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JMEPEG (2021) 30:5031–5038 ASM International

https://doi.org/10.1007/s11665-021-05604-8 1059-9495/$19.00

An Assessment of Fully Integrated Polymer Sandwich


Structures Designed by Additive Manufacturing
Bruno Dorneles de Castro, Frederico de Castro Magalhães, Túlio Hallak Panzera, and Juan Carlos Campos Rubio

Submitted: 30 November 2020 / Revised: 8 February 2021 / Accepted: 18 February 2021 / Published online: 12 March 2021

3D printing is an additive manufacturing technique (AM) widely used in the aerospace, shipbuilding,
automotive and civil construction sectors to obtain lightweight sandwich structures made with complex core
shapes to achieve excellent multifunctional properties, such as flexural stiffness, and high energy-absorption
capabilities. This study shows an experimental analysis of the mechanical behavior of three types of core,
including (i) out-of-plane and (ii) in-plane hexagonal honeycomb, and (iii) S-shape corrugated core. The
fused deposition modeling method (FDM) is applied in the manufacture of fully integrated sandwich
structures using polylactic acid (PLA) biopolymer filaments. Tensile, flexural and Charpy impact tests are
used for the experimental investigation. The failure modes of polymeric structures are analyzed. The out-of-
plane -comb and S-shape corrugated panels achieve similar mechanical behavior, however, superior tensile
modulus, tensile strength, flexural modulus, flexural strength and energy absorbed are obtained in com-
parison with in-plane -comb core panels. Sandwich panels fabricated by AM achieve acceptable mechanical
properties for secondary structural applications, especially when lightness is required.

honeycomb, allowed unusual materials with negative PoissonÕs


Keywords 3D printing, Additive manufacturing, Mechanical
testing, Metamaterials, Panel core, Sandwich ratio and multifunctional performance (Ref 3). Mousanezhad
structures et al. (Ref 4) investigated hierarchical honeycomb auxetic
metamaterials by experimental and numerical studies and
developed 2D metamaterials with negative PoissonÕs ratio,
with contractions in the transverse direction under uniaxial
compressive load, leading to improved energy absorption and
acoustic damping. On the other hand, Qi et al. (Ref 5) proposed
1. Introduction a reentrant circular honeycomb configuration and performed
experiments and numerical simulations to analyze the quasi-
Recently, the use of lightweight sandwich panels has gained static crushing response of these materials, finding greater
importance due to properties such as high flexural stiffness-to- specific energy absorption than the regular reentrant honey-
weight ratio and excellent thermal insulation. These materials comb configuration.
are made of relatively thin and rigid faces that are connected to The development of new structures has been carried out
thicker and lighter cores, usually made of foam or prismatic using additive manufacturing to replace subtractive manufac-
cores, and can offer an efficient combination in terms of turing, providing high design flexibility, excellent production
flexural stiffness and energy absorption capacity. These struc- capacity for components of complex geometries and low cost
tures have been applied in several fields, including the (Ref 6). The fused deposition modeling method (FDM) is
aerospace, automotive, naval, and military industries (Ref 1, 2). widely used for polymeric materials. With the design of a solid
Technical metamaterials that have remarkable properties 3D CAD model in STL format, a slicing process of the model
provided by architected structures have been developed for the in layers is done and a G-code file is created and sent to the 3D
optimization of material weight. Filling patterns with repetitive printer. The printing process is based on the manufacturing
cell unit configurations, such as hexagonal and reentrant parameters defined for the deposition of polymeric filaments.
Using the layer-by-layer effect until the formation of the final
This invited article is part of a special topical focus in the Journal of structure, different units of core cell can be obtained (Fig. 1).
Materials Engineering and Performance on Additive Manufacturing. 3D-printed materials have been extensively investigated in
The issue was organized by Dr. William Frazier, Pilgrim Consulting, recent years, offering promising applications as components in
LLC; Mr. Rick Russell, NASA; Dr. Yan Lu, NIST; Dr. Brandon D. industries such as construction and automotive (Ref 7-9).
Ribic, America Makes; and Caroline Vail, NSWC Carderock. The mechanical behavior of 3D-printed materials was
analyzed in the literature using experimental and numerical
Bruno Dorneles de Castro, Frederico de Castro Magalhães, and
Juan Carlos Campos Rubio, Graduate Program in Mechanical investigations (Ref 10, 11). The responses under tensile,
Engineering, Gitem Laboratory, Federal University of Minas Gerais, flexural and low-velocity impact loads have shown the effects
Av. Pres. Antônio Carlos, 6627, Pampulha, Belo Horizonte 31270-901, of printing parameters on the mechanical properties of these
Brazil; and Túlio Hallak Panzera, Department of Mechanical and structures and their limitations. Lanzotti et al. (Ref 12) studied
Production Engineering, Centre for Innovation and Technology in the effect of layer thickness and infill orientation on the tensile
Composite Materials, Federal University of São João del Rei, Praça properties of 3D-printed specimens made of polylactic acid
Frei Orlando, 170, Centro, São João del Rei 36307352, Brazil. Contact
e-mails: bdc2016@ufmg.br, fredmag.castro@gmail.com,
(PLA); better results for the tensile modulus and strength were
panzera@ufsj.edu.br, and juan@ufmg.br. obtained using lower infill orientation angles (more aligned to

