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Clean Energy, 2018, Vol. 1, No.

1, 50–67

doi: 10.1093/ce/zkx007
Advance Access Publication Date: 14 December 2017
Homepage: https://academic.oup.com/ce

Research Article
Experimental study on dense-phase pneumatic
conveying of coal powder at high pressures
Qingliang Guan*, Zhen Liu, Xinhui Fang, Bing Liu, Baozai Peng,
Ziyang Feng, Ya Suo and Wenhua Li
National Institute of Clean-and-Low-Carbon Energy, Future Science & Technology City, Changping District, Beijing
102211, China

*Corresponding author. E-mail: guanqingliang@nicenergy.com

Abstract
Clean utilization and conversion of coal resources is significant to China’s energy sustainable development.
Entrained-flow coal gasification technology is an important method used for clean and efficient conversion of
coal. The characteristics and stability of high-pressure dense-phase pneumatic conveying of pulverized coal
is crucial to the safe and stable operation of dry-feed entrained-flow coal gasifiers. Dense-phase pneumatic
conveying experiments were carried out using a high-volatile bituminous coal in pipes with diameters of 25,
15 and 10 mm, respectively, and at back pressures of 1.0–4.0 MPag. The conveying characteristics and effects of
operating and structure parameters were studied. Pressure drop models were established for horizontal and
vertical upward conveying. The prediction uncertainty was within ±30% for the horizontal conveying and ±20%
for the vertical upward conveying. The relative standard deviation of solid flow rate was proposed to explain
conveying stability. The effect of operating parameters on conveying stability was systematically analyzed. The
gas velocity-related criterion was proposed for stable conveying.

Key words: dense-phase pneumatic conveying; pulverized coal; high pressure; pressure drop; stability

Introduction and entrained-flow coal gasification. The prevailing tech-


nology in the coal chemical industry is entrained-flow
Coal is the main energy resource of China, but pollutants
gasification due to its large production capacity, high car-
such as SO2, NOx and fine dust can be produced when
bon conversion and flexible coal feeds. The feedstock of
coal is combusted. The clean utilization and conversion
entrained-flow coal gasifiers can be coal–water slurry or
of coal resources is of strategic significance to China’s
dry pulverized coal. Commercial entrained-flow gasifiers
sustainable energy development. Coal gasification is an
with coal–water slurry feed include the GE Energy gasifier,
important process for the clean and efficient conversion
ECUST’s (East China University of Science and Technology)
of coal and is the key technology for industrial processes
opposed multi-burner gasifier and Tsinghua’s water mem-
such as coal-to-chemicals, coal-to-liquid fuels, coal-to-
brane wall gasifier. Commercial entrained-flow gasifiers
synthetic-natural-gas and integrated gasification com-
with dry pulverized coal feed include the Shell gasifier,
bined cycle. The three major coal gasification technologies
the GSP gasifier and the HT-L gasifier. The preparation
are fixed bed coal gasification, fluidized bed coal gasification

Received: 23 September, 2017; Accepted: 14 November, 2017


© The Author 2017. Published by Oxford University Press on behalf of National Institute of Clean-and-Low-Carbon Energy.
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and pumping of coal–water slurry is a simple and proven with pressure at constant total differential pressure and
technology. In contrast, conveying dry pulverized coal to fluidizing gas [17]. The experimental results of Lu et  al.
gasifiers is more complicated and has a higher capital also showed that the mass flow rate of coal particles and
cost. However, gasifiers with dry pulverized coal feed have concentration increased at high pressures [18]. The past
advantages. The gasifiers can produce a higher content of research mainly focused on macroscopic characteristics at
CO and H2 in raw syngas with lower consumption of coal high pressures with particle flow and mechanism research
and oxygen and longer service life of burners due to less seldom reported.
erosion caused by the pulverized coal. The pipeline pressure drop is one of the most important
In dry pulverized coal-fed gasification processes, coal parameters of pneumatic conveying, and the additional
is pneumatically transported by N2 or CO2 from high-pres- pressure drop model developed by Barth [19] was widely
sure feeding vessels to gasifiers. A stable conveying of the used:
feedstock with minimum transport gas is important to in-
crease the content of CO and H2 in raw syngas and ensure ρg Ug2 ρg Ug2
∆PT / L = ∆Pg / L + ∆Ps / L = λg + µλz (1)
the stable operation of the gasifier. Therefore, high-pres- 2D 2D
sure and dense-phase pneumatic transport of pulverized
coal is a key technology for dry-feed entrained-flow coal where, ΔPT/L is the pressure drop of the gas and solid mix-
gasification. Pulverized coal conveying technology is used ture, ΔPg/L is the pressure drop of the gas phase, and ΔPs/L
in engineering applications such as the Shell [1] and the is the additional pressure drop due to the presence of the
GSP gasification processes [2, 3]; however, there remain solid particles. λg is the gas friction coefficient, λz is the
many problems. The design of a conveying system is coefficient of additional pressure drop. μ is solid loading
mostly reliant on limited empirical correlations with fun- ration, ρg is gas density, Ug is superficial gas velocity, and D
damental research insufficient for the scale-up principles. is inner diameter of pipe. The gas friction coefficient λg can
For example, due to limited knowledge on the conveying be calculated by Equation (2):
stability and reliability in larger pipes, the diameter of the
conveying pipeline is limited to 50–60  mm in current in- 0.3164 1
λg = 2320 < Re < 80 (2a)
dustrial applications. The lack of reliable methods to ac- Re0.25 e/D
curately measure the coal mass flow rate makes it difficult
to accurately control the oxygen-to-coal ratio resulting in
fluctuating gasification operation. The dense-phase con- æ ö
1 ç e 2.51 ÷÷
veying limit can also influence the gasifier operation. The = -2lg çç + ÷
λg çç 3.7D Re λ ÷÷÷
coal–water slurry fed gasifiers can be operated at pressures è g ø (2b)
0.85
up to ~8.7 MPa or even higher, while dry pulverized coal- 1 æ 1 ö÷
80 < Re < 4160 çç ÷ 
fed gasifiers are limited at pressures up to ~4 MPa, partly e/D èç 2e / D ÷ø
because systems of dense-phase conveying at higher pres-
sures are not yet tested or verified.
Pneumatic conveying of coal powder is a very compli- 1  1 
0.85

