities together as MH responses.  
g ζ v1 v2 + 2kx (λ3 v1 − λ2 v2 ) − 4ζ λ3 λ2 kx2 + λ1 ky2
=± ,
4[E ML (k)]3
A. Strained monolayer graphene
(19)
The graphene hosts gapless Dirac cones, located at the high
symmetry points K and K in the Brillouin zone, with vanish- where +(−) represents conduction (valence) band. Now the x
ing BC. A finite BC is generated by breaking the inversion component of the velocity of ML graphene can be written as
symmetry that can be engineered by placing the graphene 2ζ λ3 ky N2k + N1k (ζ v1 − 2λ2 kx )
sheet on a hBN substrate [75,76]. This actually reduces the vxML (k, ζ ) = ± . (20)
E ML (k)
point group of the system from C6v to C3v , and opens up a
gap at the Dirac nodes. Upon applying a uniform uniaxial We first consider strained ML graphene v1 = v2 without
strain along one of the two main crystallographic directions warping, i.e., λ1 = λ2 = λ3 = 0. It is then clear from Eq. (19)
in graphene, the massive Dirac nodes become shifted from that the BC at two different valleys (ζ = ±1) become op-
the high symmetry points along the ky = 0 line due to the posite of each other for both pristine as well as strained

ML graphene, i.e., ML z (K, ζ = +1) = − z (K , ζ = −1).
ML
combination of TRS and mirror symmetry. The application
of the strain creates a difference between hopping amplitudes Moreover, the BC in this case is directly proportional to
along the two main crystallographic directions and, therefore, the band gap of the system. On the other hand, vxML (K, ζ =
changes the corresponding Fermi velocities [29,77]. +1) = vxML (K  , ζ = −1) as evident from Eq. (20).
Considering only first-order momentum-strain coupling, The above discussion refers to the fact that there exists an
the low-energy Hamiltonian of the ML strained graphene can equal number of k modes for which vxML > 0 with both signs

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TOPOLOGICAL MAGNUS RESPONSES IN TWO- AND … PHYSICAL REVIEW B 104, 115420 (2021)

FIG. 1. Evolution of BC and Fermi surface in ML graphene (16) with warping λ1 = λ2 = λ3 = λ and strain v2 = v1 . Top panel: the BC
z (k, ζ = +1)] and x component of the velocity [vx (k, ζ = +1)] over the Fermi surface are shown for (a) unstrained ML graphene without
[ ML ML

warping (v2 = v1 , λ = 0) and strained ML graphene (v2 = 2v1 ) with C3 symmetric warping of different strengths (b) λ = 0.2, (c) λ = 0.35,
and (d) λ = 0.5 eV Å2 . Bottom panel: (e)–(h) depict ML z (k, ζ = −1) and vx (k, ζ = −1). The strength of
ML
z (k, ζ ) and vx (k, ζ ) are
ML ML

represented in the color codes side by side. The parameters (in the units of energy eV) used in the calculations are g = 0.06 eV and v1 = 0.87
eV Å. The Fermi surface is plotted for the constant energy E = −0.28 eV.

