Professional Documents
Culture Documents
1, 50–67
doi: 10.1093/ce/zkx007
Advance Access Publication Date: 14 December 2017
Homepage: https://academic.oup.com/ce
Research Article
Experimental study on dense-phase pneumatic
conveying of coal powder at high pressures
Qingliang Guan*, Zhen Liu, Xinhui Fang, Bing Liu, Baozai Peng,
Ziyang Feng, Ya Suo and Wenhua Li
National Institute of Clean-and-Low-Carbon Energy, Future Science & Technology City, Changping District, Beijing
102211, China
Abstract
Clean utilization and conversion of coal resources is significant to China’s energy sustainable development.
Entrained-flow coal gasification technology is an important method used for clean and efficient conversion of
coal. The characteristics and stability of high-pressure dense-phase pneumatic conveying of pulverized coal
is crucial to the safe and stable operation of dry-feed entrained-flow coal gasifiers. Dense-phase pneumatic
conveying experiments were carried out using a high-volatile bituminous coal in pipes with diameters of 25,
15 and 10 mm, respectively, and at back pressures of 1.0–4.0 MPag. The conveying characteristics and effects of
operating and structure parameters were studied. Pressure drop models were established for horizontal and
vertical upward conveying. The prediction uncertainty was within ±30% for the horizontal conveying and ±20%
for the vertical upward conveying. The relative standard deviation of solid flow rate was proposed to explain
conveying stability. The effect of operating parameters on conveying stability was systematically analyzed. The
gas velocity-related criterion was proposed for stable conveying.
Key words: dense-phase pneumatic conveying; pulverized coal; high pressure; pressure drop; stability
and pumping of coal–water slurry is a simple and proven with pressure at constant total differential pressure and
technology. In contrast, conveying dry pulverized coal to fluidizing gas [17]. The experimental results of Lu et al.
gasifiers is more complicated and has a higher capital also showed that the mass flow rate of coal particles and
cost. However, gasifiers with dry pulverized coal feed have concentration increased at high pressures [18]. The past
advantages. The gasifiers can produce a higher content of research mainly focused on macroscopic characteristics at
CO and H2 in raw syngas with lower consumption of coal high pressures with particle flow and mechanism research
and oxygen and longer service life of burners due to less seldom reported.
erosion caused by the pulverized coal. The pipeline pressure drop is one of the most important
In dry pulverized coal-fed gasification processes, coal parameters of pneumatic conveying, and the additional
is pneumatically transported by N2 or CO2 from high-pres- pressure drop model developed by Barth [19] was widely
sure feeding vessels to gasifiers. A stable conveying of the used:
feedstock with minimum transport gas is important to in-
crease the content of CO and H2 in raw syngas and ensure ρg Ug2 ρg Ug2
∆PT / L = ∆Pg / L + ∆Ps / L = λg + µλz (1)
the stable operation of the gasifier. Therefore, high-pres- 2D 2D
sure and dense-phase pneumatic transport of pulverized
coal is a key technology for dry-feed entrained-flow coal where, ΔPT/L is the pressure drop of the gas and solid mix-
gasification. Pulverized coal conveying technology is used ture, ΔPg/L is the pressure drop of the gas phase, and ΔPs/L
in engineering applications such as the Shell [1] and the is the additional pressure drop due to the presence of the
GSP gasification processes [2, 3]; however, there remain solid particles. λg is the gas friction coefficient, λz is the
many problems. The design of a conveying system is coefficient of additional pressure drop. μ is solid loading
mostly reliant on limited empirical correlations with fun- ration, ρg is gas density, Ug is superficial gas velocity, and D
damental research insufficient for the scale-up principles. is inner diameter of pipe. The gas friction coefficient λg can
For example, due to limited knowledge on the conveying be calculated by Equation (2):
stability and reliability in larger pipes, the diameter of the
conveying pipeline is limited to 50–60 mm in current in- 0.3164 1
λg = 2320 < Re < 80 (2a)
dustrial applications. The lack of reliable methods to ac- Re0.25 e/D
curately measure the coal mass flow rate makes it difficult
to accurately control the oxygen-to-coal ratio resulting in
fluctuating gasification operation. The dense-phase con- æ ö
1 ç e 2.51 ÷÷
veying limit can also influence the gasifier operation. The = -2lg çç + ÷
λg çç 3.7D Re λ ÷÷÷
coal–water slurry fed gasifiers can be operated at pressures è g ø (2b)
0.85
up to ~8.7 MPa or even higher, while dry pulverized coal- 1 æ 1 ö÷
80 < Re < 4160 çç ÷
fed gasifiers are limited at pressures up to ~4 MPa, partly e/D èç 2e / D ÷ø
because systems of dense-phase conveying at higher pres-
sures are not yet tested or verified.