λg = 4160  < Re
cated gas–solid two-phase flow process. Suspension flow,   D 
2
 2e / D  (2c)
dune flow, slug flow, plug flow and fluidized dense-phase 1.74 + 2lg  2e  
  
flow phenomena may be observed as gas and solid flow
through horizontal pipes [4], and suspension flow, annular
flow, turbulent fluidization flow, bubbly flow, slug flow and where, e is the roughness of pipe wall, Re (= ρgUgD/μg) is
separated plug flow can be found as gas and solid flow Reynolds number.
through vertical upward pipes [5]. The flow pattern transi-
tions are complicated with large differences in flow mech- Determination of the coefficient of the additional pressure
anisms between different flow patterns. There is currently drop λz is key to calculate the total pressure drop of two-
no matured theory to guide the design and operation of phase flow. To calculate λz some researchers [20] used power
dense-phase pneumatic conveying systems. Therefore, functions with several nondimensional parameters derived
many researchers have built experimental facilities to from experimental data. For the suspension flow in horizon-
study the dense-phase pneumatic conveying process tal pipes, the additional pressure drop of the particle clusters
[6–16]; however, only a few facilities operate at high pres- can be expressed as the sum of pressure drop caused by par-
sures [6, 7, 10–13]. The characteristics of dense-phase ticle friction and that caused by keeping the particles sus-
pneumatic conveying may differ from dilute-phase char- pended and then was applied to dense-phase conveying [21,
acteristics due to increased gas density and enhanced 22]. Based on Yang’s unified theory [23], Wang [16] put for-
gas–solid interactions. The influence of pressure on ward implicit equations to calculate λz. The gas–solid flow for
dense-phase pneumatic conveying needs further study. dense-phase flow of fine powder in horizontal pipes tends to
The experimental results of Liang et al. showed that mass be stratified. Setia et al. [24] used a ‘two-layer’ model (two dif-
flow rate of coal particles and concentration increased ferent models) that showed good prediction performance for

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Table 1  Coefficient of the additional pressure drop in horizontal pipes

Researcher Formula Experimental range

Stegmaier and
Weber [25] λz = 2.1µ −0.3Frt0.5Fr −1.21 ( D / dp )−0.1
ut Ug
Frt = , Fr =
gdp gD

0.4
 µ m
 Gs  1
∆P / L = K  
 ρg   D  Ug
K = 106, m = 0.83 Gs / D < 47 000kg / (m3s)
K = 0.838, m = 1.2 8Gs / D > 47 000kg / (m3s)
Geldart and D = 6.25–12.5 mm, carrier gas is H2, N2
Ling [6] and CO2, P < 8.27 MPa, Gs < 2000 kg/
(m2·s)
Pan [26] λz = 1.0 µ −0.2665Fr −1.4467 ρg−0.6626 D = 69 mm, lignite, dp = 25.8 µm, carrier
gas is air, P is atmospheric pressure,
μ = 3.6–63.4

Zhou et al. [8, 9]  0.07Fr


−1.4
µ = 7 − 35 D = 25 mm, P is atmospheric pressure, Gs
λz =  −0.71 < 1698 kg/(m2·s), μ = 7–200 kg/kg
0.23Fr µ = 40 − 200

ρs (1 − ε )us2
Ps / L = fs
2D
−0.902 −1.95
(1 − ε )−0.057  Ret   Ug 
fs = 1.98    
ε3  Rep   gD 

us = Ug −
(
4 ρs − ρg gdp ) fsus2 4.7
ε
3ρg CD 2gD
Wang [16] −1.80 D = 15 mm, dp = 69 µm, carrier gas is
ρ 
λz = e6.35Fr −1.34  s  N2, P < 1.5 MPa, Ug = 5.94–13.68 m/s,
 ρg  Gs = 15.8–32.8 kg/(m2·s)
He et al. [20] us 2β D = 10 mm, bituminous coal, dp = 63 µm,
λz = λs* + = 0.005 + 0.88 × 10 −4 Fr + Fr −2.16 or
Ug (us / Ug )Fr 2 P < 2.45 MPa

0.005 + 0.63Fr
−1.89
4 < Fr < 13.2
λz =  −0.19
 0.016Fr 13.2 < Fr < 40

Guo et al. [22] D = 15–26 mm, dp = 61 µm, carrier gas is


air, Ug = 2–15 m/s, Gs = 1000–4500 kg/
(m2·s), μ = 100–650 kg/kg, Fr = 4–40

Mittal et al. [27]  


−0.535
 Ut 
1.87 D = 69 mm, fly ash (ρs = 2300 kg/m3,
ms / ρs
λz = 19.26     ρb = 700 kg/m3, dp = 30 µm), carrier gas
m
 s / ρs + m g / ρg  Ug 
is air, P is atmospheric pressure

  m / ρ a  U b  * us 2β 
λz = τ 1  K  s s
    + τ 2  λs
f
+ 2
  mg / ρg   Ug   
 U ( u / U )Fr 
  g s g

Fr − Frmin Fr − Frmin
τ1 = 1 − ,τ 2 = ,
Frmax − Frmin Frmax − Frmin
Frmin = 3 − 4, Frmax = 50, β = Uf / Ug ,
K = 8.04, a = −0.22, b = 1.48, Uf = 0.06 m / s, λs* = 0.0043
Setia et al. [24] D = 69 and 105 mm, fly ash (ρs = 2300 kg/
m3, ρb = 700 kg/m3, dp = 30 µm), carrier
gas is air, P is atmospheric pressure

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Table 2  Coefficient of the additional pressure drop in vertical upward pipes

Researcher Formula Experimental range

Zhou et al. [8, 9] 0.01Fr D = 25 mm, P is atmospheric pressure,


−0.65
µ = 7 − 35
λz = 
0.25Fr
−0.82
µ = 40 − 200 Gs < 1698 kg/(m2·s), μ = 7–200 kg/kg

Pu et al. [28] ρs −2.87 D = 10 mm, carrier gas is N2, P = 2.1–3.6 MPa


λz = 4.39 Fr
ρg

Guo [15] λz = 0.82Fr −1.44 D = 20 mm, carrier gas is air, P is atmospheric


pressure, Ug = 2.1–9.6 m/s, Gs = 1030–3500 kg/(m2·s)
Wang et al. [29] λz = 9.652Re−0.795Fr −0.442 µ −0.328 D = 15 mm, dp = 69 µm, carrier gas is N2, P < 1.5 MPa,
Ug = 5.94–13.68 m/s, Gs = 15.8–32.8 kg/(m2·s)
He et al. [20] ρ 
−0.328
D = 10 mm, bituminous coal, dp = 63 µm,
λz = e−7.64 Fr −0.026  s  P < 2.45 MPa
 ρg 

