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Renewable and Sustainable Energy Reviews 134 (2020) 110374

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Renewable and Sustainable Energy Reviews


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Whether CCS technologies will exacerbate the water crisis in China? —A


full life-cycle analysis
Lin Yang a, b, Haodong Lv a, b, *, Dalin Jiang c, Jingli Fan d, Xian Zhang e, **, Weijun He f,
Jinsheng Zhou a, b, Wenjing Wu a, b
a
School of Economics and Management, China University of Geosciences, 100083, Beijing, China
b
Key Laboratory on Resources and Environment Capacity Under Ministry of Land and Resources of People’s Republic of China, Beijing, 100083, China
c
China Energy Technology and Economics Research Institute, Changping District, Beijing, 102211, China
d
Faculty of Resources & Safety Engineering, China University of Mining & Technology, Beijing (CUMTB), Beijing, 100083, China
e
The Administrative Centre for China’s Agenda 21 (ACCA21), Ministry of Science and Technology (MOST), Beijing, 100038, China
f
Donlinks School of Economics and Management, University of Science and Technology Beijing, 100083 Beijing, China

A R T I C L E I N F O A B S T R A C T

Keywords: Carbon capture and storage (CCS) is an indispensable technology for achieving emission reduction targets, but it
Carbon capture and storage is a resource-intensive process requiring a large amount of water. Based on the full life-cycle analysis, this paper
Water withdrawal firstly reviews the existing research regarding not only the water withdrawal and consumption for pulverized
Water consumption
coal (PC), nature gas combined cycle (NGCC), and integrated gasification combined cycle (IGCC) power plants,
CO2-Enhanced water recovery
Full life cycle
but also the water production resulting from CO2-enhanced water recovery (CO2-EWR). And then a case study is
conducted using the practical data of 35 PC power plants satisfying source-sink matching principle. We found
that: (1) CCS can reduce 140 Mt/a CO2 emissions with a capture rate of 90%, whereas water withdrawal will
increase by 174.9%, and water consumption will increase by 150.5% (without EWR) and 36.9% (with EWR).
Obviously, the CO2-EWR can drastically reduce water consumption. (2) Capture process contributes most to the
water usage. Particularly, PC with circulating cooling requires plenty of water while the increase rate only
doubles with CCS. By contrast, although water withdrawal for PC with air cooling is relatively small, the increase
rate expands 9 times due to cooling the high-temperature flue gas during capture process. (3) The annual water
withdrawal in Ordos Basin and Bohai Bay Basin increases by 347% and 131%, respectively, while water con­
sumption increases only by 30.1% and 45.6%, respectively. Overall, enhancing the condensate recovery treat­
ment during the capture process and the CO2-EWR during the storage process can be considered to deal with
water scarcity challenge.

reach 50% by 2050 [1], and the annual emissions reduction should
1. Introduction reach at least 1 billion tons accordingly [3]. Overall, CCS has been
proved to be an indispensable tool to tackle climate change.
Climate change represents an enormous threat to sustainable Global power generation reached 26.7 trillion kWh and its CO2
development, and reducing greenhouse gas emissions has become an emissions reached 13 billion tons in 2018, accounting for 38% of the
international focus. Carbon capture and storage (CCS), which comprises total energy-related CO2 emissions [4]. China’s natural resources have
various options to capture CO2, and then pressurize and transport it to a long been in the state of “rich in coal, low in gas and low in oil” and the
geological location for permanent storage, is an emerging technology coal-dominated energy structure cannot be fundamentally altered in the
expected to achieve large-scale low carbonization of fossil energy. CCS short term. Coal-fired plant power had exceeded 1000 GW in 2018,
will contribute 32% of the total emission reductions through 2050 in the which accounts for 60.2% of the total installed capacity in China [5].
1.5 ◦ C scenario (1.5DS) and 14% in the 2 ◦ C scenario (2DS) [1,2]. In IEA requires China to retrofit 185 GW of coal-fired power installed ca­
China, the contribution of CCS-related emissions reductions should pacity by 2035 to achieve the 2 ◦ C target set at the Paris agreement [6].

* Corresponding author. Key Laboratory on Resources and Environment Capacity Under Ministry of Land and Resources of People’s Republic of China, Beijing,
100083, China.
** Corresponding author.
E-mail addresses: lvhd318@163.com (H. Lv), zhangxian_ama@163.com (X. Zhang).

https://doi.org/10.1016/j.rser.2020.110374
Received 8 March 2020; Received in revised form 15 September 2020; Accepted 15 September 2020
Available online 24 September 2020
1364-0321/© 2020 Elsevier Ltd. All rights reserved.
L. Yang et al. Renewable and Sustainable Energy Reviews 134 (2020) 110374

Abbreviation definition IEA International Energy Agency


IECM Integrated Environmental Control Model
APH Air preheater IGCC Integrated gasification combined cycle
CCS Carbon capture and storage IPCC Intergovernmental Panel on Climate Change
CEC China Electricity Council kWh Kilowatt hour
CO2 Carbon dioxide LCA Life cycle assessment
DCC Direct contact cooler LNG Liquefied natural gas
E-Gas Two sections of coal water slurry gasification MEA Monoethanolamine
EIA Energy Information Agency MMBtu Million British thermal units
EOR Enhanced oil recovery MMscf Million standard cubic feet
ESP Electrostatic precipitator device MWh Megawatt hour
EWR Enhanced water recovery NETL National Energy Technology Laboratory
FGD Flue gas desulfurization NGCC Nature gas combined cycle
GE General Electric Company PC Pulverized coal
GTCC Gas turbine combined cycle SCR Selective catalytic reduction
GW Gigawatts US United States