Journal of Materials Engineering and Performance Volume 30(7) July 2021—5031


Fig. 1 Development and mechanical characterization of the panels: (a) CAD model in STL format, (b) 3D printer-software interface, with
model slicing and G-code file generation, (c) 3D printing using FDM method, (d) 3D-printed polymeric sandwich structures with cellular cores
and (e) mechanical tests

the test direction) and similar results using 0.10 mm and 0.20 Table 1 PLA physical and mechanical properties (12, 15,
mm layer thickness. Zaharia et al. (Ref 13) investigated the use 16)
of 3D-printed sandwich structures with honeycomb, diamond-
celled and corrugated core shapes subjected to compression, Property Nominal range
uniaxial tensile and flexural tests. Using polylactic acid/
polyhydroxyalkanoate (PLA/PHA) for 3D-printed specimens Density, g/cm3 1.24–1.26
and elastoplastic finite element analysis to predict the failure Melting point, C 150–175
Glass transition temperature, C 55–60
mode of the structures, they found a significant effect of the
Flexural modulus, GPa 2.39–4.93
core shape on the mechanical properties of the structure and Flexural strength, MPa 48–110
good similarity between experimental and numerical analysis. Tensile modulus, GPa 2.02–4.15
Gu et al. (Ref 14) presented a 3D-printed biomimetic conch Tensile strength, MPa 14–70
shell prototype to verify the influence of the hierarchy in the PoissonÕs ratio 0.33
conch shellÕs multiscale microarchitecture on impact resistance, Elongation at break, % 0.5–9.2
using drop weight tests and numerical simulations. They
noticed that the generation of pathways for crack deviation is
the main energy absorption mechanism, being suitable for
applications in helmets and armor, as suggested by the authors. printing speed of 50 mm/s and flat build orientation (layer
Traditionally, sandwich panels are made by conventional printing in x and y coordinates). Using the FDM method, PLA
manufacturing processes, in which the manufacture of core cell filaments of 1.75 mm in diameter are heated at 210 C and
geometry is limited. In addition, the 3D-printed panels lead to a extruded using a 0.4-mm-diameter nozzle. The printing bed is
fully integrated structure, which minimizes the issues related to preheated to 55 C. Table 1 shows the properties of PLA, a
the adhesiveness of the components. This work investigates the biodegradable thermoplastic polyester widely used in AM,
mechanical behavior of sandwich panels printed in 3D, made which can be obtained from renewable sources (Ref 15).
by the FDM method, designed with classic hexagonal cores The polymeric sandwich structures are printed with twenty-
(out-of-plane and in-plane oriented) and a novel type of core, two layers, including two layers for the top skin and two layers
namely S-shape corrugated cores. for the bottom skin, deposited with a Raster angle at 45/+45
with two shell perimeters per layer, to form the polymer skins,
which provide better response to the structure under bending
loads (Ref 1). The number of shell perimeters per layer
2. Experimental Investigation influences the mechanical properties of the 3D-printed material
(Ref 12), being kept constant for all conditions. The other
2.1 Sample Preparation layers are used to manufacture the cores, considering three cell
An experimental design is used to analyze the influence of geometries: hexagonal honeycomb oriented (i) out-of-plane, (ii)
the core shape on the mechanical properties of 3D-printed in-plane and S-shape corrugated, as shown in Fig. 2. The
polymeric sandwich structures. The materials are printed on a Solidworks 2018 and CuraEngine software are used to
BFB Rapman 3.1 3D printer, with a layer thickness of 0.2 mm,