Pneumatic conveying of coal powder is a very compli- 1 1
0.85
λg = 4160 < Re
cated gas–solid two-phase flow process. Suspension flow, D
2
2e / D (2c)
dune flow, slug flow, plug flow and fluidized dense-phase 1.74 + 2lg 2e
flow phenomena may be observed as gas and solid flow
through horizontal pipes [4], and suspension flow, annular
flow, turbulent fluidization flow, bubbly flow, slug flow and where, e is the roughness of pipe wall, Re (= ρgUgD/μg) is
separated plug flow can be found as gas and solid flow Reynolds number.
through vertical upward pipes [5]. The flow pattern transi-
tions are complicated with large differences in flow mech- Determination of the coefficient of the additional pressure
anisms between different flow patterns. There is currently drop λz is key to calculate the total pressure drop of two-
no matured theory to guide the design and operation of phase flow. To calculate λz some researchers [20] used power
dense-phase pneumatic conveying systems. Therefore, functions with several nondimensional parameters derived
many researchers have built experimental facilities to from experimental data. For the suspension flow in horizon-
study the dense-phase pneumatic conveying process tal pipes, the additional pressure drop of the particle clusters
[6–16]; however, only a few facilities operate at high pres- can be expressed as the sum of pressure drop caused by par-
sures [6, 7, 10–13]. The characteristics of dense-phase ticle friction and that caused by keeping the particles sus-
pneumatic conveying may differ from dilute-phase char- pended and then was applied to dense-phase conveying [21,
acteristics due to increased gas density and enhanced 22]. Based on Yang’s unified theory [23], Wang [16] put for-
gas–solid interactions. The influence of pressure on ward implicit equations to calculate λz. The gas–solid flow for
dense-phase pneumatic conveying needs further study. dense-phase flow of fine powder in horizontal pipes tends to
The experimental results of Liang et al. showed that mass be stratified. Setia et al. [24] used a ‘two-layer’ model (two dif-
flow rate of coal particles and concentration increased ferent models) that showed good prediction performance for
Stegmaier and
Weber [25] λz = 2.1µ −0.3Frt0.5Fr −1.21 ( D / dp )−0.1
ut Ug
Frt = , Fr =
gdp gD
0.4
µ m
Gs 1
∆P / L = K
ρg D Ug
K = 106, m = 0.83 Gs / D < 47 000kg / (m3s)
K = 0.838, m = 1.2 8Gs / D > 47 000kg / (m3s)
Geldart and D = 6.25–12.5 mm, carrier gas is H2, N2
Ling [6] and CO2, P < 8.27 MPa, Gs < 2000 kg/
(m2·s)
Pan [26] λz = 1.0 µ −0.2665Fr −1.4467 ρg−0.6626 D = 69 mm, lignite, dp = 25.8 µm, carrier
gas is air, P is atmospheric pressure,
μ = 3.6–63.4
ρs (1 − ε )us2
Ps / L = fs
2D
−0.902 −1.95
(1 − ε )−0.057 Ret Ug
fs = 1.98
ε3 Rep gD
us = Ug −
(
4 ρs − ρg gdp ) fsus2 4.7
ε
3ρg CD 2gD
Wang [16] −1.80 D = 15 mm, dp = 69 µm, carrier gas is
ρ
λz = e6.35Fr −1.34 s N2, P < 1.5 MPa, Ug = 5.94–13.68 m/s,
ρg Gs = 15.8–32.8 kg/(m2·s)
He et al. [20] us 2β D = 10 mm, bituminous coal, dp = 63 µm,
λz = λs* + = 0.005 + 0.88 × 10 −4 Fr + Fr −2.16 or
Ug (us / Ug )Fr 2 P < 2.45 MPa
0.005 + 0.63Fr
−1.89
4 < Fr < 13.2
λz = −0.19
0.016Fr 13.2 < Fr < 40
m / ρ a U b * us 2β
λz = τ 1 K s s
+ τ 2 λs
f
+ 2
mg / ρg Ug
U ( u / U )Fr
g s g
Fr − Frmin Fr − Frmin
τ1 = 1 − ,τ 2 = ,
Frmax − Frmin Frmax − Frmin
Frmin = 3 − 4, Frmax = 50, β = Uf / Ug ,
K = 8.04, a = −0.22, b = 1.48, Uf = 0.06 m / s, λs* = 0.0043
Setia et al. [24] D = 69 and 105 mm, fly ash (ρs = 2300 kg/
m3, ρb = 700 kg/m3, dp = 30 µm), carrier
gas is air, P is atmospheric pressure
P
3
2 11 7
8
P P
1 15
4 5
12 17
16
9
13 14
P dP
Gas
Gas and particles 10
6
Fig. 2 Flow diagram of the dense-phase conveying system. 1, nitrogen tank; 2, pressure reducing valve; 3, storage vessel; 4, delivery vessel; 5, receiv-
ing vessel; 6, conveying pipeline; 7, dust collector; 8, pressurizing gas; 9, fluidizing gas; 10, supplementary gas; 11, relieving gas; 12, load cell; 13,
pressure transducer; 14, differential pressure transducer; 15, solid mass flowmeter; 16, gas flowmeter; 17, regulating valve
1 dP
Pipe material 20# carbon steel
P dP
P
dP
dP
a bag filter. The delivery vessel and receiving vessel are inter- Table 5 Proximate and ultimate analysis of Shanbei coal
changeable, and coal powder is circulated inside the convey-
Parameter Value Parameter Value
ing system. New coal material is fed into the delivery vessel
by the screw feeder system, and used coal material can be Mar (%) 6.44 Cdaf (%) 82.46
discharged from the bottom of the bag filter. Parameters of Vdaf (%) 39.48 Hdaf (%) 4.78
the experimental facility are shown in Table 3. FCd (%) 55.66 Odaf (%) 11.49
The flow rate of supplementary gas is measured by vor- Ad (%) 8.03 Ndaf (%) 0.96
tex flowmeters, and the flow rates of pressurizing gas and Qnet, ar (MJ/kg) 25.96 Sdaf (%) 0.30
fluidizing gas are measured by mass flowmeters. Seven
pressure transducers and eight differential pressure trans- Q = Q p + Q f + Q s − Ms / ρs (4)
g
ducers are installed along the conveying line, as shown in
Fig. 3. The weights of vessels are measured by load cells
and are used to calculate the average solid flow rate during Qg Qg
Ug = = (5)
a period of time. The instantaneous solid flow rate is meas- A 0.25π D2
ured by the solid mass flowmeter of Thermo Ramsey, which
consists of a velocity sensor, a concentration sensor and Where Qp is volume flow rate of pressurizing gas, Qf is vol-
an integrator. The output signals of measuring instruments ume flow rate of fluidizing gas, Qs is volume flow rate of
are converted by A/D converters and then recorded by a PLC supplementary gas, ρs is particle density.