of (k) in each valley. Upon the momentum integration fol- case. The evolution of BC and vxML for different strengths
lowed by Eqs. (13) and (14), the MH and MN conductivities of λ are depicted in Figs. 1(b)–1(d) and Figs. 1(f)–1(h) for
for each valley in the ballistic regime can be obtained as ζ = 1 and ζ = −1 valleys, respectively. The warping terms
introduce satellite Dirac cones with θ → θ + 2nπ /3 (with
ge2 gπ KB2 Te
σζ = ζ U, αζ = ζ U. (21) n = 1, 2, 3) appearing around each Dirac point [81]; here
8h̄π μ2 12h̄μ3 θ = π (0) for valleys ζ = +1 (−1). These additional satellite
Interestingly, the above conductivities are independent of ve- Dirac cones appear with opposite chirality as compared to that
locities v1 and v2 . This leads to the fact that the uniaxial of the parent Dirac cone. The important point to note here is
strain does not affect the MH responses in ML graphene that the relative strength between v1 and v2 determines the dis-
in the absence of warping λ1,2,3 = 0. Moreover, it is also tance of satellite Dirac points from the parent Dirac point. For
clear from Eq. (21) that the contributions of MH and MN example, v1 > v2 (v1 < v2 ) would cause the satellite Dirac
conductivities for two valleys (ζ = ±1) are equal and oppo- points to move more (less) in kx direction more (less) than
site. Therefore, summing over the valleys (ζ = ±1), the total ky direction.
MH responses vanish in the strained ML graphene without Following the above discussion, it is evident that each val-
λ’s, similar to the case of pristine ML graphene. Instead the ley of ML strained graphene in the presence of warping does
valley polarized transport can lead to Magnus valley Hall not contribute to MH and MN conductivities in an equal and
and Magnus valley Nernst effects, where the electrons with opposite manner that we found for strained ML graphene. As
opposite valley index accumulate on the different edges of the a result, the nonzero MH responses are directly observed by
sample [78–80]. To be precise, considering a ML graphene summing over the contribution for both valleys. The warping
system (with λ1,2,3 = 0) with chemical potential (μ + δμ/2), results in nonlinear and anisotropic dispersion as shown in
(μ − δμ/2) at the ζ = ±1 valleys, respectively, the total Mag- Eq. (17). As a result, BC becomes anisotropic and exhibits
nus valley Hall conductivity will be finite and takes the form rich features over the Fermi surface (see Fig. 1). Since the
 e2 U δμ expressions of BC and velocity of ML graphene in the pres-
σvalley = ζ σζ (μ + ζ δμ/2)  g4h̄πμ3 . Similarly, Magnus
ence of warping are quite complicated, it is very difficult to
valley Nernst conductivity is given by αvalley = ζ αζ (μ +
calculate MH and MN conductivities analytically. Therefore,
 πK 2 TeU δμ
ζ δμ/2)  g 4Bh̄μ4 . We note that, in order to observe the below we have calculated Magnus responses numerically to
above valley polarized ballistic Magnus response, the dimen- investigate in detail.
sion of the system has to be smaller or comparable to the mean The valley integrated MH and MN conductivities as a
free path. function of chemical potential (μ) are shown in Figs. 2(a) and
We shall now discuss the effect of C3 symmetric warping 2(b), respectively. We find that the magnitude of both transport
in MH responses by considering λ1 = λ2 = λ3 = λ = 0. It is coefficients enhances with the increase of warping strength
clear from Eqs. (19) and (20) that the BC and velocity of each for a fixed strain. The window of activated momentum
valley are not equal and opposite compared to the unwarped modes over the Fermi surface changes with warping strength.

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DAS, NAG, AND NANDY PHYSICAL REVIEW B 104, 115420 (2021)

shown in Eq. (17). As a result, BC becomes anisotropic and


exhibits rich features over the Fermi surface.

B. Strained bilayer graphene


The BL graphene belongs to the D3d point group symme-
try. In order to study the BC mediated transport properties, one
has to break the inversion symmetry by applying an external
electric field perpendicular to the layers. This reduces the
symmetry of the system from D3d to C3v , and creates a gap
g as well as finite BC. The application of a uniaxial strain
further reduces the symmetry of the point group to Cv . The
low energy Hamiltonian for an inversion broken BL graphene
in the presence of a uniaxial strain is expressed below as [29]
 
g 1  2 
H0BL (k) = σz + − ky − kx2 + ζ vkx + ω σx
2 2m
 
1
− kx ky + ζ vky σy , (22)
m
where v denotes the Fermi velocity related to the skew
hopping between the layers, ζ is the valley index, and m rep-
resents the effective mass dependent on the coupling between
the layers. Here, the effect of strain is coming into the Hamil-
FIG. 2. Total valley summed contributions of (a) MH conductiv- tonian via ω (= A3 − A0 ), where A3 and A0 are pseudogauge
ity σ (in the unit of 10−3 e2 /h̄) and (b) MN conductivity α (in the
fields. Similar to the ML case, we add trigonal warping terms
unit of 10−5 ekB /h̄) in the presence of strain (v2 = 2v1 ) for different
to the above Hamiltonian to study its effect. The strained-
warping strengths λ = 0.2, 0.35, and 0.5 eV Å2 are shown for ML
warped BL graphene Hamiltonian takes the following form:
graphene. Noticeably, the warping can enhance the responses even