5032—Volume 30(7) July 2021 Journal of Materials Engineering and Performance


Fig. 2 3D-printed sandwich structures: cellular dimensional configuration of the core structures (unit in mm): (a) out-of-plane hexagonal
honeycomb, (b) S-shape corrugated and (c) in-plane hexagonal honeycomb

design the 3D CAD models and slice the solid models, specimens. The average mass of the samples is quite similar for
respectively. the three conditions, being 7.59 ± 0.30 g for tensile samples,
5.46 ± 0.07 g for flexural samples and 3.04 ± 0.03 g for
2.2 Mechanical Characterization of the 3D-Printed Materials Charpy impact samples, leading to equivalent densities of 1.07
± 0.07 g cm 3, 1.19 ± 0.12 g cm 3 and 1.23 ± 0.05 g/cm3,
The 3D-printed polymeric sandwich structures are analyzed
respectively. The equivalent density is measured by the ratio
by tensile (in-plane), three-point bending and Charpy impact
between mass and volume of the panels obtained via CAD.
tests, to investigate the effect of the type of core geometry on
Analysis of variance (ANOVA) is used to verify whether the
the mechanical properties of the structures. The tests are
mean values of the mechanical properties are significantly
performed using a 100 kN Shimadzu AG-X plus test machine
different among the three core shapes.
and an XJJ-50 Series machine (Charpy impact tests). The
According to ASTM D638-14, tensile tests are performed
tensile load direction of out-of-plane comb panels is aligned to
using Type I specimens, with a test speed of 5 mm/min and a
the W-direction of the cell, as shown in Fig. 3. Five specimens
narrow section 57 mm long and 13 mm wide. A thin layer of
and two replicates are considered for each test, totaling ninety
epoxy is added as the tab material. The tensile modulus,

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strength and elongation at break are determined. Three-point The tensile results of 3D sandwich structures are described
bending tests are performed according to ASTM D790-15. in Table 3. Higher tensile modulus and strength are obtained for
Bending specimens, with dimensions of 127 mm in length and the panels made with hexagonal honeycomb cores oriented out-
12.7 mm in width, are tested at 2 mm/min using a 72-mm of-plane and with S-shape corrugated cores. The anisotropic
support span. Flexural modulus, strength and total displacement behavior caused by deposition of filaments in the core structure
are determined. Charpy impact tests are performed at a speed of affects the tensile properties of the structures, because the
3.8 m/s following the protocols of ASTM D6110-10 and ISO greater the number of core filaments aligned in the direction of
179-1, considering a sample dimension of 80 mm long and 10 the load, the greater the stiffness and strength of the structure.
mm wide. The absorbed energy is measured using a pendulum The elongation at break is similar for the three conditions.
impact with a normal stroke on 3D-printed layers (flatwise Figure 3 shows the typical stress–strain curves for the 3D-
normal impact). printed structures. In-plane oriented -comb core panels achieve
higher strain in the ribbon of the cell walls, generating stress
concentrations and lower values for tensile modulus and tensile
strength. The mechanical behavior of panels made with in-
3. Results and discussion plane -comb cores is defined by two stages, a linear behavior up
to about 0.01 strain, and a second one, characterized by a long
Table 2 shows the results of the analysis of variance deformation at low stress levels. Moreover, this core shape has
(ANOVA) for the mean values obtained from the tensile, a smaller number of filaments aligned to the load direction, in
flexural and Charpy impact tests. A P-value less than or equal contrast to S-shape corrugated cores, which have wider cell
to 0.05 indicates that the mean values are significantly different units composed of a dense portion of bonded filaments aligned
for the mechanical property, considering the ‘‘core shape’’ to the load direction. Bodaghi et al. (Ref 3) also investigated the
factor. The adjusted R2 values show satisfactory adjustments of mechanical properties of PLA panels with in-plane hexagonal
the data to the statistical model. The assumptions of homo- cells and found a strong effect of the cell shape and applied load
geneity of variances and normality of the residuals are checked direction on the structureÕs strength, both under tensile and
and validated. ANOVA shows that the mean values for compressive stresses.
mechanical properties are significantly different within a 95% Figure 4 shows the fracture surfaces of the specimens after
confidence interval. the tensile test. Inter-layer fracture (blue arrows in Fig. 4),
which occurs between two adjacent layers (the angle between
the failure and printing orientation are 0), and in-layer fracture
(red arrows in Fig. 4), when the layers break (the angle between
the failure and broken layer is different to 0) are reported,
which are the most common failure modes of 3D-printed
specimens (Ref 17). Additionally, the presence of voids
between the filaments is an intrinsic feature of the 3D-printed
structures and does not effectively contribute to the dissipation
of energy, which was also reported by Ayatollahi et al. (Ref 18),
which investigated tensile tests on PLA specimens under
different raster orientations. The increased load causes the
layers to break in different planes, followed by a brittle fracture
of the specimen. An adequate inter-layer bonding provides
greater stiffness and strength to the structure, which causes a
more concentrated damaged area. The specimens with inter-
layer fracture in the outer layers (panel polymeric facings)
present lower values for tensile modulus and strength, due to
less load transfer through the structure. According to Chacón
et al. (Ref 19), layers not aligned in the direction of tension
Fig. 3 Tensile stress–strain curves for the sandwich structures: show flaws in adhesion to each other, resulting from the melting
(HC_OUT_PL: Out-of-plane hexagonal honeycomb core; S_SHAPE: process by the FDM method, which decrease the tensile
S-shape corrugated core; HC_IN_PL: In-plane hexagonal honeycomb strength of the 3D-printed material.
core) Table 4 shows the mean flexural properties for sandwich
structures. The out-of-plane -comb core panel achieves the

