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E-mail address: sylvia@igcar.gov.in (J.I. Sylvia).
reactive with air and catches re depending on the temperature
of sodium. Temperature in the plant ranges from150
C to 550
C.
Leaked sodium also reacts with concrete leading to damage and
loss of strength. Steam/water leak into sodium in steam genera-
tor produces hydrogen and leads to high pressure and temperature
in the system. Even though these systems are designed to make
sodium leak most improbable, it is essential to detect the leaks at
anearly stage. Detectors are providedsuchthat leak is detectedand
contained before any possible damage could occur.
As per standards on performance requirements for sodiumleak
detectors stipulated by ASME Boiler and Pressure Vessel Code, Sec-
tion XI, Division 3; a leak rate of 100g/h of sodium in air lled
vaults must be detected in 20h and a leak in inert vault within
250h.
2. Detectors based on electrical conductivity of sodium
Wire type, spark plug type and Extended spark plug type leak
detectors (ESPLD) work on the principle of electrical conductiv-
ity of sodium. The detector wire or detector electrode makes a
short circuit during sodiumleak with the pipeline which is already
electrically earthed and results in grounding.
0029-5493/$ see front matter 2012 Elsevier B.V. All rights reserved.
http://dx.doi.org/10.1016/j.nucengdes.2012.04.010
420 J.I. Sylvia et al. / Nuclear Engineering and Design 249 (2012) 419431
Fig. 1. Wire type leak detector.
2.1. Wire type leak detection system
This is the simplest method of leak detection systememployed
in the experimental sodiumsystems, single walled pipelines, com-
ponents and tanks of secondary system of PFBR. It consists of a
metallic Nickel wire insulated with ceramic bead insulators. The
cross shapedceramic insulator is stung over the wire andthis string
is laidonthesurfaceof thepipeall alongits lengthas showninFig. 1.
The exposed portion of the wire is in close proximity to the pipe
surface. Sodium leaks from the pipe make contact with the wire
and bridges the small air gap between the wire and the pipe sur-
face results in earthing. The electronics systemdetects the earthing
and gives sodiumleak alarm.
In order to make the leak system more effective, the ceramic
insulatedwireis laidunderneaththehorizontal pipelines of smaller
diameter. For larger pipes of sizes 250mmandabove(not invertical
run) the wire type leak detectors are provided at 90
, 180
and
270
taking top as 0
C
and the reading is taken fromthe probe (secondary output is mea-
sured in mV). Then the sodium level is quickly drained below the
guide tube end and the reading is again taken. The difference in
readings is the reduction in secondary output of MI probe. This
operationis for one temperature and frequency. Similarly the oper-
ations have to be repeated for temperature upto 550
C in steps
of 50
C to 550
C
the sensitivity is maximum of 49.5% at a frequency of 5.25kHz.
Sodiumtests of the probe have revealed a sensitivity ranging from
40 to 50% over the sodium temperature range of 150550
C and
the electronics is provided with alarmthreshold corresponding to
the probe output at 550
C.
Fig. 8. Experimental setup & probe.
J.I. Sylvia et al. / Nuclear Engineering and Design 249 (2012) 419431 425
Fig. 10. Assembly drawing of DSRDMleak detector.
The above assembly is qualied in three stages. Before fabri-
cation, chemical composition of raw materials and dimensional
checks are carried out, welding procedures are qualied and
approved. During fabricationdimensional checkof fabricatedparts,
surface treatments and welding qualication are carried out. After
fabrication, visual inspection and Liquid penetrant inspection of
weld joints, dimensional inspection of nal assembly, and perfor-
mance checking of sensor were carried out. Three numbers of leak
detectors are successfully fabricated with qualication procedures
as showninFig. 11. Thesensor was not onlyindigenouslydeveloped
and fabricated but also l it was nally installed inside the DSRDM
for deployment in PFBR.
3.3. MI type leak detector for double walled pipeline
In the double wall piping the leaking sodium spreads and
reaches the pocket since the piping is with little inclination. Since
the guard pipe is provided with pockets for every compartment,
the maximum distance sodium is to travel is the length of the
compartment before reaching the pocket. MI type leak detectors
are provided where the leaked sodium gets collected in a pocket
designed for the purpose. The main function of the MI type leak
detector is to detect the leak of sodium from the main pipe line
into the annulus space lled with Nitrogen envelope in the pipe.
