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Thermophysical Properties of Normal Butane
from 135 to 700 K at Pressures to 70 MPa
William M. Haynes and Robert D. Goodwin
Thermophysical Properties Division

National Engineering Laboratory
National Bureau of Standards
Boulder, CO 80303
U.S. DEPARTMENT OF COMMERCE, Malcolm Baldrige, Secretary

NATIONAL BUREAU OF STANDARDS, Ernest Ambler, Director
Issued April 1982

Library of Congress Catalog Card Number: 82-600512
National Bureau of Standards Monograph 169

Nat. Bur. Slanii. (U.S.), Mongr. \W. 197 pages (Apr. 1982)
CODEN: NBSMA6
U.S. GOVERNMENT PRINTING OFFICE

WASHINGTON: 1982
Contents
Page
1. Introduction 1
2. Physical Properties and Their Formulation 2
2.1 Fixed-Point Values 2
2.2 Melting Line and Vapor Pressures 3
2.3 The Orthobaric Densities 4
2.4 The Virial Equation 5
2.5 The Equation of State 6
2.6 The Ideal Gas Functions 8
2.7 Thermal Loop Computations 8
2.8 The Heats of Vaporization 9
2.9 Saturated Liquid Enthalpies and Entropies 9
2.10 Dielectric Constants 10
3. Computational Methods 11
3.1 The Homogeneous Domain 11
3.2 The Saturated Liquid 12
3.3 The Compressed Liquid 13
3.4 Fugacity Coefficients 13
3.5 Simplified Computation 13
4. Tests and Conclusions 13
5. Tables of Physical and Thermodynamic Properties 14
5.1 Calculated P-p-T Isochores and Isotherms 14
5.2 The Joule-Thomson Inversion Locus 14
5.3 Thermophysical Properties of the Saturated Liquid ..... 15
5.4 Thermophysical Properties Along Selected Isobars 15
6. Acknowledgments 15
7. References 16
APPENDIX A. Symbols and Units 23
APPENDIX B. Conversion of Units 25
APPENDIX C. Fixed-Point Values for Normal Butane 26
APPENDIX D. Normal Butane Properties Reference Index 27
APPENDIX E. Computer Program 30
i i i
List of Figures
Page
Figure 1. Density-temperature diagram of normal butane 49
Figure 2. P-T locus of P-p-T data for normal butane 50
List of Tables
Table 1. Comparisons of vapor pressure data with eq (2) 51
Table 2. Comparisons of saturated liquid density data with eq (3) . . 54
Table 3. Comparisons of saturated vapor density data with eq (4) . . 57
Table 4. Comparisons of second virial coefficients with eq (5). . . . 59
Table 5. Behavior of coefficients of equation of state for

normal butane (eq (6)) 62
Table 6. Calculated P(p) critical isotherm of normal butane 63
Table 7. Comparisons of experimental P-p-T data of normal butane

with eq (6) 64
Table 8. Comparisons of data for ideal gas functions with eq (7). . . 85

Table 9. Interpolated ideal gas functions from eq (7) 86
Table 10. Comparisons of heat of vaporization data with eq (9) , . . . 87

Table 11. Enthalpies of saturated liquid normal butane from eq (10) . 89
Table 12. Entropies and specific heats of saturated liquid normal

butane from eq ( 1 1 ) 90
Table 13. Comparisons of dielectric constant data with eq (12) .... 91
Table 14. Comparisons with saturated liquid specific heats 95
Table 15. Comparisons with C and C data 96

v p
Table 16. Comparisons with velocity of sound data 97
Table 17. Calculated P(T) isochores of normal butane 98

Table 18. Calculated P(p) isotherms of normal butane 113
Table 19. The Joule-Thomson inversion locus for normal butane .... 133
Table 20. Thermophysical properties of saturated liquid normal
butane 134
Table 21, Thermophysical properties of normal butane along isobars . . 136
i V
THERMOPHYSICAL PROPERTIES OF NORMAL BUTANE FROM 135 TO 700 K AT
PRESSURES TO 70 MPa
Thermophysical Properties Division
National Engineering Laboratory
National Bureau of Standards
Boulder, Colorado 80303
Using a modified version of the nonanalytic equation of state,

thermophysical properties of normal butane are derived from physical
properties data and are tabulated at integral temperatures from 135 to
700 K along isobars at pressures to 70 MPa. These isobar tables, along
with a table for the saturated liquid, give values for densities,
compressibility factors, internal energies, enthalpies, entropies, heat
capacities, fugacities, sound velocities, dielectric constants, and
isochore and isotherm derivatives. Equations, whose coefficients are
determined from a least squares fit to selected experimental data, are
also presented for vapor pressures, orthobaric liquid and vapor
densities, ideal gas properties, second virial coefficients, dielectric
constants, heats of vaporization, melting pressures, and orthobaric
liquid specific heats, enthalpies, and entropies. Comparisons between
experimental and calculated values for all properties considered here
are reported in detail.
Key words: Densities; dielectric constants; enthalpies; entropies;

equation of state; fugacities; internal energies; isobars; isochores;
isotherms; Joule-Thomson inversion; latent heats of vaporization; melting
line; normal butane; orthobaric densities; specific heats; vapor
pressures; velocities of sound.
1 . Introduction
The present work is a revision and extension of a previous provisional
report [28] from this laboratory. Since that report new compressibility
data [35] for normal butane at low temperatures have become available and are
incorporated in the work reported here. These new data cover a range from 140 to
300 K at pressures to 35 MPa. As a result of new dielectric constant measure-
ments [35,38] on normal butane, the present work also includes a correlation of
dielectric constant data. The nonanalytic equation of state used here, which is
modified from earlier versions [26-29], is also currently being employed in

correlations for propane [30] and isobutane [31].
1
other correlations on normal butane have been reported by Hanson [34],
Prengle, et al . [57], Canjar, et al. [9], Das and Kuloor [?C], and Das,
et al . [21]. Many new properties data, especially at low temperatures, have

appeared since these correlations were developed.
SI units are used throughout this report in tables and equations. Pressures
3
are given in MPa, densities in kg/m , and temperatures in K. For thermal
properties, the mol is used for amounts of substance. However, all computations
in computer programs (Appendix E) for the present work have been conducted in
units of bar for pressure and mol/L for density.
Symbols and units used in this report and in computations appear in
Appendix A; conversion factors for units are given in Appendix B. Fixed-point
values of normal butane used in this work are reported in Appendix C. A
collection of references for the major physical properties of normal butane,

along with ranges of data, is presented in Appendix D. Appendix E consists of
computer programs used for the calculation of thermophysical properties of normal
butane. In figure 1 is presented the density-temperature diagram for normal
butane.
2. Physical Properties and Their Formulation

In this section, first the fixed-point values selected in present work are
presented and their origins are briefly discussed. As the present equation of
state originates on a given liquid-vapor coexistence boundary, the P(T) melting

line, the vapor pressures, and the orthobaric densities are next formulated.
Then the truncated virial equation of state is given because it is used to derive
some needed data. The equation of state description is followed by formulation
of some thermal properties needed for the final computations of a thermodynamic
network. All symbols used in the equations are defined in Appendix A.
2.1 Fixed-Point Values

These values are listed in Appendix C.
(a) The Triple Point. The temperature (T^ = 134.86 K) is adopted from
Das, et al . [21], while the pressure is determined from the vapor pressure
equation (eq (2)). The liquid density is based on consistency with data in
eq (3). Equation (4) for saturated vapor densities is used for calculating the
vapor density.
2
(b) The Boiling Point. The temperature {J^ = 272.638 K) is froin vapor
pressure eq (2) at a pressure of 1 atm = 0.101325 MPa. Liquid and vapor
densities are from eqs (3) and (4).
(c) The Critical Point. The temperature (T^ = 425.16 K) is adopted from
Das, et al. [21] and is in agreement within acceptable limits with the values of
Beattie, et al . [2] and Kay [44]. The density and pressure (p^ = 227.85 kg/n?
(3.92 mol/L) and P^ = 3.7960 MPa) are adopted on the basis of fitting orthobaric
densities, vapor pressures, and P-p-T data and then examining the behavior of the
calculated critical isotherm. The selected values for density and pressure are
substantiated by those obtained experimentally from the data of Kay [44],
Beattie, et al . [2] and by those selected in the correlation of Das,
et al. [21].
2.2 Melting Line and Vapor Pressures

(a) The Melting Line. Experimental pressures from about two to ten
kilobars were reported by Reeves, et al . [59] as constants for the Simon eq (1).
In present work using the triple point temperature and pressure from Appendix C,
the relation,
% = Pt ^ Po [(T/T^)^ - 1] . (1)
is obtained, where P^ = 6.7358 x lO"'' MPa, T^ = 134.86 K, P^ = 363.4 MPa, and

c = 2.21.
(b) The Vapor Pressures. Data used for adjusting eq (2) appear in the
first part of table 1. Other data, weighted zero, appear in the continuation of
the table. Values at ID = 40 have been derived via thermal loops, as described
by Goodwin [27], by use of the saturated liquid specific heat data of Aston,
et al . [1] from the triple- to the normal boiling-point; the heat of

vaporization of Aston, et al . [1] at the normal boiling point; the ideal gas
thermofunctions formulated in section 2.6; the virial equation formulated in
section 2.4; and, for the minor contribution of V*dP to AH on the saturated
liquid path, the preliminary vapor pressure and saturated liquid densities
equations were also used. This procedure also has been described by Yarbrough
and Tsai [75].
The argument for eq (2) is T^ e T/T^; then, vapor pressures (P^) in MPa
are given by the relation.
3
£n(P^-10) = a/T^ + b + c-T^ + d-T^ + e-T^ + f-(l - T^)^ , (2)
where e = 1.85 and, from least squares analysis,
a = - 9.5092 4729 d = 4.8614 7936

b = 5.2015 3488 e = - 7.5581 8629
c = 10.6409 5231 f = 18.7288 6023
Exponent e was selected for a best fit of P-p-T data under the constraint that,
at the critical point, the slope of the vapor-pressure equation be equal to the
slope of the critical isochore from the equation of state, dP^/dT = (3P/3T)p .
The fit of present vapor pressure data is relatively insensitive to values o? e

in the range, 1.1 <. e <. 1.95, but the critical point slope is dependent on the
value of £. The value of e = 1.85 is consistent with scaling law equations* The
present slope at the critical point is dP^/dT = 0.064272 MPa/K»
2.3 The Orthobaric Densities

(a) Saturated Liquid Densities. Data in table 2 have been selected for
consistency. Data weighted zero, which appear in the continuation of the table,
are shown for comparison. If the variable for eq (3) is defined by
x(T) E (T^ - T)/(T^ - T^) ,
then the orthobaric liquid densities, p^, are described by
(p^ - P^)/(p^ - P^) = X + (x^ - x) -[a + b-x + c-x^] , (3)
where e = 0.35, and, from least squares analysis,
a = 0.7943 88335 c = -0.0858 29197

b = -0.0010 89476
(b) Saturated Vapor Densities. The following new type of formulation for
saturated vapor densities has been developed for consistency with the equation of
state (eq (5)) to yield a compressibility factor approaching unity in the limit
of low densities, as described earlier [26,29]. Data in table 3 used in the fit
have been selected for internal consistency. Values at ID = 40 are derived from
the vapor-pressure and virial equations. Other data, weighted zero, appear in
the continuation of table 3. The compressibility factor for saturated vapor is
formulated by use of the vapor-pressure equation, such that Z (T) approaches
4
unity as Pq-*0, (hence T^(p) -» 0). Let = (Z^ - 1), where is value of
the compressibility factor at the critical point, and define the arguments
n(T) = P^(T)/P^ , E T/T^ , u(T) e (1 - T^) .
The saturated vapor densities, e P^/(Z^«R*T), then are given by
Z = 1 + A^-n-T^^-fd) , (4)
where
f(T) E 1 + a'u^ + b'u + c*exp[n*(l - 1/u)] ,
e = 0.35, n = 2.3, and, from least squares analysis, .

*
a = -0.8665 77289 c = 4.4986 58942

b = 1 .1203 97967
The next-to-last column in table 3 gives the experimental residuals,
F(Z) E (Z^^p - 1)-t2/[A„.„] ,
used to develop a functional form for f(T).
2.4 The Virial Equation

For the truncated virial equation,
Pv/RT = 1 + B^(T).p^ + . . . , (5a)
the second virial coefficient, B^(T), is dimensionl ess through the use of the
reduced variables, e p/p^ and T^ e T/T^. The following relation,
B^(T) = + B2/T^ + B3/T^ . (5b)
is used to fit the second virial data given in the first part of table 4.
Excluded data, weighted zero, appear at the end of table 4. From least squares
analysis, the following coefficients,
B-| = 0.3703 0532 B^ = -0.6660 5953

B^ = -0.9668 8512
have been determined. The second virial s have been used to synthesize P-p-T
data, to calculate saturated vapor densities via the vapor pressure equation, and
to make thermal loop computations.
5
2.5 The Equation of State
Figure 2 shows the P-T regions covered by P-p-T data of Beattie, et al . [2],
Kay [44], Olds, et al . [51], and Haynes [35]. The data of Sage, et al . [64] are
excluded from this figure and are not used in the fit, since they are superseded
by data of Olds, et al . [51]. These P-p-T data for normal butane are also
summarized in Appendix D and table 7. Data from the virial equation along a low
density isochore are included in the fit. Equal weightings of unity have been
given to the data sets [2,35,44,51] used in fit.
The nonanalytic equation of state used here originates on the liquid vapor
coexistence boundary, as described in detail by Goodwin [26,29]. Twelve least
squares coefficients appear in the vapor pressure and orthobaric density
equations. In the equation of state there are four nonlinear parameters and only
three least squares coefficients, as described below. The equation has been
modified from earlier forms [26-29]. For any density (isochore) the coexistence
temperature, T^(p)» is obtained by iteration from eqs (3) and (4) for the
orthobaric densities. The vapor pressure, P^[T^(p)], thus is a function of
density, and the equation of state has the form,
P - P^(p) = p^-R*-[T - T^(p)] + p^R*T^-F(p.T) , (6)
where
•
F(p,T) E B(p).$(p,T) + C(p)-f(p,T) . (6a)
The density, p^ =
p/p^» is reduced at the critical point, while the constant
R* is defined by R* e (0.0083145) 'p^, MPa/K.
The temperature-dependent functions in (6a) are defined as follows.
$(p,T) = T^.exp[b-(1 - T^/T)] - (T^)^ (6b)

,
...
where b e (1 - 3) + (1 - 8)^^^ T^ e T/T^, and (T^) e T^(p)/T^.
y(p.T) = ^(P.T)/I'^(p) - 1 , (6c)
where i|'^(p) is obtained from i|j(p,T) merely by replacing T with T^(p)5 and
^(P.T) = 1 - (03 - a3'^/n)/(l - 1/n) . (6d)
6
. ,
The value for 3 was found by trial, while the value for n was determined from
critical region behavior.
a)(p.T) = [1 - 0(p)/T] , (6e)
where g(p) is a locus of temperatures inside the coexistence envelope defined by
e(p) = T^(p) •exp[-a.f(p)] ,
and (6f)
Hp) = |P^ - ll^/((pJ - 1)^ .
^
r
(Px) = reduced density at the liquid triple point. The parameter

^t^^c
r
a is found by trial
The density-dependent coefficients in (6a) are
B(p) E + B2-P^ (6g)
and
C(p) = C^-(p^ - l).(p^ - CQ)-exp[-Y.p^] , (6h)
where Cq and y aiê to be found by trial.
Parameters and coefficients of eq (6) for normal butane are
a = 1 , 3 = 0.70, Y = 0.14, n = 1 .1
B^ = 0.4565 5869 162 = 2.2

B^ = 0.1714 3942 370 = -0.2803 6114 629
Table 5 gives behavior of coefficients B(p), C(p) as a function of density

and table 6 gives behavior along the critical isotherm. (In table 6, the symbol,
Ppr f» is defined as the density reduced by the triple point density.) These
, u
tables show that the equation is smooth and well-behaved. Table 7 summarizes
experimental compressibility data and presents deviations of experimental
densities and pressures from values calculated from the equation of state.
Although the data of Sage, et al . [64] are not used in the fit, comparisons with
these data are presented in table 7. These data show systematic differences of
approximately 1 percent when compared in regions of overlap with the results of
Kay [44], Olds, et al . [51], and Haynes [35].
For normal butane, there are four comprehensive sets of liquid and gaseous
compressibility data covering a temperature range from 140 to 600 K at pressures
7
as high as 70 MPa that are internally consistent within a few tenths percent in
regions of overlap. Using these data sets, the present equation yields a
slightly better fit than that obtained from a slightly different equation used in
the provisional work [28] for which the low temperature data were not available.
In the earlier work, the single phase results at temperatures less than room
temperature were obtained by extrapolation. Thus, a significant improvement has
been made in the P-p-T behavior of normal butane at low temperatures.
It should be noted that the functional form of the equation of state used
here for normal butane has also been used in current work for propane [30] and
isobutane [31]. Identical nonlinear parameters except for insignificant
differences in y. have been obtained for all three fluids in fitting this
equation to available P-p-T data.
2.6 The Ideal Gas Functions

A formulation of the spectroscopic specific heats, C^(T), of Chen,
et al . [12] has been developed. Using x^ = T/lOO,
5 , .
C°/R - 4 = exp(-£/x^). £ A. .x^-"" , (7)
where R = 8.31434 J/(mol»K) and
e = 2.37 A3 = 257.279067
A^ = 41.110973 A^ = -170.730596
A2 = -139.304011 Ag = 40.032171
Table 8 shows the fit of data used. In this table,

'
the values for (H°-H°)
0' '
0
and for S are obtained by numerical integration, starting at T = 300 K.
Table 9 gives interpolated values at integral temperatures.
2.7 Thermal Loop Computations

At temperatures from the triple- to the normal boiling-point, new data have
been derived for vapor pressures, saturated vapor densities, and for heats of
vaporization by thermal loop computations for AH and for AS of saturated vapor
and saturated liquid. This procedure described by Goodwin [29], and more
generally by Yarbrough and Tsai [75] uses virial eq (5a), ideal gas functions
eq (7), the heat of vaporization of Aston, et al . [1] at the normal boiling
point, and the following new formulation of the specific heats of Aston,
8
et al . [1] for the saturated liquid from the triple- to the normal boiling-point.
Define Xq(T)
k^{T) =
- T/lOO; then
t^ the saturated liquid specific heats, C^(T) , in
J/(mol«K), are given by
C (T)
'
= a/x
0
+ b + c-x
0
+ d»x ^
0' . (8)
^ '
where, from least squares analysis, the coefficients, in units of J/(mol«K), are
as follov/s:
a = -104.7430 c = -97.2492
b = 284.0264 d = 20.6032
Results for the vapor pressures appear in table 1 at ID = 80, and for the
heats of vaporization in table 10 at ID = 80. Saturated vapor densities from the

thermal loop computations are replaced in table 3 at ID = 40 by derived data from
the fitted vapor-pressure eq (2) and the virial eq (5a).
2.8 The Heats of Vaporization

Table 10 shows the fit of selected data. Those at ID = 80 are derived via
thermal loops (section 2.7). Those at ID = 41 are from the Clapeyron equation.
The formulation of these heat of vaporization (Q^gp) "âta in kJ/mol uses argument
x(T) = (T^ - T)/(T^ - T^);
= A^-x + (x"^ - x)-[A2 + A3-X + A^-x^] , (9)
where
e = 0.34 A3 = 12.710873
A^ = 28.789248 A^ = -16.533537
A2 = 24.163103
The coefficients have units of kJ/mol . The uncertainty of at least one percent
in
Qy^p at the higher temperatures will affect compressed liquid thermofunctions
in this region, since
Q^^p is used to compute across the "dome."
2.9 Saturated Liquid Enthalpies and Entropies

Data for saturated liquid enthalpies and entropies have been derived at
temperatures from the triple- to the critical-point by use of the ideal gas
functions, the equation of state, and the formulated heats of vaporization. The
enthalpies then have been formulated, as shown in table 11. Define the
variabl e.
9
X = (T^ - T)/(T^ - T^) ;
then the enthalpies, H(j(T), are described in J/mol by
i-1
(H^ - H^)/(H^ H^) = X + (x^- - x) A.*x (10)
1
i =l
where e = 0.29, = 0.001 J/mol, = 45399.788 J/mol, and
0.1929 77338 kr = 2.8727 89244

0.3998 98449 Ag = -4.0526 10155
-0.0549 93612 A^ = 2.6963 77850
-1.0205 68625 A„ = -0.6834 38899
The formulation of saturated liquid entropies in J/(mol*l<) is shown in table 12,
Let
Lei X E (T^ - T)/(T^ - T^) ; then the entropies, S^(T), are given in J/(mol»l<)
by
i-1
- - = x + (x^ - X) A.'x (11)
(â V/(^t i = l
where e 0.23, = 133.54372 J/(mol»K) = 297.64652 J/(mol«K), and
A, = 0.08883 44435 A4 = -0.95683 28496

= -0.34703 04947 A. = 0.95799 92545
5
= 0.20937 24392 A. = -0.65346 07056
Specific heats along the saturated liquid path follow from the relation,
C^(T) = T*dS^/dT, and are given in the last column of table 12. All of the
above saturated liquid formulations for H^(T), S^(T), and C^(T) are used to
compute thermodynamic properties for compressed liquid states at T < T^.
2.10 Dielectric Constants

Dielectric constants, e, for the saturated vapor of normal butane are
estimated from the refractive indices, n, of Sliwinski [67] via e = n'. (These
low density data are in a region for which dispersion effects should be minimal.)
Haynes [35,38] recently has measured e for the saturated liquid at temperatures
from 135-300 K and for the compressed liquid at presures to 35 MPa along
isotherms up to 300 K. These data and their formulation via the
Clausius-Mossotti function.
10
CMF E [(£ - l)/(e + 2)]/p , (12a)
are presented in table 13. The following formulation has been used to fit the
data in table 13 and to calculate e along isobars (table 21) at temperatures
extrapolated up to 450 K, and at pressures up to 70 MPa. Define the variables,
T E T/T and p = p/p.; then, with P in units of MPa, the CI ausi us-Mossotti
3
function, in units of cm /mol , is given by
CMF = + A2-p^ + A3-p^ + A^/T^ + A^-P/IO (12b)
where
A^ = 20.654382 A^ = -0.0392 1649

A, = 0.2512 9317 A. = -0.0116 4552
2 5
A3 = -0.0972 3048
3
The least squares coefficients have units of cm /mol. Data at high pressures
have a diminished v/eighting as seen in table 13. The rms relative deviation for
152 points is 0.083 percent for the CMF and 0.017 percent for the dielectric
constant.
Comparisons with dielectric constant data for liquid normal butane not used
in the fit to eq (12) are not presented in table 13. The dielectric constants
of Thompson and Miller [70] and Luo and Miller [47] at temperatures between 220
and 289 K agree within 0.1 percent with values calculated from eq (12).
3. Computational Methods
The numerical values For E and H in this report are based on the assigned
value, E = 0 at the liquid triple-point, obtained by use of the arbitrary value,

E° = 22644.306 J/mol . Specific heats of Aston, et al . [1] could be integrated
to give the solid at T = 0 as reference state.
3.1 The Homogeneous Domain

The homogeneous domain of figure 1 includes all regions which can be
attained along isotherms starting at zero density without crossing the
vapor-liquid "dome," and without passing very close to the critical point at
T > Tc-
Computations start with ideal gas thermodynamic functions at zero density,
and then continue by integrating numerically along isotherms by use of the
equation of state in the following relations.
11
AE = / [P - T-(9P/aT)]-dp/p^ , (13)
AC^ = - T .
/ (9^P/9T^).dp/p^ , (14)
AS = R'iln[P°/(pRT)] + [R - 0P/8T)/p] -dp/p . (15)

J*
Equation (15) is for use with initial entropies in hypothetical ideal gas states
at P° = 1 atm (0.101325 MPa). For all other initial states,
AS = - / (9P/3T)'dp/p^ . (15a)
In each (p,T) state, reached by above integrations, the following are computed,
H = E + P»v , (16)
Cp = + T.(9P/9T)2/(9P/9p)/p^ , (17)
and
= Cp.(9P/9p)/Cy . (18)
3,2 The Saturated Liquid

At temperatures from the triple-point to the critical-point, thermof unctions
for the saturated vapor are obtained via eqs (13) through (16). Then eq (9) for
the heat of vaporization, Qygp» is used to compute
AH = - Q , AS = AH/T , (19)
such that the free energy of vaporization, AG = AH - T»AS, is zero (see

section 2.9). Having obtained H and S for the saturated liquid, E = H - P»v is
computed.
The single-phase specific heat, Cy(p,T), at the saturated liquid boundary,
is obtained from eq (11) using C^(T) = T«dS^/dT and the thermodynamic relation,
Cy(p,T) = C^(T) + T.(9P/9T).(dp^/dT)/p^ , (20)
where p, is density of the saturated liquid. Values for C (p,T) and W(p,T) on
X/
P
this boundary follow from eqs (17) and (18). For liquid at the normal boiling
point, the following values have been obtained.
12
, . .
= 272.638 K, = 16770.1 J/mol ,
E,^ = 16760.3 J/mol , = 218.485 J/(mol -K)
3.3 The Compressed Liquid

Starting vvith above values for E, S, and on the saturated liquid
boundary, eqs (13), (14), and (15a) are used to integrate along isotherms, and
then H, C^, and W are obtained via eqs (16), (17), and (18).
3.4 Fugacity Coefficients

The fugacity coefficients in table 21 were computed along isotherms relative
to properties in hypothetical ideal gas states at a pressure, P° = 1 atm
(0.101325 MPa)
(f/P) = (P°/P)-exp [AG/RT] . (21)
For any (P,T) point, the isothermal free energy change is
AG = (H - E°) - - T.(S - S°) , (22)
in which the arbitrary value of E° was added to tabulated values of H(P,T)
such that E(P,T) = 0 for liquid at the triple point.
3.5 Simplified Computation

Given the subroutines of Appendix E, it is necessary first to call
SUBROUTINE PVTDATA, to place constants in common statements. To obtain the
density in mol/L at a given T,K and P,bar, it is necessary merely to write the
instruction DEM = FINDENF(T,P) for single-phase domains. Coexisting densities
are given by the functions DENGASF(T) and/or DENLIQF(T), and the vapor pressure
in bar by PSATF(T)
For thermodynamic properties, the subroutine SIMPLE here is an example of
how to use the general subroutine THERMO (see Appendix E).
4. Tests and Conclusions

In the provisional report [28], comparisons were made between enthalpy
- differences from that work and those from the correlation of Das, et al . [21].
Since the results from the present work are approximately equivalent to those
from the earlier report at temperatures above 300 K, these comparisons, along
with some consistency tests, are omitted in this report.
13
It has been a routine procedure to validate equation of state computations
by comparing calculated and experimental specific heats and sound velocities.

For normal butane, there are only a few experimental specific heats and sound
velocities available, most of which are unreliable. Comparisons with available
data are presented in tables 14-16.
In the present work, an isochoric, nonanalytic equation of state has been
developed, based on thermophysical properties data, to compute thermodynamic
properties of normal butane. This equation originates on the liquid-vapor
coexistence boundary; approximately twelve constants are used in the vapor
pressure and orthobaric density equations. The equation, as used here, has only
three least squares coefficients and describes a P(p,T) surface free of
irregularities consistent with the known behavior of specific heats, especially
in the critical region. Four nonlinear parameters appear in the equation.
For normal butane, the equation of state has been developed from
comprehensive and consistent sets of vapor pressure, orthobaric vapor and liquid
density, and compressibility data. In general, the experimental data for these
properties over the range of this work are in relatively good shape except for
low temperature vapor pressures and vapor densities for which values have been
determined from thermal loop computations. However, as mentioned earlier,
accurate specific heat and sound velocity data are needed for comparisons with
computations from the equation of state.
5. Tables of Physical and Thermodynamic Properties
5.1 Calculated P-p-T Isochores and Isotherms

Tables 17 and 18 give a selection of isochores and isotherms computed by
equation of state (6). These are essential to examine behavior of the P(p,T)
surface. They are a useful supplement to the isobars of table 21 for
interpolating P-p-T values and their derivatives.
The tables of isochores show that the isochore curvatures are qualitatively
consistent with a maximum in the specific heat Cy(p,T) at the critical point.
The isotherm tables show that 3P/3p is nonnegative and that pressure increases
monotonical ly with density along isotherms.
5.2 The Joule-Thomson Inversion Locus

Table 19 gives the P-p-T locus of the JT inversion, (3T/9P)|^ = 0,
obtained from equation of state (5) under the condition, T»(3P/3T) = p'(3P/9p).
14
This table has been computed to temperatures well above those of P-p-T data, to
show approach to a maximum in P-T coordinates.
5.3 Thermophysi cal Properties of the Saturated Liquid

Table 20 gives physical and thermodynamic properties of the saturated liquid
computed by methods of section 3. (Properties of the saturated vapor can be
obtained from Table 21 from values given at the coexistence boundary for each
isobar.)
5.4 Thermophysical Properties Along Selected Isobars

Table 21 gives physical and thermodynamic properties on isobars, computed by
methods of section 3. These tables are extrapolated above the maximum
temperature and pressure of P-p-T data used for adjusting the equation of state.
Small discontinuities may be detected at T^ = 425.16 K along isobars at
P > P^ = 3.796 MPa due to a change in the paths of computation (section 3).
The first line of each table refers to freezing liquid on the P(T) melting
line. Each table at P < P contains a blank line for the transition from
c
saturated liquid to vapor, as seen by the abrupt decrease of density. Dielectric
constants are extrapolated above maximum experimental temperatures and pressures
(see section 2.10 and table 13), but have not been extrapolated above 450 K.
6. Acknov;l edgments
Many staff members of the Thermophysical Properties Division of the National

Bureau of Standards (NBS) have contributed valuable suggestions, references, and
documents. Robert D. McCarty contributed the essential least-squares program,
providing for constraints. James F. Ely indicated the new numerical integration
procedure, and the simple method for obtaining fugacities. Neil A. Olien and the
Cryogenic Data Center have been of invaluable assistance in supplying references

and in obtaining documents. Special thanks go to Karen A. Bowie for her
diligence and expertise in the preparation of the manuscript and tables for
publication. Finally, we express grateful appreciation for support of this work
by the Gas Research Institute.
15
. . . . .
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19
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22
APPENDIX A. Symbols and Units
Subscripts c and t refer to critical and liquid triple points.
Subscripts g and £ refer to saturated vapor and liquid.

Subscript a refers to liquid-vapor coexistence (usually the liquid).
Subscript r refers to reduced parameter.
Subscript o refers to reference state property.
Subscript m refers to melting line.

Subscript b refers to normal boiling point.
Superscript o refers to ideal gas state property,
expt refers to experimental value,

calc refers to calculated value.
(aP/3T)p isochore derivative, MPa/l(
(3P/3p)j isotherm derivative, MPa»m^/kg
(9^P/8T^)^ isochore curvature, MPa/K^
a,3,Y,ri nonlinear parameters in the equation of state
a,b,c,d,e,f coefficients defined in various equations
Aq
^c
~ ^ saturated vapor density equation
Aj coefficients defined in various equations
b (1 - B) + (1 - 3)^''^ in equation of state
B(p),C(p) density-dependent coefficients in the equation of state

B(T),C(T) second and third virial coefficients
Bp(T),Cp(T) reduced second and third virial coefficients
c exponent in Simon equation
Cy(p,T) molal heat capacity at constant volume, J/(mol»l()
Cp(p,T) molal heat capacity at constant pressure, J/(mol'K)
C^(T) molal heat capacity for saturated liquid, J/(mol»K)
CMF CI ausius-Mossotti function, cm-^/mol
E(p,T) the internal energy, J/mol
E° 22,644.306 J/mol (arbitrary)
e exponent in various equations
e dielectric constant
f/P fugacity/pressure ratio
f(p) used in definition of e(p)
f(T) defined in saturated vapor density equation
F(p,T) defined in the equation of state
F(Z) defined in the saturated vapor density equation
G(p,T) Gibbs free energy, J/mol
H° enthalpy for ideal gas state at T = 0
23
APPENDIX A. (Continued)
H(p,T) the enthalpy, J/mol
J the jou1 e, 1 N 'in
JT Joule-Thomson
L the liter, 10"^ n?
mo] 58.1243 grams of normal butane (C^'^ = 12 scale)
'jL)(p,T) defined in the equation of state

P ' pressure, MPa
melting pressure, MPa
P^(T) the vapor pressure, MPa
P^(p) -
P^[T^(p)], vapor pressure as a function of density
n(T) Pa(T)/''c
$(p,T) function in the equation of state
^{PiJ) function in the equation of state
^^vap' ^^^^ vaporization, J/mol

Qygp
the gas constant, 8.3145 J/(mol*K), 0.0083145 MPa'L/(mol 'K)
^
r(^)
R* 0. 00831 45 'Pc, MPa/K
p density, kg/m-^
p^ p/Pq, density reduced at the critical point
Pp ^ P/Pf density reduced at the triple point
S(p,T) the entropy, J/(mol'K)

T temperature, K
Tq constant
T/Tq, temperature reduced at the critical point
T^(p) liquid-vapor coexistence temperature, K
(T(j) T^(p)/T^, reduced temperature at coexistence for the equation

r
of state
e(p) defined locus of temperatures

u(T) defined in various equations
V 1/p, molar volume, m^/kg
W(p,T) the velocity of sound, m/s
x(T) (T^ - T)/(Tc - T^)
Xo(T) T/lOO
Z compressibility factor
The gas constant is increased slightly in value from earlier work in view
of the recent report of Rowlinson and Tildesley [60].
24
APPENDIX B. Conversion of Units
In the following table the molecular weight of normal butane is given by
mol . wt. 58.1243 g/mol . Also, 1 cal 1 cal (thermocheinical ) = 4.184 J
th
and 1 BTU = 1 BTU (International Table) = 1055.056 J.
IT
To convert from To Multiply by
Pressure, MPa bar 10.
atm 9.85923
kg/cm^ 10.1972
Ib/in- 145.038
Volume, m"^ liter (L) 1000.
ft^ 35.3147
Density, kg/m"^ g/cm^ 0.001
mol/L 1 ./(mol . wt .)
Ib/ft^ 0.062428
Molar energy, J/mol MPa»m^/kg 0.001/(mol . wt.)
bar»L/mol 0.01
calj-u/mol
'th
0.239006
BTUij/lb 0.429923/(mol . >/rt.)
Molar entropy, J/(mol«K) BTUij/(lb-°F) 0.238846/(mol . wt.)
25
APPENDIX C. Fixed-Point Values for Normal Butane
Critical Point
?^ = 3.7960 MPa
= 227.85 kg/m3 (3.92 mol/L)
= 425 .16 K
Normal Boiling Point

P = 0.101325 MPa
T = 272.638 K
Py = 2.709 kg/m^ (0.04661 mol/L)
p^ = 501 .09 kg/in^ (10.341 mol/L)
Triple Point
P^ = 6.7358 X lO"'' MPa
= 134.86 K
Py = 3.4915 X 10"^ kg/m^ (6.0071 x 10"^ mol/L)
p^ = 735.27 kg/m3 (12.650 mol/L)
26
APPENDIX D. Normal Butane Properties Reference Index
Melting Line Date Pressure Range, MPa
Reeves [59] 1964 200 - 1000
Vapor Pressures Date Temperature Range, K
Seibert [66] 1915 303 - 403
Dana [19] 1926 255 - 331
Delaplace [22] 1937 135 - 151
Sage [64] 1937 294 - 394
Beattie [2] 1939 348 - 423
Aston [1] 1940 195 - 273
Kay [44] 1940 325 - Tc

Wackher [74] 1945 205 - 279
Tickner [71] 1951 136 - 196
Connolly [15] 1962 344 - Tc

Hi rata [39] 1966 333 - 401
Carruth [11] 1973 135 - 213
Thermal loops (This report) 1982
Saturated Liquid Densities Date Temperature Range, K
Dana [19] 1926 273 - 329
Coffin [13] 1928 239 - 306
Van der Vet [73] 1937 283 - 323
Sage [64] 1937 294 - 394
Kay [44] 1940 325 - T^

Benoliel [6] 1941 213 - 293
Carney [10] 1942 228 - 333
NGAA [69] 1942 227 - 333
Olds [51] 1944 311 - 411
Foehr [24] 1949 293
Connolly [14] 1956 293 - 298
Sliwinski [67] 1969 283 - 368
Kahre [42] 1973 289 - 328
McClune [49] 1976 143 - 173
Haynes [36,37] 1976 135 - 300
Orrit [53] 1978 135 - 275
27
APPENDIX D. (Conti nued)
Saturated Vapor Densities Date Temperature Range, K
Dana [19] 1926 281 - 321
Sage [64] 1937 294 - 394

Kay [44] 1940 325 - Tr
Olds [51] 1944 311 - 411
Sliwinski [67] 1969 283 - 368
Virial/vapor pressure equations (This 1982 135 - 270

report)
Virial Coefficients Date Temperature Range, K
Sage [64] 1937 311 - 394

Beattie [3] 1939 423 - 573
Kay [44] 1940 311 - 589

Beattie [4] 1942 423 - 573
Olds [51] 1944 311 - 511
Kretshmer [45] 1951 303

Gunn [33] 1958 344 - 511
Connolly [15] 1962 344 - 444

McGlashan [50] 1962 296 - 413
Tripp [72] 1962 283 - 323
Kapallo [43] 1963 244 - 321
Bottomley [8] 1964 273 - 426
Jones [41] 1967 368 - 498
St rein [68] 1971 296 - 498
Bottomlev [7] 1977 316 - 580
Compressibility Data Date Range of T, K Range of P, MPa

Sage [64] 1937 294 - 394 0.1 - 20.7
Beattie [3] 1939 423 - 573 1.5 - 36.3
Kay [44] 1940 311 - 589 0.2 - 8.3
Olds [51] 1944 311 - 511 0.07 - 68.9
Haynes [35] 1981 140 - 300 1.7 - 36.1
Virial equation (This 1982 300 - 700 0.2 - 0.6
report)
28
APPENDIX D (Continued)
Specific Heats Date Type Range of T, K
Dana [19] 1926 Ca(T) 257 - 294
Huffman [40] 1931 Ca(T) 140 - 252
Sage [65] 1937 Cp(T) 294 - 411
Aston [1] 1940 Co(T) 140 - 268
Dailey [18] 1943 CO(T) 345 - 693
Chen [12] 1975 C°(T) Spectroscopic
Heats of Vaporization Date Temperature Range, K
Dana [19] 1926 275 - 297
Sage [64] 1937 294 - 394
Das [20] 1967 273 - 420
Das [21] 1973 280 - 420

Thermal loops (This report) 1982 T^ - 270
Clapeyron equation (This report) 1982 140 - 420
Sound Velocities Date Temperature Range, K
Rao [58] 1971 143 - 268
Dielectric Constants Date Temperature Range, K
Sliwinski [67] (index of refraction) 1969 283 - 368
Thompson [70] 1980 228
Luo [47] 1981 220 - 289

Haynes [35,38] 1981 135 - 303
29
)
APPENDIX E. Computer Program
PROGRAM NBTHRMB INPUT, OUTPUT)

(
C REVISION OF NBUTANE THERMOFUNCTIONS RDG/NBS, START MAR. 26, 1981.

,
COMMON GK,GKK, Bl ,B2 ,B3 ,B4 ,B5 C1,C2,C3, E1,E2,E3, ER, IX

,
COMMON/l/AL BE ,GA,DE EP ET DCRT ,TCRT ,PCRT DGAT ,DTRP ,TTRP PTRP

, , , , , ,
C0MM0N/3/DPDT,D2PDT2,DPSDT,DPMDT,DPDD,DPDR,DTSDR,DTHDR,DDSDT
C0MM0N/4/XBl,XB2, XC1,XC2, XE1,XE2, DXBDR ,DXCDR ,DXEDR
COMMON/6/ TSAT, THETA, PSAT
COMMON/8/ IN, IK, P,T,DEN, E,H,S, CV,CP,CSAT, W,WK
.
COMMON /9/ DNG,EG,HG,SG, CVG,CPG,WG, DPGDT,DPGDD

COMMON/11/ DELS, DELCV
C0MM0N/12/ZCRT,ZCALC,DZDT, ZSAT,DZSDT, ZFX, FRT,DFRTDT
COMMON/21/ TPS(70)
-COMMON/95/ PIS, DIS, DPTIS, DPDIS
COMMON/99/ TI,EZZ, EZ,SZ,CVZ, HZ,CPZ
. DIMENSION HZA(70), SZA(70), PP(99)
DATA (WM=58. 1243) ,(PA=1. 01325) ,(GJ=8. 3145)
1 FORMATdS, 2F10.0)
2 F0RMAT(I5, 3F10.0)
3 F0RMAT(8I10)
5 FORMAT (IX)
9 F0RMAT(8F10.0)
14 FORMATdHl 13X * NBUTANE ISOBAR AT P =* F10.6, 4H MPA / )
16 FORMAT( 9X1HT 8X3HDEN 9X3HDEN 8X1HZ 5X5HDP/DT 5X5HDP/DD

2 8X1HE 8X1HH 8X1HS 6X2HCV 6X2HCP 9X3HF/P 5X1HW 4X5HDIEL. /
3 9X1HK 6X5HM0L/L 7X5HKG/M3 9X 5X5HMPA/K 1X9HMPA-M3/KG
4 4X5HJ/M0L 4X5HJ/M0L 2X7HJ/M0L/K 1X7HJ/M0L/K 1X7HJ/M0L/K
5 12X 1X5HM/SEC 4X5HC0NST )
17 FORMATdX F9.3, Ell. 4, E12.5, F9.5, F10.6, F10.5,

1 2F9.1, F9.3, 2F8.2, E12.5, 16, F9.5)
20 F0RMAT(1H116X*TEST IDEAL FNCTNSV17X 3HT,K 7X3HHZA 7X3HSZA )
21 FORMATdOX F10.2, FlO.l, F10.3)
80 CALL PVTDATA
CALL PEEK $ CALL ISOTHRM
C COMPUTE THERMOFUNCTIONS ON ISOBARS. START ON THE MELTING LINE.
C NOTE, ISOBAR P=PCRT OK, BUT ISOTHERM T=TCRT IS EXCLUDED.
C ISOBARS AT P UNDER PORT TRAVERSE THE DOME.
C NOTE USE OF QVAP ,DATA, TO CROSS THE ,DOME,.
C NOTE USE OF CSAT ,DATA, FOR SPECIFIC HEATS IN COMPRESSED LIQUID.
C NOTE TPS(IK) USED BY COMPRES.
C GET FUGACITIES, F/P, VIA H,S, HZ{T),SZ(T). (J. F.ELY).
C SAVE HZA(70), SZA(70) FROM 90 THRU 700 K.
85 DO 86 J=9,70 $ TI = 10*J $ CALL IDEAL $ HZA(J) = HZ
86 SZA(J) = SZ
C 87 PRINT 20 $ DO 88 J=9,70 $ T = 10*J
C 88 PRINT 21, T, HZA(J), SZA(J)
89 CALL JTLOCUS $ CALL TABLIQ
90 IN = 1 $ NI = 57 $ READ 9, PP( I
( 1 = 1) NI, ,
91 DO 300 I=IN,NI $ IK = I $ LS = 0
92 P = PP(I) $ IF(I.EQ.26) P = PORT
93 PK = P/IO $ PRINT 14, PK $ PRINT 16
100 T = FINDTMF(P) $ CALL COMPRLQ $ V=1/DEN $ IW=W
101 Z = P/DEN/GKK/T $ DIE = DIELF{DEN ,T,P)
102 TI = T $ CALL IDEAL $ GIB = H-EZZ-HZ - T*(S-SZ)
103 XP = EXP(GIB/GJ/T) $ FOP = XP*PA/P $ CALL CON
30
104 PRINT 17, T,DEN,DIS,Z, DPTIS,DPDIS, E,H,S,CV,CP, FOP, IW, DIE
105 IT = T/10 $ IF(P.LT.PCRT) 110,180
C CASES FOR P LESS THAN PORT.
110 TPS(IK) = TS = FINDTSF(P) $ K = L = 0
111 DO 150 J=l,99 $ T = JT = 10*(IT+J)
112 IF{T.LT.TS) 113,117
113 CALL COMPRES $ V = 1/DEN $ IW = W
114 Z = P/DEN/GKK/T $ DIE = DIELF( DEN ,T,P)
M =JT/10 $ GIB = H-EZZ-HZA(M) - T*(S-SZA(M))
XP = EXP(GIB/GJ/T) $ FOP = XP*PA/P % CALL CON
115 PRIUT 17, T,DEN,DIS,Z, DPTIS,DPDIS, E,H,S,CV,CP, FOP, IW, DIE
116 GO TO 150
117 LS = LS + 1 $ IF{LS.EQ.l) 120,130
C CASE FOR SATURATED LIQUID AND VAPOR.
120 T = TS $ CALL COEXIST $ V=1/DEN $ VG=1/DNG $ IW=W $ IWG=Wn
121 Z = P/DEN/GKK/T $ ZG = P/DNG/GKK/T
122 DIEL = DIELF(DEN,T,P) $ DIEG = DIELF(DNG,T,P)
123 TI = T $ CALL IDEAL $ GIB = H-EZZ-HZ - T*(S-SZ)
124 FOP = EXP(GIB/GJ/T)*PA/P $ CALL CON
125 PRINT 17, T,DEN,DIS,Z, DPTIS,DPDIS, E,H,S,CV,CP, FOP, IW, DIEL
126 PRINT 5 $ DIS=DNG*WM $ DPTIS=DPGDT/10 $ DPDIS = DPGDD/IO/WM
127 PRINT 17, T, DNG,DIS,ZG,DPTIS, DPDIS, EG, HG,SG,CVG,CPG, FOP, IWG, DIEG
128 T = JT
C CASES FOR THE HOMOGENEOUS DOMAIN.
130 IF(JT.GT.500) 131,132
131 K = K+1 $ T = JT = JT + 10*K $ IF{ JT .GT .700) 300,132
132 CALL GENIUS $ V=1/DEN $ IW=W $ Z = P/DEN/GKK/T
133 IF(T.GT.450) 134,135
134 DIE = 0 $ GO TO 136
135 DIE = DIELF{DEN,T,P)
136 M =JT/10 $ GIB = H-EZZ-HZA(M) - T*(S-SZA(M))
137 XP = EXP{GIB/GJ/T) $ FOP = XP*PA/P $ CALL CON
141 PRINT 17, T,DEN,DIS,Z, DPTIS, DPDIS, E,H,S,CV,CP, FOP, IW, DIE
150 CONTINUE
C FOR P.GE.PCRT, CASES FOR T.LT.OR.T.GT.TCRT.
180 TPS(IK) = TCRT $ K = L = 0
181 DO 250 J=l,99 $ T = JT = 10*(IT+J)
182 IF(T.LT.TCRT) 190,210
C CASE A FOR T LESS THAN TCRT.
190 CALL COMPRES $ V = 1/DEN $ IW = W
191 Z = P/DEN/GKK/T $ DIE = DIELF(DEN,T,P)
192 M =JT/10 $ GIB = H-EZZ-HZA(M) - T*(S-SZA(M))
193 XP = EXP{GIB/GJ/T) $ FOP = XP*PA/P $ CALL CON
194 PRINT 17, T,DEN,DIS,Z, DPTIS, DPDIS, E,H,S,CV,CP, FOP, IW, DIE
195 GO TO 250
C CASE FOR T ABOVE TCRT, HOMOGENEOUS DOMAIN.
210 IF(JT.GT.500) 211,220
211 K = K+1 $ T = JT = JT + 10*K $ IF(JT.GT.700) 300,220
220 CALL GENIUS $ V=1/DEN $ IW=W $ Z = P/DEN/GKK/T
221 IF(T.GT.450) 222,223
222 DIE = 0 $ GO TO 224
223 DIE = DIELF(DEN,T,P)
224 M =JT/10 $ GIB = H-EZZ-HZA(M) - T*{S-SZA(M))
225 XP = EXP(GIB/GJ/T) $ FOP = XP*PA/P $ CALL CON
31
226 PRINT 17, T,DEM,DIS,Z, DPTIS,DPDIS, E,H,S,CV,CP, FOP, IW, DIE
250 CONTINUE
300 CONTINUE
999 STOP $ END
SUBROUTINE COEXIST
C T AT COEXISTENCE, GET BOTH VAPOR AND LIQUID FUNCTIONS.
GIVE^^:
C FOR VAPOR, GET DNG,EG,HG,SG, CVG,CPG,WG, DPGDT,DPGDD, -
C FOR LIQUID, GET DEN,E,H,S, CV,CP,CSAT,W. DPDT,DPDD.