after valley sum is performed, as it generates asymmetric contri- g 1  2   
butions between valleys. We consider U = 0.01 eV and kB T = HBL (k) = σz + − ky − kx2 + λ1 ky2 − λ2 kx2
2 2m
0.001 eV. All other parameters are kept the same as those in Fig. 1.   
The chemical potential μ is chosen in the unit of eV throughout the 1
paper.
+ζ vkx + ω σx − kx ky + ζ vky − 2ζ λ3 kx ky σy
m
= Nk · σ, (23)
Moreover, band bending imprints its signature through the with Nk = {N1k , N2k , N3k } = {(λ1 − 1
)k 2
2m y
+ ( 2m
1
− λ2 )kx2 +
Fermi surface distribution. All these lead to the intriguing 
ζ vkx + ω, (2ζ λ3 − m1 )kx ky − ζ vky , 2g }. The energy disper-
behavior of the response coefficients. We find that MH re-
sion of the Hamiltonian given in Eq. (23) can be obtained as
sponses show significantly different behaviors for v1 > v2 as
compared to v2 > v1 . This refers to the fact that the strain
becomes instrumental in controlling the response in the pres-
E BL (k) = |Nk | = ± N1k
2 + N2 + N2 .
2k 3k
(24)
ence of warping terms. We would like to point out that the
MH and MN conductivities can acquire both positive and Note that, in Eq. (23), the warping terms are quadratic
negative values. This is due to the fact that the BC around in momentum, and hence could be absorbed in the already
the additional satellite Dirac points take opposite values as present quadratic momentum terms which indicate interlayer
compared to that of the parent Dirac point. These are the coupling. In this way, the effective masses associated with
markedly different responses, while the warping terms are kx2 , ky2 , and kx ky terms are renormalized. Therefore, we can
introduced in the ML strained graphene. Our study further comment at the outset that addition of warping might not
supports that the Mott relation can successfully describe MN affect the system substantially as compared to strain in the
conductivity from MH conductivity even in the presence of ML graphene.
warping. Considering C3 symmetric warping (λ1 = λ2 = λ3 = λ =
In summary, for monolayer graphene without strain and 0), the BC for strained BL graphene given in Eq. (23) can be
warping, the MH and MN conductivities for two valleys are calculated as
equal and opposite and therefore, summing over the valleys,
the total MH responses vanish [23]. On the other hand, we g[A(λ, kx )A(λζ , kx ) + B(λ, ky )B(λζ , ky )]
z (k, ζ ) =∓ ,
BL
show that each valley of monolayer strained graphene in the 4[E BL (k)]3
presence of warping does not contribute to MH and MN con- (25)
ductivities in an equal and opposite manner, and hence leads to
k
a finite valley integrated MH response. This happens because with A(x, kx ) = kmx − 2xkx + ζ v and B(x, ky ) = my − 2xky ,
the warping results in nonlinear and anisotropic dispersion as where −(+) represents the conduction (valence) band. The

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velocity vxBL (k, ζ ) takes the form

A(λ, kx )N1k − B(λζ , ky )N2k


vxBL (k, ζ ) = ± . (26)
E BL (k)

A close inspection suggests that the strain factor w does not


appear in the numerator of BC for BL graphene, unlike the
ML graphene where warping factors λ’s come as corrections
over the strain factors v1 v2 . The strain factor comes in the
denominator of BC through the energy of the BL graphene.
Therefore, the evolution of BC with strain for BL graphene
will be significantly different from ML graphene.
The evolution of the BL z (k, ζ ), vx (k, ζ ), and Fermi sur-
BL