Therefore, it is imperative to deploy CCS technology in China as soon as field. It is acknowledged that China is in extreme lack of water resource
possible. and the water distribution of is uneven. Hence, China’s CCS deployment
Scarce water resources have become a severe environmental chal­ should fully take the uneven distribution of regional water resources
lenge for the development of energy industry [7,8]. In 2018, global into account. To fill the existing research gaps, firstly, this paper dis­
water withdrawal and water consumption of thermal power plant cusses the life cycle water usage for power plant with CCS. Specifically,
occupied 38.7% and 20.7%, respectively, of the total industrial water it includes the water withdrawal/consumption and water production for
[9]. In addition, approximately 122.58 billion m3 of seawater is directly pulverized coal power plants (PC), nature gas combined cycle power
used for cooling water of thermal power plants [5]. The full life-cycle of plants (NGCC), and integrated gasification combined cycle power plants
CCS technology needs to consume water resources [10,11]. It is esti­ (IGCC) with CCS retrofitting in terms of fuel production and trans­
mated that CCS retrofitting will increase water usage of power industry portation, energy conversion, CO2 transportation and CO2 storage.
by 80% through 2030 in the U.S [12]. Moreover, CCS-related water Moreover, the various technological options (e.g. capture technologies,
usage is also vulnerable to fuel production and transportation mode, as cooling technologies) are fully considered. Secondly, a case study is
well as power plant configuration [13]. Hence, water resources are most conducted using the practical data of an electricity enterprise in which
likely to be a considerable constraint on the large-scale application of 35 PC power plants (39,140 MW) satisfy the source-sink matching in
CCS in China. different regions. The results aim at providing some recommendations
Life cycle analysis (LCA) has been widely used to assess the envi­ for the optimal CCS deployment under restriction of water resources in
ronmental and resource impacts associated with CCS retrofitting of the future.
power plants [14–16]. For example, Tang et al. (2014) [17] discussed The rest of this paper is structured as follows: Section 2 introduces
the environmental influence of coal-fired power plants with CCS, noting the distribution of CO2 storage sites and power plants as well as the
that CCS has adverse effects on human health, biodiversity and pro­ status of arid areas water resources in China. Section 3 systematically
duction operations. Additionally, some scholars investigated the distri­ summarizes the water withdrawal and water consumption in the CCS
bution of energy with or without CCS from the energy balance full life cycle. Section 4 provides a detailed evaluation of the water usage
perspective [18–21]. In terms of water resource demand, the previous for power plants in major basins through a case study. The conclusions
studies mostly focused on the carbon capture process (solvent injection, and policy implications are drawn in Section 5.
CO2 absorption and CO2 precipitation) [22–24]. Among them,
Lim-Wavde et al. [25] and Sathre et al. [22] explored the water usage of 2. Distribution of carbon storage basins and water resources in
power plants with CCS by 2030 from the aspect of water equilibrium; China
Tidwell et al. [23] discussed the CCS-related water resource stress in
some water-scarce areas of the United States, indicating that the daily Distribution of underground saline aquifers is unevenness in China,
water usage may increase by nearly 1 million cubic meters; Court et al. and the high-quality storage areas are mainly concentrated in the
[26] noted that the cooling water demand for a CCS-retrofitted PC northwest and northeast regions (see Fig. 1). Offshore storage may be a
power plant is approximately double that of the unmodified power suitable option for the power plants in southeast China in the future.
plant; Merschmann et al. [27] analyzed the effects of cooling systems on Referring to the location of major sedimentary basins, China has 17
water usage during the capture process, showing that water withdrawal major sedimentary basins (specific storage sites are oil and gas fields or
will increase by 102–121% and 93–113% in coal-fired power plants saltwater beds in the basin). The basins with considerable storage po­
installed with once-trough cooling and closed cooling systems, tential are mainly concentrated in Tarim, Ordos, Songliao, the southern
respectively. part of northern China, Bohai bay, etc., while PC power plants are mainly
Nevertheless, the previous research conducted by the domestic and distributed in the northern China and the southeastern coastal areas. The
international scholars is still limited to assess the water resource pres­ source and sink exhibit reverse distribution. The CO2 storage capacity in
sure resulting from CCS deployment. Firstly, most of them focus on the the deep saline aquifers is approximately 1191.95 × 108 t, and the po­
carbon capture process, while the entire life cycle has not been tential water recovery is approximately 40.9 × 108 t, which is sufficient
adequately considered. Although CCS technology inevitably requires for 10 coal chemical enterprises with 20 years of operation [28]. The
excessive water resource, it is capable of exploiting the deep salt water sedimentary basin has an extensive distribution in the western region of
with CO2-EWR (Enhanced Water Recovery) technology so as to lighten China, including the Tarim Basin, Junggar Basin, and Qaidam Basin, and
the water resources pressure to some extent. Secondly, all of the existing the quantity of water resources recovery is abundant with a storage
literatures are theoretical discussions without empirical analysis in this capacity and potential water recovery of 661.53 × 108 t and 20.02 ×

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Fig. 1. Distribution of CO2 storage locations in China. Data source: China Geological Survey.

108 t, accounting for approximately 55.49% and 48.96% of the total 2000 (319 GW), including 1144 GW with thermal power and a 4.8-fold
storage capacity and water recovery, respectively. Obviously, enhancing increase over 2000 (237 GW) [29,30]. The installed power generation
water resources recovery can be considered as an effective way to structure has been further optimized with 113 coal-fired power units of
alleviate the water resources shortage pressure resulting from CCS 1000 MW and 44.7% of that of 600 MW or above [30]. With the further
deployment [28]. expansion of the power spatial distribution, most of the new thermal
According to the distribution map of major power plants in China [6] power capacity has been transferred to the water shortage areas in
(see Fig. 2a), most thermal power plants are concentrated in power northwest China, which has a serious influence on the water resources
centers which account for more than 60% of the total installed capacity, and environment. Generally, severe drought arears easily occur in
especially in the eastern provinces which are huge consumers of elec­ northern China, southwestern China and parts of northeastern China
tricity. By the end of 2018, China owned 1900 GW of installed (see Fig. 2b). The development of coal-fired power plant has increased
full-caliber power generation capacity and had a six-fold increase over the pressure on the fragile water resources ecosystem as the gradually

Fig. 2. Major coal mines sites and coal-fired power plants sites (a) and distribution of drought-plagued counties in China (b).

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increasing degree of drought, especially in the Ordos Basin where the including solvent selection (ammonia for environmental control sys­
concentrated distribution of power plants causes a more serious water tems), limestone and monoethanolamine (MEA), technical imple­
crisis [6]. mentation, and cooling system transformation. CO2 transport generally
Inland arid areas in China are mainly distributed in Xinjiang, Gansu, includes tank car transport, ship transport and pipeline transport, and
Ningxia, Qinghai and Inner Mongolia with a total area of 3.36 million km2 the CO2 storage process mainly refers to the CO2-EWR process. Fig. 3
[31], accounting for about 1/3 of the land area. Nevertheless, surface describes the process [36,37].
water and groundwater resources in these arears only account for 3.3% Generally, there are two commonly indicators for measuring water
and 5.5% of the total national resources, respectively [32]. The total usage. One is water withdrawal, which indicates as the total amount of
water resources of China in 2018 were 2746.3 billion m3, which is close water extraction from water sources and can either be depleted or
to the international standard of 1700 m3 per capita [33]. The State blowoff to other water sources, and the other is water consumption,
Council [34] has established three red lines for controlling water in view which regarded as the lost drainage [24,38–41]. Notably, water re­
of the current water shortage: (1) The red line for the development and sources are mainly consumed by cooling systems, steam circulation,
usage of water is set to be below 700 × 108 m3 by 2030. (2) The red line traditional environmental control and CO2 capture systems. Fig. 4
for water efficiency is set to be at or near the world’s advanced level by illustrated the water cycle and utilization during the capture process in
2030, and water usage per 10,000 yuan industrial value-added (at the power plant with CCS. Only four simplified processes (CO2 pre­
constant 2000 prices) should drop below 40 m3. (3) The red line for treatment, entering into absorption tower, regeneration tower, and
effective utilization coefficients of irrigation water is set to increase to compression to precipitation) are drawn because the key stage of CCS is
above 0.6. CO2 capture, which accounts for a large proportion of water usage.
Note: The data source of (a) is the China Electricity Council, and the
data source of (b) is the MWR [35].
3.1. Fuel extraction and transportation
Overall, the distribution shows a tendency of more east and less west
for the power plants concentrated in the central region of north China
3.1.1. Coal mining and transportation
and a relatively decentralized distribution for the sedimentary basins.
Inevitable demand for coal in China accounted for more than 70% of
For the distribution of drought-plagued counties, most of the them are
its energy needs in 2012 [42], and coal utilization is projected to in­
located in the general arid areas, whereas the severe arid areas are
crease by 30% over the next 20 years. Consequently, the capacity of the
mainly concentrated in the northeastern and southwestern regions. The
coal-fired power plants will be raised by approximately 40% [19]. With
basins in the western region have a wide distribution range but few
the increase in coal consumption, the total amount of water resource is
power plants.
projected to reach the peak of 79.91 × 108 m3 in 2030 [43,44]. The
water withdrawal of the whole coal industry chain is still increasing
3. Full life-cycle analysis
under the current situation [45], and fresh water extraction from mining
to power generation or coal chemical transformation is 5.56 × 1010 m3
The main processes of the full life cycle for power plants with CCS
with more than 10% of the national water withdrawal.
retrofitting include fuel production and processing, fuel transportation,
As a cheap and convenient semi-finished material for power gener­
energy conversion, CO2 transportation, and CO2 storage. To be specific,
ation, coal-based energy technologies have become increasingly devel­
fuel transportation refers to a rail for coal and pipeline for natural gas.
oped in recent years [46]. The development modes include open-pit
Energy conversion, as the most critical process, denotes carbon capture
mining and underground mining, and the transportation can be by train,