fly ash at atmospheric pressure and account for the upper


suspension flow and the lower non-suspension flow. Tables
1 and 2 list coefficients of the additional pressure drop in
horizontal pipes and vertical upward pipes, respectively.
There are many formulae in the literature for calculating the
coefficients of the additional pressure drop. However, the
formulae are quite different from each other and whether
those formulae can be applied to other pneumatic convey-
ing conditions is yet to be studied.
A constant supply of feedstock is important for the sta-
ble operation of gasifiers. Mallick and Wypych [30] stated
that Fr = 5.7 predicted the boundary for stable conveying of
coal powder, regarding fluctuating and ‘non-linear’ flow of
material into the receiving bin as unstable conditions. Cong
[4] used the relative standard deviation (RSD) of pressure
signals to characterize the stability of pneumatic convey- Fig. 1  Photograph of the dense-phase conveying system
ing. According to his experimental data, dense-phase flow
is stable at the Fr > 10 when the RSD of the pressure signal is
<0.1. Xie et al. [31] used peak value of power spectral density the published indicators of stable conveying are different.
and RSD of pressure signals and found that the gas–solid Researchers have not yet analyzed the differences between
flow was stable at gas velocities 1–1.5 m/s lower than the indicators and criterions of stable conveying.
gas velocity at minimum pressure drop. He et al. [32] used These experiments systematically investigated the char-
the Hurst index of differential pressure signals and found acteristics of dense-phase pneumatic conveying of coal
that the stability of pneumatic conveying decreased when powder at back pressures of 1.0–4.0 MPag, as well as the
the superficial gas velocity was lower than 1.5 times the effect of operating parameters and structure parameters on
saltation velocity. Liang et al. [12] used the RSD of solid flow the characteristics. The influencing mechanism of pressure
rate signals and analyzed the influence of total differen- on dense-phase pneumatic conveying was studied using
tial pressure on the stability of pneumatic conveying. Ma et the conveying diagram and flow behavior of coal powder.
al. [33] believed that it was stable when the solid flow rate Based on the experimental data, the prediction capabilities
fluctuated within the range of 5% for GSP gasifiers. Lin et al. of published pressure drop models were analyzed, and new
[1] showed fluctuation of solid flow rate during stable oper- pressure drop models for horizontal and vertical upward
ation of a Shell gasifier and the RSD of solid flow rate was conveying were developed. The fluctuations of different sig-
2–3% and the maximum fluctuation range (FR) was 14–17%. nals of pneumatic conveying were analyzed, and an indica-
There has been considerable attention paid to the fluc- tor and criterion for stable conveying were proposed.
tuation of solid flow rate in the industry. Statistical analy-
sis of signals was used in laboratory investigations. Most
researchers use pressure signals and differential pressure 1 Experimental system
signals for accuracy, and they are also less expensive to
1.1 Experimental facility and material property
obtain. The signals are used to do statistical analysis and
propose qualitative or quantitative indicators and criteria The experimental facility of high-pressure dense-phase
of stable conveying. The criterions of stable conveying are pneumatic conveying of coal powder is shown in Fig.  1. It
mostly related to gas velocity or Froude number. However, consists of a nitrogen supply system, screw feeder system,

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P
3
2 11 7

8
P P

1 15

4 5
12 17
16
9
13 14

P dP
Gas
Gas and particles 10
6

Fig. 2  Flow diagram of the dense-phase conveying system. 1, nitrogen tank; 2, pressure reducing valve; 3, storage vessel; 4, delivery vessel; 5, receiv-
ing vessel; 6, conveying pipeline; 7, dust collector; 8, pressurizing gas; 9, fluidizing gas; 10, supplementary gas; 11, relieving gas; 12, load cell; 13,
pressure transducer; 14, differential pressure transducer; 15, solid mass flowmeter; 16, gas flowmeter; 17, regulating valve

2. Table 3  Parameters of the experimental facility


3m
5m (H
) Item Value
(VD)

2. Volume of the delivery 5 m3


3m or receiving vessel, V
4 (H
dP
) Maximum operating pressure of 6 MPag
5 P dP
the delivery or receiving vessel, P
P Inner diameter of the conveying 10 mm, 15 mm, 25 mm
10m
dP P pipeline, D
(VU)
P Conveying Horizontal 152 m 63 m
10m
dP
8m
1.5m (H)

3 distance Vertical upward 25 m 25 m


(H (VD) 7 6
) Vertical downward 20 m 20 m
10.3m Number of bends 30 26
(VU) Total length, L 197 m 108 m
2 P

1 dP
Pipe material 20# carbon steel
P dP
P
dP

dP

8m to suppress solid deposition and to adjust gas velocity and


(H (H)
H: horizontal
particle concentration in the pipe. The pressure of vessels is
)
14m
VU: vertical upwards
VD: vertical downwards controlled by electric control valves installed at the pressur-
izing gas pipe and relieving gas pipe. The volume flow rate of
fluidizing gas is adjusted as the pressure of the vessel varies
Fig. 3  Layout of the conveying line. 1, inlet of conveying line; 2, coal dis-
tributor; 3, valves for changing conveying distance; 4,solid mass flow-
until coal powder inside the bottom of the vessel reaches
meter; 5, outlet of conveying line; 6, pressure transducer; 7, differential the optimal fluidization status. The fluidized coal powder is
pressure transducer discharged from the bottom of the delivery vessel, mixing
with the supplementary gas, and flows into the conveying
line through a coal distributor. The conveying line consists of
coal delivery system, conveying and measurement system, three parallel branches of different pipe diameters. Several
coal receiving system and data acquisition and control sys- valves are installed at the entrance and exit of the branches
tem. The flow diagram of the dense-phase conveying sys- for switching between these branches. Conveying distance
tem is shown in Fig. 2, and the layout of the conveying line can be changed by altering the length of the horizontal con-
is depicted in Fig.  3. High-pressure nitrogen flows from a veying line using a set of valves, as shown in Fig. 3. The three
nitrogen tank installed in a truck to a storage vessel through parallel branches join together through another coal distrib-
pressure-reducing valves and is then fed into a delivery ves- utor, following which is a solid mass flowmeter installed in
sel (receiving vessel). Pressurizing gas is used to pressurize a vertical downward pipe. The gas–solid mixture eventually
the vessels, fluidizing gas is used to fluidize coal powder flows into the receiving vessel, where gas and solid particles
for easier transportation and supplementary gas is used are separated, and carrier gas is vented after passing through

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Table 4  Main parameters of measuring instruments

Instrument Manufacturer Measurement range Accuracy

Gas vortex flowmeter Emerson Process Management 0–20 m3/h ±1%


Gas mass flowmeter Emerson Process Management 0–100 Nm3/h ±0.5%
Pressure transducer Emerson Process Management 0–10 MPa ±0.05%
Differential pressure transducer Emerson Process Management 0–30 kPa, 0–60 kPa ±0.05%
Load cell Yuyao Pacific Weighing Engineering Co. Ltd 0–4 t ±0.03%
Solid mass flowmeter Thermo Fisher Scientific Velocity: 0–15 m/s, ±2%
concentration: 0–700 kg/m3

