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Application of dry covers for the closure of tailings facilities

Article in Land Contamination & Reclamation · April 2007


DOI: 10.2462/09670513.849

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Land Contamination & Reclamation, 15 (2), 2007 © 2007 EPP Publications Ltd

DOI 10.2462/09670513.849

Application of dry covers for the closure of tailings


facilities
E. Mylona, A. Xenidis, M. Csövári and G. Németh

Abstract
The design and construction of a cover system represents a major issue in tailings facilities closure.
A dry cover system mainly aims to minimize water infiltration and/or inhibition of oxygen diffusion to
the underlying waste in order to control acid rock drainage production and metals leaching. Further-
more, dry covers should be resistant to water and wind erosion and provide support for vegetation.
They can be simple or complex, ranging from a single layer of earthen material to several layers of
different material types, including native soils, geosynthetic materials, inactive tailings and/or waste
rock, and organic materials. Different types of dry covers implemented at tailings facilities are
reviewed in this paper. Factors affecting the cover design and dictating the long-term performance
are discussed. Alternative covers aiming at acid rock drainage control by the incorporation of reac-
tive layers containing alkaline and/or cementitious materials are also described. Finally, a case
study, involving the design and application of a multilayered cover in the reclamation of uranium tail-
ings ponds in Pécs, Hungary, is presented.

Key words: closure, dry covers, Pécs, tailings facilities, uranium tailings

INTRODUCTION years it has been increasingly recognized that for a min-


ing project to contribute positively to an area’s develop-
Mining operations are finite economic activities, which
ment in any lasting way, closure objectives and impacts
are usually relatively short term. The tailings that
must be considered from project inception. The tailings
remain after the mining of an ore deposit has been com-
facility needs to be engineered for closure, so that sta-
pleted are often the most visible remaining signs of the
bility and environmental performance criteria can be
mining activity. The tailings or mine waste disposal
achieved.
facility has proven to be the most contentious compo-
In recent years, there have been a number of studies
nent of mining activities, and has represented the source
to consider the standards to be achieved on closure in
of significant environmental and economic impacts
the USA, Canada, Australia and, most recently, in
due, in the majority of cases, to poor management. The
Europe. The fundamental mine closure design criteria,
primary aim in the past has been to provide a well-engi-
as described in the study by MIRO (1999), involve sev-
neered structure into which the tailings can be depos-
eral issues, such as physical, chemical and biological
ited without a great deal of attention being given to
stability, hydrology and hydrogeology, geographical
closure requirements or issues related to long-term
and climatic influences, local sensitivities, land-use,
management of the storage facility. In the past 20 to 30
financial assurance and socio-economic considerations.
A requirement to draw up closure plans for mine
Received November 2006; accepted February 2007 waste management facilities in order to ensure that clo-
sure operations form an integral part of the operator’s
Authors
E. Mylona,1 A. Xenidis,1* M. Csövári2 and G. Németh2 overall exploitation plan is contained in the recent
1. Laboratory of Metallurgy, National Technical University of European Directive 2006/21/EC on the ‘Management
Athens, Greece
2. MECSEK ÖKO Rt., Pécs, Hungary of waste from extractive industries and amending
* Corresponding author. Email axen@central.ntua.gr Directive 2004/35/EC’. In Article 12, the tasks that

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Land Contamination & Reclamation / Volume 15 / Number 2 / 2007

have to be carried out by the operator, and the role of infiltration);


the competent authority in supervising closure and • minimize radon emission from uranium tailings;
aftercare procedures, are laid out. The operator shall and
control the physical and chemical stability of the facil- • provision of a growth medium for the establishment
ity and minimize any negative environmental effects, of vegetation.
in particular with respect to surface and groundwater.
The reclamation of tailings impoundments com- On the basis of design objectives, the various types
monly involves the placement of dry or water covers of tailings covers can be classified in three categories
over the tailings. Cover design is site-specific, depend- (Elander et al. 1998; DeVos et al. 1999; Ritchie 1999):
ing on the climatic conditions, material availability and
the sensitivity of the receiving environment. • low water flux covers that aim to inhibit infiltration
to the waste. Covers of this type include the low-
A water cover is often the method of choice for
permeability cover (water-shedding cover), the cap-
reclaiming tailings, which are potentially acid generat-
illary barrier and the store and release or eva-
ing. The tailings voids remain permanently water-filled
potranspiration cover;
and thus unavailable to oxygen, while a water depth of
• oxygen barrier covers that limit the transport of
two to three metres sufficiently reduces dissolved oxy-
oxygen into the tailings either by acting as a barrier
gen at the submerged tailings surface. However, a
against oxygen diffusion or by consumption of oxy-
water cover is not suitable if: (i) it would result in too
gen, which penetrates into the cover, thereby con-
much contaminated seepage; (ii) the embankments
trolling the rate of sulphide oxidation;
would not be stable and/or could not be economically
stabilized; and (iii) the water balance for the cover • after-use cover that aims to improve the appearance
pond would be such that the water cover could not be of the tailings surface; to prevent surface erosion; to
sustained (Wels et al. 2000). Under any of the above limit contact between the tailings and the surface
circumstances, a dry cover represents the method of run-off; and to provide a growth medium for the
choice for reclamation of the tailings. The design of a establishment of sustainable vegetation.
dry cover can vary widely, ranging from a single soil
Common components (layers) of a dry cover system
layer to promote revegetation, to a complex (multi-
are summarized in Table 1 (Rumer and Mitchell 1996).
layer) cover to control radiological, oxidation, and/or
Undoubtedly, not all layers are needed for all types
leaching effects.
of covers. The design criteria are based on a number of
In the present paper, the different types of dry covers
site-specific factors, including:
applied to the closure of tailings management facilities
are reviewed. Critical characteristics of the covers, and • climatic conditions of the site;
the parameters affecting their long-term performance, • geomechanical/geochemical properties and envi-
are described. Finally, the cover systems applied in the ronmental risks of the disposal area;
reclamation of two uranium tailing disposal areas at • borrow-material type and availability;
Pécs, Hungary, are presented.
• closure strategy;
• cost.
DRY COVER SYSTEMS
Types and characteristics of dry covers
The objectives of a cover system may vary from site to A low water flux cover, containing a low-permeability
site, but generally include: layer, has been commonly applied for covering the
waste disposal areas, in compliance with regulations on
• dust and erosion control; the landfill of waste. This type of cover, as well as alter-
• chemical stabilization of potentially acid-generating native types aiming to inhibit water infiltration to the
tailings (through control of oxygen ingress and/or waste, such as capillary barrier, store-and-release cov-
water infiltration); ers and geochemical barriers, are described in the fol-
• control of contaminant release (through control of lowing sections. Organic covers aiming principally to

164
Application of dry covers for the closure of tailings facilities

Table 1. Layers of the final cover at the waste disposal sites (Rumer and Mitchell 1996)
a/a Layer Primary functions Potential materials Factors affecting
performance
• Separation of underlying layers from the ground – Topsoil vegetated
surface – Geosynthetic layer over Erosion, evapo-
1 Surface layer • Resistance to wind and water erosion topsoil transpiration,
• Protection of underlying layers from temperature – Cobbles vegetation
and moisture extremes – Paving material
• Storage of infiltrated water until its removal by
– Soil
evapo-transpiration Erosion, slope failure
– Cobbles
Protection • Separation of waste from humans, burrowing due to pore pressure
2 – Recycled or reused waste
layer animals and plant roots buildup, animal
(e.g. fly ash, bottom ash
• Protection of underlying layers from wet–dry and burrows
and paper mill sludge)
freeze–thaw cycles, which may cause cracking
• Reduction of water head on the barrier layer
• Reduction of pore water pressures in the overlying
– Sand or gravel Clogging, insufficient
Drainage layers, thus increasing slope stability
3 – Geonet or geocomposite capacity and drainage
layer • Reduction of the time during which the overlying
– Recycled or reused waste outlets
layers are saturated following rainfall events,
thereby decreasing erosion
– Compacted clay Cracking due to
Hydraulic – Geomembrane desiccation, de-
and/or • Inhibition of water percolation and/or – Geosynthetic clay liner formation from
4
oxygen* • Prevent oxygen diffusion – Recycled waste settlement or seismic
barrier layer – Asphalt action, root
– Capillary barrier penetration, stability
– Sand or gravel
Foundation
5 • Foundation for the cover – Soil Adequate strength
layer
– Waste