Fig. 3. The full life cycle flow chart of power plants with CCS.

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Fig. 4. Water flow diagram of the capture process. Note: FGD refers to flue gas desulfurization. DCC refers to the direct contact cooler.

car or mud pipeline [47,48]. Environmental controls such as dust sup­ acknowledged that coal resources are inflammable goods, and therefore
pression cause underground mining to consume more water than surface the constant friction between coal and carriages will continuously raise
mining. In addition, mining equipment has also led to more indirect the temperature of surrounding environment to pose a fire risk during
water usage in underground mining [49]. long-time transportation. Therefore, it is essential to wet coal by
Meldrum et al. [50] collected a large number of studies on fuel spraying water during transportation. In additional, coal attaches to a lot
production and water usage for power generation, and the water usage of dust and the dust will pollute the surrounding air with the continuous
coefficient of the fuel supply was expressed in the form of gallon/t. By movement of the train. Thus, the dust inside the coal will be agglom­
applying the Integrated Environmental Control Model (IECM), the erated resulting from the sprinkling.
calculated water usage of fuel production is estimated as the water use According to the research on the relationship between CCS and coal
coefficient of fuel multiplied by its mass or volume. Table 1 lists the consumption [19], the average water usage for coal in power plants is
minimum, standard and maximum value of water usage for fuel supply 158.3 t/h, whereas it will increase to approximately 200.4 t/h due to
based on the hypothesis for a PC unit net efficiency of 35.4% and a fuel CCS retrofitting. The difference in maximum coal demand with and
calorific value of 21 MMBtu/t [36]. The coal mining mode and transport without CCS is 21–31% depending on the retrofitting approach [51],
type are mainly to be underground mining and train transportation, which is significantly higher than the current levels of coal consumption.
respectively, in order to ensure environmentally friendly and sustain­ Supposing water usage is calculated according to the standard coal life
able resource development. The water usage for transportation refers to cycle, the hourly water usage of power generation with and without CCS
the water consumption during the process of coal-related railway configuration in the whole coal supply process is expressed in Table 2.
transport and slurry transport [36]. To be specific, it is widely Overall, the water withdrawal and consumption of the coal supply stage
will increase by 4210.6 gal and 4164.8 gal, respectively, during the unit
hours of power generation with CCS retrofitting.
Table 1
Water usage during fuel supply stage.
3.1.2. Natural gas extraction and transportation
Process Water withdrawals Water consumption At present, the transportation mode of natural gas is mainly pipeline
(gal/t) (gal/t)
transportation characterized by long distances, fast speed, resource
(minimum, nominal, (minimum, nominal, saving and environmental protection [52]. Once the temperature of
maximum) maximum)
natural gas is approximately − 162 ◦ C, it will be converted into liquefied
Production Open-pit mining (1.09, 6.54, 28.3) (1.09, 6.54, 28.3) natural gas (LNG). As an essential means of natural gas transportation,
Underground (17.4, 58.8, 392) (14.7, 58.8, 392)
LNG transportation is a more flexible model that can save storage space
mining
Processing (19.6, 39.2, 2179.2) (19.6, 39.2, 2179.2)
Transport Train (1.09, 2.18, 4.36) (0.22, 1.09, 2.18) Table 2
Slurry (218, 240, 893) (218, 240, 893) Standard water usage accounting for coal supply.
Note: The above data were obtained from Ou et al. [36]; however, water con­ Without CCS With CCS Δ (Added value)
sumption is equivalent to water withdrawal due to the small water usage and the
Water withdrawals (gal/h) 15,860.5 20,071.1 4210.6
absence of relevant data. The reference value used in this paper is normal value
Water consumption (gal/h) 15,687.9 19,852.7 4164.8
for the maximum value, and minimum value are affected by the type of coal.

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and cost [53]. Meldrum et al. [50] expressed the water usage coefficient Table 4
of the natural gas supply based on natural gas per million standard cubic Estimates of water usage for the different power plant equipment technologies.
feet of gallons (gallons/MMscf). Table 3 shows the water usage range of Technology Water withdrawals Water consumption Additional details
the natural gas supply process from exploitation to transportation based (gal/MWh) (gal/MWh) about estimate
on the hypothesis of an NGCC unit net efficiency of 51% and fuel calo­ PC 1.45–16.3 0.89–2.85 (construction only)
rific value of 1031 MMBtu/MMscf. PC + CCS 2.1–30.9 1.58–5.55 CCS retrofit
Natural gas demand per generation hour is the same with and (construction only)
without CCS because of the data deficiency, and it cannot calculate the IGCC 1.16 0.55 (construction only)
IGCC + CCS 2 1.49 CCS retrofit
specific amount of water increase. For the convenience of calculation, (construction only)
according to Ref. [36], the water withdrawal and consumption in the NGCC 0.61–5.62 0.39–1.03 (construction only)
natural gas supply process are 5.6 gal/MWh and 4.6 gal/MWh without NGCC + 1–14.1 0.76–2.59 CCS retrofit
CCS and 6.5 gal/MWh and 5.3 gal/MWh with CCS, respectively. CCS (construction only)