C COEXIST CALLED BY COMPRLQ. P NOT USED, MUST NOT CHANGE.
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT,TCRT,PCRT, DGAT ,DTRP ,TTRP ,PTRP
C0MM0N/3/DPDT ,D2PDT2 ,DPSDT ,DPMDT ,DPDD ,DPDR ,DTSDR ,DTHDR ,DDSDT
C0MM0N/9/DNG,EG,HG,SG, CVG,CPG,WG, DPGDT,DPGDD
DATA (Q=l. 01325) (0=0.083145)
,
1 FORMAT! IHO 9X *T EXCEEDS TCRT IN COEXIST. * / )
2 IF(T.GT.TCRT) 3,4
3 PRINT 1 $ STOP
4 PS = PSATF(T) $ DNG = DB = DENGASF(T)
5 TI = T $ CALL IDEAL $ $ M=15 DA=L=0
6 EG = EZZ + EZ + EDELF(L,M,T,DA,DB) $ HG = EG + 100*PS/DB
7 SG = SZ + DELS - 100*G*AL0G(Gn*DB/Q)
8 IF(T.EQ.TCRT) 9,11
9 PX = PVTF(T,DB,1) $ DPGDT = DPDT $ DPGDD = DPDD
10 CPG = CVG = WG = 0 $ GO TO 15
11 CVG = CVZ + DELCV $ PX = PVTF(T,DB,1)
12 CPG = CVG + 100*T/DPDD*(DPDT/DB)**2 $ WG = SQRT( WK*CPG*DPDD/CVG)
13 DPGDT = DPDT $ DPGDD = DPDD
C NOW TRAVERSE THE ,DOME, USING QVAP ,DATA,.
15 DEN = DL = DENLIQF(T) $ DDLDT = DDSDT $ QV = QVAPXF{T)
15 H = HG - QV $ S = SG - QV/T $ E = H - 100*PS/DL
C THIS RETURN AT 16+ USED ONLY WHEN CALLING SSATFIT, HSATFIT.
17 IF{T.EQ.TCRT) 18,19
18 PX = PVTF(T,DL,1) $ CP=CV=CSAT=W=0 $ RETURN
19 CSAT = CSATXF(T) $ PX = PVTF(T,DL,1)
22 CV = CSAT + 100*T*DPDT*DDLDT/DL/DL
23 CP = CV + 100*T/DPDD*(DPDT/DL)**2
30 W = SQRT(WK*CP*DPDD/CV) $ RETURN $ END
SUBROUTINE COMPRES
C SAVES COMPUTER TIME INTEGRATING COMPRLIQ AT T.LT.TCRT.
C FOR T = INTEGER MULTIPLES OF 10 K. FIRST ISOBAR USES COMPRLQ.
C FOR SUCCEEDING ISOBARS, START ON PREVIOUS ISOBAR, EXCEPT -
C AT TEMPS GE TPS(IK-l) ON PREVIOUS ISOBAR, MUST USE COMPRLQ.
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT TCRT PORT DGAT ,DTRP ,TTRP ,PTRP
, , ,
C0MM0N/3/DPDT,D2PDT2,DPSDT,DPMDT, DPDD, DPDR,DTSDR,DTHDR, DDSDT

COMMON/8/ IN, IK, P,T,DEN, E,H,S, CV, CP, CSAT, W,WK
COMMON/21/ TPS(70)
DIMENSION DK(50) ,EK{50) ,SK{50) ,CK(50)
1 FORMAT! IHO 9X *T G.E. TCRT IN COMPRES. * / )
2 IF(T.GE.TCRT) 3,4
32
3 PRINT 1 STOP
$
4 J = T/10 $ IF(T - 10*J) 5,6
5 CALL COMPRLQ $ RETURN
6 IF(IK.EQ.IN) 7,9
7 CALL COMPRLQ
8 DK{J)=DEN $ EK(J) = E $ SI<{J)=S $ CK(J)=CV $ RETURN
C INTEGRATE FROM OLD DEN TO NEW DEN ON GIVEN ISOTHERM -
C EXCEPT IF T EXCEEDS OLD TMAX USE COMPRLQ.
,
9 IF(T.GE.TPS(IK~1)) GO TO 7
10 DA=DK(J) $ DK(J) = DEN = DB = FINDENF{T,P) $ N = 13
11 EK(J) = E = EK(J) + EDELF(1,N,T,DA,DB) $ H = E + 100*P/DB
12 SK{J) = S = SK(J) + DELS $ CK(J) = CV = CK(J) + DELCV
C GET NEW DP/DT, DP/DD, CP, W.
15 PX = PVTF{T,DB,1) $ CP = CV + 100*T/DPDD*(DPDT/DB)**2
30 W = SQRT(WK*CP*DPDD/CV) $ RETURN $ END
SUBROUTINE COMPRLQ
C GIVEN P,T FOR COMPR.LIQ. AT T.LT.TC, GET DEN AND FUNCTIONS.
C REVISED TO USE HSATF, SSATF, CSATXF, BUT NOT COEXIST. TIMESAVER.
C INTEGRATE ALONG ISOTHERM T FROM SATLIQ UP TO POINT (P,T).
C0MM0N/3/DPDT,D2PDT2,0PSDT,DPMDT,DPDD,DPDR,DTSDR,DTHDR,DDSDT
1 FORMAT! IHO 9X *T NOT UNDER TCRT IN COMPRLQ.*/)
2 IF{T.GE.TCRT) 3,4
3 PRINT 1 $ STOP
C GET PSAT, DENLIQ, AND SATLIQ FUNCTIONS FOR START.
4 PS = PSATF(T) $ DL = DENLIQF{T) $ DDLDT = DDSDT
6 HS = HSATF(T) $ ES = HS - 100*PS/DL $ SS = SSATF(T)
C 7 IF(T.GT.340) 8,9
C 8 CVS = CVSATF(T) $ GO TO 10
9 PX=PVTF(T,DL,0) $ CVS = CSATXF{T) + 100*T*DPDT*DDLDT/DL/DL
C INTEGRATE UP TO POINT (P,T).
10 DB = FINDENF(T,P) $ DX = DB - DL $ IF(DX.GT.O) 11,20
11 M = 14 $ E = ES + EDELF(1,M,T,DL,DB)
12 H = E + 100*P/DB $ S = SS + DELS $ CV = CVS + DELCV
13 PX = PVTF{T,DB,1) $ CP = CV + 100n/DPDD*( DPDT/DB)**2
14 W = SQRT(WK*CP*DPDD/CV) $ DEN = DB $ RETURN
20 DEN=DL $ E=ES $ H=HS $ S=SS $ CV=CVS $ PX = PVTF{T,DL,1)
21 CP = CV + 100*T/DPDD*{DPDT/DL)**2 $ W = SQRT( WK*CP*DPDD/CV)
30 RETURN $ END
SUBROUTINE CON
C CONVERT TO SI UNITS FOR P, DEN, DP/DT, DP/DD,
C0MM0N/3/DPDT ,D2PDT2 DPSDT ,DPMDT DPDD ,DPDR DTSDR DTHDR DDSDT
, , , , ,

COMMON/95/ PIS, DIS, DPTIS, DPDIS
DATA (WM = 58.1243)
1 PIS = P/10 $ DIS = DEN*WM
2 DPTIS = DPDT/10 $ DPDIS = DPDD/IO/WM
9 RETURN $ END
FUNCTION CSATXF (T)
33
) .
C NBUTANE SATLIQ CSAT, J/MOL/K.

C CONSTRAINED AT TRIPLE AND CRITICAL POINTS.
C Y # (S-SCRT)/{STRP-SCRT) X #
, TC-T) /( TC-TT)
(
C Y = X + (XE-X)*(A1 + A2*X + A3*X2 + .). . .
DIMENSION AS(6)
DATA {NFS=6) ,(ES=0.23) ,(TTRP=134.86) ,{TCRT=425.16)
DATA (STRP = 133. 54372), (SORT = 297.64652)
DATA (AS = 0.08883444348, -0.3470304947, 0.2093724392,
1 -0.9568328496, 0.9579992545, -0.6534607056)
1 FORMATdHO 9X *CSATXF, T.GT.TCRT. * / )
2 IF(TCRT-T) 3,4,5
3 PRINT 1 $ STOP
4 CSATXF =0 $ RETURN
5 XN=TCRT-TTRP $ X = (TCRT-T)/XN $ DXDT = -1/XN $ SN=STRP-SCRT
6 XE = X**ES $ V = XE -X $ VI = ES*XE/X - 1
7Z1=Z=0 $ DO 9 K=1,NFS $ L=K-1 $ XL= X**L
8 Z = Z + AS(K)*XL $ Zl = Zl + L*AS{K)*XL/X
9 CONTINUE $ DSDT = SN*(1 + V*Z1 + V1*Z)*DXDT
10 CSATXF = T*DSDT $ RETURN $ END
FUNCTION DELTAF(T,D)
C GET (T*DP/DT - D*DP/DD) FOR THE J-T INVERSION CURVE.
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT ,TCRT ,PCRT, DGAT ,DTRP ,TTRP ,PTRP
C0MM0N/3/DPDT,D2P0T2,DPSDT,DPMDT,DPDD,DPDR,DTSDR,DTHDR,DDSDT
1 IF(T-TCRT) 2,4,4
2 DL - DENLIQF(T) $ IF{D-DL) 3,3,4
3 DELTAF l.OE+100
= $ RETURN
4 P = PVTF(T,D,1)
5 DELTAF = ABS (T*DPDT-D*DPDD) $ RETURN $ END
FUNCTION DENGASF(T)
C DESIGNED FOR ZSAT = 1 AT LOW DENSITIES, 5/29/77.
C USE ZSAT # PS/DS/GK/TS WITH VAPOR PRESSURES, AND ZCRT.
C Z = 1 + (ZCRT-1)*PI*F(X)/X/X.
C F(X) # 1 + A1*UE + A2*U + A3*EXP( EGX*{ 1-1/U) )
C NOTE ZSMl FOR FUGACTY, NOT IN COMMON HERE.
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT ,TCRT PORT DGAT ,DTRP ,TTRP ,PTRP
, ,
DIMENSION AV(3)
DATA (EG=0.35) ,{ EGX=2. 30) ,( GKK=0 .083145
DATA(AV = -0.8665772894, 1.120397967, 4.498658942)
1 FORMATdHO 9X *T EXCEEDS TC IN DENGASF. * / )
2 IF(TCRT-T) 3,4,5
3 PRINT 1 $ STOP
4 DENGASF = DCRT $ DDSDT = l.OE+10 $ RETURN
5 ZN = ZCRT-1 $ PC = PORT $ P = PSATF(T)
6 PI = P/PC $ PIT = DPSDT/PC $ TC = TCRT $ X = T/TC
7 X2 = X*X $ U = 1-X
8 UE = U**EG $ UEl = -EG*UE/U
9 EGXU = EGX*(1-1/U) $ IF(EGXU.LT.-270) 10,11
10 XP = XPl = 0 $ GO TO 12
11 XP = EXP(EGXU) $ XPl = -EGX*XP/U/U
12 F = 1 + AV(1)*UE + AV(2)*U + AV(3)*XP $ ZFX = F
34
.
13 Fl = AV(1)*UE1 - AV(2) + AV(3)*XP1

15 ZSMl = ZN*PI*F/X2 $ ZSAT = Z = 1 + ZSMl $ ZCALC = Z
16 DZSDT = DZDT = {PI*( F1-2*F/X)/TC + F*PIT)*ZN/X2
17 DENGASF = P/T/Z/GKK
18 DDSDT = (DPSDT - P/T - P*DZDT/Z) /T/Z/GKK $ RETURN $ END
FUNCTION DENLIQF(T)
C NBUTANE SAT. LIQUID DEN, MOL/L, (DCRT=3.92), RDG, IÎAR. 19, 1981.
C DEN = DCRT + YNL*(X + (XE-X)*Y), YNL # DTRP - DCRT.
C Y # Al + A2*X + A3*X2 + A4*X3.
C0MM0N/3/DPDT,D2PDT2, DPSDT, DPMDT,DPDD,DPDR,DTSDR,DTHDR, DDSDT
DIMENSION AW(3)
DATA (EL=0.35) ,(NFL=3)
DATA (TTRP=134.86) ,(TCRT=425.16) ,(DCRT=3.92) ,(DTRP=12.65)
DATA(AW = 0.794388335, -0.001089476, -0.085829197)
1 FORMATdHO 9X *DENLIQF = 0, T EXCEEDS TCRT. * / )
2 IF(TCRT-T) 3,4,5
3 PRINT 1 S STOP
4 DENLIQF = DCRT $ DDSDT = -l.OE+10 $ RETURN
5 XN=TCRT-TTRP $ X=(TCRT-T)/XN $ X2 = X*X $ DXDT = -1.0/XN
6 XE = X**EL $ U = XE - X $ Ul = EL*XE/X - 1
7Y1-Y=0 $ DO 9 K=1,NFL $ L = K-1 $ XL = X**L
8 Y = Y + AW(K)*XL $ Yl = Yl + AW(K)*L*XL/X
9 CONTINUE $ YNL = DTRP - DCRT
11 DENLIQF = DCRT + YNL*(X + U*Y)
12 DDSDT = YNL*(1 + U*Y1 + U1*Y)*DXDT $ RETURN $ END
FUNCTION DIELF(D,T,P)
C NBUTANE CONSTS., RDG, OCT. 14, 1980, VIA HAYNES DATA.
C CM,RMSPCT = 0.083, E,RMSPCT = 0.017.
C CM = Al + A2*R + A3*R2 + A4/X + A5*PI.
DIMENSION A(5)
DATA (DCRT=3.92) ,{TCRT=425.16)
DATA(A = 20.654382, 0.25129317, -0.097230479,
1 -0.039216489, -0.011645515)
1 R = D/DCRT $ X = T/TCRT $ G = 1/X $ PI = P/100
2 CM = A(l) + A(2)*R + A(3)*R*R + A(4)*G + A{5)*PI
3 Z = CM*D/1000 $ DIELF = (2*Z+1 )/( 1 .0-Z)
5 RETURN $ END
FUNCTION EDELF(L,M,T,DA,DB)
C GET CHANGE OF E, S, CV WITH DENSITY ALONG ISOTHERMS.
C GET EDELF, DELS, DELCV FROM DA TO DB ON ISOTHERM T.
C ROMBERG NUMERICAL INTEGRATION VIA -
C CARNAHAN/LUTHER/WILKES, APPLIED NUMERICAL METHODS, P. 90,
C JOHN WILEY AND SONS, INC., N.Y., 1969.
C NOTE, VALUE OF LD CONTROLS CONVERGENCE LIMITS.
C NOTE, NMAX = M, NK = FINAL, TOTAL SUBDIVISIONS OF INTERVAL DX
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT, TCRT, PORT, DGAT ,DTRP ,TTRP ,PTRP
C0MM0N/3/DPDT,D2PDT2, DPSDT, DPMDT,DPDD,DPDR,DTSDR,DTHDR, DDSDT
C0MM0N/12/ZCRT, ZCALC, DZDT, ZSAT, DZSDT, ZFX, FRT,DFRTDT
DIMENSION E(20), S(20), C(20)
DATA (LD=2) ,(DI=0. 00001) , (0=0.083145)
35
)
1 F0RMAT(1H09X*EDELF L =*I2,5H, N =13, 5H, T = F8.3,6H, DA =E10.4,

1 6H, DB =E10.4, 6H, LD =12//
2 lOX IHN 7X5HEDELF 8X4HDELS 7X5HDELCV )
2 FORMATdHO 9X 6HEDIF =F10.3, 8H, SDIF =F10.5, 9H, CVDIF =F10.3)

3 F0RMAT(6X 15, F12.3, F12.5, F12.3)
4 FORMATdHO 9X *EOELF NG AT TCRT FOR CV AT DEN NEAR OR GT CP.*/)
C FOR DA=0 AND DB.LE.DI, IDEAL GAS, EDELF=DELS=DELCV=0.
C FOR DA=0 AND DB.GT.DI, START ROMBERG WITH DA = DI, -
C TO AVOID INFINITIES IN ORDINATE FUNCTIONS AT DA = 0.

5 NK = 1 $ DM = DCRT/2 $ DZ = 0.98*DCRT
9 ZK = 1.0 - 1/ZCRT $ RK = 100*GnCRT/DCRT
10 IF(L.EQ.O) 11,14
11 IF(DB.LE.DI) 12,13
12 EDELF = DELS = DELCV =0 $ RETURN
13 DA = DI
C GET FIRST TRAPEZOID AREA, E(l) ETC., FROM DA TO DB.
14 DX = DB - DA $ P = PVTF(T,DA,0) $ IF(DA,LT.DM) 16,17
16 EA - RK*(ZK*ZSAT*ZFX + FRT - T*DFRTDT) $ GO TO 18
17 EA = 100*(P-T*DPDT)/DA/DA
18 IF{L.EQ.O) 19,20
19 SA = -RK*DFRTDT $ GO TO 21
20 SA = -100*DPDT/DA/DA
21 CA = -100*T*D2PDT2/DA/DA
22 P = PVTF(T,DB,0) $ IF{DB.LT.DM) 23,24
23 EB = RK*(ZK*ZSAT*ZFX + FRT - T*DFRTDT) $ GO TO 25
24 EB = 100*(P-T*DPDT)/DB/DB
25 IF(L.EQ.O) 26,27
26 SB = -RK*DFRTDT $ GO TO 28
27 SB = -100*DPDT/DB/DB
28 CB = -100*T*D2PDT2/DB/DB
29 E(l)=(EA+EB)*DX/2 $ S(l)=(SA+SB)*DX/2 $ C(l)=(CA+CB)*DX/2
C INTERVAL HALVING, GET E(N+1), ETC.
30 DO 60 N=1,M $ K = N + 1
31 JM = 2**N - 1 $ DXN = DX/2**N $ E(K) = S(K) = C(K) = 0
33 DO 45 J=1,JM,2 $ NK = NK+1 $ DN = DA + J*DXN
34 P = PVTF(T,DN,0) $ IF(DN.LT.DM) 35,36
35 EB = RK*(ZK*ZSAT*ZFX + FRT - T*DFRTDT) $ GO TO 37
36 EB = 100*{P-T*DPDT)/DN/DN
37 IF{L.EQ.O) 38,39
38 SB = -RK*DFRTDT $ GO TO 40
39 SB = -100*DPDT/DN/DN
40 CB = -100*T*D2PDT2/DN/DN
41 E(K) = E(K) + EB $ S(K) = S(K) + SB $ C(K) = C(K) + CB
45 CONTINUE $ E(K) = E{N)/2 + E(K)*DXN
46 S{K) = S(N)/2 + S(K)*DXN $ C(K) = C{N)/2 + C(K)*DXN
C
C TEST FOR CONVERGENCE.
50 ED=ABS{E(K)-E(N)) $ SD=ABS( S(K) -S( N) ) $ CD=ABS(C(K)-C(N)
53 IF(ED.LT.0.4/LD) 54,60
54 IF(SD.LT.0.002/LD) 55,60
55 IF(T.EQ. TCRT. AND. DB.GT.DZ) GO TO 57
56 IF(CD.LT.0.04/LD) 57,60
57 EDELF = E{K) $ DELS = S(K) $ DELCV = C(K) $ RETURN
60 CONTINUE $ N = M $ NM = N-1 $ NP = N+1
36
61 PRINT 1, L, N, T, DA, DB, LD
62 PRINT 3, NM,E(NM) ,S(NM) ,C(NM) $ PRINT 3, N ,E( N) , S( N ) ,C( N)
64 PRINT 3, NP,E(NP) ,S{NP) ,C(NP) $ PRINT ?., ED, SD, CD
99 STOP $ END
FUNCTION FIMDENF(T,P)
C ON ISOTHERM T, FIND DEN, MOL/L, TO MINIMIZE (P-PC) VIA EQNSTATE.
C0MM0N/1/AL,BE,GA,0E,EP,ET, DCRT,TCRT,PCRT, DGAT ,DTRP ,TTRP ,PTRP
C0MM0N/3/DPDT,D2PDT2,0PSDT,DPMDT,DPDD,0PDR,DTSDR,DTHDR,D0SDT
DATA (GKK = 0.083145)
41 FORMATdHO 9X *FINDENF = 0, FAILS TO CONVERGE. * / )
42 FORMATdHO 9X *FINDENF = DCRT, DP/DR ZERO OR NEG. * / )
43 FORMATdHO 9X *FINDENF = 0, DOUBLE-VALUED AT P = PSAT. * / )
DM = 1.05*DTRP
IF(P.GT.O) 1,35
1 IF(T-TCRT) 2,5,8
2 DG=DENGASF(T) $ DL=DENLIQF(T) $ PS=PSATF(T) $ IF{P-PS) 3,32,4
3 D = DG/2 $ GO TO 11
4 D = (DL+DTRP)/2 $ GO TO 11
5 DG=DL=DCRT $ PS=PCRT $ IF(P-PS) 6,33,7
6 D = DCRT/2 $ GO TO 11
7 D = 2*DCRT $ GO TO 11
8 IF(T.LT. 450.0) 9,10
9 PC = PVTF(T,DCRT,0) $ IF{P-PC) 6,33,7
10 D = DCRT
11 DO 30 J=l,50 $ DP=P-PVTF{T,D,1) $ IF(ABS (DP/P)-1 .OE-7) 31,31,12
12 IF(DPDD.GT.O) 13,34
13 DD = DP/DPDD $ IF(ABS DD/D )-l .OE-7 ) 31,31,14
(
14 D = D + DD $ IF{D.GT.O.O) 16,15
15 D = P/GKK/T $ GO TO 30
16 IF(D.GT.DM) 17,18
17 D = DM $ GO TO 30
18 IF(T-TCRT) 19,24,30
19 IF{P.LT.PS) 20,22
20 IF(D.GT.DG) 21,30
21 D = DG $ GO TO 30
22 IF(D.LT.DL) 23,30
23 D = DL $ GO TO 30
24 IF(P.LT.PCRT) 25,27
25 IF(D.LT.DCRT) 30,26
26 D = DCRT - 0.02 $ GO TO 30
27 IF{D.GT.DCRT) 30,28
28 D = DCRT + 0.02
30 CONTINUE $ PRINT 41 $ STOP
31 FINDENF = D $ RETURN
32 PRINT 43 $ STOP
33 FINDENF = DCRT $ RETURN
34 FINDENF = DCRT $ PRINT 42 $ RETURN
35 FINDENF=DPDT=D2PDT2=0 $ DPDD=GKK*T $ DPDR=DPDD*DTRP
36 RETURN $ END
FUNCTION FINDTMF(P)
C GIVEN P ON THE MELTING LINE, FIND T FOR NBUTANE.
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT,TCRT,PCRT, DGAT,DTRP ,TTRP ,PTRP
37
DATA (A=3634.0) ,(E=2.210)
1 X = (P-PTRP)/A + 1 $ FINDTMF = TTRP*X**( 1 .0/E) $ RETURN $ END
FUNCTION FINDTSF(P)
C GIVEN VAPOR PRESSURE P, ITERATE T TO MINIMIZE (P-PC).
C0MM0M/1/AL,BE,GA,DE,EP,ET, DCRT,TCRT,PCRT, DGAT ,DTRP ,TTRP ,PTRP
C0MM0N/3/DPDT,D2PDT2,DPSDT,DPMDT,DPDD,DPDR,DTSDR,0THDR,DDSDT
1 FORMATdHO 9X *FINDTSF = 0, FAILS TO CONVERGE. * / )
2 FORMATdHO 9X *FINDTSF = 0, P EXCEEDS PCRT. * / )
3 IF(P-PCRT) 4,11,12
4 T = 300 $ DO 9 J=l,50 $ DP = P - PSATF{T) $ ADP = ABS (DP)
5 IF(ADP/P-1.0E-7) 10,6,6
6 IF(ADP/DPSDT/T-1.0E-7) 10,7,7
7 T = T + DP/DPSDT $ IF(T-TCRT) 9,9,8
8 T = TCRT
9 CONTINUE S PRINT 1 $ STOP
10 FINDTSF = T $ RETURN
11 FIMDTSF = TCRT $ RETURN
12 PRINT 2 $ STOP S END
SUBROUTINE GEMEOUS
C GIVEN P,T FOR THE HOMOGENEOUS DOMAIN -
C GET DEN AND FUNCTIONS AT ANY TEMPERATURE.
C0MM0M/3/DPDT,D2PDT2,DPSDT,DPMDT,DPDD,DPDR,DTSDR,DTHDR,DDSDT
DATA (Q=l. 01325) (0=0.083145)
,
3 TI = T $ CALL IDEAL $ IF(P.GT.O) 4,10

4 DEN = DB = FINDENF(T,P) $ M = 15 $ DA = L = 0
5 E = EZZ + EZ + EDELF(L,M,T,DA,DB) $ H = E + 100*P/DB
6 S = SZ + DELS - 100*G*AL0G(G*T*DB/Q)
7 CV = CVZ + DELCV $ PX = PVTF(T,DB,1)
8 CP = CV + 100*T/DPDD*(DPDT/DB)**2
q W = SQRT(WK*CP*DPDD/CV) $ RETURN
10 DEN=S=0 $ E = EZZ + EZ $ H = E + 100*G*T S CV=CVZ $ CP=CPZ
12 W = SQRT(WK*CP*G*T/CV) $ RETURN $ END
SUBROUTINE GENIUS
C VALID ONLY FOR THE HOMOGENEOUS DOMAIN.
C SAVES COMPUTER TIME WHEN TABULATING FUNCTIONS ALONG ISOBARS.
C SAVES DEN,E,S,CV ALONG ISOBARS FOR USE IN INTEGRATING TO NEXT
C HIGHER ISOBAR. VALID ONLY FOR MONOTONICALLY INCREASING ISOBAR
C PRESSURES, AND AT TEMPS. T = INTEGER MULTIPLES OF 10 K.
C0MM0N/3/DPDT,D2PDT2,DPSDT,DPMDT,DPDD,DPDR,0TSDR,DTHDR,DDSDT
DIMENSION DK(70) ,EK(70) ,SK(70) ,CK{70)
1 FORMATdHO 9X *GENIUS T NOT INTEGRAL. * / )
2 = T/10
J $ IF(T - 10*J) 3,4
3 CALL GENEOUS $ RETURN
4 IF(IK.EQ.IN) 5,9
5 CALL GENEOUS
6 DK(J) = DEN $ EK(J) = E $ SK(J) = S $ CK(J)=CV $ RETURN
C INTEGRATE FROM OLD DEN UP TO NEW DEN ON GIVEN ISOTHERM.
38
9 DA = DK{J) DK(J) = DEN = DB = FIND£MF(T,P)
$ $ M = 14
11 EK(J) =E =
EK(J) + EDELF(1,N,T,DA,DB) $ H = E + 100*P/DB
13 SK(J) = S = SK{J) + DELS $ CK{J) = CV = CK(J) + DELCV
C NOW GET NEW DP/DT, DP/DD, CP, W.
15 PX = PVTF(T,DB,1) $ CP = CV + 100*T/DPDD*(DP0T/DB)**2
30 W = SQRTfWK*CP*DPDD/CV) $ RETURN $ END
FUNCTION HSATF(T)
C NBUTANE SATLIQ ENTHALPY, J/MOL.
C DEFINE YH # {H-HC)/( HT-HC) ,X # (TC-T)/(TC-TT) WHEN -,
C YH = X + (XE-X)*(A1 + A2*X + A3*X2 + .) . .
DIMENSION AH(8)
DATA (NFH=8) ,(EH=0.29) ,(TTRP=134.86) ,(TCRT=425.16)
DATA (HTRP = 0.001),(HCRT = 45399.788)
DATA (AH = 0.1929773377, 0.3998984487, -0.05499361241,
1 -1.020568625, 2.872789244, -4.052610155, 2.696377850,
2 -0.6834388986)
1 FORMATdHO 9X 3HT =F10.5, * IN HSATF(T).*/)
2 IF{T.GT.TCRT) 3,4
3 PRINT 1, T $ STOP
4 X = (TCRT-T)/(TCRT-TTRP) $ IF(X.LE.O) 5,6
5 HSATF = HCRT $ RETURN
6 V = X**EH -X $ FX=X $ DO 7 K=1,NFH
7 FX = FX + V*AH(K)*X**{K-1)
8 HSATF = HCRT - (HCRT-HTRP)*FX $ RETURN $ END
SUBROUTINE IDEAL
C N-BUTANE, VIA DATA OF CHEN ET AL (1975).
C CPZ/R = 4 + (Al + A2/X + A3/X2 + . . )*EXP{-E/X), X # T/IOO.
DIMENSION A(5)
DATA (E=2. 37) ,(R=8. 3145 ),(HI=7. 7980) ,(SI=37. 3495)
DATA(A = 41.1109726, -139.304011, 257.297067, -170.730596,
1 40.0321709)
1 NK = 5 $ XI = Tl/lOO $ XP = EXP(-E/XI)
2 CP = 4.0 $ DO 3 K=1,NK
3 CP = CP + A(K)*XP*XI**(1-K)
C NUMERICAL INTEGRATION FOR HZ/R, SZ/R -
5H=S=0 $ N= ABS(TI-300)/4 +4 $ DX = (XI-3)/N
6 DO 10 J=1,N $ X = 3.0 + (J-0.5)*DX $ XP = EXP(-E/X)
7 CPX = 4.0 $ DO 8 K=1,NK
8 CPX = CPX + A(K)*XP*X**(1-K)
9 H = H + CPX*DX $ S = S + CPX*DX/X
10 CONTINUE $ H = (HI*3 + H)/XI $ S = SI + S
C CONVERT TO JOULES, MOLES, KELVINS.
11 HZ = R*TI*H $ EZ = HZ - R*TI $ SZ = R*S
12 CPZ = R*CP $ CVZ = CPZ - R $ RETURN $ END
SUBROUTINE ISOTHRM
C PRINTOUT THE CRITICAL ISOTHERM.
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT,TCRT,PCRT DGAT ,DTRP ,TTRP PTRP
, ,
39
. )
DATA (WM =
58.1243)
1 FORMATdHl14X *THE CRITICAL ISOTHERM, NBUTANE* //
1 5X6HTC,K = F7.2, 12H, 0C,KG/M3 = F9.4, lOH, PC,MPA = F10.7/ 6X
2 *AT THE CP., DPS/DT =*F9.6, 9H, DP/DT =F9.6, * MPA/K.* //
3 5X4HD/DC 9X5HTS/TC 9X5HPS/PC 10X4HP/PC 9X5HDP/DR 4X6H0TS/DR
4 4X6HDTH/DR 4X5HDPS/DR 4X6HDXB/DR 4X6HDXC/DR )
2 F0RMAT(2X F8.3, 3F14.10, F14.9, 5F10.5)

3 PC = PVTF(TCRT,DCRT,0) $ PCS = PCRT/10 $ DCS = DCRT*WM
DPST = DPSDT/10 $ DPT = DPDT/10
4 PRIMT 1, TCRT, DCS, PCS, DPST, DPT $ DO 8 J=l,41
5 DR = 0.895 + O.OOS^J $ DN = DR*DCRT
'
6 PR = PVTF(TCRT,DN,1)/PCRT $ DPSDR = DPSDT*DTSDR

7 TSN = TSAT/TCRT $ PSN = PSAT/PCRT
DPDR = DPDR/10 $ DPSDR = DPSDR/10
8 PRINT 2, DR, TSN,PSN, PR, DPDR, DTSDR,DTHDR, DPSDR, DXBDR,DXEDR
9 RETURN $ END
SUBROUTINE JTLOCUS
€ THE JOULE-THOMSON P-V-T LOCUS FOR HBUTANE.
C DERIVE THE J-T INVERSION CURVE. USE ROUTINE DELTAF(T ,DI )
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT, TCRT, PORT, DGAT,DTRP,TTRP,PTRP
DIMENSION DK{60) ,DN{60) ,TT{60) ,PP(60)
DATA (A=1 .2275) ,{ B=0. 485) ,(WM=58. 1243)
1 FORMATdHl 16X nHE JOULE-THOMSON INVERSION LOCUS FOR NBUTANE* //
2 17X 3HT,K 8X2HDI 5X5HKG/M3 5X5HP,MPA
3 7X 3HT,K 8X2HDI 5X5HKG/M3 5X5HP,MPA )
2 FORMATdOX 110, 2F10.1, F10.3, 110, 2F10.1, F10.3)
C SAVE INITIAL, TRIAL DENSITY, DK(I) = DI.
5 TA = 340 $ NP = 52
6 PRINT 1 $ DO 25 1=1, NP $ DX = 0.4
7 T = TA + 10*1 $ X = T/TCRT $ DK(I) = DI = DCRT*EXP{ A-B*X
10 IF(T-TCRT) 11,12,12
. 11 DL = DENLIQF(T) $ IF(DI.LT.DL) 23,12
12 SS = DELTAF(T,DI) $ DO 20 IT=1,14
14 D=DI-DX $ SL=DELTAF(T,D) $ D=DI+DX $ SP=DELTAF(T,D)
15 IF(SS-SL) 18,16,16
.
16 IF(SP-SL) 19,17,17
17 SS = SL $ DI = DI - DX $ GO TO 20
18 IF(SS-SP) 20,20,19
19 SS = SP $ DI = DI + DX
20 DX = DX/2 $ TT(I) = T $ DN{I) = DI $ PP(I) = PVTF(T,DI,0)
21 GO TO 25
23 TT(I) = T $ DK(I) = DN(I) = PP(I) = 0
25 CONTINUE $ N = NP/2
26 DO 35 J=1,N $ K = J + N
27 IT = TT(J) $ ITT = TT(K)
28 DKJ = WM*DK(J) $ DNJ = WM*DN(J)
29 DKK = WM*DK(K) $ DNK = WM*DN{K)
30 PPJ = PP(J)/10 $ PPK = PP(K)/10
35 PRINT 2, IT, DKJ, DNJ, PPJ, ITT, DKK , DNK, PPK
40 RETURN $ END
SUBROUTINE PEEK
C EXAMINE BEHAVIOR OF THE PVT COEFFICIENTS.
40
. .
C B{S) # Bl + B2*S2, E(S) # El*( S-l)*( S-ER)*EXP{ -GA*S**IX)

C WHERE, R # DEN/DTRP, S # DEN/DCRT.
COMMON GK,GKK, Bl ,B2 ,B3 ,B4 ,85 C1,C2,C3, E1,E2,E3, ER,IX
,

C0MM0N/3/DPDT,D2PDT2,DPSDT,DPMDT,DPDD,DPDR,DTSDR,DTHDR,D0S0T
DATA (WM = 58. 1243), (EX = 1.10)
4 FORMATdHl 14X ÊQUATION OF STATE COEFFS., NBUTANE * //
1 15X 6HTTRP =F7.3, 8H, TRLP =F9.4, 8H, TCRT =F8.3, * K* /
2 15X 6HPTRP =E12.6, 8H, PBLP =F8.6, 8H, PCRT =F9.6, * MPA* /
3 15X 6HDTRP =E11.5, 8H, DLBP =E11.5, 8H, DCRT =E11.5, * KG/M3* /
3 15X 6HDGAT =E11.5, 8H, DGBP =E11.5, * KG/M3* /
3 15X *DPS/DTB,MPA/K =* Ell. 5, *, QVAPB,KJ/MOL =* F7.3//
4 15X 4HIX =12, 6H, EX =F5.2, 6H, ER =F5.2, *, S # DEN/DCRT* /
5 15X 4HAL =F10.7, 6H, BE =F10.7, 6H, GA =F10.7/
6 15X 4HDE =F10.7, 6H, EP =F10.7, 6H, ET =F10.7//
7 15X 4HB1 =F14.11, 6H, B2 =F14.11, 6H, B3 =F14.11/
8 15X 4HC1 =F14.11, 6H, C2 =F14.11, 6H, C3 =F14.11/ )
5 FORMAT! 15X 4HD/DC 5X4HTSAT 5X5HTHETA 4X6HPS,MPA 9X1HB 9X1HC )
6 F0RMAT(9X F10.2, 2F10.3, F10.4, 2F10.5)
8 TB=FINDTSF(1. 01325) $ DGB=DENGASF( TB) $ DLB=DENLIQF(TB)
9 QB = TB*DPSDT*(1/DGB - 1/DLB)/10.0
PTR = PTRP/10 $ PBLP = 0.101325 $ PCR = PCRT/10
DTR = DTRP*WM $ DLBI = DLB*WM $ OCR = DCRT*WM
DGA = DGAT*WM S DGBI = DGB*WM $ DPSB = DPSDT/10
10 PRINT 4, TTRP,TB, TCRT, PTR, PBLP, PCR, DTR, DLBI, DCR, DGA, DGBI, DPSB, QB,
1 IX,EX,ER, AL,BE,GA,DE,EP,ET, B1,B2,B3, E1,E2,E3
11 PRINT 5 $ N = 10*DTRP/DCRT + 1
12 DO 20 J=1,N $ S = 0.1*J
13 DN = S*DCRT $ S2=S*S $ SN=S-1 $ SX = S**IX
14 SR = 1 $ IF(ER.GT.O) SR = S-ER
16 B = Bl + B2*S2
17 E = (El + E2*S)*SN*SR*EXP(-GA*SX)
19 TSAT=TS=TSATF(DN) $ TH=THETAF( DN) $ PS=PSATF(TS) $ PIS=PS/10
20 PRINT 6, S, TS,TH,PIS, B,E $ RETURN $ END
FUNCTION PMELTF(T)
C NBUTANE MELTING LINE, BAR, VIA REEVES, SCOTT, AND BABB(JR),
C J. CHEM. PHYS. 40(12), 3662 (1964).
COMMON/l/AL ,BE ,GA,DE ,EP ,ET DCRT TCRT, PCRT, DGAT ,DTRP ,TTRP ,PTRP
, ,
C0MM0N/3/DPDT ,D2PDT2 ,DPSDT,DPMDT ,DPDD ,DPDR ,DTSDR ,DTHDR ,DDSDT

DATA (A = 3634.0) ,(E = 2.210)
1 X = T/TTRP $ XE = X**E $ PMELTF = PTRP + A*(XE-1)
2 DPMDT = A*E*XE/X/TTRP $ RETURN $ END
FUNCTION PSATF(T)
C NBUTANE VAPOR PRESSURE, BAR, RDG, FEB. 19, 1981. (0CRT=3.92).
C LN(P) = Pl/X + P2 + P3*X + P4*X2 + P5*X3 + P6*( 1-X)**EPP
C0MM0N/3/DPDT,D2PDT2,DPSDT, DPMDT, DPDD,DPDR,DTSDR,DTHDR,DDSDT
DIMENSION PJ(6)
DATA (EPP = 1.85)
DATA (TTRP=134.86) ,(TCRT=425.16) ,(DCRT=3.92),(DTRP=12.65)
DATA(PJ = -9.50924729, 5.20153488, 10.64095231,
1 4.86147936, -7.55818629, 18.72886023)
41
.
1 9X *T ABOVE TCRT IN PSATF(T). *

FORMATdHO / )
4 X = T/TCRT $ V = 1.0 - X $ IF(V) 7,8,9

7 PRINT 1 STOP$
8 Z = Zl = 0GO TO 10
$
9 2= v**EPP $ Zl = -EPP*Z/V
10 PL = PJ(6)*Z $ PLl = PJ(5)*Z1
11 DO 13 K=l,5 $ L = K-2 $ XL = X**L
12 PL = PL + PJ(K)*XL $ PLl = PLl + PJ(K)*L*XL/X
13 CONTINUE $ PSATF = EXP(PL)
15 DPSCT = PL1*PSATF/TCRT $ RETURN $ END
SUBROUTINE PVTDATA
C NBUTANE EOS CONSTANTS, RDG/NBS, FEB. 19, 1981. (DCRT=3.92).
COMMON GK,GKK, 81 ,B2,B3,B4,B5, C1,C2,C3, E1,E2,E3, ER, IX
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT, TCRT, PORT DGAT,DTRP ,TTRP ,PTRP
,

'
10 WM = 58.1243 $ TTRP = 134.86 $ TCRT = 425.16
12 DCRT = 3.92 $ DTRP = 12.650
13 PTRP = PSATF(TTRP) $ PORT = PSATF(TCRT)
20 GKK = 0.083145 $ GK = GKK*DCRT $ ZCRT = PCRT/DCRT/GKK/TCRT
21 IX = 2 $ AL = 1.0 $ BE = 0.7 $ GA = 0.14 $ DE = 0
22 EP = 0 $ ER = 2.20 $ ET = 1.1
23 Bl = 0.45555869162 $ B2 = 0.17143942370
24 El =-0.28036114629 $ B3=B4=E2=E3=0
25 DGAT = DENGASF(TTRP) $ WK = 100000/WM $ EZZ = 22644.306
99 RETURN $ END
FUNCTION PVTF(T,D,M)
C NBUTANE EQNSTATE, PVTF = P,BAR. SIMPLIFIED, FEB. 12, 1981.
C NOTE, M=0 RETURNS DP/DT, D2P/DT2. M=l RETURNS ALSO DP/DD.
C P-PSAT = S*GK*(T-TSAT) + S*S*GK*TCRT*F( S ,T) ,WHERE -
C F(S,T) # B(S)*XBF(S,T) + E( S) *XEF( S ,T), AND -
C B(S) # Bl + B2*S2, E(S) # El*{ S-1 )*{ S-ER)*EXP{ -GA*S**IX)

C WHERE, R # DEN/DTRP, S # DEN/DCRT.
COMMON GK,GKK, Bl ,B2 ,B3 ,B4 ,B5 C1,C2,C3, E1,E2,E3, ER,IX
,
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT, TCRT, PORT, DGAT DTRP TTRP PTRP

, , ,
C0MM0N/12/ZCRT,ZCALC,DZDT, ZSAT,DZSDT,ZFX FRT,DFRTDT
,
1 S = D/DCRT $ S2=S*S $ SN=S-1 $ SR=S-ER $ SX=S**IX

5 GK = DCRT*GKK $ TC = TCRT $ DSDR = DTRP/DCRT
6 RG = S*GK $ GKT = GK*TC
7 TSAT=TS=TSATF(D) $ PSAT=PS=PSATF( TS) $ THETA=THETAF(D)
8 XB = XBF(T,D) $ XE = XEF(T,D)
9 B = B1*S2 + B2*S2*S2
10 XP = EXP(-GA*SX) $ SM = S2*SN*SR $ E = E1*SM*XP
12 F = B*XB + E*XE $ Fl = B*XB1 + E*XE1 $ F2 = B*XB2 + E*XE2
13 PVTF = PS + RG*(T-TS) + GKT*F $ FRT=F/S2 $ DFRTDT=F1/S2/TC
14 DPDT = RG + GK*F1 $ D2PDT2 = GK*F2/TC $ IF{M) 15,30
15 BD = (2*B1 + 4*B2*S2)*S*DSDR
16 XPl = -IX*GA*SX/S $ SMI = (SN+SR)*S2 + 2*S*SN*SR
42
)
18 ED = E1*(SM*XP1 + SM1)*XP*DSDR
20 Fl = B*DXBDR + BD*XB + E*DXEDR + ED*XE
26 DPDR = (DPSDT-RG)*DTSDR + T-TS)*GK*DSDR + GKT*F1(
27 DPDD = DPDR/DTRP
30 RETURN $ END
FUNCTION QVAPXF(T)
C = A1*X + (XE-X)*(A2 + A3*X + A4*X2 +
QVAP ). . .
C X # {TC-T)/(TC-TT), XE # X**E.
DIMENSION AQ(4)
DATA NFQ=4 ( EQ=0 34
) , ( TTRP=134 .86
. TCRT=425 16
) , ( ) , ( .
DATA (AQ = 28.789248, 24.163103, 12.710873, -16.533537)

1 FORMATdHO 9X *T EXCEEDS TCRT IN QVAPXF{T). * / )
2 IF(TCRT-T) 3,4,5
3 PRINT 1 $ STOP
4 QVAPXF = 0 $ RETURN
5 XN = TCRT - TTRP $ X = (TCRT-T)/XN $ XE = X**EQ
6 F = 0 $ DO 7 K=2,NFQ
7 F = F + AQ(K)*X**{K-2)
9 Q = AQ(1)*X + {XE-X)*F
10 QVAPXF = Q*1000 $ RETURN $ END
SUBROUTINE SIMPLE
C FOR ANY GIVEN T,K AND P,MPA, CONVERT TO P,BAR, AND USE SUBROUTINE
C THERMO (OR ENTRIES THEREIN) TO GET THERMOPHYSICAL PROPERTIES.
C THEN CONVERT TO MPA, AND KG/M3 IN PRESENT ROUTINE.
C0MM0N/3/DPDT ,D2PDT2 DPSDT ,DPMDT DPDD , DPDR ,DTSDR DTHDR ,DDSDT
, , ,

DATA (R=0. 083145) {GJ=8. 3145) ,(PA=1. 01325) ,{WM=58. 1243)
,
14 FORMATdHl 18X *TEST OF THERMO AT P,MPA =* F8.5/

1 19X ^DENSITIES KG/M3, HEATS J/MOL. * / )
16 F0RMAT(6X4HPMPA 9X1HT 6X3HDEN 8X1HZ 5X5HDP/DT 5X5HDP/DD
1 8X1HE 8X1HH 8X1HS 6X2HCV 6X2HCP 5X1HW 9X3HF/P 5X4HDIEL )
17 FORMATdX F9.4, F10.3, F9.2, F9.5, F10.5, F10.6, 2F9.1, F9.3,

1 2F8.2, 16, E12.5, F9.5)
C LET US EXAMINE A SUBCRITICAL ISOBAR.
19 PMPA = 3.5
20 P = 10*PMPA $ PRINT 14, PMPA $ PRINT 16
21 DO 90 J=l,39 $ TIK = T = 130 + 10*J
22 CALL THERMO $ IW = W $ Z = P/DEN/R/T
C GET DIEL. CONST., AND FUGACITIES.
25 GIB = H-EZZ-HZ -T*(S-SZ) $ FOP = EXP{GI8/GJ/T)*PA/P
26 IF(T.GT.450) 27,28
27 DIE = 0 $ GO TO 30
28 DIE = DIELF(DEN,T,P)
C CONVERT PRESSURES, DENSITIES, AND DERIVATIVES.
30 PMPA=P/10 $ DEN=DEN*WM $ DPDT=DPDT/10 $ DPDD=DPDD/10/WM
31 DPMDT = DPMDT/10 $ DPSDT = DPSDT/10 $ DDSDT = DDSDT*WM
40 PRINT 17, PMPA, T, DEN, Z, DPDT,DPDD, E,H,S, CV,CP,IW, FOP, DIE
90 CONTINUE $ RETURN $ END
FUNCTION SSATF(T)
C NBUTANE SATLIQ ENTROPY, J/MOL/K.
43
.
C CONSTRAINED AT TRIPLE AND CRITICAL POINTS.

C Y #(S-SCRT)/(STRP-SCRT) , X # (TC-T)/(TC-TT)
C Y =X + (XE-X)*(A1 + A2*X + A3*X2 + . ).
. .
DIMENSION AS(6)
DATA (NFS=6) ,(ES=0.23) ,(TTRP=134.86) ,(TCRT=425.16)
DATA (STRP = 133.54372) ,(SCRT = 297.64652)
DATA (AS = 0.08883444348, -0.3470304947, 0.2093724392,
1 -0.9568328496, 0.9579992545, -0.6534607056)
1 FORMATdHO 9X 3HT =F10.5, * IN SSATF(T). * / )
2 IF{TCRT-T) 3,4,5
3 PRINT 1, T $ STOP
4 SSATF = SCRT $ RETURN
5 YN = STRP-SCRT $ XN = TCRT-TTRP
6 X = {TCRT-T)/XN $ XE = X**ES $ V = XE - X
7 Y = X $ DO 8 K=1,NFS
8 Y = Y + V*AS(K)*X**{K-1)
9 SSATF = SCRT + YN*Y $ RETURN $ END
SUBROUTINE TABLIQ
COMMON/l/AL BE ,GA ,DE EP ET DCRT .TCPJ ,PCRT DGAT ,DTRP ,TTRP PTRP
, , , , , ,
C0MM0N/9/DNG,EG,HG,SG, CVG,CPG,WG, DPGDT,DPGDD
C0MM0N/12/ZCRT,ZCALC,DZDT, ZSAT,DZSDT,ZFX FRT,DFRTDT
,

DIMENSION DSA(50) ,TSA(60) ,PSA(50) ,DLT(60) ,DPT(50) ,DPD(60)
DATA (0=0.083145) ,(WM=58. 1243)
4 FORMATdHl 13X ^PROPERTIES OF SATURATED LIQUID NBUTANE* //
1 14X IHT IIXIHP 3X5HDEN,L 7X5HDEN,G 5X3HZ,L 5X3HZ,G
2 5X6HDPS/DT 3X6HDDL/DT 3X5HDP/DT 6X5HDP/DD /
3 14X IHK 9X3HMPA 3X5HKG/M3 7X5HKG/M3 16X
4 5X5HMPA/K 2X7HKG/M3/K 3X5HMPA/K 2X9HMPA-M3/KG )
5 F0RMAT(5XF10.3, E12.5, F8.2, E12.5, 2F8.5, Ell .4,F9.4,F8.4,E11 .4)
11 FORMATdHl 13X ^PROPERTIES OF SATURATED LIQUID NBUTANE * //
1 14X IHT 4X5HQ,VAP 8X1HE 8X1HH 8X1HS
2 6X2HCV 6X2HCS 6X2HCP 6X3HF/P 6X1HW 4X5HDIEL. /
. 3 14X IHK 4X5HJ/M0L 4X5HJ/M0L 4X5HJ/M0L 2X7HJ/M0L/K
4 1X7HJ/M0L/K 1X7HJ/M0L/K 1X7HJ/M0L/K IIX 5HM/SEC 4X5HC0NST )
12 F0RMAT(5X F10.3, 3F9.1, F9.3, 3F8.2, F9.5, 17, F9.5)

C FOR PAGE ONE OF TABLIQ.
C REPLACE T = 230 BY B.P. AT J = 30.
120 NP = 59 PRINT 4
$
121 DO 150 J=1,NP $ IF(J.EQ.l) 122,123
122 T = TTRP $ GO TO 139
123 IF{J.EQ.29) 124,125
124 T = FINDTSFd. 01325) $ GO TO 139
125 IF(J.EQ.NP) 126,128
126 T = TCRT $ DSA(J)=DG=DL=DCRT $ DLT(J) = DDLDT = 0
127 VG = VL = 1.0/DCRT $ ZG = ZCRT $ GO TO 141
128 T = 130 + 5*J
139 DSA{J) = DL = DENLIQF(T) S DLT(J) = DDLDT = DDSDT
140 DG = DENGASF{T) $ ZG = ZSAT $ VG = 1/DG $ VL = 1/DL
141 TSA(J) =T $ PX = PVTF{T,DL,1) $ DPT(J)=DPDT $ DPD(J)=DPDD
44
147 PSA{J) = PS = PSAT $ Z = PS/DL/G/T
148 PS=PS/10 $ DPSDT=DPSDT/10 $ 0PDT=DP0T/10 $ 0PDD=DPDD/10
149 DL=DL*WM $ DG=DG*WM $ OOLDT=ODLDT*WM $ DPDD = DPOD/WM
150 PRINT 5, T,PS, DL,DG, Z,ZG, DPSDT,DDLDT, DPDT,DPDD
C PAGE 2, TABLIQ. AVOID COEXIST, TIMESAVER.
C USE COEXIST AT ALL TEMPERATURES.
160 PRUJT 11 $ DO 180 J=1,NP $ T = TSA(J) $ P = PSA(J)
161 CALL COEXIST $ DL = DEN $ IW = W
162 DIEL = DIELF(DL,T,P) $ QX = QVAPXF(T)
C GET FUGACITY COEF., (F/P), VIA HZ, SZ, HG, SG.
C NOTE, DI = 0.00001 MOL/L IN EDELF.
170 GIBS = HG-EZZ-HZ - T*(SG-SZ)
171 GO = 100*G $ XP = EXP(GIBS/GJ/T) $ FOP = XP*1.01325/P
172 IF(DNG.LE. 0.00001) FOP = 1.0
180 PRINT 12, T,QX, E,H,S, CV,CSAT,CP, FOP, IW, DIEL
999 RETURN $ END
SUBROUTINE THERMO
C FOR COMPUTATION AT ANY (T,P) POINT.
C ASSUMES AN ISOTHERM IN SINGLE-PHASE ONLY.
C CASES FOR ISOTHERMS BELOW, EQ., ABOVE TCRT,
C GIVEN (T,P), RETURNS DEN, E,H,S, CV,CP,W, DPDT, DPDD.
C ENTRIES BELOW FOR PHASE BOUNDARIES ASSUME A GIVEN ISOBAR P, OR -
C ENTRIES BELOW FOR PHASE BOUNDARIES ASSUME A GIVEN ISOTHERM, T.
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT, TCRT, PORT, DGAT ,DTRP ,TTRP ,PTRP
C0MM0N/3/DPDT,D2PDT2,DPSDT,DPMDT,DPDD,DPDR,DTSDR,DTHDR,DDSnT
COMMON/9/ DNG,EG,HG,SG, CVG,CPG,WG, DPGDT,DPGDD
1 FORMATdHO 9X *THERMO, P.GE.PMELT. * / )
2 FORMATdHO 9X *THERMO DOUBLE-VALUED AT P = PSAT. * / )
3 FORMATdHO 9X *THERMO, DEN GE. DCRT AT T = TCRT. * / )
10 IF(T-TCRT) 11,20,25
C SUBCRITICAL ISOTHERMS.
11 PM = PMELTF(T) $ IF(P.GE.PM) 12,13
12 PRINT 1 $ CALL COMPRLQ $ TI=T $ CALL IDEAL $ RETURN
13 PS = PSATF(T) $ IF(P-PS) 14,15,16
15 PRINT 2 $ RETURN
16 CALL COMPRLQ $ TI = T $ CALL IDEAL $ RETURN
C THE CRITICAL ISOTHERM.
20 CALL GENEOUS $ IF(DEN.LT.DCRT) RETURN
21 CP = CV = W = 0 $ PRINT 3 $ RETURN
C ISOTHERMS AT T ABOVE TCRT.
C THERMOM FOR GIVEN ISOBAR AT THE MELTING LINE, GET T.
C RETURNS T,DEN, E,H,S, CV,CP,W, DPMDT, DPDT, DPDD.
ENTRY THERMOM
40 T = FINDTMF{P) $ PM = PMELTF(T) $ CALL COMPRLQ
41 TI = T $ CALL IDEAL $ RETURN
C THERMOL FOR GIVEN ISOBAR AT SATURATED LIQUID LINE, GET T.
C RETURNS T,DEN, E,H,S, CV ,CP ,CSAT,W, DPSDT,DDSDT, DPDT, DPDD.
ENTRY THERMOL
43 T = FINDTSF(P) $ CALL COEXIST $ RETURN
45
,
C THERMOV FOR GIVEN ISOBAR AT THE SATURATED VAPOR LINE, GET T.