Table 2 ANOVA for the mean mechanical properties


Tensile tests Flexural tests Charpy impact tests
Source variation ‘‘core shape’’ Tensile modulus Tensile strength Flexural modulus Flexural strength Energy absorbed

P-value £ 0.05 0.004 0.002 0.004 0.006 0.002


R2 (adj) 96.02% 97.68% 95.66% 94.25% 97.19%
Anderson–Darling test (P-Value ‡ 0.05) 0.440 0.809 0.248 0.856 0.943
Bartlett test (P-value ‡ 0.05) 0.539 0.361 0.848 0.439 0.235

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Table 3 Tensile properties of the 3D-printed sandwich structures
Core shape Tensile modulus, GPa Tensile strength, MPa Elongation at break, %

Out-of-plane hexagonal honeycomb 2.76 ± 0.24 43.23 ± 5.24 2.46 ± 0.33


S-shape corrugated 2.69 ± 0.23 47.38 ± 5.10 2.44 ± 0.34
In-plane hexagonal honeycomb 1.27 ± 0.10 16.06 ± 1.81 2.82 ± 0.35

Fig. 4 Failure mode of the 3D-printed sandwich structures after tensile tests

Table 4 Flexural properties of the 3D-printed sandwich structures


Core shape Flexural modulus, GPa Flexural strength, MPa Maximum displacement, mm

Out-of-plane hexagonal honeycomb 2.23 ± 0.21 46.32 ± 5.46 8.07 ± 0.60


S-shape corrugated 1.90 ± 0.12 43.44 ± 1.82 8.29 ± 0.67
In-plane hexagonal honeycomb 1.73 ± 0.10 29.81 ± 1.97 7.82 ± 1.00

highest flexural modulus and strength. On the other hand, the change in the color of the polymer, making it whiter (white
in-plane -comb core panel reaches the lowest values for flexural arrows in Fig. 6). The cracks are propagated vertically (cross-
properties, which is attributed to its strong anisotropic behavior section) from the bottom to the top skin. The occurrence of
of the core shape. The maximum displacements of the cracks without total rupture of the structure is obtained for all
specimens under bending loading are quite similar for the conditions. In-layer (red arrows in Fig. 6) and inter-layer (blue
three core shapes. Typical bending force–displacement curves arrows in Fig. 6) fractures are found in the specimens. The S-
are shown in Fig. 5. shape corrugated core panels present delamination, similar to
The failure modes of the specimens under bending loads are that found in the study by Somireddy and Czekanski (Ref 21),
shown in Fig. 6. It is well known that bending loads provide in- especially attributed to tensile stresses in the bottom skin. In
plane compressive stresses on the top skins (in-plane) and in the contrast, in-plane -comb core panels, which have a higher
central pin of the machine, tensile stresses in the bottom skin density of connections between the filaments, tend to propagate
and shear stresses in the neutral line (Ref 20). The presence of cracks in the direction of the applied load (the transverse
plastic strain caused by the tensile stresses induced below the direction of the specimen), leading to lower maximum failure
neutral line, especially in the bottom skin, is observed by the loads. In general, out-of-plane -comb core and S-shape