Data source: [36,50,59]. Note that there is a big gap in the water usage for
3.2. Energy conversion infrastructure transformation as the types of coal-fired PC are divided into or­
dinary sub-critical, supercritical and ultra-supercritical. Similarly, the water
usage for NGCC power plant infrastructure is also different considering that fuel
The energy conversion process mainly includes CCS infrastructure
sources are divided into conventional natural gas and shale gas. Due to the data
retrofitting and carbon capture. CCS infrastructure retrofitting refers to
deficiency, there is no range value for water usage in IGCC power plants.
the construction of components (such as adsorbent treatment systems
and combustion turbines) and power plants [54]. In addition, carbon
common unit of gal/MWh.
capture is affected by the unit type, the capture mode, the complement
solvent type, and the cooling system.
3.2.2. Water usage for CCS capture
The CCS full life cycle consumed a great deal of water resource,
3.2.1. Water usage for CCS infrastructure retrofitting
especially during the carbon capture process. Moreover, carbon capture
The water withdrawal and consumption factors for PC power plants
patterns and types affect water demand to some extent [60–62].
are mainly affected by three kinds of water: boiler make-up water, flue
gas desulfurization make-up water and cooling water [55]. Water de­
(1) Capture modes and types
mand for IGCC power plants and NGCC power plants came from
fundamental research programmed by NETL [12] in 2007. The water
Some studies have estimated water usage in different capture sys­
requirement of NGCC and IGCC power plants is different from that of
tems and power plants, including power plant types, capture technology
coal-fired power plants. Although all need cooling water, the water
and cooling modes. Carbon capture mainly consists of post-combustion
demand of NGCC and IGCC is minimal due to the fact most of the output
capture, pre-combustion capture and oxy-combustion capture.
is generated by gas turbine, which consumes less fuel and water than the
Post-combustion technology is generally applied in traditional PC
old-fashioned steam turbine technology. In addition, since IGCC relies
and NGCC power plants [24]. The purpose of the pre-combustion cap­
on water only in important processes, saline water is generally not
ture system is to segregate carbon dioxide from the high-pressure syngas
required [56].
released by the IGCC power plant while the oxy-combustion capture
Ou et al. [36] calculated the total water usage of the infrastructure
system is also commonly applied in traditional PC power plants [56].
construction and CCS retrofitting in power plants on the basis of water
Recent analyses by Marion et al. [63], IEAGHG [64] have shown that
usage estimation of various economic sectors by applying the economic
oxy-combustion with CO2 capture is conventional air-based combustion
input-output combined life cycle assessment (EIO-LCA) model [57].
utilizing amine scrubbing for CO2 control. The post-combustion capture
Water usage for parts manufacturing and construction of the power
system does not require major transformation to the boiler, and how­
plant mainly depends on the scale, structure and process design. Ac­
ever, the reconfiguration is necessary for steam cycle must be recon­
cording to the assumptions of NETL [58], the net installed capacity of
figured so as to extract low-pressure steam and use for solvent
the PC and IGCC power plant is 550 MW with or without CCS retrofit­
reconstruction [6,65,66]. Moreover, flue gas must undergo a purifica­
ting, whereas the net installed capacity of the NGCC plant with and
tion process before CO2 capture to remove sulfur, nitrous oxide, dust
without CCS is 474 MW and 555 MW, respectively. Meldrum et al. [50]
[51]. Post-combustion capture system is envisioned to be a promising
summarized the water demand of equipment construction life cycle for
model for near-term, state-of-the-art carbon capture technologies. There
different PC, IGCC and NGCC power plants (see Table 4) based on the
are three simplified process flow diagrams of different CO2 capture types
hypothesis for the power plant capacity of 85% and the lifetime of 60
shown in Fig. 5, Fig. 6 and Fig. 7, respectively, which describe the water
years. All values were converted into units so that the water usage for
flow during the capture process.
CCS infrastructure retrofitting could be uniformly converted into a
The fundamental reason for the difference in capture mode lies in the
power plant type. That is the power plant determines the CO2 capture
Table 3
technology to be adopted in the future. In addition, compared with
Water usage during natural gas supply stage.
power generation technology, the influence of cooling system on water
Process Water withdrawals Water consumption withdrawal and water consumption is more prominent. Koornneef et al.
(gal/MMscf) (gal/MMscf)
[67] summarized the water usage of three carbon capture technologies
(minimum, nominal, (minimum, nominal, and further explained the range of capture efficiency corresponding to
maximum) maximum)
each technology (see Table 5).
Production Traditional (15.4, 154, 2927) (15.4, 154, 2927) Pre-combustion carbon capture is a potential decarbonization tech­
drilling nology at present; however, the selection of capture solvent would affect
Hydraulic (154, 1849, 28,655) (154, 1849, 28,655)
fracturing
the water usage of the CCS full life cycle to a certain extent. Pre-
Processing (77, 77, 77) (77, 77, 77) combustion capture can also be divided into the membrane separa­
Transport Pipeline (616, 616, 2003) (154, 462, 924) tion, adsorption, physical absorption, low-temperature separation and
Note: The water consumption is equivalent to water withdrawal due to the small chemical absorption technology from the perspective of capture tech­
water usage and the absence of relevant data. Based on Meldrum et al. [50], the nology [69]. Based on the above classification, Sharma et al. [70]
minimum nominal values are equal. Normal values are referenced in this paper. analyzed the average water usage and unit generation of coal-fired

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Fig. 5. Brief process flow chart of the post-combustion CO2 capture system. Note that the SCR is short for selective catalytic reduction, APH is short for air preheater,
ESP is short for electrostatic precipitator device, and FGD is the abbreviation of flue gas desulfurization.

Fig. 6. Process diagram of the pre-combustion capture system.

power plants in India under different capture solvent configurations post combustion capture in PC power plants. The result describes the
(amine, ammonia and membrane) (see Table 6). Amine based capture is additional cooling water demand of power plants with subcritical, su­
the most common. However, the cost of membrane capture technology percritical and ultra-supercritical increased by 47%, 33% and 31%
is relatively high, and ammonia capture technology requires more compared with power plants without CO2 capture, respectively. Sharma
water. et al. [70] analyzed the impact of various capture technologies on the
A once-through system or cooling tower is often applied in tradi­ total water demand for power plants. The cooling system has a different
tional power plants. A once-through system typically takes water from influence on water demand of PC power plant. Notably, the air-cooling
rivers or lakes and drains it back after generating while a cooling tower system has more advantages than wet cooling towers under a highly
system can recycle the water many times [66]. Compared with the two water-stressed condition.
cooling systems, cooling tower evaporates a great quantity of water so Subcritical and supercritical boilers for PC power plants use different
that water usage average is 30%–70% more than that of the water use scaling factors. Concerning the same amount of power output,
once-through system [71]. A study from EPRI [72] estimated that the the supercritical boiler has higher efficiency with less cooling water. The
water consumption of once-through cooling system and closed-loop schematic diagram of three different cooling systems is shown in Fig. 8.
cooling system is 300 gal/MWh and 480 gal/MWh, respectively. How­ Based on the original literature, professor Macknick [74] and
ever, it did not account for the evaporative loss. Lim-Wavde [25] estimated the water usage factors of power generation
Brandl et al. [73] evaluated the cooling water requirement for the technology operation, which provided a basis for the electric power

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Fig. 7. Brief process flow chart of the oxy-combustion capture system.