control system at a frequency of 2 Hz. Main parameters of
measuring instruments are shown in Table 4. It is worth noting that Qg and Ug are dependent on local
The conveying material is a high-volatile bituminous coal pressure and thus changed at different positions. The solid
from China, as shown in Table 5. Properties of coal particles loading ratio µ was calculated by Equation (6):
and parameters of flowability are shown in Table 6. Fig. 4
Ms
shows the particle size distribution of coal particles. The µ=
ρgQ g (6)
particles are cohesive [34–36] since the compressibility is
between 30 and 50%, the angle of repose is between 45° and There is currently no common definition for dense phase.
55° and the flow function is between 4 and 10. According to The solid loading ratio is widely used. For example, µ >
Geldart’s classification [37], the particles are A-type particles 10 was used by Klinzing and Mathur [39] as an indica-
and are suitable for dense-phase pneumatic conveying [35]. tor for dense phase. However, the solid loading ratio is
According to Pan’s classification [38], the particles are PC1- influenced by properties of solid particles and carrier
type particles and can be transported smoothly and gently gas. Gas density changed greatly as the pressure varied
from dilute phase to fluidized dense phase. in the experiments, so solid loading ratio alone was not
suitable. Many researchers regarded the region of super-
ficial gas velocity larger than the saltation velocity as the
1.2 Data processing
dense-phase region based on Zenz’s diagram [40], which
The slopes of weight loss curves and weight gain curves of was inconvenient for use. The particle concentration of
the vessels were calculated as average solid flow rate and dense-phase conveying of coal powder is 400 and 300–
were used to calibrate the instantaneous mass flow rate Ms 500 kg/m3 for Shell gasifiers [41] and GSP gasifiers [33],
and concentration C, which were measured by the solid mass respectively. Therefore, in this article, dense-phase region
flowmeter. The solid mass flux was calculated by Equation (3): is considered where particle concentration is larger than
Ms Ms 300 kg/m3.
Gs = = (3) Table 7 lists the experimental range of pneumatic con-
A 0.25π D2
veying. Most of the experiments were in the dense-phase
where the volume flow rate of carrier gas (Qg) and superfi- region for 25 and 15 mm pipes, while experiments were in
cial gas velocity (Ug) are as follows: dilute-phase region for 10 mm pipe.
External moisture content (%) 4.84 Median particle diameter (µm) 35.3
Internal moisture content (%) 1.60 Compressibility (%) 39.2
Particle density (kg/m3) 1449 Angle of repose (°) 48
Tap density (kg/m3) 852 Angle of wall friction (°) 27
Loosely packed density (kg/m3) 518 Flow function 3.1
5 Diameter of pipe mm 25 15 10
Volume percentage (%)
Fig. 4 Particle size distributions of coal particles with total differential pressure, as shown in Fig. 5a and b.
It is worth noting that critical velocity increased with solid
flow rate (total differential pressure), which is the same as
2 Results and discussion the conclusion of former researcher [42].
At back pressures of 2.5 and 4.0 MPag, no remarkable
2.1 Characteristics of high-pressure dense-phase
effects of back pressure on solid mass flux curves and solid
conveying
concentration curves were found in the region of low gas vel-
Diagram of conveying was widely used to investigate the ocity, and back pressure hardly affected the value of critical
characteristics of high-pressure dense-phase conveying. In velocity, as shown in Fig. 5a and b. However, in the region of
the diagram, the pressure drop per unit length was plotted high gas velocity, solid flow rate was lower at high back pres-
against the superficial gas velocity with the solid flow rate sures, which was due to higher pressure drops of gas phase
as a parameter, or the solid flow rate was plotted against as gas density increased at high back pressures, as shown in
the superficial gas velocity with the total differential pres- Fig. 5a. Thus, conveying of coal powder would be affected by
sure as a parameter. The latter method was chosen in this pressure through gas density, especially in the dilute-phase
article because it is convenient to control the pressure dif- region.
ference between the delivery vessel and receiving vessel in At back pressure of 1.0 MPag, first of all, the trend of
the experimental facility. a slow increase followed by a rapid increase of solid con-
Fig. 5 showed the effect of operating parameters on centration with decreasing gas velocity was more notice-
conveying characteristics. At a constant back pressure and able, as shown in Fig. 5b; second, solid mass flux was lower
total differential pressure, the solid flow rate increased to for 1.0 MPag at the region of low gas velocity, as shown
a maximum and decreased as the superficial gas velocity in Fig. 5a. One possible explanation was that coal parti-
decreased, as shown in Fig. 5a. The superficial gas velocity cles were more likely to deposit in the bottom of hori-
at the maximum solid flow rate was a critical velocity. When zontal pipes at 1.0 MPag, due to larger density differences
superficial gas velocity was high, the flow was in a dilute- between solid particles and gas. Therefore, the transition
phase region with low solid concentrations, and the pres- of flow patterns from dilute-phase suspension flow to non-
sure drop of the gas phase was the main part of the total uniform stratified flow gave rise to more sharp transitions
pressure drop. As the gas velocity decreased, the pressure of solid concentration curves. Moreover, the effective sec-
drop of the gas phase decreased and the solid flow rate tional area of pipes decreased as coal particles deposited,
increased. As gas velocity decreased further, solid concen- which resulted in lower solid mass fluxes at 1 MPag.