face under strain for valley ζ = +1 and valley ζ = −1 are


shown in the left and right column of Fig. 3, respectively. For
w = 0, the three leg gapped Dirac cones (one along ky = 0
and the other two symmetrically placed around the kx = 0
line) are observed at θ → θ + 2π /3 with θ = 0 following the
C3 symmetric warping [82]. The BC does not change its sign
for the three leg gapped Dirac cones within a given valley.
This structure of BC for BL graphene is very different from
the ML graphene, where BC around satellite Dirac nodes
reverses its sign as compared to the parent Dirac node within
a given valley. For w  −3m, there exist two symmetrically
placed Dirac cones around the ky = 0 line, while two cones
appear on the ky = 0 line for w  3m. The threefold rotational
symmetry is lost in the presence of uniaxial strain. Interest-
ingly, the Fermi surface is also deformed for the strained case
from its unstrained triangular distribution. To be precise, a
singly connected Fermi surface for the unstrained case splits
into disconnected ones for sufficiently large values of strain.
The shape and orientation of the Fermi surfaces appear to be
different for larger strain in opposite valleys, which leads to
nonidentical MH responses in these valleys.
We now investigate the MH and MN conductivities for
the individual valleys as shown in Figs. 4(a) and 4(b), re-
spectively. The unstrained case leads to asymmetric response
in the valleys which is markedly different from ML strained
graphene without warping. Upon inclusion of strain, we find
that the positive MH responses for the valley ζ = +1 are more
pronounced than the negative responses for the other valley
ζ = −1. This is due to the fact that activated momenta over
the Fermi surface do not have exactly opposite BC in terms
of their magnitudes and sign. Moreover, the peak or dip of
MHC do not appear at the same chemical potential μ. The
Fermi surface distribution strongly depends on valley as well
as strain explaining the above observation for MH responses.
Therefore, valley polarized transport can in principle be pos-
sible like ML strained graphene.
The total valley integrated Magnus responses for BL
graphene are shown in Fig. 5 by varying strain parameter
w. For negative values of strain parameter, i.e., w < 0, MH FIG. 3. Evolution of BC and Fermi surface in BL graphene (23)
conductivity always acquires negative values and a dip ap- with strain w for warping λ1 = λ2 = λ3 = λ = 0.001 eV Å2 . Left
pears at a certain μ value. The height of the dip increases and column: the BC BL z (k, ζ = +1) and vx (k, ζ = +1) over the Fermi
BL

its position moves toward μ → 0 with decreasing negative surface of BL graphene (a) w = −3m, (c) w = −m, (e) w = 0,
strain. On the other hand, by changing the sign of strain, i.e., (g) w = m, and (i) w = 3m are shown. Right column: we repeat
w > 0, the dip structure of MH conductivity gets bifurcated the same set of calculations for ζ = −1 valley. The parameters (in
into a dip and peak structure. The valley polarized structure the units of eV) used are g = 0.06 eV, m = 0.008 eV Å2 , and
of MH responses can explain these observations. We notice v = 0.5 eV Å. The Fermi surface is plotted for the constant energy
qualitatively similar response in MN conductivity. E = −0.04 eV.

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In summary, for bilayer graphene, we find that strain en-


hances asymmetry between the valley polarized contribution,
resulting in distinct transport signatures for positive and neg-
ative strain as compared to the unstrained bilayer graphene.

C. Hexagonal warped topological insulator


We consider the two-dimensional surface Hamiltonian of
a TRS invariant TI namely, Bi2 Te3 , hosting a unique Fermi
surface that encloses an odd number of Dirac cones in the sur-
face Brillouin zone. The spin-orbit coupling that is the linear
order term in k leads to the band inversion in this system. The
minimal two band model contains cubic terms in k in addition
to the linear terms in k. This warping can be considered as a
counterpart of the cubic Dresselhaus spin-orbit coupling term.
We note that hexagonal warping incorporates one order higher
momentum coupling than the trigonal warping terms. This
further allows us to investigate the nontrivial effects of this
term that are not captured by the trigonal warping terms.
Considering the threefold rotation C3 around the z axis and
mirror symmetry M: x → −x, the low-energy model around
the gapless  point thus reads [31]
λ 3
H HW (k) = E0 (k) + v(kx σy − ky σx ) + (k + k−3 )σz , (27)
FIG. 4. Valley responses of (a) MH (in the unit of 102 e2 /h̄) and 2 +
(b) MN (in the unit of 10−1 ekB /h̄) conductivities in BL graphene 2
where E0 (k) = 2mk
∗ causes the particle-hole asymmetry. Dirac
with U = 0.01 eV, and kB T = 0.001 eV for w = −3m, 0, 3m. All
other parameters are kept the same as those in Fig. 3. The prominent
velocity v can be considered k independent without loss of
and asymmetric valley responses in the presence of strain for BL generality. Here k± = kx ± iky and λ is the strength of hexag-
graphene are markedly different from the symmetric responses for onal warping.
ML graphene. The energy spectrum becomes
E HW (k) = E0 (k) ± v 2 k 2 + λ2 k 6 cos φ, (28)
k
where φ = arctan kxy . Using Eq. (18), the BC and x component
of the velocity for the above Hamiltonian can be obtained as
 