* Applicable to sulphidic wastes with acid generation potential

inhibit oxygen transport to the sulphidic wastes are also • a compacted clay layer;
presented. • flexible membrane liners; and
• geosynthetic clay liners.
Covers with low-permeability layers
A cover incorporating low-permeability layers is the Historically, a compacted clay liner has been the
cover type recommended by Council Directive 1999/ most commonly used barrier layer. For sites where the
31/EC on the landfill of waste, as shown in Figure 1. available soil does not contain enough clay to be capa-
The low-permeability barrier consists of a mineral ble of being compacted to the desired low hydraulic
layer having a hydraulic conductivity of 10–9 m/sec. conductivity, commercially available clay minerals,
For hazardous wastes, the incorporation of an artificial such as sodium bentonite, may be mixed with the soil.
sealing liner is also recommended. It is noted, however, A number of physical/geotechnical parameters control
that tailings currently fall within the scope of Directive the engineering properties of soil barriers, including the
2006/21/EC and are not subject to the Landfill Direc- grain-size distribution, Atterberg limits, water content
tive. and energy of compaction and bonding of lifts (US
The barrier – a low-permeability layer – is consid- EPA/625/4-91/025).
ered the most critical engineered component of this The main problems associated with compacted clay
type of cover system. The theory and practice of barrier liners include damage due to desiccation during dry
layers is broadly applicable, regardless of waste type. periods and differential settlement. The in-place costs
Conventional artificial barriers, applied as single liners of a single compacted clay liner typically vary from 3
or combinations (composite barriers), include (Daniel to 25 €/m2, depending on thickness, availability, size
1993): and type of facility. Under extreme conditions (e.g.

165
Land Contamination & Reclamation / Volume 15 / Number 2 / 2007

depletion of antioxidants from HDPE geomembranes


may take from 45 to 115 years, and the geomembrane
Topsoil service life may be about 250 to 900 years, depending
>1m on the specific product, and in-place conditions.
The range of installed costs for the geomembranes
typically used in cover systems is relatively narrow in
Drainage layer comparison to the other liner materials. For geomem-
>0.5 m
branes with good out-of-plane deformation properties
and a thickness of approximately 1 mm, the installed
Low cost amounts to 5–9 €/m2 (Daniel 1993; Adam and
permeability Mylona 2001).
barrier
Geosynthetic clay liners (GCLs) have also gained
acceptance as a barrier system in solid waste landfill
applications. These are factory-manufactured hydrau-
lic barriers consisting of a thin layer of bentonite (∼ 5.0
Wastes
kg/m2) sandwiched between two geotextiles or bonded
to a geomembrane (US EPA 530-F-97-002). The struc-
tural integrity of GCLs is maintained by stitching or
needle-punching, and/or binding the geotextile or
Figure 1. Surface barrier for waste disposal areas in
compliance with the European legislation on the geomembrane to the bentonite by adding an adhesive to
landfill of waste (1999/31/EC) the bentonite. GCL technology can provide barrier sys-
tems with very low hydraulic conductivity, in the range
lack of clay locally), the cost could be much higher of 10–11 to 10–12 m/sec, performing at or above stand-
(Daniel 1993). ard European and international performance levels.
Some of the GCL brands currently available include
Polymeric geomembranes or flexible membrane lin-
Bentofix®, Bentomat®, Claymax ®, Gudseal® and
ers (FMLs) are usually made of continuous polymeric
NaBento®. The primary differences between GCLs
sheets that are flexible. Polyethylene (PE) is probably
include the mineralogy and form of bentonite (e.g.
the most common synthetic lining material, either as
woven vs. non-woven geotextiles); the addition of a
high-density polyethylene (HDPE) or less commonly
geomembrane; and the bonding methods. The ben-
low-density polyethylene (LDPE), whereas polyvinyl
tonite thickness of GCLs varies between 7 and 10 mm.
chloride (PVC) may also be used. They typically range
Based on the review and evaluation of alternative
in thickness from 0.06 to 0.24 cm, and come in sheets
covers by Rumer and Mitchell (1996), a final cover
and rolls of various sizes. Critical parameters in the
incorporating a GCL barrier layer can outperform one
design of a geomembrane in a landfill cover include
with a compacted clay layer. While a clay layer will
liner compatibility, vapour transmission, biaxal
frequently crack due to differential settlement, wet-
stresses via subsidence, and planar stresses mobilized
ting–drying and freezing–thawing cycles, a GCL has
by friction (US EPA/625/4-91/025).
the ability to self-repair any rips or holes caused when
Durability and ageing of geomembranes have to be subjected to these stresses due to the swelling proper-
taken into account when the long-term performance of ties of bentonite. One of the primary concerns with
the cover in the post-closure period is assessed. Degra- using GCLs in covers is the low shear strength at mid-
dation processes such as ultraviolet radiation are pre- plane. Furthermore, this technology requires additional
vented by burying the geomembrane in soil soon after field and laboratory testing to further assess its effec-
installation. However, long-term oxidation of tiveness as a landfill barrier system in terms of key per-
geomembranes is a degradation mechanism that can formance standards including hydraulic conductivity,
only be retarded, via anti-oxidants, but not eliminated bearing capacity, slope stability, long-term reliability
(US EPA/625/4-91/025). Based on recent studies, and resistance under freeze–thaw cycles. The cost of an