tration increased rapidly and the inter-particles and par- Fig. 6 showed the effect of operating parameters on
ticle–wall friction resistance, which resulted in an increased particle velocity. The results showed that the particle
pressure drop due to particles and decreased solid flow rate. velocity decreased with decreasing local superficial gas
Total differential pressure was the main driver for con- velocity, and the particle velocity was lower than the local
veying coal particles. At a constant back pressure and gas superficial gas velocity. The variation of velocity differ-
velocity, solid flow rate and solid concentration increased ence between local superficial gas velocity and particle
of 2.5 and 4.0 MPag, the transition took place at critical veloc-
14
ity, whereas at a lower back pressure and lower solid flow
12 rate, the transition was more obvious and took place at a gas
Particle velocity (m/s)
5 5 5
Velocity difference between 1.0MPag 1.0MPag 1.0MPag
2 2 2
critical velocity critical velocity critical velocity
1 1 1
0 0 0
0 2 4 6 8 10 12 14 0 2 4 6 8 10 12 14 0 2 4 6 8 10 12 14
Average superficial gas velocity (m/s) Average superficial gas velocity (m/s) Average superficial gas velocity (m/s)
Fig. 7 Velocity difference between local Ug and us versus average superficial gas velocity (D = 25 mm, L = 197 m)
2000
1.0MPag 4000 10mm
2.5MPag 15mm
25mm
3000
L=108m
1200 2000
0
400 3 6 9 12 15
0 3 6 9 12 15
Average superficial gas velocity (m/s)
Average superficial gas velocity (m/s)
Fig. 9 Effect of pipe diameter on solid flow rate (L = 108 m, P = 2.5 MPag,
Fig. 8 Effect of conveying distance on solid mass flux (D = 25 mm,
∆P = 0.75 MPa)
∆P = 0.75 MPa)
near atmospheric pressures, while in this article, the carrier loading ratio (µ), the density ratio of solid to gas ( ρs / ρg ), the
gas was nitrogen and conveying pressure exceeded 1 MPa. Reynolds number (Re), the Froude number (Fr) and the diam-
It should be noted that pipe diameters were in the range of eter ratio ( dp / D ). The solid loading ratio was correlated with
15–26 mm in Guo et al.’s experiments, which was very simi- the solid concentration: a higher solid loading ratio indicated
lar to those in this article. In addition, in Mittal et al.’s and a higher solid concentration, and thus higher frequencies of
Setia et al.’s experiments, carrier gas was also air, conveying particle–particle and particle–wall inelastic collisions, which
material was fly ash, conveying pressure was near atmos- would result in larger momentum losses. The density ratio of
pheric pressure and pipe diameter was 69 and 105 mm. solid to gas was used to represent the particle-carrying capac-
While the experimental conditions were very different from ity in dilute suspension flow [44]. The Reynolds number rep-
those in this article, those models still gave better results. resented the ratio of inertia forces to viscous forces and could
Comparisons of pressure drop per unit length between be used to represent the change of turbulent kinetic energy
experimental data and model calculations from Table 2 for of the carrier gas as operating parameters varied. The Froude
vertical upward pipes are shown in Fig. 11. It was shown that number represented the ratio of inertia forces to gravity and
Zhou et al.’s and Wang et al.’s model underpredicted the pres- could be used to represent the effect of gravity on conveying.
sure drop, while predictions of Pu et al.’s and He et al.’s model The effect of gravity was larger at lower gas velocities; thus,
diverged for pipes of different diameters. Guo’s model was solid particles were more likely to deposit on the bottom of
in agreement with experimental data within the deviation horizontal pipes and flow backward along the wall of vertical
of ±50%, which is the best among all the models investigated upward pipes, which could affect the pressure drop of the gas–
although it was developed from very different experimental solid mixture. The diameter ratio in fact represented merely
conditions from this article, as shown in Table 2. the effect of pipe diameter, such as those due to wall rough-
Since the predictive ability of existing models was not yet ness of different pipes, since the particle size was constant in
adequate for engineering applications, a new additional pres- this article.