λv 2 3kx ky2 − 2kx3
z (k) = ± 3 ,
HW
(29)
2(v 2 k 2 + λ2 k 6 cos φ) 2
kx 2v 2 kx + λ2 k 3 ky2 + 6λ2 k 4 kx cos φ
vxHW (k) = ± , (30)
m∗ 2 v 2 k 2 + λ2 k 6 cos φ
where +(−) represents the conduction (valence) band. The
band structure is sixfold symmetric under φ → φ + 2π /6.
It is clear from Eq. (29) that the BC is zero in the absence
of warping. The band structure is sixfold symmetric under
φ → φ + 2π /6. The BC distribution with different strengths
of warping parameter is depicted in Fig. 6. The BC always
shows a snowflakelike distribution irrespective of the strength
of warping. However, the BC acquires a substantially large
value around the  point with increasing λ as also suggested
from Eq. (29). Moreover, it reverses sign between two sub-
sequent intervals 2nπ /6 → 2(n + 1)π /6. On the other hand,
the shape of the Fermi surface changes with warping. Specif-
ically, for small warping the Fermi surface takes a circular
shape. With increasing warping strength, it becomes noncircu-
lar with relatively sharp tips extending along a high symmetry
FIG. 5. Valley summed (a) MH (in the unit of 10e2 /h̄) and direction and curves inward in between. Such transformation
(b) MN (in the unit of 10−2 ekB /h̄) conductivities in BL graphene of the Fermi surface from circular to snowflake would initiate
for w = −3m, 0, 3m. The transport behavior changes with strain interesting transport behavior which we discuss below.
substantially. We consider the same parameters as those used in The MH and MN conductivities as a function of chemi-
Fig. 4. cal potential for different strengths of warping parameter are

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FIG. 6. Evolution of BC and Fermi surface, calculated from Eq. (27), with different warping strengths (a) λ = 50 eV Å3 , (b) λ = 200
eV Å3 , and (c) λ = 400 eV Å3 are shown. Fermi surface is plotted for E = −0.05 eV. We note that, for λ = 50 eV Å3 , the Fermi surface
remains circular, which gradually evolves to hexagonal shape with increasing λ. We consider v = 1 eV Å and E0 = 0 in our calculation.

shown in Figs. 7(a) and 7(b), respectively. We find that the analog of graphene [83]. The low-energy effective Hamilto-
magnitude of the MH responses are increasing as well as nian describing the Weyl node with topological charge n and
becoming more pronounced and sharp with the increase of chirality ζ is written as [44,45,84,85]
warping strength. In addition, the position of the dips (peaks)
in MH (MN) conductivities moves toward μ = 0 with increas- Hkζ = Cζ (kz − ζ Q) + ζ αn σ · (nk − ζ e), (31)
ing λ. Moreover, the negative sign of MH conductivity appears √
where ζ = ±1, k⊥ = kx2 + ky2 , φk = arctan(ky /kx ), and e =
because of the majority of negative BC over the activated (0, 0, Q). The Weyl nodes of opposite chirality are shifted
momentum modes in the Fermi surface. by an amount ±Q in momentum space due to broken
TRS. Cζ indicates the tilt parameter associated with the
D. Weyl semimetals Weyl node with chirality ζ . Here, σ = {σx , σy , σz } and nk =
Going beyond the 2D systems, we will now calculate MH {αn k⊥n cos(nφk ), αn k⊥n sin(nφk ), vkz }. The factor αn bears the
responses in 3D WSMs which can be thought of as a 3D connection to the Fermi velocity. v is equivalent to the velocity
associated with the z direction. For the sake of simplicity,
we consider Q = 0 and take into account the Weyl nodes of
opposite chirality separately. For Cζ = 0, electron and hole
bands touch at the Weyl point leading to a pointlike Fermi
surface. When the magnitude of the tilt parameter is small
enough, i.e., |Cζ |/v 1, the Fermi surface is still pointlike
and is characterized as the type-I Weyl node. With the increase
of Cζ , electron and hole pockets now appear at the Fermi
surface for |Cζ |/v  1 leading to a distinct phase, which is
designated as a type-II Weyl node. In this work, we consider
two types of tilt configuration for the WSM: (i) chiral tilt, i.e.,
C+ = −C− , and (ii) achiral tilt, i.e., C+ = C− .
Now the energy dispersion of the multi-Weyl node with
ζ = +1 is given by
E W SM (k, ζ ) = Cζ kz ± k, (32)

