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Young Ju Kim, Ji Sub Hwang, Bui Xuan Khuyen, Bui Son Tung, Ki Won Kim, Joo
Yull Rhee, Liang-Yao Chen & YoungPak Lee
To cite this article: Young Ju Kim, Ji Sub Hwang, Bui Xuan Khuyen, Bui Son Tung, Ki Won Kim,
Joo Yull Rhee, Liang-Yao Chen & YoungPak Lee (2018) Flexible ultrathin metamaterial absorber
for wide frequency band, based on conductive fibers, Science and Technology of Advanced
Materials, 19:1, 711-717, DOI: 10.1080/14686996.2018.1527170
CONTACT YoungPak Lee. yplee@hanyang.ac.kr Department of Physics and RINS, Hanyang University, Seoul 04763, Korea
© 2018 The Author(s). Published by National Institute for Materials Science in partnership with Taylor & Francis Group.
This is an Open Access article distributed under the terms of the Creative Commons Attribution License (http://creativecommons.org/licenses/by/4.0/), which permits
unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
Sci. Technol. Adv. Mater. 19 (2018) 712 Y. J. KIM et al.
reflection is minimized owing to the impedance match- the boundary conditions: the x-y plane and the z
ing between whole MMA and free space by elaborately direction indicate the E-H fields and the k, propaga-
adjusting the permittivity and the permeability tion direction. The absorption can be calculated by
pffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
[ZðωÞ ¼ μðωÞ=ðωÞ]. Along with rapidly-advancing A(ω) = 1 – R(ω) – T(ω) = 1 – jS11 ðωÞj2 – jS21 ðωÞj2 ,
information and communications technology, MMAs where A(ω), R(ω) and T(ω) are the absorption, the
have been optimized for single- [18], multi- [19], and reflection and transmission coefficients, respectively,
wide-band [20–22] by using the frequency selective and S11 ðωÞ and S21 ðωÞ are the scattering parameters
surface. Many researchers have also focused on of reflection and transmission, respectively.
MMAs of thin and flexible materials so that they can The unit cell of MMA without conductive fibers
be utilized easily in the real life [23]. Since MMAs is presented in Figure 1(a). The proposed unit cell
basically utilize the resonance phenomenon, it is very consists of three layers: patterned-copper, FR4-
difficult to realize thin and flexible broadband MMAs. dielectric and continuous copper layers. The
In our previous study, a broadband MMA was dielectric layer is located between patterned copper
realized by connecting adjacent absorption peaks, patterns at the front and copper plane at the bot-
based on multi-resonance by utilizing multilayered tom. The unit cell contains rectangular copper
structure but, since the multilayered structure is patches, which are most suitable for our frequency
thick, it was inflexible [24]. Since then, we have band of interest and for the integration with con-
implemented the high-performance broadband ductive fibers, with different sizes, and the opti-
absorber with thin thickness using resistive sheets mized unit cell reveals periodic dimensions of
[25]. Although the reduction in thickness was p = 400 mm in the x-y plane. The top patterned
achieved, it was not thin enough to be flexible copper and the bottom copper plane have electric
owing to the fact that there are several layers of conductivity of σ ¼ 5:8 107 S/m and thickness of
dielectric and resistive sheet. In this work, we tm = 0.035 mm. The employed dielectric FR4 has
introduce and realize an ultrathin and wide-band dielectric constant and loss tangent of ¼ 4:3 and
MMA using metallic square patches with different δ ¼ 0:025, respectively, and its thickness is ts
size and conductive fibers. Furthermore, comple- = 0.8 mm. The length and the width of rectangular
mentary research was also carried out to improve patch (Sn ) are ln and wn . When conductive fibers
the flexible performance by changing the dielectric are connected to the metallic rectangular patches,
substrate. l1 and w1 of the largest rectangular patch were
varied to determine the starting point of absorp-
tion band, resulting in high absorption at that
2. Simulation and experiment frequency. After determining the absorption band,
The three-dimensional model for our proposed the number of rectangular patches was selected. In
MMA was simulated by using a finite-element- order to maintain the high performance in broad-
method software, CST Microwave Studio. We set band, the absorption at the corresponding
(a) (b)
S7
S6
S4
S3
R7
R4
R6
E k E k
R3
H H
R5
S1 S5
S2 R1
R2
Figure 1. Design of the unit cell for ultrathin MMA. Three-dimensional periodic structure of the unit cell (a) without and (b) with
conductive fibers.