The primary and secondary coils of the detector are wound on
a cylindrical bobbin of length 22mmand diameter of 32mmusing
SS sheathed 1mm dia. MI cable, with copper conductor and mag-
nesium oxide insulation. The sensitive portion of the detector is
of hollowcylindrical cross section made of SS316. This detector as
shown in Fig. 12 is a probe type, which can be kept inserted into a
thimble fromthe pocket bottom.
The electronics as shown in Fig. 13 is made simple as tempera-
ture compensation over an operating range from150
C to 550
C is
not required as the length of the probe is much smaller. The sodium
leak of the order of 100gm/h can be detected in a few hours with
this detector.
4. Sodiumionization detector (SID)
SIDis usedas global leakdetectionsysteminPFBRsecondarycir-
cuit area. Details of developmental works related to SID is given in
Elumalai et al. (1984). Sodiumcooled fast reactors have numerous
requirements for instrumentation capable of detecting the leakage
of sodium from component or piping faults into the surrounding
gaseous atmosphere. Detection of these leaks by a sensitive early
warning system is highly desirable to limit piping deterioration,
component destruction, re damage or corrosive effects from the
sodium. The amount of oxygenandwater impurities guarantee that
any leaking sodiumwill be partially reacted to oxide or hydroxides
and that sodium aerosol will be generated in addition to sodium
vapour. Therefore the leak detector should be capable of respond-
ing to sodium compounds as well as to elemental sodium. One of
the major advantages of SIDis its operating simplicity. Detection of
leak is obtained under ambient atmospheric conditions.
Fig. 11. Photograph of DSRDMleak detector.
426 J.I. Sylvia et al. / Nuclear Engineering and Design 249 (2012) 419431
Fig. 12. Leak detector for double walled pipeline.
Fig. 13. Electronics for MILD.
4.1. Theory of operation
The SID works on the principle of preferential ionization of
aerosols of sodium and its compounds (oxides and hydroxides) in
carrier gases such as argon, nitrogen and air. The schematic of SID
is as shown in Fig. 14. The detector carries a heated lament on
which the sodium aerosols in the carrier gas fall and get ionized.
These ions are then collected on an adjacent electrode which is
maintained at a negative potential relative to the lament, leading
to readily detectable current. In the absence of an easily ionisable
substance like sodium near the lament, the SID produces only
a small background current, arising primarily from alkali metal
impurities inthe lament material as discussedinRef. Bauerle et al.
(1976).
The most critical and also the most complex aspect of SID oper-
ation involve the detailed processes by which the sodiumparticles
are converted to free sodiumions. This can be thought of as occur-
ring in the following steps:
[1] The collision of sodiumparticles with the hot lament surface
and their subsequent Melting. The rapid surface diffusion of the
melted sodium over the lament to form a layer of adsorbed
sodiumatoms
[2] The transfer of valence electrons from some of the adsorbed
sodium atoms to the lament, converting them to adsorbed
sodiumions
[3] The desorptionof these sodiumions fromthe surface tobecome
free ions; also the desorption of neutral sodiumatoms.
The rst andsecondsteps produce a monolayer of sodiumatoms
in the lament surface. In the third and fourth steps, these atoms
are theneither thermallyionizedtobecome free sodiumions, or are
evaporated as neutral sodiumatoms. Only the free ions contribute
to the SID response. Temperature of the lament contributes to
the ionization efciency. The work function of the lament metal
Fig. 14. Schematic of SID.
J.I. Sylvia et al. / Nuclear Engineering and Design 249 (2012) 419431 427
Fig. 15. Photograph of SID.
surface should be greater or comparable to the ionizationefciency
of the sodiumatoms.
4.2. Sensor design
The optimumsensor designusedinPFBRis toachieve maximum
sensitivity with minimumbackground sodiumion current. The SID
as shown in Fig. 15 scores over other detectors in the sense that it
can detect a quantity of as lowas one nanogramof sodiumpresent
in a cubic centimeter of carrier gas.
Filament used : platinumlament of 50mmlong, 25
micron thick and 1mmwidth
Collector plate material : perforated cylinder made of Stainless
Steel (12mmOD 10mmID, 35mm
long) 1.8mmdia perforated hole
Filament to collector spacing : 5mm
Collector voltage : 200V
Filament temperature : 9501000
C
Carrier gas ow : 1l/min
Maximumbackground current : 0.08nA
Sensitivity : varies from0.1 to 1 nanoampere per
nanogramof sodiumper cubic
centimeter of gas
Minimumdetectable sodium
concentration
: better than 0.3 nanogramof sodium
per cubic centimetre of gas
4.3. Electronics for the SID
The electronics unit for the SID consists of
[1] an adjustable current source for heating the lament
[2] a mediumvoltage power supply to provide the electric eld for
collecting the sodiumions
[3] a wide range electrometer (10
12
to 10
6
ampere) for measur-
ing sodiumion current
[4] Thermal cycling circuitry to maintain the sensitivity of the la-
ment
The electronics chassis was qualied for immunity level to EMI
noise. To maintain the sensitivity of the lament, thermal cycling
circuit has also been incorporated in the SID electronics.