a bag filter. The delivery vessel and receiving vessel are inter- Table 5  Proximate and ultimate analysis of Shanbei coal
changeable, and coal powder is circulated inside the convey-
Parameter Value Parameter Value
ing system. New coal material is fed into the delivery vessel
by the screw feeder system, and used coal material can be Mar (%) 6.44 Cdaf (%) 82.46
discharged from the bottom of the bag filter. Parameters of Vdaf (%) 39.48 Hdaf (%) 4.78
the experimental facility are shown in Table 3. FCd (%) 55.66 Odaf (%) 11.49
The flow rate of supplementary gas is measured by vor- Ad (%) 8.03 Ndaf (%) 0.96
tex flowmeters, and the flow rates of pressurizing gas and Qnet, ar (MJ/kg) 25.96 Sdaf (%) 0.30
fluidizing gas are measured by mass flowmeters. Seven
pressure transducers and eight differential pressure trans- Q = Q p + Q f + Q s − Ms / ρs (4)
g
ducers are installed along the conveying line, as shown in
Fig.  3. The weights of vessels are measured by load cells
and are used to calculate the average solid flow rate during Qg Qg
Ug = = (5)
a period of time. The instantaneous solid flow rate is meas- A 0.25π D2
ured by the solid mass flowmeter of Thermo Ramsey, which
consists of a velocity sensor, a concentration sensor and Where Qp is volume flow rate of pressurizing gas, Qf is vol-
an integrator. The output signals of measuring instruments ume flow rate of fluidizing gas, Qs is volume flow rate of
are converted by A/D converters and then recorded by a PLC supplementary gas, ρs is particle density.
control system at a frequency of 2 Hz. Main parameters of
measuring instruments are shown in Table 4. It is worth noting that Qg and Ug are dependent on local
The conveying material is a high-volatile bituminous coal pressure and thus changed at different positions. The solid
from China, as shown in Table 5. Properties of coal particles loading ratio µ was calculated by Equation (6):
and parameters of flowability are shown in Table  6. Fig.  4
Ms
shows the particle size distribution of coal particles. The µ=
ρgQ g (6)
particles are cohesive [34–36] since the compressibility is
between 30 and 50%, the angle of repose is between 45° and There is currently no common definition for dense phase.
55° and the flow function is between 4 and 10. According to The solid loading ratio is widely used. For example, µ >
Geldart’s classification [37], the particles are A-type particles 10 was used by Klinzing and Mathur [39] as an indica-
and are suitable for dense-phase pneumatic conveying [35]. tor for dense phase. However, the solid loading ratio is
According to Pan’s classification [38], the particles are PC1- influenced by properties of solid particles and carrier
type particles and can be transported smoothly and gently gas. Gas density changed greatly as the pressure varied
from dilute phase to fluidized dense phase. in the experiments, so solid loading ratio alone was not
suitable. Many researchers regarded the region of super-
ficial gas velocity larger than the saltation velocity as the
1.2 Data processing
dense-phase region based on Zenz’s diagram [40], which
The slopes of weight loss curves and weight gain curves of was inconvenient for use. The particle concentration of
the vessels were calculated as average solid flow rate and dense-phase conveying of coal powder is 400 and 300–
were used to calibrate the instantaneous mass flow rate Ms 500  kg/m3 for Shell gasifiers [41] and GSP gasifiers [33],
and concentration C, which were measured by the solid mass respectively. Therefore, in this article, dense-phase region
flowmeter. The solid mass flux was calculated by Equation (3): is considered where particle concentration is larger than
Ms Ms 300 kg/m3.
Gs = = (3) Table 7 lists the experimental range of pneumatic con-
A 0.25π D2
veying. Most of the experiments were in the dense-phase
where the volume flow rate of carrier gas (Qg) and superfi- region for 25 and 15 mm pipes, while experiments were in
cial gas velocity (Ug) are as follows: dilute-phase region for 10 mm pipe.

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Table 6  Properties of coal particles and parameters of flowability

Parameter Value Parameter Value

External moisture content (%) 4.84 Median particle diameter (µm) 35.3
Internal moisture content (%) 1.60 Compressibility (%) 39.2
Particle density (kg/m3) 1449 Angle of repose (°) 48
Tap density (kg/m3) 852 Angle of wall friction (°) 27
Loosely packed density (kg/m3) 518 Flow function 3.1

6 Table 7  Experimental range

5 Diameter of pipe mm 25 15 10
Volume percentage (%)

Back pressure MPag 1–4 1–4 1–4


4 Solid flow rate kg/h 448–4718 171–1757 96–586
Solid mass flux kg/(m2·s) 254–2670 268–2761 338–2072
3
Particle concentrationa kg/m3 46–641 20–437 18–180
2 Solid loading ratio kg/kg 1–25 1–15 1–7
Superficial gas velocityb m/s 1.5–11.2 4.3–20.5 8.8–22.6
1
a
At local pressure and temperature where the solid mass flowmeter
0 installed.
0.1 1 10 100 1000 b
Average superficial gas velocity.
Particle diameter (μm)

Fig. 4  Particle size distributions of coal particles with total differential pressure, as shown in Fig. 5a and b.
It is worth noting that critical velocity increased with solid
flow rate (total differential pressure), which is the same as
2 Results and discussion the conclusion of former researcher [42].
At back pressures of 2.5 and 4.0 MPag, no remarkable
2.1 Characteristics of high-pressure dense-phase
effects of back pressure on solid mass flux curves and solid
conveying
concentration curves were found in the region of low gas vel-
Diagram of conveying was widely used to investigate the ocity, and back pressure hardly affected the value of critical
characteristics of high-pressure dense-phase conveying. In velocity, as shown in Fig. 5a and b. However, in the region of
the diagram, the pressure drop per unit length was plotted high gas velocity, solid flow rate was lower at high back pres-
against the superficial gas velocity with the solid flow rate sures, which was due to higher pressure drops of gas phase
as a parameter, or the solid flow rate was plotted against as gas density increased at high back pressures, as shown in
the superficial gas velocity with the total differential pres- Fig. 5a. Thus, conveying of coal powder would be affected by
sure as a parameter. The latter method was chosen in this pressure through gas density, especially in the dilute-phase
article because it is convenient to control the pressure dif- region.
ference between the delivery vessel and receiving vessel in At back pressure of 1.0 MPag, first of all, the trend of
the experimental facility. a slow increase followed by a rapid increase of solid con-
Fig.  5 showed the effect of operating parameters on centration with decreasing gas velocity was more notice-
conveying characteristics. At a constant back pressure and able, as shown in Fig. 5b; second, solid mass flux was lower
total differential pressure, the solid flow rate increased to for 1.0 MPag at the region of low gas velocity, as shown
a maximum and decreased as the superficial gas velocity in Fig.  5a. One possible explanation was that coal parti-
decreased, as shown in Fig. 5a. The superficial gas velocity cles were more likely to deposit in the bottom of hori-
at the maximum solid flow rate was a critical velocity. When zontal pipes at 1.0 MPag, due to larger density differences
superficial gas velocity was high, the flow was in a dilute- between solid particles and gas. Therefore, the transition
phase region with low solid concentrations, and the pres- of flow patterns from dilute-phase suspension flow to non-
sure drop of the gas phase was the main part of the total uniform stratified flow gave rise to more sharp transitions
pressure drop. As the gas velocity decreased, the pressure of solid concentration curves. Moreover, the effective sec-
drop of the gas phase decreased and the solid flow rate tional area of pipes decreased as coal particles deposited,
increased. As gas velocity decreased further, solid concen- which resulted in lower solid mass fluxes at 1 MPag.
tration increased rapidly and the inter-particles and par- Fig.  6 showed the effect of operating parameters on
ticle–wall friction resistance, which resulted in an increased particle velocity. The results showed that the particle
pressure drop due to particles and decreased solid flow rate. velocity decreased with decreasing local superficial gas
Total differential pressure was the main driver for con- velocity, and the particle velocity was lower than the local
veying coal particles. At a constant back pressure and gas superficial gas velocity. The variation of velocity differ-
velocity, solid flow rate and solid concentration increased ence between local superficial gas velocity and particle

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2000 P=1.0MPag : 700 P=1.0MPag:


critical velocity

S o lid c o nc e ntra tio n ( k g /m 3 )


∆P=0.25MPa 600 critical velocity ∆P =0.25MPa
1600 ∆P =0.5MPa ∆P =0.5MPa
S o lid flu x ( k g /s m 2 )