C RETURNS T,DEN, E,H,S, CV,CP,W, DPSDT,DDSDT, DPDT,DPDD.
ENTRY THERMOV
45 T = FINDTSF(P) $ CALL COEXIST $ DEN=DNG $ E=EG $ H=HG $ S=SG
47 CV=CVG $ CP=CPG $ W=WG $ DPDT=DPGDT $ DPDD=DPGDD $ RETURN
C THRMM FOR ISOTHERM AT THE MELTING LINE, GET P.
C RETURNS P,DEN, E,H,S, CV,CP,W, DPMDT, DPDT, DPDD.
ENTRY THRMM
50 P = PMELTF(T) $ CALL COMPRLQ $ TI=T $ CALL IDEAL $ RETURN
C THRML FOR ISOTHERM AT SAT. LIQ. LINE, GET P.
C RETURNS P,DEN, E,H,S, CV ,CP ,CSAT ,W DPSDT,DDSDT, DPDT, DPDD.
,
ENTRY THRML
55 P = PSATF(T) $ CALL COEXIST $ RETURN
C THRMV FOR ISOTHERM AT SAT. VAPOR LINE, GET P.
C RETURNS P,DEN, E,H,S, CV,CP,W, DPSDT,DDSDT, DPDT, DPDD
ENTRY THRMV
60 P = PSATF(T) $ CALL COEXIST
61 DEN=DNG $ E=EG $ H=HG $ S=SG $ CV=CVG
62 CP=CPG $ W=WG $ DPDT=DPGDT $ DPDD=DPGDD
99 RETURN $ END
FUNCTION THETAF{DEN)
C THETA = TSAT*EXP(U(S)).
C LET Q = (S-1)/(ST-1) WHERE ST = DTRP/DCRT, THEN -
,
C IF S < 1, U = AL*Q**3, IF S > 1, U = -AL*Q**3

COMMON/l/AL BE ,GA ,DE EP ET DCRT ,f CRT PORT DGAT ,'dTRP TTRP PTRP
, i , , , , , ,
C0MM0N/3/DPDT,D2PDT2,DPSDT, DPMDT, DPDD, DPDR,DTSDR,DTHDR,DOSDT

1 S = DEN/DCRT $ DSDR = DTRP/DCRT $ C = DSDR-1
2 Q = (S-l)/C $ Q2 = Q*Q $ U = AL*Q*Q2
3 Ul = AL*3*Q2*DSDR/C $ IF{Q) 5,9,4
4 U = -U $ Ul = -Ul
5 XP =
EXP(U) $ THETAF = TSAT*XP
6 DTHDR = (TSAT*U1 + DTSDR)*XP $ RETURN
9 THETAF = TCRT $ DTHDR =0 $ RETURN $ END
FUNCTION TSATF(DEN)
C ITERATE T TO MINIMIZE (DEN-DCALC) VIA DENGASF(T), DENLIQF(T).
C IF ITERATION FAILS, PRINTOUT ONCE ONLY AND STOP AT K = 2.
COMMON/l/AL, BE, GA,DE,EP,ET, DCRT, TCRT, PORT, DGAT ,DTRP TTRP PTRP , ,
C0MM0N/3/DPDT ,D2PDT2 ,DPSDT DPMDT DPDD ,DPDR ,DTSDR DTHDR ,DDSDT

, , ,
DATA (Q=2.0) ,(FN=6. 3890561)

C NOTE, FN # EXP{Q) - 1.0.
1 FORMATdHl 14X *TSATF(DEN) FAILS AT DEN =* E15.7//
1 15X 5HDCALC 13X2HDD 10X5HDDSDT 13X2HDT 12X3HT,K )
2 F0RMAT(5X 5E15.7)
3 K = 0 $ D = DEN
4 S = D/DCRT $ YN = TCRT/TTRP-1 $ IF(D-DCRT) 5,30,6
5 ST=DGAT/DCRT $ F=ALOG(S)/ALOG{ ST)*( (1-S)/(1-ST) )**2 $ GO TO 7
6 ST=DTRP/DCRT $ U=( S-l)/( ST-1) )**3 $ F=( EXP(Q*U)-1)/FN
(
7 T = TCRT/(YN*F+1)
8 DO 20 J=l,50 $ IF(D-DCRT) 9,30,10
9 DC = DENGASF(T) $ GO TO 11
10 DC = DENLIQF(T)
46
11 DD = D - DC $ IF(ABS(DD/D) .LT.l.OE-7) 25,12
12 DT = DD/DDSDT $ IF(ABS(DT/T) .LT.l .OE-7) 25,13
13 T = T + DT $ IF(T) 14,14,15
14 T = TTRP $ GO TO 18
15 IF(T.LT.TCRT) 18,16
16 T = TCRT - 0.05
18 IF(l<.EQ.l) PRIMT 2, DC, DD, DDSOT, DT, T
20 CONTINUE $ K = K+1 $ IF(K.NE.l) STOP
21 PRINT 1, DEN $ GO TO 4
25 TSATF = T $ DTSDR = DTRP/DDSDT $ RETURN
30 TSATF = TCRT $ DTSDR = 0 $ RETURN $ END
FUNCTION XBF{T,D)
C XBF(R,T) # (X**BE)*EXP(A*(1-TS/T)) - XS**BE, WHERE -
C X # T/TC, XS # TS/TC, A # (1-BE) + SQRT(l-BE),
C XBF = U*EXP(A*V) - US, U # X**B, US # XS**B, V # (1-TS/T).
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT, TCRT, PORT, DGAT,DTRP ,TTRP ,PTRP
C0MM0N/3/DPDT ,D2PDT2 ,DPSDT ,DPMDT ,DPDD ,DPDR, DTSDR ,OTHOR ,DDSDT
C0MM0N/4/XBl,XB2, XC1,XC2, XE1,XE2, DXBDR,DXCDR ,DXEDR
COMMON /6/ TSAT, THETA, PSAT
1 B = BE $ BN = 1-B $ A = BN + SQRT(BN)
2 TC=TCRT $ TS=TSAT $ X=T/TC $ XS=TS/TC $ XS1=DTSDR/TC
3 U = X**B $ Ul = B*U/X $ U2 = -BN*U1/X
4 US = XS**B $ USl = B*US*XS1/XS
5 V = 1-TS/T $ VIR = -DTSDR/T $ VIX = TS/T/X $ V2X = -2*V1X/X
6 P = EXP(A*V) $ PI = A*P $ P2 = A*P1
7 PIR = P1*V1R $ PIX = P1*V1X $ P2X = P1*V2X + P2*V1X*V1X
8 XBF = U^P - US $ XBl = U*P1X + U1*P
9 XB2 = U*P2X + 2*U1*P1X + U2*P $ DXBDR = U*P1R - USl
10 RETURN S END
FUNCTION XEF(T,D)
C ULTRA REVISION, MARCH 29, 1981.
C XEF = H(R,T)/HS(R) - 1.0,
C H(R,T) # 1 - {W-WE/E)/1-1/E) E = ET.
,
C X#T/TC, F#TS/T, W#(1-TH/T), WE#W**E

C A = DE, B = 1-A, C = EP, E = ET.
C0MM0N/1/AL,BE,GA,DE,EP,ET, DCRT,TCRT,PCRT, DGAT,DTRP,TTRP,PTRP
C0MM0N/3/DPDT,D2PDT2,DPSDT,DPMDT,DPDD,nPDR, DTSDR, DTHDR,DDSDT
C0MM0N/4/XBl,XB2, XC1,XC2, XE1,XE2, DXBDR ,DXCDR,DXEDR
1 E = ET S EK = E/(E-1) $ TC = TCRT
2 TS = TSAT $ TH = THETA $ X = T/TC
3 W = 1.0 - TH/T $ IF(W) 30,30,4
4 CONTINUE
5 WIR = -DTHDR/T $ WIX = TH/T/X $ W2X = -2*W1X/X
6 WE = W**E $ WEI = E*WE/W $ WEIR = WE1*W1R
7 WEIX = WEI^WIX $ WE2X = WE1*W2X + E-1 )*WE1*W1X*W1X/W
{
8 H = 1 - EK*{W-WE/E) $ HIR = -EK*( WIR-WEIR/E)

9 HIX = -EK*(W1X-WE1X/E) $ H2X = -EK*{ W2X-WE2X/E)
10 WS = 1.0 - TH/TS $ IF(WS) 11,11,12
11 HS = 1 $ HSl = 0 $ GO TO 16
12 WSl = (TH*DTSDR/TS - DTHDR)/TS
13 WSE = WS**E $ WSEl = E*WSE*WS1/WS
47
14 HS = 1 - EK*{WS-WSE/E) $ HSl = -EK*( WSl-WSEl/E)
16 U = 1.0/HS $ UlR = -U*HS1/HS
17 P = H*U $ DXEDR = H*U1R + 'rllR*U
18 XEl = H1X*U $ XE2 = H2X*U $ XEF = P --1 $ RETURN
30 XEF = XEl = XE2 = DXEDR =0 $ RETURN $ END
48
o
ooooooooo
oooooooo
O0h-(OIO^COC>JT-
49
100 200 300 400 500 600
Temperature, K
Figure 2. P-T locus of P-p-T data for normal butane.
50
1 , ) 1 .
Table 1, Comparisons of vapor pressure data with eq (2).

Data sources and ID numbers (UAston, (2)8eattie, ( 10)Dana , (19)Kay, (29)Sage, (35)Wackher,
:
(37)Connol ly. (95)Seibert, (96)Carruth (97)Hirata, (98)Tickner, (99)De laplace, (40)Thermal

Loops.
ID Weight Temp. T/Tc P(j(expt) Pg ( ca c 1 Di ff dPa/dT
K MPa MPa % MPa/K
40 1.000 134.860 .31720 .67437E-06 .67358E-06 .12 .128E-06
40 1 .000 140.000 .32929 . 17216E-05 . 17210E-05 .03 .301E-06
40 1.000 145.000 .34105 .39908E-05 .39917E-05 -.02 .646E-06
40 1.000 150.000 ,35281 .86893E-05 .86943E-05 -.06 .130E-05
40 1 .000 155.000 .36457 .17884E-04 . 17897E-04 -.07 .249E-05
40 1 .000 160.000 .37633 .34986E-04 .35012E-04 -.07 .453E-05
40 1 .000 165.000 .38809 .65366E-04 .6541 lE-04 -.07 .789E-05
40 1.000 170.000 .39985 .1 1714E-03 .11721E-03 -.05 .132E-04
40 1.000 175.000 .41161 .20212E-03 .20220E-03 -.04 .213E-04
40 1.000 180.000 .42337 .33690E-03 .33697E-03 -.02 .333E-04
40 1.000 185.000 .43513 .5441 1E-03 .5441 1E-03 -.00 .505E-04
40 1.000 190.000 .44689 .85368E-03 .85357E-03 .01 .745E-04
40 1 .000 195.000 .45865 .13044E-02 .13040E-02 .03 .107E-03
1 1 .000 195.107 .45890 .13200E-02 .13155E-02 .34 .108E-03
40 1.000 200.000 .47041 . 19449E-02 .19442E-02 .04 .151E-03
40 1.000 205.000 .48217 .28356E-02 .28345E-02 .04 .208E-03
40 1.000 210.000 .49393 .40497E-02 .40479E-02 .04 .281E-03
1 1.000 212.668 .50021 .48340E-02 .48572E-02 -.48 .327E-03
40 1.000 215.000 .50569 .56740E-02 .56716E-02 .04 .372E-03
40 1.000 220.000 .51745 .78102E-02 .78075E-02 .03 .486E-03
40 1 .000 225.000 .52921 .10576E-01 .10574E-01 .03 .625E-03
1 1 .000 226.276 .53221 .1 141 lE-01 .11396E-01 .13 .565E-03
40 1.000 230.000 .54097 .14106E-01 .14104 E-01 .01 .792E-03
40 1 .000 235.000 .55273 .18550E-01 .18550E-01 .00 .992E-03
1 1 .000 235.822 .55467 .19409E-01 .19379E-01 .15 . 103E-02
40 1.000 240.000 .55449 .24076E-01 .24079E-01 -.01 .123E-02

40 1 .000 245.000 .57625 . 30869 E-01 .30877E-01 -.03 .150E-02
1 1 .000 246.51 .57981 .33268E-01 .3321 1E-01 .17 .159E-02
40 1 .000 250.000 .58801 .39131E-01 .39147E-01 -.04 . 182E-02
40 1 .000 255.000 ,59977 .49080E-01 .49 106 E-01 -.05 .218E-02

1 1.000 256.204 .60261 .51832E-01 .51782E-01 . 10 .227E-02
40 1 .000 260.000 .611 53 .60950E-01 .60989E-01 -.06 .259E-02
1 1 .000 262.267 .61 687 .67106E-01 .67078E-0 .04 .279E-02
40 1 .000 265.000 .62329 .74991 E-01 .75047E-01 -.07 .305E-02
1 1.000 266.789 .62750 .80656E-01 .80655E-01 .00 .322E-02
40 1 .000 270.000 .63506 .91469E-01 .91543E-01 -.08 .356E-02
1 1 .000 270.397 .63599 .92943E-01 .92966E-0 -.02 .360E-02
1 1 .000 272.027 .63982 .98952E-01 .98989E-01 -.04 .379E-02
1 1 .000 272.806 .64 165 .10193E+00 .10197E+00 -.05 .388E-02
29 1 .000 294.260 .69212 .21580E+00 .21562E-K)0 .08 .691E-02
29 1 .000 327.590 .77051 .55660E+00 .5 5724 E+OO -.11 .141 E-01
97 1 .000 333.130 .78354 .64017E+00 .63961 E+OO .09 . 156E-01
97 1 .000 336.420 .79128 .69357E+00 ,69259E+00 .14 . 166E-01
19 1.000 336.480 .79142 .68950E+00 .69359E+00 -.59 . 166E-01
97 1 .000 340.940 .80191 .76916E+00 .77056E+00 -.18 .179E-01

97 1.000 343.070 .80692 .80878E+00 .80946E+00 -.08 . 186E-01
29 1.000 344.260 .80972 .83420E+00 .83180E+00 .29 .190E-01

97 1.000 344.710 .81078 .83836E+00 .84037E+00 -.24 . 191E-01
19 1.000 345.650 .81299 .86180E+00 .85848E+00 .39 .194E-01

2 1.000 348.140 .81884 .90790E+00 .90782E+00 .01 .202E-01
97 1 .000 348.660 .82007 .91476E+00 .9 1838 E+OO -.39 .204 E-01
97 1 .000 348.990 .82084 .92571 E+OO .92513E+00 .06 .205E-01
97 1 .000 352.640 .82943 .99917E+00 .10022E+01 -.30 .217E-01
19 1 .000 353.870 .83232 .10342E+01 .10292E+01 .48 .222E-01
97 1 .000 355.080 .83517 .10550E+01 .10563E+01 -.12 .226 E-01
97 1.000 357.020 .83973 .10981E+01 .1 1008E+01 -.25 .233E-01
97 1 .000 359.020 .84444 .n475E+01 .1 1481E+01 -.05 .240 E-01
29 1.000 360.930 .84893 .12024E+01 .1 1946E+01 .65 .247E-01
97 1.000 361.140 .84942 .1 1995E+01 .11998E+01 -.03 .248 E-01
19 1.000 361.210 .84959 .12066E+01 .12016E+01 .42 .248E-01
97 1.000 363.450 .85485 .12579E+01 .12581 E+01 -.02 .257E-01
97 1.000 365.700 .86015 .13144E+01 .13169E+01 -.19 .266E-01
97 1.000 366.620 .86231 .13399E+01 .13415E+01 -.12 .269E-01
97 1.000 367.850 .86520 .13746E+01 .13749E+01 -.02 .274E-01
19 1.000 367.980 .86551 .13790E+01 .13785E+01 .04 .275E-01
51
) . y 0 11 , .
1 1
Table 1. (Continued).
Data sources and ID numbers (l)Aston, (2)3eattie, ( 10)Dana1, (19)Kay, (29)Sage, (35)Wackher,
:
\5 1 uonno ,
I (yD)beiDerT, \ yo / uarruTri (97)Hirata, (98)Tickner, (99) De ap lace , (40)Thermal
I 1
Loops
ID Weight Temp. T/Tc Pg( expt) Pij(calc) Di f f dPrr/dT
K MPa MPa t MPa/K
97 1 .000 359.620 .86937 . 14225E+01 . 14240E+01 -. 1 .281 E-01
2 1 .000 373. 40 1 .87765 .15290E+01 .15256E+01 .22 .296E-01
97 1 .000 373.580 .87868 .15385E+01 .15386E+01 -.01 .298E-01
19 1 .000 373.980 .87962 .15513E+01 .15506E+01 .05 .299E-01
97 1 .000 375 .040 .8821 .15785E+01 .15826 E+01 -.25 .304 E-01
97 1 .000 377.240 .88729 . 16505E+01 . 16505E+01 -.00 .314E-01
19 1 .000 379 .430 .89244 . 17237E+01 . 17202 E+01 .20 .323 E-01
19 1 .000 384.710 .90486 .18961E+01 . 18974E+01 -.07 .348 E-01
97 1 .000 385.710 .90721 .19319E+01 .19324 E+01 -.03 .353 E-01
19 1.000 389.370 .91582 . 20684 E+01 .20648E+01 .17 .371 E-01
97 1.000 391 .010 .91968 .21239E+01 .21263E+01 -. 12 .379E-01
97 1 .000 396.090 .93163 .23251E+01 .23259E+01 -.03 .407E-01
2 1 .000 398, 140 .93645 .24207E+01 .24104 E+01 .43 .418E-01
97 1 .000 401 .300 .94388 .25465E+01 .25455E+01 .04 .437E-01
2 1 .000 423. 140 .99525 .36730E+01 ,36696 E+01 .09 .612E-01
10 0.000 255.030 .59984 .49620E-01 .49171E-01 .91 .218E-02

10 0.000 260.490 .61269 .62230E-01 ,62266E-01 -.06 .263 E-02
10 0.000 271 .350 .63823 .97540E-01 ,96451E-01 1.13 .371 E-02
10 0.000 272.960 .64202 .10172E+00 .10257E+00 -.83 .389 E-02
10 0.000 272.960 .64202 .10230E+00 . 10257E+00 -.26 .389 E-02
10 0.000 283.420 .66662 .15040E+00 .15007 E+00 .22 .523 E-02
10 0.000 290.530 .68346 .19330E-K)0 .19130E+00 1 .04 .631 E-02
10 0.000 29 1 . 9 1 .68659 .19520E+00 .19984 E+00 -2.32 .652 E-02
10 0.000 298.690 .70254 .25000E+00 .24794E+00 .83 .769E-02
10 0.000 304.860 .71705 .30320E+00 .29894 E+00 1 .42 .886E-02
10 0.000 31 0.280 .72980 .35210E+00 ,3499&E+00 .61 .998E-02
10 0.000 314.420 .73953 . 39690 E+00 ,39313E+00 .96 .109E-01
10 0.000 322.080 .75755 .48140E+00 ,48338E+00 -.41 . 127E-01
10 0.000 TOO r\Ci r\

322.080 .75755 .48640E+00 ,48338E+00 .62 . 27 E-0
1
10 0.000 322. 50 1 .75771 .48930E+00 ,48427E+00 1.04 .127E-01

10 0.000 330. 100 .7764 .59080E+00 ,593 52 E+00 -.46 .148E-01
10 0.000 330. 100 .77641 .59770E+O0 ,59352E+00 .70 .148E-01
10 0.000 330.630 .77766 .60010E+00 ,60140E+00 -.22 .149E-01
10 0.000 330.630 .77766 .60480E+00 ,60140E+00 .57 .149E-01
19 0.000 325.040 .76451 .51710E+00 ,52209 E+00 -.96 .135E-01
29 0.000 310.930 .73132 .35180E-K)0 ,35649E+00 -1.31 .101E-01
35 0.000 205.450 .48323 .31300E-02 . 29293 E-02 6.85 .214E-03
35 0.000 213. 150 .50134 .56700E-02 ,50169E-02 13.02 .336E-03
35 0.000 228. 50 1 .53662 .13280E-01 .12699E-01 4.57 .727E-03
35 0.000 241 .850 .56884 .27650E-01 ,26436E-01 4.59 .132E-02
35 0.000 250.450 .58907 .41450E-01 ,39970E-01 3.70 .185E-02
35 0.000 255.450 .60083 .51260E-01 ,50093E-01 2.33 .221 E-02
35 0.000 261 .850 .61589 .66390E-01 .65923E-01 ,71 .275 E-02
35 0.000 266.050 .62576 .78570E-01 ,78300E-01 .35 .315E-02
35 0.000 273. 150 .64246 .10338 E+00 .10331 E+00 ,06 .392E-02
35 0.000 278.750 .65564 .12732E+00 .12713E+00 .15 .460E-02
37 0.000 344.260 .80972 .83086E+00 .83180E+00 -.11 .190E-01
37 0.000 360.930 .84893 .1 1946E+01 .1 1946E+01 -.00 .247E-01
37 0.000 377.590 .8881 .16638 E+01 .16615E+01 .14 .315E-01
37 0.000 394.260 .92732 .22575E+01 .22524E+01 .23 .397 E-01
37 0.000 406.870 .95698 .28 037 E+01 .2798 5 E+01 .18 .472E-01
37 0.000 410.930 .96653 .300T3E+01 .29959E+01 .18 .501 E-01
37 0.000 425. 120 .99991 .3784 5 E+01 .37934 E+01 -.24 .642 E-01
95 0.000 303. 150 .71303 .34000E+00 .28408E+00 19.68 .853E-02
95 0.000 313. 150 .73655 .44660E+00 .37949E+00 17.69 .106E-01
95 0.000 323. 150 .76007 .57330E+O0 .49712E+00 15.33 .130E-01
95 0.000 333. 150 .78359 .71990E+00 .63992E+00 12.50 .156E-01
95 0.000 343.150 .8071 .89330E+00 .81095E+00 10.16 .186E-01
95 0.000 363. 150 .85415 .14265E+01 .12505E+01 14.08 .256E-01
95 0.000 373. 150 .87767 .16665E+01 ,15259E+01 9.22 .296E-01
95 0.000 383. 150 .901 19 . 19598E+01 ,18437 E+01 6.30 .341 E-01
95 0.000 393.150 .92471 .24131 E+01 ,22087E+01 9.25 .391 E-01
95 0.000 403.150 .9482_ .27464E+01 .26274 E+01 4.53 .448 E-01
96 0.000 135.430 .31854 .90230E-06 .75036E-06 20.25 . (41E-06
52
. 1
Table 1. (Cont nued )

i
Data sources and ID numbers: (l)Aston, (2)Beattie, (lO)Oana, 19)l<ay, (29)Sage, (35)Wackher,
(
(37)Connol ly, (95)Seibert, (96)Carruth, (97)Hirata, (98)Tickner, 99) De ap ace , (40)Thermal ( I I
Loops.
ID Weight Temp, T/Tc P„(expt) Prf(calc) Di ff. dPg/dT
K MPa MPa % MPa/K
96 0.000 137. 730 .32395 . 10800E-05 . 1 1483E-05 -5 .95 .208E-06
96 0.000 138.930 .32677 . 14490E-05 . M248E-05 1 .70 .254E-06
96 0.000 146. 320 .344 15 . 51 320E-05 .493 1 1 E-05 4.08 .78 E-061
A 11
96 0.000 148. 100 .34834 .678 OE-05
1 .651 32t-05 4.11 . lOOE-05
96 0.000 1 54.840 .36419 . 18450E-04 . 17503E-04 5. 4 . 244 E-05

96 0.000 1 59.790 .37583 .32260E-04 .3407 E-04 1 -5.32 .442E-05
96 0.000 171 .430 .40321 . 12590E-03 . 13750E-03 -8.44 . 52 E-04
1
96 0.000 184.090 .43299 .4do50E-03 .49978t-03 -2.64 .469 b-U4

96 0.000 194 .650 .45783 . 12420E-02 . 25d9E-02
1 -1 .97 . 105E-03
96 0.000 196.710 .46267 . 5390E-02

1 . 4988t-02
1 2.68 .121E-03
96 0.000 205.270 .48281 .31320E-02 .28910E-02 8.33 .21 E-031
96 0.000 209.280 .49224 .37740E-02 .38501 E-02 -1 .98 .269E-03

96 0.000 212.900 .50075 .49480E-02 .49335E-02 .29 .331 E-03
98 0.000 135.850 .31953 .66660E-06 .81 196E-06 -17.90 . 152E-06
98 0.000 139.950 .32917 . 3330E-05

1 . 17060E-05 -21 .86 .299E-06
98 0.000 144.250 .33928 .26660E-05 .35332E-05 -24.54 .578E-06
98 0.000 149.950 .35269 .66660E-05 .86294E-05 -22.75 . 129E-05
98 0.000 154.750 .36398 . 13330E-04 . 17284E-04 -22.88 .241 E-05

98 0.000 159.850 .37598 .26660E-04 .34338 E-04 -22.36 .445E-05
98 0.000 166.950 .39268 .66660E-04 .82509E-04 -19.21 .969E-05
98 0.000 172.850 .40655 . 13330E-03 . 16065E-03 -17.02 . 174 E-04
98 0.000 179.250 .42161 .26660E-03 .31277E-03 -14.76 .312E-04

98 0.000 188.450 .44324 .66660E-03 .74455E-03 -10.47 .663E-04
98 0.000 195.850 .46065 . 13330E-02 . 3979E-02
1 -4.64 . 14E-03
1
99 0.000 135. 1 50 .31788 . 17330E-05 .71 170E-06 143.50 . 135E-06
99 0.000 136. 1 50 .32023 .20000E-05 .85875E-06 132.90 . 160E-06
99 0.000 137. 150 .32258 .22660E-05 . 10330 E-05 119.36 . 189E-06
99 0.000 138. 150 .32494 .25730E-05 . 12390E-05 107.67 .223E-06

99 0.000 139. 150 .32729 .30000E-05 . 14816E-05 102.48 .263 E-06
99 0.000 140.150 .32964 .39060E-05 .17667E-05 121.09 .308E-06
99 0.000 142.150 .33434 .45330E-05 .24913E-05 81 .95 .421 E-06
99 0.000 143.150 .33670 .53330E-05 .29465E-05 80.99 .491 E-06
99 0.000 144.150 .33905 .62000E-05 .34758E-05 78.38 .570 E-06
u.uuu • /ZUUvJt:-U-5 /D.UO .DDUt-(JD
99 0.000 146.150 .34375 .83330E-05 .47998E-05 73.51 .763 E-06
99 0.000 147.150 .34610 .96790E-05 .56196E-05 72.24 .879E-06
99 0.000 148.150 .34846 .11332E-04 .65636E-05 72.65 .101 E-05
99 0.000 149.150 .35081 .14000E-04 .76483E-05 83.05 .1 16E-05
99 0.000 150.150 .35316 .17065E-04 .88917E-05 91 .92 . 133E-05
99 0.000 151.150 .35551 .19865E-04 .10314E-04 92.60 . 152E-05
Number of data points used in fit = 80; rms pressure deviation = 0.189^.
53
1 51 /
1 1 4
11 /
11
1 0
6
0
4
8
4
5
Table 2. Comparisons of saturated liquid density data with eq (3).
Data sources and ID numbers: (2)Carney, (7)Coffin, (8)Connolly, (lO)Dana, (15)Foehr,

( 17)Benol iel , (18)Kahre, (19)Kay, (25)0lds, (29)Sage, ( 32) S w nsk , (33)NGAA, (90)Haynes, I i i
i
(91)0rrit, (92)McClune, (93)Van der Vet.
1 n
U we y nT Temp • (T^ T\/<T Pi o n c
U"n i>
1 "t" \/
( expt) U TT. /Ha. /HT
1 1
1 I
y 1
IS mo // L
rrw~» 1
1
1 k
IN
-1 /fii3
J/ flM p Ky/ ^ m-^»is 1
90 1
1
AAA
.000 1
1
T C;
35.0 A"7 K
ID .yyyzo 1 O CO C 11
"7"^
/35.3 It. c; A~7 Ayl
.04 C\A A
- .944 \
1
O 1 1
1
AAA
.000 1
1
"^Q A^
JO .04 1
1 •yoyu4 1
1
1
Z •
c^QR
0^0 AQ ! DZ %/Li A"^ Q/l ICS
90 1
1
AAA
.000 1 A A~7 c
140.0/3
yi A OOA
.yo.d04 >1
/30.OD Ay!
.04 Ayl OT
-•y4^3
n 1 1
1
AAA
.000 1
1
/IA/1 n
4zo .04y .y /5/4 I Z • DDZ "700
/<CO
AO
.4Z /zo .49 A
-.01 1
y4 1 Q
-. CiA 1
no
92 1
1
AAA
.000 1
1
^
43. CA
"Z
PO 1
1
at i A A
• 9 /144 1 Z. 31
"70"7
1 Z 1 ,5o 1 Z 1 .40
A1
-.01 y4 c
- . Ayl 1
1
An
90 1
1
AAA
.000 Â c A"?
145.0/3 c;
•yoHo 1
1
O •4yz
z ACi'~> ~70(^ AO
izo* oy /z 0-?
A^
.00 - . y4
Qyl A 1
1
91
1
1
AAA
.000 14/. loo AC cyt "7
•y554 1 z .44
"70 "Z 11
iZ5» 1 /z J .1)9 AA
.00 Ayl Ayl
-.y404
"7-1 O 1 u. AA - . 94 04
92 1 .000 148 . 50 1 .95422 1 2»435 722 .76 .00
90 1 .000 1 50.075 .94759 1 2»409 72 . 28 1 720.94 .05 -.9401
92 1 .000 1 53. 50 1 .93700 12 .357
~7 O OO
718.22
1 T 0
71 0
AC
1
.05 AO
.02 -.9397
91 1 .000 1 53.204 A"Z O 1
1 z»354
~7 O A
1
/ 0 .04
1
y1 T10
/
AA
0 .00
1
A1
.01 A "ZA "7
- .9597
90 1 .000 1 55.075 .93037 12 .330 716.67 7 6 .24
1 .06 -.9395
92 1 .000 158. 50 1 .91977 1 2.276 71 3.53 71 3.36 .02 -.9394
ICO COT A O OT
•91827 1 1 o ^cc T/ O Ayl
1
^.94
"7 1 '>
2 . r\A AA
-.00 -.9394
91 1 .000 158 . 587 1 / 1 94
90 1 .000 160.075 .91314 1 2.248 71 1 . 93 71 1 .55 .05 -.9394
92 1 .000 163. 1 50 .90255 1 2 . 96 1 708.87 708.65 .03 -.9395
91 1 .000 164.010 : .89959 12. 179 707.91 707.85 .01 -.9395
90 1 .000 165.075 .89592 12. 163 705.99 706.85 .02 -.9396
92 1 .000 168. 50 1 .88533 12.116 704.25 703.96 .04 -.9400
9 1 .000 169. 522 .88050 12.092 702.8 702.67 .02 -.9402
90 1 .000 170.075 .87869 12.084 702.37 702. 15 .03 -.9403
92 1 .000 173. 150 .86810 12.035 599. 55 699.26 .04 -.9409
91 1 .000 174.925 .85198 12.003 597.59 597.59 .01 - . 94 1
91 1 .000 180.442 .84298 11.915 692.52 692.39 .02 -.9431

91 1 .000 186.368 .82257 1 1 .8 17 686.88 585.79 .01 -.9456
1 O "70 C\
191 •789
1
.80390 .728 -.00 - . 94 84
9 1 .000 1 1 68 1 .66 68 .66 1
91 1 .000 1 97.248 .78509 1 1 .636 676.35 676.47 -.02 -.9519

91
1
1
AAA
.000 Z04 • ZOO .
"7ÂO
/60o4 yl 11
1 1
coo
. 522 009.08 569.75 A1
-.01 -.9572
y 1
1
1
AAA
. 000 ZUo •ZZ /
"7 A "70 "7
1 .458 1 665.96 665.98 AA
-.00 -.9606
O
y 1
1
1
1
AAA
.000 Z ^» o4o
1 »
"70"7AO
1 z. lyz
1
1
TÔ
»5oZ 1 A .4^
DOO o yi /CCA C/C
D00.5D AO
-•Oz -.9061
y 1
1
1
AAA
.000 O 1
1
TCI
Z 9»353 .
AO A C
"7
70895 1 OT
11.2/1 1 1 £CC
655. 14 1 yi ^CC
655. 23
0*7 A1
-•01 -,'9 IZZ
A~700
y 1
1
1
AAA
.000 ZZ4%^ /O C O A£ A
.68960 11
11.1/4 1 "7 yi
64y .45 C A
649.75 C C\ ~7 A^
".04 -.yA~7 A
/91 1
33 1 .000 226.820 .68322 1 143 1 . 647.70 647.93 -.04 -. 98 1
AAA O'ZA AAA "700*7 11 A A cc

a A A .00 a A A OA AO
yu 1
1 .000 Z30.000 mOiZZ/ 1 .091 1 D44 d44 .oU -•Oz -.yaoo
A
y 1
1
1
1
AAA
.000 O'Z T TA
z33.3y 1 ^C^f\ CA
.DD05y 1 1 .034 CLA
04 "^C
.35 1
1 04^ .45c
yr 1
1
yl no
-•Uz QO A
-. yy 1
1
AAA a coAc AAO CKO AA XZQ A Ayl Q

Z"Z 1
1 .000 O C Q "7A
Z35.0 /O .o5Z05 1
1
A
o.yy-i 638. yo 638. AO
yy A1
-.01 -.yy48
A"2
55 1. 000 238 .650 .64247 10.942 636. 00 636.22 -.03 -.9993
A
y 11 1
1
AAA
.000 24 1 . 557 .63245 10.892 633.07 633.31 -.04 A A "Z
-11 .0043 yi
91 1.000 247.21 .61 297 10.793 627.35 627.50 -.04 -1 .0146

33 1.000 247.760 . 6 11 09 10.791 627.20 627.04 .03 -1 .0157
91 1.000 252.249 .59553 10.702 522.05 622.46 -.07 -1 .0246
33 1.000 255.370 .58488 10.662 51 9.70 519.26 .07 -1 .0312
33 1.000 255.430 .58467 10.558 519.50 619. 19 .05 - 103 . 1
91 1.000 258.254 .57494 10.597 61 5.95 615.27 -.05 -1 .0377

91 1.000 263.785 .55589 10.496 6 1 0 . 09 6 1 0 . 50 -.07 -1 .0508
33 1.000 266.480 .54661 10.464 608.20 607.66 .09 -1 .0576
91 1.000 269.401 .53654 10.393 604. 1 604 . 56 -.07 -1 .0652
91 1. 000 274.973 .51735 10.289 598.05 598.58 -.09 -1 .0808
33 1.000 277. 150 .50985 10.259 596.30 596.22 .01 -1 .0873
32 1.000 283.200 .48901 1 0. 145 589.67 589.58 .01 -1 . 1064
90 1.000 288.706 .47004 10.033 583.13 583.44 -.05 -1 .1253

33 1.000 288.710 .47003 10.047 584.00 583.44 . 10 -1 .1253
90 1.000 290.000 .46559 10.007 581 .63 581 .98 -.06 -1 .1299
32 1.000 293.190 .45460 9.949 578.28 578.36 -.01 -1.1418
33 1.000 299.820 .43176 9.822 570.90 570.70 .04 -1 .1685
90 1.000 300.000 .431 14 9.810 570.22 570.49 -.05 -1 . 1693
32 1.000 303.150 .42029 9.752 566.82 566.79 .01 -1 .1829
33 1.000 310.930 .39349 9.597 557.80 557.44 .06 -1.2197
25 1.000 310.930 .39349 9.585 557.16 557.44 -.05 -1.2197
32 1.000 313.120 .38595 9.545 554.78 554.76 .00 -1.2309
33 1.000 322.040 .35522 9.363 544 . 20 543.56 .12 -1.2809
32 1.000 323.120 .35150 9.327 542.13 542.17 -.01 -1.2875
32 1.000 333.110 .31709 9.102 529.06 528.99 .01 -1 .3547
54
D
7 I • A 5 y 01 2 ) 1 1 3
3
11
Table 2. (Continued),

( 17)Benol iel , (18)Kahre, (19)Kay, (25)0lds, (29)Sage, (3:-? S wi nski , (33)NGAA, (90)Haynes, ) I i
(91 )Orr it. ( 92) McO une p (93)Van der Vet.

1
Weight Temp. ( rc-T)/( Ic-Tt) Dens ty 1 ( expt) Dens ty ( ca c

1 1 U 1 T T •
Â- / A'V
apj_/a 1
1
K mol/L kg/in3 kg/m3 % kg/(m3.K)
33 1 .000 333. 50 1 .31695 9. 108 529.40 528.93 .09 -1 .3550

32 1 .000 343.080 .28274 8.863 515.18 5 1 5 . 09 .02 -1 .4354
25 1 .000 344.260 .27868 8.833 51 3.4 51 3.39 .00 -1 .4450
32 1 .000 353.090 .24826 8.606 500.24 500. 24 -.00 -1 .5348
32 1 .000 363. 10 1 .21374 8.330 484.20 484.26 -.01 -1 .6603
32 1 .000 368. 100 .19656 8. 186 475.82 475.79 .01 -1 .7360
25 1 .000 377.590 .16386 7.899 459. 1 458.51 .13 -1 .91 48
25 1 .000 410.930 .04902 6.405 372.26 373.21 -.25 -3.8043
2 0.000 227.594 .68055 11.131 647.00 647. 17 -.03 -.9825

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2 0.000 238.706 .64228 10.944 635. 10 635. 15 -.01 -.9994
2 0.000 244.261 .6231 10.849 530.60 530. 59 .00 - 1 . 009
2 0.000 249.817 .60401 10.755 525. 10 524 .95 .02 -1 .0197
2 0.000 255.372 .58487 10.662 619.70 61 9. 25 .07 - 1 . 03 1
2 0.000 266.483 .54660 10.464 508.20 607.55 .09 -1 .0576

277. 150 .50985 0.259 596.30 595.22 A1
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2 0.000 288.706 .47004 10.047 584.00 583.44 .10 -1 .1253
2 0.000 310.928 .39350 9. 597 557.80 557.45 •06 -1 .2197
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17 0.000 253.150 .59252 10.701 522.00 521.54 •07 -1 .0265
17 0.000 263.150 .55808 10.519 511.40 51 1 .16 .04 -1.0492
17 0.000 273.150 .52363 10.337 600.80 600.54 •04 -1.0756
17 0.000 283.150 .48918 10.147 589.80 589.64 • 03 -1.1062
17 0.000 293.150 .45474 9.955 578.70 578.40 .05 -1.1417
18 0.000 288.750 .46989 10.054 584.40 583.39 • 17 -1.1254
18 0.000 327.550 .33624 9.238 535.95 535.41 • 10 -1.3158
19 0.000 325.040 .34488 9.309 541.10 539.59 • 26 -1.2995
55
1 1 Q 11

( 17)Benol iel , ( 18)Kahre, (19)Kay, (25)0lds, (29)Sage, (32)SI iwinski , {33)NGAA, (90)Haynes,
(91)0rrit, (92)McClune, (93)Van der Vet.
ID Weight Temp. {Tc-T)/(Tc-Tt) Dens ty i ( expt) Density (calc) Diff. dP£,/dT

K mol/L kg/m3 kg/m3 % kg/(m3.K)
19 0.000 336.480 .30548 9.045 525.73 524.38 .26 -1.3802

19 0.000 345.650 .27389 8.827 513.07 51 1 .37 .33 -1 .4589
19 0.000 353.870 .24557 8.618 500.90 499.04 .37 -1.5436
19 0.000 361 .310 .21994 8.414 489.05 487.23 .37 -1 .6354
19 0.000 367.980 .19697 8.215 477.51 476.00 .32 -1.7341
19 0.000 373.980 .17630 8.031 466.78 465.29 .32 -1 .8404
19 0.000 379.430 .15753 7.854 456.53 454.95 .35 -1.9564
19 0.000 384.710 .13934 7.670 445.00 444.27 .34 -2.0925
19 0.000 389.370 .12329 7.493 435.54 434.19 .31 -2.2392
19 0.000 393.760 .10816 7.314 425. 13 424.00 .27 -2.4093
19 0.000 402.040 .07964 6.931 402.87 402.32 .14 -2.8669
19 0.000 405.870 .06645 6.730 391 .17 390.76 .10 -3. 1830
19 0.000 409.320 ,05456 6.529 379.48 379.15 .09 -3.5714
19 0.000 412.870 .04234 6.292 365.70 365.51 .05 -4.1501
19 0.000 415.980 .03162 6.046 351.44 351.47 -.01 -4.9439
19 0.000 419.260 .02032 5.743 333.83 333.05 .23 -6.4725
19 0.000 422.320 .00978 5.330 309.80 308.68 .36 -10. 1943
29 0.000 294.260 .45091 10.007 581 .64 577. 13 .78 -1 .1460
29 0.000 310.930 .39349 9.650 560.87 557.44 .61 -1.2197
29 0.000 327.590 .33610 9.301 540.61 536.36 .79 -1 .3161
29 0.000 344.260 .27868 8.919 518.40 513.39 .98 -1 .4460
29 0.000 350.930 .22125 8.449 491 .06 487.85 .66 -1 .6303
29 0.000 377.590 .16386 7.928 460.83 458.51 .51 -1 .9148
29 0.000 394.260 .10644 7.258 421.87 422.79 -.22 -2.431
91 0.000 135.366 .99826 12.640 734.70 734.79 -.01 -.9439
91 0.000 139.441 .98422 12.574 730.88 730.95 -.01 -.9425
91 0.000 144.783 .96582 12.489 725.91 725.92 -.00 -.941
91 0.000 150.530 .94602 12.397 720.55 720.52 .00 -.9400
91 0.000 155.930 .92742 12.310 715.48 715.44 .01 -.9395
91 0.000 161 .370 .90868 12.221 710.35 710.33 .00 -.9394
91 0.000 166.654 .89048 12.138 705.49 705.37 .02 -.9398
91 0.000 172. 198 .87138 12.047 700.24 700. 15 .01 -.9407
91 0.000 177.707 .85240 11.959 695.10 694.97 .02 -.9422
91 0.000 183.502 .83244 11.864 689.57 689.50 .01 -.9443
91 0.000 189.090 .81319 11.772 684.23 684.22 .00 -.9470
91 0.000 194.492 .79458 11.683 679.09 679.09 -.00 -.9501
91 0.000 202.744 .76616 11.544 670.99 671 .23 -.04 -.9559
91 0.000 205.434 .75689 1 .503
1 668.61 668.66 -.01 -.9582
91 0.000 21 1.023 .73764 1 1.41 663.23 663.29 -.01 -.9633
91 0.000 216.623 .71835 1 .318
1 657.86 657.88 -.00 -.9691
91 0.000 222.085 .69953 11.226 652.52 652.57 -.01 -.9755
91 0.000 230.623 .67012 11.083 644.16 644.19 -.00 -.9869
91 0.000 236.1 1 .65122 10.988 638.64 638.75 -.02 -.9952
91 0.000 244.335 .62289 10.844 630.28 630.51 -.04 -1 .0092
91 0.000 249.972 .60347 10.744 624.47 624.79 -.05 -1.0200
91 0.000 255.364 .58490 10.649 618.94 619.26 -.05 -1.0312
91 0.000 261.019 .56542 10.547 613.04 613.40 -.06 -1.0441
91 0.000 266.732 .54574 10.443 607.00 607.39 -.06 -1 .0582
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93 0.000 283. 150 .48918 10.130 588.80 589.64 -. 14 -1.1062

93 0.000 288.710 .47003 10.023 582.60 583.44 -.14 -1.1253
93 0.000 293.150 .45474 9.944 578.00 578.40 -.07 -1 . 1417
93 0.000 298.150 .43751 9.846 572.30 572.65 -.06 -1.1615
93 0.000 303.150 .42029 9.746 566.50 566.79 -.05 -1. 1829
93 0.000 308.150 .40307 9.641 560.40 560.81 -.07 -1.2061
93 0.000 313.150 .38584 9.538 554.40 554.72 -.06 -1.2311
93 0.000 318. 150 .36862 9.435 548.40 548.50 -.02 -1.2582
93 0.000 323.150 .35140 9.328 542.20 542.14 .01 -1 .2877
Number of data points used in f i t = 71; rms density deviation = 0.054^.
56
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58
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D1 5 A 1 , O
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1 Z ,
Table 4. Comparisons of second virial coefficients with eq (5).
Data sources and ID numbers: (2)Beattie (1939), (3)Beattie (1942), (4)Bottomley (1964),
(5)Bottom!ey (1977), ( 19)Kay, (25)0ids, (26)Gunn, (?7)Jones, (28)Kapal!o, (29)Sage,
(30)Kretsclimer, (31 )McGlashan, (32)Tripp, (33)Strein, (35)Das, (37)Connolly.
We g ht Temp. T /T Q
D Bp( expT) bp ( Cd C Di tt.
ID i
T/Tc 1
) D tt 1
w cm^/mo
IS %
OQ 1 r\f\(\ 9/1A
Z4'4 •
AA
UU ,9/4 - 1 9TA
1 Z_)U, A
UU Q99
A ,oZZ
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-4A ,090 A1 7 ,
T/I
34
4 1 •UUU 97X
Z / j.UuA<^ tkA 9
, D4Z
QQ 7/ ,uu
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9 lo 1
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133 T R
3,09
Zo 1 .UUU 97/ J • 4U
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,04 J 09^J , UU
-yZ AA -_),o O 1 -9,09o •
A9A
UZU RR
99
,
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1
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. UUU
90 A AA
ZoUoUU .opy A A9 AA
-yuz ,uu -9 , 9 JO -JT ,49UTA/I A^
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, UZU
RQ
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79 \ . UUU 9R^
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1 zy
j£. 1 nnn , ODD -Rfi9
OD^ oUU nn J•J1 y J , J9D , UH9 _ 1 OA
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1 nnn 9Qfi 1 n , O jD -7d^ nn -9Z,y Q 9 1
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71
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3U3.U4 71X AQ RJ.UU
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-Z,Do4 AOT
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3,4o y1
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31U.y4
1
. 73 1
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-/U/,dU Cf\ O , / /4
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"7~7 /I O £ 94
-Z,0 R /I A
-,119 1 1 A
-4, RA
50
zo 1
1
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.000 Z T AA
311
z.OO , /34 O
-0/4,00 AA yl o
-Z,d4Z o /I o czz
-z,533 AAA
-,009 Z^
-,36
35 1
1
AAA
.000 Z O A AA
3z0 .00 TCZ
,753 -d44 AA
C A A ,0U -2 , 524 O ,4A1/O
-Z -,048 -1 ,94
ZD 1
1
AAA
.UUU ZO
32 AA
.UU 1
1 .
7/55 CZ^5,UU
-o3 AA O ^ OA
-z,4oy O
-Z,458 RO /I ATI
-,031 1 O "7
-1,2/
32 1 .000 323.2 ,760 -599.00 -2.348 -2,418 ,070 2,88
32 1 .000 323.21 .760 -602.00 -2.360 -2,418 ,058 2,39
32 1 .000 323.21 ,760 -619.00 -2,426 -2,418 -,009 -,37
32 1 .000 323.21 ,760 -64 .00 1 -2,513 -2,418 -,095 -3,93
4 1 .000 323. 16 ,760 -606.00 -2,376 -2,419 ,043 1 ,78
4 1 .000 325.68 ,766 -595.00 -2,332 -2,374 ,041 1 ,74
33 1 .000 334 . 60 ,787 -555.70 -2, 178 -2,225 ,046 2,08
35 1 .000 340.00 ,800 -554,00 -2, 172 -2,141 -,031 -1 ,43
25 1 .000 344.27 ,810 -544,20 -2. 33 1 -2,078 -,055 -2,55
26 1 .000 344,30 ,810 -505,70 - .982
1 -2,078 ,095 4,60
4 1 .000 346.46 ,81 -522,00 -2.046 -2,047 ,001 ,04
33 1 .000 353, 10 ,831 -489.20 -1.918 -1 ,957 ,039 1 .99
35 1 .000 360,00 ,847 -48 .00 1 -1 .886 -1 ,869 -,017 -.90
27 1 .000 368.25 ,865 -443.49 -1 .738 -1 ,77 ,033 1.84
z7 1 .000 368.25 ,865 -444.20 -1 .74 -1 ,771 ,030 1.58
4 1
1
AAA
.000 370.86 ,872 -449 .00 -1 ,760 -1 ,742 -,018 -1 .06
Z/ 1
1
AAA
.UUU Z "7 Z OO
373, zZ O "TO
,878 -427.53 - 11 C ~1 c
,576 - 1 .716 ,040 2.32
Z/ 1
1
AAA
.UUU ZTZ OO 0"70
,878 -429. 50 - 1 ,684 -1 .716 ,032 .87
1
•z*z 1
1
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.UUU Z7
3/4, OA
ZU
>1
•ooUOOA >1 OA
-43Z 1 .oO 1
- 11 £AZ
,693 -11 ~7 A R
.705 A Z
,013 1
.73
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ZP 1
1
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3/ tz.r\ oc o
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-433.21
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-11 AO
,698 -1 .569 AO A
-, 029 - .74
1
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1
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.UUU Z7 7/,DU
3/ CA ooo
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1
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- ,640
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-1 .563 ,023 1 .40
Z/ 1
1
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3/0, O
lo
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,890 -4 8.00 1 -1 ,639 -1 ,563 ,025 1 .48
33 1
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3oU,UUAA oA yi ^ O
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1
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-.35 £i
•» -z
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1
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.UUU XQX QA
3y3, oU 09A
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-3o5.yu R Z
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-11 RIO
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-,UU 1
1
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-.00
4 1
1
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.UUU Z07/, 34
3y 1.A QT R z Q o AA
-3oy, UU -11 RO
jZjR Ô A
- ,4o
1
1 -, A
U49R /I Z A
-3.01 1
9"7
Z/ 1 AAA
« UUU
ZQQ
3yo, 14A 1 "Z7 A AO
-3 /U,UZ A RA
- ,450
1 7Z
-1 ,4/3 AO Z 1 RR
1 ,y3D 1
1 /I
,UZ3 1.55
97
Z/ 1
1
AAA
. UUU
Z QQ
3yo, 1A
14 ,y3o Z7^^
-3 AA
/D,UU 1
A ~l A
- 1 ,4/4 A' iX
- ,4/3
1
1 -, AA
UU 1 1 -. A/1
U4
35 1.090 400,00 ,941 -371,00 -1,454 -1,457 ,003 .20
26 1.000 410,90 ,966 -353,60 -1,386 -1 ,358 -,018 -1 .33
25 1.000 410,94 .967 -358,02 -1,403 -1,368 -.035 -2.62
33 1.000 413,00 ,971 -345.90 -1 .356 -1,352 -.004 -.31
35 1.000 420.00 .988 -329.00 -1.290 -1,299 ,010 .75
27 1.000 423. 14 .995 -325.61 -1 ,276 -1 ,277 .000 .04
27 1.000 423.14 ,995 -326,10 -1,278 -1,277 -.001 -.12
2 1.000 423. 16 ,995 -328,75 -1,289 -1 ,277 -.012 -.94
3 1.000 423,16 ,995 -328,70 -1,289 -1,277 -.012 -.92
4 1.000 426,37 1,003 -331,00 -1 ,298 -1 ,254 -.043 -3.45
26 1.000 427,60 1,006 -322,10 -1,263 -1,246 -.017 -1.35
59
11
Data sources and ID numbers: (2)3eattie (1939), (3)Beattie (1942), (4 ) Bottom ey (1964), I
(5)Bottomley (1977), ( 19)Kay, (25)Olds, (26)Gunn, (27)Jones, (28)Kapallo, (29)Sage,

(30)Kretschmer, (31 ) McG ashan , (32)Tripp, (33)Strein, (35)Das, (37 )Connol y.
I
I
ID Weight Temp. T/Tc B Br.(expt) Bp(calc) Diff. Diff.