166
Application of dry covers for the closure of tailings facilities

installed GCL can amount to up to 11.5 € /m2 (GSI


2000).
Composite covers include the geomembrane/com-
pacted clay liner, which is recommended by the US Topsoil
Environmental Protection Agency (US EPA/625/4-91/
025) for the covering of hazardous waste disposal facil-
Drainage layer
ities, the geomembrane/GCL liner; and very conserva-
tive options like the geomembrane/compacted clay/
geomembrane and the geomembrane/GCL/geomem- Coarse grained layer
brane liners. Based on the study of Kim and Benson
(1999), multilayer caps containing a composite Fine grained layer
geomembrane/GCL or compacted clay barrier can also
be very effective at limiting oxygen transport into sul- Coarse grained layer
phidic mine wastes, inhibiting acid generation. The
geomembrane was considered a key component in Wastes
impeding oxygen diffusion.
The cost of composite covers is estimated to be the
sum of costs accounted for each component of the
cover system. Thus, the cost of a composite cover con-
Figure 2. Cross-section of a capillary barrier system
sisting of a geombrane in intimate contact with a com-
pacted clay liner will average 17 € /m2.
material is placed over a fine material, shown in Figure
Covers with capillary barriers 2. Such configuration prevents water rising by capillary
An alternative, appealing technique for the sealing of force, from the fine to the coarse material. In this typi-
waste disposal facilities relies on the use of natural cal layered cover system, the upper and lower coarse-
soils to generate a capillary barrier system where a grained layers inhibit the flow of water from the fine
fine-grained soil layer overlies a coarse-grained soil material layer and help to maintain a high degree of sat-
(Figure 2). At most water contents, except near satura- uration. Given that oxygen diffusion is low in water
tion, fine-grained soils have higher matric suctions than saturated soils, capillary barriers could also perform as
coarse-grained soils, due to their different soil-water a barrier against oxygen transport from the atmosphere
characteristic curves. As a result, the apparent hydrau- into the sulphidic wastes, preventing their oxidation
lic gradient in a capillary barrier near the fine-grained/ and subsequent acid generation (Nicholson et al.
coarse-grained interface is normally upward, except 1989). A wet fine-grained layer can be also effective in
when the upper layer becomes nearly saturated. In limiting outward diffusion of radon from uranium tail-
addition, infiltrated water is stored in the fine-grained ings (Benson 2000).
layer until the matric suction becomes low enough to For the design of a capillary barrier cover, detailed
permit water entry into the coarse-grained layer. characterization of the construction materials – includ-
Because coarse-grained soils have very low unsatu- ing grain-size distribution, hydraulic conductivity, soil-
rated hydraulic conductivities at low water content, the water characteristic curve and careful consideration of
coarse-grained layer impedes flow. These factors con- the site water balance and the geometry of the deposit –
stitute the ‘capillary barrier effect’ which inhibits water is required.
infiltration (Khire et al. 1996). Water stored in the fine-
grained layer due to the capillary barrier effect may be Store and release covers
diverted in a horizontal direction away from the under- A store and release cover, also referred to as an eva-
lying waste layers (applicable at humid sites), or potranspiration cover, consists of one or several layers,
removed via evapotranspiration (semi-arid and arid which are designed to maximize root penetration and
sites). A similar effect can be created when a coarse soil moisture storage (Figure 3). Such a cover stores

167
Land Contamination & Reclamation / Volume 15 / Number 2 / 2007

infiltrating water in the root zone long enough to allow these studies is to compare the performance of store/
evapotranspiration to remove it, thereby reducing infil- release systems with cover systems incorporating bar-
tration to the underlying wastes (Swanson et al. 1997). rier layers. The water balance of 21 landfill final cover
This type of cover is applicable in arid and semi-arid test sections has been evaluated as part of the United
climates, and relies on the moisture retention and stor- States Environmental Protection Agency’s Alternative
age characteristics of the cover material. It is noted that Cover Assessment Program. Based on data from the
the root zone is not limited to the cover layer but may test sections, the alternative covers in arid and semi-
extend into the upper layers of the mine waste. In this arid climates generally are transmitting significantly
case, the cover material would primarily serve as a less percolation than that in humid climates (Roesler et
medium for initiating plant growth and to avoid wind al. 2002). Percolation rates for the alternative covers in
and water erosion of the underlying waste material arid and semi-arid climates typically are less than 1
(Wels and O’Kane 2003). mm/yr. For the humid sites, percolation typically is
between 37 and 144 mm/yr; however, it should
decrease over time as the vegetation matures, and is
capable of removing more soil water. Data from the test
sections simulating a composite cover (i.e. a geosyn-
thetic clay liner or compacted clay barrier overlain by a
geomembrane) indicate that these covers are very
effective when constructed properly. Percolation rates
for the composite covers are generally less than 1 mm/
Store and
release material yr in semi-arid and arid regions, and 5 mm/yr in humid
regions. Data from the test sections simulating com-
pacted clay covers show that clay barriers are highly
susceptible to desiccation cracking and can transmit
percolation at large rates (several hundred mm/yr). Pro-
tection of geomembranes is also a key factor. Methods
or materials that damage the geomembrane during con-
struction will lead to higher than anticipated percola-
Wastes
tion rates.
An indicative cost of a two-layer store-and-release
cover is $50,000 per hectare, as compared to $400,000
per hectare for composite covers incorporating a GCL
Figure 3. Cross-section of a store-and-release cover and drainage layers (Wilson et al. 2003). The cost asso-
ciated with large-scale mining applications is consid-
ered the limiting factor for the extensive use of the
Vegetation plays an important role in the perform- various materials proposed as mining covers. Although
ance of store and release covers. Actual evaporation both natural and synthetic covers may be cost-effective
from a bare or non-vegetated soil cover will generally when applied in relatively small disposal areas, they
only be about 10% of the potential rate of evaporation may not be feasible for the large tailings disposal facili-
available. High evapotranspiration can only be ties typical in the mining industry. Thus, further
obtained with a fully developed plant canopy (Wilson research studies were performed into the potential use
et al. 2003). of other readily available, inexpensive and potentially
The performance of such covers has been tested at non-phytotoxic, non-polluting waste products, includ-
field scale within the Alternative Landfill Cover Dem- ing depyritized tailings, granulated slags, paper-mill
onstration, ALCD (www.sandia.gov) and the Alterna- sludge and fly ash. For potentially acid-generating sul-
tive Cap Assessment Project, ACAP (www.dri.edu/ phidic wastes, organic oxygen-consuming materials
Projects/EPA/boston-brochure2.html). The purpose of like peat, lime-stabilized sewage sludge and municipal

168
Application of dry covers for the closure of tailings facilities

solid-waste compost have also been used (Elander et The addition of cement to tailings, often practised in
al. 1998). Use of waste products is not only considered underground mine backfill applications, also has
economical, but it also eliminates the need for the envi- potential benefits for use as a cover material during the
ronmentally safe storage of such materials. However, decommissioning of tailings dams. The addition of
these wastes often contain potentially toxic substances, ordinary Portland cement (OPC), however, is consid-
which may inhibit plant growth or eventually leach into ered to be too costly for a large-volume tailings cover.
the surrounding environment. However, other low-cost alternatives, including blast
furnace slag (BFS), pulverized fly ash (PFA) and lime,
Covers with geochemical barriers can be locally available and can be easily substituted in
This type of cover involves the formation of a geo- the cement mixtures.
chemically stable layer at the tailings surface, by the The use of phosphate rock and related materials
application of selected reactive materials such as alka- exhibiting increased neutralization potential can also
line and cementitious materials. The geochemical bar- be considered for the formation of a geochemical bar-
rier may inhibit infiltration of rainfall to the tailings, act rier at the sulphidic tailings surface (Watkin and Watkin
as an oxygen diffusion barrier and provide mechanical 1983). Neutralization reactions will produce secondary
stability to the tailings. minerals such as gypsum and ferrous phosphate, and
The natural formation of such layers (hardpan) in these compounds may block pore spaces and reduce
inactive sulphidic mine tailings impoundments has tailings permeability with time.
been reported in a number of studies (Blowes et al. Other studies have shown the potential for inducing
1991; Tasse et al. 1997; Johnson et al. 2000; Moncur et precipitation processes in order to reduce permeability
al. 2005). Hardpans may act as an oxygen diffusion and and immobilize contaminants through the injection of
water transport barrier, thus resulting in a considerable supersaturated solutions. These solutions promote pre-
reduction in acid generation and metal dissolution. Fur- cipitation of gypsum, barium sulphate, calcium
thermore, adsorption of dissolved metals like Zn, Cd, hydroxide, calcium carbonate and aluminium or iron
As, Mn, Ni, Co to the precipitated compounds in the hydroxides, which reduce permeability through crys-
hardpan layer limits their downward migration and tallization in pore spaces, provided that precipitation
subsequent groundwater contamination. can be delayed through pH adjustment and/or addition
Given the significant environmental and economic of degradable polymers (IAEA 2004).
implications of hardpan layers, laboratory studies aim- Depending on the composition of the tailings mate-
ing at elucidating the mechanisms that lead to the for- rial and leachates, different types of geochemical barri-
mation of natural hardpans, as well as methods of ers can be formed. These layers, however, are
creating such barriers, have been reported in the litera- chemically and subsequently physically active, thus the
ture. Alkaline additives, such as limestone and lime, prediction and engineering of such a technology may
have been proposed to create a barrier to oxidized sul- well be very difficult.
phidic wastes (Chermak and Runnells 1997; Mylona et
al. 2003). Fly ash, i.e. the material trapped by electro- Oxygen-consuming cover
static precipitators in coal- and lignite-burning power- Municipal solid waste (MSW) and other organic-based
generating plants, may be also beneficially used to cre- materials could be used as an oxygen barrier cover for
ate a barrier to sulphidic wastes. Class C fly ash, due to tailings. The compost layer would function as both a
its increased Ca content, mainly as CaO, Ca(OH)2, physical barrier and as an oxygen-consuming layer that
CaCO3, has a significant neutralization capacity, and would permanently prevent sulphide oxidation and the
can be employed to counteract the acid potential of the resultant acid drainage. The organic layer on sulphide
mine wastes. Class C fly ash also has pozzolanic and tailings can be beneficial in five ways:
cementitious properties, resulting in the reduction of
the permeability of the wastes, thus hindering oxidation 1. physical oxygen barrier – the compost would be
of the contained reactive minerals (Mohamed et al. saturated with water over at least part of its depth,
2001; Xenidis et al. 2002). so that the limiting factor in oxygen diffusion