4.4. Sampling system
The SID system consists of SID sensor and the sampling sys-
tem with uted pipelines as shown in Fig. 16. Hence a single
detector can cater to many locations through sampling of the
carrier gas. The inherent response time of the SID to a single
Fig. 16. SID as area monitoring.
428 J.I. Sylvia et al. / Nuclear Engineering and Design 249 (2012) 419431
Fig. 17. Sensitivity of SID with long sampling lines.
aerosol particle should be comparable to the ion drift time between
the lament and the collector, typically less than a millisecond.
In a practical detection system employing aerosol sampling line,
however the time response is controlled by the much slower
processes of gas ow to the sensor chamber and mixing in the
chamber as discussed in Swaminathan and Elumalai (1984). The
sensitivity of SID system using long sampling lines, has been
demonstrated experimentally as shown in Fig. 17. The SID work-
ing on sampling method has been used in experimental area and
secondary circuit area of PFBR. The installation of SID is shown
in Fig. 18. The response of SID to burning 5g of sodium in the
experimental area is shown in Fig. 19. Every time the test is car-
ried out, the alarm threshold set at 1nA is exceeded by the SID
response, conrming the sensitivity and effectiveness of the SID
system.
During the operation of SID system it was observed that
there was an increase in background value crossing the thresh-
old limit. After cleaning the sensor, sampling lines and blower
with water the background started coming down. As part of the
surveillance periodic cleaning of sensor and sampling system is
recommended.
Fig. 18. Installation of SID.
Fig. 19. Sodiumre test.
5. Cross wire type leak detector
The main function of the Cross Wire type Leak Detector (CWLD)
is to detect the discharge of sodiumand its reaction products at the
downstreamof the rupture disc due to bursting of the rupture disc.
This provides the informationonsodiumwater reactioncauseddue
to water/steamleak inthe SteamGenerator (SG) and the developed
hydrogen gas pressure bursts the rupture disc. Literature survey
shows that this type of sensor is deployed in Monju reactor works
on bursting technique as in Takahashi et al. (1983). These S. S. foils
are located at the downstream of the rupture disc in the vertical
pipe as shown in Fig. 20. When sodium/sodium reaction products
ow past the S. S. foils break themand the loss of electrical conti-
nuity of the foils is detected and alarm signal is given. The CWLD
was designed with following specication and the functionality
was checked in experimental water test setup.
5.1. Sizing of SS foil
Based on calculations the width and thickness of the SS foil
were xed to 15mm& 50 microns respectively. Experiments were
carried out to optimize the design of the foil. Based on these exper-
iments, the depth and number of V-notches were determined. The
effect of thermal stress in the foil due to the temperature difference
between pipe and foil was studied by numerical simulation. It was
foundthat, inorder toavoidyieldingof the foil due tothermal stress
J.I. Sylvia et al. / Nuclear Engineering and Design 249 (2012) 419431 429
Fig. 20. Location of CWLD.
Fig. 21. Dimensions of CWLD.
430 J.I. Sylvia et al. / Nuclear Engineering and Design 249 (2012) 419431
the foil temperature (whichwill be nearly equal to the temperature
of argongas surrounding the foil) shouldbe limitedto 15
Conly. As
this is difcult toachieve, slight extra length(23mm) of foil will be
provided. This will prevent any thermal stress getting developed in
the foil and thus prevent the breakage of the foil due to differential
temperature.
5.2. Specication of SS Foil
Material : SS304
Length of foil : 338mm
Width of foil : 15mm
Thickness : 0.05mm
Number of V notches : 7 NOS.
Depth of V notches : 6mm
V notches are kept at a distance of 40mmas shown in Fig. 21.