K cm-" /mo 1
%
33 1.000 433.30 1.019 -314.30 -1 .232 -1,208 -.024 -2.02

35 1.000 440.00 1.035 -294.00 -1.152 -1.165 .012 1.06
25 1.000 444.27 1.045 -289,98 -1 . 137 -1.139 .002 .18
26 1.000 444.30 1.045 -293.40 -1.150 -1 . 1 39 -.012 -1.02
2 1.000 448.16 1.054 -286. 14 -1.122 -1.116 -.006 -.54
3 1.000 448,16 1,054 -287.30 -1. 126 -1.1 16 -.01 -.95
27 1.000 448, 18 1,054 -286.24 -1.122 -1.116 -.007 -.59
27 1.000 448.18 1,054 -284.80 -1.1 16 -1.116 -.001 -.08
26 1.000 460.90 1.084 -272.20 -1.067 -1.044 -.023 -2. 16
35 1.000 470.00 1.105 -250.00 -.980 -.997 .017 1.74
33 1.000 472.80 1.112 -253.30 -.993 -.983 -.009 -.96
2 1.000 473.16 1,1 13 -252.71 -.991 -.982 -.009 -.91
3 1.000 473. 16 1,113 -254,20 -.996 -.982 -.015 -1 .50
27 1.000 473,21 1,113 -255,50 -1.002 -.981 -.020 -2.05
27 1.000 473,21 1,113 -256,30 -1.005 -.981 -.023 -2.37
25 1.000 477,60 1,123 -237,28 -.930 -.960 .030 3.14
26 1.000 477,60 1,123 -245,90 -.964 -.960 -.004 -.38
33 1.000 498,00 1,171 -220,30 -.864 -.870 .006 .69
2 1.000 498,16 1,172 -223,37 -.876 -,869 -.007 -.77
3 1.000 498.16 1,172 -224,50 -.880 -,869 -.01 -1.28
27 1.000 498 70 1 77
. 1 -228. 48 - 077
27 1.000 498.20 1.172 -228.70 -.897 -,869 -.028 -3.19
35 1.000 500.00 1,176 -215.00 -.843 -,861 .019 2.16
26 1.000 510.90 1,202 -199.90 -.784 -,818 .035 4.22
25 1.000 510.94 1.202 -193.83 -.779 -.818 .039 4.72
2 1,000 523.16 1,231 -193.19 -.777 -.773 -.004 -.51
3 1.000 523,16 1,231 -198.10 -.777 -.773 -.004 -.47
35 1,000 530,00 1,247 -186.00 -.729 -.749 .020 2.67
35 1.000 560,00 1,317 -161.00 -.631 -,655 .024 3.68
2 1.000 573,16 1.348 -154.09 -.604 -,619 .015 2.38
3 1.000 573.16 1.348 -157.40 -.617 -,619 .002 .28
5 0.000 316,18 .744 -612.30 -2.400 -2.549 .149 5.85

5 0.000 341 ,49 .803 -518.90 -2.034 -2,119 .085 4,00
5 0.000 341,54 .803 -503.60 -1 .974 -2,1 18 .144 6,80
5 0.000 341,75 .804 -512.00 -2.007 -2,115 .108 5,11
5 0.000 341,83 .804 -513,30 -2.012 -2,114 .102 4,81
5 0.000 367,09 .863 -432,90 -1 .697 -1 .784 .087 4,90
5 0.000 367,13 .864 -432.30 -1 .695 -1.784 .089 5,00
5 0.000 367,83 .865 -435.30 -1.706 -1.776 .069 3,91
5 0.000 367,99 ,866 -429.70 -1.684 -1.774 .090 5.05
5 0.000 396,39 ,932 -368.60 -1 .445 -1.489 .044 2.94
5 0.000 396,46 .932 -367.60 -1.441 -1.488 .047 3.16
5 0.000 396,60 .933 -363.80 -1 .426 -1 .487 .061 4.08
5 0.000 427,88 1.006 -303.80 -1.191 -1.244 .053 4.26
5 0.000 427.88 1.006 -306.50 -1 .201 -1.244 .042 3.41
5 0.000 462.69 1.088 -248.60 -.975 -1.035 .060 5.84
5 0.000 462,86 1.089 -246.60 -.967 -1 .034 .067 6.51
5 0.000 463,32 1.090 -243.90 -.956 -1.032 .076 7.32
5 0.000 498,81 1.173 -213.90 -.838 -.866 .028 3.21
5 0.000 498,98 1.174 -201.40' -.789 -.866 .076 8.79
5 0.000 537,16 1.263 -167.10 -.655 -.725 .070 9.68
5 0.000 537,32 1.264 -160.50 -,629 -.725 .096 13.19
5 0.000 537,38 1.264 -158.10 -,620 -.725 .105 14.46
5 0.000 579,46 1.363 -125,90 -,494 -.602 .109 18.05
5 0.000 580,48 1.365 -124,60 -.488 -.600 .111 18.54
19 0.000 310,94 .731 -742,80 -2.912 -2.554 -.257 -9.69
19 0.000 338,72 .797 -585.19 -2,294 -2. 161 -. 133 -6. 18
19 0.000 366,49 .862 -502,69 -1,971 -1.791 -.179 -10.01
19 0.000 394.27 .927 -421.99 -1,654 -1.508 -. 147 -9.73
19 0.000 422.05 .993 -333.38 -1,307 -1.285 -.022 -1.73
19 0.000 449.83 1.058 -294.38 -1,154 -1 .106 -.043 -4.34
19 0.000 477.60 1.123 -257.05 -1,008 -.960 -.047 -4.93
60
1 . . / /
. ; A
0 9
Table 4. (Cont inued )
Data sources and ID numbers: (2)Beattie (1939), (3)Beattle (1942), (4 ) Bottom ay (1964), I
(5)Bottomley (1977), ( 19)Kay, (25)Olds, (26)Gunn, (27)Jones, (28)Kapallo, (29)3age,

(30)Kretschmer, (31 )McGlashan, (32)Tripp, (33)Strein, (35)Das, (37)Connol y. I
n We g ht Temp. T/T D Dp \ Co C n f n f
T f
1
1 U i D dpi ex p r 1
J u ;
1
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r T . U I
1 T .
cm^ /mo d
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1 .
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— ZU 1 . J^^7
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n uuu "iRft 79 1 . JO J 1oo 9Q
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n non n Qd
1
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n nnn ^77 fin 771 '^^ -9 "^4.0 - .u
n7fi
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n • uuu ^44 97 .O n
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n.onn .723 -667.00 -9.797
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31 0.000 368.40 .866 -440.00 -1.725 -1 .769 .045 2.52
J U« UUU J / / .yu .otsy -4 n
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U. on
1
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1
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1 - .boo
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3.53
31 0.000 387.60 .912 -383.00 -1 .501 -1 .569 .068 4.33
—' 1 0.000 400.40 .949 -353 on
J J J . (Jv - 1I . ^R4
JO^ 4S4
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4 ft9
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31 0.000 413.40 .972 -322.00 -1 .262 -1.349 .086 6.40
37 0.000 344.26 ,810 -517.00 -2.027 -2.078 .052 2.49
37 0.000 360.93 .849 -464.70 -1.822 -1.857 .036 1.92
37 0.000 377.59 .888 -418.60 -1.641 -1.669 .028 1.70
37 0.000 394.26 .927 -381 .30 -1 .495 -1 .508 .013 .86
37 0.000 406.87 .957 -356.10 -1.396 -1.400 .004 .29
37 0.000 410.93 .967 -348.60 -1 .367 -1.368 .001 .09
37 0.000 444.26 1.045 -289.80 -1.136 -1.139 .003 .24
Number of data points = 94; rms deviation = 2.11?.
61
Table 5. Behavior of coefficients of equation of state for
normal butane (eq (6)).
P/Pc To e Pg B(P) C(p)

K K MPa
.10 348,775 326.499 .9207 .45827 -.52914

.20 379.794 362.591 1.7320 .46342 -.44607
.30 397.551 385.396 2.3859 .47199 -.36821
.40 408.763 400.847 2.8891 .48399 -.29608
.50 415.972 41 1.292 3.2581 .49942 -.23011
.60 420.518 418.089 3.5131 .51828 -.17061
.70 423.211 422.177 3.6739 .54056 -.1 1780
.80 424.589 424.282 3.7597 .56628 -.07177
.90 425.091 425.053 3.7916 .59542 -.03254
1.00 425.160 425. 160 3.7960 .62800 0.00000
1.10 425.081 425.043 3.7909 .66400 .02603
1.20 424.595 424.287 3.7600 .70343 ,04583
1.30 423.384 422.351 3.6845 .74629 .05975
1.40 421 ,193 418.760 3.5526 .79258 .06819
1.50 417,816 413.115 3.3593 .84230 .07161
1.60 413,099 405.099 3.1062 .89544 .07053
1.70 406,927 394.485 2.8012 .95202 .06547
1.80 399,224 381.141 2.4561 1.01202 .05700
1.90 389,940 365.035 2.0860 1.07546 .04567
2.00 379,049 346,239 1.7079 1.14232 .03203
2.10 366,541 324.930 1.3394 1.21261 .01663
2.20 352,424 301.385 .9975 1.28633 .00000
2.30 336,719 275.985 .6976 1.36347 -.01738
2.40 319,471 249.196 .451 1 1.44405 -.03505
2.50 300,745 221.563 .2641 1.52806 -.05259
2.60 280,642 193.688 .1361 1.61549 -.06964
2.70 259,299 166.199 .0592 1 .70635 -.08588
2.80 236,894 139,716 .0205 1.80064 -.10103
2.90 213,646 1 14.817 .0052 1.89836 -.1 1488
3.00 189.803 91,993 .0008 1.99951 -.12724
3.10 165.632 71,616 .0001 2.10409 -.13800
3.20 141.394 53,922 .0000 2.21210 -. 14707
3,30 117.329 38,996 .0000 2.32353 -. 15442
62
63
)
Table 7. Comparisons of experimental P-p-T data of normal butane

with eq (6).
Summary of P-p-T data comparisons.
Authors
. —
T(K)
Range of Data
P(MPa) p( kg/m3
IMo.
Poi nts
of
Ap/p, rms
Dev at ions
i
AP/P,mean
(%) {%)
Beattie [31 423-573 1.5 - 36.3 29-494 115 0.54 0.56

Kay [441 311-589 0.2 - 8.3 5-513 437 0.50 0.43
Olds [51] 311-511 0.07- 68.9 1-632 209 0.27 1.18
Sage [64] 294-394 0.1 - 20.7 2-610 154 0.75 11.27
Haynes [351 140-300 1.7 - 36.1 572-745 105 0.06 4.55
Virial equation
(this report) 300-700 0.2 - 0.6 5.8 41 0.26 0.24
Total number of points used in fit = 907

Overall rms density deviation = 0.42?
Overall mean pressure deviation = \.09%
64
1 1
Table 7. (Continued)
Data sources and ID numbers: (l)Virial Equation, (3)Beattie, (19)Kay, (25)0lds, (29)Sage
(XXXX)Haynes.
ID Data Weight Temp. Dens ty

i Dens tyi Dens tyi
fêxpt ^ca c
1
Pressu
Point ex pt calc Diff. Diff.
No. K mol/L kg/m^ kg/m-5 i MPa MPa %
1 1.000 300.000 .100 5.81 5.78 .52 .2310 .2321 -.48

2 1.000 310.000 .100 5.81 5.79 .40 .2402 .241 -.38
3 1.000 320.000 .100 5.81 5.80 .30 .2493 .2500 -.28
4 1.000 330.000 .100 5.81 5.80 .20 .2583 .2588 -. 19
5 1.000 340.000 .100 5.81 5.81 .12 .2673 .2676 -.11
6 1.000 350.000 .100 5.81 5.81 .05 .2762 .2763 -.04
7 1.000 360.000 .100 5.81 5.81 -.02 .2851 .2850 .01
8 1.000 370.000 .100 5.81 5.82 -.07 .2939 .2937 .07
9 1.000 380.000 .100 5.81 5.82 -.11 .3027 .3024 .11
10 1.000 390.000 .100 5.81 5.82 -.15 .3115 .31 10 .15
1 1.000 400.000 .100 5.81 5.82 -.19 .3202 .3196 .18
12 1.000 410.000 .100 5.81 5.82 -.21 .3289 .3283 .21
13 1.000 420.000 .100 5.81 5.83 -.24 .3376 .3369 .23
14 1.000 430.000 .100 5.81 5.83 -.25 .3463 .3455 .25
15 1.000 440.000 . 100 5.81 5.83 -.27 .3550 .3540 .26
16 1.000 450.000 .100 5.81 5.83 -.28 .3636 .3626 .27
17 1.000 460.000 . 100 5.81 5.83 -.29 .3722 .3712 .28
18 1.000 470.000 .100 5.81 5.83 -.30 .3808 .3797 .29
19 1.000 480.000 .100 5.81 5.83 -.30 .3894 .3883 .29
20 1.000 490.000 .100 5.81 5.83 -.30 .3980 .3968 .30
21 1.000 500.000 .100 5.81 5.83 -.31 .4066 .4054 .30
22 1.000 510.000 .100 5.81 5.83 -.31 .4152 .4139 .30
23 1.000 520.000 . 100 5.81 5.83 -.31 .4237 .4224 .30
24 1.000 530.000 .100 5.81 5.83 -.30 .4322 .4310 .30
25 1.000 540.000 .100 5.81 5.83 -.30 .4408 .4395 .30
26 1.000 550.000 .100 5.81 5.83 -.30 .4493 .4480 .29
27 1.000 560.000 .100 5.81 5.83 -.29 .4578 .4565 .29
28 1.000 570.000 .100 5.81 5.83 -.29 .4663 .4650 .28
29 1.000 580.000 . 100 5.81 5.83 -.28 .4748 .4735 .28
30 1.000 590.000 .100 5.81 5.83 -.28 .4834 .4820 .27
31 1.000 600.000 .100 5.81 5.83 -.27 .4918 .4905 .27
32 1.000 610.000 .100 5.81 5.83 -.26 .5003 .4990 .26
33 1.000 620.000 .100 5.81 5.83 -.26 .5088 .5075 .25
34 1.000 630.000 .100 5.81 5.83 -.25 .5173 .5160 .25
35 1.000 640.000 .100 5.81 5.83 -.24 .5258 .5245 .24
36 1.000 650.000 .100 5.81 5.83 -.24 .5343 .5330 .24
37 1.000 660.000 .100 5.81 5.83 -.23 .5427 .5415 .23
38 1.000 670.000 . 100 5.81 5.83 -.22 .5512 .5500 .22
39 1.000 680.000 .100 5.81 5.82 -.22 .5597 .5585 .21
40 1.000 690.000 . 100 5.81 5.82 -.21 .5681 .5669 .21
41 1.000 700.000 .100 5.81 5.82 -.20 .5766 .5754 .20
65
Data sources and ID numbers: (l)Virial Equation, (3)Beattie, (19)Kay, (25)Olds, (29)Sage,
(XXXX)Haynes.
Data Weight Temp. Density Density Density êxpt ^calc Pressure

Point expt caic Diff. Diff.
No, K mol/L kg/m- I<g/m^ % MPa MPa %
3 42 1.000 423.150 .500 29.06 28.97 .33 1.4875 1.4915 -.27

3 43 1.000 448.150 .500 29.06 29.00 .22 1 .6121 1.6151 -.19
3 44 1.000 473.150 .500 29.06 29.01 . 19 1.7337 1.7366 -.17
3 45 1.000 498.150 .500 29.06 29.02 .14 1.8542 1.8566 -.13
3 46 1.000 523.150 .500 29.06 29.04 .09 1.9738 1.9754 -.08
3 47 1.000 548.150 .500 29.06 29.05 .05 2.0924 2.0933 -.04
3 48 1.000 573.150 .500 29.06 29.06 .02 2.2099 2.2104 -.02
3 49 1.000 423.150 1.000 58.12 57.67 .77 2.5007 2.5133 -.50
3 50 1.000 448.150 1.000 58.12 57.67 .79 2.7864 2.8022 -.56
3 51 1.000 473.150 1.000 58.12 57.69 .74 3,0641 3.0814 -.56
3 52 1.000 498.150 1.000 58.12 57.73 .68 3.3356 3.3539 -.54
3 53 1.000 523.150 1.000 58.12 57.75 .64 3.6021 3.6213 -.53
3 54 1.000 548.150 1.000 58.12 57.84 .49 3.8686 3.8850 -.42
3 55 1.000 573.150 1.000 58.12 57.87 .43 4.1300 4.1456 -.38
3 56 1.000 423.150 1.500 87.19 86.46 .83 3.1350 3.1469 -.38
3 57 1.000 448.150 1.500 87.19 86.31 1.00 3.6153 3.6360 -.57
3 58 1.000 473.150 1.500 87.19 86.31 1.01 4.0753 4.1022 -.65
3 59 1.000 498.150 1.500 87.19 86.44 .85 4.5262 4.5538 -.61
3 60 1.000 523.150 1.500 87.19 86.51 .77 4.9659 4.9951 -.58
3 61 1.000 548.150 1.500 87.19 86.68 .58 5.4037 5.4287 -.46
3 62 1.000 573.150 1.500 87.19 86.79 .45 5.8343 5.8562 -.37
3 63 1.000 423.150 2.000 116,25 115.51 .63 3.4846 3.4905 -.17
3 64 1.000 448.150 2.000 116.25 115.22 .89 4. 1857 4.2023 -.39
3 65 1.000 473.150 2.000 116.25 115.24 .87 4.8514 4.8750 -.48
3 66 1.000 498.150 2.000 116.25 115.44 .70 5.5009 5.5257 -.45
3 67 1.000 523.150 2.000 116.25 115.74 .43 6. 1423 6. 1612 -.31
3 68 1.000 548.150 2.000 116.25 115.91 .29 6.7705 6.7856 -.22
3 69 1.000 573.150 2.000 116.25 116.10 .13 7.3937 7.4012 -.10
3 70 1.000 423.150 2.500 145.31 144.87 .30 3.6406 3.6419 -.04
3 71 1.000 448.150 2.500 145.31 144.31 .69 4.5748 4.5859 -.24
3 72 1.000 473.150 2.500 145.31 144.55 .52 5.4634 5.4776 -.26
3 73 1.000 498.150 2.500 145.31 144.91 .28 6.3328 6.3433 -.17
3 74 1.000 523.150 2,500 145.31 145.17 . 10 7. 1870 7. 1918 -.07
3 75 1.000 548.150 2.500 145.31 145.59 -.19 8.0391 8.0275 .15
3 76 1.000 573.150 2.500 145.31 145.84 -.36 8.8791 8.8531 .29
3 77 1.000 448.150 3.000 174.37 173.57 .46 4.8525 4.8591 -.14
3 78 1.000 473.150 3.000 174.37 174.12 .15 5.9772 5.9813 -.07
3 79 1.000 498.150 3.000 174.37 174.60 -.13 7.0857 7.0801 .08
3 80 1.000 523.150 3.000 174.37 174.91 -.31 8.1810 8.1632 .22
3 81 1.000 548.150 3.000 174.37 175.44 -.61 9.2793 9.2344 .49
3 82 1.000 573.150 3.000 174.37 175.70 -.76 10.3635 10.2961 .65
3 83 1.000 448.150 3.500 203.44 202.22 .60 5.0744 5.0835 -. 18
3 84 1.000 473.150 3.500 203.44 203.09 .17 6.4493 6.4551 -.09
3 85 1.000 498.150 3.500 203.44 203.85 -.21 7.8233 7.8124 .14
3 86 1.000 523.150 3.500 203.44 204.21 -.38 9.1871 9. 1594 .30
3 87 1.000 548.150 3.500 203.44 204.86 -.70 10.5631 10.4980 .62
3 88 1.000 573.150 3.500 203.44 205.17 -.85 11.9260 11.8292 .82
3 89 1.000 448.150 4.000 232.50 229.40 1.33 5.2861 5.31 18 -.48
3 90 1.000 448.150 4.000 232.50 229.77 1.17 5.2892 5.31 18 -.43
3 91 1.000 473.150 4.000 232.50 231.80 .30 6.9519 6.9650 -.19
3 92 1.000 473.150 4.000 232.50 231.15 .58 6.9397 6.9650 -.36
3 93 1.000 498.150 4.000 232.50 232.98 -.21 8.6329 8.6183 .17
3 94 1.000 498.150 4.000 232.50 232.27 .10 8.61 16 8.6183 -.08
3 95 1.000 523.150 4.000 232.50 233.69 -.51 10.3189 10.2698 .48
3 96 1.000 523.150 4,000 232.50 232.90 -.17 10.2865 10.2698 .16
66
1
Data sources and ID numbers: (l)Virial Equation, (3)Beattie, (19)Kay, (25)0lds, (29)Sage,
(XXXX)Haynes.
ID Data Weight Temp. Density Density Density êxpt '^calc

Pressure
Point expt calc Diff. Diff.
No. K mol/L kg/m^ Wg/m^ % MPa MPa %
3 97 1 .000 548. 150 4.000 232.50 234.31 -.78 12.0141 1 .9183 1 .80
3 98 1 .000 548.150 4.000 232.50 233.66 -.50 11.9797 11.9183 .51
3 99 1 .000 573. 150 4.000 1S32.50 234.71 -.95 13.7062 13.5629 1 .05
3 100 1 .000 573. 150 4.000 232.50 234.09 -.68 13.6657 13.5629 .76
3 101 1 .000 448. 150 4.500 261 .56 257.05 1.72 5.5354 5.5818 -.83
3 102 1.000 473.150 4.500 261 .56 259.28 .87 7.5143 7.5663 -.69
3 103 1 .000 498. 150 4.500 261 .56 260.68 .34 9.5367 9.5684 -.33
3 104 1.000 523.150 4.500 261 .56 261.49 .03 11.5754 .5789
1 1 -.03
3 105 1.000 548.150 4.500 261.56 262.27 -.27 13.6383 13.5930 .33
3 106 1.000 573.150 4.500 261 .56 262.67 -.42 15.6932 15.6074 .55
3 107 1.000 425.160 5.000 290.62 288.79 .63 3.8260 3.8302 -.11
3 108 1.000 448.150 5.000 290.62 287.60 1.04 5.9072 5.9536 -.78
3 109 1.000 448.150 5.000 290.62 286.51 1 .41 5.8910 5.9536 -1 .05
3 110 1.000 473.150 5.000 290.62 289.42 .41 8.3046 8.3417 -.44
3 111 1.000 473.150 5.000 290.62 288.16 .85 8.2661 8.3417 -.91
3 112 1.000 498.150 5.000 290.62 290.60 .01 10.7638 10.7647 -.01
3 113 1 .000 498.150 5.000 290.62 289.54 .37 10.7141 10.7647 -.47
3 114 1.000 523. 150 5.000 290.62 291.36 -.25 13.2533 13.2064 .35
3 1 15 1.000 523.150 5.000 290.62 290.35 .09 13. 1895 13.2064 -.13
3 116 1.000 548.150 5.000 290.62 291 .95 -.46 15.7652 15.6581 .68
3 117 1.000 548.150 5.000 290.62 290.93 -.11 15.6831 15.6581 .16
3 118 1.000 573.150 5.000 290.62 292.48 -.64 18.2952 18. 1 142 1.00
3 119 1.000 573.150 5.000 290.62 291 .32 -.24 18. 1818 18.1 142 .37
3 120 1.000 425.160 5.500 319.68 318.19 .47 3.9669 3.9798 -.33
3 121 1 .000 448.150 5.500 319.68 317.90 .56 6.5041 6.5506 -.71
3 122 1.000 473.150 5.500 319.68 318.97 .22 9.4101 9.4425 -.34
3 123 1.000 498.150 5.500 319.68 319.80 -.04 12.3900 12.3822 .06
3 124 1 .000 523.150 5.500 319.68 320.41 -.23 15.4105 15.3483 .41
3 125 1 .000 548 . 1 50 5.500 319.68 320.87 -.37 18.4553 18.3291 .69
3 126 1 .000 573.150 5.500 319.68 321 .27 -.50 21 .5174 21 .3169 .94
3 127 1 .000 425. 160 6.000 348.75 347.41 .38 4.3975 4.4284 -.70
3 128 1 .000 448. 150 6.000 348.75 347.61 .32 7.5305 7.5823 -.68
3 129 1 .000 473. 150 6.000 348.75 348. 17 . 16 1 .0677
1 1 .10811 -.36
3 130 1 .000 498. 150 6.000 348.75 348.83 -.02 14.6942 14.6861 .05
3 131 1 .000 523. 150 6.000 348.75 349.23 -.14 18.3510 18.2935 .31
3 132 1 .000 548. 150 6.000 348.75 349.59 -.24 22.0382 21 .9166 .55
3 133 1 .000 573. 150 6.000 348.75 349.85 -.32 25.7325 25.5466 .73
3 134 1 .000 425. 160 6.500 377.81 376.37 .38 5.4047 5.4769 -1 .32
3 135 1 .000 448. 150 6.500 377.81 376.76 .28 9.2885 9.3713 -.88
3 136 1 .000 473. 50 1 6.500 377.81 377. 15 .17 13.6171 13.6886 -.52
3 137 1 .000 498. 150 6.500 377.81 377.58 .06 18.0207 18.0530 -. 18
3 138 1 .000 523. 150 6.500 377.81 377.88 -.02 22.4556 22.4427 .06
3 139 1 .000 548. 150 6.500 377.81 378.1 -.08 26.9048 26.8444 .23
3 140 1.000 573.150 6.500 377.81 378.32 -.14 31 .3662 31 .2488 .38
3 141 1 .000 425. 160 7.000 406.87 405.33 .38 7.4241 7.5699 -1 .93
3 142 1.000 448.150 7.000 406.87 405.63 .31 12.2188 12.3801 -1 .30
3 143 1.000 473.150 7.000 406.87 405.95 .23 17.5161 17.6701 -.87
3 144 1.000 498.150 7.000 406.87 406.24 .16 22.8640 22.9929 -.56
3 145 1.000 523. 150 7.000 406.87 406.41 .11 28.2200 28.3301 -.39
3 146 1.000 548.150 7.000 406.87 406.47 .10 33.5588 33.6696 -.33
3 147 1.000 425.160 7.500 435.93 434.23 .39 1 .0404
1 11.3183 -2.46
3 148 1 .000 448.150 7.500 435.93 434.54 .32 16.9507 17.2358 -1 .65
3 149 1 .000 473. 150 7.500 435.93 434.63 .30 23.3767 23.7006 -1.37
3 150 1.000 498.150 7.500 435.93 434.94 .23 29.8848 30.1760 -.97
3 151 1.000 523.150 7.500 435.93 434.98 .22 36.3281 36.6481 -.87
3 152 1.000 425.160 8.000 464.99 463.13 .40 17.0337 17.5247 -2.80
3 153 1.000 448.150 8.000 464.99 463.42 .34 24.2663 24.7575 -1 .98
3 154 1.000 473.150 8.000 464.99 463.27 .37 31 .9893' 32.6184 -1 .93
3 155 1.000 425.160 8.500 494.06 492.07 .40 26.4134 27.2128 -2.94
3 156 1.000 448.150 8.500 494.06 492.26 .36 35.1618 35.9860 -2.29
67
1 .
(XXXX)Haynes.
ID Data Weight Temp. Dens ty i Dens ty i Dens tyi

expT p ca c
1
Pressure
Poi nt expt ca c1 Diff Diff.
No. K mol/L kg/m-^ kg/m^ % MPa MPa $
19 157 1.000 310.928 .079 4.58 4.56 .41 .1924 .1931 -.39
19 158 1.000 338.706 .079 4.58 4.57 .23 .21 17 .2121 -.22
19 159 1.000 366.483 .079 4.58 4.58 .01 .2310 .2310 -.01
19 160 1.000 394.261 .079 4.58 4.57 .07 .2496 .2498 -.07
19 161 1.000 422.039 .079 4.58 4.58 -. 17 .2689 .2684 .17
19 162 1.000 449.817 .079 4.58 4.58 -.15 .2875 .2871 .15
19 163 1.000 477.594 .079 4.58 4.57 .08 .3054 .3057 -.08
19 164 1.000 505.372 .079 4.58 4.57 .06 .3241 .3242 -.06
19 165 1.000 533. 150 .079 4.58 4.57 .04 .3427 .3428 -.04
19 156 1.000 560.928 .079 4.58 4.57 .20 .3606 .3613 -.20
19 167 1.000 588.706 .079 4.58 4.57 .17 .3792 .3798 -.17
19 168 1.000 310.928 .085 4.93 4.90 .52 .2062 .2072 -.49
19 169 1.000 338.706 .085 4.93 4.92 .10 .2275 .2277 -.09
19 170 1.000 366.483 .085 4.93 4.92 .25 .2475 .2481 -.24
19 171 1.000 394.261 .085 4.93 4.94 -.21 .2689 .2684 .20
19 172 1.000 422.039 .085 4.93 4.95 -.37 .2896 .2885 .36
19 173 1.000 449.817 .085 4.93 4.93 -.08 .3089 .3086 .08
19 174 1.000 477.594 .085 4.93 4.93 -.05 .3289 .3287 .05
19 175 1.000 505.372 .085 4.93 4.93 -.04 .3489 .3487 .04
19 176 1.000 533. 150 .085 4.93 4.92 .16 .3682 .3687 -.15
19 177 1.000 560.928 .085 4.93 4.92 .15 .3882 .388 7 -.14
19 178 1.000 588.705 .085 4.93 4.91 .30 .4075 .4087 -.30
19 179 1.000 310.928 .092 5.34 5.32 .33 .2227 .2234 -.31
19 180 1.000 338.706 .092 5.34 5.33 .15 .2455 .2458 -.14
19 181 1.000 366.483 .092 5.34 5.33 .17 .2675 .2680 -.16
19 182 1.000 394.261 .092 5.34 5.33 .14 .2896 .2900 -.13
19 183 1.000 422.039 .092 5.34 5.35 -.15 .3123 .31 19 .15
19 184 1.000 449.817 .092 5.34 5.34 .00 .3337 .3337 -.00
19 185 1.000 477.594 .092 5.34 5.33 .12 .3551 .3555 -. 12
19 186 1.000 505.372 .092 5.34 5.34 .03 .3771 .3772 -.03
19 187 1.000 533. 150 .092 5.34 5.33 .11 .3985 .3990 -.11
19 188 1.000 560.928 .092 5.34 5.33 .18 .4199 .4206 -. 18
19 189 1.000 588.706 .092 5.34 5.33 .24 .4413 .4423 -.24
19 190 1.000 310.928 .100 5.82 5.80 .47 .2413 .2424 -.44
19 191 1.000 338.706 .100 5.82 5.82 .05 .2568 .2570 -.05
19 192 1.000 365.483 .100 5.82 5.82 .10 .2910 .2912 -.10
19 193 1.000 394.261 .100 5.82 5.82 .08 .3151 .3153 -.08
19 194 1.000 422.039 .100 5.82 5.84 -.18 .3399 .3393 .17
19 195 1.000 449.817 .100 5.82 5.83 -.04 .3634 .3632 .04
19 196 1.000 477.594 .100 5.82 5.82 .07 .3868 .3870 -.06
19 197 1.000 505.372 .100 5.82 5.83 -.03 .4109 .4108 .03
19 198 1.000 533.150 .100 5.82 5.82 .04 .4344 .4346 -.04
19 199 1.000 560.928 .100 5.82 5.81 .25 .4571 .4583 -.25
19 200 1.000 588.706 .100 5.82 5.82 .15 .4813 .4820 -.14
19 201 1.000 310.928 .110 6.41 6.39 .32 .2641 .2649 -.30
19 202 1.000 338.706 .1 10 6.41 6.40 .16 .2916 .2921 -.15
19 203 1.000 366.483 .110 6.41 6.38 .36 .3178 .3190 -.35
19 204 1.000 394.261 .1 10 6.41 6.40 .05 .3454 .3456 -.05
19 205 1.000 422.039 .1 10 6.41 6.41 -.07 .3723 .3721 .07
19 206 1.000 449.817 .1 10 6.41 6.41 -.02 .3985 .3984 .02
19 207 1.000 477.594 .1 10 6.41 6.42 -.16 .4254 .4247 .16
19 208 1.000 505.372 .1 10 6.41 6.41 .01 .4509 .4510 -.01
19 209 1.000 533.150 .1 10 6.41 5.40 .15 .4764 .4771 -.15
19 210 1.000 560.928 .110 6.41 6.40 .13 .5026 .5033 -.13
19 21 1.000 588.706 .110 5.41 6.39 .24 .5281 .5294 -.24
68
51 0
. .
1
(XXXX)Haynes.

i Dens ty i Dens ty i
fêxpt ^ca c
1
Pressure
Poi nt expt z
ca c 1 Di f f D i f f
No. K mol/L kg/m-^ kg/m-' % MPa MPa %
19 212 1.000 310.928 .122 7.12 7.09 .35 .2910 .2919 -.32
19 213 1.000 338.706 .122 7.12 7.1 .15 .3220 .3224 -.14
19 214 1 .000 366.483 .122 7.12 7.10 .25 .3516 .3525 -.24
19 215 1.000 394.261 .122 7.12 7. 1 .07 .3820 .3822 -.07
19 216 1.000 422.039 .122 7.12 7.13 -.13 .4123 .41 18 .12
19 217 1.000 449.817 .122 7.12 7,12 -.01 .4413 .4412 .01
19 218 1.000 477.594 .122 7.12 7.11 .07 .4702 .4705 -.07
19 219 1.000 505.372 .122 7.12 7.12 -.02 .4999 .4998 .02
19 220 1.000 533. 150 .122 7.12 7.12 .03 .5288 .5290 -.03
19 221 1.000 560.928 .122 7.12 7.11 .06 .5578 .5581 -.06
19 222 1 .000 588.706 .122 7.12 7.10 .20 .5861 .5872 -.20
19 223 1.000 310.928 .138 8.01 7.97 .54 .3234 .3250 -.49
19 224 1 .000 338.706 .138 8.01 7.98 .36 .3585 .3597 -.33
19 225 1.000 366.483 .138 8.01 7.99 .23 .3930 .3938 -.21
19 226 1.000 394.261 .138 8.01 8.01 .02 .4275 .4276 -.02
19 227 1 .000 422.039 .138 8.01 8.01 -.06 .4613 .4610 .05
19 228 1 .000 449.817 .138 8.01 8.01 -.01 .4944 .4943 .01
19 229 1.000 477.594 .138 8.01 8.00 .13 .5268 .5274 -.13
19 230 1 .000 505.372 .138 8.01 8.01 -.01 .5605 .5605 .01
19 231 1 .000 533. 150 .138 8.01 8.00 .09 .5929 .5935 -.09
19 232 1 .000 560.928 .138 8.01 8.01 .05 .6260 .6264 -.05
19 233 1 .000 588.706 .138 8.01 8.00 .12 .6584 .6592 -. 12
19 234 1 .000 338.706 .157 9.15 9.14 . 16 .4061 .4067 -.15
19 235 1 .000 366.483 .157 9.15 9. 14 . 18 .4454 .4461 -. 16
19 236 1 .000 394.261 .157 9.15 9.13 .22 .4840 .4850 -.21
19 237 1 .000 422.039 .157 9.15 9. 5 1 .05 .5233 .5236 -.05
19 238 1 .000 449.8 17 .157 9. 15 9. 14 . 12 .5612 .5619 -. 1
19 239 1 .000 477.594 .157 9.15 9. 16 -. 1 .6005 .6000 .09

19 240 1 .000 505.372 .157 9.15 9. 16 -.08 .6385 .6380 .08
19 241 1 .000 533. 150 .157 9.15 9. 1 .02 .6757 .6758 -.02
19 242 1 .000 560.928 .157 9.15 9.15 .00 .7136 .7136 -.00
19 243 1 .000 588.706 .157 9.15 9. 1 5 .07 .7508 .7514 -.07
19 244 1 .000 338.706 .184 10.68 10.66 .19 .4668 .4676 -.17
19 245 1 .000 366.483 .184 10.68 10.68 -.01 .5143 .5143 .01
19 246 1 .000 394.261 .184 10.68 10.66 .21 .5592 .5603 -.19
19 247 1.000 422.039 .184 10.68 10.67 .06 .6054 .6057 -.06
19 248 1 .000 449.817 .184 10.68 10.67 .10 .6502 .6508 -.10
19 249 1 .000 477.594 .184 10.68 10.69 -.11 .6964 .6956 .10
19 250 1.000 505.372 .184 10.68 10.68 -.03 .7405 .7403 .03
19 251 1 .000 533. 150 .184 10.68 10.70 -. 16 .7860 .7848 .15
19 252 1.000 560.928 .184 10.68 10.68 -.03 .8294 .8292 .03
19 253 1 .000 588.706 .184 10.68 10.67 .07 .8729 .8735 -.07
19 254 1 .000 338.706 .197 11.44 1 .40
1 .34 .4957 .4972 -.30
19 255 1 .000 366.483 .197 11.44 1 1 .42 .20 .5468 .5477 -.18
19 256 1 .000 394.261 .197 1 .44
1 1 1 .42 .16 .5964 .5973 -.15
19 257 1 .000 422.039 .197 1 1 .44 1 1 .44 .03 .6460 .6462 -.03
19 258 1.000 449.817 .197 11.44 1 1 .43 .07 .6943 .6948 -.07
19 259 1 .000 477.594 .197 11.44 11.45 -.03 .7433 .7430 .03
19 260 1.000 505.372 .197 11.44 11 .46 -.15 .7922 .7910 .15
19 261 1.000 533.150 .197 11.44 1 1 .43 .06 .8384 .8389 -.06
19 262 1.000 560.928 .197 11.44 11.45 -.09 .8874 .8866 .08
19 263 1.000 588.706 .197 11.44 1 1.44 -.00 .9342 .9342 .00
19 264 1.000 338.706 .212 12.32 12.30 .14 .5302 .5308 -. 12
19 265 1.000 366.483 .212 12.32 12.30 .20 .5847 .5857 -.18
19 266 1.000 394.261 .212 12.32 12.30 .18 .6385 .6395 -.16
19 267 1.000 422.039 .212 12.32 12.32 .05 .6922 .6925 -.05
69
1 ) 1.
1 1
Table 7. { Cont nued

i
(XXXX)Haynes.

i Dens ity Dens ty i
'êxpt '^ca 1 c Pressui
Point expt ca c 1 Diff Diff.
No. K mol/L kg/m^ kg/m-' % MPa MPa %
19 268 1.000 449.817 .212 12.32 12.31 .07 .7446 ,7451 -.06
19 269 1 .000 477.594 .212 12.32 12.35 -.23 .7991 ,7973 .22
19 270 1.000 505.372 .212 12.32 12.36 -.27 ,8515 ,8493 .26
19 271 1 .000 533.150 .212 12.32 12.35 -.25 ,9032 ,9010 .24
19 272 1 .000 560.928 .212 12.32 12.35 -.25 .9549 ,9526 .25
19 273 1 .000 588.706 .212 12.32 12.33 -.05 1 .0046 1,0040 .05
19 274 1 .000 338.706 .230 13.35 13.30 .36 ,5674 ,5692 -.31
19 275 1.000 366.483 .230 13.35 13.32 .22 ,6281 .6294 -.20
19 276 1 .000 394.261 .230 13.35 13.33 .1 ,6874 ,6881 -.10
19 277 1,000 422.039 .230 13.35 13,32 .20 .7446 .7460 -. 18
19 278 1 .000 449.817 .230 13.35 13,35 .01 ,8032 .8033 -.01
19 279 1 .000 477.594 .230 13.35 13.38 -.21 .8618 .8602 .19
19 280 1 .000 505.372 .230 13.35 13.41 -.42 .9205 .9167 .40
19 281 1 .000 533.150 .230 13.35 13.40 -.42 .9770 .9731 .40
19 282 1 .000 560.928 .230 13.35 13.38 -.23 1 .0315 1 .0292 .22
19 283 1 .000 588.706 .230 13.35 13.37 -.14 1.0866 1.0852 .13
19 284 1 .000 338.706 ,251 14.56 14.57 -.05 .6136 .6134 .05
19 285 1 .000 366.483 .251 14.56 14.54 .12 .6791 .6799 -. 1
19 286 1 .000 394.261 .251 14.56 14.55 . 10 .7439 .7446 -.09

19 287 1.000 422.039 .251 14.56 14.56 .03 .8081 .8083 -.03
19 288 1.000 449.817 .251 14.56 14.57 -.02 .8715 .8713 .02
19 289 1.000 477.594 .251 14.56 14.60 -.29 .9363 .9338 ,27
19 290 1 .000 505.372 .251 14.56 14.63 -.48 1.0004 ,9958 ,46
19 291 1.000 533.150 .251 14.56 14.63 -.48 1.0625 1,0576 .46
19 292 1 .000 560.928 .251 14.56 14.61 -.31 1.1225 1 . 1 1 92 .29
19 293 1.000 588.706 .251 14.56 14.59 -.17 1,1825 1.1805 .16
19 294 1 .000 338.706 .276 16.02 16.00 .12 ,6640 .6646 -.10
19 295 1.000 366.483 .276 16.02 16.00 .09 .7384 .7390 -.08
19 296 1.000 394.261 .276 16.02 15.98 .23 .8094 .8111 -.21
19 297 1.000 422.039 .276 16.02 16.03 -.07 .8825 .8819 .07
19 298 1.000 449.817 .276 16.02 16.05 -.19 .9535 .9518 .18
19 299 1.000 477.594 .276 16.02 16.1 1 -.58 1.0266 1.0211 .54
19 300 1.000 505.372 .276 16.02 16.12 -.62 1.0963 1.0899 .58
19 301 1.000 533.150 .276 16.02 16,10 -.50 1.1638 1. 583 1 .48
19 302 1.000 560.928 .276 16,02 16.08 -.36 1.2307 1.2264 .35
19 303 1 .000 588.706 .276 16.02 16.04 -.15 1.2962 1.2943 .14
19 304 1.000 338.706 .306 17,80 17.86 -.34 .7267 .7247 .27
19 305 1.000 366.483 .306 17.80 17.79 .05 .8088 .8091 -.05
19 306 1.000 394.261 .306 17,80 17.76 .23 .8887 ,8905 -.20
19 307 1.000 422.039 .306 17,80 17.81 -.07 .9708 ,9702 ,06
19 308 1.000 449.817 .306 17,80 17.84 -.21 1.0508 1,0487 ,19
19 309 1 .000 477.594 .306 17,80 17.88 -.48 1.1314 1, 264 1 .44
19 310 1.000 505.372 .306 17,80 17.89 -.51 1.2093 1,2035 .48
19 31 1.000 533.150 .306 17,80 17.88 -.47 1,2859 1,2802 .44
19 312 1 .000 560.928 .306 17.80 17.86 -.35 1,3610 1,3565 .34
19 313 1.000 588.706 .306 17.80 17.82 -.12 1 ,4341 1,4325 .12
19 314 1 .000 366.483 .344 20.02 20.05 -. 1 ,8942 .8934 .09
19 315 1.000 394.261 .344 20.02 20.00 .10 ,9860 ,9868 -.09
19 316 1.000 422.039 .344 20.02 20.05 -.12 1,0790 1.0779 .11
19 317 1.000 449.817 .344 20.02 20.11 -.44 1,1721 1.1674 .40
19 318 1.000 477.594 .344 20.02 •
20.12 -.50 1,2617 1.2559 .46
19 319 1.000 505.372 .344 20.02 20.14 -.56 1.3507 1.3436 .52
19 320 1.000 533.150 .344 20.02 20.13 -.56 1.4382 1.4307 .52
19 321 1.000 560.928 .344 20,02 20.11 -.44 1.5237 1.5174 .42
19 322 1.000 588.706 .344 20,02 20.06 -.19 1.6065 1.6036 .18
19 323 1.000 366.483 .394 22,88 22,92 -.16 .9977 .9964 .13
70
1
Data sources and ID numbers: (DVirial Equation, (3)Beattie, {19)Kay, (25)0lds, (29)Sage,
(XXXX)Haynes.
ID Data Weight Temp. Density Density Density êxpt ^calc Pressure

No. K mol/L kg/m^ kg/m^ % MPa MPa %
19 324 1.000 394.261 .394 22.88 22.87 .07 1.1052 1.1059 -.06
19 325 1.000 422.039 .394 22.88 22.90 -.07 1.2128 1.2121 .06
19 326 1.000 449.817 .394 22.88 22.91 -.12 1.3176 1.3162 .10
19 327 1.000 477.594 .394 22.88 22.99 -.48 1.4251 1.4189 .44
19 328 1.000 505.372 .394 22.88 23.04 -.67 1.5299 1.5206 .62
19 329 1.000 533.150 .394 22.88 23.06 -.79 1.6334 1.6214 .74
19 330 1.000 560.928 .394 22.88 23.04 -.68 1.7327 1.7217 .64
19 331 1.000 588.706 .394 22.88 23.05 -.73 1.8340 1.8214 .69
19 332 1.000 366.483 .459 26.70 26.77 -.28 1. 266
1 1.1242 .21
19 333 1.000 394.261 .459 26.70 26.66 .15 1.2548 1.2564 -.12
19 334 1.000 422.039 .459 26.70 26.67 .11 1.3824 1.3837 -.09
19 335 1.000 449.817 .459 26.70 26.72 -.09 1.5093 1.5080 .08
19 336 1.000 477.594 .459 26.70 26.78 -.30 1.6347 1.6303 .27
19 337 1.000 505.372 .459 26.70 26.84 -.53 1.7595 1 .751 1 .48
19 338 1.000 533.150 .459 26.70 26.86 -.63 1.8816 1.8708 .58
19 339 1.000 560.928 .459 26.70 26.89 -.72 2.0029 1.9896 .67
19 340 1.000 588.706 .459 26.70 26.86 -.59 2.1 194 2.1077 .56
19 341 1.000 366.483 .501 29. 12 29.30 -.59 1.2052 1.2000 .43
19 342 1.000 394.261 .501 29.12 29.10 .08 1.3465 1.3473 -.06
19 343 1.000 422.039 .501 29.12 29.12 .00 1.4886 1.4886 -.00
19 344 1.000 449.817 .501 29.12 29.14 -.07 1.6272 1.6262 .06
19 345 1.000 477.594 .501 29.12 29.21 -.28 1.7657 1.7613 .25
19 346 1.000 505.372 .501 29.12 29.27 -.49 1.9030 1.8947 .44
19 347 1.000 533.150 .501 29.12 29.26 -.47 2.0353 2.0266 .43
19 348 1.000 560.928 .501 29.12 29.25 -.44 2. 1663 2.1575 .41
19 349 1.000 588.706 .501 29.12 29.24 -.39 2.2960 2.2875 .37
19 350 1.000 366.483 .551 32.04 32.21 -.54 1.2900 1.2852 .38
19 351 1.000 394.261 .551 32.04 31.97 .21 1.4493 1.4516 -. 16
19 352 1.000 422.039 .551 32.04 31.98 .18 1.6079 1.6102 -.15
19 353 1.000 449.817 .551 32.04 32.06 -.06 1.7651 1.7642 .05
19 354 1.000 477.594 .551 32.04 32.12 -.27 1.9195 1.9151 .23
19 355 1.000 533.150 .551 32.04 32.20 -.50 2.2208 2.2107 .46
19 356 1.000 560.928 .551 32.04 32.21 -.55 2.3683 2.3564 .51
19 357 1.000 588.706 .551 32.04 32.16 -.37 2.5097 2.501 .35
19 358 1.000 394.261 .612 35.60 35.56 .11 1.5706 1.5719 -.08
19 359 1.000 422.039 .612 35.60 35.57 .09 1.7513 1.7525 -.07
19 360 1.000 449.817 .612 35.60 35.61 -.04 1.9278 1.9271 .03
19 361 1.000 477.594 .612 35.60 35.66 -.17 2.1008 2.0978 .14
19 362 1.000 505.372 .612 35.60 35.71 -.31 2.2718 2.2657 .27
19 363 1.000 533.150 .612 35.60 35.72 -.36 2.4394 2.4315 .32
19 364 1.000 560.928 .612 35.60 35.71 -.33 2.6035 2.5957 .30
19 365 1.000 588.706 .612 35.60 35.68 -.24 2.7648 2.7586 .22
19 366 1.000 394.261 .689 40.05 39.86 .47 1.7058 1.71 14 -.33
19 367 1.000 422.039 .689 40.05 39.92 .32 1.9161 1 .9207 -.24
19 368 1.000 449.817 .689 40.05 39.98 .16 2.1 194 2.1222 -.13
19 369 1.000 477.594 .689 40.05 40.05 -.01 2.3187 2.3184 .01
19 370 1.000 505.372 .689 40.05 40.08 -.09 2.5131 2.51 1 1 .08
19 371 1.000 533.150 .689 40.05 40.15 -.27 2.7076 2.701 1 .24
19 372 1.000 560.928 .689 40.05 40.15 -.26 2.8958 2.8891 .23
19 373 1.000 588.706 .689 40.05 40.14 -.23 3.0820 3.0754 .21
19 374 1.000 394.261 .787 45.77 45.69 .17 1.8712 1.8733 -.11
19 375 1.000 422.039 .787 45.77 45.58 .42 2.1 153 2.1218 -.31
19 376 1.000 449.817 .787 45.77 45.58 .40 2.3518 2.3592 -.31
19 377 1.000 477.594 .787 45.77 45.68 .20 2.5855 2.5897 -.16
19 378 1.000 505.372 .787 45.77 45.79 -.04 2.8165 2.8155 .04
19 379 1.000 533.150 .787 45.77 45.88 -.24 3.0440 3.0376 .21
71
1 9
Data sources and ID numbers: (l)Virial Equation, (3)8eattie, (19)Kay, (25)0lds, (29)Sage,
(XXXX)Haynes.
ID Data Weight Temp. Density Density Density êxpt '^calc Pressure