sure drop model was developed in this article. Several non- The coefficient of the additional pressure drop was
dimensional parameters were analyzed, including the solid regressed with experimental data using the power
30 30 30
25mm +50% 25mm +50% 25mm +50%
15 15 15
5 5 5
0 0 0
0 5 10 15 20 25 30 0 5 10 15 20 25 30 0 5 10 15 20 25 30
Experimental measurement (kPa/m) Experimental measurement (kPa/m) Experimental measurement (kPa/m)
(a) Stegmaier and Weber (b) Geldart and Ling (c) Pan
30 30 30
25mm +50% 25mm +50% 25mm +50%
Model calculation (kPa/m)
15 15 15
5 5 5
0 0 0
0 5 10 15 20 25 30 0 5 10 15 20 25 30 0 5 10 15 20 25 30
Experimental measurement (kPa/m) Experimental measurement (kPa/m) Experimental measurement (kPa/m)
30 30 30
25mm +50% 25mm +50% 25mm +50%
Model calculation (kPa/m)
15 15 15
5 5 5
0 0 0
0 5 10 15 20 25 30 0 5 10 15 20 25 30 0 5 10 15 20 25 30
Experimental measurement (kPa/m) Experimental measurement (kPa/m) Experimental measurement (kPa/m)
Fig. 10 Comparisons of pressure drop per unit length between experimental data and model calculations from Table 1 for horizontal pipes
18 18 18
25mm +50% 25mm +50% 25mm +50%
9 9 9
3 3 3
0 0 0
0 3 6 9 12 15 18 0 3 6 9 12 15 18 0 3 6 9 12 15 18
Experimental measurement (kPa/m) Experimental measurement (kPa/m) Experimental measurement (kPa/m)
18 18
25mm +50% 25mm +50%
Model calculation (kPa/m)
9 9
6 -50% 6 -50%
3 3
0 0
0 3 6 9 12 15 18 0 3 6 9 12 15 18
Experimental measurement (kPa/m) Experimental measurement (kPa/m)
Fig. 11 Comparisons of pressure drop per unit length between experimental data and model calculations from Table 2 for vertical upward pipes
0.12 0.12
Experiment (25 mm) Experiment (25 mm)
0.10 Experiment (15 mm) 0.10 Experiment (15 mm)
Experiment (10 mm) Experiment (10 mm)
0.08 Calculation 0.08 Calculation
0.06 0.06
λz
λz
0.04 0.04
0.02 0.02
0.00 0.00
-0.02 -0.02
0 5 10 15 20 25 30 35 40 0 10 20 30 40 50 60
Fr Fr
high-pressure conveying. It was likely that pressure could In horizontal pipes, additional pressure drop was
influence the pressure drop of gas–solid two-phase flow mainly solid frictional pressure drop, while in vertical
only through gas density and dynamic head. Comparisons upward pipes, additional pressure drop also included solid
of pressure drop per unit length between experimental gravitational pressure drop. Thus, solid frictional pressure
data and model calculations are shown in Fig. 13. It was drop could be calculated from total pressure drop as in
shown that the developed models from this article agreed Equations (12) and (13):
with experimental data within ±30% for horizontal pipes
and ±20% for vertical upward pipes, which showed better
∆PsfH / ∆L = ∆Ps / ∆L = ∆PT / ∆L − ∆Pg / ∆L (12)
performance than previous models.
30 15
25mm +20%
25 25mm +30% 15mm
12
0 0
0 5 10 15 20 25 30 0 3 6 9 12 15
Experimental measurement (kPa/m) Experimental measurement (kPa/m)
Fig. 13 Comparisons of pressure drop per unit length between experimental data and model calculations
(a) 15 (b) 3.0
25mm 25mm
9 1.5
6 1.0
0.5
3
0
0 −0.5
−3 0 3 6 9 12 15 0 10 20 30 40 50 60
∆P Vsf/∆L (kPa/m) Fr
Fig. 14 Comparisons of solid frictional pressure drop between horizontal and vertical upward pipes
∆PsfV / ∆L = ∆Ps / ∆L − ∆Psg / ∆L = ∆PT / ∆L − ∆Pg / ∆L − ∆Psg / ∆L due to the increased normal stress resulted from grav-
ity. In addition, the difference of solid frictional pres-
(13)
sure drop between horizontal pipes and vertical upward
pipes was larger at a lower Froude number as shown in
where solid gravitational pressure drop was calculated by Fig. 14b due to more coal particles tending to deposition.
Equation (14) When the Froude number was very low, negative values
occurred for the solid frictional pressure drop in vertical
Ms g 1 Gs g
∆Psg / ∆L = ≈ upward pipes, as shown in Fig. 14a. That was considered
A us Ug (14)
to be the result of a change of the direction of the shear
force due to the backflow of particles in vertical upward
Comparisons of solid frictional pressure drop between
flow when gas velocity was very low [15]. The phenom-
horizontal and vertical upward pipes are shown in
enon had been observed during experiments [45].
Fig. 14, where solid frictional pressure drop of horizontal
pipes was calculated from Equation (10) and that of verti-
cal upward pipes was calculated from Equations (13) and 2.3 Conveying stability
(14). It was shown that solid frictional pressure drop of Unstable conveying of coal powder always occurred
horizontal pipes was larger than that of vertical upwards with simultaneous signal fluctuations. For discrete
pipes, except for some data from 25 mm pipeline. That signal data series ( y1 , y2 , yN ) , the average fluctuation
was because the deposition of coal particles on the bot- amplitude was represented by its RSD as calculated by
tom of horizontal pipes increased particle–wall friction Equation (15), and its maximum FR was calculated by
0.25 250%
y=5.9x
0.02 0.20 200%
RSD(Ph)
RSD(∆ Ph)
FR(Ms)
0.15 150%
0.05 50%
0 0 0%
0 0.1 0.2 0.3 0.4 0 0.1 0.2 0.3 0.4 0 0.1 0.2 0.3 0.4
RSD(Ms) RSD(Ms) RSD(Ms)
P1 1400 1200
Ph 4
4.2 1200 3
1000
∆Ph/∆L (kPa/m)
Pressure(MPag)
Ms 1000 3 800
C(kg/m3)
Ms(kg/h)
us(m/s)
4.1 800 2
us 2 600
600
∆Ph/∆ L 400
4.0 P2
400 1
1
200 200
C
3.9 0 0 0 0
0 1 2 3 4 5 6
Time(min)
Fig. 16 Signal fluctuations of experimental condition A (D = 25 mm, P1 = 4.25 MPag, P2 = 4 MPag, Qf = 20 Nm3/h, Qs = 188 Nm3/h)
Ms 1000 3 800
C(kg/m3)
Ms(kg/h)
us(m/s)
4.1 800 2
us 2 600
600
∆Ph/∆ L 400
4.0 P2 400 1
1
C 200 200
3.9 0 0 0 0
0 1 2 3
Time(min)
Fig. 17 Signal fluctuations of experimental condition B (D = 25 mm, P1 = 4.25 MPag, P2 = 4 MPag, Qf = 20 Nm3/h, Qs = 168 Nm3/h)
Equation (16). RSD and FR were used to represent the Three representative signals were investigated to study
fluctuation of signals. the conveying stability, including the pressure of a hori-
zontal pipe (Ph), the pressure drop per unit length of a hori-
1 zontal pipe (ΔPh/ΔL) and solid flow rate (Ms). Comparisons
∑ ( y − y)2
N
N − 1 i=1 i 1 N (15)
RSD( y) =
y
, y= ∑yi
N i=1
of fluctuation calculated from the three signals are shown
in Fig. 15. It was shown that RSD(Ph) was the smallest and
was one magnitude smaller than RSD(ΔPh/ΔL) and RSD(Ms).