3.3. Transport and processing with CO2


Table 5
Water usage and capture performance with different capture modes.
CO2 transportation refers to the process of transporting captured CO2
CO2 capture Power plant Water usage Water usage Capture to a storage or utilization site; this is similar to oil and gas transportation
technology w/o capture with capture efficiency
in some respects [76,77]. Some power plants do not have sufficient CO2
(gal/MWh) (gal/MWh) (%)
storage capacity due to the geological structure; therefore, it is crucial
Post- PC 676 1331 85–90
for suitable transportation approaches to meet the storage needs of large
combustion subcritical
PC 594 1146 85–90 amounts of CO2. Several studies and reports [78–80] have published
supercritical CO2 transport system cases. There are two ways of CO2 transportation
NGCC 269 486 85–90 from power plants to storage sites: 1) by ship for liquefied carbon di­
Pre- IGCC 356–375 478 85–90 oxide, and 2) by pipeline. The transport distance is about 700–1000 km
combustion
by ships and 120 km by pipeline [81].
Oxyfuel PC – 784–795 90–100
combustion At present, pipelines are the primary mode of CO2 transportation
NGCC – 50–100 [82]. To calculate the water usage of the CCS full life cycle more
effectively, this paper refers to the basic parameters of natural gas
Data source: [12,68]. Note that the water usage for post-combustion, pre-
combustion and oxyfuel capture is on the basis of power plants with cooling transportation (see Table .3). It assumes that water withdrawal and
towers system, and the ranges refer to kinds of gasifier technologies and the water consumption are similar, taking the standard value of 616
oxygen purity. gal/MMscf as the water withdrawal for CO2 transportation and 465
gal/MMscf as the water consumption value. Table .8 shows the values
with the unit conversion of gal/t CO2.
Table 6 However, a more consistent and transparent multi-standard analysis
Water usage of PC power plants with different capture solvents. should be conducted to ensure complete evaluation of all stages of the
(2) Cooling system CCS full process transformation, which can provide the best support for
Water withdrawal (gal/MWh) Water consumption (gal/ decision-makers to make CCS commercial application as early as
MWh) possible and make the sustainable development of CO2 transport chain
Min Average Max Min Average Max possible.
Without capture 6110 6113 6115 214 215 217
Amine capture 11,094 11,210 11,671 514 524 534
Ammonia capture 14,419 14,531 14,644 411 416 421
3.4. Carbon storage with CO2-EWR
Membrane capture 12,711 12,780 12,872 417 421 426
CO2 geologic storage in deep salt water aquifers is the best storage
approach currently [83,84]. At present, many scholars have put forward
sector to assess the impact of water use (see Table 7). According to the a CO2-enhanced water recovery technology, that is CO2-EWR [85–87],
results from IECM [75], due to the increased production load of CCS which could greatly relieve the reservoir pressure and the CO2 leakage
deployment, the net power generation capacity of the retrofitted hazard. More importantly, it would enable the exploitation of deep salt
coal-fired power plant decreased from 550 MW to 468 MW. For the same water so as to reduce regional water resource pressure [83,88].
reason, the net generation capacity of NGCC plants decreases from 555 Although CO2-EWR technology is still under development in China,
MW to 474 MW with CCS retrofitting. CCS retrofitting is unlikely to its direct and indirect economic benefits are inestimable. Applying the
adopt the once-through cooling system due to its huge water demand. techno-economic resource-reserve pyramid evaluation method [50], the
CO2 storage capacity in deep saline salt water aquifers from 17 signifi­
cant basins in China reached 1191.95 × 108 t. The main application

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L. Yang et al. Renewable and Sustainable Energy Reviews 134 (2020) 110374

Fig. 8. Schematic diagram of three cooling systems. Note: (a) Once-through cooling; (b) Recirculating cooling; (c) Air Cooled.

Table 7 Table 8
Statistics of water usage in power plants under different cooling system Water usage assessment of the CO2 pipeline transport in CCS.
conditions. Water usage (gal/t CO2) Pipeline transport
Plant Technology Rate of water Rate of water
Water withdrawal 11.2
type withdrawal (gal/ consumption (gal/
Water consumption 8.4
MWh) MWh)
Data source: Meldrum et al. [50].
W/O With W/O With
CCS CCS CCS CCS

PC Once-through 28,864 / 132 /


areas are the central and western regions and the southern regions with
Recirculating 583 1098 494 846 capacities of 66.153 billion tons and 11.064 billion tons, respectively.
Hybrid (wet-dry) 345 929 292 716 CO2-EWR would extract fresh water for 715.17 × 108 m3 based on the
cooling projection that 1.5 m3 of salt water is produced by 1 t of CO2 with a 40%
Dry type air cooler 86 732 73 563
recovery rate [89]; fresh water is undoubtedly a very valuable treasure
IGCC Recirculating 424 662 381 550
NGCC Once-through 13,057 / 119 / for the eastern and western regions with huge waters demand and a
Recirculating 243 576 204 431 serious shortage of water. In addition, this technology can effectively
Hybrid (wet-dry) 124 512 104 383 solve the water shortage crisis caused by power plants and coal chemical
cooling
enterprises in the Great Western Development Strategy so as to ensure
Dry type air cooler 6 418 2 313
the energy security and balanced development of regional economies.
Data source: [25,58,74]. Note that wet flue gas desulfurization technology (Wet
FGD) is assumed to be adopted.

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L. Yang et al. Renewable and Sustainable Energy Reviews 134 (2020) 110374