19 380 1.000 560.928 .787 45.77 45.94 -.38 3.2681 3.2571 .34
19 381 1.000 588.706 .787 45.77 45.97 -.45 3.4887 3.4745 .41
19 382 1 .000 394.261 .919 53.39 53. 17 .43 2.0546 2.0597 -.25
19 383 1.000 422.039 .919 53.39 53.08 .60 2.3546 2.3641 -.40
19 384 1.000 449.817 .919 53.39 53.29 .20 2.6483 2.6522 -.15
19 385 1 .000 477.594 .919 53.39 53.39 .01 2.9303 2.9305 -.01
19 386 1.000 505.372 .919 53.39 53.40 -.01 3.2026 3.2023 .01
19 387 1.000 533.150 .919 53.39 53.39 .01 3.4688 3.4692 -.01
19 388 1.000 560.928 .919 53.39 53.24 .28 3.7232 3.7324 -.25
19 389 1.000 588.706 .919 53.39 53.13 .50 3.9748 3.9928 -.45
19 390 1.000 394.261 1.002 58.25 58.36 -.19 2.1636 2. 1614 .10
19 391 1.000 422.039 1.002 58.25 57.80 .78 2.491 1 2.5036 -.50
19 392 1.000 449.817 1.002 58.25 57.81 .75 2.8103 2.8254 -.54
19 393 1.000 477.594 1.002 58.25 57.97 .47 3.1240 3.1354 -.36
19 394 1.000 505.372 1.002 58.25 58.02 .39 3.4267 3.4375 -.32
19 395 1.000 533.150 1.002 58.25 58.05 .34 3.7232 3.7339 -.29
19 396 1.000 560.928 1.002 58.25 58.1 1 .24 4.0176 4.0260 -.21
i9 397 1.000 588.706 1.002 58.25 58.1 1 .23 4.3058 4.3147 -.21
19 398 1.000 422.039 1.102 64.07 63.52 .86 2.6428 2.6567 -.52
19 399 1.000 449.817 1.102 64.07 63.55 .8 5 3.0027 3.0204 -.59
19 400 1.000 477.594 1.102 64.07 63.67 .63 3.3536 3.3695 -.47
19 401 1.000 505.372 1.102 64.07 63.85 .35 3.6990 3.7092 -.27
19 402 1.000 533.150 1.102 64.07 63.91 .26 4.0334 4.0420 -.21
19 403 1.000 560.928 1.102 64.07 63.87 .32 4.3575 4.3696 -.28
19 404 1.000 588.706 1.102 64.07 63.79 .45 4.6746 4.6932 -.39
19 405 1 .000 422.039 1.225 71 .19 70.41 1.10 2.8062 2.8235 -.61
19 406 1.000 449.817 1.225 71 .19 70.55 .91 3.2212 3.2403 -.59
19 407 1.000 477.594 1.225 7.1 . 1 70.78 .58 3.6239 3.6391 -.42
19 408 1.000 505.372 1.225 71.19 70.89 .43 4.0127 4.0261 -.33
19 409 1.000 533. 150 1.225 71 .19 71 .08 .17 4.3989 4.4047 -.13
19 410 1.000 560.928 1 .225 71 .19 71 .09 .15 4.7712 4.7772 -.13
19 41 1.000 588.706 1.225 71 .19 70.95 .34 5. 1297 5. 1448 -.29
19 412 1 .000 422.039 1 .378 80.09 79.01 1 .35 2.9827 3.0028 -.67
19 413 1.000 449.817 1 .378 80.09 79.31 .98 3.4681 3.4889 -.60
19 414 1 .000 477.594 1 .378 80.09 79.61 .60 3.9355 3.9518 -.41
19 415 1 .000 505.372 1.378 80.09 79.64 .57 4.3816 4.4002 -.42
19 416 1 .000 533. 150 1 .378 80.09 79.77 .41 4.8229 4.8384 -.32
19 417 1 .000 560.928 1 .378 80.09 79.81 .35 5.2538 5.2690 -.29
19 418 1 .000 588.706 1 .378 80.09 79.89 .25 5.6813 5.6937 -.22
19 419 1 .000 422.039 1 .450 84.31 83.57 .87 3.0647 3.0772 -.41
19 420 1 .000 449.817 1 .450 84.31 83.70 .72 3.5818 3.5971 -.42
19 421 1 .000 477.594 1 .450 84.31 83.87 .52 4.0769 4.0912 -.35
19 422 1.000 505.372 1.450 84.31 83.83 .57 4.5505 4.5694 -.41
19 423 1 .000 533.150 1 .450 84.31 83.86 .53 5.0159 5.0366 -.41
19 424 1.000 560.928 1.450 84.31 83.98 .39 5.4779 5.4955 -.32
19 425 1.000 588.706 1.450 84.31 84.06 .30 5.9329 5.9480 -.25
19 426 1 .000 422.039 1.531 88.99 88.00 1.12 3.1371 3.1524 -.49
19 427 1.000 449.817 1.531 88.99 88.21 .87 3.6921 3.7105 -.50
19 428 1.000 477.594 1.531 88.99 88.45 .61 4.2230 4.2399 -.40
19 429 1.000 505.372 1.531 88.99 88.51 .54 4.7333 4.7518 -.39
19 430 1.000 533.150 1.531 88.99 88.66 .37 5.2366 5.2517 -.29
19 431 1.000 560.928 1.531 88.99 88.68 .35 5.7261 5.7426 -.29
19 432 1.000 588.706 1.531 88.99 88.75 .28 6.2122 6.2266 -.23
19 433 1.000 422.039 1.621 94.23 93.14 1.15 3.2130 3.2278 -.46
19 434 1.000 449.817 1.621 94.23 93.48 .80 3.8128 3.8293 -.43
19 435 1 .000 477.594 1.621 94.23 93.77 .49 4.3851 4.3987 -.31
72
9
(XXXX)Haynes.
ID Data Weight Temp, Density Density Density êxpt '^calc Pressure

19 436 1.000 505.372 1.621 94.23 93.80 .4 5 4.9332 4.9490 -.32

19 437 1.000 533.150 1.621 94.23 93.96 .28 5.4744 5.4861 -.21
19 438 1 .000 560.928 1.621 94.23 93.93 .31 5.9984 6.0135 -.25
19 439 1.000 588.706 1.621 94.23 93.86 .39 6,5121 6.5335 -.33
19 440 1 .000 422.039 1.722 100.12 98.87 1 ,25 3,2874 3.3023 -.45
19 441 1.000 449.817 1.722 100.12 99.64 ,48 3.9438 3.9535 -.24
19 442 1 .000 477.594 1.722 100.12 99.60 .52 4.5540 4.5686 -.32
19 443 1 .000 505.372 1.722 100.12 99.77 .35 5, 1504 5.1628 -.24
19 444 1 .000 533.150 1.722 100.12 99.81 .31 5,7295 5,7427 -,23
19 445 1 .000 560.928 1.722 100.12 99.98 .14 6,3053 6.3121 -.11
19 446 1 .000 588.706 1.722 100.12 100.01 .11 6,8672 6.8734 -.09
19 447 1 .000 422.039 1.837 106.79 105.13 1.56 3.3577 3.3746 -.50
19 448 1 .000 449.817 1.837 106.79 105.98 .76 4.0679 4.0830 -.37
19 449 1 .000 477.594 1.837 106.79 106.26 .50 4.7367 4,7509 -,30
19 450 1 .000 505.372 1.837 106.79 106.37 .40 5.3814 5.3958 -,27
19 451 1 .000 533.150 1.837 106.79 106.48 .29 6.0122 6,0252 -.22
19 452 1 .000 560.928 1.837 106,79 106.58 .20 6.6328 6.6433 -.16
19 453 1 .000 588.706 1.837 106.79 106.68 ,10 7.2464 7.2526 -.09
19 454 1 .000 422.039 1.968 114.42 112.45 1 .72 3.4267 3.4430 -.47
19 455 1 .000 449.817 1.968 114.42 113.71 .62 4.2058 4.2177 -.28
19 456 1 .000 477.594 1.968 114.42 113.73 .60 4.9298 4.9468 -.34
19 457 1 .000 505.372 1.968 114.42 114.08 .30 5.6399 5.6510 -.20
19 458 1 .000 533.150 1.968 114.42 114.20 . 19 6.3294 6.3384 -.14
19 459 1 .000 560.928 1.968 114.42 114,31 .09 7.0085 7.0135 -.07
1 460 1 .000 588.706 1.968 114.42 114.45 -.03 7.6808 7.6792 .02
19 461 1 .000 422.039 2.120 123.22 121.72 1.21 3.4956 3.5050 -.27
19 462 1 .000 449.817 2.120 123.22 122.55 .55 4.3471 4.3572 -.23
19 463 1 .000 477.594 2.120 123.22 122.73 .40 5. 1469 5.1583 -.22
19 464 1 .000 505.372 2.120 123.22 122.80 ,34 5.9191 5,9323 -.22
19 465 1 .000 533.150 2.120 123.22 123.21 ,01 6.6879 6.6884 -.01
19 466 1 .000 560.928 2.120 123.22 123.46 -.20 7.4429 7.4314 .15
19 467 1 .000 588.706 2.120 123.22 123.77 -.45 8.1944 8.1642 .37
19 468 1 .000 422.039 2.297 133.49 131.89 1.20 3.5508 3.5578 -.20
19 469 1.000 449.817 2.297 133.49 132.25 ,92 4.4850 4.5014 -,36
19 470 1.000 477.594 2.297 133.49 133.03 ,34 5.3779 5,3878 -.18
19 471 1.000 505.372 2.297 133.49 133.41 .06 6.2432 6.2455 -.04
19 472 1.000 533.150 2.297 133.49 133.76 -.21 7.0947 7.0842 .15
19 473 1 .000 560.928 2.297 133.49 133.92 -.32 7.9290 7.9091 .25
19 474 1.000 436.428 2.505 145.62 143.07 1.75 4.1369 4.1557 -.45
19 475 1.000 455.150 2.505 145.62 144.35 .88 4.8263 4.8431 -.35
19 476 1.000 474.428 2.505 145.62 144.97 .45 5.5158 5.5283 -.23
19 477 1.000 494.094 2.505 145.62 145.35 .19 6.2053 6.2120 -.11
19 478 1.000 513.983 2.505 145.62 145.71 -.06 6.8948 6.8921 .04
19 479 1.000 533.983 2.505 145.62 146.09 -.32 7,5842 7.5669 .23
19 480 1.000 554.150 2.505 145.62 146.40 -.53 8.2737 8.2400 .41
19 481 1.000 434.317 2.756 160.18 155.84 2.71 4.1369 4.1592 -.54
19 482 1.000 450.817 2.756 160.18 158,39 1,12 4.8263 4.8446 -.38
19 483 1 .000 467,706 2.756 160.18 159.49 .43 5.5158 5.5265 -.19
19 484 1.000 484.983 2.756 160.18 159.91 .17 6.2053 6,2110 -,09
19 485 1.000 502.594 2.756 160.18 160.04 .09 6.8948 6.8986 -.06
19 486 1.000 519.817 2.756 160,18 160,83 -.40 7.5842 7.5634 .28
19 487 1.000 537.039 2.756 160.18 161.55 -.85 8.2737 8.2220 .63
19 488 1.000 432.650 3,062 177,98 172,67 2.99 4.1369 4.1542 -.42
19 489 1.000 447.039 3.062 177,98 176,67 .74 4.8263 4.8365 -.21
19 490 1.000 461.983 3.062 177.98 176,91 .61 5.5158 5.5294 -.25
19 491 1.000 476.983 3.062 177.98 177.44 .30 6.2053 6.2148 -.15
73
1
(XXXX)Haynes.

i Dens ty
i Dens ty i
''êxpt '
ca c
i
Pressure
Poi nt expt calc Diff, Diff,
No. K mol/L l<g/m^ kg/m^ MPa MPa
19 492 1.000 491 .983 3.062 177.98 178.07 -,05 6,8948 6,8928 ,03
19 493 1.000 507.039 3.062 177.98 178.59 -,34 7,5842 7,5674 .22
19 494 1.000 522.317 3.062 177.98 178.79 -,45 8,2737 8,2469 ,33
19 495 1.000 431.150 3.445 200,23 203.58 -1 ,67 4.1369 4.1306 .15
19 496 1.000 444.094 3.445 200.23 198.09 1,07 4,8263 4.8395 -.27
19 497 1.000 456.928 3.445 200.23 198.59 ,82 5,5158 5.5332 -.31
19 498 1.000 469.594 3.445 200.23 199.76 ,23 6,2053 6,2123 -.11
19 499 1.000 482.261 3.445 200,23 200.60 -,19 6,8948 6,8874 .11
19 500 1.000 494.983 3.445 200,23 201 ,14 -,45 7,5842 7,5620 .29
19 501 1.000 507,706 3.445 200,23 201 .59 -,68 8,2737 8,2336 ,49
19 502 1.000 430.761 3,675 213,58 216,60 -1,41 4.1369 4,1318 ,12
19 503 1.000 443.039 3,675 213,58 207,90 2,66 4,8263 4,8593 -,68
19 504 1.000 454.650 3,675 213.58 210,90 1 ,26 5.5158 5.5427 -,49
19 505 1.000 466.261 3,675 213.58 212.33 ,58 6.2053 6,2233 -,29
19 506 1.000 477.706 3,675 213.58 213.73 -,07 6.8948 6.8918 ,04
19 507 1.000 489.261 3,675 213,58 214.40 -,38 7.5842 7.5650 .25
19 508 1.000 500.928 3,675 213,58 214.67 -,51 8.2737 8.2428 ,37
19 509 1.000 441 .650 3,937 228,84 222.59 2,73 4.8263 4,8614 -,72
19 510 1.000 452.150 3.937 228,84 226.35 1,09 5.5158 5,5400 -,44
19 51 1 1.000 462.983 3,937 228,84 226.37 1,08 6,2053 6,2401 -,56
19 512 1.000 473.539 3,937 228,84 227.37 ,64 6,8948 6,9220 -.39
19 513 1.000 483.928 3,937 228,84 228.47 ,16 7.5842 7, 5927 -, 1
19 514 1.000 494.428 3,937 228,84 228.96 -,05 8.2737 8,2703 ,04
19 515 1.000 438.372 4,593 266,97 263.49 1,30 4,8263 4,8481 -,45
19 516 1.000 446.928 4.593 266,97 264.55 .91 5,5158 5,5411 -,46
19 517 1.000 455.428 4,593 266,97 264.94 ,76 6.2053 6,2352 -,48
19 518 1.000 463.872 4.593 266,97 265.20 ,67 6,8948 6.9287 -,49
19 519 1.000 472.428 4.593 266,97 264.85 ,80 7.5842 7,6343 -,66
19 520 1.000 480.817 4,593 266.97 265.02 ,73 8.2737 8,3286 -,66
19 521 1.000 433.039 5.512 320.37 318.41 ,61 4.8263 4,8554 -,60
19 522 1.000 439.150 5,512 320.37 318.99 ,43 5.5158 5,5428 -,49
19 523 1.000 445.206 5,512 320.37 319.28 ,34 6.2053 6,2317 -,42
19 524 1.000 451 .261 5,512 320,37 319.27 ,34 6.8948 6.9267 -,46
19 525 1.000 457.428 5,512 320,37 318.73 ,51 7.5842 7,6394 -,72
19 526 1.000 463.261 5,512 320,37 319.23 ,36 8,2737 8,3175 -.53
19 527 1.000 417.039 6,124 355,97 354.19 ,50 3,4474 3,4821 -1.00
19 528 1.000 426.983 6.124 355,97 354.30 ,47 4.8263 4.8769 -1 .04
19 529 1.000 431.594 6,124 355,97 355.41 ,16 5,5158 5.5356 -.36
19 530 1.000 436.428 6.124 355,97 355.31 ,18 6,2053 6.2320 -.43
19 531 1.000 440.928 6,124 355,97 356.18 -.06 6,8948 6.8850 .14
19 532 1.000 445.872 6, 124 355,97 355.52 ,13 7,5842 7.5068 -.30
19 533 1.000 450.428 6,124 355,97 355.94 ,01 8,2737 8,2753 -.02
19 534 1.000 413.706 6,484 376,91 373.78 ,83 3,4474 3,5525 -2.96
19 535 1.000 422,039 6,484 376,91 374.93 ,52 4,8263 4,9150 -1 .80
19 536 1.000 425.928 6.484 376,91 376.05 ,23 5,5158 5,5587 -.77
19 537 1.000 429.872 6.484 376,91 376.72 ,05 6.2053 6,2156 -.17
19 538 1.000 433.928 5.484 376,91 376.91 0,00 5.8948 6,8948 -.00
19 539 1.000 438.039 6.484 376,91 376.87 ,01 7.5842 7,5866 -.03
19 540 1.000 442,039 6,484 376,91 377.06 -.04 8.2737 8,2626 .13
19 541 1.000 403.261 6,890 400.46 401.24 -,20 2.7579 2,7173 1.49
19 542 1.000 407.039 6,890 400.46 400,53 -,02 3.4474 3,4436 .11
19 543 1.000 414.317 6,890 400.46 400.01 ,11 4.8263 4.8573 -.64
19 544 1.000 418.150 6,890 400.46 399.20 ,32 5,5158 5,6082 -1.65
19 545 1.000 421,539 6,890 400.46 399,57 ,22 6,2053 6.2750 -1.11
19 546 1.000 424,928 6.890 400.46 399,87 ,15 6,8948 6.9443 -.71
19 547 1.000 428.206 6.890 400.46 400,35 ,03 7,5842 7.5939 -.13
74
Q D
J 7 6/ . J
1\ 311
(XXXX)Haynes.
ID Data Weight Temp. Density Density Density ^êxpt '^calc

Pressure
19 548 1 .000 43 .483 1 6.890 400.46 400.76 -.08 8.2737 8.24 54 .34
19 549 1 .000 394 .81 7.349 427. 1 427.37 -.05 2.7579 2.7394 .67
19 550 1 .000 397.761 7.349 427. 16 427.32 -.04 3.4474 3.4321 .45
19 551 1 .000 403.706 7.349 427. 16 427.05 .03 4.8263 4.8376 -.23
19 552 1 .000 406.817 7.349 427. 16 426.60 .13 5.5158 5.5765 -1 .09
19 553 1 .000 409.872 7.349 427. 16 426.29 .20 6.2053 6.3042 -1 .57
19 554 1 .000 413.039 7.349 427. 16 425.77 .33 6.8948 7.0601 -2.34
19 555 1 .000 415.928 7.349 427. 16 425.81 .31 7.5842 7.751 -2.16
19 556 1 .000 419.094 7.349 427. 16 425.33 .43 8.2737 8.5104 -2.78
19 557 1 .000 388.817 7.602 441 .89 442.26 -.08 2.7579 2.7161 1 .54
19 558 1 .000 391 .483 7.602 44 .89 1 442. 15 -.06 3.4474 3.4 160 .92
19 559 1 .000 396.539 7.602 441 .89 442.50 -. 14 4.8263 4.7474 .66
1
19 560 1 .000 399.261 7.602 44 .89 1 442.26 -.08 5.5158 5.4664 .90
19 561 1 .000 401 .817 7.602 44 .89 1 442.34 -. 10 6.2053 6. 1425 .02
1
19 562 1 .000 404.261 7.602 44 .89 1 442.61 -.16 6.8948 6.7903 .54
1
19 563 1 .000 407. 50 1 7.602 44 .89 1 442.07 -.04 7.5842 7.5570 .36
19 564 1 .000 41 0.872 7.602 44 .89 1 440. 12 .40 8.2737 8.5466 -3. 19
19 565 1 .000 38 .872 1 7.874 457.67 457.33 .07 2.7579 2.8068 -1 .74
1 nnn 384 .094 7 R74. 457 fi7 4'57 57 09
. u^ 3,4474 3.462 -.43
Jyj 1 1 nnn ^RR 7nfi 7.R74 4. '57 fi7 457
^ uu
J 1 . fiR - . on
uu 4.8263 4.8245 .04
19 1 nnn 3qn 92R 7 R74 457 .67 457.87 -.04
. u^ 5. 5 1 58 5.4822 .61
1Q 1 nnn ^Q"? R79 7 R74. 4'i7 ft7 4 5R w\ - . 1Q
y1 0. £-\jJJ n5R'^
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0 fifi 474 fi9 474 R - n4 4 . 7R8
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19 579 1.000 387.150 8.166 474.62 474.83 -.04 7.5842 7.5381 .61
19 580 1 .000 390.317 8.166 474.62 473.17 .30 8.2737 8.5985 -3.78
19 581 1.000 367.594 8.480 492.88 492.81 .01 4.8263 4.8427 -.34
19 582 1.000 369.261 8.480 492.88 493.03 -.03 5.5158 5.4770 .71
19 583 1.000 370.928 8.480 492.88 493.24 -.07 6.2053 6. 1 1 14 1.54
19 584 1.000 372.594 8.480 492.88 493.44 -.11 6.8948 6.7458 2.21
19 585 1.000 374.594 8.480 492.88 493.16 -.06 7.5842 7.5072 1.03
19 586 1.000 377.039 8.480 492.88 492.28 .12 8.2737 8.4377 -1 .94
19 587 1.000 349.483 8.819 512.59 512.16 .08 2.7579 2.8876 -4.49
19 588 1.000 351.039 8.819 512.59 512.20 .08 3.4474 3.5684 -3.39
19 589 1.000 353.706 8.819 512.59 512.88 -.06 4.8263 4.7353 1.92
19 590 1.000 355.094 8.819 512.59 513.13 -. 10 5.5158 5.3428 3.24
19 591 1.000 356.483 8.819 512.59 513.37 -.15 6.2053 5.9502 4.29
19 592 1.000 359.594 8.819 512.59 513.41 -.16 7.5842 7.3103 3.75
19 593 1.000 361 .650 8.819 512.59 512.78 -.04 8.2737 8.2086 .79
75
11 1 11 .
1 11 .
Data sources and ID numbers; (l)Virial Equation, {3)Beattie, (19)Kay, (25)0lds, (29)Sage,
(XXXX)Haynes.
ID Data We ight Temp. Density Dens ty i Dens tyi p expt p ca c

,
I
Pressur
Poi nt expt ca c 1 Di ff Diff
No. K mol/L kg/m-^ kg/m^ % MPa MPa %
4302 594 1.000 140.000 12.809 744.53 743.88 .09 31.2779 32.8854 -4.89
4303 595 1 .000 140.000 12.784 743.04 742.49 .07 27.8345 29. 1743 -4,59
4304 596 1 .000 140.000 12,758 741.56 74 1 .08 .06 24.3914 25.5359 -4.48
4305 597 1.000 140.000 12.733 740.07 739.65 .06 20.9481 21.9549 -4.59
4306 598 1.000 140.000 12.707 738.59 738.20 .05 17.5051 18.4307 -5.02
4307 599 1.000 140.000 12.681 737.08 736.72 .05 14.0619 14.8951 -5.59
4308 600 1.000 140.000 12.655 735.54 735.22 .04 10.6191 .3508
1 1 -6.45
4309 601 1 .000 140.000 12.628 733.98 733.69 .04 7.1760 7.8265 -8.31
4310 602 1.000 140.000 12.601 732.44 732. 14 .04 3.7333 4.4005 -15.16
3601 603 1 .000 160.000 12.548 729.37 729.01 .05 36.0986 36.9184 -2.22
3602 604 1 .000 160.000 12.516 727.45 727. 18 .04 31 .9664 32.5829 -1 .89
3603 605 1 .000 160.000 12.483 725.55 725.31 .03 27.8343 28.3496 -1 .82
3604 606 1 .000 160.000 12.454 723.90 723.73 .02 24.391 24.7550 -1 .47
3605 607 1.000 160.000 12.426 722.25 722,12 .02 20.9479 21 .2376 -1 .36
3606 608 1 .000 160.000 12.397 720.58 720.47 .01 7.5048
1 7.7234
1 -1 .23
3607 609 1 .000 160.000 12.368 718.90 718.80 .01 14.0617 14,2744 -1 .49
3608 610 1 .000 160.000 12.345 71 7.55 717.44 .02 1 1 .3074 1 .5312
1 -1 .94
3609 61 1 .000 160.000 12.322 716.19 716.06 .02 8.5529 8.8182 -3.01
3610 612 1 .000 160.000 12.298 714.83 714.65 .02 5.7987 6. 1467 -5.66
361 613 1 .000 160.000 12.281 713.81 713.58 .03 3.7330 4. 1760 -1 0.61
3612 614 1 .000 160.000 12.263 71 2.77 712.50 .04 .6672 1 2. 1727 -23.27
3701 61 5 1 .000 180.000 12.263 712.75 712.48 .04 36.0984 36.6620 -1 .54
3702 616 1 .000 180.000 12.226 710.65 710.44 .03 31 .9664 32.3878 -1 .30
3703 617 1 .000 180.000 12. 189 708.47 708.35 .02 27.8343 28.0762 -.86
3704 618 1 .000 180.000 12. 157 706.62 706.57 .01 24.391 24.4925 -.41
3705 619 1 .000 180.000 12. 125 704.77 704.76 .00 20.9478 20.9834 -. 17
3706 620 1.000 180.000 12.093 702.90 702.90 0.00 17.5047 17.5051 -.00
3707 621 1 .000 180.000 12.061 701 .03 701 .01 .00 14.0616 14.1012 -.28
3708 622 1.000 180.000 12.034 699.49 699.46 .00 1 .3073 1 1 .3552 1 -.42
3709 623 1 .000 180.000 12.008 697.93 697.89 .01 8.5528 8.6180 -.76
3710 624 1.000 180.000 1 .980
1 696.33 696.29 .01 5.7986 5.8816 -1 .41
371 625 1.000 180.000 1 1 .961 695.20 695.06 .02 3.7329 3.9557 -5.63
3712 626 1 .000 180.000 1 1 .940 694.01 693.82 .03 1.6671 1 .9791 -15.76
3801 627 1 .000 200.000 1 1 .981 696.38 696.14 .03 36.0981 36.5395 -1 .21
3802 628 1 .000 200.000 1 .940
1 694.00 693.86 .02 31 .9662 32.2189 -.78
3803 629 1 .000 200.000 1 .899
1 691 .63 691 .53 .01 27.8341 28 . 0 1 44 -.64
3804 630 1 .000 200.000 1 .864
1 689.58 689.54 .01 24.3910 24.4689 -.32
3805 631 1 .000 200.000 1 .828
1 687.48 687.49 -.00 20.9477 20.9206 .13
3806 632 1 .000 200.000 1 .792
1 685.38 685.40 -.00 17.5047 17.4691 .20
3807 633 1 .000 200.000 1 .755
1 683.25 683.25 -.00 14.0616 14.0573 .03
3808 634 1 .000 200.000 1 . 725
1 68 . 50
1 681 .50 0.00 1 .3073 1 1 .3074 1 -.00
3809 635 1 .000 200.000 1 M/l
1 679.70 .00 8.5528 8.5718 -.22
3810 636 1 .000 200.000 1 663
1 677.89 677.86 .00 5.7986 5.8354 -.63
381 1 637 1 .000 200.000 1 .639
1 676.50 676.46 .0 3.7329 3.7939 -1 .61
3812 638 1 .000 200.000 11.615 675.10 675.02 .01 1 .6671 .7793 1 -6.31
3901 639 1.000 220.000 11.701 680.1 679.94 .02 36.0987 36.3776 -.77
3902 640 1.000 220.000 11.655 677.44 677.40 .01 31.9668 32.0217 -.17
3903 641 1.000 220.000 11.608 674.72 674.79 -.01 27.8346 27.7285 .38
3904 642 1.000 220.000 1 . 569
1 672.44 672.55 -.02 24.3914 24.2220 .70
3905 643 1.000 220.000 1 . 530
1 670.15 670.25 -.01 20.9481 20.8026 .70
3906 644 1.000 220.000 11.489 667.77 667.88 -.02 17.5050 17.3531 .88
3907 645 1.000 220.000 11.446 665.30 665.44 -.02 14.0618 13.8668 1.41
3908 646 1.000 220.000 11.410 663.20 663.43 -.03 11.3076 10.9962 2.83
3909 647 1.000 220.000 11.374 661 .1 661 .37 -.04 8.5530 8.2088 4.19
3910 648 1.000 220.000 11.338 658.98 659.25 -.04 5.7987 5.4583 6.24
76
D2 11 51 1 1 71
(XXXX)Haynes.
1 Data We ght
i Temp. Dens ty i Dens ty i Dens tyi p
expt p ca
1 c Pressur
Poi nt expt ca c 1 Diff. Diff.
No. K mol/L kg/m-^ kg/m-^ % MPa MPa %
391 549 1 .000 220.000 1 .310

1 657.39 657.62 -.04 3.7331 3.4357 8.66
391 650 1 .000 220.000 1 .283
1 655.79 655.96 -.03 1.6672 1 .4551 14.57
4001 651 1 .000 240.000 1 .424
1 663.98 663.83 .02 36.0977 36.3296 -.64
4002 652 1 .000 240.000 1 .372
1 661 .00 661 .00 .00 31 .9657 31 .9687 -.01
4003 653 1 .000 240.000 1 .320
1 657.98 658.07 -.01 27.8336 27.7063 .46
4004 654 1 .000 240.000 1 .275
1 655.36 655.55 -.03 24.3909 24. 1434 1.03
4005 655 1 .000 240.000 1 .229
1 652.66 652.94 -.04 20.9473 20.5820 1 .77
4006 656 1 .000 240.000 11.181 649.91 650.25 -.05 17.5042 17.0823 2.47
4007 657 1 .000 740.000 1 . 33
1 1 647.07 647.46 -.06 14.061 13.5989 3.40
4008 658 1 .000 240-000 1 .092
1 644.74 645. 1 -.06 1 .3069
1 10-8748 4.45
4009 659 1 .000 240.000 1 1 .051 642.31 642.77 -.07 8.5522 8.0299 6.50
660 1 .000 240.000 1 1 .008 639.86 640.3 -.07 5.7980 5.2994 9.41
40 1 661 1 .000 740.000 10.976 638.00 638.41 -.06 3.7324 3.2889 13.49
4012 662 1 .000 240.000 10.945 636 . 18 636.46 -.04 .6665
1 1 .3777 20.96
4101 663 1 .000 760.000 1 . 149
1 648.02 647.76 .04 36.0979 36.4519 -.97
4 102 664 1 .000 760-000 1 .092
1 644.71 644.60 .02 31 .9659 32 . 1 1 1 -.45
4 1 03 665 1 .000 760-000 1 .033
1 64 .31
1 64 .30
1 .00 27 .8339 27 .8391
4104 666 1 .000 260-000 10.983 638 . 39 638.45 -.01 24. 3908 24 . 3 6 1 .31
4 105 667 1 .000 260-000 10.931 635.35 635.49 -.02 20.9475 20.7759 .82
4106 668 1 .000 260-000 10.876 632. 17 632.42 -.04 17. 5045 17 .2294 1 .60
4107 669 1 .000 260-000 10.819 628.84 629.21 -.06 14.0613 13.5707 2.86
4 108 670 1 .000 260.000 10.771 626.07 626. 54 -.07 1 1 .3071 10.8399 4.31
4109 671 1 .000 260.000 10.723 623.27 623.76 -.08 8,5526 8.0753 5.91
4110 672 1 .000 260.000 10.673 620.36 620.88 -.08 5.7984 5.3 147 9. 10
4111 673 1 .000 260.000 10.635 618.17 618.64 -.08 3.7328 3.3 16 1 1 2 .72
41 12 674 1 .000 260.000 10.597 61 5.91 616.32 -.07 .6669
1 1.3154 26.72
4201 675 1 .000 280.000 10.846 630.43 630 . 52 -.01 34.7206 34.6103 .32
4202 676 1 .000 280.000 10.794 627.38 627.54 -.02 31 .2773 31.1014 .57
4203 677 1 .000 280.000 10.739 624. 17 624.44 -.04 27.8338 27.5496 1 .03
4204 678 1 .000 280.000 10.681 620.80 621 .20 -.07 24.3907 23.9675 1 .77
4205 679 1 .000 280.000 10.620 617.26 617.83 -.09 20.9475 20.3804 2.78
4206 680 1.000 280.000 10.557 613.59 614.29 -. 1 17.5045 16.8400 3.95
4207 681 1.000 280.000 10.491 609.80 610.58 -.13 14.0614 13.3646 5.21
4208 682 1.000 280.000 10.437 606.64 607.46 -.14 1 1.3071 10.6033 6.54
4209 683 1 .000 280.000 10.381 603.39 604. 19 -.13 8.5526 7.8982 8.29
4210 684 1 .000 280.000 10.323 600.02 600.77 -.12 5.7984 5.2 194 1.091
421 685 1.000 280.000 10.279 597.45 598.08 -.11 3.7328 3.2524 14.42
4212 686 1.000 280.000 10.234 594.83 595.27 -.07 1 .6669 .3515
1 23.33
3501 687 1 .000 300.000 10.573 614.53 614.27 .04 34.7208 34.9909 -.77
3502 688 1.000 300.000 10.514 61 1.1 1 610.92 .03 31.2774 31.4665 -.60
3503 689 1.000 300.000 10.452 607.49 607.41 .01 27.8340 27.9054 -.26
3504 690 1.000 300.000 10.386 603.65 603.73 -.01 24.3909 24.3144 .31
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1 J . /oyD 13.6869 .75
9R
ZD 1 1
1
nnn
.UUU 310.928 10.084 586.11 585.10 1 7 17/
1 . D'^ftQ
ZDoy 18.0005 -4.24
9R ODS. 1
1
nnn
. UUU 344.261 9.520 553.31 552.43 1ft 1
1
7/ . 9^ftQ
ZDoy 17.7406 -2.84
9R
ZD OJ D 1
1
nnn
.UUU 377.594 8.925 518.73 517.73 .
1 Q
ly 17/
1
9'^ftQ
.ZDoy 17.6585 -2.39
ZD 0 J4 1
1
nnn
.UUU 410.928 8.291 481.90 480.58 97 1
1
7/ .ZDDy
9XftQ 17.6406 -2.29
9^
ZD ODD 1
1
nnn
.UUU 444.261 7.598 441.64 440.75 9n
• zu 17/
1 . 9'^ftQ
ZDoy 17.4305 -1.11
9S
ZD 1
1
nnn
. UUU 477.594 6.842 397.68 398.50 - .Z
9 1
1
17 . 9'^ftQ
1 ^ joy
/ 17.1102 .74
9R
ZD OD / 1
1
nnn
.UUU 510.928 6.085 353.69 355.09 AO
— .4U 17/
1 . 9'^ftQ
zDoy 17.0750 ,95
9R
ZD 0 JO 1
1
nnn
.UUU 310.928 10.154 590.22 589.57 .
1
1
1
1
9n ftRA'^
ZU.D04D 21,2051 -2.46
9R
ZD 1
1
nnn
.UUU 344.261 9.619 559.11 558.26 . 1 D 9n 004
zu. ftR/1'^
J 21.2133 -2.49
9R
ZD R/10
O'tU 1
1
nnn
.UUU 377.594 9.054 526.23 525.49 .
1
1
4
4 9n
zu . ftRid'^
004 21.0366 -1.67
9
ZDR Q 1 /I 1
1
nnn
.UUU 410.928 8.474 492.57 491.08 .
^n
jU 9n ftQ>i T
ZU.004 21.2216 -2.53
ZD 842 1.000 444.261 7.845 455.98 455.07 9n
.ZU 9n ft QA
ZU.0043 T.
20.9289 -1.17
ZD 843 1
1
nr\A
.000 477.594 7.179 417.26 417.85 A
-. 114 9n ftQyl
ZU.D04 20.5648 ,58
ZD 844 1
1
Ann
.000 510.928 6.517 378.78 380.29 An
-.4U 9n ft Qyl
ZU.D04J 20.4452 1.17
1 A 24.6478 -2.09
25 845 1.000 310.928 10.226 594.38 593.77 . 1 24. 1315
25 846 1.000 344.261 9.707 564.23 563.63 .1
1 1
1 24. 1316 24.5336 -1.64
25 847 1.000 377.594 9.171 533.06 532.44 . 12 24. 1316 24.4558 -1.33
25 848 1.000 410.928 8.626 501.36 500.15 .24 24. 1316 24.6249 -2.00
25 849 1.000 444.261 8.049 467.83 466.91 ,20 24. 1316 24.4237 -1.20
25 850 1.000 477.594 7.442 432.58 433.11 -. 1 24. 1316 24.0008 .55
25 851 1.000 510.928 6.844 397.78 399.40 -.41 24. 13 16 23.8062 1.37
25 852 1.000 310.928 10.287 597.93 597.74 .03 27.5790 27.7434 -.59
25 853 1.000 344.261 9.787 568.84 568.62 .04 27.5790 27.7331 -.56
25 854 1.000 377.594 9.273 538.98 538.77 .04 27.5790 27.7010 -.44
25 855 1.000 410.928 8.760 509.17 508.19 .19 27.5790 28.0273 -1.60
25 856 1.000 444.261 8.227 478.16 477.07 .23 27.5790 27.9790 -1.43
25 857 1.000 477.594 7.664 445.45 445.78 -.07 27.5790 27.4837 .35
25 858 1.000 510.928 7.108 413.17 414.82 -.40 27.5790 27.1768 1.48
25 859 1.000 310.928 10.345 601.29 601.52 -.04 31 .0264 30.8183 .68
25 860 1.000 344.261 9.864 573.32 573.29 .00 31 .0264 31.0428 -.05
25 861 1.000 377.594 9.374 544.85 544.58 .05 31 .0264 31.1915 -.53
25 862 1.000 410.928 8.879 516.06 515.42 .12 31 .0264 31.3489 -1.03
25 863 1.000 444.261 8.377 486.88 486.00 .18 31 .0264 31.3901 -1.16
25 864 1.000 477.594 7.856 456.63 456.65 -.01 31.0264 31.0184 .03
25 865 1.000 510.928 7.353 426.25 427.79 -.36 31.0264 30.5886 1.43
80
(XXXX)Haynes.
D Data Weight Temp. Dens ity Dens ty i Dens tyi

^C3 C
I
Pressur
No. K mol/L kg/m^ i<g/m^ % MPa MPa %
25 866 1.000 310.928 10.404 604.70 605.11 -.07 34.4738 34.0697 1.19
25 867 1.000 344.261 9.935 577.45 577.69 -.04 34.4738 34.2789 .57
25 868 1.000 377.594 9.464 550.08 549.97 .02 34.4738 34.5517 -.23
25 869 1.000 410.928 8.989 522.45 522.01 .09 34.4738 34.7202 -.71
25 870 1.000 444.261 8.516 495.01 493.99 .21 34.4738 34.9397 -1.33
25 871 1.000 477.594 8.023 466.33 466.20 .03 34.4738 34.5225 -.14
25 872 1.000 510.928 7.526 437.42 439.00 -.36 34.4738 33.9619 1.51
25 873 1.000 310.928 10.515 61 1.16 61 1.84 -.11 41.3685 40.6438 1.78
25 874 1.000 344.261 10.076 585.68 585.79 -.02 41.3685 41.2710 .24
25 875 1.000 377.594 9.629 559.69 559.72 -.00 41.3685 41 .3507 .04
25 876 1.000 410.928 9.186 533.95 533.69 .05 41.3685 41.5322 -.39
25 877 1.000 444.261 8.754 508.85 507.87 .19 41.3685 41.8994 -1 .27
25 878 1.000 477.594 8.306 482.77 482.47 .06 41.3685 41 .5091 -.34
25 879 1.000 510.928 7.847 456.11 457.75 -.36 41.3685 40.7022 1 .64
25 880 1.000 310.928 10.612 616.81 618.05 -.20 48.2633 46.8447 3.03
25 881 1.000 344.261 10.199 592.84 593.14 -.05 48.2633 47.9678 .62
25 882 1.000 377.594 9.773 568.03 568.39 -.06 48.2633 47.9615 .63
25 883 1.000 410.928 9.364 544.29 543.87 .08 48.2633 48.5648 -.62
25 884 1.000 444.261 8.959 520.76 519.71 .20 48.2633 48.9193 -1.34
25 885 1.000 477.594 8.545 496.70 496.08 .12 48.2633 48.6023 -.70
25 886 1.000 510.928 8.118 471.83 473.16 -.28 48.2633 47.6182 1.35
25 887 1.000 310.928 10.703 622.08 623.82 -.28 55. 1581 53.0290 4.01
25 888 1.000 344.261 10.318 599.72 599.88 -.03 55.1581 54.9898 .31
25 889 1.000 377.594 9.910 576.00 576.23 -.04 55.1581 54.9459 .39
25 890 1.000 410.928 9.520 553.31 552.93 .07 55.1581 55.4693 -.56
25 891 1.000 444.261 9.129 530.59 530.08 .10 55.1581 55.5157 -.64
25 892 1.000 477.594 8.741 508.04 507.82 .04 55.1581 55.2935 -.24
25 893 1.000 510.928 8.351 485.41 486.29 -.18 55. 1581 54.6653 .90
25 894 1.000 310.928 10.795 627.44 629.22 -.28 62.0528 59.7311 3.89
25 895 1.000 344.261 10.419 605.61 606.11 -.08 62.0528 61 .4836 .93
25 896 1.000 377.594 10.032 583.13 583.39 -.05 62.0528 61 .7870 .43
25 897 1.000 410.928 9.656 561 .26 561.11 .03 62.0528 62.1925 -.22
25 898 1.000 444.261 9.288 539.89 539.34 .10 62.0528 62.4870 -.69
25 899 1.000 477.594 8.916 518.23 518.18 .01 62.0528 62.0842 -.05
25 900 1.000 510.928 8.553 497.16 497.76 -.12 62.0528 61.6728 .62
25 901 1.000 310.928 10.876 632.14 634.30 -.34 68.9476 65.9679 4.52
25 902 1.000 344.261 10.515 61 1.16 61 1.92 -.13 68.9476 68.0138 1.37
25 903 1.000 377.594 10.147 589.78 590.00 -.04 68.9476 68.7078 .35
25 904 1.000 410.928 9.790 569.04 568.58 .08 68.9476 69.3934 -.64
25 905 1.000 444.261 9.444 548.95 547.71 .23 68.9476 70.0280 -1.54
25 906 1.000 477.594 9.086 528. 14 527.48 .13 68.9476 69.4654 -.75
25 907 1.000 510.928 8.729 507.40 507.96 -.11 68.9476 68.5440 .59
81
5
1 1 1
Data sources and ID numbers: (DVirial Equation, (3)Beattie, (19)Kay, (25)01ds, (29)Sage,
(XXXX)Haynes,
D Data We ight Temp, Dens ty i Dens ty i Dens ity ^©x pi" P C9 C

1
Pressur
Poi nt expt ca c1 Diff, Diff.
No, K moi/L kg/frP kg/m-^ % M.Pa MPa %
29 908 .000 294.261 .043 2.48 2.49 -,21 .1013 .101 .21
29 909 .000 294.261 .059 3.42 3.43 -,09 .1379 .1378 .09
29 910 .000 294.261 .091 5.26 5.26 ,09 .2068 ,2070 -.08
29 91 1 .000 294.261 10.062 584.83 579.62 ,89 1.7237 5,0879 -66. 12
29 912 .000 294.261 10.121 588.27 582.34 1,01 3.4474 7.4607 -53.79
29 913 .000 294.261 10, 173 591.31 584.95 1,07 5. 171 9.6655 -46.50
29 914 .000 294.261 10.218 593,94 587.46 1.09 6.8948 1 1.5557 -40.85
29 915 .000 294.261 10,256 596, 15 589.88 1.05 8,6184 13.3881 -35.63
29 916 .000 294.261 10.299 598,60 592.21 1.07 10,3421 15.3744 -32.73
29 917 .000 294.261 10.341 601 ,07 594.47 1.10 12,0658 17.4482 -30.85
29 918 .000 294.261 10,380 603,33 596.65 1,11 13,7895 19.4126 -28.97
29 919 .000 294.261 10.41 605.38 598.77 1,09 15,5132 21.2471 -26.99
29 920 .000 294.261 10.447 607.22 600.82 1,05 17,2369 22.9325 -24.84
29 921 .000 294.261 10.475 608.84 602.82 ,99 18,9606 24.4507 -22.45
29 922 .000 294.261 10.487 609.53 604.76 .78 20,6843 25.1 140 -17.64
29 923 .000 310.928 .040 2.34 2.34 -. 18 ,1013 .1012 .17
29 924 .000 310.928 .055 3.22 3.22 -.12 ,1379 .1377 .12
29 925 .000 310.928 .085 4.92 4.92 -,02 ,2068 ,2068 .02
29 926 .000 310.928 .115 6.70 6.69 ,13 ,2758 ,2761 -.12
29 927 .000 310.928 .148 8.58 8.55 ,33 ,3447 ,3458 -.30
29 928 .000 310.928 9.71 564,43 560.20 ,75 1.7237 3,9457 -55.31
29 929 .000 310.928 9,773 568,03 563,51 ,80 3.4474 5,9663 -42.22
29 930 .000 310.928 9,825 571.07 566,64 ,78 5.1711 7,7630 -33.39
29 931 .000 310.928 9.881 574.34 569,62 ,82 6.8948 9,7990 -29,64
29 932 .000 310.928 9.935 577.45 572.47 ,86 8.6184 11,8259 -27,12
29 933 .000 310.928 9.982 580. 17 575.19 .86 10.3421 13,6799 -24,40
29 934 .000 310.928 10.025 582.70 577.81 .84 12.0658 15,4753 -22,03
29 935 .000 310.928 10.073 585.47 580.33 .88 13.7895 17,5152 -21,27
29 935 .000 310.928 10.117 588.05 582.75 .90 15.5132 19,4898 -20,40
29 937 .000 310.928 10.166 590.87 585.10 .98 17.2369 21,7325 -20,69
29 938 .000 310.928 10.207 593.28 587.37 1.00 18.9606 23,7179 -20,06
29 939 .000 310.928 10.241 595.26 589.57 .96 20.6843 25,4044 -18,58
29 940 .000 327.594 .038 2.21 2.22 -.11 .1013 ,1012 ,11
29 941 .000 327.594 .052 3.04 3.04 -.06 .1379 .1378 ,06
29 942 .000 327.594 .080 4.63 4.63 ,04 .2068 .2069 -,04
29 943 .000 327.594 .108 6.28 6.27 ,16 .2758 .2762 -,15
29 944 .000 327.594 .138 8.00 7.98 ,22 .3447 .3454 -,21
29 945 .000 327.594 .168 9.79 9.75 ,40 .4137 .4152 -,36
29 946 .000 327.594 .201 11.66 11.61 ,48 .4826 .4847 -,42
29 947 .000 327.594 ,235 13.63 13.55 ,58 .5516 .5543 -,49
29 948 .000 327.594 9,355 543.74 539.31 ,81 1.7237 3.5829 -51,89
29 949 .000 327.594 9,432 548.20 543.43 ,87 3,4474 5,6109 -38,56
29 950 .000 327.594 9,500 552. 17 547.26 ,89 5.1711 7,5451 -31.46
29 951 .000 327.594 9,566 556.00 550,87 ,92 6.8948 9,5360 -27,70
29 952 .000 327.594 9,633 559.89 554,27 1,00 8.6184 11,6824 -26,23
29 953 .000 327.594 9,690 563.24 557,49 1,02 10.3421 13,6372 -24,16
29 954 .000 327.594 9,742 566.22 560, 56 1,00 12.0658 15,4674 -21,99
29 955 .000 327.594 9.790 569.04 563,49 ,98 13.7895 17,2595 -20,15
29 956 .000 327.594 9.846 572.29 566.30 1,05 15.5132 19,4459 -20,22
29 957 .000 327.594 9.896 575.17 568.99 1,07 17.2369 21,4577 -19,57
29 958 .000 327.594 9.94 5 578.08 571.58 1,12 18.9606 23,5748 -19,57
29 959 .000 327.594 9.985 580.38 574.08 1,09 20.6843 25.3154 -18,29
29 960 .000 344.261 .036 2. 10 2.10 -,09 .1013 .1012 ,09
29 961 .000 344.261 .050 2.88 2,88 -.05 .1379 .1378 ,04
29 962 .000 344.261 .075 4.38 4,38 .03 .2068 .2069 -,03
82
1 1
Data sources and ID numbers: (l)Virial Equation, (3)Beattle, {19)Kay, (25)0lds, (29)Sage,
(XXXX)Haynes,
ID Data Weight Temp, Dens ty