∆P =0.75MPa 500 ∆P =0.75MPa


1200 P=2.5MPag: P=2.5MPag:
400
∆P =0.25MPa ∆P =0.25MPa
800 ∆P =0.5MPa 300 ∆P =0.5MPa
∆P =0.75MPa ∆P =0.75MPa
P=4.0MPag: 200 P=4.0MPag:
400 ∆P =0.25MPa
∆P =0.25MPa 100
∆P =0.5MPa ∆P =0.5MPa
0 ∆P =0.75MPa 0 ∆P =0.75MPa
0 3 6 9 12 0 3 6 9 12
Average superficial gas velocity (m/s) Average superficial gas velocity (m/s)

(a) Solid mass flux (b) Solid concentraion

Fig. 5  Effect of operating parameters on conveying characteristics (D = 25 mm, L = 197 m)

of 2.5 and 4.0 MPag, the transition took place at critical veloc-
14
ity, whereas at a lower back pressure and lower solid flow
12 rate, the transition was more obvious and took place at a gas
Particle velocity (m/s)

velocity near, which solid concentration changed rapidly (as


10 shown in Fig. 5b) and was higher than the critical velocity.
The effect of conveying distance on solid mass flux is
8
shown in Fig. 8. It was shown that solid mass flux increased
6 by ~40% as the conveying distance decreased from 197
to 108 m (by decreasing the length of horizontal convey-
4 ing line) at constant total differential pressures. That was
because the pressure drop per unit length increased as the
2
conveying distance decreased, and the driving force for
0 conveying coal powder increased. It could be observed that
0 2 4 6 8 10 12 14 the effect of conveying distance was very similar to that of
Local superficial gas velocity (m/s) total differential pressure.
The effect of pipe diameter on solid flow rate is shown
Fig. 6  Particle velocity versus local superficial gas velocity (D = 25 mm,
L = 197 m)
in Fig. 9. It was shown that the solid flow rate was larger for
larger pipes at the same superficial gas velocity. Compared
with pipe of 10 mm diameter, the solid flow rate increased
velocity with average superficial gas velocity is shown in
approximately four times and nine times to that of the solid
Fig.  7. At higher gas velocities, the particle–wall friction
flow rate in pipes of 15 and 25 mm diameter, respectively.
force was larger because of larger particle velocities, and
That was because resistance was smaller for pipes of larger
the gas–solid drag force was also larger according to the
diameters, and more coal particles can be transported.
force balance of particles in the dilute phase; therefore, the
velocity difference between gas and solid should be larger
to drive the particles. That trend was similar to the results 2.2 Pressure drop through straight pipes
predicted by the correlation developed by Arastoopour and
Comparisons of pressure drop per unit length between
Gidaspow [43], namely the velocity difference between gas
experimental data and model calculations from Table 1 for
and solid was proportional to the superficial gas velocity,
horizontal pipes are shown in Fig. 10. It was shown that in
as shown in Equation (7):
most cases both Stegmaier and Weber’s model and Wang’s
and He et  al.’s model overpredicted the pressure drop. In
us = Ug (1 − 0.68dp0.92 ρs0.5 ρg−0.2 D−0.54 ) (7) contrast, Geldart and Ling’s, Pan’s and Zhou et al.’s model
underpredicted the pressure drop. It was interesting that
or the prediction results were very similar for Geldart and
Ling’s, Pan’s and Zhou et al.’s model, while the three mod-
Ug − us = 0.68dp0.92 ρs0.5 ρg−0.2 D−0.54 Ug (8) els were in quite different forms, as shown in Table 1.

Model predictions by Guo et  al., Mittal et  al. and Setia
et al. were in agreement with experimental data within the
As gas velocity decreased, the slope of variation of the veloc- deviation of ±50%, which are the best among all the models
ity difference with superficial gas velocity changed at a cer- investigated, despite that they were developed from very
tain gas velocity, which might indicate a transition of flow different experimental conditions from this article. Guo et al.
patterns, as shown in Fig. 7. For conveying at back pressures used air as the carrier gas and carried out experiments at

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5 5 5
Velocity difference between 1.0MPag 1.0MPag 1.0MPag

Velocity difference between

Velocity difference between


local Ug and us (m/s) 4 2.5MPag 4 2.5MPag 4 2.5MPag

local Ug and us (m/s)

local Ug and us (m/s)


4.0MPag 4.0MPag 4.0MPag
3 3 3

2 2 2
critical velocity critical velocity critical velocity

1 1 1

0 0 0
0 2 4 6 8 10 12 14 0 2 4 6 8 10 12 14 0 2 4 6 8 10 12 14
Average superficial gas velocity (m/s) Average superficial gas velocity (m/s) Average superficial gas velocity (m/s)

(a) ∆P =0.25MPa (b) ∆P =0.50MPa (c) ∆P =0.75MPa

Fig. 7  Velocity difference between local Ug and us versus average superficial gas velocity (D = 25 mm, L = 197 m)

2000
1.0MPag 4000 10mm
2.5MPag 15mm
25mm

Solid flow rate (kg/h)


1600 4.0MPag
Solid flux (kg/sm2)

3000

L=108m
1200 2000

800 L=197m 1000

0
400 3 6 9 12 15
0 3 6 9 12 15
Average superficial gas velocity (m/s)
Average superficial gas velocity (m/s)
Fig. 9  Effect of pipe diameter on solid flow rate (L = 108 m, P = 2.5 MPag,
Fig.  8  Effect of conveying distance on solid mass flux (D  =  25  mm,
∆P = 0.75 MPa)
∆P = 0.75 MPa)

near atmospheric pressures, while in this article, the carrier loading ratio (µ), the density ratio of solid to gas ( ρs / ρg ), the
gas was nitrogen and conveying pressure exceeded 1 MPa. Reynolds number (Re), the Froude number (Fr) and the diam-
It should be noted that pipe diameters were in the range of eter ratio ( dp / D ). The solid loading ratio was correlated with
15–26 mm in Guo et al.’s experiments, which was very simi- the solid concentration: a higher solid loading ratio indicated
lar to those in this article. In addition, in Mittal et al.’s and a higher solid concentration, and thus higher frequencies of
Setia et al.’s experiments, carrier gas was also air, conveying particle–particle and particle–wall inelastic collisions, which
material was fly ash, conveying pressure was near atmos- would result in larger momentum losses. The density ratio of
pheric pressure and pipe diameter was 69 and 105  mm. solid to gas was used to represent the particle-carrying capac-
While the experimental conditions were very different from ity in dilute suspension flow [44]. The Reynolds number rep-
those in this article, those models still gave better results. resented the ratio of inertia forces to viscous forces and could
Comparisons of pressure drop per unit length between be used to represent the change of turbulent kinetic energy
experimental data and model calculations from Table 2 for of the carrier gas as operating parameters varied. The Froude
vertical upward pipes are shown in Fig. 11. It was shown that number represented the ratio of inertia forces to gravity and
Zhou et al.’s and Wang et al.’s model underpredicted the pres- could be used to represent the effect of gravity on conveying.
sure drop, while predictions of Pu et al.’s and He et al.’s model The effect of gravity was larger at lower gas velocities; thus,
diverged for pipes of different diameters. Guo’s model was solid particles were more likely to deposit on the bottom of
in agreement with experimental data within the deviation horizontal pipes and flow backward along the wall of vertical
of ±50%, which is the best among all the models investigated upward pipes, which could affect the pressure drop of the gas–
although it was developed from very different experimental solid mixture. The diameter ratio in fact represented merely
conditions from this article, as shown in Table 2. the effect of pipe diameter, such as those due to wall rough-
Since the predictive ability of existing models was not yet ness of different pipes, since the particle size was constant in
adequate for engineering applications, a new additional pres- this article.
sure drop model was developed in this article. Several non- The coefficient of the additional pressure drop was
dimensional parameters were analyzed, including the solid regressed with experimental data using the power