169
Land Contamination & Reclamation / Volume 15 / Number 2 / 2007

would be the diffusivity of oxygen in water; For the design of a cover system, the geotechnical
2. oxygen-consuming barrier – the continued decom- and geochemical characteristics of the tailings should
position of compost creates a large biological oxy- be considered. Detailed investigation of the potential
gen demand that acts as a sink for diffusion of cover materials should be also carried out in order to
atmospheric oxygen or dissolved oxygen; determine critical physical–geotechnical (e.g. grain
3. chemical inhibition – compounds and decomposi- size, compaction, hydraulic conductivity, moisture
tion products in the MSW compost that leach into retention curve, etc.) and geochemical parameters (e.g.
the tailings inhibit the growth and metabolism of pH, acid generation potential, metals leachability, etc.),
sulphate-producing bacteria; and assess their suitability.
4. chemical amelioration – organic constituents in Numerical modelling can be used to evaluate the
the MSW compost can cause the reductive dissolu- relative performance of alternative options. It is good
tion of ferric oxides and prevent indirect ferric sul- practice to also perform field trials, in which the per-
phide oxidation and acid generation; and formance of selected cover options can be monitored
5. reduced water infiltration – reduced hydraulic under actual field conditions.
conductivity of compacted compost may prevent The design and construction of soil covers on tail-
infiltration of precipitation, thus decreasing tail- ings often presents a formidable challenge, due to the
ings groundwater flow. low shear strength, poor trafficability, and high settle-
ment of underconsolidated tailings at the time of recla-
Long-term efficiency seems to depend on the degree mation.
of water saturation at the bottom of the pile, probably A review of dry cover placement on extremely
because of the build-up of a microbial mass in such an weak, compressible tailings was presented by Wels et
anaerobic environment. The addition of nutrients al. (2000). It was concluded that the optimal technique
would promote composting and create a more func- (or combination of techniques) for placing a dry cover
tional and longer-lasting barrier (Tasse 2000). At mine will vary from site to site and is influenced by the envi-
sites in the USA, coarse woody debris is now being ronmental and geotechnical circumstances, as well as
incorporated into tailings, with the addition of up to cost and availability of materials and equipment used
seven tons per acre to provide a substrate for essential for cover placement. The geotechnical issues to be con-
microorganisms. sidered include:

Aspects of cover design and application • consolidation of near-surface tailings to achieve


The design criteria for covers are related to the remedi- strength gains, improve trafficability, and allow the
ation objectives, and address geotechnical, radiologi- safe placement of the initial cover layer;
cal, hydrological, geochemical, ecological and • stability of tailings slopes during dewatering of tail-
aesthetic requirements. The selection of a cover system ings ponds and/or cover placement; and
design is site-specific. Key variables that need to be • long-term settlement of tailings and its impact on
evaluated during the initial selection process include cover integrity and final surface shaping.
climate, tailings characteristics, size and geometry of
The environmental issues to be considered include:
the tailings management facility, and available cover
materials. • management of contaminated (free) pond water;
The predicted performance of cover systems should • management of contaminated pore water expelled
be assessed by utilizing a design philosophy that inte- during tailings consolidation; and
grates the waste material within its environmental con- • management of (uncontaminated) surface water on
text. The cover system must be designed as an top of the cover.
unsaturated system exposed to the atmosphere, the per-
formance of which will be significantly influenced by Natural processes of consolidation may take tens of
daily, seasonal, annual, and long-term site climate con- years before pore pressures dissipate and settlement
ditions (O’Kane Consultants Inc. 2002). ceases. Thus reclamation profiles must either allow for

170
Application of dry covers for the closure of tailings facilities

such long-term consolidation or the process must be permeable drains or drainage layers may also result in
accelerated. Numerous techniques have been devel- clogging of the drains. Burrowing intrusion by animals
oped to allow access on to the surface of weak uncon- also has the potential in the long term to significantly
solidated tailings. The most widely used approach is to alter the hydraulic conductivity of low-permeability
allow drying to form a ‘crust’ of desiccation-strength- capping layers.
ened tailings, reinforce this with a synthetic geogrid, Direct measurement of field performance is the
and then advance thin layers of cover fill using light state-of-the-art method for measuring the performance
equipment. High-permeability drainage elements, most of a dry cover system. Field performance monitoring
commonly in the form of band drains, may be also can be implemented during the design stage with test
placed into the upper layers of the slimes. The band cover plots, or following construction of the full-scale
drains reduce the effective drainage path length (from cover (O’Kane Consultants Inc. 2003). The main
the total tailings depth to half the horizontal spacing of objectives of field performance monitoring include:
the drains), significantly accelerating the consolidation
process and allowing earlier access and faster advance • estimation of a water balance for the site;
rates during actual cover placement. • collection of an accurate set of field data to calibrate
a numerical model;
Long-term performance of dry covers − monitoring • development of stakeholders’ confidence with
Based on a study by the International Network for Acid respect to cover system performance; and
Prevention (INAP) on the long-term performance of • development of an understanding of key character-
dry cover systems for mine waste, the processes affect- istics and processes that control performance.
ing the long-term performance of a dry cover system
can be grouped into physical, chemical, and biological The desired field performance monitoring system
processes (O’Kane Consultants Inc. 2003). The effects should include monitoring of the various components
of these processes are related to the change in three key that influence the performance of a dry cover system,
properties of the cover materials, including the satu- including meteorological parameters, moisture storage
rated hydraulic conductivity, the soil-water characteris- changes, net percolation, surface run-off, and erosion.
tic curve (SWCC) and the physical integrity of the Vegetation monitoring is also necessary to determine
cover system. whether the revegetation programme is successful and
A summary of the physical processes identified, and is progressing towards a desirable, sustainable vegeta-
possible effects on the performance of dry covers, is tive cover.
given in Table 2.
Chemical processes including osmotic consolida-
CASE STUDY − URANIUM TAILINGS PONDS IN
tion, dispersion/erosion, dissolution/precipitation, PÉCS, HUNGARY
acidic hydrolysis, mineralogical consolidation, sorp-
tion, oxidation and salinization have the potential to Site description
change the fabric of a cover material, affecting the One uranium ore deposit exists in Hungary, located at
long-term performance of a cover system. Osmotic the foot of the Mecsek Mountains in Pécs, south of the
consolidation and dispersion/erosion may affect the country. Before 1989, production was 500−550 tonnes
properties of a clay layer incorporated in the cover sys- of uranium per year from ores at grades of 0.1%, all of
tem. Chemical processes such as dissolution/precipita- which was shipped to the Soviet Union. Production
tion are important in geochemical barriers. stopped in 1997.
Biological processes include root penetration, bur- Ore processing in Mecsek included radiometric
rowing animals, bioturbation, human intervention, bac- upgrading, crushing, milling, and leaching with sul-
terial clogging and vegetation establishment. Roots phuric acid. Uranium was removed by the anion
may penetrate low-permeability layers, and also create exchange process. Yellow cake was precipitated with
seepage channels, which would increase infiltration lime milk, and the calcium diuranate obtained was the
through covers. Extensive root development in moist, commercial end-product. Wastes from processing were