where k = αn2 k⊥2n + v 2 kz2 and +(−) represents the conduc-
tion (valence) band. It is now clear that the dispersion around a
Weyl node with n = 1 is isotropic in all momentum directions.
On the other hand, for n > 1, we find that the dispersion
around a double (triple) Weyl node becomes quadratic (cu-
bic) along both kx and ky directions, whereas varies linearly
with kz .
Using Eq. (18), the explicit form of z-component BC asso-
ciated with the multi-Weyl node can be written as
FIG. 7. (a) MH (in the unit of 10−2 e2 /h̄) and (b) MN (in the unit 1 ζ n2 vαn2 k⊥2n−2
of 10−4 ekB /h̄) conductivities as a function of chemical potential for
W SM
z (k, ζ ) =± 3
kz . (33)
2 k
different warping strengths λ = 50, 200, and 400 eV Å3 are depicted.
The parameters used are v = 1 eV Å, U = 0.01 eV, and kB T = It is clear from Eq. (33) that, similar to energy dispersion,
0.001 eV. the BC is isotropic in all momentum directions for single

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FIG. 8. Distribution of the BC and the Fermi surfaces, calculated from Eq. (31), in (a) [(d)] single Weyl node with n = 1, (b) [(e)] double
Weyl node with n = 2, and (c) [(f)] triple Weyl node with n = 3 for the untilted case, i.e., C+ = 0 [tilted case, i.e., C+ = 2.0] are shown. The
Fermi surface is calculated for E = −0.05 eV with v = 1 eV Å. The deformation of BC is clearly observed with increasing nonlinearity and
anisotropy in the WSM.

WSM, whereas it becomes anisotropic for WSMs with n > 1, Fig. 9. Interestingly, we find that both MH and MN conductiv-
i.e., for double WSM (n = 2) and triple WSM (n = 3) due to ities vanish identically for an untilted Weyl node. This is due
the presence of k⊥2n−2 factor and topological charge n. More- to the fact that, for a given untilted Weyl node, the positive
over, the BC reverses its sign, retaining the magnitude same, and negative BC for the activated momentum modes over the
for Weyl nodes of opposite chiralities W z
SM
(k, ζ = +1) =
− W z
SM
(k, ζ = −1). The behavior of BC for both untilted
(Cζ = 0) and tilted (Cζ = 0) multi-Weyl nodes with ζ = +1
are shown in Fig. 8. With increasing the topological charge n,
the single positive and negative lobe of BC gets divided into
one pair of lobes. These lobes for n = 2 and 3 are deformed
with respect to that of n = 1. The separation between these
lobes increases over the kz = 0 line. The BC changes sign
with the chirality of the Weyl node for all WSMs as indicated
in Eq. (33). However, the BC is identical in both tilted and
untilted WSMs because the tilt does not affect BC. On the
other hand, in contrast to BC, the Fermi surface drastically
changes in tilted WSM compared to untilted WSM as shown
in Fig. 8.
The x component of the quasiparticle velocity associated
with the multi-Weyl node is given by
kx nαn2 k⊥2n−2
vxW SM (k, ζ ) = . (34)
k
A close inspection suggests that the x component of the
velocity is also independent of the tilt parameter Cζ (chirality
ζ ) like (unlike) the BC. Therefore, the effect of the tilt is only
incorporated by the Fermi surface properties. The Fermi sur-
face for the n = 1 case is circular in shape that gets elongated
along the kx direction with increasing n. In the kx − kz plane, FIG. 9. (a) MH (in the unit of 10e2 /h̄) and (b) MN (in the unit
the Fermi surface does not close which is in accordance with of ekB /h̄) conductivities are shown for tilted and untilted Weyl nodes
the nonpointlike nature of the Fermi surface for tilted WSM. with ζ = +1. We consider v = 1 eV Å, U = 0.01 eV, and kB T =
With increasing topological charge n, the Fermi surface gets 0.001 eV. We observe that the untilted Weyl node with C+ = 0
flattened. Therefore, tilt and nonlinear dispersion imprint their (tilted Weyl node with C+ = 0.6) results in null (substantial) Magnus
signature in the transport through Fermi surface properties. responses. We note that MH and MN conductivities are exactly
The numerically computed MH responses for single, dou- opposite at two opposite Weyl nodes with ζ = +1 and −1 owing
ble, and triple Weyl nodes as a function of μ are shown in to the antisymmetric nature of BC [Eq. (33)].