3.5. Summary of water usage for the CCS full life cycle carbon dioxide emission, etc. A total of 99 units and 42 power plants met
the requirements of CCS transformation, with an entire installed ca­
Through reviewing the existing research on water usage in each stage pacity of 55,890 MW under the conditions above. At the same time, the
of the CCS full life cycle, the water withdrawal and consumption of PC power plants distributed throughout the country will be used as emis­
power plants, NGCC power plants and IGCC power plants with CCS sion sources of CO2 and the storage sites of CO2-EWR in the onshore
technologies were presented in Table 9. saline aquifer will be used as sinks. According to the preliminary results
It should be noted that the increased water withdrawal and con­ of source-sink matching in Fig. 9, the bottom figure is the suitability
sumption of different cooling systems depends on the wet desulfuriza­ evaluation for storage sites of CO2 saline aquifers in the basin. CO2
tion technologies [56,66,90,91]. In addition, the type and performance emissions are divided into three levels, with the number of units with
of the power plant also affect water usage during the process of fuel CO2 emissions greater than 1 Mt accounting for 80.8% of the total unit.
supply. For CO2 transportation and storage, the factors affecting water Within the search radius of 250 km, 79 units of 35 power plants (44,140
withdrawal and consumption usually involve the transportation mode MW) found suitable storage sites with geological storage and utilization
and storage approach. conditions, whereas 20 units of 7 power plants indicated by the orange
circle found no suitable storage sites with an average CO2 emissions of
4. Case study for power plants 5.9 Mt and a total emission of 40.9 Mt. Based on the actual power
generation in 2016, the total emissions is 165.0 Mt, and the trans­
4.1. Design and selection portation distance is 20.4 km–244.4 km. In terms of regional distribu­
tion, northern China and eastern China have the largest number of
Generally, the new PC power generation units should adopt ultra- power plants with a total of 22 PC power plants and an installed capacity
supercritical units with a capacity of 600 MW or above according to of 27,460 MW, accounting for 62.2% of the total installed capacity.
the upgrade and renovation plan for coal power conservation and Data source: Jiang et al. [97].
emissions reduction (2014–2020) [92]. Therefore, in the construction of The site suitability of CO2-EWR was divided into 6 levels, with white
CCS reserved power plants, the total capacity in the future should be indicating areas not recommended and green indicating high suitability
considered to be no less than 600 MW, and the average annual gener­ (see Fig. 9) with the potential for CCS retrofitting. Preliminary studies
ation time is 4500 h. The CO2 emission source selection criteria refer to show good storage sites (very suitable to the appropriate level) in the
the IEA report in 2016 on CCS retrofitting of PC power plants. The Zhugeer Basin, Tarim Basin, Qaidam Basin, Songliao Basin, Ordos Basin,
capture rate is set based on the emission standard of gas turbine com­ Sichuan Basin, Erlian Basin, Subei Basin and Bohai Bay Basin for the
bined cycle (GTCC) plants with the CO2 emission intensity of 450 g/kWh storage of CO2 saline aquifers. PC power plants were used as an example
[93,94]. Currently, the maximum CO2 capture rate is 90%, and the cycle considering that the types in this enterprise are all coal-fired power
of operation with CO2 capture and EWR project is 20 years [6,95]. The plants. Notably, a range of values will appear in the statistical data
transportation distance of CO2 is set as the upper limit of 250 km in order affected by the power plant scale and coal type, and the range should be
to achieve source-sink matching [86,96]. averaged in order to facilitate calculation (based on Table 9). The CO2
The unit of an enterprise power plant was selected for research ac­ capture is mainly post-combustion, whereas the cooling style is mainly
cording to the evaluation conditions of carbon capture transformation; recirculating cooling and air cooling according to the power plant
the capacity of each unit was required to be more than 300 MW, and the performance.
operation life of the unit was selected after 2005. The unit parameters
were subject to the actual operating conditions in 2016, including
cooling mode, operating hours, power generation, coal consumption,

Table 9
Life cycle water usage of power plant with CCS.
Plant type CCS stage Unit Water withdrawal Water consumption

W/O CCS With CCS (Δ) W/O CCS With CCS (Δ)

PC
Coal supply gal/h 15,860.50 20,071.06 4210.56 15,687.93 19,852.68 4164.75
Energy conversion
Infrastructure retrofitting gal/MWh 1.45–16.3 2.1–30.9 0.65–14.6 0.89–2.85 1.58–5.55 0.69–2.70
Post-combustion capture (recirculating) gal/MWh 583 1098 515 494 846 352
Post-combustion capture (hybrid cooling) gal/MWh 345 929 584 292 716 424
Post-combustion capture (air cooler) gal/MWh 86 732 646 73 563 490
CO2 transportation gal/t CO2 / 11.2 11.2 / 8.4 8.4
CO2 storage gal/t CO2 / − 396 − 396 / − 396 − 396
IGCC
Coal supply gal/h 15,860.50 20,071.06 4210.56 15,687.93 19,852.68 4164.75
Energy conversion
Infrastructure retrofitting gal/MWh 1.16 2 0.84 0.55 1.49 0.94
Pre-combustion capture (recirculating) gal/MWh 424 662 238 381 550 169
CO2 transportation gal/t CO2 / 11.2 11.2 / 8.4 8.4
CO2 storage gal/t CO2 / − 396 − 396 / − 396 − 396
NGCC
Gas supply gal/MWh 5.6 6.5 0.9 4.6 5.3 0.7
Energy conversion
Infrastructure retrofitting gal/MWh 0.61–5.62 1–14.1 0.39–8.48 0.39–1.03 0.76–2.59 0.37–1.56
Post-combustion capture (recirculating) gal/MWh 243 576 333 204 431 227
Post-combustion capture (hybrid cooling) gal/MWh 124 512 388 104 383 279
Post-combustion capture (air cooler) gal/MWh 6 418 412 2 313 311
CO2 transportation gal/t CO2 / 11.2 11.2 / 8.4 8.4
CO2 storage gal/t CO2 / − 396 − 396 / − 396 − 396

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L. Yang et al. Renewable and Sustainable Energy Reviews 134 (2020) 110374

Fig. 9. Preliminary results of power plant source-sink matching in enterprise. Note that the red dot represents power plants position. (For interpretation of the
references to colour in this figure legend, the reader is referred to the Web version of this article.)

4.2. Case methodology standard coal, and QLnet denotes the low calorific value of coal used by PC
power plants. Car refers to the carbon content as received basis. MCO2 and
The total life-cycle water usage of power plants with CCS retrofitting MC refer to the molar mass of CO2 and C, respectively. tCO2 is the pro­
can be calculated as follows: portion of carbon in coal that is oxidized into CO2 [98,99].
FLCW = WUFS + WUIR + WUCC + WUCT + WUCS (1) Qcapture
CO2 = Qemit
CO2 × ηCO2 (3)

where FLCW is the annual water usage in the full life cycle (gal/a). WUFS where Qcapture is the amount of captured CO2, and ηCO2 refers to the CO2
co2
is the water usage for the fuel supply process (gal/a). WUIR refers to the
capture rate (%).
water usage amounts for power plant infrastructure. WUCC refers to the
Because the statistical caliber of water withdrawal intensity and
water usage for CO2 capture in the energy conversion process (gal/a),
water consumption intensity is not uniform in each CCS, the CO2
which accounts for the largest proportion in CCS. WUCT refers to the
emission was calculated according to power plant operating parameters
water usage of the captured CO2 in the transportation process (only
so as to accurately measure the water usage of the full CCS life cycle.
pipeline transportation is considered in the case study). WUCS refers to
There are separate calculation formulas and required parameters in each
the water replaced with CO2-EWR.
CCS stage with the definitions and values shown in Table 10.
To figure up the water consumption in the supplementary process,
the CO2 emissions of the PC power plant should first be calculated. ∑
n
WU wFS = wuwfs ⋅RTi (4)
QSnet Mco2 i=1
Qemit
co2 = PSCC × Pinst × RT × L × Car × × tCO2 (2)
Qnet Mc

n
WU cFS = wucfs ⋅RTi (5)
where Qemit
CO2 is
the annual CO2 emissions from PC power plants (t/a). i=1

PSCC is the coal consumption per unit of power supply (t/MWh). Pinst
where wuwfs andwucfs refers to the water withdrawal and water con­
refers to the installed capacity for PC power plants (MW). RT is the
annual operating hours (h/a). QSnet refers to the low calorific value of sumption per unit of generation hour within the coal supply,

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L. Yang et al. Renewable and Sustainable Energy Reviews 134 (2020) 110374