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Guan et al.  |  59

30 30 30
25mm +50% 25mm +50% 25mm +50%

Model calculation (kPa/m)

Model calculation (kPa/m)

Model calculation (kPa/m)


25 15mm 25 15mm 25 15mm
10mm 10mm 10mm
20 20 20

15 15 15

10 -50% 10 -50% 10 -50%

5 5 5

0 0 0
0 5 10 15 20 25 30 0 5 10 15 20 25 30 0 5 10 15 20 25 30
Experimental measurement (kPa/m) Experimental measurement (kPa/m) Experimental measurement (kPa/m)

(a) Stegmaier and Weber (b) Geldart and Ling (c) Pan

30 30 30
25mm +50% 25mm +50% 25mm +50%
Model calculation (kPa/m)

Model calculation (kPa/m)

Model calculation (kPa/m)


25 15mm 25 15mm 25 15mm
10mm 10mm 10mm
20 20 20

15 15 15

10 -50% 10 -50% 10 -50%

5 5 5

0 0 0
0 5 10 15 20 25 30 0 5 10 15 20 25 30 0 5 10 15 20 25 30
Experimental measurement (kPa/m) Experimental measurement (kPa/m) Experimental measurement (kPa/m)

(d) Zhou et al. (e) Wang (f) He et al.

30 30 30
25mm +50% 25mm +50% 25mm +50%
Model calculation (kPa/m)

Model calculation (kPa/m)

Model calculation (kPa/m)


25 15mm 25 15mm 25 15mm
10mm 10mm 10mm
20 20 20

15 15 15

10 -50% 10 -50% 10 -50%

5 5 5

0 0 0
0 5 10 15 20 25 30 0 5 10 15 20 25 30 0 5 10 15 20 25 30
Experimental measurement (kPa/m) Experimental measurement (kPa/m) Experimental measurement (kPa/m)

(g) Guo et al. (h) Mittal et al. (i) Setia et al.

Fig. 10  Comparisons of pressure drop per unit length between experimental data and model calculations from Table 1 for horizontal pipes

functions of the above-mentioned nondimensional λz = 2.990 × 10 −3 Fr −0.946 (dp / D)−0.637 (10)


parameters. Preliminary studies showed that power num-
bers of solid loading ratio, density ratio of solid to gas and For vertical upward conveying:
Reynolds number were small, and thus, the three non-
dimensional parameters were removed from the fitting
λz = 2.047 × 10 −4 Fr −1.095 (dp / D)−1.233 (11)
formula to ignore their effect on the coefficient of the addi-
tional pressure drop. The formula is shown in Equation (9):
The experimental and calculated coefficients of additional

λz = xFr (dp / D)z (9)


y pressure drop were plotted against the Froude number in

Fig. 12. It was shown that the coefficient of additional pres-
sure drop increased as the Froude number decreased, and it
The experimental coefficient of addition pressure drop
was calculated according to Equations (1) and (2) and was increased rapidly when the Froude number was lower than
then fitted by Equation (9) in Excel using multiple regres- 10–15 for horizontal pipes and 15–20 for vertical upward
sion analysis. The resultant formulae of coefficient of pipes. Pressure had minor impacts on the coefficient of
the additional pressure drop are shown as Equations (10) additional pressure drop, which was also proved by Figs. 10
and (11). and 11 where models derived from conveying at near atmos-
For horizontal conveying: pheric pressures could be used to predict pressure drop of

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60 | Clean Energy, 2018, Vol. 1, No. 1

18 18 18
25mm +50% 25mm +50% 25mm +50%

Model calculation (kPa/m)

Model calculation (kPa/m)

Model calculation (kPa/m)


15 15mm 15 15mm 15 15mm
10mm 10mm 10mm
12 12 12

9 9 9

6 -50% 6 -50% 6 -50%

3 3 3

0 0 0
0 3 6 9 12 15 18 0 3 6 9 12 15 18 0 3 6 9 12 15 18
Experimental measurement (kPa/m) Experimental measurement (kPa/m) Experimental measurement (kPa/m)

(a) Zhou et al. (b) Pu et al. (c) Guo

18 18
25mm +50% 25mm +50%
Model calculation (kPa/m)

Model calculation (kPa/m)


15 15mm 15 15mm
10mm 10mm
12 12

9 9

6 -50% 6 -50%

3 3

0 0
0 3 6 9 12 15 18 0 3 6 9 12 15 18
Experimental measurement (kPa/m) Experimental measurement (kPa/m)

(d) Wang et al. (e) He et al.

Fig. 11  Comparisons of pressure drop per unit length between experimental data and model calculations from Table 2 for vertical upward pipes

0.12 0.12
Experiment (25 mm) Experiment (25 mm)
0.10 Experiment (15 mm) 0.10 Experiment (15 mm)
Experiment (10 mm) Experiment (10 mm)
0.08 Calculation 0.08 Calculation

0.06 0.06
λz

λz

0.04 0.04

0.02 0.02

0.00 0.00

-0.02 -0.02
0 5 10 15 20 25 30 35 40 0 10 20 30 40 50 60
Fr Fr

(a) Horizontal (b) Vertical upward

Fig. 12  Plot of λz with Fr

high-pressure conveying. It was likely that pressure could In horizontal pipes, additional pressure drop was
influence the pressure drop of gas–solid two-phase flow mainly solid frictional pressure drop, while in vertical
only through gas density and dynamic head. Comparisons upward pipes, additional pressure drop also included solid
of pressure drop per unit length between experimental gravitational pressure drop. Thus, solid frictional pressure
data and model calculations are shown in Fig.  13. It was drop could be calculated from total pressure drop as in
shown that the developed models from this article agreed Equations (12) and (13):
with experimental data within ±30% for horizontal pipes
and ±20% for vertical upward pipes, which showed better
∆PsfH / ∆L = ∆Ps / ∆L = ∆PT / ∆L − ∆Pg / ∆L (12)
performance than previous models.