Sci. Technol. Adv. Mater. 19 (2018) 713 Y. J. KIM et al.
frequencies was optimized by changing ln and wn imaginary parts of the relative impedance, as shown
of the other six rectangular patches in the order of in Figure 2(a). As mentioned above, it is a well-
the size of rectangle. The optimized values for the known method to explain the perfect-absorption
length of the rectangular patch become l1 ¼ 160, properties using the free-space impedance-matching
l2 ¼ 75, l3 ¼ 42, l4 ¼ 35, l5 ¼ 15, l6 ¼ 5 and l7 ¼ 2 theory [25]. By using the reflection and the transmis-
mm, and the corresponding widths come to be sion scattering parameters, the effective impedance
w1 ¼ 180, w2 ¼ 90, w3 ¼ 60, w4 ¼ 45, w5 ¼ 30, can be calculated as [26]
w6 ¼ 20 and w7 ¼ 15 mm. The largest rectangular sffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
patch (S1 ) is designed to exhibit the resonance at ð1 þ S11 ðωÞÞ2 S221 ðωÞ
ZðωÞ ¼ : (1)
0.95 GHz, and the other optimized patches are ð1 S11 ðωÞÞ2 S221 ðωÞ
devised to have periods of 1/2 (S2 ), 1/3 (S3 ), 1/4
(S4 ), 1/6 (S5 ), 1/9 (S6 ) and 1/12 (S7 ) of the largest It can be observed that the real part of effective
rectangular patch. Figure 1(b) shows the unit cell impedance of the MMA without the conductive fibers
of the MMA with conductive fibers. The electric is much smaller than 1 at 0.95, 1.36, 1.70, 2.00 and
conductivity of conductive fiber (Rn ) connected 4.40 GHz except the wild fluctuation, but weak peaks
with the rectangular patches (Sn ) above and appear. The imaginary part of effective impedance
below is designated as σ Rn . The optimized values also presents the weak peaks at the frequencies
for the electric conductivity of conductive fiber where the weak ones are observed in the real part of
come to be σ R1 ¼ 1:0 104 , σ R2 ¼ σ R3 ¼ effective impedance. However, the real part of effec-
tive impedance for the MMA with conductive fibers
4:0 104 , σ R4 ¼ 1:6 103 , σ R5 ¼ 1:4 103 ,
is larger than that for the MMA without conductive
σ R6 ¼ 3:0 103 and σ R7 ¼ 4:0 103 S/m. The
fibers, and the difference in the real part of effective
thickness of conductive fiber is tR ¼ 0:050 mm.
impedance between the MMA with conductive fibers
The minimum size of fabricated MMA is 800
and the free space [Zreal ðωÞ ¼ 1] at 0.66–6.09 GHz is
800 mm2 because of the large periodicity in the x-y
less than 0.4. When the real part of effective impe-
plane and the low operating frequency. The pat-
dance is similar to the free space, the reflection of
terned-copper layer was delicately etched by using a
entire MMA structure is minimized for the incident
conventional photolithography process. We selected
EM wave. The imaginary part of effective impedance
polypyrrole as the material of conductive fibers
become 0 at 2.28, 3.26, 4.2, 4.4 and 5.28 GHz. The
because its electrical conductivity can be controlled
real parts of effective impedance at 2.28, 3.26, 4.2, 4.4
by doping. The electrical conductivity of fibers was
and 5.28 GHz, which are all the magnetic resonance
measured with a four-point probe. The fibers were
frequencies indicated by the imaginary parts above,
cut slightly longer than the marked parts (Rn )
are 1.22, 0.76, 1.08, 0.89, and 1.37, which mean the
between the metallic rectangular patches. They were
impedance matching at these frequencies of the mag-
taped to connect with the copper rectangular patches
netic resonance. The difference in the imaginary part
as shown in Figure 1(b).
of effective impedance between the MMA with con-
ductive fibers and the free space [Zimag ðωÞ ¼ 0] in the
region below 0.91 GHz or above 6.03 is more than
3. Results and discussion
0.4. Figure 2(b) presents that the improved absorp-
In order to compare the MMAs without and with the tion by connecting the conductive fibers. The simu-
conductive fibers, we present both calculated real and lated absorption spectra of the MMAs without and
(a) (b)
2 1.0
0.6
0
0.4
-1 Real (without)
Imaginary (without) 0.2
Real (with)
Imaginary (with)
-2 0
2 4 6 1 2 3 4 5 6
Frequency (GHz) Frequency (GHz)
Figure 2. Difference between MMA without and with conductive fibers. (a) Effective impedance and (b) simulated absorption
spectrum of the proposed MMA without and with conductive fibers.
