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COBALT-60 PRODUCTION IN CANDU POWER REACTORS

G.R. Malkoske
MDS Nordion
447 March Road
Kanata, Ontario, K2K 1X8, Canada
613-592-2790
gmalkoske@mds.nordion.com

J. Slack J.L. Norton


Atomic Energy of Canada Limited MDS Nordion
2251 Speakman Drive 447 March Road
Mississauga, Ontario, L5K 1B2, Canada Kanata, Ontario, K2K 1X8, Canada
905-823-9060 613-592-2790
slackj@aecl.ca jnorton@mds.nordion.com

ABSTRACT designed and developed by MDS Nordion and


key words: cobalt, reactor, CANDU AECL, has been safety, economically and
®
MDS Nordion has been supplying cobalt-60 successfully employed in many CANDU reactors
sources to industry for industrial and medical with over 195 reactor years of production.
purposes since 1946. These cobalt-60 sources
are used in many market and product segments, This paper will describe, at an overview level, the
but are primarily used to sterilize single-use MDS Nordion proprietary technology and know
medical products including; surgical kits, gloves, how that is used to provide CANDU reactors with
gowns, drapes, and cotton swabs. Other a safe and economical capability to produce
applications include sanitization of cosmetics, cobalt-60.
®
microbial reduction of pharmaceutical raw CANDU (CANada Deuterium Uranium) is a
materials, and food irradiation. registered trademark of Atomic Energy of Canada
Limited (AECL).
The technology for producing the cobalt-60
isotope was developed by MDS Nordion and 1. BACKGROUND
Atomic Energy of Canada Limited (AECL) almost MDS Nordion has been supplying cobalt-60
55 years ago using research reactors at the AECL sources to industry for industrial and medical
Chalk River Laboratories. purposes since 1946. These cobalt-60 sources
are used in many market and product segments.
®
In order to produce cobalt-60 in CANDU power The major application is in the health care industry
reactors, the stainless steel adjusters are replaced where irradiators are used to sterilize single use
with neutronically equivalent cobalt-59 adjusters. medical products. These irradiators are designed
With its very high neutron flux and optimized fuel and built by MDS Nordion and are used by
burn-up, the CANDU has a very high cobalt-60 manufacturers of surgical kits, gloves, gowns,
production rate in a relatively short time. drapes and other medical products. The irradiator
Many design considerations and requirements for is a large shielded room with a storage pool for the
®
the production of cobalt-60 in CANDU must be cobalt-60 sources. The medical products are
assessed, such as; operator and public safety, circulated through the shielded room and exposed
minimum impact on station efficiency and reactor to the cobalt-60 sources. This treatment sterilizes
operations, shielding requirements during reactor the medical products which can then be shipped to
operation with cobalt-60 adjusters and removal of hospitals for immediate use. Other applications for
the cobalt-60 adjusters from core, transportation this irradiation technology include sanitization of
within the station, and finally the processing and cosmetics, microbial reduction of pharmaceutical
shipment off-site. This Canadian technology for raw materials and food irradiation.
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cobalt-60 production in CANDU reactors,
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The cobalt-60 sources are manufactured by AECL’s CANDU Reactor
®
MDS Nordion in their Cobalt Operations Facility in AECL’s CANDU Reactor is unique among the
Kanata. More than 75,000 cobalt-60 sources for power reactors of the world, being heavy water
use in irradiators have been manufactured by moderated and fuelled with natural uranium. They
MDS Nordion. The cobalt-60 sources are double are also designed and supplied with stainless steel
encapsulated in stainless steel capsules, seal adjusters as part of the reactor regulating system,
welded and helium leak tested. Each source may which is to shape the neutron flux to optimize
contain up to 14,000 curies. These sources are reactor power and fuel burn-up, and to provide
shipped to over 170 industrial irradiators around excess reactivity needed to overcome xenon-135
the world. poisoning following a reduction of power. The
reactor is designed to develop full power output
This paper will focus on the MDS Nordion with all of the adjuster elements in the core.
proprietary technology used to produce the cobalt-
60 isotope in CANDU reactors. For cobalt-60 production, the reactor’s full
complement of stainless steel adjusters is
Almost 55 years ago MDS Nordion and Atomic replaced with neutronically equivalent cobalt-59
Energy of Canada developed the process for adjusters, which are essentially invisible to reactor
manufacturing cobalt-60 at the Chalk River Labs, operation. With its very high neutron flux and
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in Ontario, Canada. A cobalt-59 target was optimized fuel burn-up, the CANDU has a very
introduced into a research reactor where the high cobalt-60 production rate in a relatively short
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cobalt-59 atom absorbed one neutron to become time. This makes CANDU an excellent vehicle
cobalt-60. Once the cobalt-60 material was for bulk cobalt-60 production.
removed from the research reactor it was Prior to a utility engaging in Cobalt-60 production,
encapsulated in stainless steel and seal welded and notwithstanding the obvious initial change in
using a Tungsten Inert Gas weld. The first cobalt- licensing requirements and submissions, there are
60 sources manufactured using material from the many engineering design considerations and
Chalk River Labs were used in cancer therapy requirements for the production of cobalt-60 in
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machines. Today the majority of the cancer CANDU which must be assessed. These include
therapy cobalt-60 sources used in the world are operator and public safety, minimum impact on
manufactured using material from the NRU reactor station efficiency and reactor operations, shielding
in Chalk River. requirements during reactor operation with cobalt-
60 adjusters, removal of the cobalt-60 adjusters
The same technology that was used for producing from core, transportation within the station, and
cobalt-60 in a research reactor was then adapted finally the processing and shipment off-site.
and transferred for use in a CANDU power Execution of the above mentioned results in the
reactor. In the early 1970s, in co-operation with design and supply of the specialized equipment
Ontario Power Generation (formerly Ontario required for the production and handling of Cobalt
Hydro), bulk cobalt-60 production was initiated in Adjuster Rods.
the four Pickering A CANDU reactors located east
of Toronto. This was the first full scale production CANDU Reactors currently produce many millions
of millions of curies of cobalt-60 per year. of curies per year of Cobalt-60 for MDS Nordion’s
use in industry and commerce. Following the
As the demand and acceptance of sterilization of removal and replacement of stainless steel
medical products grew, MDS Nordion expanded adjusters with cobalt adjusters, the cobalt
its bulk supply by installing the proprietary adjusters are removed from the reactor at
Canadian technology in additional CANDUs. Over approximately 2 year irradiation intervals, and
the years MDS Nordion has partnered with transported to the remote Secondary Irradiated
CANDU reactor owners to produce cobalt-60 at Fuel Bay (SIFB) for storage and processing. In
various sites. CANDU reactors that have, or are the SIFB the cobalt adjusters are disassembled
still producing cobalt-60, include Pickering A, and the individual cobalt bundles prepared for
Pickering B, Gentilly 2, Embalse in Argentina, and offsite shipment to MDS Nordion in their purpose
Bruce B. built and licensed transportation flasks.