The value of pressure fluctuations was small compared
max( yi ) − min( yi ) with the value of the pressure itself. The fluctuation of pres-
FR( y) = × 100% (16)
y sure drop and solid flow rate was in the same order of
RSD(us) or RSD(C)
while RSD(Ms) was substantially correlated with FR(Ms). The
value of FR(Ms) was ~5.9 times that of RSD(Ms), as shown in
0.2
Fig. 15c, which was similar to the case in Shell gasifiers [1].
The stable supply of feedstock in industrial gasifiers
required that the solid flow rate of coal was stable, so y=0.63x, R 2=0.86
as to match with the flow rate of oxygen and keep the 0.1
oxygen-to-coal ratio stable. The average fluctuation ampli-
tude could be used to denote the operating stability of gas-
ifiers in long-term runs, while the maximum FR could be 0.0
used to denote the possibility of triggering the interlocks 0.0 0.1 0.2 0.3 0.4
and causing unplanned shutdown. Based on the above- RSD(Ms)
mentioned analysis, RSD of the solid flow rate signal was
Fig. 18 Comparisons of RSDs of solid flow rate, particle velocity and
used as an indicator for conveying stability in this article.
solid concentration
Signal fluctuations of two experiments with similar
conditions are shown in Figs 16 and 17. In the experiments,
differences were found for the RSD of solid flow rate, indi-
the pressure of the delivery vessel and the receiving vessel
cating that there were minor effects of solid loading ratio
was controlled by control valves. When the vessel pressure
on conveying stability for 25 mm pipes in this article.
was not well controlled, periodic fluctuations occurred,
The effect of back pressure on conveying stability for
which led to similar periodic fluctuations of signals in the
25 mm pipes is shown in Fig. 20. It was shown that at the
conveying pipeline, as shown in Fig. 16. The conveying in-
same gas velocity, there were no big differences in solid con-
stability induced by fluctuations of the vessel pressure
centrations between different back pressures, although solid
had been observed by many researchers [33]. Fluctuations
concentration was a little bit lower at 1.0 MPag. When solid
of the vessel pressure would result in fluctuations of the
concentration was high, such as those higher than 300 kg/m3,
total differential pressure, which had a direct impact on
there were no obvious differences in conveying stability
the solid flow rate. After the pressure control strategy was
between different back pressures. While when solid concen-
improved and periodic fluctuations of vessel pressure were
tration was low, more stable conveying could be achieved at
diminished, no obvious periodic fluctuations of signals in
higher back pressures. That was because gas density was
the conveying pipeline could be observed, as shown in
higher and particle-carrying capacity of gas was larger at
Fig. 17. The conveying stability improved since RSDs of all
higher back pressures, making it easier for suspending the
the signals investigated decreased, as shown in Table 8.
particles and thus enhancing the conveying stability.
Comparisons of RSDs of solid flow rate, particle velocity
Variations in RSD(Ms) with superficial gas velocity for
and solid concentration are shown in Fig. 18. It was shown
pipes of different diameters are shown in Fig. 21. There
that RSD(Ms), RSD(us) and RSD(C) were in the same order
was a trend that RSD(Ms) increased as superficial gas vel-
of magnitude, and generally, RSD(us) < RSD(Ms) < RSD(C).
ocity decreased. It was shown that when superficial gas
Besides, RSD(C) was in a stronger correlation with RSD(Ms)
velocity was lower than ~6 m/s for 25 mm pipes and 8 m/s
than RSD(us) was in with RSD(Ms), which demonstrated that
for 15 mm pipes, RSD(Ms) increased rapidly and might
the fluctuation of solid flow rate was mainly caused by the
exceed 7%, which was regarded as unstable conveying in
fluctuation of solid concentration. That was possible when
this article. It should be noted that when superficial gas
cross-sectional solid concentration fluctuated dramatically
velocity was lower than above-mentioned values, stable
in dense-phase plug flow or dune flow at horizontal pipes.
conveying with RSD(Ms) less than 7% still might appear.