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30 15
25mm +20%
25 25mm +30% 15mm
12

Model calculation (kPa/m)

Model calculation (kPa/m)


15mm 10mm
10mm
20
9
15 -20%
6
10 -30%
3
5

0 0
0 5 10 15 20 25 30 0 3 6 9 12 15
Experimental measurement (kPa/m) Experimental measurement (kPa/m)

(a) horizontal (b) vertical upward

Fig. 13  Comparisons of pressure drop per unit length between experimental data and model calculations


(a) 15 (b) 3.0
25mm 25mm

(∆P Hsf/∆L - ∆P Vsf/∆L)/(∆P Vsf/∆L)


15mm 2.5 15mm
12
10mm 10mm
2.0
∆P Hsf/∆L (kPa/m)

9 1.5

6 1.0

0.5
3
0

0 −0.5
−3 0 3 6 9 12 15 0 10 20 30 40 50 60
∆P Vsf/∆L (kPa/m) Fr

Fig. 14  Comparisons of solid frictional pressure drop between horizontal and vertical upward pipes

∆PsfV / ∆L = ∆Ps / ∆L − ∆Psg / ∆L = ∆PT / ∆L − ∆Pg / ∆L − ∆Psg / ∆L due to the increased normal stress resulted from grav-

ity. In addition, the difference of solid frictional pres-
(13)
sure drop between horizontal pipes and vertical upward
pipes was larger at a lower Froude number as shown in
where solid gravitational pressure drop was calculated by Fig. 14b due to more coal particles tending to deposition.
Equation (14) When the Froude number was very low, negative values
occurred for the solid frictional pressure drop in vertical
Ms g 1 Gs g
∆Psg / ∆L = ≈ upward pipes, as shown in Fig. 14a. That was considered
A us Ug (14)
to be the result of a change of the direction of the shear
force due to the backflow of particles in vertical upward
Comparisons of solid frictional pressure drop between
flow when gas velocity was very low [15]. The phenom-
horizontal and vertical upward pipes are shown in
enon had been observed during experiments [45].
Fig. 14, where solid frictional pressure drop of horizontal
pipes was calculated from Equation (10) and that of verti-
cal upward pipes was calculated from Equations (13) and 2.3 Conveying stability
(14). It was shown that solid frictional pressure drop of Unstable conveying of coal powder always occurred
horizontal pipes was larger than that of vertical upwards with simultaneous signal fluctuations. For discrete
pipes, except for some data from 25  mm pipeline. That signal data series ( y1 , y2 , yN ) , the average fluctuation
was because the deposition of coal particles on the bot- amplitude was represented by its RSD as calculated by
tom of horizontal pipes increased particle–wall friction Equation (15), and its maximum FR was calculated by

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62 | Clean Energy, 2018, Vol. 1, No. 1

(a) 0.03 (b) 0.30 (c) 300%

0.25 250%
y=5.9x
0.02 0.20 200%
RSD(Ph)

RSD(∆ Ph)

FR(Ms)
0.15 150%

0.01 0.10 100%

0.05 50%

0 0 0%
0 0.1 0.2 0.3 0.4 0 0.1 0.2 0.3 0.4 0 0.1 0.2 0.3 0.4
RSD(Ms) RSD(Ms) RSD(Ms)

Fig. 15  Comparisons of fluctuations calculated from various signals

4.3 1600 5 1400 4

P1 1400 1200
Ph 4
4.2 1200 3
1000

∆Ph/∆L (kPa/m)
Pressure(MPag)

Ms 1000 3 800

C(kg/m3)
Ms(kg/h)

us(m/s)
4.1 800 2
us 2 600
600
∆Ph/∆ L 400
4.0 P2
400 1
1
200 200
C
3.9 0 0 0 0
0 1 2 3 4 5 6
Time(min)

Fig. 16  Signal fluctuations of experimental condition A (D = 25 mm, P1 = 4.25 MPag, P2 = 4 MPag, Qf = 20 Nm3/h, Qs = 188 Nm3/h)

4.3 1600 5 1400 4


P1 1400 1200
Ph 4
4.2 1200 3
1000
∆Ph/∆L (kPa/m)
Pressure(MPag)

Ms 1000 3 800
C(kg/m3)
Ms(kg/h)

us(m/s)

4.1 800 2
us 2 600
600
∆Ph/∆ L 400
4.0 P2 400 1
1
C 200 200

3.9 0 0 0 0
0 1 2 3
Time(min)

Fig. 17  Signal fluctuations of experimental condition B (D = 25 mm, P1 = 4.25 MPag, P2 = 4 MPag, Qf = 20 Nm3/h, Qs = 168 Nm3/h)

Equation (16). RSD and FR were used to represent the Three representative signals were investigated to study
fluctuation of signals. the conveying stability, including the pressure of a hori-
zontal pipe (Ph), the pressure drop per unit length of a hori-
1 zontal pipe (ΔPh/ΔL) and solid flow rate (Ms). Comparisons
∑ ( y − y)2
N

N − 1 i=1 i 1 N (15)
RSD( y) =
y
, y= ∑yi
N i=1
of fluctuation calculated from the three signals are shown
 in Fig.  15. It was shown that RSD(Ph) was the smallest and
was one magnitude smaller than RSD(ΔPh/ΔL) and RSD(Ms).
The value of pressure fluctuations was small compared
max( yi ) − min( yi ) with the value of the pressure itself. The fluctuation of pres-
FR( y) = × 100% (16)
y sure drop and solid flow rate was in the same order of

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Guan et al.  |  63

Table 8  Signal RSDs of two experiments of similar conditions

Condition RSD(P1) RSD(P2) RSD(Ph) RSD(ΔPh/ΔL) RSD(us) RSD(C) RSD(Ms)

A 7.1 × 10−4 2.8 × 10−3 2.0 × 10−3 0.09 0.06 0.14 0.12


B 4.8 × 10−4 2.2 × 10−4 1.3 × 10−3 0.06 0.03 0.10 0.08

magnitude. In addition, the correlation coefficients for RSD(Ph) 0.4


solid concentration
and RSD(Ms), RSD(ΔPh/ΔL) and RSD(Ms), FR(Ms) and RSD(Ms)
particle velocity
were 0.23, 0.16 and 0.92, respectively, as shown in Fig.  15a–c.
It could be seen that no strong correlations were found between 0.3 y=1.24x, R 2=0.96
RSD(Ph) and RSD(Ms) or between RSD(ΔPh/ΔL) and RSD(Ms),