In compliance with the above and to facilitate


cobalt production, the Cobalt Adjuster Element

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Processing System (CAEPS) was designed to pencils, acting in compression, add to the bending
permit the replacement of all of the cobalt adjuster structural stiffness of the bundle assembly.
rods during routine reactor maintenance
shutdowns. The cobalt removal and transfer The cobalt bundles, loaded with pencils as
equipment was designed to be used intensively for required, are threaded onto the center rod in a
relatively short periods of time and to function sequence to match the negative reactivity
quickly and reliably so that the limited time requirements for each adjuster type, due to its
“window” available for the replacement process particular location in the reactor core. A special
would not be missed. The cobalt removal and nut is screwed onto the upper end of the center
transfer system is mechanized extensively in order rod. To provide a shoulder for a compression
to minimize labour and operator skills required. spring to apply tension to the center rod. The
The system is designed for high productivity, to cobalt bundles are thus kept under reasonable
minimize the demands upon the station constant load despite varying tolerance and
maintenance staff during the critical maintenance thermal expansion effects. The upper nut and
interval, and to increase the profitability of the lower fitting on the center rod are designed to
operation. permit tensioning, and the lower fitting is designed
to rupture the center rod at the bottom rivet for
Cobalt Adjusters disassembling the element in the SIFB.
As previously stated a set of cobalt adjuster rods
are provided in the reactor as part of the Reactor Removal of Cobalt Adjusters from the Reactor
Regulating System (RRS). Initially, the design A.General
provided for D2O cooling of the adjuster to address Heavily shielding apparatus is required to safely
perceived thermal requirements. However, D2O discharge and transfer the irradiated cobalt
cooling has since been demonstrated as adjusters from the reactor adjuster position to the
unnecessary and the system valved out. designated section of the SIFB. Prior to
The requirements for flux flattening in the core commencing the cobalt production program, and
result in a number of different types of adjuster as a primary requirement, the reactivity
rods. Each cobalt adjuster rod assembly consists mechanism decks were provided with extra
of a number of bundles, each bundle containing up shielding to facilitate the handling of the irradiated
to 6 cobalt pencils. The adjuster rods are cobalt elements.
assembled from standard design components.
Only the centre rod and stainless steel cable The following items of CAEPS equipment are
lengths are special for each adjuster application, supplied or are used to safely unload the cobalt
as determined by the number of bundles required adjusters from the reactor, transport them to the
due to its location in the reactor. SIFB and process them in the SIFB.