1 Dens tyi Dens tyi
êxpt '^ca 1 c Pressure
Pol nt expt calc DIff, Diff.
No. K mol/L kg/m-' kg/rn^ % MPa MPa %
29 963 .000 344.261 .102 5,92 5,91 ,16 ,2758 ,2762 -.16
29 964 .000 344.261 .129 7,52 7.50 .26 ,3447 .3456 -.24
29 965 .000 344.261 .158 9,17 9.13 .38 ,4137 .4151 -.35
29 966 .000 344.261 ,187 10.87 10.82 .43 ,4826 .4845 -.38
29 967 .000 344.261 ,217 12.63 12.57 .49 ,5516 .5540 -,43
29 968 .000 344.261 ,249 14.47 14.39 .53 ,6205 .6234 -,45
29 969 .000 344.261 .282 16.37 16.29 .50 ,6895 .6924 -.42
29 970 .000 344.261 8.977 521.77 516.36 1.04 1,7237 3.4838 -50.52
29 971 .000 344.261 9.074 527.44 521.67 1.10 3,4474 5.5245 -37.60
29 972 .000 344.261 9. 159 532.35 526.50 1.10 5. 171 7.4631 -30,71
29 973 .000 344.261 9.236 536.81 530.96 1.09 6,8948 9.3704 -26,42
29 974 .000 344.251 9.314 541.35 535.09 1.16 8.6184 11.4587 -24,79
29 975 .000 344.261 9.380 545.22 538.96 1.15 10.3421 13.3641 -22,61
29 976 .000 344.261 9.448 549. 14 542.61 1.19 12.0658 15.4180 -21 ,74
29 977 .000 344.261 9.510 552.74 546.05 1.21 13.7895 17.4131 -20,81
29 978 .000 344.261 9.569 556.20 549.32 1.24 15.5132 19.431 -20. 16
29 979 .000 344.261 9.623 559.30 552.43 1.23 17.2369 21,3355 -19.21
29 980 .000 344.261 9.670 562.05 555.41 1. 18 18.9606 23,0919 -17.89
29 981 .000 344.261 9.707 564.23 558.26 1.06 20.6843 24,5336 -15.69
29 982 .000 360.928 .034 2,00 2.00 -.05 .1013 ,1013 ,04
29 983 .000 360.928 .047 2,74 2,74 -.00 ,1379 ,1379 ,00
29 984 .000 360.928 .071 4,16 4,15 .07 ,2068 ,2070 -,07
29 985 .000 360.928 .097 5,61 5.60 .21 ,2758 .2763 -,20
29 986 .000 360.928 ,122 7,10 7.08 .32 ,3447 .3458 -,30
29 987 .000 360.928 .149 8,64 8.60 .41 ,4137 .4153 -,38
29 988 .000 360.928 .176 10,21 10. 16 .47 ,4826 .4847 -,43
29 989 .000 360.928 .203 11,83 11.77 .48 ,5516 .5540 -,43
29 990 .000 360.928 .232 13.50 13.42 .55 ,6205 .6236 -,49
29 991 .000 360.928 .262 15.21 15.13 .53 ,6895 .6927 -,46
29 992 .000 360.928 .340 19.79 19.68 .57 ,8618 .8659 -,47
29 993 .000 360.928 .427 24.79 24.71 .33 1,0342 1.0369 -,26
29 994 .000 360.928 8.495 493.79 490.31 .70 1,7237 2.5204 -31,61
29 995 .000 360.928 8.620 501.05 497.55 .70 3,4474 4.3730 -21,17
29 996 .000 360.928 8.729 507.40 503.89 .69 5,1711 6.2172 -16,83
29 997 .000 360.928 8.830 513.25 509.55 .72 6,8948 8.1 161 -15,05
29 998 .000 360.928 8.925 518.73 514.70 ,78 8,6184 10.0799 -14.50
29 999 .000 360.928 9.015 523.99 519.43 .87 10,3421 12.1408 -14.82
29 1000 .000 360.928 9.095 528,66 523.81 .92 12,0658 14,1236 -14,57
29 1001 .000 360.928 9. 171 533,06 527.90 .97 13,7895 16, 1297 -14.51
29 1002 .000 360.928 9.242 537,17 531.74 1.01 15,5132 18,1320 -14.44
29 1003 .000 360.928 9.307 540,98 535.37 1.04 17,2369 20, 1012 -14.25
29 1004 .000 360.928 9.205 535,02 538.80 -.71 18.9606 17,0679 1 1.09
29 1005 .000 360.928 9.415 547.27 542.07 .95 20.6843 23,5998 -12.35
29 1006 .000 377.594 .033 1.91 1.91 -.01 .1013 ,1013 .01
29 1007 .000 377.594 .045 2.61 2.61 .04 .1379 ,1380 -.04
29 1008 .000 377.594 .068 3.96 3.95 .14 .2068 .2071 -.14
29 1009 .000 377.594 .092 5,33 5.32 .27 .2758 .2765 -.26
29 1010 .000 377.594 .1 16 6.74 6.72 .34 .3447 .3459 -.33
29 1011 .000 377.594 .141 8. 18 8, 14 .47 .4137 ,4155 -.44
29 1012 .000 377.594 ,166 9,65 9,60 .52 ,4826 ,4850 -.49
29 1013 .000 377.594 .192 11.15 11,09 ,55 ,5516 ,5544 -.51
29 1014 .000 377.594 .218 12.69 12,62 ,56 ,6205 ,6237 -.51
29 1015 .000 377.594 .245 14.26 14, 18 ,55 ,6895 ,6929 -.49
29 1016 .000 377.594 .316 18,38 18,29 ,51 ,8618 ,8656 -,44
29 1017 .000 377.594 .392 22,81 22,71 ,45 1,0342 1.0380 -,37
29 1018 .000 377.594 ,476 27,66 27,53 ,46 1,2066 1.2109 -,36
83
1 1 1 1 .1
Table 7, (Continued)
Data sources and ID numbers: (l)Virlal Equation, (3)Beattie, (19)Kay, (25)0lds, (29)Sage,
(XXXX)Haynes.
D Data We ght
i Temp. Dens ity Dens ty i Dens ty I
expt P„^
'
„
ca c 1
1
Pressure
Point expt ca c 1 Dlff. Di f f
No. K mol/L kg/m-^ kg/m-^ % MPa MPa
29 1019 .000 377.594 .569 33.07 32.88 .57 .3790

1 1 .3847 -.4 1
29 1020 .000 377.594 .675 39.24 38.96 .72 .5513

1 1 .5587 -.47
29 1021 .000 377.594 7.937 461 .36 458.95 .52 .7237
1 2.0697 -16.72
29 1022 .000 377. 594 8.113 471 .55 469.84 .36 3.4474 3.7570 -8. 24
29 1023 .000 377.594 8.254 479.74 478.67 .22 5.171 5.4023 -4.28
29 1024 .000 377. 594 8. 392 487. 77 486. 18 .33 6.8948 7. 2934 -5.47
29 1 025 .000 377.594 R S97 40S fi9 492.75 .58 8.6184 9.4314 -8.62
29 1026 .000 377. 594 o. uû S01 '^fi 498.66 .54 10.3421 1 1 . 1923 -7.60
29 1 027 .000 377. 594 ft 79 SOfi 0 1
504.01 .57 17.0658 13.0660 -7.65
1 09R .000 377. 594 ft ftOft ill
J \ \
04
• 7*T 508.93 .59 13.7895 14.9132 -7 5"^
1 090 oon 377. 504 ft ftft4 R

J 1 fi
\
^0
\J% _?7 51 3.4R .56
. JU 1 5. 51 39 16.6R00 -7 no
?9 1 030 000 377 m. J504
J 1 17^ ft Qfi? S90 O'^ 51 7.73 .61 17,2369 1ft. 6074 -7 ^7
1 f)"^ 1 000 377 "504 0 09 1 i94 "^4 .50 1ft OfiOfi -5 ftQ
9Q 000 377. 504 7. 077
0 U/ / K97/ . CO
DZ .40 90.6R43 91 7n^*S -4 70
000 ^04
J 9fi1
7*+ . ^(J I
O'^ 1 R9
1 1 ft? 101 1 ni4
90 000 '104
-J7H . 9fi1
1
04 9
Z. "lO
IjU 9 • AQ
^ .
"^70
11 -J /7 • 1
1
'^RC\
DO\J
9Q 1 (W^ 000 ^04
7H . Z.U
9fi1 I
7ft ^ 77 1Q • £.\J f £-
- ft
1
1 (T^fi 000 "^04 9fi1 ORft S

J. 00
U7 ^ 07 97 Sft
• ^,1 JO m £. 1 \J 1
- "^9
90 1t
\JJ 1 000 ^04
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7*T . ^ U 1
I 10 fi 49 u• 44 "^447 •
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DZ, - 49
90 1 U JO 000 394 961 . 1
1
7 7ft 7/ • 74.
/ *T • -û 4 1
^^7 4 1 SQ - 54
90 1i O'Ô
U J7 000 394.261 . 11
JO
Sft 0 U
7 . Ifi I • \j \
4ft 54 - 57
90 000 ^04 9fi1 1 fl9 1 0 R7 in sn • u^
90 lOil 1 000 ^04 9fil 907 19
1 Z. U01 1
1 1
Q"^ 6905 - fi4
90 1 049 000 ^04 9fi1 1 47 1 J • DO .uo 7 J - 5Q
90 1 043 000 394.961 907
^7. / 1 7 9'=; 1 7. 1 S D\j .R6
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90 1 044 000 "^04 9fi1 JUQ
. 91 96 1 .0349 - 45
99 1 045 .000 394.261 440 25.41 -54 1 .2066 K? 1 ?n -.45
90 000 304 96 570 30 9 90.00
^7.77 .71 1 .3790 5fi
90
^7 1 047 000 304.961 .60R 35. 36 ^4.97 1.10 11 .5513
m JJ J \
29 1 048 .000 394.261 .706 4 . 06

1 40.46 1.47 1 .7237 1 .74 16 -1 .03
90 1 049 .000 394.261 810 47. 59 46.63 2.02 1 .8961 1 .9209 -1 .29
29 1050 .000 394. 261 .949
. 7t 7 55.16 53.79 2.49 2.0684 2.0982 -1 .42
29 1 051 .000 394.261 7.471 434.22 435.83 -.37 3.4474 3.2783 5. 16
29 1052 .000 394.261 7.709 448.07 449. 50 -.32 5. 17 1 4.9656 4. 14
29 1053 .000 394.261 7.897 458.98 460.08 -.24 6.8948 6.6991 2.92
29 1054 .000 394.261 8.049 467.83 468.83 -.21 8.6184 8.4059 2.53
29 1055 .000 394.261 8. 178 475.33 476.38 -.22 10.3421 10.0880 2.52
29 1056 .000 394.261 8.293 482.05 483.03 -.20 12.0658 11.7982 2.27
29 1057 .000 394.261 8.397 488.07 489.02 -. 19 13.7895 13.5049 2.1
29 1058 .000 394.261 8.488 493.33 494.47 -.23 15.5132 15.1406 2.46
29 1059 .000 394.261 8.569 498.09 499.49 -.28 17.2369 16.7421 2.96
29 1060 .000 394.261 8.647 502.62 504.14 -.30 18.9606 18.3830 3.14
29 1061 .000 394.261 8.718 506.75 508.49 -.34 20.6843 19.9820 3.51
84
. . .
1
Table 8. Comparisons of data for ideal gas functions with eq (7).
Normal butane ideal gas functions from Chen, et al. (12]
Temp. J/ mo 1 Di tf S*^, J/(mol K) Di f f C°, J/(mo 1 K) Di f f
expt. cal c. expt. ca c. expt. cal c. d

K % 1
%
50.00 1718.0 1750.3 -1.88 198.363 198.892 -.27 38.07 38.08 -.01
100.00 4048.9 4041.8 .17 229.994 229.925 .03 55.35 55.34 .03
150.00 7142.7 7143.6 -.01 254.889 254.915 -.01 67.32 67.37 -.07
200.00 10736.1 10733.0 .03 275.516 275.505 .00 76.44 76.33 .14
273.15 16883.5 16881 .3 .01 301 .583 301 .574 .00 92.30 92.40 -. 1
298.15 19267.0 19268.1 -.01 309.909 309.931 -.01 98.49 98.59 -.10
300.00 19450.6 19450.9 -.00 310.536 310.542 -.00 98.95 99.05 -. 10
400.00 30636.9 30632.2 .02 342.544 342.533 .00 124.77 124.54 . 18
500.00 44333.7 44299.9 .08 373.004 372.932 .02 148.66 148.37 . 19
600.00 60259.6 60207.1 .09 401.999 401.877 .03 169.28 169.26 .01
700.00 78096.5 78054.9 .05 429.446 429.354 .02 187.02 187.23 -. 1
800.00 97584.3 97567.5 .02 455.428 455.386 .01 202.38 202.63 -.12
900.00 118507.2 118509.3 -.00 480.072 480.037 .01 215.73 215.88 -.07
1000.00 140674.4 140684.2 -.01 503.419 503.390 .01 227.36 227.35 .00
1100.00 163928.3 163930.2 -.00 525.552 525.538 .00 237.48 237.35 .06
1200.00 188124.4 188113.2 .01 546.640 546.574 .01 246.27 246.13 .06
85
111 • 8
11
11 9 3
I aD e y 1 1 n r er po d cu i i lUtJdl IUIH-.I lUHo ÎIr* \J\\\

r\rf\ cii^ (
V
1
'
\
/ •
Tornp • H°-H°
II IQ 1
V P
K J/mo 1 J/mo 1 J/ Cmol »K) J/ (mo 1 •t\.) J/ (mo 1
130.0 4753.0 5833.9 245.551 55. 17 63.48

£ C CI
140.0 5315. 6479. 250.331 57. 20 55.51
"7 "7 "7
150.0 5896.4 7143.6 254.915 59.05 67.37
160.0 6495.8 7826. 259.3 1 60.82 69. 1
170.0 71 12.7 8526.2 263.563 62. 56 70.88

180.0 7747. 9243.7 267.663 64.32 72.54
1 A A C
74.45
190.0 8399.4 9979. 271.639 66. 14
200.0 9070. 10733.0 275. 505 68. 02 76.33
210.0 9760.0 11506.0 279.276 69.98 78.29
220.0 10469.9 12299. 282.965 72.02 80.33
230.0 11200.6 131 12.9 286.583 74. 14 82.45
240.0 11952.9 13948.4 290. 138 76. 34 84 .65
250.0 12727.6 14806.2 293.639 78.61 86.92
260.0 13525.2 15687.0 297.094 80.94 89. z5
270.0 14346.5 16591 .4 300.507 83.32 9 .541
280.0 15191 .9 17519.9 303.883 85.76 94.07

290.0 16061.8 18473.0 307.227 88.23 96.55
300.0 16956.6 19450.9 310.542 90.74 99.05
310.0 17876.6 20454. 313.831 93.27 10 .58 1
320.0 18822.0 21482.6 31 7.097 95.82 104. 13

330.0 19792.9 22536.7 320.340 98.38 106.69
340.0 20789.5 2361 6.4 323.563 1 00.94 1U9. z6
350.0 2181 1 .8 24721 .8 326.767 103.51 1 1 1 .82
360.0 22859.7 25852.9 329.953 106.07 1 14.39
370.0 23933.2 27009.6 333. 122 108.63 1 16.95
380.0 25032.3 28 9 1 1 . 336.275 111.18 1 19.49
390.0 26156.7 29399.4 339.4 12 113.71 1 22.02
16.22 1 O . 1)4
Z4 C^/l
/I
400.0 27306.4 30632.2 342. 533 1 1
8.72 1 O ~7
z / . CtA
U4
410.0 28481 . 31890. 34 5.639 1 1 1
1O .ZU
O^
420.0 29680.7 331 72.8 348.730 Izl 1 1
430.0 30905.0 34480.2 35 .806

1 1 J 1 . yo
1 0£
Z6. A~7 j4. jy
440.0 321 53.6 3581 2.0 354.867 1 U/ 1
450.0 33426.4 37167.9 357.9 14 1 28.48 1JO. /y

460.0 34723.0 38547.7 360.947 1 30.85 139. Id
470.0 36043.3 39951 . 363.965 133. 19 141.51
1 O "7 "Z
480.0 37386.8 41377.8 366.969 135.51 1 43.83
j1
1 11
490.0 38753.4 42827.5 369.958 137.80 146.yl
1 1
1 yi o x~i
500.0 40142.7 44299.9 372.932 140.06
CA CA
510.0 41554.4 45794.8 375.893 142.28 1
150.50
520.0 42988.2 4731 1 .8 378.838 144.48 152.79
530.0 44443.9 48850.6 381.769 146.64 154.96
540.0 45921.0 50410.9 384.686 148.78 157.09
550.0 47419.4 51992.4 387. 588 150.88 159.20
560.0 48938.6 53594.7 390.475 152.96 161 .27
570.0 50478.4 55217.7 393.347 155.00 163.32
580.0 52038.5 56861 .0 396.205 1 57.01 165.33
590.0 53618.6 58524.2 399.048 159.00 167.31
600.0 55218.4 60207. 401 .877 160.95 169.26
610.0 56837.5 61909.4 404.690 162.87 171.19
620.0 58475.8 63630.8 407.489 164.77 173.08
630.0 60132.8 65371 .0 410.274 166.63 174.95
640.0 61808.4 67129.6 413.043 168.47 176.78
650.0 63502. 68906.6 415.798 170.28 178. 59
660.0 65213.9 70701.4 , 418.539 172.06 180.37
670.0 66943.3 72514.0 421.264 173.81 182.13
680.0 68690.0 74343.9 423.975 175.54 183.86
690.0 70454.0 76191 .0 426.672 177.24 185.56
700.0 72234.8 78054.9 429.354 178.91 187.23
85
1
1
1 1 . 1 . 7
Table 10. Comparisons of heat of vaporization data with

eq (9).
Data sources and ID numbers: (lO)Dana, (ll)Das (1967), (29)Sage,
(35)Das ( 1973) , (40) nerma Loops, (4 1) C apeyron
1 1
ID Weight Temp. Heat of Vaporization Diff,

K kj/mo %
expt. ca c 1
40 1 .000 A OCA 28.746 28.789

40 .998 1 40.000 28.499 28.521 -•03
1C A AAA AO
40 .995 150.000 28.022 28.016 .02
1 /IA AAA
60.000 27.553 27.533 A~7
40 .992 1 .0 /
40 •
AOO
988 170.000 27.090 27.067 AO
.08
O A AAA A "7
40 .984 1
180.000 26.635 26.615 .07
40 A~7 A AA AAA
1
26. 186 26. 174 AC
.05
40 AT>I
.y /4 OAA AAA 25.742 25.739 .UA 1
1
A A
40 .yoy O A AAA
1
25.301 25.307 -. AO
Uz
AA
40 .yoj OOA AAA 24.861 24.875 AC^
-.UP
A A OR"?/
.yp 24.417 24.438 AQ
Uo
A A •ysu Z4U»UUU 23.965 23.992 — • 11 1 1
Ar\
4U »y4j Z.^\J • UUU 23.503 23.535 — A 1
AA .yj4 23.024 23.061 .10

z / U ©UUU 22.524 22.567 _ 1 A
4U . yzz>
A 1
.yyo 28.521 28.521 nn
.UU
A 1
. yy3 23.032 28.016 . UP
j1 1
•yy 1 1 DU •UUU 27.551 27.533 .un7/
yi 1
•yoD nn nnn
/U aUUU
1 27.082 27.067 AA
.uo
/
4 1
1 •yoz ion nnn
oU«UUU
1 26.624 26.615 A"^
.UP
A
4 1
1 .y / /„ 1on
1
nnn
yu .UUU 26.176 26.174 A
.U 1
1
A
4 1
1
ATI
.971 OAA AAA 25.735 25.739 A
-.U 1
1
4
>i 1
1 •yoD Z A
O AAA
U.UUU
1
1 25.299 25.307 A'^
-.Up
4 .ypy OOA AAA
ZZU.UUU 24.865 24.875 - .U4
4 1 •yDii OX A AAA
ZÛ.UUU 24.429 24.438 A/t
-. U4
A O ^ A AAA 23.987 23.992 AO
-.02
4 1
1 .945 Z4 U.UUU
A 1
.yjo OCA AAA
zdU .UUU 23.536 23.535 AA
.UU
4 1
AOT
.92/ OjCA AAA
zoU.UUU 23.070 23.061 r\A
.U4
4
yi 1
1
AIT/
.y 1
0~lf\ AAA
Z/U .UUU 22.586 22.567 AA
.uy
4 1
AAC OOA AAA
ZoUpUUU 22.077 22.048 . I 5
A
4 1
1
QQO
.cjy^ OOA • Ann
zVU UUU 21 .535 21 .500 . 1 /
A "ZAA AAA
4 1
1 .875 500.000 20.955 20.917 . 18
4 D KA
•859 "Z 1A AAA
510.000 20.328 20 . 294 . 1
1 T O A AAA
it
4 1 • 859 520.000 19.650 19.626 . 12
O c T A AAA
"2 AC
4 \ •815 1
530.000 18.915 18.906 .05
41 • 786 340.000 18.118 18.125 -.04
41 • 751 350.000 17.253 17.274 -.12
1 A AAA
411
yi
• 708
£r
350.000 16.312 16.340 -. 1 7
A 1
4 1 • o53 37U AAA
ZTA .UQU 15.282 15.306 -.15
A 1 T O A AAA
41 • 581 580.000 14.139 14.147 -.06
4 •484 7AA AAA
590.000 12.841 12.824 1 "Z
15
1 .
A A AAA
4 0.000 400.000
>I
11.306 11.262 .39
A ^ A AAA
4 1
0.000 1
4 1 0 .000 9.344 9.292 .56
A
4 1
1
A AAA
0.000 O A AAA
y»
420.000 6.264 6.273 -.15c 1
1 1
A AAA
0.000 2/2.550 22.389 22.431 A
-. 119
1 A A AAA 0~7 ATA >1
22.252 22.312 O "7
1
1
A
u A AAA OIC.
/LIO»
COA
PZU 22.162 22.284 A
-.40
1
1
A
u A AAA
U.UUU QTQ
z /y . TÂ
/5U 22.009 22.062 OA
1
1
1
1
A AAA
U.UUU OQA AAA
ZBU .UUU 22.016 22.048 A
-. 114
JJ A AAA
U.UUU OQA AAA
ZO U.UUU 22.037 22.048 -.up
1
1
A
u A AAA
U.UUU Zo4 .y4U 21.768 21 .781 A^^
-.U5
1
1
A
u A AAA
U.UUU OQC; TOA
zop. /yu 21.749 21 .734 A*7
.U /
1
1
1
1
A AAA
U.UUU OAA • AAA
zyu UUU 21 .481 21.500 AQ
-.uy
A AAA
U.UUU OAA AAA
zyu.uuu 21.548 21 .500 OZ
.ZP
1
1
A
(J
A AAA
U.UUU OAA >10A
zyu.4oU 21.515 21.472 OA
.ZU
10 0.000 295.310 21.240 21.195 .21
10 0.000 297.480 21.092 21.067 .12
1 0.000 300.000 20.887 20.917 -.14
35 0.000 300.000 21 .037 20.917 .57
11 0.000 310.000 20.251 20.294 -.21
35 0.000 310.000 20.510 20.294 1.06
1 0.000 320.000 19.581 19.626 -.23
35 0.000 320.000 19.933 19.626 1 .56
87
1
1 , 7
9

^T3 CT/^ 1 1 r~ £i C ^ I'l
1 u 1 1 uiiiUo r b , (lOOana, ( )Das ( 1967), (29)Sage,
1 1
IJ)-) ; UaS i \ y j)
/
, K 4u J 1 nerrna i Loops, (41 )Clapeyron.
ID Weight Temp. Heat of Vaporization Diff,
K K J/ mo
1
%
ex pt. ca c1
-1
1
1
1
r\ Ann
u.uuu z"ZA Ann 18.903 18.906 A
-.01 1
DO A AAA
U.UUU 19.255 18.906 1
1
OC
.OD
II U.UUU JÛ •UUu 18. 184 18.125 . JJ
jD A AHA
U.UUU z / n nnn
18.477 18.125
u. uuu xc^n nnn 17.405 17.274
1 1
Jp A AAA
U.UUU XRn nnn 17.569 17.274 1 ~l 1
1 1
u. uuu 'z.f.r)
_30U
nnn
• uuu 16.552 16.340 1 7n
JJ u.uuu Tcn nnn
J>OU« UUU 16.564 16.340 ^7
I.J/
1
1 1
1 1 U. nno
n ^J\JU J / u • uuu 15.573 15.306 1
JJ n nnn D 1 \J • nnn
UUU 15.443 15.306 on
•y u
It
1 1
n nnn JO nnn
w • uuu
"^^^n 14.447 14.147 9 1
J J- n nnn
U.UUU ôn nnn
J>OU eUUU 14.209 14.147
1 1
1 I
n nnn
U.UUU ->yu nnn
"ôn .uuu 13.138 12.824 Z. Hj
JJ n nnn
U.UUU j^yj nnn
"ôn ©uuu 12.837 12.824 . 1
1
n
u
1 1
1 1 u. nnn
n uuu Ann
'+UU nnn
uuu • 11.506 11.262 9 1
tR n nnn
U.UUU Ann nnn
'lUU.UUU 11.209 11.262 -47
jO n nnn
U.UUU Ar\^ • nnn
4Uy uuu 10.251 10.347 _ Q9
1
1 1
n nnn
U.UUU 4 U«
y! nnn
n UUU
1
1 9.263 9.292 —.J 1
XR n nnn
U.UUU 4 n
A nnn
u .uuu
1
I 9. 184 9.292 — I o . I
A AAA ^ c nnn 1
— .40
Afi
jO U.UUU 4 !3«UUU
I 7.895 8.012 1
1
1
r 1 U. AAA
A UUU yi'7n nnn
4ZU« UUU 6.138 6.273 9 . 10
-Z *^ 1
XK
j5 A AAA
U.UUU ^ on nnn
4zU«UUU 5.916 6.273 -5.oy
n nnn
U.UUU lri"t • ZDU 21.479 21.256 1
1
nR
. uu
29 0.000 310.930 20.382 20.234 .73

29 0.000 327.590 19.120 19.085 .19
29 0.000 344.260 17.712 17.771 -.33
29 0.000 360.930 16.094 16.248 -.95
29 0.000 377,590 14.096 14.440 -2.38
29 0.000 394.260 11.622 12.194 -4.69
Number of data points used in fit = 41; rms deviation = 0.095|.
88
. 4 • /
Table 11, Enthalpies of saturated liquid normal butane frorn

eq (10).
Tsnp M Mq eq n i f f
"a I \ \ )
J/ mO 1 J/mO 1
h
1 j4 .OO •U U. AAA
A UUU
1 41).UU ou^«y AOT
1 3U.UU 1 ~7
1 / /
7 1
1
C
.0 1 T7 1 a AA 1
.UU1
loU.UU OQ X 7 O AA R
1 /U.UU >1 AO
4 IU^«4
1 /I A AO
loU.UU COT A C AA
-.UUl 1
1 on HA (LA
0444A /I C
D d444 • AAT
- .UUj
OA A AA /D^ / • y -. AAT
UU3
o A AA
1
^ lU.UU OOZ J«4 Q QO X c; AAA
-.UUU
OO A AA 1UUj4. o 1 UUj4« 4 AAO
O"^ A AA O^L"^ "7 AA'^
/jU. uu I ^d4
1
I
I Add m I
1
I .UU3
O/l A AA O A AA1
Z4U.UU 1^:5 4,/ 1
1
\^z> 4.U
c; 1
\
/I
• UUl
OCA
ZDU.UU AA 1 "70 "7 O 1
1
"70 ~7 A
3 /o / .y AAA
.UUU
ôu A • AA
UU 1
1
C^nO "7
-)Uo / • J 1 c; AO "7 c -. AA
UU 1
1
OTA
Z /U.UU AA 1
1
gLA
d4 \
1
A Q
.o 1 04 1
AAO
OQ
zyu A . AA
UU 1
\
~t~I~JO
1 1 1
X 1 / / /Z .D
AAO
OQ A AA 1
1
Q 1
A
y 1 D .4 1
1 1 y o ©o
1 1
AA
-.UU
TAA
JUU. UU AA ZUD04 • 1 iU-)04 • U .UU 1
J A
•Z 1
U.UU
1
AA 9904 Q 1 9904 1 R nn
UU
• 1
1
•ZO A AA OX^Xf. nn9

JZU.UU x.
9sn7n
^ u» R
o /
9sn7n
£.J\J \) %\J 1 • nm
uu 1
X/IA . AA
-JHU UU ûut • / 1
_ • AA1
UU 1
j-û . uu 9R9fift ft nm
- .UUl
360.00 29940.6 29941.2 -.002
370.00 31668.3 31668.7 -.001
380.00 33460.0 33459.6 .001
390.00 35327.5 35326.6 .003
400.00 37293.8 37293.1 .002
410.00 39414.3 39416.2 -.005
420.00 41932.5 41931.6 .002
425.16 45399.8 45399.8 0.000
Number of points = 29; rms deviation = 0.005^.
1 Derived from ideal gas functions, the equation of state, and the formulated
heats of vaporization.
89
.
1
Table 12. Entropies and specific heats of saturated liquid

norma! butane from eq (11).
1
1 emp. So S o ( eq (11)) D 1 ff Ca
K J/(mol 'K; J/(moi 'K) % J/(mol 'K)
134.86 133.544 133.544 0.000 1 17.39

140.00 137.932 137.929 .002 1 17.07
1 50.00 145.992 145.989 .002 1 16.61
1 60 . 00 153.507 153.507 .000 1 16.42
170.00 160.565 160.567 -.001 1 16.54
180.00 167.237 167.239 -.001 1 16.99

190.00 173.582 173.584 -.001 1 17.77
200.00 179.652 179.651 .000 1 18.88
21 0.00 185.486 185.484 .001 120.29

220.00 191 . 120 191.118 .001 121 .98
230.00 196.584 196.582 .001 123.92
240,00 201 .902 201 .901 .000 126, 10
250.00 207.096 207,097 -.000 128.48
260.00 212. 183 212. 185 -.001 131 .05
270.00 21 7. 180 21 7. 182 -.001 133.79
280.00 222.098 222. 100 -.001 136.70
290.00 226.950 226.950 -.000 139.78
300.00 231 .744 231 .743 .000 143.02
310.00 236.490 236.488 .001 146.44
320.00 241 .196 24 1 . 1 94 .001 150.05
330.00 245.870 245.869 .000 153.88
340.00 250.521 250.522 -.000 157.94
350.00 255. 160 255. 163 -.001 162.29
360.00 259.797 259.800 - . 00 167.03
370.00 264.446 264.447 -.000 172,29
380.00 269. 122 269. 120 .001 178.40
390.00 273.354 273.848 .002 186.05
400.00 278.689 278.686 .001 196.99
410.00 283.753 283.765 -.004 217.06
420.00 289.605 289.598 .002 287.81
425.16 297.647 297.647 0.000
Number of points = 29; rms deviation = 0.001$.
Derived from ideal gas functions, equation of state, and formulated heats of
vaporization.
90
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Data sources and ID numbers: (l)Aston, (2)Huffman, (3)Dana.
ID Temp. ^0' J/(mol ^K) Di f f

K expt ca c 1
%
1 139.880 1 13.24 1 17.08 -3.28

1 142.220 1 13.45 1 16.95 -2.99
149.500 1 14.71 1 16.53 -1 .55
1 56.030 1 6.00
1 1 16.46 -.39
162.290 1 15.92 1 16.42 -.43
168.490 1 16.84 1 16.50 .29
174 .590 1 16.80 1 15.70 .08
180.830 1 17.09 1 1 7.04 .05
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222.7 0 1 122.53 122.48 .04
230.810 123.91 124.09 -. 1 5
238.430 124.83 125.74 -.73
247.010 127.00 127.75 -.58
251 .430 129.22 128.84 .30
262.040 130.94 131 .59 -.50
268. 140 131.61 133.27 -1 .25
2 139.700 1 13.55 1 7 . 09
1 -3.02
2 150.200 1 14.04 1 16.61 -2.20
2 1 52.500 1 14.77 1 6.54
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2 170.200 1 15.25 116.54 -1.11
2 187.000 1 17.69 117.50 .16
2 190. 1 00 1 17.44 117.78 -.29
2 230.000 123.03 123.92 -.72
2* 261 .800 129.60 131 .53 -1 .47
3 256.950 125.973 130.246 -3.39
3 270.550 131.324 133.948 -2.00
3 277.280 135.458 135.895 -.32
3 285.020 137.647 138.227 -.42
3 289.930 139. 106 139.757 -.47
3 267.020 130.594 132.957 -1.81
3 276.380 141.295 135.631 4.01
3 284.770 139.106 138.150 .69
3 289.760 140.808 139.704 .78
3 294.380 143.727 141 .179 1.77
Number of data points = 39; rms deviation = 1.49|.
95
Table 15. Comparisons with Cv and Cp data,
Cp data of Sage [551
P = 0. 101325 MPa ( 1 atm)
Temp. Cp, J/(nnol»K) Diff.

K expt calc %
294.261 95.964 99.246 -3.42

310.928 98.541 103.081 -4.61
327.594 101.314 107.088 -5.70
344.261 104.208 111.189 -6.70
360.928 107.223 115.333 -7.56
377.594 110.312 119.487 -8.32
394.261 113.400 123.625 -9.02
410.928 116.416 127.730 -9.72
Number of data points of Sage [651 = 8; rms deviation = 7.18^.
Cp data of Dai ley [ 18]
Temp. Cp, J/(mol»K) Diff.

K expt calc %
344.900 110.583 110.514 .06

359.600 114.934 114.285 .56
387.500 121.754 121.392 .30
451.600 137.988 137.171 .59
521.000 154.013 153.011 .65
561.300 162.256 161.540 .44
600.800 170.331 169.420 .53
692.600 185.853 185.9^3 -.08
Number of data points of Dai ley [181 = 8; rms deviation = 0.46^.
96
Table 16. Comparisons with velocity of sound data.
Saturated liquid velocities of sound from Rao (581
Temp. Dens ty
i Vel . of Sound, m/s Dif f.
K kg/m3 expt ca c
1
%
268. 150 605.89 1085 1049 3.31

263. 150 61 1.16 1115 1074 3.62
253. 150 621.54 1173 1125 4.03
243.150 631.71 1230 1176 4.33
233. 150 641 .69 1286 1227 4.54
223. 150 651.53 1343 1278 4.81
213.150 661 .24 1400 1328 5.08
203. 150 670.84 1459 1379 5.46
193.150 680.37 1515 1429 5.65
183. 150 689.83 1573 1479 5.95
173.150 699.26 1630 1529 6. 18
158.150 713.36 1715 1603 6.48
153. 150 718.05 1743 1628 6.55
148. 150 722.75 1772 1653 6.66
143. 150 727.46 1800 1679 6.71
of data points of Rao (581 =: 15; mean deviation = 5.29^.
97
1 1 1 1
Table 17. Calculated P{T) isochores of normal butane.
Normal Butane 1 sochore at 25 kg/m"^
1sotherm 1 sochore 1sochore

Temp. Pressure Z Der vat ve
i i Der vat ve
i i Curvature
K MPa MPaMn3/kg MPa/K
352.827 1.0063 .79753 .03014 .00465 -,0000149

360.000 1.0393 .80729 .03187 .00456 -.00001 15
368.000 1.0755 .81721 .03371 .00448 -.0000091
376.000 1.1110 .82627 .03547 .00441 -.0000074
384.000 1 .1461 .83461 .03719 .00436 -.0000062
392.000 1.1808 .84232 .03886 ,00431 -.0000053
400.000 1.2152 .84948 .04050 ,00427 -.0000046
408.000 1.2492 .85616 .04211 .00424 -.0000040
416.000 1.2830 .86241 .04370 .00421 -.0000036
424.000 1.3166 .86827 .04526 ,00418 -.0000032
432.000 1.3499 .87379 .04680 .00416 -.0000028
440.000 1.3831 .87899 .04833 .00414 -.0000025
448.000 1.4161 .88390 .04984 .00412 -.0000023
456.000 1.4490 .88855 .05134 ,00410 -,0000021
464.000 1.4817 .89296 .05282 ,00408 -,0000019
472.000 1.5143 .89715 .05430 ,00407 -.0000018
480.000 1.5468 .901 13 .05576 ,00406 -.0000016
488.000 1.5792 .90492 .05722 .00404 -.0000015
496.000 1.6115 .90853 .05867 .00403 -.0000014
504.000 1.6438 .91 199 .0601 .00402 -.0000013
512.000 1.6759 .91529 .06154 ,00401 -.0000012
520.000 1.7079 .91844 .06297 ,00400 -.000001
528.000 .7399
1 .92147 .06439 ,00399 -.0000010
536.000 1.7719 .92437 .06580 .00399 -.0000010
544.000 .8037
1 .92715 .06721 .00398 -.0000009
552.000 1.8355 .92983 .06861 .00397 -.0000008
560.000 1.8673 .93240 .07001 .00397 -,0000008
568.000 1.8990 .93487 .07141 .00396 -,0000007
576.000 1.9306 .93725 .07280 .00395 -,0000007
584.000 1.9622 .93955 .07419 ,00395 -,0000007
592.000 ,9938
1 .94176 .07557 .00394 -.0000006
600.000 2.0253 .94389 .07695 .00394 -.0000006
608.000 2.0568 .94596 .07833 ,00393 -.0000006
616.000 2.0883 .94795 .07970 ,00393 -.0000005
624.000 2.1197 .94987 .08108 ,00392 -.0000005
632.000 2.1510 .95173 .08244 .00392 -.0000005
640.000 2. 1824 .95353 .08381 .00392 -.0000005
648.000 2.2137 .95528 .08517 .00391 -.0000004
656.000 2.2450 95696 .08654 .0039 -.0000004
664.000 2.2763 .95860 .08789 .00391 -.0000004
672.000 2.3075 .96019 .08925 ,00390 -.0000004
680.000 2.3387 .96173 .09061 ,00390 -.0000004
688.000 2.3699 .96322 .09196 ,00390 -.0000004
696.000 2.401 .96467 .09331 .0 0 389 -.0000003
98
1
Normal Butane I sochore at 50 kg/m-

Temp, Pressure Z Der vat ive
i Der vat ve
i 1 Curvature
K MPa MPa.m3/kg MPa/K MPa/K^
383.962 1.8715 .68148 .02109 .01085 -.0000535

384.000 1.8719 .68156 .02111 .01085 -.0000534
392.000 .9572
1 .69808 .02354 .01050 -.0000375
400.000 2.0401 .71308 .02580 .01023 -.0000288
408.000 2.1211 .72686 .02796 .01003 -.0000232
416.000 2.2006 .73961 .03003 .00986 -.0000193
424.000 2.2789 ,75147 .03204 .00972 -.0000164
432.000 2.3561 .76254 .03400 .00959 -.0000142
440.000 2.4324 ,77293 .03591 .00949 -.0000124
448.000 2.5079 .78269 .03779 .00939 -.00001 10
456.000 2.5828 .79190 .03964 .00931 -.0000098
464.000 2.6569 .80060 .04146 .00924 -.0000088
472.000 2.7306 .80884 .04326 .00917 -.0000079
480.000 2.8037 .81666 .04503 .0091 -.0000072
488.000 2.8763 .82409 .04679 .00906 -.0000065
496.000 2.9486 .831 16 .04853 .00901 -.0000060
504.000 3.0204 ,83790 .05026 .00896 -.0000055
512.000 3.0919 .84433 .05197 .00892 -.0000051
520.000 3.1631 .85048 .05366 .00888 -.0000047
528.000 3.2340 .85636 .05535 .00884 -.0000043
536.000 3.3046 .86200 .05702 .00881 -.0000040
544.000 3.3749 .86740 .05869 .00878 -.0000038
552.000 3.4450 ,87258 .06034 .00875 -.0000035
560.000 3.5149 .87757 .06199 .00872 -.0000033
568.000 3.5846 .88235 .06363 .00870 -.0000031
576.000 3.6541 .88696 .06526 .00867 -.0000029
584.000 3.7233 .89140 .06688 .00865 -.0000027
592.000 3.7925 ,89567 .06850 .00863 -.0000026
600.000 3.8614 .89980 .07011 .00861 -.0000024
608.000 3.9302 .90378 .07171 .00859 -.0000023
616.000 3.9988 .90762 .07331 .00857 -.0000022
624.000 4.0673 .91 133 .07490 .00855 -.0000021
632.000 4.1357 .91492 .07649 .00854 -.0000020
640.000 4.2039 .91839 .07807 .00852 -.0000019
648.000 4.2721 ,92175 .07965 .00851 -.0000018
656.000 4.3401 ,92501 .08123 .00849 -.0000017
664.000 4.4080 .92816 .08280 .00848 -.0000016
672.000 4.4758 .93122 .08436 .00847 -.0000016
680.000 4.5435 .93418 .08592 .00846 -.0000015
688.000 4.6111 .93705 .08748 .00844 -.0000014
696.000 4.6786 .93984 .08904 .00843 -.0000014
99
11 .
Table 17. ( Cont nued

i )

Temp Pressure Z Der vat ve
i i Der ivat ve
i Curvature
•
MPa MPa.m3/kg MPa/K MPa/K^

K
411 .953 3.0475 .51715 .00819 .02600 -.0002358

416 .000 3. 151 ,52952 .00973 .02523 -.0001567
424.000 3.3487 .55212 .01245 .02426 -.0000967
432.000 3.5400 .57286 .01499 .02360 -.0000705
3.7268 .59211 .01742 .02310 -.0000554
440.000
448.000 3.9100 .61012 .01978 .02270 -.0000455
4.0902 .62705 .02209 .02237 -.0000384
456.000
464.000 4.2680 .64302 .02435 .02208 -.0000330
4.4437 .65814 .02659 .02184 -.0000288
472.000
480.000 4.6175 .67249 .02880 .02162 -.0000255
4.7896 .68613 .03098 .02143 -.0000227
488.000
4.9604 .69912 .03315 .02126 -.0000205
496.000
5.1298 .71 152 .03530 .02110 -.0000185
504.000
512.000 5.2980 .72337 .03743 .02096 -.0000169
5.4651 .73472 .03954 .02083 -.0000154
520.000
5.6313 .74558 .04165 .02071 -.0000142
528.000
5.7965 .75601 .04374 .02060 -.0000131
536.000
5.9609 .76601 .04582 .02050 -.0000121
544.000
6.1246 .77564 .04789 .02041 -.00001 13
552.000
6.2875 .78489 .04996 .02032 -.0000105
560.000
6.4497 .79380 .05201 .02024 -.0000098
568.000
6.61 13 .80239 .05406 .02016 -.0000092
576.000
584.000 6.7723 .81067 .05609 .02009 -.0000087
592 .000 6.9328 .81867 .05813 .02002 -.0000082
7.0927 .82639 .06015 .01996 -.0000077
600.000
7.2522 .83385 .06217 .01990 -.0000073
608 .000
616.000 7.41 1 .84106 .06418 .01984 -.0000069
7.5697 .84804 .06619 .01979 -.0000066
624.000
7.7278 .85479 .06819 .01974 -.0000062
632.000
640.000 7.8855 .86133 .07018 .01969 -.0000059
8.0428 .86767 .07217 .01964 -.0000057
648.000
656.000 8.1998 .87382 .07416 .01960 -.0000054
664.000 8.3564 .87978 .07614 .01956 -.0000052
672.000 8.5127 .88556 .07812 .01952 -.0000050
8.6687 .891 18 .08009 .01948 -.0000048
680.000
688.000 8.8244 .89664 .08206 .01944 -.0000046
8.9797 .90194 .08402 .01940 -.0000044
696.000
100
• J1 / 1 31
u /
1 4
u
U
b
1
Normal Butane I sochore at 150 kg/ttr
1 1 t III
1
1
Q(^r^hAf~f^
^\J\^ WKJi "3
Tsmp • r 1 o Ul t; 7 \jss\ 1 Va 1 1 Vc Hpr

L/d i1 Wrii"
V CJ 1
i1 VP
VU P iir\/;^ i" iirp
IS
MP 3 MPp^
o m3 kn
• Ml—'// r\y I t a / IN
^ZZ» Z /o T A 1 "7 1
•
AA yo
uu Q*^ 1
1 .U4Z3y •UUUODoO
A AAA A /I r\^Â • UUZOJ) .U4 34 1
~ • UUUh D J) I
A "Ô AAA A
4 A 1 OR
•U ZD I •4 jZO •UUPZO AZQCA
• UJjy J4 ~ •UUU IP/!
vl A AAA
y!
4 • j>Z4!? CO A c
y1
•UU OU / .U JO 00 nnnnQQ/i
_ •uuuuy
~ y4
O AAA TAA A A"Â
UjU — •UUUU
44o«UUU
>l >I
4 DjUU
y1
.40 103 •U 1
• U_) /o / /J)4
ytcc AAA AQ A 01/ Q nz7z CI
- • nnnn rq"^
4 •yj>Uo
yl
.!3Ujy4 •u 1
1 z y UUUUPoJ)
4o4
>1 AAA
£ •UUU y1 A
•U 1
1
c:OP
PZO •u joyz _ nnnn/iQO
~ •UUUU40Z
A "70 AAA C CO 1 -J C/1 CO 1
•Ujop / —• UUUU4
4 /z •UUU •U 1 / / D 1
/IO A AAA C O 1 "ZA AOAOt^

•UzUzP .UjD2tD AAA A "Z ^1/
- •UUUUpP
O O AAA C AO A C OO T C AO 0"7 A A "2 CA A A AA A "Z A
488.000
>1
D.
1
1 OzO .582 /5 .u35yy -•UUUU3 1
1
A f\£ AAA C 1 O AA A A "Z A O COT A A A A OO A

- •UUUUzoU
495.000 .50031 1
•Oz5z3 .Oji> /5
Cir\ A
504.000AA A D^D /4
"7
.51 /Id 1 C 1 AO"7"7
• Uz / Id
A Z C C^ AAA AO
-• UUUUzPP
CI'Z
CIO AAA
512.000 •yp / / •Oj3j2 A AOO
•U3UzZ "Z AT CTC
.Uj535 A A A AO OA
- •uuuuzzy
COA AAA
5zO. 000
~7 TZ AO
/ •z3yo
/Tyl Q Q C
.54ooD A "Z 0"7 1 AT C 7/
.0351 1
- • AAAAO
UUUUz 1 A 1
coo AAA .5ojol A"Z CÔ

•U3Pz 1
1
AT CA
.0350 1 A AAA dT.
- .UUUU ^
1y3
CZX AAA "7
/
Q A AA
•oUUU •D /o2 1 •
A'Z"7
\}D I f\J
"7 A AT D
.U340D /I A AAA ~I/y
-•UUUU 1
1
O
C A A AAA A A A C £1
- .0000
544.000 8 .0784 .69208 •040 19 .03473 \
156
ceo AAA
552.000 8^3557 .70545 •04268 .03460 A AA A 1 C C
-.00001 55
CrCA AAA A C O AT ^ ^ Q AAA A A C
- .0000145
5dU«UUU O •DJZU • U4 Plo
>1 1
.03448 1
C£iQ AAA A A"71 T

Q .yu "7Z AQ C A T T7 A AAA 3 T7
POO .UUU y •U4 10 .0343/ /I
-.UUUU 1
1 /
C^"7£ AAA
/D.UUU A Q 1lo
y • 1] o O "7/1 OA 1 A CA 1
• UpU id
AT ^ OiC
.03425 AAAA OA
-.UUUUl 291
CO AAA A ^ pR "7 C/1 C"7 A T/1 AAAA OO

!>o4 .UUU
/I
y • 4DDD . / 34D •UPZD4 .U34 1
15 -.UUUU 221
1
CAO
-)yz. AAA
UUU A
y • 70Q>1
/zo4 . /DDot) AK
•UPP c; 1 "z
1
A T^
.U34U5 AAAA
-.UUUU C \
1
^
1
CAA AAA
duu»uuu 1A
1
AAAPi
U^ UUUD
-7-7^:-7A
•U D / OZ .uj jy AAAA A
- . UUUU 1
1
1
1
zTAQ AAA
oUo .UUU 1 A
1 U•O z "70A
/zU
"7Q "TZT A£: A A
•UdU 1
1
AT TOO
.03389 AAAA lU5
-.UUUU AC1
r AAA AT TQ AAAA AA
1
D D •UUU
1 1 U •P4zo . / y / 5J •Udzpo .U33o 1
-.UUUU UU1
1
r\f. ^Pif.
O^H • UUU 1 u • o zy 1 •UDPUD .uuuuuyo
632.000 11.0824 .81723 .06754 .03365 -.0000092
640.000 11.3513 .82660 .07002 .03358 -.0000089
648 .000 11.6197 .83570 .07249 .03351 -.0000085
656.000 11.8875 .84453 .07497 .03344 -.0000082
664.000 12.1548 .85312 .07744 .03338 -.0000079
672.000 12.4215 .86146 .07990 .03332 -.0000077
680.000 12.6878 .86958 .08237 .03326 -.0000074
688.000 12.9536 .87747 .08483 .03320 -.0000072
696.000 13.2190 .88515 .08729 .03314 -.0000070
101
1 1
Normal Butane Isochore at 200 kg/m^
1 sotherm 1 sochore 1sochore

i i Der vat ve
1 i Curvature
425.033 3.7879 .31 150 .00008 .05803 -.0067339

432.000 4. 1771 .33797 .00216 .05515 -.0001 184
440.000 4.6154 .36665 .00475 .05449 -.0000628
448.000 5.0496 .39398 .00747 .05407 -.0000441
456.000 5.4809 .42012 .01026 .05376 -.0000345
464.000 5.9099 .44520 .0131 .05351 -.0000286
472.000 6.3371 .46929 .01601 .05330 -.0000246
480.000 6.7628 .49246 .01896 .0531 -.0000218
488.000 7.1870 .51478 .02193 .05295 -.0000196
496.000 7.6100 .53628 .02494 .05280 -.0000179
504.000 8.0318 .55702 .02796 .05266 -.0000165
512.000 8.4526 .57705 .03101 .05253 -.0000154
520.000 8.8724 .59639 .03408 .05241 -.0000145
528.000 9.2912 .61508 .03716 .05230 -.0000138
536.000 9.7092 .63315 .04026 .05219 -.0000131
544.000 10. 1263 .65065 .04337 .05209 -.0000126
552.000 10.5426 .66758 .04649 .05199 -.0000121
560.000 10.9582 .68398 .04962 .05190 -.00001 17
568.000 1 .3730
1 .69987 .05275 .05181 -.0000113
576.000 11.7871 .71528 .05589 .05172 -.00001 10
584.000 12.2005 .73022 .05904 .05163 -.0000107
592.000 12.6132 .74472 . .06220 .05155 -.0000104
600.000 13.0252 .75880 .06535 .05146 -.0000102
608.000 13.4366 .77246 .06852 .05138 -.0000100
616.000 13.8474 .78574 .07168 .05130 -.0000098
624.000 14.2575 .79864 .07485 .05123 -.0000096
632.000 14.6670 .81118 .07801 .05M5 -.0000094
640.000 15.0759 .82337 .081 18 .05108 -.0000092
648.000 15.4842 .83523 .08435 .05100 -.0000091
656.000 15.8920 .84677 .08752 .05093 -.0000090
664.000 16.2991 .85800 .09070 .05086 -.0000088
672.000 16.7057 .86894 .09387 .05079 -.0000087
680.000 17.1 1 18 .87958 .09704 .05072 -.0000086
688.000 17.5172 .88996 .10021 .05065 -.0000085
696.000 17.9222 .90006 .10337 .05058 -.0000084
102
1 .
Table 17 . ( Cont nued i )
Normal Butane Isochore at 227.847 kg/m^

i i Der vat ve
i i Curvature
K MPa MPa.m3/kg Wa/K MPa/K2
425. 160 3.7960 .27394 .00000 .06427 -.0000000

432.000 4.2356 .30082 .00216 .06427 -.0000007
440.000 4.7497 .33120 .00505 .06426 -.0000014
448.000 5.2638 .36049 .0081 .06425 -.0000021
456.000 5.7777 .38875 .01 128 .06423 -.0000028
464.000 6.2914 .41601 .01453 .06420 -.0000034
472.000 6.8049 - .44234 .01786 .06417 -.0000039
480.000 7.3182 .46778 .02123 .06414 -.0000044
488.000 7.8311 .49236 .02466 .06410 -.0000048
496.000 8.3438 .51613 .02812 .06406 -.0000052
504.000 8.8561 .53913 .03161 .06402 -.0000056
512.000 9.3681 .56138 .03514 .06397 -.0000060
520.000 9.8797 .58293 .03869 .06392 -.0000063
528.000 10.3909 .60380 .04226 .06387 -.0000066
536.000 10.9017 .62403 .04585 .06382 -.0000068
544.000 11.4120 .64364 .04945 .06376 -.0000071
552.000 11.9219 .66265 .05307 .06371 -.0000073
560.000 12.4313 .68109 .05670 .06365 -.0000075
568.000 12.9402 .69899 .06035 .06359 -.0000077
576.000 13.4486 .71636 .06400 .06352 -.0000079
584.000 13.9566 .73324 .06766 .06346 -.0000080
592.000 14.4640 .74963 .07133 .06340 -.0000081
600.000 14.9709 .76555 .07501 .06333 -.0000083
608.000 15.4773 .78103 .07869 .06326 -.0000084
616.000 15.9831 .79608 .08237 .06320 -.0000085
624.000 16.4884 .81072 .08606 .06313 -.0000085
632.000 16.9931 .82496 .08975 .06306 -.0000086
640.000 17.4973 .83882 .09344 .06299 -.0000087
648.000 18.0010 .85231 .09714 .06292 -.0000087
656.000 18.5041 .86545 .10083 .06285 -.0000088
664.000 19.0066 .87824 .10453 .06278 -.0000088
672.000 19.5085 .89070 .10822 .06271 -.0000089
680.000 20.0099 .90285 .1 1 192 .06264 -.0000089
688.000 20.5108 .91468 .1 1562 .06257 -.0000089
696.000 21.01 10 .92622 .1 1931 .06250 -.0000089
103
1
1 sotherm sochore
1 1sochore
i i Der vat ve
i i Curvature
K MPa MPa.m3/kg NPa/K MPa/K^
425.087 3.7913 .24940 .00005 .06934 .0121526