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the presence (absence) of warping. From a low energy model,


it can be shown that the node integrated MH responses are
proportional to that of a single tilted Weyl node. All these
findings together refer to very interesting Magnus transport
properties of WSM in general.
It is pertinent to discuss the anomalous Hall effect that
will present alongside the MHE for the TRS broken WSM as
far as the first order responses are concerned. The anomalous
Hall conductivity for type-I mWSM is found to be σ  ∝ nk,
where k is the separation between two Weyl nodes in mo-
mentum space of opposite chirality [64,86]. On the other
hand, the MHE in type-I mWSM (|Cζ /v| 1) for a given
FIG. 10. MH (in the unit of 10e2 /h̄) conductivity is shown for chemical potential can be analytically found as σ ∝ n U v
. It
different strengths of the tilting parameter (C+ ) for fixed n = 1. Grad- is clear from the above expressions that the intrinsic AHE in-
ual increase in the response is observed with increasing tilt strength creases with increasing the k-space separation between Weyl
C+ . All other parameters are kept the same as those mentioned in nodes while remaining insensitive to the tilt parameter. By
Fig. 9. contrast, the magnitude of MH conductivity increases with
increasing the built-in electric field. Using the above ex-
pressions, one can in general find σσ ∝ vk U
(in an arbitrary
Fermi surface are equal, which results in a complete cancel- unit) for type-I WSM. Since this comparison is based on the
lation. This situation remarkably changes in the presence of low-energy model of mWSM, one should consider the lattice
a tilted Weyl node. In this case, the positive and negative BC model to make a correct estimate of σσ . In addition, we would
for the activated momentum modes over the Fermi surface are like to point out that the intrinsic linear AHE can in principle
unequal and, therefore, do not cancel each other completely. be found to be quantized, while MHE is not expected to
The MH conductivity of a tilted WSM, considering the exhibit a quantized response [87].
contribution from two opposite chirality nodes, is given by
σ = ζ G(μ)ζCζ , where G(μ) is the μ dependent part of a
IV. CONCLUSIONS
transport coefficient associated with an individual Weyl node.
For a pair of Weyl nodes at the same energy E0 such that In conclusion, we first investigate the effect of strain and
G(μ = E0 ) = G0 , the MHE is only finite when relative sign warping on MHE and MNE in a ballistic regime for 2D topo-
of the tilt parameter between them is opposite, referring to the logical systems such as ML, BL graphene, and surface states
chiral tilt configuration (C+ = −C− ). On the other hand, the of TIs. We find that, in a strained ML graphene system without
MHE vanishes in the absence of tilt (C+ = C− = 0), and even warping, the total Magnus responses are zero after summing
in the presence of achiral tilt (C+ = C− ) of the Weyl node. In over the valleys because the contribution from each valley
other words, MH responses from an opposite Weyl node add cancels each other. One instead obtains Magnus valley Hall
up (cancel each other) leading to a node integrated (polarized) and Magnus valley Nernst effects from the valley polarized
Magnus (Magnus valley) response in the presence of chiral contribution. Interestingly, we find that the warping leads to
(achiral) tilt. Two Weyl nodes of opposite chirality, residing finite total Magnus responses as BC contributions from each
at two different energies E+ and E− , can in principle lead valley to Magnus responses are unequal and do not cancel
to the Magnus valley Hall effect, while Weyl nodes exhibit each other for the asymmetric nature of the Fermi surface
achiral tilt such that G(μ = E+ ) = G(μ = E− ). The MNE shape. The magnitude of the total Magnus responses is found
follows the same behavior as MHE. This is because the sign to increase with increasing the strength of the warping param-
of BC is opposite, whereas the vxW SM has the same sign for eter. For BL graphene, strain enhances asymmetry between
two different nodes of opposite chirality. To shed more light the valley polarized contribution resulting in distinct transport
into the tilt mediated MH response, we show the systematic signatures for positive and negative strain, while the effect of
growth of MH conductivity while increasing the tilt strength warping remains minimal. In the case of surface states of TI,
in Fig. 10. we find that the magnitude of both MH and MN conductivities
Therefore, the MH and MN conductivities can become are enhanced with increased hexagonal warping strength.
useful probes in distinguishing tilted WSM from an untilted Going beyond 2D, we study Magnus responses in the
WSM in experiments. We also notice that the responses for ballistic regime for 3D Weyl semimetals using a low-energy
n = 1 single WSM are found to be most prominent as com- model to probe the effect of tilt and anisotropic nonlinear
pared to the WSMs with n > 1. This can be explained as the dispersion. In particular, we find that the MHE is identi-
BC reduces its value for the activated momentum modes over cally zero for each Weyl node without tilt, whereas for tilted
the Fermi surface. Moreover, the MH responses decrease as WSMs, Magnus responses coming from the nodes acquire
the Fermi surface becomes more flattened for mWSMs. An- finite values. Notably, MH responses from an opposite Weyl
other interesting feature, coming out from Eqs. (33) and (34), node add up (cancel each other) leading to a node integrated
is that MH responses from two opposite nodes with chiral (polarized) Magnus (Magnus valley) response in the presence
(achiral) tilt simply add up (cancel each other) leading to a of chiral (achiral) tilt. The magnitude of both MH and MN
finite node integrated (polarized) transport coefficient similar conductivities increases with increasing the tilt parameter of
to the Magnus (Magnus valley) responses for ML graphene in the Weyl nodes. Moreover, with increasing the topological