Sci. Technol. Adv. Mater. 19 (2018) 714 Y. J. KIM et al.
pffiffiffiffiffiffi
with conductive fibers are illustrated in a frequency Here, f0 is the resonance frequency [f0 ¼ 1=ð2π LCÞ].
range of 0.50–6.20 GHz. The MMA without conduc- By connecting with the conductive fibers, the absorp-
tive fibers has absorption peaks at 0.95, 1.70, 2.00, tion band is widened by manipulating the resistance
4.40 and 5.49 GHz with absorption of 15.5%, 18.0%, component. As the Ohmic loss responsible for the
30.5%, 40.0% and 35.6%, respectively. In addition, resistive part increases, the absorption also increases.
negligible weak absorption peaks also exist. On the To further understand the mechanism of energy
other hand, the absorption of MMA with conductive dissipation, we simulate the surface current and the
fibers is over 97% at 0.97–6.12 GHz. In the generic power-loss density of MMA with conductive fibers at
equivalent RLC circuit, Q-factor associated with the 0.95 1.70, 2.00 and 4.40 GHz, as shown in Figure 3.
loss of metallic part can be expressed by [27] The selected frequencies are for the absorption peaks
of MMA without conductive fibers, marked by purple
L
Qc ¼ ω0 : (2) dashed circles in Figure 2(b), since the resonance
R frequencies are unchanged significantly even when
In equation (2), the angular resonance frequency, the the conductive fibers are connected. At all the fre-
effective inductance and the effective quencies, the induced surface currents in the pat-
pffiffiffiffiffiffi resistance of
circuit are denoted by ω0 ð¼ 1= LCÞ, L and R. The terned layers (the first column) are accumulated in
operating bandwidth can be approximately deter- the upward direction (indicated by red arrows) by
mined as excitation along the E field, and those in the contin-
uous-copper plane layers (the second column) behave
f0 R in the downward direction. The induced antiparallel
BW ¼ ¼ : (3)
Qc 2πL surface currents induce a strong magnetic field in the
0.95 GHz
1.70 GHz
2.00 GHz
4.40 GHz
Figure 3. Physical mechanism of the broadband absorption. Simulated the induced surface currents in the metallic pattern (first
column), the continuous metallic plane (second column) and three-dimensional distributions for the power loss (third column)
at 0.95, 1.70, 2.00 and 4.40 GHz.
Sci. Technol. Adv. Mater. 19 (2018) 715 Y. J. KIM et al.
(c) 1.00
0.96
Absorption
0.92
0.88
0.84
Simulation
Measurement
0.80
1 2 3 4 5 6
Frequency (GHz)
Figure 4. Experiment and performance of the MMA. Photos of (a) the fabricated sample with conductive fibers and (b) the
measurement set-up. (c) Simulated and measured absorption spectra for the proposed structure.