Table 10

n
Parameter information involved in calculating CO2 emissions. WU cCC = wuccc ⋅ETi (9)
Parameters Description Value Sources i=1

wuwfs Water withdrawal per unit of 15,860.5–20,071.1 [19,36,51] where wuwcc and wuccc refer to the water withdrawal and consumption per
power generation hour in
coal supply process (gal/h)
unit of generation with CCS capture during the energy conversion,
wucfs Water consumption per unit 15,687.9–19,852.7 [19,36,51] respectively.
of power generation hour in

n
coal supply process (gal/h)
WU wCT = wuwct ⋅Qcapture (10)
wuwir Water withdrawal per unit of 8.88–16.5 [36,50,59]
i,co2
i=1
power generation for
infrastructure retrofitting ∑
n
(gal/MWh) WU cCT = wucct ⋅Qcapture (11)
i,co2
wucir Water consumption per unit 1.9–3.6 [36,50,59] i=1
of power generation for
infrastructure retrofitting where wuwct andwucct refer to the water withdrawal and consumption for
(gal/MWh)
wuwcc Water withdrawal per unit of 583-1098 a
[28,58,74]
transport per unit mass during the CO2 transportation, respectively.
power generation for CCS 86–732b ∑
n
capture (gal/MWh) WUcs = wucs ⋅Qcapture
i,co2 (12)
a
wuccc water consumption per unit 494–846 [28,58,74] i=1
of power generation for CCS 73–563b
capture (gal/MWh) where wucs refers to the amount of salt water that can be replaced by 1
wuwct Water withdrawal for 11.2 [50]
transport per unit mass of
ton of CO2 during CCS storage.
CO2 (gal/t CO2)
wucct Water consumption for 8.4 [50]
transport per unit mass of 4.3. Case results
CO2 (gal/t CO2)
wucs Salt water replaced by 1 t of 396 [89]
Combined with the source-sink matching results of the power plant
CO2 stored (gal/t CO2)
SPCC Coal consumption per unit 272.1–409.4 Enterprise
(see Fig. 9), this paper calculated the water withdrawal with CCS full
power supply (g/kWh) statistics life-cycle retrofitting of power plants in the six basins; this was regarded
Pinst Installed capacity for coal- 300/600/1000 as the evaluation objective (the other two basins in the figure only
fired power plant (MW) contain oil fields, so we will not analyze them for the moment) within a
RT Annual operating hours of 378.2–8370.4
range of 250 km. When implementing the CO2-EWR project, the CO2
PC power plant (h/a)
ET Annual output of power 2501,311–7260,000 emitted is piped to the suitable deep salt water aquifer for saltwater
plant (MWh/a) replacement, which may greatly reduce the water pressure caused by
QLnet Low calorific value of coal 13.1–23.1 CCS.
used by power plant (MJ/kg) The total water usage of CCS in the whole process is expressed in the
QSnet Low calorific value of 29.3 [98]
standard coal (MJ/kg)
six basins (Junggar Basin, Ordos Basin, Hailar basin, Bohai Bay Basin,
Car Average carbon content as 56.6 (average) [100–103] Hehuai basin, and Sichuan Basin) where the power plants and storage
received basis (%) sites are concentrated (see Fig. 10). The higher the CO2 emissions, the
MCO2 Molar mass of CO2 (g/mol) 44 [98,104] greater water consumption and correspondingly, the greater water re­
MC Molar mass of C element (g/ 12 [98,104] sources displaced by CO2-EWR. Firstly, all power plants can reduce CO2
mol)
emissions by approximately 140 Mt per year at a 90% replacement rate
tCO2 Carbon percentage oxidized 98 [105]
to CO2 in coal (%) with CCS retrofitting, which produces a positive emission reduction ef­
ηCO2 Capture rate (%) 90 [36] fect. However, considering the water usage in the full life cycle of CCS,
water withdrawal will be raised by 174.9%, and consumption will in­
Data source: The water withdrawal and consumption per unit were obtained
crease by 150.5% (without EWR) and 36.9% (with EWR), respectively.
from a literature review, the performance data of power plant were obtained
With the geographical constraints in the Junggar Basin, Hailar Basin and
from enterprises, and other data were obtained from relevant studies. Note that a
refers to the water usage for recirculating cooling while b refers to the water
Ordos Basin, most power plant units adopt air-cooling for cooling, while
usage for air cooling. the high-temperature flue gas from capture process needs a great
quantity of water to cool down, resulting in a large increase in water
demand. Therefore, it is necessary for the promotion and application of
respectively, and i represents different power plants.
CO2-EWR technology in the carbon sequestration process and gratifying

n
that the replacement of underground salt water by CO2-EWR can reduce
WU wIR = wuwir ⋅ETi (6)
i=1
water consumption to a large extent, with the overall reduction reaching
75.5%. CCS can still minimize water consumption and effectively relieve

n water stress in key coal supply areas to some extent; however, less water
WU cIR = wucir ⋅ETi (7) can be developed through CO2-EWR in terms of quantity.
Specifically, the considerable generating units in the Ordos Basin and
i=1

where wuwir andwucir refer to the water withdrawal and consumption per Bohai Bay Basin increase the local water demand. The total annual water
unit of generation for infrastructure retrofitting of power plants, withdrawal increases by 35.5 (347%) and 42.4 (131%) billion gal,
respectively, and ETi refers to the annual output of power plant i (MWh/ whereas water consumption increases by 2.6 (30.1%) and 12.5 billion
a). gal (45.6%), respectively, due to CO2-EWR technology. Water with­
drawal by power plants can be used repeatedly or even completely
∑ reused, while water consumption is usually non-recyclable; therefore,
n
WU wCC = wuwcc ⋅ETi (8)
i=1 water consumption in power plants is regarded as the controlling factor
from the perspective of water resource protection. In parts of the Ordos
Basin and Bohai Bay Basin (see Fig. 3), which are located in severe arid

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L. Yang et al. Renewable and Sustainable Energy Reviews 134 (2020) 110374

Fig. 10. Water usage for full CCS life-cycle retrofitting and water recovery potential for CO2-EWR under the scenario of source-sink matching. The location of the red
dots represents the power plant. Unit: B gal = billion gal. (For interpretation of the references to colour in this figure legend, the reader is referred to the Web version
of this article.)