432.000 4.2872 .27751 .00258 .07243 .0001 153
440.000 4.8695 .30947 .00588 .07307 .0000587
448.000 5.4557 .34053 .00936 .07345 .0000389
456.000 6.0445 .37066 .01297 .07372 .0000283
464.000 6.6351 .39986 .01668 .07392 .0000213
472.000 7.2270 .42815 .02046 .07407 .0000164
480.000 7.8200 .45556 .02431 .07418 .0000126
488.000 8.4139 .48212 .02820 .07427 .0000096
496.000 9.0083 .50786 .03214 .07434 .0000071
504.000 9.6032 .53280 .03612 .07438 .0000050
512.000 10.1984 .55698 .04012 .07442 .0000032
520.000 10.7938 .58043 .04416 .07444 .0000017
528.000 11.3893 .60318 .04822 .07444 .0000004
536.000 1 .9849
1 .62525 .05230 .07444 -.0000007
544.000 12.5804 .64666 .05641 .07443 -.0000018
552.000 13.1758 .66745 .06052 .07442 -.0000027
560.000 13.7710 .68764 .06465 .07439 -.0000035
568.000 14.3660 .70725 .06880 .07436 -.0000042
576.000 14.9608 .72630 .07295 .07432 -.0000048
584.000 15.5552 .74481 .0771 .07428 -.0000054
592.000 16.1493 .76280 .08128 .07424 -.0000059
600.000 16.7430 .78030 .08546 .07419 -.0000064
608.000 17.3363 .79732 .08964 .07414 -.0000068
616.000 17.9292 .81388 .09383 .07408 -.0000072
624.000 18.5216 .82999 .09802 .07402 -.0000075
632.000 19.1 135 .84568 .10221 .07396 -.0000078
640.000 19.7049 .86095 .10641 .07389 -.0000081
648.000 20.2958 .87582 .1 1060 .07383 -.0000084
656.000 20.8862 .89030 .1 1480 .073 7 6 -.0000086
664.000 21 .4760 .90441 .1 900
1 .07369 -.0000088
672.000 22.0652 .91816 .12320 .07362 -.0000090
680.000 22.6539 .93157 .12740 .07355 -.0000092
688.000 23.2420 .94464 .13159 .07347 -.0000093
696.000 23.8295 .95738 .13579 .07340 -.0000094
104
3
2 2 8
71 .
Table 17 ( Cont nued i )
Mnrma 1 Ru'f^nG 1 sochorG ai" 300
1 1 1 1^ 1 III 1 sochore 1sochore

1 c^Mip • Pr pc CM rfi Der val" ve
i i Dsr vat ve
i i Curvature
I\ MPa MPa . m3 /kn MPa/K
.20 95 1 • \J\J c.^ J .09168 .00 18610

H H • VJ'J'-/ .2061 .00309 .09299 .001 1452
m\J\J ^ t.
1 1
4 5 1 50 24^54 008 5 1 09 724 -0002997

5 '^nOQ 09907 nOOl 7Q7
44ft nnn o . \jyoj 7 1 721 10028 nnn ?77 i
A'lfi nnn 6 Q04 5 .^ 5283 .02361 .101 17 .0000975

Af,A nnn
HUH • UUU 7 7 67 1 ^87 54 02893 .10186 .0000774
A17 nnn -42 1 32 0"S430 . 0242
1 -0000627
4ftn nnn -454 16 03972 . 0288
1 -000051 5
4Rfi .000 10. 1798 .48609 .0451 .10325 .0000427
AQfi onn 1 1 0071 51712 05068 10^^56 0000"^ 54
^n4 nnn 1 1 ft'^fi7 54 727 n5fi2 nnnn9Q4
s 9 nnn
1 1 2 fififi2 57fi5fi Ofi 1 77 10404 onno?4"^
5?0 .000 13.501 .60502 .06735 .1 0421 .00001 99
528-000
J C\J %\J\J\J 14.3355 .63267 .07295 . 10436 .0000161
5"56.000 15. 1708 .65954 .07856 .10447 .00001 28
544 .000 16.0070 .68566 .084 19 . 10456 .0000099
552.000 16.8437 .71 105 .08983 .1 0463 .0000073
560.000 17.6810 .73573 .09548 . 10468 .0000050
568.000 18.5186 .75973 .101 14 . 0471
1 .0000030
576.000 19.3563 .78307 . 10680 . 10473 .0000012
584 .000 20. 1942 .80578 .1 1247 . 0473
1 -.0000004
592.000 2 .0320
1 .82787 .11814 . 10472 -.00000 19
600.000 21 .8697 .84936 .12381 .10470 -.0000032
608.000 22.7072 .87028 . 1 2949 . 10467 -.0000044
616.000 23. 5444 .89065 . 1351 . 0463
1 --0000055
624 .000 24 .381 .91048 . 1 4084 .10458 - 0000065
fi^9 nnn 95 2177 Q9C}R0 1 4fi59 1 045^^ - (\C$\C\(\1A
fi40 noo Q4ftfi2 1 52 19 10447 m\J\J\J\J\J\J L.
648.000 26.8892 .96695 .1 5786 . 0440

1 -.OOOOORQ
656.000 27.7241 .98481 .16353 .10432 -.0000096
664.000 28.5583 1.00222 .16919 .10424 -.0000102
672.000 29.3920 1.01920 .17485 .10416 -.0000107
680.000 30.2249 1.03575 .18050 .10407 -.00001 12
688.000 31.0571 1.05190 .18615 .10398 -.00001 17
696.000 31.8886 1.06764 .19180 .10389 -.0000121
105
5 1 5
21 1 31
Normal Butane 1 sochore at 350 kg/m-
sotherm
1 1 sochore 1 sochor©
Temp • pppc c rp
1 1
Der vat vei i Der vat ve
i i P.ij
V./ kJ rva
1V U "furp
1Ul ^
MPa MPa . m3/kg Mâ/K ^/lPa/1^2
4 6. 274
1 3 .7745 • 1 571 .01512 . 1 3054
474 nnn
H ^ H . VJWVJ 4.3018 .20265 .07334
4"57.nnn
*+ _^ • vju 5.3921 .24930 .03142 . 3749
1 000765?!
440.000 6.4997 .29505 .03937 . 393
1 .0001961
448.000 7.6200 .33973 .04728 . 14070 .000 578 1
4 5fi 000 8.7501 .38327 .0551 .14179 .0001 778

464.000 9.8881 .42565 .06304 . 14268 .000 1005
9\J\J$ \\J\J J
472 .000 1 1.0326 .46686 .0709 .14341 .000083

480.000
^ W W • v/W w 12. 1824 .50693 .07878 .14402 .0000691
488.000 13.3366 .54586 .08664 .14453 .0000576
496.000 14.4946 , 58368 .09451 .14495 .0000480
504.000 15.6556 .62043 . 0238
1 .14530 .0000398
51 2.000 16.8192 .65613 . 1 1024 . 14559 .0000328
520.000 17.9849 .69081 .11810 .14583 .0000267
528.000 19.1 523 .72450 . 2595
1 .14602 .0000214
536 .000 20.3211 .75724 .13380 .14617 .0000167
544.000 21 .4909 .78906 . 1 4 1 64 .14628 .0000125
552 .000 22.661 .8 1998 .14947 .1 4637 .0000088
560.000 23.8327 .85004 . 5730
1 . 14643 .0000055
568.000 25.0043 .87927 .1651 .14646 .0000026
576.000 26. 1760 .90768 . 7293
1 . 14647 -.0000001
584 000 27 .3478 .93532 . 18073 . 14646 -.0000074
5Q7.000 28. 51 93 .96221 . 18851 . 14643 -.0000046
600.000 29 .6906 .98837 .19629 . 14639 -.0000065
608.000 30-861 1.01 383 .20406 . 14633 -.0000083
6 6 .000
1 32.0318 .03861
• w
11 ww 1 .21 181 . 4625
1 -.0000099
624.000
W ^ " • w WW 33.2015 1.06274 .2 1956 .14617 -.00001 1
632.000 34.3705 1.08623 .22729 .14607 -.0000126

640.000 35.5386 1.10911 .23501 .14597 -.0000138
648.000 36.7059 1.13140 .24271 .14585 -.0000149
656.000 37.6723 1.15311 ,25040 .14573 -.0000159
664.000 39.0376 1.17427 .25808 .14560 -.0000167
672.000 40.2018 1.19490 .26574 .14546 -.0000176
680.000 41.3650 1.21500 .27339 .14532 -.0000183
688.000 42.5269 1.23461 .28103 .14517 -.0000190
696.000 43.6877 1.25373 .28865 .14502 -.0000196
106
Normal Butane I sochore at 400 kg/m^
1 sotherm 1sochore 1sochore

i i Der vati ve
i Curvature
K (wpa MPa.m3/kg MPaA MPa/K^
402.840 2.6135 . 338

1 1 .04987 .19052 .0004716
408.000 3.6023 .15431 .05801 .19265 .0003636
416.000 5.1540 .21653 .07021 .19513 .0002653
424.000 6.7228 .27710 .08210 .19699 .0002049
432.000 8.3048 .33597 .09378 .19846 .0001630
440.000 9.8973 .39312 .10532 .19963 .0001320
448.000 11.4983 ^ .44856 .1 1676 .20059 .0001078
456.000 13.1062 .50231 . 1 28 1 0 .20137 .0000884
464.000 14.7198 .55443 .13937 .20201 .0000725
472.000 16.3380 .60495 .15057 .20253 .0000591
480.000 17.9601 .65393 . 16172 .20296 .0000477
488.000 19.5852 .70141 .17281 .20330 .0000379
496.000 21 .2127 .74744 .18386 .20357 .0000295
504.000 22.8421 .79208 .19486 .20378 .0000221
512.000 24.4730 .83537 .20581 .20393 .0000155
520.000 26.1048 .87736 .21673 .20403 .0000098
528.000 27.7373 .91810 .22760 .20408 .0000047
536.000 29.3701 .95764 .23844 ^ .20410 .0000001
544.000 31 .0029 .99601 .24924 .20409 -.0000039
552.000 32.6354 1.03326 .26000 .20404 -.0000076
560.000 34.2674 1.06944 .27073 .20397 -.0000108
568.000 35.8988 1.10457 .28142 .20387 -.0000138
576.000 37.5293 1.13870 .29208 .20375 -.0000164
584.000 39.1587 1.17186 .30271 .20361 -.0000188
592.000 40.7869 1.20410 .31330 .20345 -.0000210
600.000 42.4138 1.23543 .32387 .20327 -.0000229
608.000 44.0392 1.26590 .33440 .20308 -.0000247
616.000 45.6631 1.29553 .34490 .20288 -.0000263
624.000 47.2852 1.32435 .35537 .20266 -.0000277
632.000 48.9056 1.35239 .36580 .20243 -.0000290
640.000 50.5241 1.37959 .37621 .20220 -.0000302
648.000 52.1407 1.40625 .38659 .20195 -.0000313
656.000 53.7553 1.43212 .39694 .20170 -.0000322
664.000 55.3679 1.45731 .40726 .20144 -.0000331
672.000 56.9783 1.48184 .41755 .201 17 -.0000338
680.000 58.5865 1.50574 .42781 .20089 -.0000345
688.000 60.1926 1.52903 .43804 .20062 -.0000351
696.000 61 .7964 1.55173 .44825 .20033 -.0000357
107
1
Normal Butane I sochore at 450 kg/in^

i i Der vat ve
i i Curvature
K MPa MPa-m3/kg MPa/K MPa/K^
38 1 . 922 1.8022 .07331 .12106 .27769 .0002405

384.000 2.3797 .09627 .12558 .27817 .0002239
392.000 4.61 17 .18276 .14270 .27975 .0001731
400.000 6.8547 .26622 .15946 .28097 .0001358
408.000 9.1065 .34674 . 17592 .28194 .0001069
416.000 1 .3652
1 .42442 .19215 .28270 .0000837
424.000 13.6293 .49936 .20819 .28329 .0000646
432.000 15.8975 .57168 .22405 .28374 .0000486
440.000 18.1688 .64148 .23975 .28407 .0000350
448.000 20.4424 .70886 .25532 .28431 .0000233
456.000 22.7175 .77394 .27077 .28445 .0000131
464.000 24.9934 .83679 .28609 .28452 .0000042
472.000 27.2697 .89753 .30132 .28452 -.0000036
480.000 29.5457 .95623 .31644 .28447 -.0000105
488.000 31.8210 1, 01298 .33146 .28436 -.0000166
496.000 34.0952 1.06788 .34640 .28420 -.0000220
504.000 36.3681 1.12098 .36125 .28401 -.0000269
512.000 38.6392 1.17238 .37602 .28377 -.0000312
520.000 40.9084 1.22213 .39072 .28351 -.0000351
528.000 43. 1753 1.27031 .40533 .28321 -.0000385
536.000 45.4397 1.31698 .41988 .28289 -.0000416
544.000 47.7015 1.36220 .43436 .28255 -.0000444
552.000 49.9605 1.40604 .44877 .28218 -.0000469
560.000 52.2164 1.44853 .4631 .28180 -.0000491
568.000 54.4692 1.48974 .47739 .28140 -.0000511
576.000 56.7187 1.52972 .49161 .28098 -.0000529
584.000 58.9649 1.56852 .50576 .28055 -.0000545
592.000 61 .2076 1.60617 .51986 .28011 -.0000559
600.000 63.4466 1.64273 .53390 .27966 -.0000571
608.000 65.6821 1.67823 .54789 .27920 -.0000583
616.000 67.9138 1.71272 .56182 .27873 -.0000592
624.000 70.1417 1.74623 .57569 .27825 -.0000601
108
. 11
Table 17. ( Cont nued

i )

i i Der vat ve
i i Curvature
353,249 1 .0155 .04019 .24622 .40030 .0000067

356.000 2. 1 169 .08314 .25413 .40031 .0000020
360.000 3.7181 .14440 .26554 .40030 -.0000045
364.000 5.3193 .20432 .27686 .40027 -.0000106
368.000 6.9203 .26292 .28810 .40022 -.0000164
372.000 8.5210 .32026 .29925 .40014 -.0000218
376.000 10.1214 .37636 .31033 .40004 -.0000270
380.000 11.7213 .43127 .32134 .39993 -.0000319
384.000 13.3208 .48501 .33227 .39979 -.0000366
388.000 14.9196 .53762 .34315 .39963 -.0000410
392.000 16.5178 .58914 .35396 .39946 -.0000452
396.000 18. 1 153 .63959 .36471 .39927 -.0000492
400.000 19.7120 .68900 .37540 .39907 -.0000529
404.000 21.3078 .73741 .38604 .39885 -.0000565
408.000 22.9027 .78484 .39662 .39862 -.0000599
41 2.000 24.4967 .83131 .40715 .39837 -.0000631
416.000 26.0897 .87685 .41764 .3981 -.0000661
420.000 27.6816 .92150 .42807 .39784 -.0000690
424.000 29.2724 .96526 .43846 .39756 -.0000718
428.000 30.8621 1.00817 .44880 .39727 -.0000743
432.000 32.4505 1.05024 .45910 .39697 -.0000768
436.000 34.0378 1.09151 .46936 .39665 -.0000791
440.000 35.6237 1.13198 .47958 .39633 -.0000813
444.000 37.2084 1.17168 .48975 .39600 -.0000834
448.000 38.7918 1.21063 .49989 .39567 -.0000854
452.000 40.3737 1.24886 .50999 .39532 -.0000872
456.000 41.9543 1.28636 .52005 .39497 -.0000890
460.000 43.5335 1.32317 .53007 .39461 -.0000906
464.000 45.1112 1.35931 .54006 .39424 -.0000922
468.000 46.6874 1.39478 .55002 .39387 -.0000937
472.000 48.2621 1.42961 .55994 .39349 -.0000950
476.000 49.8353 1.46380 .56983 .3931 -.0000964
480.000 51.4070 1.49738 .57968 .39272 -.0000976
484.000 52.9771 1.53036 .58951 .39233 -.0000987
488.000 54.5457 1.56276 .59930 .39193 -.0000998
492.000 56. 1126 1.59458 .60906 .39153 -.0001008
496.000 57.6779 1.62585 .61879 .391 13 -.0001018
500.000 59.2416 1.65656 .62849 .39072 -.0001027
504.000 60.8036 1.68675 .63816 .39031 -.0001035
508.000 62.3640 1.71641 .64781 .38989 -.0001043
512.000 63.9228 1.74557 .65742 ,38947 -.0001050
516.000 65.4798 1.77423 .66701 ,38905 -.0001057
520.000 67.0352 1.80240 .67657 ,38863 -.0001063
524.000 68.5888 1.83009 .68610 ,38820 -.0001069
528.000 70.1407 1.85733 .69561 .38777 -.0001074
532.000 71.6910 1.88410 .70509 ,38734 -.0001079
109
1 5
1 11 1
1 1 4
Normal Butane 1 sochore at 550 kg/m^

Temp. Pressure Z Der vat vei i Der vat ve
i i Curvature
K MPa MPa* m->/Kg MPa/K MPa/K^
316.955 .42 1 .01 690 ,44649 .57026 -.0003 178

320.000 2, 5dd .Uo5oD •4578 .5693 -.0003082
324.000 4,4314 . 7384
1 .47261 .56810 -.0002970
C "7A C 1
328.000 0.701 .25959 ,48/32 ,56693 -.0002875
332.000 8.9670 .34329 ,50195 ,55580 -.0002792
335.000 1 ,2279
1 .42474 ,51650 .56470 -.0002720
340.000 13.4846 .50410 ,53096 .56362 -.0002657
344.000 15,7370 .58146 .54535 .55257 -.0002603
348.000 17,9852 .65689 ,55966 .56154 -.0002555
352.000 20,2293 .73046 .57389 .55053 -.000251
356.000 22.4694 .80223 .58805 .55953 -.0002477
360.000 24.7055 ,87227 ,60214 .55854 -.0002444
364.000 25.9378 .94063 .61616 .55757 -.0002416
368.000 29. 1661 1 .00737 ,6301 .55651 -. 0002390
372.000 31 .3907 1 .07255 ,64399 .55566 -.0002357
376.000 33.51 14 1 . 13521 .65781 .55472 -.0002347
380.000 35.8284 1 19840
. .67156 .55378 -.0002328
384.000 38.0417 1.25918 .68525 .55285 -.0002312
388.000 40.2513 1.31858 .59888 .55193 -.0002297
392.000 42.457 1,37665 .71244 .55102 -.0002283
396,000 44.5594 1.43343 .72595 ,5501 -.0002270
400.000 46,8580 1.48896 .73940 .54920 -.0002258
404.000 49,0530 1.54327 ,75279 .54830 -.0002247
408.000 51 .2444 1.59641 ,75513 .54740 -.0002237
412.000 53,4322 1,64841 ,77941 .54651 -,0002228
416.000 55,6165 -
1.69930 .79254 .54552 -,0002219
420.000 bl ,1912 1 .7491 .80582 .54473 -,0002210
424.000 59,9744 1.79787 .81894 .54385 -.0002202
428.000 62.1480 1.84552 .83202 .54297 -.0002193
432.000 54.3181 1.89238 .84504 .54210 -.0002186
436.000 66.4848 1.93818 ,85802 .54122 -.0002178
440.000 68,6479 1.98305 .87095 .54035 -.0002171
444.000 70.8076 2.02701 .88383 .53949 -.0002163
Normal Butane I sochore at 600 kg/m-^
273.655 .1053 ,00448 .74460 ,80593 -.0008644

276.000 1.9925 ,0841 .75571 ,80394 -.0008386
280.000 5.2016 ,21645 .77460 ,80066 -.0007986
284.000 8.3980 ,34453 .79341 ,79754 -.0007630
288.000 1 1,5821 .45856 .81216 ,79456 -.0007311
292.000 14,7546 .58873 .83082 .79169 -.0007024
296.000 17,9158 .70520 .84940 ,78893 -.0005766
300.000 21.0662 .81815 .86790 .78627 -.0006534
304.000 24.2061 .92773 .88632 .78370 -.0006323
308.000 27.3359 1.03408 .90465 .78121 -.0006131
312.000 30.4559 1.13733 .92290 .77880 -.0005957
316.000 33,5664 1.23762 .94107 .77644 -.0005797
320.000 35,5675 1.33506 .95915 .77416 -.0005652
324.000 39.7597 1.42978 ,97716 .77192 -.0005517
328.000 42.8430 1.52187 '
.99508 .76974 -,0005394
332.000 45.9177 1.61 143 1,01291 .76751 -.0005280
335.000 48.9839 1.69857 1 .03067 .76551 -,0005174
340.000 52.0418 1.78338 1.04835 .76346 -,0005075
344.000 55.0917 1.86594 1.06595 .76145 -.0004985
348.000 58,1335 1.94633 1.08347 .75948 -.0004900
352.000 51,1675 2.02464 1.10091 .75753 -.0004820
356.000 64, 1938 2.10094 1.11327 .75562 -.0004745
360.000 67,2125 2.17529 1,13556 .75374 -.0004675
364.000 70,2237 2.24777 1,15278 .75188 -.0004609
110
1 1
Normal Butane I sochore at 650 kg/rn-^
1 sotherm I sochore Isochore

Temp, Pressure Der vat ve
i i Der vat vei i Curvature
K MPa MPaTTt3/kg MPa/K MPa/K^
224,71 .0104 .00050 1.16166 13762 -.0019286

226.000 1.4747 .07018 1. 16929 13515 -.0018906
228,000 3,7413 .17648 1.18115 13143 -.0018345
230.000 6,0005 .28059 1.19300 12781 -.0017816
232.000 8,2526 .38257 1,20484 12430 -.0017316
234.000 10,4978 .48249 1.21668 12089 -.0016845
236.000 12.7362 .58041 1.22851 I1756 -.0016399
238.000 14.9681 .67639 1.24033 11432 -.0015977
240.000 17.1936 .77048 1.25214 I I 1 17 -.0015578
242.000 19,4128 ,86274 1.26394 1. 10809 -.0015199
244.000 21.6260 ,95322 1.27572 1.10509 -.0014811
246.000 23.83 52 1,04197 1.28748 1,10215 -.0014500
248.000 26.0347 1,12904 1.29923 1.09929 -.0014177
250.000 28.2304 1,21447 1.31096 1.09648 -.0013869
252.000 30.4206 1,29830 1.32268 1.09374 -.0013577
254.000 32.6054 1,38059 1.33437 1,09105 -.0013298
256.000 34.7849 1.46136 1.34604 1.08842 -.0013033
258.000 36.9591 1,54067 1.35770 1,08584 -.0012781
260.000 39.1283 1,61855 1.36933 1,08331 -.0012539
262.000 41 .2924 .69503
1 1,38094 1,08082 -.0012309
264.000 43.4516 1.77015 1,39253 1,07838 -.0012089
266.000 45,6059 1.84394 1.40410 1.07598 -.001 1879
268.000 47.7555 1.91645 1,41564 1.07363 -.001 1678
270.000 49.9005 1.98769 1.42716 1.07131 -.001 1485
272.000 52.0408 2.05771 1.43866 1.06903 -.001 1301
274.000 54.1766 2.12652 1.45013 1.06679 -.001 1124
276.000 56,3080 2.19416 1,46158 1,06458 -.0010954
278.000 58,4350 2.26067 1.47300 1.06241 -.0010791
280.000 60.5577 2.32605 1.48441 1,06027 -.0010635
282.000 62.6761 2.39035 1.49578 1,05816 -.0010485
284.000 64.7903 2,45358 1.50713 1,05607 -.0010340
286.000 66.9004 2,51577 1.51846 1,05402 -.0010201
288.000 69.0064 2.57694 1.52976 1,05199 -.0010066
290.000 71 .1084 2.63713 1.54103 1,04999 -.0009937
Normal Butane I sochore at 700 kg/m-^
172.361 ,0002 .00001 1.72229 1.62029 -.0043399

174.000 2,6501 .15210 1.73404 1.61329 -.0042017
176.000 5.8684 .33299 1.74843 1,60505 -.0040433
178.000 9.0705 .50890 1.76287 1,5971 -.0338954
180.000 12.2570 .68004 1.77737 1.58946 -.0037570
182.000 15.4285 .84660 1.79191 1.58208 -.0036275
184.000 18.5855 1.00874 1.80648 1.57495 -.0035061
186.000 21 .7284 1. 16665 1.82107 1.56805 -.0033923
188.000 24.8578 1.32047 1.83569 1.56137 -,0032853
190.000 27.9741 1,47037 1.85033 1.55490 -,0031847
192.000 31.0776 1,61648 1.86498 1.54863 -.0030901
194.000 34.1687 1,75894 1.87964 1.54254 -.0030009
196.000 37.2478 1,89788 1.89430 1.53662 -.0029168
198.000 40.3153 2,03343 1.90897 1.53087 -.0028374
200.000 43.3714 2.16569 1.92363 1,52527 -.0027624
202.000 46.4165 2.29480 1.93828 1,51982 -.0026914
204.000 49.4508 2.42084 1.95293 1,51450 -.0026243
206.000 52.4746 2.54393 1.96757 1,50932 -.0025606
208.000 55,4881 2.66416 1.98219 1,50426 -.0025002
210.000 58.4917 2.78162 1.99680 1,49931 -.0024429
212.000 61.4855 2,89641 2.01139 1,49448 -.0023884
214.000 64.4697 3.00861 2.02596 1,48976 -.0023366
216.000 67.4446 3.11829 2.04051 1,48514 -.0022873
218.000 70.4103 3.22555 2.05504 1.48061 -.0022403
111
2
1 6
1 3
1 51 1
Normal Butane Isochore at 735.272 kg/m-

i i Der vat ve
i 1 Curvature
134.860 .0000 .00000 2.23494 2. 1009

1 -.0082374
136.000 2.4002 .16780 2.24373 2. 10083 -.0080029
137.000 4.4971 .31209 2.25150 2.09293 -.0078062
138.000 6.5861 .45376 2.25932 2.08522 -.00761 75
139.000 8.6676 .59286 2.26720 2.07759 -.0074365
140.000 10.74 16 .72948 2.27513 2.07034 -.0072627
141. 000 12.8083 .86367 2.28310 2.06316 -.0070958
142.000 14.8679 .99549 2.291 12 2.0551 -.00693 54
143.000 16.9207 1 . 12500 2.29918 2.04929 -.0067813
144.000 18.9666 1 .25228 2.30727 2.04258 -.0066332
145.000 2 .0059
1 1 .37736 2.31540 2.03602 -.0064907
146.000 23.0387 1 .50030 2.32356 2.02960 -.0063535
14 7.000 25.0651 1 . 62 1 1 2.33175 2.02331 -.0062716
148.000 27.0853 1 .73999 2.33998 2.01715 -.006094 5
149.000 29.0995 1 .85683 2.34823 2.01 1 12 -.00 59770
150.000 31 1075
. 1 .971 74 2.35651 2.0052 -. 0058 540
151.000 33. 099 1 2.08475 2.36481 1.9994 -.0057403
152.000 35. 1065 2. 19592 2.373 1 1.99373 -. 0056306
153.000 37.0974 2.30529 2.38147 1.988 1 -.0055248
154.000 39 .0828 2.41290 2. 38983 1.98268 -.0054727
55.000
^
1t ^ 9 \J \J\J 4 .0628
1 2.51878 2.39821 1.97730 -.005324
156.000 43. 0375 2.62298 7.40660 1.97203 -.0057 789
157.000 " 5.0069
4 ^9 \J\J\J7 2.72554 2.4 501 1 1.96685 -.0051 370
000
Sft 9 \J\J\J
11 46. 97 1 2.82549 1.961 75 - 0050481
159.000 48.9304 2.92587 2.43136 1.95675 -.0049677
160.000
\J\J 9 \J\J\J
1 50.8847 3.0237 2.44030 1.951 83 -.0048791
161. 000 52.834 3. 12005 2.44876 1.94699 -.0047987
162.000 54.7787 3.21492 2.45722 1.94223 -.0047209
163.000 56.7186 3.30835 2.46569 1.93755 -.0046456
164.000 58.6538 3.40037 2.47416 1.93294 -.0045727
165.000 60.5845 3.49101 2.48265 1.92840 -.0045021
166.000 62.5107 3.58030 2.491 13 1.92393 -.0044336
167.000 64.4324 3.66827 2.49962 1.91953 -.0043673
168.000 66.3498 3.75494 2.50812 1.91520 -.0043030
169.000 68.2628 3.84035 2.51561 1.91093 -.0042406
170.000 70. 1716 3.92451 2.5251 1.90672 -.0041801
112
9 1 1 1
1 5
3
1
Table 18. Calculated P( p) isotherms of normal butane.
Normal Butane Isotherm at 140 K
1 sotherm 1sochore 1sochore

Dens ty
i Pressure z Der vat ve
i 1 Der vat ve
i i Curvature
kg/m-5 MPa MPa •m3/kg MPa/K MPa/K^
.00 .0000 .99999 .02003 .00000 -.0000000
730.42 .0000 .00000 2. 15683 2.03252 -.0075018

730.62 .4335 .02962 2. 16164 2.03406 -.0074912
731 .25 1.7892 . 12217 2. 17666 2.03886 -.0074536
731 .88 3.1543 .21521 2.19176 2.04369 -.0074266
' -.0073952
732.50 4.5290 .30874 2.20693 2.04854
733.12 5.9131 .40274 2.22217 2.05341 -.0073643
733.75 7.3067 .49724 2.23749 2.05831 -.0073341
734.38 8.7099 .59223 2.25289 2.06323 -.0073044
735.00 10.1228 .68771 2.26336 2.06818 -.0072752
735.63 11.5453 .78369 2.28391 2.07315 -.0072466
736.25 12.9777 .88017 2.29954 2.07814 -.0072185
736.87 14.4198 .97715 2.31524 2.08316 -.0071910
737.50 15.8718 1.07463 2.33102 2.08820 -.0071641
738.12 17.3337 1.17261 2.34688 2.09327 -.0071376
738.75 18.8053 1.27109 2.36282 2.09836 -.0071 1 17
739.38 20.2871 1.37009 2.37883 2.10347 -.0070864
740.00 21.7789 1.46960 2.39493 2.10860 -.0070615
740.63 23.2808 1.56961 2.41 1 10 2.1 1376 -.0070372
741 .25 24.7928 1.67015 2.42736 2. 1 1894 -.0070134
741 .87 26.3150 1 .771 19 2.44369 2.12414 -.0069901
742.50 27.8474 1.87276 2.4601 1 2. 12937 -.0069673
743. 13 29.3901 1.97485 2.47660 2. 13461 -.0069450
743.75 30.9432 2.07746 2.49318 2. 13988 -.0069232
Norma 1 1 Butane 1 sotherm at 150 K
.00 .0000 .99997 .02146 .00000 -.0000000
721 .01 .0000 .00000 2.01286 1.89224 -.006291

721 .25 .4770 .03082 2.01827 1.89403 -.0062820
722.50 3.01 78 . 19466 2.04699 1.90352 -.0062354
723.75 5.5946 .36026 2.07598 1.91309 -.0061 905
725.00 8.2078 .52762 2. 10524 1.92275 -.0061474
726.25 10.8578 .69677 2. 13479 1.93249 -.0061059
727.50 13.5449 .8677 2.16461 1.94232 -.0060661
728.75 16.2695 1 .04046 2.19472 1.95222 -.0060779
730.00 1 9 . 03 1 1 .21503 2.2251 1.9622 00599 1
731 .25 21 .8324 1 .39144 2.25580 1.97228 -.0059563

732.50 24.6716 1 .56971 2.28677 1.98242 -.0059228
733.75 27.5495 1 .74983 2.3 1803 1.99265 -.0058909
735.00 30.4667 1 .93183 2.34959 2.00296 -.0058605
736.25 33.4236 2. 15721 2.38145 2.01334 -.005831
737.50 36.4205 2.301 52 2.41361 2.02379 -.0058041
738.75 39.4577 2.48923 2.44607 2.03433 -.0057781
740.00 42.5357 2.67888 2.47885 2.04494 -.0057535
741.25 45.6549 2.87047 2.51 193 2.05562 -.0057304
742.50 48.8157 3.06403 2.54533 2.06638 -.0057086
743.75 52.0184 3.25957 2.57904 2.07721 -.0056883
745.00 55.2634 3.45710 2.61308 2.0881 -.0056692
746.25 58.5512 3.65664 2.64744 2.09908 -.0056516
747.50 61.8822 3.85820 2.68212 2.11012 -.0056352
748.75 65.2567 4.06180 2.71714 2.12123 -.0056202
750.00 68.6751 4.26745 2.75249 2.13241 -.0056064
113
1 1
Isotherm sochore
1 1sochore
Dens ty i Pressure Z Derivative Der vat vei i Curvature
kg/m3 MPa MPa.m3/kg MPa/l< MPa/K2
.00 .0000 .99990 .02288 .00000 -.0000000
71 1 .62 .0000 .00000 1.87808 1.76421 -.00531 12

712.50 1.6660 .10216 1.89736 1.77075 -.0052872
713.75 4.0549 .24822 1.92488 1.78008 -.0052543
715.00 6.4783 .39587 1.95266 1,78948 -.0052228
716.25 8.9366 .54514 1.98069 1,79895 -.0051925
717.50 1 1.4301 .69603 2.00897 1,80850 -.0051635
718.75 13.9592 .84856 2.03752 1,81812 -.0051358
720.00 16.5240 1.00273 2.06633 1,82781 -.0051093
721.25 19. 1251 1.15856 2.09540 1,83757 -.0050841
722.50 21.7626 1.31606 2.12474 1,84741 -.0050600
723.75 24.4370 1.47524 2.15434 1,85731 -.0050371
725.00 27.1486 1.6361 2.18422 1,86728 -.0050154
726.25 29.8977 1.79868 2.21437 1,87733 -.0049948
727.50 32.6847 1.96297 2,24479 1,88744 -.0049753
728.75 35.5098 2.12898 2.27550 1.89762 -.0049570
730.00 38.3735 2.29673 2.30648 1.90787 -.0049398
731.25 41 .2761 2.46624 2.33774 1.91818 -.0049237
732.50 44.2181 2.63751 2,36930 1.92857 -.0049086
733.75 47. 1995 2.81055 2.401 13 1.93901 -.0048947
735.00 50.2210 2.98538 2.43326 1.94953 -.0048817
736,25 53.2828 3. 16201 2.46568 1.9601 1 -.0048699
737.50 56.3854 3.34046 2.49840 1.97075 -.0048590
738.75 59.5289 3.52072 2.55142 1.98146 -.0048492
740.00 62.7140 3.70283 2.56474 1.99223 -.0048404
741 .25 65.9409 3.88679 2.59836 2.00306 -.0043325
742.50 69.2100 4.07262 2.63230 2.01395 -.0048257
Normal Butane 1 sotherm at 180 K
.01 .0003 .99937 ,02572 .00000 -.0000000
692.81 .0003 .00002 1,63122 1.53821 -.0038429

693.75 1.5495 .08674 1,64998 1.54483 -.0038301
695.00 3.6276 .20271 1,67501 1.55364 -.0038139
696.25 5.7371 .32002 1,70026 1.56250 -.0037986
697.50 7.8783 .43867 1,72574 1.57143 -.0037840
698.75 10.0515 ,55867 1,75144 1.58042 -.0037701
700.00 12.2570 .68004 1,77 73/ 1.58946 -.0037570
701.25 14.4950 ,80278 1,80353 1.59856 -.0037447
702.50 16.7659 .92689 1 ,82992 1.60772 -.0037331
703.75 19.0699 1.05240 1,85654 1.61694 -.0037222
705.00 21 .4074 1.17930 1,88340 1.62621 -.0037120
706.25 23.7785 1.30760 1,91049 1.63555 -.0037025
707.50 26.1837 1,43732 1,93782 1.64493 -.0036937
708.75 28.6232 1,56846 1,96538 1.65438 -.0036856
710.00 31.0972 1,70103 1,99319 1,66388 -.0036781
71 1.25 33.6062 1,83504 2,02124 1,67344 -.0036714
712.50 36.1504 1,97051 2,04954 1,68305 -.0036653
713.75 38 . 7302 2, 10743 2,07808 1,69272 -.0036598
715.00 41 .3457 2,24581 2,10686 1,70244 -.0036550
716.25 43.9974 2,38568 2.13590 1,71222 -.0036508
717.50 46.6856 2,52703 2. 16519 1,72206 -.0036473
718.75 49.4105 2,66987 2.19473 1.73195 -.0036444
720.00 52.1725 2,81422 2.22453 1.74189 -.0036421
721.25 54.9720 2,96009 2.25459 1.75188 -.0036404
722.50 57.8091 3, 10747 2.28491 1.76194 -.0036394
723.75 60.6843 3,25640 2.31548 1.77204 -.0036389
725.00 63.5979 3,40686 2.34633 1.78220 -.0036391
726.25 66.5503 3,55887 2.37743 1.79241 -.0036398
727.50 69.5416 3,71245 2.40881 1.80267 -.003641
114

Density Pressure Z Der vat ve
i i Der vat ve
1 1 Curvature
kg/m3 MPa MPa-m3/kg MPa/K MPa/K^
.07 .0019 .99751 .02847 .00001 -.0000000
673.85 .0019 .00010 1.40894 1.34406 -.0028162

675.00 1.6332 .08457 1.42965 1.35158 -.0028097
676.25 3.4345 .17752 1.45235 1.35981 -.0028031
677.50 5.2642 .27159 1.47527 1.36808 -.0027970
678.75 7.1227 ^ .36680 1.49838 1.37641 -.0027914
680.00 9.0102 .46315 1.52170 1.38478 -.0027863
681.25 10.9271 .56065 1.54522 1.39320 -.0027816
682.50 12.8734 .65930 1.56895 1.40167 -.0027773
683.75 14.8495 .75911 1.59289 1.41019 -.0027735
685.00 16.8557 .66010 1.61704 1.41875 -.0027702
686.25 18.8922 .96226 1.64140 1.42736 -.0027672
687.50 20.9593 1.06560 .66597
1 1.43603 -.0027647
688.75 23.0572 1.17014 1.69076 1.44474 -.0027627
690.00 25.1863 1.27587 1.71576 1.45349 -.0027610
691.25 27.3467 1.38281 1.74097 1.46230 -.0027598
692.50 29.5388 1.49096 1.76640 1.471 15 -.0027589
693.75 31.7628 1.60032 1.79205 1.48005 -.0027585
695.00 34.0190 1.71092 1.81792 1.48900 -.0027585
696.25 36.3077 1.82274 1.84401 1.49800 -.0027589
697.50 38.6292 1.93581 1.87033 1.50704 -.0027597
698.75 40.9836 2.05012 1.89686 1.51613 -.0027608
700.00 43.3714 2.16569 1.92363 1.52527 -.0027624
701.25 45.7928 2.28253 1.95062 1.53445 -.0027643
702.50 48.2481 2.40063 1.97783 1.54369 -.0027667
703.75 50.7375 2.52001 2.00528 1.55297 -.0027694
705.00 53.2614 2.64067 2.03296 1.56229 -.0027725
706.25 55.8200 2.76263 2.06087 1.57167 -.0027759
707.50 58.4136 2.88589 2.08902 1.58108 -.0027798
708.75 61 .0426 3.01045 2.1 1740 1.59055 -.0027840
710.00 63.7072 3.13633 2. 14602 1.60006 -.0027886
71 1.25 66.4078 3.26353 2.17488 1.60962 -.0027936
712.50 69.1445 3.39207 2.20398 1.61923 -.0027989
713.75 71 .9178 3.52194 2.23332 1.62888 -.0028046
115
1 1 7
sotherm
1 Isochore 1sochore
Density Pressure Z Derivative Der vat ive
i Curvature
kg/m-J MPa MPa •m-J/kg MPa/K MPa/K^
.25 .0078 .99302 .03105 .00004 -.0000000
654.60 .0078 .00038 1 .20671 1. 174 55 -.0020734

655.00 .4948 .02400 1.21 322 1 . 7698
1 -.0020729
656.25 2.0240 .09800 1.23355 1 . 18457 -. 002071
657. 50 3. 5788 .17296 .25406
1 1 . 9220
1 -.0020708
658.75 5. 593 1 .24887 1.27477 1 .19987 -.0020702
660.00 6.7658 .32574 1.29566 1 .20758 -.0020699
661 .25 8.3985 .403 59 1.31673 1 .21533 -,0020699
662.50 10.0577 .48240 1.33800 1 .22312 -.0020701
663.75 1 .7436
1 .56221 .35946
1 1 .23095 -.0020707
665.00 13.4564 .64299 1 .381 1 1 .23883 -.0020715
666.25 15. 1965 .72478 1.40296 1 .24674 -.0020726
667.50 16.9639 .80756 1.42499 1 .25470 -.0020739
668.75 18.7590 .89134 1.44723 1 .26270 -.0020755
670.00 20.5821 .97614 1.46965 1 .27074 -.0020774
671 .25 22.4333 1.06196 1.49228 1 .27882 -.0020795
672.50 24.3129 1. 14880 1.51510 1 .28694 -.0020818
673.75 26.221 1 1.23666 1.53812 1.2951 -.0020845
675.00 28.1583 1.32556 1.56134 1.30331 -.0020873
676.25 30. 1246 1 .4 1551 1.58477 1.31 156 -.0020905
677.50 32. 1203 1.50650 1.60839 1.31985 -.0020938
678.75 34. 1456 1.59854 1.63222 1.32818 -.0020975
680.00 36.2009 1.69165 1.65625 1.33655 -.0021013
681 .25 38.2863 1.78581 1.68049 1.34497 -.0021054
682.50 40.4022 1 .88105 1.70494 1.35342 -.0021098
683.75 42.5488 1.97737 1.72959 1.36192 -.0021 144
685.00 44.7263 2.07478 1.75445 1.37046 -.0021 192
686.25 46.9350 2. 17327 1.77952 1.37904 -.0021243
687.50 49. 1752 2.27286 1 .80481 1.38766 -.0021296
688.75 51 .4471 2.37355 1 .83030 1.39633 -.0021351
690.00 53.7510 2.47535 1.85601 1.40503 -.0021409
691.25 56.0872 2.57827 1.88194 1.41378 -.0021469
692.50 58.4560 2.68230 1.90808 1.42257 -.0021531
693.75 60.8575 2.78747 1.93444 1.43140 -.0021596
695.00 63.2921 2.89377 1.96102 1.44027 -.0021663
696.25 65.7601 3.00121 1.98781 1.44918 -.0021733
697.50 68.2618 3.10980 2.01483 1.45814 -.0021805
698.75 70.7973 3.21954 2.04207 1.46714 -.0021879
116
7
1 9
5 0
11 8

Dens ty i Pressure Z Der ydt ve
i i Der vat ve
i i Curvature
kg/m-5 MPa MPa •rrP/kg MPa/K MPa/K^
.71 .0241 .98456 .03532 .00010 -.0000000
634.87 .024 .001 10 1 .02168 1 .02453 -.001 5203

635.00 . 576
1 .00723 1 .02356 1 .02526 -.00 5205
1
637. 50 2.7618 . 1261 1 .05990 1 .03922 -.001 5250

640.00 5.4577 .24839 1 .09693 1 .05332 -.001 5302
642.50 8.2471 .37388 1 . 13467 1 .06757 -.001 5361
645.00 1 1.1317 .50270 1 . 1 731 1 .08 196 -.00 15427
647.50 14. 1 132 .63489 1 .21226 1.09649 -.001 5499
650.00 17. 1936 .77048 1 .25214 1.11117 -.0015578
652.50 20.3745 .90953 1 .29274 1. 12600 -. 0015663
655.00 23.6578 1 .05207 1 .33409 1.14097 -.0015754
657.50 27.0455 1 . 1981 1 .37617 1.15609 -.0015851
660.00 30.5394 1 .34780 1.41901 1. 7135
1 -.0015954
662.50 34.1412 1.50108 1.46260 1.18677 -.0016063
665.00 37.8530 1 .65802 1 .50696 1.20233 -.0016178
667.50 41.6767 1 .81866 1.55210 1.21805 -.0016299
670.00 45.6142 1 .98306 1.59802 1.23391 -.0016426
672.50 49.6674 2.15124 1.64472 1.24993 -.0016558
675.00 53.8385 2,32327 1 .69223 1.26609 -.0016697
677.50 58.1292 2.49917 1.74054 1.28241 -.0016842
680.00 62.5418 2.67900 1.78967 1.29887 -.0016992
682.50 67.0783 2.86279 1 .83962 1.31549 -.0017149
685.00 71,7406 3.05060 1 .89040 1.33226 - .0017312
Norma 1 I
3utane Isotherm at 260 K
1 .69 .0610 .97089 .0351 .00025 -.0000001
614.46 .0610 .00267 .85208 .8901 -.0010979

61 5.00 .5249 .02295 .85896 .89293 -.0010998
617.50 2.7122 .11810 .89 105 .90569 -.001 1084
620.00 4.9806 .21 599 .92379 .91858 -.001 1 174
622.50 7.331 .31668 .95717 .931 59 -.001 1268
625.00 9.7671 .42018 .99122 .94473 -.001 1366
627 . 50 12.2883 .52654 1 .02592 .95799 -.001 1467
630.00 14.8972 .63579 1 .06130 .971 39 -.001 1572
632.50 17.5954 .74798 1 .09736 .98491 -.001 1681
635.00 20.3846 .86313 1 . 1341 .99857 -.001 1793
637. 50 23.2665 .98 29 1 1 . 1 7 53
1 1 .01 236 -.001 1909
640.00 26.2429 1 . 10250 1.20967 1 .02628 -.0012028
642.50 29.31 54 1 .22679 1.24851 1 .04033 -.001 2150
645.00 32.4860 1 .35421 1.28806 1 .05452 -.0012277
647. 50 35.7563 1 .48478 1.32833 1 .06885 -.001 2406
650.00 39.1283 1.61855 1.36933 1.08331 -.0012539
652.50 42.6036 1 .75555 1.41 106 1.09790 -.0012676
655.00 46.1841 1.89583 1.45354 1 . 12631 -.0012817
657.50 49.8719 2.03943 1.49676 1.12751 -.0012961
660.00 53.6686 2.18637 1.54074 1.14251 -.0013109
662.50 57.5762 2.33671 1.58549 1.15766 -.0013261
665.00 61.5967 2.49049 1.63100 1.17295 -.0013416
667.50 65.7319 2.64773 1.67729 1.18838 -.0013575
670.00 69.9838 2.80848 1,72437 1.20395 -.0013739
117
1 1
Isotherm 1 sochore 1sochore

Dens ity Pressure Z Der vat ve
i i Der vat ve
i i Curvature
kg/m-J MPa MPa •m3/kg MPa/K MPa/K^
2.50 .0965 .96392 .03728 .00037 -.0000002

3.49 .1330 .95069 .03620 .00053 -.0000004
593. 1 . 1330 .00560 .69689 .76860 -.0007679

595.00 1.4717 .06175 .71 778 .77732 -.0007762
597.50 3.301 . 13794 .74589 .78894 -.0007873
600.00 5.2016 .2 1 64 5 .77460 .80066 -.0007986
602.50 7. 1746 .29731 .80390 .81250 -.0008101
605.00 9.2217 .38055 .83382 .82446 -.0008218
607.50 1 .3442
1 .46622 .86435 .83653 -.0008336
610.00 13.5440 .55434 .89551 .84872 -.0008456
612.50 15.8223 .64495 .92730 .86102 -.0008577
615.00 18. 1810 .73808 .95972 .87344 -.0008701
617.50 20.6215 .83377 .99279 .88598 -.0008826
620.00 23. 1455 .93205 1 .02651 .89864 -.0008953
622.50 25.7546 1 .03295 1 .06089 .91 143 -.0009082
625.00 28.4505 1. 13651 1 .09593 .92433 -.00092 12
627.50 31 .2348 1 .24276 1 . 1 3 1 64 .93736 -.0009345
630.00 34 . 092 1 1 .351 75 1. 16803 .95051 -.0009480
632.50 37.0755 1.46349 1.20511 .96378 -.0009616
635.00 40. 1354 1. 57804 1.24288 .97718 -.0009755
637.50 43.2905 1.69542 1.28135 .99071 -.0009896
640.00 46.5427 1.81566 1.32052 1.00436 -.0010039
642.50 49.8937 1.93881 1.36041 1.01815 -.0010185
645.00 53.3453 2.06491 1.40101 1.03206 -.0010332
647.50 56.8994 2.19397 1.44234 1.04610 -.0010482
650.00 60.5577 2.32605 1.48441 1.06027 -.0010635
652.50 64.3220 2.461 18 1.52721 1.07457 -.0010790
655.00 68. 1943 2.59938 1.57076 1.08900 -.0010948
118
1 1
Normal Butane Isotherm at 298.150 K
1 sotherm Isochore 1sochore

Dens ty
i Pressure Z Der vat ve
1 1 Der vat ve
i i Curvature
kg/m3 MPa MPa.m3/kg MPa A MPa/K^
2.50 .1032 .96802 .04006 .00037 -.0000001

5.00 .2003 .93919 .03757 .00076 -.0000007
6. 18 .2438 .92534 .03634 .00096 -.0000012
572.65 .2438 .00998 .56807 .66742 -.0005261

575.00 1.6070 .06553 .59049 .67726 -.0005378
577.50 5.1136 . 264
1 .61484 .68781 -.0005502
580.00 4.6817 .18926 .63973 .69847 -.0005627
582.50 6.3127 .25410 .66517 .70923 -.0005752
585.00 8.0080 .32096 .691 17 .72009 -.0005877
587.50 9.7690 .38988 .71774 .73105 -.0006002
590.00 11.5972 .46088 .74489 .74213 -.0006128
592.50 13.4939 .53400 .77261 .75330 -.0006255
595.00 15.4608 .60926 .80093 .76459 -.0006382
597.50 17.4991 .68670 .82984 .77599 -.0006510
600.00 19.6105 .76634 .85935 .78749 -.0006638
602.50 21.7964 .84823 .88948 .7991 -.0006768
605.00 24.0584 .93239 .92022 .81084 -.0006898
607.50 26.3980 1.01885 .95158 .82268 -.0007029
610.00 28.8168 1.10765 .98358 .83463 -.0007160
612.50 31.3164 1.19882 1.01621 .84670 -.0007293
615.00 33.8984 1.29238 1.04949 .85889 -.0007428
617.50 36.5644 1.38838 1.08341 .871 19 -.0007563
620.00 39.3160 1.48684 1.1 1800 .88361 -.0007699
622.50 42.1549 1.58780 1.15325 .89615 -.0007837
625.00 45.0828 1.69129 1.18917 .90881 -.0007976
627.50 48.1013 1.79734 1.22576 .92158 -.00081 17
630.00 51.2122 1.90598 1.26304 .93448 -.0008259
632.50 54.4171 2.01726 1.30102 .94750 -.0008402
635.00 57.7178 2.13119 1.33969 .96064 -.0008547
637.50 61.1 161 2.24782 1.37906 .97391 -.0008694
640.00 64.6137 2.36718 1.41915 .98729 -.0008843
642.50 68.2125 2.48930 1.45995 1.00081 -.0008993
645.00 71.9141 2,61421 1.50148 1.01444 -.0009145
119
11 D
C1
1