RSD(us) or RSD(C)
while RSD(Ms) was substantially correlated with FR(Ms). The
value of FR(Ms) was ~5.9 times that of RSD(Ms), as shown in
0.2
Fig. 15c, which was similar to the case in Shell gasifiers [1].
The stable supply of feedstock in industrial gasifiers
required that the solid flow rate of coal was stable, so y=0.63x, R 2=0.86
as to match with the flow rate of oxygen and keep the 0.1
oxygen-to-coal ratio stable. The average fluctuation ampli-
tude could be used to denote the operating stability of gas-
ifiers in long-term runs, while the maximum FR could be 0.0
used to denote the possibility of triggering the interlocks 0.0 0.1 0.2 0.3 0.4
and causing unplanned shutdown. Based on the above-­ RSD(Ms)
mentioned analysis, RSD of the solid flow rate signal was
Fig.  18  Comparisons of RSDs of solid flow rate, particle velocity and
used as an indicator for conveying stability in this article.
solid concentration
Signal fluctuations of two experiments with similar
conditions are shown in Figs 16 and 17. In the experiments,
differences were found for the RSD of solid flow rate, indi-
the pressure of the delivery vessel and the receiving vessel
cating that there were minor effects of solid loading ratio
was controlled by control valves. When the vessel pressure
on conveying stability for 25 mm pipes in this article.
was not well controlled, periodic fluctuations occurred,
The effect of back pressure on conveying stability for
which led to similar periodic fluctuations of signals in the
25 mm pipes is shown in Fig. 20. It was shown that at the
conveying pipeline, as shown in Fig. 16. The conveying in-
same gas velocity, there were no big differences in solid con-
stability induced by fluctuations of the vessel pressure
centrations between different back pressures, although solid
had been observed by many researchers [33]. Fluctuations
concentration was a little bit lower at 1.0 MPag. When solid
of the vessel pressure would result in fluctuations of the
concentration was high, such as those higher than 300 kg/m3,
total differential pressure, which had a direct impact on
there were no obvious differences in conveying stability
the solid flow rate. After the pressure control strategy was
between different back pressures. While when solid concen-
improved and periodic fluctuations of vessel pressure were
tration was low, more stable conveying could be achieved at
diminished, no obvious periodic fluctuations of signals in
higher back pressures. That was because gas density was
the conveying pipeline could be observed, as shown in
higher and particle-carrying capacity of gas was larger at
Fig. 17. The conveying stability improved since RSDs of all
higher back pressures, making it easier for suspending the
the signals investigated decreased, as shown in Table 8.
particles and thus enhancing the conveying stability.
Comparisons of RSDs of solid flow rate, particle velocity
Variations in RSD(Ms) with superficial gas velocity for
and solid concentration are shown in Fig. 18. It was shown
pipes of different diameters are shown in Fig.  21. There
that RSD(Ms), RSD(us) and RSD(C) were in the same order
was a trend that RSD(Ms) increased as superficial gas vel-
of magnitude, and generally, RSD(us) < RSD(Ms) < RSD(C).
ocity decreased. It was shown that when superficial gas
Besides, RSD(C) was in a stronger correlation with RSD(Ms)
velocity was lower than ~6 m/s for 25 mm pipes and 8 m/s
than RSD(us) was in with RSD(Ms), which demonstrated that
for 15  mm pipes, RSD(Ms) increased rapidly and might
the fluctuation of solid flow rate was mainly caused by the
exceed 7%, which was regarded as unstable conveying in
fluctuation of solid concentration. That was possible when
this article. It should be noted that when superficial gas
cross-sectional solid concentration fluctuated dramatically
velocity was lower than above-mentioned values, stable
in dense-phase plug flow or dune flow at horizontal pipes.
conveying with RSD(Ms) less than 7% still might appear.
The effect of solid loading ratio on conveying stability
for 25 mm pipes is shown in Fig. 19. It was shown that at
the same gas velocity, the solid loading ratio was higher 3 Conclusions
for a conveying distance of 108 m, compared with that Dense-phase pneumatic conveying of a high-volatile bitu-
for a conveying distance of 197 m.  Whereas no obvious minous coal powder was carried out in an experimental

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64 | Clean Energy, 2018, Vol. 1, No. 1

0.4 0.4
L=197m 25 L=197m 25
L=108m L=108m

Solid loading ratio, µ(kg/kg)

Solid loading ratio, µ(kg/kg)


0.3 L=197m 0.3 L=197m
L=108m 20 L=108m 20
RSD(Ms)

RSD(Ms)
15 15
0.2 0.2

10 10
0.1 0.1
5 5

0 0 0 0
2 4 6 8 2 4 6 8
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)

(a) P=1.0MPag, ∆P=0.50MPa (b) P=1.0MPag, ∆P=0.75MPa

0.4 15 0.4 15
L=197m L=197m
L=108m Solid loading ratio, µ(kg/kg) L=108m

Solid loading ratio, µ(kg/kg)


L=197m 12 L=197m
0.3 0.3
L=108m L=108m
10
9
RSD(Ms)

0.2 RSD(Ms) 0.2


6
5
0.1 0.1
3

0 0 0 0
2 4 6 8 2 4 6 8 10 12
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)

(c) P=2.5MPag, ∆P=0.50MPa (d) P=2.5MPag, ∆P=0.75MPa

0.4 8 0.4 10
L=197m L=197m
L=108m L=108m
Solid loading ratio, µ(kg/kg)

Solid loading ratio, µ(kg/kg)


0.3 L=197m 6 0.3 L=197m
L=108m L=108m
6
RSD(Ms)

RSD(Ms)

0.2 4 0.2
4

0.1 2 0.1
2

0 0 0 0
1 2 3 4 5 6 2 4 6 8
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)

(e) P=4.0MPag, ∆P=0.25MPa (f) P=4.0MPag, ∆P=0.50MPa

Fig. 19  The effect of solid loading ratio on conveying stability (D = 25 mm)

facility using 25, 15, and 10 mm pipes and at back pres- and structure parameters were studied. Pressure drop
sures of 1.0–4.0 MPag. The conveying characteristics and models for horizontal pipes and vertical upward pipes
the influencing mechanism of operating parameters were established. The indicator and criterion for stable

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Guan et al.  |  65

0.20 500 0.20 500


P=1.0MPag
P=2.5MPag P =1.0MPag

Solid concentration, C(kg/m3)

Solid concentration, C(kg/m3)


P=4.0MPag 400 P =2.5MPag 400
0.16 0.16
300 300
0.12 0.12
RSD(Ms)

RSD(Ms)
200 200
0.08 0.08
100 100

0.04 0 0.04 0

0 -100 0 -100
2 4 6 8 2 4 6 8
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)
(a) ∆P=0.50MPa, L=197m (b) ∆P=0.75MPa, L=197m

0.20 600 0.4 600


P=1.0MPag
P=2.5MPag P =1.0MPag
500
Solid concentration, C(kg/m3)

Solid concentration, C(kg/m3)


P=4.0MPag P =2.5MPag 500
0.16
400 0.3
400
0.12
RSD(Ms)

300 RSD(Ms)
0.2 300
0.08 200
200
100
0.1
0.04 100
0

0 -100 0 0
2 4 6 8 2 4 6 8 10 12
Superficial gas velocity, Ug(m/s) Superficial gas velocity, Ug(m/s)
(c) ∆P=0.50MPa, L=108m (d) ∆P=0.75MPa, L=108m

Fig. 20  The effect of back pressure on conveying stability (D = 25 mm)

0.3 (1) At constant total differential pressures, solid flow rate


reached the maximum when superficial gas velocity
25mm
15mm reached the critical velocity. As superficial gas veloc-
10mm ity decreased, initially the solid concentration increased
0.2 slowly while the velocity difference between gas and solid
decreased rapidly, then the solid concentration increased
RSD(Ms)

rapidly while the velocity difference between gas and solid


0.1 slowly decreased. The shift between the two processes
0.07 took place at a superficial gas velocity equaled to or larger
than the critical gas velocity, which indicated a transfor-
mation of flow patterns inside the pipeline (such as par-
0 ticle deposition in horizontal pipes). The shift was more
obvious at lower back pressure and lower solid flow rate.
0 2 4 6 8 10 12 14 (2) In dense-phase region, no remarkable effects of back
pressure on solid mass flux and solid concentration
Superficial gas velocity, Ug(m/s)
were found at back pressures of 2.5 and 4.0 MPag, while
Fig. 21  Variations of RSD(Ms) with superficial gas velocity for pipes of solid mass flux and solid concentration were lower at
different diameters back pressure of 1.0 MPag.
(3) Solid flow rate improved with increasing total differential
conveying were proposed, and the effect of operating pressure or decreasing conveying distance since pressure
parameters on the conveying stability was systemati- drop per unit length increased. Solid flow rate increased
cally analyzed. with pipe diameter at a constant total differential pressure.

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66 | Clean Energy, 2018, Vol. 1, No. 1

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