areas, the increased total water consumption of the CCS full life cycle reduced by 86.1% when applying CO2-EWR technology. The water de­
can be reduced by 90% and 59%, respectively, with CO2-EWR. mand of the Subei Basin is not as great as other basins from its location in
The annual water consumption in Junggar Basin and Hailar Basin will a coastal area; however, water withdrawal and consumption with CCS
increases by 4.6 and 4.7 billion gal, respectively, without considering retrofitting increased by 87.5% and 34.5%, respectively, under such
storage process, while it can be reduced 96.8% and 95.5%, respectively, geographical conditions. By implementing the CO2-EWR, water con­
with CO2-EWR. The water resources flow in the Junggar Basin, Tuha sumption during CCS whole process is reduced by 51%.
Basin and Tarim Basin can be improved by expanding the matching area Coal supply, infrastructure retrofitting and carbon capture all have
of source-sink or extending the distance of pipeline transportation in the water requirements with and without CCS. According to the contribu­
future. Similarly, the Hailar Basin located in northeastern China has a tion of increased water demand to the full life cycle of CCS (see Fig. 11),
relatively suitable CO2-EWR storage condition for CCS retrofitting, water withdrawal and consumption within carbon capture processes
which will increase the potential for underground salt water develop­ account for the largest proportion of water usage, 95.9% and 96.2%,
ment surrounding the Songliao Basin. Moreover, further expansion of the respectively. They are the critical factors for the increase in CCS water
source-sink matching area will also promote the environmental pro­ consumption. The increased water consumption during fuel supply and
tection and sustainable development of water resources. CCS retrofitting CO2 transport is slightly greater than the increased water withdrawal
has little impact on the water withdrawal and consumption of the with a similar proportion of water usage; this is a necessary reason for
Sichuan Basin in general arid areas (increases of 87.5% and 10%, CO2-EWR to reduce water demand. During the infrastructure retrofitting
respectively), and the water consumption during CCS whole process is process, increased water consumption accounts for only 0.38% less than

13
L. Yang et al. Renewable and Sustainable Energy Reviews 134 (2020) 110374

have a large number of generating units, and the total annual


water withdrawal will increase by 35.5 (347%) and 42.4 (131%)
billion gal, respectively, while water consumption will only in­
crease by 2.6 (30.1%) and 12.5 (45.6%) billion gal, respectively,
as a result of CO2-EWR technology.

In comparison, the water resource pressures in Junggar Basin, Tuha


Basin and Tarim Basin are relatively small, while the Ordos Basin and
Bohai Bay Basin in the North China are face with the dilemma of more
power plants and storage potential and less water resource. In addition,
the overall water usage in capture process increases greatly because the
air-cooling technology needs to cool the high-temperature flue gas
Fig. 11. Increased proportion of water withdrawal and consumption in generated within CO2 capture. More importantly, regarded as a signif­
different stages of CCS. Note: FS = fuel supply, IR= Infrastructure retrofit, CC = icant approach to reduce CO2 emissions, CCS can reduce approximately
carbon capture, CT = carbon transportation.
140 Mt per year with a capture rate of 90%, with a significant effect on
emission reduction.
the increased water withdrawal. The results above can provide an
essential judgment on water usage at different stages of CCS. 5.2. Policy implications

5. Conclusion and policy implications (1) Expanding the scope of CCS research to comprehensively and
systematically consider the water demand of the CCS full life
5.1. Conclusions cycle. It is necessary to explore not only the upstream water usage
of CCS (fuel supply, carbon capture) but also the downstream
CCS has been widely recognized as a critical role in reducing CO2 water usage of CCS (CO2 transport and storage) with an emphasis
emissions. Nevertheless, it is a resource-intensive process that requires a on the water recovery characteristics in the carbon storage pro­
large amount of water resource. Based on the full life cycle analysis, this cess. Through policy advocacy, the negative opinions on CCS-
paper investigates the China’s water resource stress resulting from CCS related water consumption should be reversed, and the positive
deployment through reviewing the existing research on water with­ effect on mitigation can be further popularized.
drawal and consumption of power plant with CCS technologies. The (2) Upgrading and optimizing each stage of CCS technology from a
main conclusions can be drawn as follows: technical perspective in combination with the water consumption
factor to reduce the water usage of the full life cycle. Water
(1) According to characteristics of CCS technologies, the main pro­ consumption control should be implemented during fuel extrac­
cesses of the full life cycle for power plants with CCS retrofitting tion and transportation. Burning high-quality coal for power
are divided into fuel production and processing, fuel trans­ generation in PC power plants could reduce the water demand.
portation, energy conversion, CO2 transportation, and CO2 stor­ The technology of condensate water recovery and treatment in
age. This paper summarizes the unit water withdrawal and water the CO2 capture process should be improved to reduce the cooling
consumption of PC, NGCC and IGCC power plants with and load and promote water recycling in the life cycle. Moreover,
without CCS retrofitting. The water demand for the capture better carbon capture processes or better solvent choices should
process contributes most to the total water usage and is signifi­ take into consideration that could reduce steam consumption in
cantly affected by the cooling type. Specifically, increased water the reboiler of the stripper column to achieve water savings.
withdrawal and consumption for recirculating cooling have a Furthermore, pipeline transport technology needs to be opti­
range of 333.4–529.6 gal/MWh and 227.4–266 gal/MWh, mized during the CO2 transport process, and the improvement of
respectively, while it for air cooling is 412.4–660.6 gal/MWh and CO2-EWR technology during the CO2 storage process would
311.4–492.7 gal/MWh, respectively. The type of power plant also provide potential for underground saltwater development.
causes a difference in water withdrawal and consumption with (3) Reasonable design of CCS retrofitting deployment. The govern­
average increases of 588.1 gal/MWh and 422.7 gal/MWh for PC ment should attach great importance to the water recovery effect
power plants, 238.9 gal/MWh and 170 gal/MWh for IGCC power generated by CO2-EWR technology and integrate it into the CCS
plants, and 376.9 gal/MWh and 270 gal/MWh for NGCC power retrofitting potential evaluation system. The CCS technology
plants, respectively. Water consumption during the trans­ should be optimized under the guidance of the full life cycle
portation and storage process is 11.2 gal/t CO2 and 8.4 gal/t CO2, concept combined with the distribution characteristics of China’s
respectively. The potential of CO2-EWR to exploit subsurface salt arid water resources to accurately grasp the CCS potential and
water is 396 gal/t CO2. geological storage conditions in key areas; this would promote
(2) Taking a Chinese energy enterprise as a case study, the rough the deployment of a CCS demonstration project in accordance
water resource pressure resulting from CCS deployment is with local conditions to reduce the regional water resource
investigated in line with the source-sink matching principle. pressure.
Moreover, the mitigation effect of CO2-EWR on water consump­
tion is also been fully taken into consideration. Specifically, water Overall, this study debunks the view that CCS retrofitting would
withdrawal will increase by 174.9%, and water consumption will consume large amounts of water and is probably to create the water
increase by 36.9% (with EWR) and 150.5% (without EWR) for PC crisis in some area of China, while the role of CO2-EWR technology in
power plant with CCS retrofitting. Notably, the recovery of un­ reducing water consumption during the carbon storage process should
derground saline water through CO2-EWR can effectively reduce also not be ignored. Moreover, the water-saving technologies applied in
water consumption by 75.5%. The water usage at all stages of capture and storage process are bound to have a significant impact on
CCS technology indicates that the water withdrawal and con­ CCS retrofit deployment. Overall, our results can provide further theo­
sumption in the carbon capture process account for the largest retical and practical support for CCS projects, provide a reference for the
proportion, with the percentage of 95.9% and 96.2%, respec­ future implementation of CCS related water resources evaluation man­
tively. It should be noted that the Ordos Basin and Bohai Bay Basin agement from an enterprise perspective, and provide a reference for

14
L. Yang et al. Renewable and Sustainable Energy Reviews 134 (2020) 110374

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