171
Land Contamination & Reclamation / Volume 15 / Number 2 / 2007

Table 2. Physical processes affecting long-term performance of dry covers


Physical processes Effects
Erosion Reduction in cover thickness, affecting its integrity
Reduction in the ability of topsoil to sustain vegetation
Process significant in climates experiencing short-duration high-intensity rainfall events
Slope instability Slope instability is attributed to gravitational, seepage and seismic forces and affects the physical
integrity of the cover system.
Wet/dry cycles Shrinkage cracks in fine-textured materials, affecting the integrity and hydrological performance
of the cover system
Freeze/thaw cycles Changes in hydraulic conductivity and moisture retention characteristics of soil covers
Consolidation/settlement Reduction of thickness of cover layers, affecting the physical integrity, geometry and drainage
patterns of the cover system
Extreme climate events Erosion, changes in hydraulic conductivity and moisture retention characteristics of the cover
system
Brush fires Reduction of vegetation, increasing run-off and erosion

treated with limestone and lime milk to pH ~7. A percentage of 90% of fine tailings, mainly found
The neutralized tailings were disposed of in tailings in the slime core (central part) of tailings ponds, had a
ponds 1 (TPI) and 2 (TPII) constructed at a distance of grain size finer than 0.05 mm.
2–4 km from the mill and covering a total area of 154
ha (Figure 4). TPI is a ring dyke and had been operating Chemical–mineralogical composition
since 1962. TPII, put into operation in 1979, belongs to The chemical composition of three samples collected
the valley type. Approximately 14.2 and 4.6 Mt of tail- from the different tailings zones is given in Table 3.
ings were disposed of in TPI and TPII, respectively.
Due to the segregation of the tailings, the three
The tailings in TPI were very weak and some were
zones present different chemical–mineralogical com-
even underwater in 1998. For the design and applica-
positions. Dam material consists mainly of quartz,
tion of remediation actions, detailed investigation of
whereas the slimes contain silt, gypsum (formed during
the tailings was required. The studies included determi-
the leaching), etc. The mineralogical composition of
nation of the physical characteristics of tailings, chemi-
the fine tailings is given in Table 4.
cal–mineralogical analysis, radiological characteriz-
ation, geotechnical investigation, etc. The results of the It is seen that the fine tailings contain a significant
studies performed, and the remediation measures amount of gypsum. The clay minerals are mainly
applied subsequently, are described in the following present in the finest tailings. The clayey part of the tail-
paragraphs. ings was investigated separately for montmorillonite
content, in order to obtain information regarding the
Tailings characteristics possible thixotropy (liquefaction behaviour) of the tail-
ings. Montmorillonite occurred only in the form of a
Grain-size distribution
mixed-layer illite–montmorillonite, and its average
A percentage of 40% of tailings had grain size >0.1 mm
content in fine tailings was estimated to be 6–8%, indi-
and 60% <0.1 mm. Deposition of tailings following the
cating that it cannot lead to the liquefaction of the tail-
separation of the coarse sand fraction for dam construc-
ings.
tion by hydrocyclones resulted, however, in the signifi-
cant segregation of tailings. As a result, in practice, The heavy-metal content of the tailings is low. Prac-
tailings ponds consist of three zones: tically only the manganese (which was used as an oxi-
dizing agent) and the vanadium content present
• fine slime zone; elevated values. Furthermore, the pyrite content of the
• intermediate zone; tailings is low (in the processed ore it is <0.2%) and
• sandy zone (dam). thus they do not exhibit net acid-generation potential.

172
Application of dry covers for the closure of tailings facilities

Table 3. Elemental analysis of tailings

ZT I 14/1 6-17 (R4176) I. Z. D TP II Dam


Number Element Concentration StdErr Concentration StdErr Concentration StdErr
% % %
Sum Be..F Be-F 0,073 0 0,08 0 0,086
11 Na 0,48 0,02 0,51 0,03 0,98 0,04
12 Mg 1,14 0,04 2,46 0,06 0,51 0,02
13 Al 6,09 0,08 4,5 0,07 6,21 0,08
14 Si 19,3 0,1 13,8 0,1 29,3 0,1
15 P 0,058 0,004 0,052 0,004 0,03 0,002
16 S 0 0,56 0 0,71 0 0,26
16 So 5,71 0,07 7,21 0,08 2,62 0,05
17 Cl 0,19 0,01 0,47 0,03 0,003 0,002
18 Ar 0 0,001 0 0,001 0 0,002
19 K 3,68 0,08 2,71 0,07 4,73 0,09
20 Ca 6,6 0,1 9,9 0,1 3,89 0,08
21 Sc 0 0,0008 0 0,0008 0 0,001
22 Ti 0,26 0,02 0,2 0,01 0,27 0,02
23 V 0,056 0,004 0,067 0,005 0,56 0,004
24 Cr 0,011 0,001 0,0095 0,0008 0,015 0,001
25 Mn 0,94 0,04 1,5 0,05 0,28 0,02
26 Fe 2,89 0,07 2,79 0,07 1,48 0,05
27 Co 0,0055 0,0007 0,0029 0,0007 0,001 0,0007
28 Ni 0 0,0009 0 0,0009 0 0,0009
29 Cu 0,0066 0,0007 0,002 0,0006 0,0046 0,0008
30 Zn 0,0109 0,001 0,03 0,003 0,0105 0,0009
31 Ga 0,001 0,0004 0,0011 0,0004 0,0007 0,0004
32 Ge 0,0006 0,0005 0 0,0003 0,0003 0,0003
33 As 0,012 0,001 0,009 0,001 0,01 0,001
34 Se 0,0031 0 0,003 0,0004 0,0019 0,0004
35 Br 0 4 0 0,0003 0 0,0003
37 Rb 0,014 0,0003 0,0101 0,0009 0,019 0,002
38 Sr 0,029 0,001 0,031 0,003 0,024 0,0004
39 Y 0,0039 0,002 0,003 0,0004 0,0017 0,001
40 Zr 0,015 0,0005 0,0105 0,0009 0,021 0,001
41 Nb 0,0003 0,001 0 0,0003 0,0003 0,001
42 Mo 0 0,0003 0 0,001 0 0,0009
44 Ru 0 0,001 0 0,001 0 0,0008
45 Rh 0 0,001 0 0,001 0,001 0,0009
46 Pd 0 0,001 0 0,001 0 0,001
47 Ag 0 0,001 0 0,0008 0 0,001
48 Cd 0,0008 0,001 0 0,0008 0,0014 0,002
49 In 0 0,0008 0 0,0007 0 0,003
50 Sn 0 0,0008 0 0,0009 0,0008 0,006
51 Sb 0 0,0009 0 0,0009 0 0,029
52 Te 0 0,0009 0 0,001 0 0,001
53 I 0 0,001 0 0,001 0 0,001
55 Cs 0 0,001 0 0,002 0 0,001
56 Ba 0,042 0,001 0,041 0,003 0,069 0,001
Sum La..Lu La-Lu 0,009 0,002 0,014 0,027 0,012 0,001
72 Hf 0,002 0,004 0,001 0,001 0 0,001
73 Ta 0 0,026 0 0,001 0,002 0,001
74 W 0 0,001 0 0,001 0 0,001
75 Re 0,002 0,001 0 0,001 0,003 0,001
76 Os 0,001 0,001 0 0,001 0 0,001
77 Ir 0,001 0,001 0 0,001 0 0,001
78 Pt 0 0,0008 0 0,0009 0 0,001
79 Au 0,0004 0,0008 0 0,0009 0 0,001
80 Hg 0,0009 0,0008 0 0,0009 0,0008 0,001
81 Tl 0 0,001 0 0,001 0 0,001
82 Pb 0,022 0,002 0,032 0,003 0,0018 0,002
83 Bi 0 0,0007 0 0,0009 0,001 0,001
90 Th 0,001 0,001 0 0,001 0 0,002
92 U 0,008 0,001 0,024 0,002 0,014 0,001
Note:
I. Z. D. TP I, south part
TP I 14/1 6-17 m TP I, intermediate zone S Sulphur as sulphide
TP II Dam TP II, from the dam So Sulphur as sulphate