Journal of Materials Engineering and Performance Volume 30(7) July 2021—5035


corrugated core panels have a greater damage area, which compressive stresses are applied to the top surface of the
contributes to energy absorption, observed by the presence of material and tend to cause a global deflection of the structure,
cracks along the longitudinal direction of these specimens. generating shear stresses, leading to the rupture of the polymer
The energy absorbed during the Charpy impact tests is panel by in-layer fractures, as reported by Turner et al. (Ref 22).
shown in Fig. 7. Greater energy absorption is obtained by the A brittle fracture of the layers can be noticed (red arrows in
out-of-plane -comb core panels (0.58 ± 0.05 J) and S-shape Fig. 8), with transverse cracks along the direction of the
core panels (0.54 ± 0.03 J), followed by in-plane -comb core pendulum. According to Desu et al. (Ref 23), there is a
panels (0.44 ± 0.05 J). The results evidence a better transfer of transition state between elastic flexural and rupture (induced
energy through the longitudinal filament network, especially for between flexural and transverse shear) in the dynamic impact
out-of-plane -comb panels, which was previously found for the response of 3D-printed PLA plates. When the flexural stiffness
tensile and flexural properties. In low-velocity impact tests, exceeds a specific threshold value, energy dissipation is
dominated by fracture energy and low energy dissipation is
provided by elastic deflection. The sandwich structures made
with in-plane hexagonal honeycomb core show less energy

Fig. 5 Bending force–displacement curves for the sandwich Fig. 7 Energy absorbed of the 3D-printed sandwich structures:
structures: (HC_OUT_PL: Out-of-plane hexagonal honeycomb core; (HC_OUT_PL: Out-of-plane hexagonal honeycomb core; S_SHAPE:
S_SHAPE: S-shape corrugated core; HC_IN_PL: In-plane hexagonal S-shape corrugated core; HC_IN_PL: In-plane hexagonal honeycomb
honeycomb core) core)

Fig. 6 Failure mode of the 3D-printed sandwich structures after three-point bending tests

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Fig. 8 Failure mode of the 3D-printed sandwich structures after impact tests

absorption due to the less energy dissipation capacity along its The out-of-plane -comb core panels achieved a higher
longitudinal direction. Besides, the damaged area of the flexural modulus (29%) and flexural strength (55%) compared
specimen has a strong relationship with the values obtained to in-plane -comb core. Panels made with an S-shape corru-
for the energy absorbed in impact tests, due to the inertial gated core reached a lower flexural modulus (15%) than those
effects. with an out-of-plane hexagonal honeycomb core, although the
The results of the Charpy impact tests show that there is a results for flexural strength were similar.
significant effect of the core shape on energy absorption, as The impact energy absorbed by the sandwich structures was
shown in ANOVA (Table 2). However, for better energy similar for the out-of-plane -comb and S-shape corrugated core
absorption of these structures under low-velocity impact tests, it panels, in addition to having higher mean values (32 and 23%,
is recommended to use external skins with greater stiffness respectively) when compared to the in-plane -comb core panels.
along with films and adhesives that provide a better distribution The core structures fabricated by additive manufacturing
of loads between the 3D-printed cores and the skins (Ref 22, showed good mechanical behavior, enabling their application in
24). This can lead to higher sandwich structures that can offer secondary structural sandwich panels.
greater energy absorption capacity, greater buckling resistance
under static and dynamic loads. At the same time, it makes the
structures lighter, with low relative density and a good stiffness- Acknowledgments
to-weight ratio (Ref 25).
This study was partially funded by CAPES (Brazil) - Finance
Code 001. The authors would like to thank the Brazilian Research
Agencies, CNPq and FAPEMIG, and the Centre for Innovation and
4. Conclusions Technology in Composites (CITeC) from the Federal University of
São João del-Rei (UFSJ) and the Graduate Program in Mechanical
This study investigated the mechanical behavior of 3D- Engineering from the Federal University of Minas Gerais (UFMG),
printed polymeric sandwich panels under tensile, flexural and for the infrastructure and the support provided.
Charpy impact loadings. It was concluded that the use of
additive manufacturing is a promising and efficient way to
create polymeric structures with different core shapes, offering References
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5038—Volume 30(7) July 2021 Journal of Materials Engineering and Performance

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