The cobalt bundle assembly is the basic building 1. Flask and Pedestal
block of an adjuster rod. It consists of two circular 2. Reactor Building Crane (existing)
end-plates held apart by two welded support 3. Flask Positioner
tubes. The plates feature an outer ring of holes, 4. Transporter/Erector
which are precisely aligned so that one to six 5. Discharge Port
pencils can be inserted into them as required. 6. Element Processing and Handling in
Once inserted, the pencils are held in position by a the Bay
snap ring, secured by a groove in the upper end
plate and a shoulder on the bottom end plate. B.Flask and Pedestal
The flask was designed to safely contain one
The pencils are seal-welded zircaloy tubes filled irradiated cobalt adjuster on its suspension cable
with cobalt slugs. They are standardized plus the lower shield plug. The flask shielding is
components, made to suit service conditions as sufficient as to give a surface contact dose rate on
well as reactor requirements. The cobalt in the the outside of the flask of 50 mR/h or less during
pencils constitutes the bulk of neutron absorbing normal operations. Special appendages on the
material, the rest of the adjuster assembly being flask permit its safe transport by the reactor
built mostly of zircaloy and designed for the building crane and the CAEPS transporter/erector.
smallest practical neutron absorption. The pencil
and bundle lengths are matched so that the

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The CAEPS pedestal is designed to bridge the or unintended movement of the flask during any
gap between the adjuster thimble and the flask, operation. Stabilizing devices are provided on the
and provide a shielded passage for the cobalt Transporter/Erector, to ensure the basic stability of
adjuster during its removal from the reactor. The the Transporter/Erector whenever the flask is in a
pedestal is dimensioned such that it fits within the partially or fully raised position. The stabilizers are
confines of adjacent Reactivity Control Units which equipped with interlocks to the elevating
are closely pitched on the reactivity mechanism mechanism such that no erecting or lowering
deck. The pedestal is mounted in and positioned motion can be effected unless the
around the adjuster thimble by the positioner. The Transporter/Erector is fully stabilized.
shielding provided by the pedestal is designed to
minimize man-rem exposure to the operator. At the SIFB, and depending upon the reactor site
Auxiliary shielding blocks are used to improve configuration, the positioning of the flask onto the
local shielding effectiveness within the space discharge port is performed by the SIFB service
restrictions caused by adjacent Reactivity Control crane and/or the Transporter/Erector. The
Unit mechanisms and which vary from position to Transporter/Erector is required to park, be
position. The number and complexity of stabilized, and then erect the flask to the vertical
assembling these is minimized so as to not position. The flask is then held vertical by the
impede the cobalt adjuster discharge process. crane or the Transporter/Erector until discharging
Both the flask and pedestal are capable of being of the cobalt adjuster into the bay via the
used in turn on all reactor units as required. discharge port is complete.

C.Flask Positioner The handling and processing of cobalt adjusters


The CAEPS flask positioner is designed to accept, are carried out at such depth in the SIFB as to
carry and position the flask and pedestal at each provide sufficient water shielding and minimize
of the adjuster thimble positions on the reactivity radiation hazards to cobalt operations personnel.
mechanism deck. Its high accuracy of positioning The equipment involved is primarily comprised of
of the pedestal is essential to avoid damaging the the discharge port, and cobalt adjuster storage
thimble when lowering the pedestal into the deck. and processing equipment.
The flask positioner is very similar to a crane and
runs on rails located approximately 3 meters E.Discharge Port
above the reactivity mechanism deck. Due to the The cobalt discharge port is located in the SIFB
use of the positioner in the cobalt adjuster cobalt discharge slot. The port provides shielding
replacement process, only a few CAEPS when the cobalt adjuster is lowered from the flask
operations require the use of the overhead reactor into the SIFB cobalt slot. The top section of the
building crane. port is designed to allow the flask to be located
and mounted to it. The cobalt then passes
D.Transporter/Erector through a centrally located bore in the discharge
After each irradiated Cobalt Adjuster Rod is port.
removed from the reactor into the CAEPS flask,
the boiler room crane is used to lift the flask from Beneath the discharge port resides the discharge
the positioner and to lower it into the trough, it is used to accept and provide visual
Transporter/Erector. The Transporter/Erector is confirmation that the cobalt adjuster has been fully
comprised of a simple tractor drawn carriage on lowered from the flask.
which a mechanized cradle is mounted to support From the discharge trough, the cobalt adjuster is
and elevate the CAEPS flask. The transferred to the storage rack via the transfer arm
Transporter/Erector is used to safely transport the and monorail trolley, where it awaits processing.
CAEPS flask, containing the cobalt adjuster rod,
between the reactor building and the secondary F.Cobalt Adjuster Processing Equipment
irradiated fuel bay (SIFB). It is thus designed to The Cobalt Adjuster Processing Equipment is
function both indoors and outdoors and travel comprised of the Inspection Table, Bundle
anywhere within the reactor site. Separator, Center Rod Muncher and Control
Panel.
The Transporter/Erector is equipped with an
integral erecting mechanism which is fully power
operated and fail safe to prevent any uncontrolled