The effect of solid loading ratio on conveying stability
for 25 mm pipes is shown in Fig. 19. It was shown that at
the same gas velocity, the solid loading ratio was higher 3 Conclusions
for a conveying distance of 108 m, compared with that Dense-phase pneumatic conveying of a high-volatile bitu-
for a conveying distance of 197 m. Whereas no obvious minous coal powder was carried out in an experimental
0.4 0.4
L=197m 25 L=197m 25
L=108m L=108m
RSD(Ms)
15 15
0.2 0.2
10 10
0.1 0.1
5 5
0 0 0 0
2 4 6 8 2 4 6 8
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)
0.4 15 0.4 15
L=197m L=197m
L=108m Solid loading ratio, µ(kg/kg) L=108m
0 0 0 0
2 4 6 8 2 4 6 8 10 12
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)
0.4 8 0.4 10
L=197m L=197m
L=108m L=108m
Solid loading ratio, µ(kg/kg)
RSD(Ms)
0.2 4 0.2
4
0.1 2 0.1
2
0 0 0 0
1 2 3 4 5 6 2 4 6 8
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)
facility using 25, 15, and 10 mm pipes and at back pres- and structure parameters were studied. Pressure drop
sures of 1.0–4.0 MPag. The conveying characteristics and models for horizontal pipes and vertical upward pipes
the influencing mechanism of operating parameters were established. The indicator and criterion for stable
RSD(Ms)
200 200
0.08 0.08
100 100
0.04 0 0.04 0
0 -100 0 -100
2 4 6 8 2 4 6 8
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)
(a) ∆P=0.50MPa, L=197m (b) ∆P=0.75MPa, L=197m
300 RSD(Ms)
0.2 300
0.08 200
200
100
0.1
0.04 100
0
0 -100 0 0
2 4 6 8 2 4 6 8 10 12
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)
(c) ∆P=0.50MPa, L=108m (d) ∆P=0.75MPa, L=108m
(4) Experimental data of pressure drop from horizontal [6] Geldart D, Ling SJ. Dense phase conveying of fine coal
and vertical upward conveying of coal powder were at high total pressures. Powder Technol 1990; 62:243–52.
obtained. The previous models calculate pressure drop [7] Geldart D, Ling SJ. Saltation velocities in high pressure
of dense two-phase flow with prediction deviations no conveying of fine coal. Powder Technol 1992; 69:157–62.
better than ±50%, while the additional pressure drop [8] Zhou J, Zhang S, Wang B. Experimental study on the
model developed in this paper through dimensional pressure drop of pneumatic conveying pulverized coal
analysis yielded prediction deviations within ±30% in a pipeline (I). J Iron Steel Res 1993; 5:1–7. (in Chinese)
for horizontal conveying and ±20% for vertical upward [9] Zhou J, Zhang S. Experimental study on the pressure
conveying. Solid frictional pressure drop was larger in drop of pneumatic conveying pulverized coal in a
pipeline (II). J Iron Steel Res 1994; 6:1–7. (in Chinese)
horizontal pipes than that in vertical upward pipes, and
[10] Shen X, Xiong Y. Experimental study on dense-phase
the difference between them increased as the Froude
pneumatic conveying of pulverized coal at high pres-
number decreased.
sures. Proc CSEE 2005; 25:103–7. (in Chinese)
(5) The value of pressure signal fluctuations was one mag-
[11] Liang C, Xu P, Xu G, et al. Comparison on flow char-
nitude smaller than that of pressure drop and solid flow
acteristics of dense-phase pneumatic conveying of
rate. The fluctuation of pressure and pressure drop was
biomass powder and pulverized coal at high pressure.
barely correlated with the fluctuation of solid flow rate. Energ Source Part A 2015; 37:583–9.
The maximum FR was ~5.9 times that of the average [12] Liang C, Shen L, Chen X, et al. Conveying character-
fluctuation amplitude for solid flow rate. In this article, istics and resistance properties in high-pressure
the RSD of solid flow rate was used as an indicator for dense-phase pneumatic conveying of anthracite and
conveying stability. petroleum coke. J Chem Eng Jpn 2015; 48:163–74.
(6) The stability of vessel pressure could affect the sta- [13] Liang C, Shen L, Xu P, et al. Influence of carbonaceous
bility of conveying. The fluctuation of solid flow rate powders on flow characteristics of dense-phase pneu-
was mainly caused by the fluctuation of solid concen- matic conveying at high pressure. Exp Therm Fluid Sci
tration. No obvious effects of solid loading ration and 2014; 58:121–30.
back pressure on conveying stability were observed. [14] Gong X, Guo X, Dai Z, et al. High solids loading pneu-
There was a trend that conveying stability increased as matic conveying of pulverized coal. J Chem Ind Eng
superficial gas velocity decreased. When superficial gas 2006; 57:640–4. (in Chinese)
velocity was lower than ~6 m/s for 25 mm pipes or 8 [15] Guo X. Dense phase pneumatic conveying of pulver-
m/s for 15 mm pipes, unstable conveying might occur ized coal and its application in pilot plant. Ph.D. Thesis.
with average fluctuation amplitude of solid flow rate East China University of Science and Technology, 2010.
larger than 7%. (in Chinese)
[16] Wang W. Studies on flow characteristics of horizontal
pneumatic conveying of pulverized coal. Ph.D. Thesis.
Tsinghua University, 2012. (in Chinese)
Funding [17] Liang C. Studies on flow characteristics of high pressure
This article was funded by Shenhua S&T Innovation dense phase pneumatic conveying of pulverized coal.
Project (ST930014SH02). Ph.D. Thesis. Southeast University, 2007. (in Chinese)
[18] Lu P, Han D, Pu W, et al. Study on the flow character-
istics of high-pressure and dense-phase pneumatic
References conveying of different pulverized coal in igcc field. Proc
[1] Lin W, Wang Y, Gong X, et al. Stability analysis of pneu- ASME Turbo Expo 2012; 1:577–82.
matic conveying of pulverized coal in Shell coal gasifi- [19] Barth W. Strömungsvorgänge beim transport von
cation plant. Chem Eng 2014; 42:50–4. (in Chinese) festteilchen und flüssigkeitsteilchen in gasen. mit
[2] Jiang L. Analysis on industrial application of GSP besonderer berücksichtigung der vorgänge bei pneu-
gasification technology. Coal Eng 2016; 48:88–91. (in matischer förderung. Chem Ing Tech 1958; 30:171–80.