173
Land Contamination & Reclamation / Volume 15 / Number 2 / 2007

TP

Pipeline TPI

Mill TPII

Figure 4. Location of the mill, and the tailings ponds TPI and TPII, in Pécs, Hungary

Geotechnical characteristics ings, because the mill process recovered only uranium
The results of in situ measurements of the shear (app. 90%), and tailings contain practically all the other
strength on TPI are shown in Figure 5. Shear strength decay products of uranium. Therefore, the total activity
was measured up to 9 m below water level. The fine for the ore with 0.1% of original uranium (Hungarian
tailings have a very low shear strength under water, i.e. ore grade) is 170 Bq/g. Due to the radium content (12
<5 kN/m2, which increases at greater depth. In the tran- Bq/g), the tailings show a radon exhalation value which
sition zone, shear strength values are a little higher (5– depends on the physical characteristics of the tailings
15 kN/m2), whereas the values of the shear strength in (water content, porosity, grain-size). Actually, the
the sandy zone were high (>40 kN/m2). Based on the
radon exhalation rate of the dam is between 3 and 8 Bq/
results, stabilization of an area of approximately 13 ha
m2s, two orders of magnitude higher than the back-
in the fine slime zone was required prior to the start of
ground level.
the covering works.

Composition of tailings water


Radiological characteristics
In Hungary, relatively low-grade ore was processed, Tailings water was highly contaminated with non-radi-
therefore the radio-element content of the tailings is oactive components originating from the leaching
low. Nevertheless, the major part of the radioactive process. The composition of the process water dis-
nuclides contained in the ore is also present in the tail- charged at the tailings ponds together with the solid

Table 4. Mineralogical composition of fine tailings


Mineral Formula Amount of minerals (%)
I.Z.K. I.Z.D. II.Z.D.
Bassanite CaSO4.0.5H 2O 16 17 37
Gypsum CaSO4.2H2O 40 31 4
Feldspar NaAlSi3O8 13 8 7
Quartz SiO2 19 20 18
Muscovite KAl2(Si3Al)O 10(OH)2 3 3 3
Clayey minerals (illite,
Na0.3(Al,Mg)2Si4O10 8 18 28
montmorillonite)

I.Z.K. (TPI, fine tailings zone, east part)


I.Z.D. (TPI, fine tailings zone, south part)
II.Z.D. (TPII, the finest tailings zone, south part)

174
Application of dry covers for the closure of tailings facilities

TPI
Date: 11.2001 I I_1
II_ 2
II_3
II_ 4
II_5
III_1
II I_2
III_ 3
II_6 III_4
I /1
I/2 II/1
III_5

IV_1
100
z=-0.5 m
X V III/1 IV _2
I/3 II/2 II I/1 IV /1
XV III/2
I/4 II/3 III/2 IV/2
X VII/1
XV II/2 IV /3
XV
XVII/3
III/3
XV
II/4II/4 X VII/5 XV II/6 XV II/7 IV /4
V /1

52
XV I/1 X VI/2 V/2
V /3
X V /1 X V/2 PP
/1/2 V/4
PP/4
/3
P/5 V/5 0+10
0+9
0+80+7
PP/7
/6 0+6
0+5
0.+3
0.+4
0.+1
0.+2 0.1
XIII /1XIII/2 P /8 I+10I+9I+7 0.2
0.30.4
0.5
0.60.7
X III/3 X IV /1 P/9
P/10 VI/3 I+8 I+I+5
6I.+
I.+4
I.+3 I.+
1 I.2
2
X IV /2 PP/11
/12 V I/4 II+10
VI/2
II+9
II+7
II+.II+6
8II+5
II.+4 I.1
V I.3 I.4
I/1I.5I.6
I.7I.8
I.10
XIV /3 X IV /4 II.+3 II.II.1
II.+1 +2
II.2
II.II.4
3 II.6 I.9I.11I.12
I.13I.14
XIV /5 X IV/6 VI I/7 III+10
III+9
III+8
III+7
IIIII+5
I+6
III.+
III.+4 II.5 II.8
II.7 II.10 I.15 I.16
XIII/5 XIII/6 V III/6 VII/6 I3
III.+1
II.+2
III.1
III.2
IIIIII.4
III.5
.3III.6
II.9
II.11
II.12
II.13
II.14
II.15II.16
XII/1 X
XIII/1
II/2 XIII/2 XIII/3 X III/4 III.7
IX/5 V II /5
XII/4 V III/5 V II/4
X I/3 X /4 VII/3
X II/3 IX/4 V III/4 V II/2

48
XII/2 X I/2 V III/3 VII/1
X /3 IX/3
X II/1
XI/1 X I/1 VIII/2
X/2 IX /2
VIII/1
X /1 IX/1
X/2
X /1

44
I I_1
II_ 2
II_3
40
III_1
II_ 4
II I_2
II_5 III_ 3
II_6 III_4

z=-1.0 m
III_5

36
I /1
I/2 II/1 IV_1
X V III/1 IV _2
I/3 II/2 II I/1 IV /1
XV III/2
I/4 II/3 III/2 IV/2
X VII/1
XV II/2 IV /3
XV
XV III/3
II/3 XV II/7
XV
II/4II/4 X VII/5 XV II/6 IV /4
V /1
V/2
XV I/1 X VI/2

32
V /3
X V /1 X V/2 P /1 V/4
PP /2/3
P/4
P/5 V/5 0+10
PP/7
/6 0+9
0+80+7
0+60+5
0.+3
0.+4
0.+1
P /8 0.+2 0.1
0.2
0.3
0.4
0.5
0.6
XIII /1XIII/2 P/9 I+10I+9
I+8I+7
I+I+5 6I.+
I.+4 0.7
X III/3 X IV /1 P/10
PP/11 V I/4 VI/3 II+10
VI/2
II+9
II+7 I.+3 I.+1 VI.2
2
I.1I.3 I.4
I/1 I.6
X IV /2 XIV /3 /12 II+.II+6
8II+5II.+4
II.+3 II.II.1
II.+1 +2II.2 I.5 I.7II.9
.8
I.10
I.11
X IV /4 XIV /5 X IV/6 VI I/7 III+10
III+9
III+8
III+7
IIIII+5
I+6 II.II.4
3II.5
II.6II.8
II.7 II.9
II.10
I.12I.13 I.14I.15I.16
V III/6 III.+
III.+4
III.+1
I II.+2
3III.1
III.2
IIIIII.4
.3 II.11
II.12
II.13II.14
II.15
XIII/2 XIII/3 X III/4 XIII/5 XIII/6 VII/6 III.5
III.6
III.7 II.16
XII/1 X
XIII/1
II/2 IX/5 V II /5
XII/4 V III/5 V II/4
X I/3 X /4
X II/3 VII/3
IX/4 V III/4 V II/2
XII/2 X I/2 VII/1
X /3 V III/3