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G.Inspection Table control panel which shows the position of the
The inspection table provides an area for cutter assembly.
inspection of the cobalt bundles and storage for
individual bundles and bundle carriers. In J.Control Panel
addition, the table provides support for the bundle The operation of the bundle separator/inspection
separator, hydraulic cylinders, tubing and in case table and centre rod muncher hydraulics are
of separator malfunction, a manual adjuster cone manually initiated from the control panel. The
cutting facility. working medium of the hydraulic system is
demineralised water taken from and recirculated to
The table rests on the bay bottom and is secured the SIFB.
to the edge of the bay by two straps. A cut-out at
one end of the table provides for containment of In addition, two controlex cable levers are located
the catenary hoses that connect the valve panel to on the panel, one for operating the bundle shuffler
the inspection table/bundle separator assembly control valve, and the second for position
hydraulics. indication of the muncher cutter. The hand lever
operated control valve of the muncher is also
H.Bundle Separator located on the panel.
The bundle separator grips the cobalt adjuster
assembly head cup and lower cone, placing the K.Cobalt Bundle Shipping
adjuster centre rod in tension. The tensile force After the individual cobalt bundles have been
applied is sufficient to fracture the centre rod at a removed from the adjuster rod assembly,
designed weak point located at the lower cone inspected, and measured for their curie content,
area of the center rod. The fractured centre rod they are placed in MDSN’s F231 shipping flask for
allows the adjuster to be disassembled into cobalt transportation to MDSN’s processing facility in
bundles and waste component. Kanata, Ontario. MDSN’s F231 shipping flask, as
used for transporting the cobalt, is a purpose built
A rotating shaft anchors the bundle separator to flask which is licensed by the CNSC for the
the inspection table. A hydraulic cylinder bolted to transportation of up to 400,000 curies of cobalt 60.
the inspection table enables the separator to be
rotated from a horizontal to near vertical position
for easy acceptance of the cobalt adjuster rod SUMMARY
from the storage rack and monorail. The hydraulic The technology for cobalt-60 production in
cylinders and controlex cable of the separator CANDU reactors, designed and developed by
inspection table assembly are remotely operated MDS Nordion and Atomic Energy of Canada, has
from the control panel located at the edge of the been safely, economically and successfully
bay. employed in CANDU reactors with over 195
reactor years of production.
I.Centre Rod Muncher
The muncher, located on the bay bottom adjacent Today over forty percent of the world’s disposable
to the inspection table, consists of a pedestal, medical supplies are made safer through
cutter assembly, storage bin, catenary hoses and sterilisation using cobalt-60 sources from
a controlex cable. The storage bin receives MDS Nordion. Over the past 40 years,
adjuster waste components resulting from the MDS Nordion with its CANDU reactor owner
adjusters disassembly. partners, has safely and reliably shipped more
than 500 million curies of cobalt-60 sources to
The waste components from the bundle separator customers around the world.
are discharged into the bin via a chute system
located at the end of the bundle separator and MDS Nordion is presently adding three more
under the inspection table. In addition, the bin CANDU power reactors to its supply chain. These
receives lengths of the adjuster centre rod and three additional cobalt producing CANDU’s will
cable fed through the cutter assembly. The cutter help supplement the ability of the health care
assembly is actuated by a double acting water industry to provide safe, sterile, medical
operated piston, controlled from the control panel. disposable products to people around the world.
The controlex cable actuates an indicator on the As new applications for cobalt-60 are identified,
and the demand for bulk cobalt-60 increases,

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MDS Nordion and AECL continue to identify
additional CANDU reactor owners who recognise
the mutual benefits of cobalt-60 production.

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