Chinese) [20] He C, Chen X, Wang J, et al. Conveying characteristics
[3] Zhang G, Li Z, Chen P, et al. Influence factors in flow and resistance characteristics in dense phase pneu-
fluctuation of GSP pulverized coal dense-phase trans- matic conveying of rice husk and blendings of rice
portation and control measures. Chem Fertil Ind 2014; husk and coal at high pressure. Powder Technol 2012;
41:23–6. (in Chinese) 227:51–60.
[4] Cong X. Study on relationship between flow patterns [21] Mallicka SS, Wypych PW. On improving scale-up pro-
and pipeline pressure signals in dense-phase pneumatic cedures for dense-phase pneumatic conveying of
conveying of pulverized coal. Ph.D. Thesis. East China powders. Particul Sci Technol 2011; 5:407–27.
University of Science and Technology, 2013. (in Chinese) [22] Guo X, Lu W, Lu H, et al. Pressure drop prediction for
[5] Rabinovich E, Kalman H. Flow regime diagram for ver- horizontal dense-phase pneumatic conveying of pul-
tical pneumatic conveying and fluidized bed systems. verized coal associated with feeding to gasifier. Chem
Powder Technol 2011; 207:119–33. Eng Res Des 2013; 91:2509–14.
[23] Yang WC. Correlations for solid friction factors in ver- [32] He C, Shen X, Zhou H. Stability analysis of dense phase
tical and horizontal pneumatic conveyings. Aiche J pneumatic conveying of pulverized coal at high pres-
1974; 20:605–7. sure. J Chem Ind Eng 2014; 65:820–8. (in Chinese)
[24] Setia G, Mallick SS, Pan R, et al. Modeling solids friction [33] Ma Y, Luo C, Jing Y, et al. Conveying problem of GSP
factor for fluidized dense-phase pneumatic transport gasification pulverized coal and optimizing measures.
of powders using two layer flow theory. Powder Technol China Powder Sci Technol 2015; 21:96–9. (in Chinese)
2016; 294:80–92. [34] Carnavas PC, Page, NW. Particle shape factors and
[25] Stegmaier W, Weber M. Untersuchungen zur pneuma- their relationship to flow and packing of bulk materi-
tischen dichtsromfoerderung in horizontalen und ver- als. Mech Eng Congr 1994; 2:241–6.
tikalen rohren. Verfahrenstechnik 1978; 12:794–8. [35] Mills D. Pneumatic Conveying Design Guide, 3rd edn.
[26] Pan R. Improving Scale-up Procedures for the Design Oxford, UK: Butterworth-Heinemann, 2016.
of Pneumatic Conveying Systems. Ph.D. Thesis. New [36] Xie X, Shen X, Tang X, et al. Study on some factors
South Wales, Australia: University of Wollongong, impacting flowability of pulverized coal. J China Coal
1992. Soc 2008; 33:85–8. (in Chinese)
[27] Mittal A, Setia G, Mallick S, et al. An investigation into [37] Geldart D. Types of gas fluidization. Powder Technol
pressure fluctuations and improved modeling of sol- 1973; 7:285–93.
ids friction for dense-phase pneumatic conveying of [38] Pan R. Material properties and flow modes in pneu-
powders. Particul Sci Technol 2014; 33:67–75. matic conveying. Powder Technol 1999; 104:157–63.
[28] Pu W, Zhao C, Xiong Y, et al. Research on resistance [39] Klinzing GE, Mathur MP. The dense and extrusion flow
properties for dense phase pneumatic conveying of regime in gas-solid transport. Can J Chem Eng 1981;
pulverized coal in vertical pipe at different pressures. 59:590–4.
Proceedings of the 5th International Symposium on [40] Zenz FA. Two-phase fluid-solid flow. Ind Eng Chem 1949;
Measurement Techniques for Multiphase Flows(5th 41:2801–6.
ISMTMF). Macau, China: AIP Conference Proceedings [41] Xia K, Chen H, Wang X, et al. Entrained-bed coal gasifi-
914, 2007. cation technology and its development tendency. Coal
[29] Wang W, Guan Q, Zhang J. Experimental study of Conversion 2005; 28:69–73. (in Chinese)
dense-phase pneumatic conveying of pulverized coal [42] Klinzing GE, Rizk F, Marcus RD, et al. Pneumatic
at elevated pressures. J Tsinghua Univ (Sci & Tech) 2011; Conveying of Solids, 3rd edn. Dordrecht, Netherlands:
51:277–81. (in Chinese) Springer, 2010.
[30] Mallick SS, Wypych PW. Minimum transport bounda- [43] Arastoopour H, Gidaspow D. Analysis of IGT pneumatic
ries for pneumatic conveying of powders. Powder conveying data and fast fluidization using a thermohy-
Technol 2009; 194:181–6. drodynamic model. Powder Technol 1979; 22:77–87.
[31] Xie K, Guo X, Cong X, et al. Minimum pressure drop [44] Molerus O. Overview: pneumatic transport of solids.
velocity and stability analysis in pneumatic convey- Powder Technol 1996; 88:309–21.
ing of pulverized coal in commercial-scale horizontal [45] Rautiainen A, Sarkomaa P. Solids friction factors in upward,
pipe. J Chem Ind Eng 2013; 64:1969–75. (in Chinese) lean gas-solids flows. Powder Technol 1998; 95:25–35.