28
X II/1 IX/3
XI/1 X I/1 VIII/2
X/2 IX /2
VIII/1
X /1 IX/1
X/2
X /1

I I_1
24
II_ 2
II_3
III_1
II_ 4 II I_2
II_5

20
III_ 3

z=-2.0 m
II_6 III_4
I /1 III_5

I/2 II/1 IV_1


X V III/1 IV _2
I/3 II/2 II I/1 IV /1
XV III/2
I/4 II/3 IV/2
III/2
X VII/1 IV /3
XV II/2 XV III/3
XV II/3
XV
II/4II/4 X VII/5 XV II/6 XV II/7 IV /4

16
V /1
XV I/1 X VI/2 V/2
V /3
X V /1 X V/2 PP
/1/2 V/4
PP/4
/3 V/5
P/5 0+10
0+9
0+80+7
PP/7
/6 0+6
0+50.+3
0.+4
0.+1
0.+2 0.1
0.2
0.3
XIII /1XIII/2 P /8
P/9 I+10I+9
I+8I+7 0.40.5
0.60.7
X III/3 X IV /1 P/10 V I/4 VI/3 I+I+56I.+4
I.+3
I.+I.+ 1 I2
I.1 .2 I.4
X IV /2 PP/11
/12 VI/2
II+9
II+10II+
II+7
8II+5
.II+6 II.+4 V I.3
I/1I.5I.6
I.7I.8
I.9
I.10
XIV /3 X IV /4 III+10
III+9 II.+3 II.II.1
II.+1 +2II.2
II.II.4
3
II.5
II.6II.8 I.11
I.12I.13I.14I.15
XIV /5 X IV/6 VI I/7 III+8
III+7
IIIII+5
I+6
III.+
III.+4
III.+1
I II.+2
3III.1 II.7 II.10
II.9
II.11
II.12
II.13 I.16
X III/4 XIII/5 XIII/6 V III/6 VII/6 III.2
IIIIII.4
.3
III.5
III.6
III.7 II.14
II.15II.16
XII/1 X
XIII/1
II/2 XIII/2 XIII/3
IX/5 V II /5
XII/4 V III/5 V II/4
X I/3

12
X /4 VII/3
X II/3 IX/4 V III/4 V II/2
XII/2 X I/2 VII/1
X /3 IX/3 V III/3
X II/1
XI/1 X I/1 VIII/2
X/2 IX /2
VIII/1
X /1 IX/1
X/2
X /1

8
4
0
[kN/m2]
[kN/m] 2
Figure 5. In situ shear strength measurements on TPI

tailings changed, depending on the technology used. • water management;


Taking into account the volume of process water and • stabilization of fine tailings;
the quantity of reagents used, the average concentration • recontouring the dam and relocation of some part of
of total dissolved solids (TDS) in the tailings water was tailings;
estimated to 20–22 g/L. The high TDS in the process • covering;
water was attributed to the magnesium sulphate which • revegetation;
remained in the neutralized solution, given the rela- • groundwater restoration.
tively low pH (~7–8) at the stage of the barren pulp
neutralization. A major issue in the remediation of the tailings
ponds involved the design and construction of the dry
The tailings ponds were constructed with no, or very
cover system described in the following sections.
poor, sealing. Therefore, process water from the tail-
ings ponds could have partly seeped into the soil Application of dry cover systems
beneath the ponds. According to the estimates, approx- Stabilization of the tailings surface
imately 20 Mm3 of process water (from the total of 32 The first step in the long-term stabilization of tailings
Mm3) seeped into the soil beneath the ponds over the ponds was the stabilization of the very weak fine tail-
period of operation of the mill. Based on these calcula- ings in TPI. TPII had been out of operation for some
tions, the quantity of chemical compounds which years, and all the three zones were stable enough for the
seeped from the tailings into the surroundings was esti- construction of the cover system.
mated to be 400 kt or even more. Groundwater contam- For the stabilization of fine tailings in TPI, dewater-
ination was detected as early as 1977, but systematic ing by earth loading and removal of compression water
site investigations and monitoring only started in 1989. by drainage was recommended. To prepare the fine
slime zone for stabilization, first the free water from the
Remediation works tailings pond was discharged. As a result, the surface of
For the remediation and closure of the tailings ponds, a the fine slimes became sufficiently stable after some
series of actions were taken, including: months. Following dewatering, geotextiles and geog-

175
Land Contamination & Reclamation / Volume 15 / Number 2 / 2007

rids were used for further stabilization, as shown in Taking into account the above, the application of a
Figure 6. multi-layered cover was considered. The cover should
A 0.5-m-thick sand layer from dam recontouring (c. consist of a low-permeability barrier layer, a water-
0.8 Mm3) was placed on the geogrid, overlain by a storage layer for further inhibition of water infiltration,
layer of material loaded from different parts of the dam. and vegetation to increase the evapotranspiration rate
To enhance the stabilization, a vertical drain was also and protect against erosion. The placement of a drain-
used. age layer between the water storage layer and the bar-
rier layer would be also desirable in order to protect the
Cover design barrier from root and animal intrusion, etc.
The objectives of the uranium tailings cover included: To select the appropriate cover configuration, exten-
sive modelling work was undertaken by Mecsek ÖKO
• reduction of radon exhalation and gamma-dose rate; Zrt in cooperation with Golder Hungary Ltd and Wis-
• minimization of the rate of seepage through the tail- mut GmbH. Estimation of the seepage rate was carried
ings to prevent further water contamination; out using the HELP model (Allisson et al. 1990).
• prevention of any unauthorized removal of hazard- Sensitivity analysis was carried out for, among oth-
ous material; ers:
• long-term stabilization of the tailings ponds.
• the water-storage layer (effective depth of root pen-
Based on ‘The Environmental License for Remedia- etration: 50, 60, 80, 100 cm, hydraulic conductivity
tion’, specific criteria of cover design also included: (k): 1 × 10–6, 8 × 10–9 m/s);
• the barrier layer (k: 1 × 10–8 to 5 × 10 –10 m/s, thick-
• reduction of the radon flux (max. 0.74 Bq/m2s); ness: 30, 40, 50 cm);
• decrease in the gamma-dose rates (max. 300 nGy/ • slope of the surface (5–20%);
h); • length of run-off on the surface (20, 30, 250 m).
• minimization of the seepage rate;
• design life of 200 years. Following the evaluation of different options, the

Figure 6. Placement
Figure of the geogrid,
6: Placement of
vertical drains and loading the
geogrid, vertical
enforced surface drains and
loading the enforced surface

176
Application of dry covers for the closure of tailings facilities

two types of cover shown in Figure 7 were selected. For the calculation of the expected radon exhalation
A sand-drainage layer was not included in the cover rate, the following internationally recommended equa-
design of TPI, because the settlement of tailings is still tion (IAEA 1992) was applied:
in progress and thus unequal consolidation rates on the 1⁄2
F c = F t exp ⎛⎝ – ( λ D c ) × X c⎞⎠ (1)
area after covering (deformation of layers) may result
in the formation of a ‘water sack’ in some parts of the
fine tailings area. The formed ‘sacks’ can lead to a where Fc is the radon flux from covered tailings pile, Ft
more intensive seepage rate. It is also possible that the is the radon flux from uncovered tailings, λ is the radon
drainage layer will lose some of its hydraulic conduc- decay constant, Dc is the diffusion coefficient, and Xc
tivity because of layer deformation. the thickness of the covering layer.
Based on the results of the HELP model, the annual The radon diffusion coefficient strongly depends on
seepage rate from the tailings pile will be around 30 the porosity and the saturation of the covering soil, and
mm, in compliance with the Environmental Licence. is calculated from equation (2).