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DAS, NAG, AND NANDY PHYSICAL REVIEW B 104, 115420 (2021)

charge associated with the Weyl node, the Magnus responses performed. In the case of MHE, the choice of suitable gate
get suppressed. This key feature can be a useful probe in dis- potentials, causing the built-in electric field, becomes very
tinguishing untilted (type-I), tilted (type-I or type-II) WSM, important to generate the appropriate transverse Hall voltage.
and the nonlinearity in the dispersion through experiments. In contrast to the linearized model we use in this work,
Moreover, from the application point of view, such MH re- a real mWSM may contain Weyl nodes with different tilt
sponses can pave the way for a new generation of current with respect to one another, as well as a number of pair of
rectification devices where the alternating-current signal is nodes that can be greater than one. One of the interesting
converted into a direct-current signal. This is due to the fact extensions of this work would be to implement the MH re-
that linear Hall effects, the transverse MH voltage (say in sponses’ calculation on a real mWSM material using DFT
y direction) is developed due to the Magnus velocity of the or at least on a lattice model in order to directly compare
carriers having positive longitudinal velocity (vx > 0) only. with the experiments. For this purpose, one can perform a
Related to the experimental realization of MH response in four terminal Landauer-Büttiker conductance calculation [98]
3D, we would like to first point out that the bulk quantum Hall on a lattice. Following our theoretical analysis on mWSMs,
effect has been realized earlier in quasi-2D systems [88–91]. we expect MH responses to be negligible for materials like
Recently, 3D systems, such as ZrTe5 , HfTe5 , and Cd3 As2 , NbAs and TaAs, which have symmetric untilted Weyl cones.
have been shown to exhibit the quantum Hall effect in ex- On the other hand, type-II Weyl materials (MoTe2 and WTe2 )
periments [92–95]. Moreover, the nonlinear Hall effect has can show substantial MH responses. Moreover, investigating
already been experimentally observed in bilayer nonmagnetic MH responses in twisted BL graphene would be an interesting
quantum material WTe2 [15], in few layers of WTe2 [96], direction which we leave for future study.
and in type-II WSM at room temperature [97]. In light of
the above experiments, it is in principle possible to extend the
ACKNOWLEDGMENTS
nonlinear Hall effect setup, fabricated in 2D, to 3D platforms,
where MHE can be experimentally observed. For example, 2D S.N. acknowledges the National Science Foundation Grant
systems can be stacked together in order to form quasi-2D/3D No. DMR-1853048. S.K.D. would like to thank U. Nitzsche
structure over which multiterminal Hall measurements can be for technical assistance.

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