5.3. Experimental setup
In order to validate the design, experiment was carried out. The
experimental test set up for testing the S.S. foils along with the
detector electronics is shown in Fig. 22. The tests were carried out
in a water loop in Engineering Hall-II by suddenly allowing water
at some pressure to owover the foils. To measure the pressure in
the pipeline at the time of opening of the valve, a dynamic pressure
Fig. 22. Experimental test setup of CWLD.
transmitter is installed. Inthis set-up, all the 3 foils are installed ina
pipe at uniformgap of 10mmand 60 degree apart without making
contact with each other. To electrically insulate the foils from the
metallic pipeline, a spark plug is installed in pipe with the help of
Fig. 23. SS foils before and after breaking.
Fig. 24. Graph showing specimen vs. breaking pressure.
J.I. Sylvia et al. / Nuclear Engineering and Design 249 (2012) 419431 431
sleeves. A triangular piece welded to the central electrode of the
spark plug is used to hold the foil rmly. Electronic connections
are given to the terminals of the spark plug. Fig. 23 shows the SS
foils before and after breaking. The breaking of these SS foils are
detected electronically using two out of three logic.
It was found from the hydraulic experiments repeated over
42 trials that all the SS foils break at an average pressure of
0.150.25MPa which corresponds to a velocity of 2m/s as shown
in Fig. 24. The expected minimum pressure and velocity in PFBR
is 0.37MPa and 2m/s respectively. It is found that the results are
conservativeandthesnapping/breakingtechniqueof theCWLDhas
been demonstrated successfully.
6. Conclusion
As the commercially available conventional sensors cannot be
used for sodium leak detection, the sensors and instrumentation
are specially designed using the state-of-art technology to suit this
hostile environment. Wire type and spark plug type leak detectors
working on earthing principle is used on pipelines and different
capacities such as bellow sealed valves and leak collection trays
respectively with improved electronics in PFBRs. Miniature Mutual
Inductance type leak detectors with remote insertion/withdrawal
facility was developed for MV leak detector of PFBR. The selec-
tion of SS410 bobbin for improving the sensitivity of this sensor
was experimentally proved. ESPLDs are used as diverse method
for detecting leak in Main vessel. The sensor was assembled and
tested for its functionality and easy insertion and withdrawal. The
DSRDM leak detectors with longer length of free leads (15m) has
been fabricated, qualied and installed in the DSRDMelectromag-
net successfully. For double walled pipe line where pockets are
provided at the lowermost elevation, MI type leak detectors of
larger size was designed and used in multiple numbers. This type
of leak detector is non-intrusive and easily replaceable and hence
it gains importance for usage in the reactor systems. Sodium Ion-
isation leak detectors with improved electronics have been used
in secondary system as area monitoring in PFBR. As this sys-
tem has been employed in sodium facilities, lot of expertise has
been gained in maintaining the same. The Cross wire type leak
detectors are designed and experimentally tested at required pres-
sure of PFBR. The different types of sodium leak detectors were
designed, developed and tested in various sodiumfacilities which
gave us enough condence for deploying themin PFBR and future
FBRS.
Acknowledgements
Authors acknowledge the encouragement, guidance and sup-
port received from K. Swaminathan, Former Head, Component &
Instrumentation Development Division, FRTG, Shri S.C. Chethal,
Director, Indira Gandhi Centre for Atomic Research (IGCAR) and
all other agencies who supported during the course of this
work.
References
Bauerle, J.E., Reed, W.H., Berkey, E., 1976. Development of a sodium ionization
detector for sodium-to-gas leaks. In: International Conference on Liquid Metal
Technology in Energy Production.
Elumalai, G., et al., 1984. Development of sodiumionization detector for sodium-to-
gas leaks. In: 3rd International Conference on LMET, Oxford, UK.
Mcgonigal, G., Dean, S.A., Ferguson, B.G., Harrison, E., U.K. AEA, 1971. Measurement
of sodiumlevel in PFR. Nucl. Eng. Int. 16 (175/6), 6265.
Swaminathan, K., Elumalai, G., 1984. Development of a sodiumionization detector
for sodium-to-gas leaks. In: Liquid Metal Engineering and Technology. BNES,
London.
Takahashi, T., Ohmori, Y., Hoshi, Y., 1983. Inuence of sodium, water reaction on
MONJU steamgenerator, IWGFR/50, Netherlands.
Vijayakumar, V., et al., 2004. Sodium and Steam Generator Leak Detection for Pro-
totype Fast Breeder Reactor (PFBR), ICONE12-ICONE49362.
Vijayakumar, G., et al., 2011. Performance evaluation of PFBR wire type leak detec-
tors. Nucl. Eng. Des. 241 (2011), 22712279.