opposite direction of the magnetic field of incident different size and with conductive fibers connected
EM wave by Ampere’s law, which dissipates the inci- by taping is thin enough to bend. To prevent the
dent EM wave [28]. The evidence for the magnetic interference effect between incident and reflected
resonance can be demonstrated with the antiparallel waves at an incident angle of 5°, we set the two
surface currents between patterned- and continuous- antennas at an appropriate distance. A copper plate
copper layers, and it is also noticed that the induced of the same size was used to gain the reference
surface currents affect the effective permittivity. In perfect-reflection spectrum, and the reflection spec-
short, the high absorption occurs according to the trum (jS21 j2 ) was measured differently from the
impedance matching by the magnetic resonances. simulation because there was no transmission, as
The power-loss density (dielectric loss) in the third shown in Figure 4(b). The simulated (black curve)
column of Figure 3 provides a simple route to iden- and the measured (red dots) are plotted in Figure 4
tify the areas that strongly absorb the EM wave at (c). It can observed that the experimental result
specific frequencies. At 0.95 GHz, the absorption is display that the absorption band over 97% is slightly
caused by the second-largest rectangular patches (S2 ), widened from 0.97–6.12 GHz to 0.87–6.11 GHz in
and it can be observed that the third-largest rectan- comparison with the simulated one, and the overall
gular patches (S3 ) also contribute greatly to the absorption is maintained in all the measured fre-
absorption. The absorption peaks at 2.00 and 4.40 quency range. The experimental absorption band is
GHz are affected by the fourth-largest rectangular red-shifted, but the experimental absorption is
patches (S4 ) and the fifth-largest rectangular patches higher more or less than the simulation, because
(S5 ), respectively. the electric conductivity of conductive fibers and
Figure 4(a,b) show the photographs of fabricated the real properties of FR4 are slightly different
sample and experimental configuration, set in a from the simulation. The ratio of total thickness
microwave anechoic chamber, respectively. The fab- ttotal of the MMA to the wavelength λ at 0.97 GHz
ricated MMA of copper rectangular patches with comes to be ttotal ¼ λ=349.
Sci. Technol. Adv. Mater. 19 (2018) 716 Y. J. KIM et al.
(c) (d)
1.0 1.0
0.8 0.8
Absorption
Absorption
0.6 0.6
0.4 0.4
Φ=0
Φ = 15º
0.2 0.2 Φ = 30º
Simulation Φ = 45º
Measurement Φ = 60º
0 0
1 2 3 4 5 6 7 1 2 3 4 5 6 7
Frequency (GHz) Frequency (GHz)
Figure 5. Application of the MMA model for flexibility. Photographs of (a) the fabricated flexible sample with conductive fibers
and (b) the measurement configuration. (c) Simulated and experimental absorption spectra of the suggested flexible MMA. (d)
Simulated absorption spectra according to the incident angle for the TE polarization.
In order to take advantage of the flexible prop- with the case of FR4 substrate, the case of absorp-
erty of conductive fibers, the simulation and the tion band is red-shifted. In the case of the operat-
experiment are implemented by substituting poly- ing frequency of 0.97 GHz, the ratio of total
imide for FR4 and changing the thickness of cop- thickness ttotal of MMA to wavelength λ is realized
per for the same conditions. The employed flexible to be as small as λ=5194. It is possible to obtain the
dielectric polyimide has the dielectric constant and flexible high-absorption performance in the desired
the loss tangent of ¼ 3:5 and δ ¼ 0:0027, respec- frequency range by adjusting the appropriate para-
tively, and its thickness is ts = 0.025 mm. The top meters of unit cell. To verify that the absorption of
patterned copper and the bottom copper plane flexible MMA is maintained with respect to the
were prepared with the thickness of tm ¼ 0:017 incident angle, Figure 5(d) exhibits the absorption
mm. Figure 5(a,b) present the photographs of spectra at incident angles of 0, 15°, 30°, 45° and 60°
rolled flexible sample, emphasizing the flexibility, at 0.7–7.5 GHz. As the angle of incidence increases
and experimental configuration, respectively. The up to 30°, the valleys become deeper, but the over-
simulated (black curve) and the measured (red all absorption over 90% is maintained in the broad-
dot) are illustrated in Figure 5(c). In the simula- band. However, the absorption is slightly lower at
tion, the absorption spectrum shows that the the absorption peaks and the valleys come to be
absorption is over 90% at 0.87–7.34 GHz, and the even deeper at incident angles of 45° and 60°.
absorption is slightly lower compared with the FR4 These results mean that the absorption properties
substrate, but the absorption bandwidth is can be maintained even when this MMA is bent.
expanded toward higher frequency. The corre- Therefore, it can be used not only to protect elec-
sponding experimental results indicate that the tronic devices from the electromagnetic interfer-
absorption band over 90% is divided into ranges ence, but also to conceal civil and military devices
of 0.75–5.67 and 6.23–6.97 GHz, and, in common from radar.
Sci. Technol. Adv. Mater. 19 (2018) 717 Y. J. KIM et al.