Cover design for TPI (loess cover with clay as barrier layer)
Layer type Material
Vegetation Grass and bushes

0.4 (0.45) m Storage layer Loess


(Degree of compaction
≤90%)
0.4 (0.45) m Storage layer Loess
(Degree of compaction
90 to 93%)
0.4 m Protection layer Compacted loess 2
(compaction c. 95%)
0.4 (0.3)m Sealing layer Compacted clay
(compaction 95 to 97%)
Tailings

Cover design for TPII (loess with sand drainage and clay as sealing
layer)
Layer type Material
vegetation grass and bushes

0.6 m storage layer loess


0.3 m drainage layer sand
0.3 m protection layer compacted loess
0.3 m sealing layer clay
tailings
(Data in brackets indicate the thickness of cover on slopes)
Figure 7. Covering scheme for TPI and TPII

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Land Contamination & Reclamation / Volume 15 / Number 2 / 2007

Radon exhalation rate (1.5 m cover) as function of the cover saturation

1.2

Tailings saturation 0.5


Tailings saturation 0.6
1
Tailings saturation 0.8
0.74 Bq/m2s
Exhalation rate in Bq/ms
Exhalation rate in Bq/m2s2

0.8

0.6

0.4

0.2

0
0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8
Cover saturation

Figure 8. Radon exhalation as a function of soil and tailings saturation (thickness:1.5 m)

D = 0.07exp[–4(m – mn2 + m5)] (2) were determined for the selection of cover materials.
Cover construction involved the monitoring of criti-
where m is the moisture saturation, and n the porosity. cal parameters of cover layers, including moisture,
Using the recommended evaluation procedure, it degree of compaction, thickness, and hydraulic con-
can be determined that the radon flux from tailings cov- ductivity. Compaction and the thickness of the sealing
ered with soil (thickness 1.5 m) will be well below the layer were measured by a PANDA-penetrometer,
limit (0.74 Bq/m2s). This is demonstrated in Figure 8, which determines the cone resistance (MPa) depending
where the radon exhalation rate is presented for differ- on the type of material, its density and thickness. The
ent cover and tailings saturation for a cover thickness ‘handy CPT’ proved to be a valuable device for the
of 1.5 m. It can be seen that the radon flux remains determination of the homogeneity of the earth layer.
below the limit, even if the moisture content is far from Therefore, it was used for measuring both the thickness
the saturated state. of cover and the degree of compaction. For controlling
The attenuation of radon concentration for the layer the moisture of the sealing layer, a Mobile Moisture
sequence in the cover proposed for TPII is presented in Meter was used (TRIME® FM), which is recom-
Figure 9. It is deduced that the radon concentration mended for measurement of volumetric moisture in
drops very sharply in the radon barrier constructed porous material. The operating principle is based on
from clay and compacted loess, whereas the overlying measurement of the dielectric constant of materials. It
layers have only a small effect on it proved to be a reliable instrument for rapid in situ
determination of the moisture content of the soil. In situ
Cover construction measurements of hydraulic conductivity were also car-
Prior to the start of covering works, the characteristics ried out using a simple infiltrometer. These measure-
of candidate materials, including chemical–mineralog- ments were performed every 500 m2. Quality control
ical composition and soil mechanical characteristics, was carried out by MECSEKERC Zrt.

178
Application of dry covers for the closure of tailings facilities

Attenuation of radon flux in the covering


layers

4
0 0
0 0.5 1 1.5 2 2.5 3 3.5 4 4.5 5
-50 -60 3
Depth, cm

-100 -90 2
-120
1
-150 -150
T -180
-200 1 – Sealing layer, clay
-210
2 – Protecting layer, compressed loess
-250 3 – Drain, sand
2 4 – Water storage layer, loess
Radon flux, Bq/m s
T – Tailings

Figure 9. Attenuation of radon concentration in the cover

Revegetation is very important in reducing water for every month. Data are handed over to the munici-
infiltration and ensuring erosion stability. Some ero- palities.
sion gullies were formed when there was heavy rainfall
during the summer following the first covering of the Consolidation process
tailings. The revegetation scheme applied involved the To monitor the consolidation process of the tailings,
seeding of grass species at a rate of 200 kg of mixed settlement is measured monthly. 166 settlement-gauges
seeds per hectare, and the planting of bushes and trees. have been installed. The data collected are subse-
In total, 8000 plants per hectare were planted, with the quently processed and evaluated, as shown in Figure
distance between the rows being around 2.5 m. Chemi- 11.
cal fertilizers with N (120 kg/ha), P2O5 (100 kg/ha) and Based on the results, it can be seen that the largest
K2O (170 kg/ha) were also applied. Revegetated areas settlement, of approximately 1.6 m, was observed in
on tailings ponds are shown in Figure 10. the central part of the TPI on the fine tailings area, as
expected.
Monitoring
During the initial period, an intensive monitoring pro-
gramme of remediated tailings ponds was carried out. CONCLUSIONS
The performance of reclamation measures will be mon-
itored for a long time; however, the frequency of the The reclamation of tailings impoundments commonly
involves the placement of dry or water covers over the
monitoring will be decreased. Sampling and on-site
monitoring is carried out in accordance with the annual tailings. In the case of ‘dry’ rehabilitation, from a geo-
monitoring programme approved by the authorities. technical point of view, the biggest challenge is the sta-
bilization of the very fine tailings (slimes). From an
Radiological monitoring environmental perspective, the challenge is how to pre-
This work involves the measurement of radioactivity in vent acid generation in tailings containing pyrite or
the vicinity of inhabited areas; regular measurement of other sulphides, and how to control the release of con-
aerosols; and radon exhalation on the covered tailings taminants (such as As, Ra, U, Ni, etc.).
ponds. A monitoring station was installed in the nearby There are a number of dry cover systems that can be
villages for continuous monitoring of the ambient considered for use in the closure of tailings facilities.
gamma dose rate; the concentration of radon and its The applicability of the options depends mainly on the
daughter elements; long-lived alpha-contamination of conditions present at the site. Factors such as climate,
aerosols, and a cumulative additional dose is calculated physical–geotechnical/geochemical properties and

179
Land Contamination & Reclamation / Volume 15 / Number 2 / 2007

Figure 10. Establishment of vegetation on TPI

0.08
0.04
0
-0.08
-0.16
-0.24
-0.32
-0.4
-0.48
-0.56
-0.64
-0.72
-0.8
-1.2
-1.6
-1.9

Figure 11. Monitoring of the consolidation process (settlement) on tailings piles

180
Application of dry covers for the closure of tailings facilities

environmental risks associated with the disposal area, and GROWTH (Contract No. G1RD-CT-2001-00480)
the availability of potential cover materials and the cost of the 5th Framework Programme for Research and
will influence the options applicable at a given site. Technological Development.
A low-permeability clay layer historically applied
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International Atomic Energy Agency (IAEA) (1992)
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