Density Pressure Z Der ivat ve 1 Der Ivat Ive Curvature
kg/m^ MPa MPa 'm^/kg MPa/K MPa/K^
2.50 .1039 .96839 .04034 .00037 -.0000001

5.00 .201 7 .93998 .03788 .00076 -.0000006
6.52 .2582 .92233 .03630 .00102 -.0000014
570.49 .2582 .01055 .55557 .65753 -.0005039

572.50 1.3934 .05671 .57438 .66585 -.0005140
575.00 2.8591 .1 587
1 .59826 .67628 -.0005265
577.50 4.3851 . 17694 .62268 .68681 - .0005391
.54764 .69744 AAA C C ^
-•000551 1
580.00 5.9729 .23997
.673 16 .70817 AA A C O y1
582.50 7.6238 .30498

.69924 .71 901
AAA
U0U5C*?^: Q
/ DO
585.00 9.3392 .37201
A A A CQ A>t
587.50 1 1205
1 . .44 108 .72589 .72995
AAA^r AO 1
590.00 12.9691 222
.51 .7531 .74 001 UUUoUZ
.75216 AAA C Q 1 >1
592.50 14.8865 .58547 .78092
.8093 .76342 AA AÔ
595.00 16.8742 .66085
A A A^ A
-.0005404 Vl >l
597.50 18.9336 .73840 .83830 .77479

.78627 AA A CZ A
-.0006534z;
600.00 21 .0662 .81815 .86790
A A Ail CdL'Z
-.0006553
602.50 23.2736 .90013 .8981 .79787
A AAC TAyl
-.0005794
605.00 25.5572 .98437 .92893 .80957
A A A£ AO
-.0005925
607.50 27.9187 1.07090 .96038 . 82 39
1
A A AT A C O
-.0007058
610.00 30.3597 1. 5976
1 .99246 .83332
.84536 AAA T A
-.00071 1
612.50 32.8816 1.25097 1 .02517 91
615.00 35.4861 1.34457 1 .05854 .85752 -.0007325
617.50 38. 1748 1.44059 1.09255 .86980 -.0007461
AAA T C AO
620.00 40.9494 1.53906 1.12722 .88220 -.0007598
AAA"7"7Ttf^
622.50 43.81 15 1.64002 1 . 16256 .89471 -.UUU / /3d
625.00 46.7627 1.74349 1.19857 .90734 -.0007875

627.50 49.8048 1.84952 1.23525 .92009 -.0008016
630.00 52.9395 1.95812 1 .27262 .93296 -.0008158
632.50 56.1685 2.06935 1 .31069 .94595 -.0008302
635.00 59.4936 2.18322 1.34945 .95907 -.0008447
637.50 62.9164 2.29977 1.38891 .97231 -.0008594
640.00 66.4387 2.41903 1.42909 .98567 -.0008743
642.50 70.0624 2.54104 1.46998 .99915 -.0008893
120
1 0 4 51

Dens ity Pressure Z Derivative Der ivative Curvature
kg/m-' MPa fâ •m3/kg MPa/K MPa/K^
2.50 .1112 .97194 .04336 .00037 -.0000001

5.00 .2168 .94743 .041 12 .00075 -.0000004
7.50 .3168 . 92270 ,03881 .001 17 -.000001
10.00 .41 08 .89751 .03643 .001 62 -.0000025
1 1 .30 .4575 .884 18 .03516 .00187 - .0000035
546. 16 .4575 .01830 .42794 .55518 -.0002873

547.50 .0367
1 .04 36 1 .43823 .56008 -.0002945
550.00 2. 566 1 .08566 .45781 .5693 1 -.0003082
"Z
3.3261 "Z 1 CO
1 "Z 1
3 52 .47788 . 57863 -.0003z
552. 50 . 1 1 1
555.00 4 . 54 64 .17896 .49843 .58804 -.0003348

'
557. 50 5.8187 .22801 .51 946 .59754 -.0003479
560.00 7. 1442 .27870 .54 001 .5071 -.0003509
562. 50 8.5241 .33 05 1 .56304 .61683 -.0003739
565.00 9.9598 .3851 .58560 .62661 -.0003867
567.50 1 .4525
1 .44087 .60867 .63649 -.0003995
570.00 13.0036 .49838 .63227 .64647 -.0004123
572.50 14 . 6 43 1 . 55767 .65641 .65654 -.0004250
575.00 16.2861 .61 876 .68108 .66672 -.0004377
577.50 18.0202 .68 168 .70631 .67700 -.0004 504
580.00 19.8181 .74646 .73209 .68737 -.000463
582.50 21 .681 .81312 .75843 .69785 -.0004757
585.00 23.6107 .88171 .78534 .70844 -.0004884
587.50 25.6083 .95224 .81283 .71912 -.000501
590.00 27.6753 1.02474 .84090 .72992 -.00051 39
592.50 29.8133 1.09924 .86956 .74081 -.0005266
595.00 32.0236 1. 17578 .89882 .75182 -.0005394
597.50 34.3079 1.25438 .92868 .76293 -.0005523
600.00 36.6675 1.33506 .95915 .77416 -.0005552
602.50 39. 1042 1.41787 .99025 .78549 -.0005781
605.00 41 .6193 1. 50283 1.02196 .79693 -.000591
607.50 44.2145 1.58997 1.05431 .80848 -.0006042
610.00 46.8914 1.67932 1.08729 .82015 -.0006174
612.50 49.6515 1.77092 1.12092 .83193 -.0006307
615.00 52.4965 1.86478 1.15521 .84382 -.0006441
617.50 55.4281 1.96094 1.19014 .85582 -.0006575
620.00 58.4478 2.05944 1.22575 .86794 -.000671
622.50 61 .5574 2.16029 1.26202 .88018 -.0006847
625.00 64.7585 2.26354 1.29898 .89253 -.0006985
627.50 68.0528 2.36921 1.33661 .90500 -.0007124
630.00 71 .4421 2.47734 1.37494 .91759 -.0007265
121
D 1
sotherm
1 1sochore 1sochore
Dens ity Pressure Z Der vat ve
i i Der vat ve
i i Curvature
kg/m3 MPa MPaTti3/k<j MPa/K MPa/K2
5.00 .2318 .95339 .04429 .00075 -.0000002

10.00 .4428 .91037 .04005 .00158 -.0000014
15.00 .6322 .86662 .03572 .00252 -.0000044
18.56 .7538 .83513 .03260 .00328 -.0000088
519.47 .7538 .02984 .31403 .46003 -.0001035

520.00 .9207 .03641 .31724 .46172 -.0001066
525.00 2.5845 .10122 .34853 .47787 -.0001355
530.00 4.4088 .17104 .38148 .49434 -.0001632
535.00 6.4022 .24605 .41614 .51114 -.0001898
540.00 8.5732 .32643 .45257 .52828 -.0002157
545.00 10.9309 .41238 .49082 .54577 -.0002409
550.00 13.4846 .50410 .53096 .56362 -.0002657
555.00 16.2438 .60178 .57304 .58184 -.0002902
560.00 19.2183 .70562 .61712 .60043 -.0003145
565.00 22.4184 .81583 .66325 .61940 -.0003385
570.00 25.8543 .93261 .71 148 .63877 -.0003625
575.00 29.5368 1.05618 .76189 .65852 -.0003864
580.00 33.4769 1.18675 .81451 .67868 -.0004104
585.00 37.6858 1.32454 .86942 .69925 -.0004345
son no Hi. « \ t vU 1
1. &Mlfi
HO V / . / ^\J^.J — • UUU'f JO 1
595.00 46.9563 1.62263 .98628 .74163 -.0004830

600.00 52.0418 1.78338 1.04835 .76346 -.0005076
605.00 57.4439 1.95223 1.1 1291 .78573 -.0005325
610.00 63.1752 2.12941 1.18002 .80843 -.0005577
615.00 69.2485 2.31514 1.24974 .83158 -.0005832
Normal Butane 1 sotherm at 360 K
5.00 .2467 .95829 .04741 .00074 -.0000002

10.00 ,474 1 .92065 .04352 .00156 -.0000009
15.00 .6819 .88284 .03962 .00245 -.0000027
20.00 .8703 .84502 .03573 .00345 -.0000059
25.00 1.0393 .80729 .03187 .00456 -.0000115
29.39 1.1718 .77422 .02847 .00565 -.0000200
489.36 1.1718 .04650 .21405 .37071 .0000609

490.00 1.3100 .05192 .21699 .37246 .0000567
495.00 2.4534 .09625 .24058 .38624 .0000250
500.00 3.7181 .14440 .26554 .40030 -.0000045
505.00 5.1111 .19654 .29192 .41466 -.0000321
510.00 6.6397 .25281 .31977 .42932 -.0000584
51 5.00 8.31 14 .31339 .34915 .44429 -.0000836
520.00 10.1338 .37843 .3801 .45959 -.0001080
525.00 12.1 152 .44812 .41270 .47521 -.0001317
530.00 14.2637 .52261 .44699 .491 18 -.0001549
535.00 16.5880 .60209 .48302 .50748 -.0001777
540.00 19.0969 .68673 .52085 .52414 -.0002001
545.00 21.7996 .77673 .56054 .541 16 -.0002224
550.00 24.7055 .87227 .60214 .55854 -.0002444
555.00 27.8243 .97353 .64571 .57630 -.0002664
560.00 31 .1660 1.08072 .69130 .59443 -.0002884
565.00 34.7408 1.19402 .73898 .61294 -.0003103
570.00 38.5593 1.31363 .78878 .63184 -.0003323
575.00 42.6323 1.43976 .84078 .651 14 -.0003544
580.00 46.9709 1.57261 .89502 .67083 -.0003766
585.00 51.5864 1.71237 .95157 .69094 -.0003990
590.00 56.4905 1.85927 1.01047 .71 145 -.0004216
595.00 61.6952 2.01351 1.07179 .73238 -.0004444
600.00 67.2125 2.17529 1.13556 .75374 -.0004675
122
. 2JR
Isotherm 1 sochore 1sochore

Pressure Z Derivative Der vat ve Curvature
Dens ity i i
MPa MPa .m3/kg MPa/K Mra/K

kg/in3
.2616 .96242 .05050 .00074 -.0000001

5.00
.5051 .92915 .04689 .00154 -.0000007
10.00
.7306 .89600 .04332 .00241 -.00000 18
15.00
.9383 .86310 .03980 .00336 -.0000038
20.00
1.1286 .83052 .03634 .00439 -.0000068
25.00
1.3018 .79829 .03294 .00550 -.00001 1
30.00
1.4581 .76639 .02959 .00672 -.0000 177
35.00 .
\,5911 .73482 .02629 .00804 -.0000272

40.00
1.7210 .70357 .02303 .00948 -.0000422
45.00
45.78 1.7387 .69873 .02252 .00972 -.0000453
453.83 1. 7387 .07048 .12849 .28570 .0002238

455.00 1.8910 .07646 .13216 .28832 .0002143
460.00 2.5923 .10367 . 14849 .29965 .0001769
465.00 5.1111 .13363 .16588 .31 122 .0001 438
470.00 4.2529 . 6647
1 .1 8437 .32305 .0001 137
r\i\(^ r\c> ^ o
475.00 5.2234 .20230 .20403 .33514 .0000860
480.00 6.2952 .24127 .22488 .34751 .0000601
485.00 7.4743 .28351 .24699 .36017 .0000355
490.00 8.7673 .32916 .27041 .37312 .00001 23
495.00 10.1806 .37836 .29517 .38637 -.00001 Ql
500.00 11.7213 .43127 .32134 .39993 -.uouu^ ly
505.00 13.3964 .48802 .34896 .4 3801
510.00 15.2134 .54877 .37808 .42799 -.oouu /jy

r\r\r\r\CiA
515.00 17.1798 .61369 .40876 .44251 -.uuuuy4
C "7*2 "7 r\r\r\ / R
520.00 19.3036 .68293 .44 104 .45737
>1
-.UUU i
114 5 1
21.5930 .75664 .47499 .472 56 -. UUU j44

525.00 1
530.00 24.0564 .83501 .51066 .48809 -.UUU 134z 1
535.00 26.7025 .91820 .54809 .50398 UUU "7*zn

-. r\r\r\ 1
/jy
1
. 52022
Ann yjp
-.UUU 1
540.00 29.5403 1.00637 .58735 1
545.00 32.5791 1.09972 .62849

550.00 35.8284 1 .
1 9840 .67156 .55378 -.0002328
555.00 39.2980 1.30261 .71662 .571 12 -.0002526
560.00 42.9981 1.41253 .76373 .58883 -.0002724
565.00 46.9389 1.52835 .81295 .60692 -.0002923
570.00 51.1311 1.65025 .86432 .62541 -.0003124
575.00 55.5857 1.77842 .91790 .64428 -.0003327
580.00 60.3139 1.91306 .97375 .66355 -.0003532
585.00 65.3271 2.05436 1.03192 .68322 -.0003739
590.00 70.6371 2.20252 1.09248 .70330 -.0003948
123
3
1 A 1
I SO therm 1 sochore I sochore

Den s ty
i Pressure z \J\^\ 1 V <J 1 1 VJsD 1 1 V u 1 1
0 u p \/V a
o 1 1 ^1 1
11 r"
u( c
kq/m-5 MPa MPa •m3 /kg MPa/K (i^Pa/K 2
5.00 .2764 .96595 .05356 .00074 - nnnnnni

in on 5357 .93637 0'5n7n nni s'^ - nnnnnns
1 5.00 ,11 nn7'^R - nnnnni
20.00 1 . 0048 .87802 .04366 nn^79
25.00 1 .2 52 1 .84948 .04050 .00427 • \J\J\J\J\JH\J
30.00 1.4099 .82136 .03742 .00532 -.0000073

35.00 1.5894 .79366 .03440 .00644 -.0000108
40.00 1.7540 .76638 .03146 .00763 - nnnni S4
45.00 1 .9041 . 73951 07859 nnRQn - nnnn7 17
50 on 2. 0401 .7 308
1 n7Sftn - nnnn7Hft
55.00 2 . 623 1 .687 10 .0231 .01 165 - nnnn'^RS
60 . 00 2 . 27 1 .661 59 .02050 .01315 -.0000514
65.00 2.3675 .63655 .01798 .01474 -.0000691
70.00 2.4513 .61 200 .01 555 .01643 -.000094 7
72.54 2.4892 .59973 .01435 . 0 734
1 -.0001 128
408 .02 2.4892 . 0662

1 .05843 .20249 .0004306
410.00 2.6082 .11118 .061 93 .20585 .0004060
415.00 2.9409 .12385 .07129 .21447 .0003528
420.00 3.3223 .13824 .08138 .22328 .0003089
425.00 3.7560 .15445 .09223 .23230 .0002716
430.00 4.2460 .17257 . 10390 .24 55 1 .0002389
435.00 4.7964 .19270 . 1 641 1 .25103 .0002097
440.00 5.4 16 1 .21495 . 12982 .26075 .0001832
445.00 6. 0961 .23942 .14415 .27073 .0001 587
450.00 6.8547 .26622 . 15946 .28097 .0001358
455.00 7.6924 .29547 .17577 . 29 48 1 .0001 141
460.00 8.6142 .32726 .19314 .30227 .0000935
465.00 9.6256 .361 77 .21161 .31333 .0000736
470.00 10.7322 .39907 .23121 .32468 .0000544
475.00 .9397
1 1 .43930 .25201 .33632 .0000357
480.00 13.2543 .48259 .27403 .34825 .0000175
485.00 14.6822 .52907 .29734 .36050 -.0000005
490.00 16.2299 .57887 .32197 .37304 -.0000181
495.00 17 .904 .63214 .34797 .38590 -.00003 56
500 on 1 9. 7 120 .68900 .37540 .39907 -.0000529
5n5 on 9 1
1 fifinfi
• \JKJ\J\J .74962 .40430 .4 1256 -.0000702
sin nn 9"^ 7S7R - 0000ft7"S
5 5.00
1 .46673 .44052 -.0001045
s^n nn 4 55ni - 0001716
nn ^1 0170 .53568 .46983 -.0001 388
s^n nn • 1 O fJ \ 1 1 4 1 - OOOISfiO
535.00 36.7473 1.20042 .61 158 .50051 -.0001733
540.00 39.9062 1.29154 .65227 .51638 -.0001907
545.00 43.2732 1.38766 .69486 .53261 -.0002082
550.00 46.8580 1.48896 .73940 .54920 -.0002258
555.00 50.6705 1.59560 .78595 .56616 -.0002436
560.00 54.7210 1.70776 .83457 .58350 -.0002616
565.00 59.0198 1.82562 .88532 .60121 -.0002798
570.00 63.5778 1.94936 .93824 .61931 -.0002982
575.00 68.4059 2.07916 .99339 .63779 -.0003168
124
z
11 41 y . 6
5/
1 1 J
A
2
3
/
1/
11
Norma I Butane Isotherm at 410 K
1sotherm Isochore 1sochore

Dens ity Pressure Z Derivative Der vat ve
i i Curvature
kg/fti^ MPa MPa •m3/kg MPa/K MPa/K
.2837 .96753 .05508 AA AT A

.00074 AAAAAA
-.000000
5.00
.5510 .93950 .05183 A A 1 52
.001 no -.AAAAAA
0000004
10.00
r\r\r\r\r\ 0
15.00 .8022 . 91 1 83 .04864 .00237 -.000001 1
20.00 1.0376 .88457 .04554 .00327 UUUUUZ

A A ^ OT
.00423 -•UUUUU
25.00 1.2577 .85776 .04251
A A COiT
.00526 r\r\r\r\r\c i
30.00 1.4628 .83 139 .03956
•03667 AA £ZX A
.00034 -•UuUUUoy
35.00 1.6534 .80544
A A-7/I A
40.00 1.8297 .77992 .U3jod .00 /4y UUUU /.^ 1
45.00 1.9921 .75481 .031 13 .00871 -.0000168

50.00 2. 141 .7301 .02848 .00998 -.0000221
A A A A OOC
-•UUUU/oo
55.00 2.2771 .70592 .02592 .01 132
A A A A'Z C C
-.000036!)
60.00 2.4005 .68217 .02346 .01272
A
.01418 0 1 J1 1 AAAA C
-•000U4D /I 1
65.00 2.51 19 .65890 .021 10
70.00 2.61 17 .63614 .01883 .01 570 -. A AAA C 0 A
0000580
A A A A ~7"Z A
-•0000730
75.00.. 2 . 7004 .61391 .01668 .01 729
A 895
0 AC 1
-• A A A AAO
uouoyz3 "Z
80.00 2.7786 .59221 .01462 .01
2.8468 .57105 .01 267
AO A^ 0
.020DO r\r\r\
-•UUU 0
1 1 "z
85.00 \OJ
r\
r\ r\ c CT
1
90.00 2.9055 .55045 .01 082 .02250 -.0001 553
94.40 2.9496 .53278 .00927 .024 19 -.0002043
A A A ^ AC 1
376.69 2.9496 .13351 .03006 . 5957
1 .00051 05
A AA C A C Ct
380.00 3.0554 .13709 .03375 . 164 1 .0005485
.14344 .03973 .17120 AAA A ~l a C
.0004756
385.00 3.2388
3.4536 .04626 . 17839
AAA A 185
.0004 0C ^
390.00 . 5099
1
AAA 0A
"7 *7
395.00 3.7024 . 5982
1 .05337 .18577 .0003724
400.00 3.9883 .17001 .061 10 .19335 .0003335
405.00 4.3145 .18164 .06948 .201 14 .0002999
r\r\ f\^~i f^T
410.00 4.6843 .19480 .07855 .2091 .0002703
A AA 0 7
415.00 1012
5. .20959 .08833 .2 1740 .0002436
420.00 5.5689 .22608 .09887 .22588 .0002193
425.00 6.0912 .24437 .11020 .23462 .0001968
430.00 6.6722 .26457 . 2235
1 .24360 .0001757
AAA d C 1 "7
435.00 7.3162 .28677 .13537 .25284 .0001 557
AAA T 1 1 tl
440.00 8.0274 . 3 1 1 07 . 14929 .26234 .0001367
445.00 8.8107 .33759 .16416 .272 1 .0001 183
450.00 9.6706 .36642 . 18000 .2821 .0001006
455,00 .39768 9587 A A A AO "Z
10.61 24 . 1 .29246 .0000834 j1
460.00 1 1 . 64 1 .43149 .2 1480 .30306 .0000665

465.00 12.7622 .46796 O
.23384O "Z /! ZA C
"Z 1
.3 395 A AAA C A
.0000500
1
470.00 13.9813 .50721 .254UZ zo c 0

.^2512 1 AAAAZ JZ"?
.OOOOj
4 /5.00 15.3044 .54937
0-7 Cyl 1 X X^ c:q AAAA ~7C
.0000 /o 1
1
480.00 16.7375 .59455 . ^ôUj XA QX c: AAAAA

.00000 1
1
-7
485.00 18.2869 .64289 .JZ 193 z A^0

.30042 AAAA 0
-.0000142 1 yl
490.00 Z "700 A AAAA'ZAA

-.0000300
19.9592 .69452 .34/19 .3 /2o0
493 .00 O 1 •751
21
~7 C 1 O
.74957 .J/3o3 ZQ CACl
.30 549 AAAA
-.0000430 yl
500.00 23.6999 .808 19 .40 o9 1

ZAO CA
.39850 AAAA C C
-.OOOOol 1
A X A A Q0 AAAA"7"7"Z
505.00 25.7826 .87051 .4 J 44 i
1 .4 /I 1
1
1
lo2 -.0000 / /3
51 0.00 28.0 168 .93667 .4DZ52 .4254 AAAAAZ

-.000093
51 5.00 30.4 05 1 1.00682 .4yj 1
A xnA ^
.4 jy4D A A A AAA
-. 000 oyo 1
1
520.00 32.9715 1.08112 .5<i9P0 A C Z~7T

.453 /
A A A 249
-.000 0 A 1
1
y1
525.00 35.7083 1.15971 .56550 .46843 -.0001410

530.00 38.6294 1.24274 .60325 .48343 -.0001571
535.00 41.7438 1.33038 .64279 .49878 -.0001734
540.00 45.0605 1.42279 .68419 .51448 -.0001899
545.00 48.5889 1.52012 .72750 .53053 -.0002065
550.00 52.3388 1.62255 .77278 .54696 -.0002232
555.00 56.3200 1.73024 .82007 .56374 -.0002402
560.00 60.5429 1.84337 .86944 .58090 -.0002574
565.00 65.0180 1.9621 .92094 .59844 -.0002748
570.00 69.7560 2.08663 .97463 ,61635 -.0002924
125
1 1 0

i i Der vat ve
i i Curvature
kg/m3 MPa MPa •m3/kg MPaA MPa/K^
10.00 .5662 .94246 .05346 .00152 -.0000004

20.00 1.0702 .89062 .04739 .00325 -.0000020
30.00 1.5151 .84060 .04164 .00520 -.0000052
40.00 1.9040 .79229 .03619 .00738 -.0000103
50.00 2.2399 .74564 .03104 .00978 -.0000178
60.00 2.5260 .70074 .02624 .01240 -.0000281
70.00 2.7661 .65772 .02183 .01521 -.0000418
80.00 2.9641 .61670 .01784 .01821 -.0000602
90.00 3. 1243 .57780 .01427 .02137 -.0000849
100.00 3.2509 .54109 .01 1 12 .02469 -.0001 192
110.00 3.3481 .50661 .00839 .02816 -.0001701
120.00 3.4199 .47436 .00604 .03180 -.0002547
130.00 3.4701 .44429 .00405 .03566 -.0004309
133.47 3.4830 .43436 .00342 .0371 -.0005514
328.06 3.4830 .17672 .00760 .11119 .001 1287

330.00 3.4985 .17646 .00840 .1 1304 .0010246
340.00 3.6053 . 17650 .01315 .12277 .0007067
350.00 3.7658 .17909 .01918 .13303 .0005459
360.00 3.9940 .18466 .02671 . 14398 .0004450
370.00 4.3058 .19370 .03595 .15571 .0003732
380.00 4.7195 .20672 .04712 . 16829 .0003176
390.00 5.2554 .22429 .06045 . 8 74
1 1 .0002717
400.00 5.9365 .24703 .07618 .19612 .0002320
410.00 6.7880 .27557 .09457 .21 146 .0001964
420.00 7.8377 .31061 .1 1588 .22778 .0001636
430.00 9.1 162 .35287 .14039 .24513 .0001326
440.00 10.6571 .40314 .16839 .26353 .0001028
450.00 12.4967 .46223 .20019 .28301 .0000737
460.00 14.6746 .53098 .23612 .30362 .0000451
470.00 17.2339 .61032 .27651 .32537 .0000167
480.00 20.2209 .70118 .32172 .34830 -.00001 16
490.00 23.6855 .80456 .3721 .37245 -.0000402
500.00 27.6816 .92150 .42807 .39784 -.0000690
510.00 32.2668 1.05307 .49000 .42452 -.0000983
520.00 37.5029 1.20042 .55832 .45251 -.0001280
530.00 43.4558 1.36472 .63343 .48185 -.0001583
540.00 50.1957 1.54720 .71579 .51258 -.0001892
550.00 57.7972 1.7491 .80582 .54473 -.0002210
560.00 66.3391 1.97176 .90396 .57835 -.0002536
126
1 1 1
Norma I Butane Isotherm at 425. 160 K

Dens ty
i Pressure z Der ivat ve 1 Der ivat ive Curvature
kg/ m3 MPa MPa.m3/kg MPa/K MPa/K2
10.00 .5741 .94390 .05429 .00152 -.0000004

20.00 1.0869 .89557 .04833 .00324 -.0000018
30.00 1.5419 .64507 .04271 .00517 -.0000048
40.00 1.9420 .79827 .03736 .00733 -.0000094
50.00 2.2902 .75312 .03233 .00970 -.0000161
60.00 2.5896 .70967 .02763 .01226 -.0000250
70.00 2.8440 .66804 .02331 .01501 -.0000365
80.00 3.0573 .62837 .01940 .01792 . -.0000510
90.00 3.2335 .59074 .01591 .02098 -.0000691
100.00 3.3768 .55523 .01283 .02415 -.0000918
1 10.00 3.4914 .52189 .01015 .02743 -.0001201
120.00 3.5812 .49069 .00786 .03078 -.0001560
130.00 3.6498 .46163 .00593 .03419 -.0002022
140.00 3.7009 .43465 .00433 .03763 -.0002635
150.00 3.7375 .40969 .00303 .04108 -.0003476
160.00 3.7625 .38665 .00201 .04451 -.0004680
170.00 3.7786 .36547 .00124 .04791 -.000651
180.00 3.7881 .34603 .00069 .05123 -.0009514
190.00 3.7930 .32825 .00033 .05445 -.0014992
200.00 3.7952 .31201 .00012 .05752 -.0026725
210.00 3.7959 .29721 .00003 .06036 -.0060057
220.00 3.7960 .28371 .00000 .06285 -.0251804
230.00 3.7960 .27137 .00000 .06455 .3759035
240.00 3.7960 .26007 .00001 .06684 .01 13369
250.00 . 3.7964 .24969 .00008 .06985 .0044633
260.00 3.7979 .24018 .00025 .07348 .0025343
270.00 3.8021 .23154 .00062 .07770 .0016947
280.00 3.81 12 .22381 .00127 .08253 .0012437
290.00 3.8287 .21708 .00230 .08798 .0009687
300.00 3.8590 .21 151 .00385 .09408 .0007860
310.00 3.9079 .20728 .00605 .10086 .0006567
320.00 3.9827 .20464 .00905 .10835 .0005603
330.00 4.0921 .20389 .01301 .1 1657 .0004855
340.00 4.2466 .20537 .0181 .12556 .0004251
350.00 4.4586 .20946 .02453 .13534 .0003748
360.00 4.7422 .21660 .03248 .14595 .0003317
370.00 5. 1138 .22726 .04215 .15742 .0002937
380.00 5.5918 .24196 .05378 . 16977 .0002593
390.00 6.1966 .26125 .06758 .18303 .0002277
400.00 6.9514 .28575 .08380 .19723 ,0001979
410.00 7.8816 .31608 .10269 .21240 .0001695
420.00 9.0151 .35293 .12452 .22857 .0001420
430.00 10.3827 .39702 .14957 .24576 .0001 151
440.00 12.0182 .4491 .17812 .26402 .0000886
450.00 13.9579 .51001 .21050 .28336 .0000621
460.00 16.2419 .58056 .24701 .30382 .0000357
470.00 18.9130 .66166 .28800 .32543 .0000091
480.00 22.0179 .75423 .3338: .34823 -.0000177
490.00 25.6068 .85927 .38485 .37223 -.0000449
500.00 29.7335 .97779 .44146 .39748 -.0000725
510.00 34.4560 1.1 1087 .50407 .42400 -.0001007
520.00 39.8362 1.25963 .57307 .45184 -.0001294
530.00 45.9401 1.42523 .64889 .48103 -.0001588
540.00 52.8381 1.60888 .73197 .51 161 -.0001890
550.00 60.6051 1.81 182 .82274 .54360 -.0002199
560.00 69.3201 2.03535 .92165 .57704 -.0002518
127
3
/ 0
2 . 3
7
5
1
Table 18. (Conti nued)
Norma i Butane Isotherm at 430 K

Dens ty i Pressure Z Der vat ve i i Der vat ve
i i Curvature
kg/m3 MPa MPa •mJ/kg MPa/K MPa/K^
10.00 .5814 .94521 .05507 .00152 -.0000003

20.00 1 025
. 1 .89623 .04922 .00323 -.0000017
30.00 1. 5668 .84910 .04369 .00515 -.0000044
40.00 1.9773 .80366 .03845 .00729 -.0000087
50.00 2.3369 .75984 .03351 .00962 -.0000147
60.00 2.6487 .71 769
AOO A
.02891 1 A O C
.01215 1 1
-. 0000226
70.00 2.9163 .67730 .02467 .01 484 -.0000325
AAAA X A C
80.00 3. 1434 .63880 .02083 .01 769 -.0000445
90.00 3.3342 .60229 A
.0
~7 A
/4U 1
1
>1
.0206 / A AAA CO A
-•0000589
100.00 3.4927 .56782 A ~7 1 >1 "Z AO T C
.02375 "Z A A A A C^T
-.0000755 ~7
1 0.00
1 3.5228 . 53544
All
.011/3 m A A
.02591 1 AAAAAyl O
-•0000948
120.00 3. 7285
CAC 1 7
.5051 A A A it
.00946 >1 AZA
.0301 1 Z AAA 161
-•000 £ 1
1
1 1
130.00 3.0 132 .4 /DO AA 1^/1

.00/54 "7
.03330 AAA jyz
-•uoo "ZAO1
1
140.00 3.8804 .45061 .00594 .03554 AAA £ A

-.0001530 1 "Z
.42628 AA A O C
-.0001854 1
1 50.00 3.9331 .00463 .03988 yl
160.00 3.9740 .40379 .00359 .04308 -. A AAOA C

0002035 "Z
1 70.00 4.0056 .38307 .00278 .04623 AAAO "20

-.0002132 1
180.00 4.0303 .36402 .00219 .04932 AAAO A T

-.0002103 1
AAA A ^
-.0001916 1 1
190.00 4.0500 .34654 .00178 .05238
A AA C A
-.0001 1 "7
200.00 4.0665 .33056 . 00 54 1 .05544 570
210.00 4.0813 .31 596 AA 144
.00 A A \ A C O CO
.05852 AAA AO
-•0001 0871 1
AAAA C AA
220.00 4.0956 .30266 .00144 .061 69 -.0000508
230.00 4. 1 103 .29053 .00 50 1 .06499 .0000139
240.00 4. 1257 .27947 .001 60 .06847 .0000832
250.00 4. 1426 .26939 .00180 .072 16 AAA 1544
.000 CA A ^
AAAOOO 1
260.00 4. 1623 .26027 .00217 .0761 .0002221
270.00 4. 1868 .25210 .00277 .08050 .0002802
280.00 4.2189 .24496 .00369 .08531 .0003238
290.00 4.2621 .23893 .00503 .09064 .0003508
300.00 4.3212 .23417 .00690 .09658 .0003620
310.00 4.4022 .23087 .00943 . 031 1 .0003605
320.00 4.5126 .22926 .01279 . 11047 .0003498
330.00 4.6612 .22964 .01712 . 11850 .0003331
340.00 4.8588 .23233 .02260 . 12732 .0003128
350.00 5.1177 .23771 .02942 . 13694 .0002905
360.00 5.4523 .24622 .03778 .14739 .0002672
370.00 5.8790 .25832 .04788 .15871 .0002435
380.00 6.41 63 .27451 .05994 . 17092 .0002198
390.00 7.0850 .29534 .074 19 . 18405 .0001960
400.00 7.9082 .32 142 .09087 .19812 .0001 723
AAA A Q C
1
4 0.00
1 8.91 15 .35336 . 1024
1 .21317 .0001485
AA A O A
1
420.00 10. 1229 .39184 .13257 .2292 .0001248 jl
430.00 .24629 AAA 1 AAA

1 . 5735
1 .43757 . 1581 .0001 009
A A A AT£ O
440.00 13.2970 .491 31 .18719 .26442 .0000768
.28364 A AAA CO A
.0000524
45U.UU 13.3301 .2201
"Z A "ÔQ AAAAo-7-7
460.00 17.7128 .62601 ml.0 1 lb .3U3yo
470.00 20.4882 .70869 .29871 .32546 .0000026
480.00 23.7031 .80282 .34511 .34813 -.0000229
490.00 27.4078 .90935 .39673 .37200 -.0000490
500.00 31.6564 1.02931 .45396 .39712 -.0000756
510.00 36.5070 1.16375 , .51719 .42351 -.0001028
520.00 42.0216 1.31378 .58683 .45121 -.0001307
530.00 48.2664 1.48055 .66331 .48026 -.0001593
540.00 55.3121 1.66525 .74707 .51069 -.0001887
550.00 63.2335 1.86912 .83854 .54253 -.0002190
128
J
15
/1 J1 1 1 . 4
Table 18. ( Cont nuedi )
1sotherm 1 sochore sochore

1
r\ y-\ r\
Uwii b
i
1 1
y Pressure L Der vat ve
i i Der vat ve i i Curvature
kg/ tTi3 rlr a MPa .rfi3/kg MPa/K fMPa/K^
Z'J •uu .yU A^

OA 145 \
,05 02
1 .00321 -,0000015
A n nn
4U» UU O QQ
A/1 O1 o .1 1
•o 1 4 y 1 .04067 ,00721 -,0000075
O A
"7£:
/oy 1
z. .73326 .03148 .01 194 -,0000187
on An
J . 3 0.5 1 .6530 .02369 .01 730 -,0000351
1 nn nn Z T OC O
3 . / ZOO .5921 .01742 ,02310 -,0000554
I zU.UU 4 . 0248 .53288 .01 262 ,02919 -,0000769
1 ^ r\ rvA
1 4U»U(J 4.2401 .481 19 ,00912 ,03542 -,0000943
1nn f^n A "ZA TA
4. jy /U .43662 ,00674 ,04 168 -,0001009
ion nn A
4.5 CA
loU 1
.39861 ,00532 .04800 -,0000908
OA A AA 4.61 54 .36665 ,00475 ,05449 -.0000628
oon nn A
4
"7 AO
08 1
,34021
. / 1 ,00488 ,06139 -,0000207
240.00 4.8132 .31863 .00542 ,06895 ,0000307
A AA 4 . 93 1 .30135 .00656 ,07748 ,0000870
5.0836 ,26346 ,00891 ,08736 ,0001399
A AA
jUU.OU 5.3009 ,28073 .01321 ,09907 ,0001797
TOO AA 5.o3 1!) .27960 .02043 , 308
1 1 .0002001
340.00 6.1453 .28717 ,03175 .12981 .0002014
7/r
JOU AA
A . UU C A*Z O A
6.9380 .30620 ,04857 . 14963 .0001876
380.00 8.1355 .34015 .07250 .17281 ,0001633
400.00 9.8973 .39312 ,10532 . 19963 .0001 320
420.00 12.4208 .46986 .14901 .23031 .0000959
1 A
44U
>1 AA
. UU 5 .y44 .57575 ,20575
1
.26508 .0000561
A Â AA
'ôu.uu ZUt 1051 .7 1681 ,27794 .30418 .0000132
/lOA AA Q A A~7
ôu • UU .syy /6 ,36825 .34785 -.0000326
KAA AA
3UU.UU 1 1 "2 1 AO
1 . 1 3 198 ,47958 .39633 -,0000813
KOA AA
J^\J • UU AA RO 7 1 1 >10 c:q
,4z 1
1 5o 1 ,61 506 .44990 -,0001331
A AA fÂ ^ AQA
Du.4uyo 1 "7~7"7'20
1 , / / /3o ,77805 .50881 -,0001882
Norma 1 [Butane 1 sotherm at 450 K

ACOO
,U5zol 1
.00320 -.0000014
dn . UU
nn Z. 9
9 IZ 1 QO jy
,oz
"2
,04284
1
1 1} ,0071 -.0000065
OU. nn
ftn UU Z.OC) /O » I'i loo ,03398 ,01 177 -,0000158
Rn
OU . nn
UU _>.4oyo »o 1 / 1)3 .02645 ,01698 -.0000287
1 AA
uu.uu AA A A c
,Ol445
IZ ^
1
,02036 ,02261 -.0000435
1 OA
Z AA
U . UU 4. J J
1 1 ,55839 .01 566 .02853 -.0000574
A AA
'JU.UU
1 >1 >l C: AA 1
'
,50934
1
.01222 .03463 -.0000670
fÂ AA
DU .UU A O AA A
1
1 4.0094 ,46696 .00988 ,04086 -.0000685
1 Q A AA
ou.uu A A AO
4.yyzi 1
1 ,43084 .00855 ,04727 -.0000599
OA A AA
/UU.UU 5. 15/6 ,40062 ,00816 ,05399 -.0000412
OO
ZZU.A AAUU 5.3238 ,37593 ,00857 ,06122 -.0000145
O ^ A AA
5.5040 ,35627 ,00953 ,06919 .0000180
OC A A A
/:o0.00 5.7100 ,341 17 ,01 125 ,07816 .0000539
^80 . 00 5.9633 .33085 ,01437 ,08847 .0000892
300.00 6.2994 .32620 ,01967 .10052 .0001 188
320.00 6.771 .32871 ,0281 .11473 .0001382
XAr\ AA
u.uu A ROA
1 .4DZ4
~I "Z AC 1
,34051 /I
.04085 . 1 3 52 1 .0001454
360.00 8,4428 .36433 .05926 .15125 .0001406
380.00 9.8711 .40354 ,08492 .17425 .0001256
400.00 1 1.8997 .46215 .1 1960 .20080 .0001026
420.00 14.7283 .54477 ,16527 .23115 .0000734
440.00 18.5980 .65663 .22410 .26555 .0000393
460.00 23.7959 .80363 .29851 .30425 .0000010
480.00 30.6598 ,99229 .391 15 .34748 -.0000409
500.00 39.5829 1,22984 .50494 .39549 -.0000863
520.00 51 .0194 1.52420 .64303 .44855 -.0001351
540.00 65.4883 1,88399 ,80875 ,50693 -.0001876
129
11
sotherm
i 1sochore 1sochore
Dens ty i Pressure Z Derivative Der vat ve
i i Curvature
kg/ni3 MPa MPa.m3/kg MPa/K MPa/K^
20.00 1.3253 .92648 .06157 .00315 -.0000008

40.00 2.4716 .86392 .05323 .00689 -.0000036
60.00 3.4603 .80634 .04580 .01 120 -.0000082
80.00 4.3107 ,75338 .03943 .01599 -.0000138
100.00 5.0452 .70539 .03422 .021 18 -.0000194
120.00 5.6878 .66269 .03023 .02671 -.0000239
140.00 6.2624 .62541 .02743 .03258 -.0000264
160.00 6.7931 .59360 .02583 .0388 -.0000261
180.00 7.3040 .56734 .02548 .04549 -.0000230
200.00 7.8210 .54675 .02645 .05273 -.00001 72
220.00 8.3704 .53195 .02869 .06069 -.0000091
240.00 8.9754 .52287 .03199 .05954 .0000007
260.00 9.6594 .51943 .03669 .07949 .00001 15
280.00 10.4575 .52218 .04355 .09078 .0000224
300.00 11.4216 .53230 .05344 .10370 .0000323
320.00 12.6222 .55149 .06738 .11854 .0000397
340.00 14.1514 .58193 .08651 .13564 .0000435
360.00 16.1263 .62630 .11219 .15531 .0000428
380.00 18.6924 .68775 ,14590 .17789 .0000369
400.00 22.0272 .76993 .18936 .20368 .0000256
420.00 26.3446 .87699 .24449 .23298 .0000092
440.00 31 .8990 1.01362 .31344 .26606 -.0000121
460.00 38.9903 1.18509 .39861 .30320 -.0000380
480.00 47.9691 1.39724 .50265 .34467 -.0000683
500.00 59.2416 1.65656 .62849 .39072 -.0001027
Normal 1Butane Isotherm at 550 K
20.00 1.4817 .94166 .07009 .0031 -.0000005

40.00 2.8124 .89368 .06312 .00675 -.0000023
60.00 4.0117 .84983 .05693 .01088 -.0000050
80.00 5.0956 .80959 .05162 .01545 -.0000083
100.00 6.0837 .77327 ,04738 .02043 -.00001 15
120.00 6.9985 .74128 ,04430 .02580 -.0000140
140.00 7.8641 .71397 ,04247 .03157 -.0000155
160.00 8 . 7064 .69 641 .04200 .03781 -.00001 57
180.00 9.5541 .67465 .04303 .04458 -.0000146
200.00 10.4386 .66340 .04571 .05202 -.0000122
220.00 1 .3935
1 ,65826 .05005 .06024 -.0000088
240.00 12.4505 .65938 .05590 .06942 -.0000047
260.00 13.6422 .66692 .06367 .07973 -.000000''
280.00
JL~\J\J 9 \J\J 15.01 54 .68161 .07419 ,09138 .0000042
300.00 16.6345 .70477 .08842 . 10462 .0000079
320.00 18.5839 .73815 .10742 .1 1969 .0000103
340.00 20.9709 .78397 .13238 .13687 .0000105
360.00 23.9279 .84481 .16465 .15647 .0000081
380.00 27.6158 .92370 .20574 .17876 .0000025
400.00 32.2273 1.02405 .25731 .20406 -.0000067
420.00 37.9908 1.14971 .32128 .23263 -.0000197
440.00 45.1750 1.30498 .39975 .26478 -.0000364
460.00 54.0936 1.49467 '
.49513 .30077 -.0000571
480.00 65.1105 1.72412 .61006 .34088 -.0000815
130
0
2
5
1 51 A
1
1
sotherm
1 1sochore 1sochore
1 i Der va t ve
i i Curvature
kg/tn-> MPa MPa •nrP/kg MPa/K MPa/K^
20.00 1 .6368 ,95353 .07847 ,00309 -.0000004

40.00 3. 1474 .91677 .07272 ,00665 -.0000016
60.00 4.5501 .88356 .06766 .01067 -.0000034
80.00 5.8591 .85332 .06340 .0151 -.0000055
100.00 7.0927 .82639 ,0601 .0 1996 -.0000077
120.00 8.2731 .80326 ,0581 .02522 -.0000095
140.00 9.4258 .78444 ,05740 .03093 -.0000107
160.00 10. 5795 .77040 ,05824 .037 1 -.00001 12
180.00 1 .7669
1 .76165 .06082 .04395 -.00001 10
200.00 13.0252 .75880 ,06535 .05145 -.00001 02
220.00 14.3945 .76234 .07191 .05980 -.0000089
240.00 15.9143 .77259 ,08039 .0691 1 -.00000 72
260.00 17.6259 .78985 ,09124 .07957 -.0000055
280.00 19. 5858 .81499 ,10538 .09136 -.0000041
300.00 21.8697 .84936 ,12381 .10470 -.0000032
320.00 24.5744 .89475 ,14755 .11982 -.0000034
340.00 27.8202 .95335 ,17814 .13697 -.0000050
360 . 00 31 .7535 1 .OZ /DO ,Z 1553 .
1
554
1
CiC A 1 AAA A AO C
A A A A 44
-.00001 A A
^
380.00 36.5489 1 . 2063
1 ,26455 . /84z
1
400.00 42.4138 1 .23543 ,32387 .20327 -. AA A AOO

0000229
4y.5yuo 1 .3 /5oy ,39010 0"Z 1 OA nAAAT/l J
- .UUOUjA "Z
440.00 58.3624 1 . >4 344 .4837 .z5/:5 1 -.000048 /

.74910 CO O O -.0000553
460.00 59.0562 1 .58881 1
.zy /55
Norma 1 Butane 1 soTnerm ax 650 K

A A A A A A "I
20.00 .7909
1 .96307 .08674 .00307 -.0000003
A/\ A A 1
40.00 3.4784 .93524 .082 1 .00559 -. /^
000001 1
60.00 5.0798 .91055 .07813 .01053 -.0000025

80.00 6.6084 .88842 ,07489 .01487 -.0000040
100.00 8.0821 .86923 ,07257 .01953 -.0000055
120.00 9,5236 .85355 ,071 71 .02482 -.0000070
140.00 10.9604 .84199 ,07223 .03047 -.0000081
160.00 12.4241 .83513 ,07446 .03656 -.0000087
180.00 13.9519 .83362 ,07868 .04345 -.0000091
200.00 15.5862 .83814 ,08515 .05099 -.000009
220.00 17.3735 .84933 ,09398 .05936 -.0000089
240.00 19.3603 .85758 ,10510 .06871 -.0000086
260.00 21.5961 .89333 ,1 1903 .07922 -.0000084
280.00 24, 1467 .92749 .13674 .09104 -.0000084
300.00 27,0980 .97145 ,15928 .10438 -.0000091
320.00 30.5577 1.02702 ,18780 .11945 -.0000106
340.00 34.6584 1.09632 ,22359 .13649 -.0000133
360.00 39,5589 1.18182 ,26803 .15574 -.0000174
380.00 45.4475 1.28528 ,32266 .17745 -.0000234
400.00 52.5446 1.41278 ,38918 .20189 -.0000315
420.00 6 1 . 1 064 1.55475 .46947 .22932 -.0000419
440.00 71 ,4292 1,74595 .56555 .25001 -.0000548
131

i 1 Der vat ve
i i Curvature
kg/m3 MPa MPa •m3/kg MPa/K MPa/K2
20.00 1.9444 .97089 .09495 .00306 -.0000002

40.00 3.8064 .95035 .09138 .00654 -.0000009
60.00 5.6032 .93264 .08840 .01042 -.0000019
80.00 7.3475 .91723 .08618 .01470 -.0000031
100.00 9.0573 .90453 .08500 .01939 -.0000043
120.00 10.7565 .89518 .08516 .02451 -.0000055
140.00 12.4746 .88986 .08694 .03011 -.0000065
160.00 14.2467 .88924 .09062 .03626 -.0000073
180.00 16.1141 .89404 .09652 .04304 -.0000079
200.00 18.1245 .90502 .10496 .05055 -.0000083
220.00 20.3304 .92288 . 1 1608 .05892 -.0000087
240.00 22.7850 .94812 .12985 .06827 -.0000092
260.00 25.5458 .98123 .14684 .07876 -.0000098
280.00 28.6870 1.02318 .16807 .09055 -.0000108
300.00 32.3040 1.07537 .19462 .10384 -.0000123
320.00 36.5153 1.13959 .22770 .1 1882 -.0000145
340.00 41.4642 1.21792 .26862 .13570 -.0000178
360.00 47.3217 1.31275 .31880 .15473 -.0000223
380.00 54.2884 1.42675 .37981 .17615 -.0000282
400.00 .
62.5974 1.56286 .45334 .20019 -.0000360
132
1
Table 19. The Joule-Thomson Inversion locus for normal butane.
Temp. Den si ty Pressure

K kg/m3 MPa
350 51 1.2 2.707

360 505.9 5.584
370 500.6 7.91 1
380 495.4 10.297

390 490.2 12.551
400 485.0 14.680
410 479.9 16.693
420 474.7 18.595
430 469.7 20.394
440 464.7 22.095
450 459.7 23.703
460 454.8 25.224
470 449.9 26.661
480 445.0 28.020
490 440.2 29.304
500 435.5 30.517
510 430.8 31.662
520 426. 32.743
530 421.5 33.762
540 416.9 34.723
550 412.3 35.627
560 407.8 36.477
570 403.4 37.275
580 398.9 38.025
590 394.5 38.726
600 390.2 39.381
610 385.8 39.991
620 381 .5 40.560
630 377.3 41 .087
640 373.0 41 .575
650 368.8 42.024
660 364.6 42.436
670 360.5 42.812
680 356.4 43.154
690 352.3 43.462
700 348.2 43.738
710 344.1 43.981
720 340.1 44.196
730 336.1 44.380
740 332.1 44.537
750 328.1 44.666
760 324.1 44.768
770 320.2 44.845
780 316.3 44.898
790 312.4 44.927
800 308.5 44.934
810 304.6 44.919
820 300.8 44.884
830 297.0 44.828
840 293.2 44.754
850 289.4 44.662
860 285.6 44.553
133
• 111 U/ 7 .. 7D
J1
1 . U
4
1 y 111
111
Tab e 20.
1 Thermophys ca i 1 properties of saturated 1 iquid normal I butane.
1 sochore sotherm
1
Temp. Pil dPa/dT dPJt/dT Der vat ve

i i Der vat ve i i
, y
K MPa kg/fTP kg/m3 kg/(nfi3.K) MPa/l< MPa.m3/kg
1
1
"^4 Rfin
JH • oou . fi7'^SftF-nft
D / -J JO C UO 7^5 77 .34916E-04 .00000 1 .00000 . 1282E--06 - 044 1 9.
z 1
1
1
1
n
u 1
1
99'^RF-»/1
1 hU«UUU . /z nF-nR
77
1
1uc— uj? 1
1 1S)\J»H^ .85937E-04 .00000 .99999 .3012E--06 — Q4 94 9 n"^9R
Z .UjZ9 . Z R7P4.n
9 1 -) / c +U
1
1
1
1 4 D . uuu zQQ 7P_nR

. Jyy / ll~UI?
1
1
77 R 77
/ Z -J . / Z . 1924 5E-03 .00000 .99998 .6456E--06 — . 04
y4 nu 1
1 1 » 70 J J . ZU04 t+U
1 Rn nnn .
pcQ/i zp_nRJ
ouy^ jtiû 77
/ Z
1 n1
. U1 1 .40521E-03 .00000 .99997 .1303E.-05 — . Q4n
~ y4u 1 1
1
RQ99
.oyzz 9n jL+U
•ZU XP-t-H 1
1
1
1 R s uuu
\DD nfin 1 7SQ7P-n4 7/ 1 D . J?
1
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134
1 0
Table 20. ( Cont i iiue'l)
Heat of Internal Fugacity/ Vel. of

Temp. Vap. Energy Enthalpy Entropy Cy Cg Cp Pressure Sound Di el ectr ic
K J /mo I J /mo
I J /mo
I J/(mol.K) J/(mol.| J/(mol .K) J/(mol .K) Ratio m/s Constant
134.860 28789.2 .0 .0 133.544 88.51 1 17 . 39 1 7 . 39
1 1 .00000 1721 2.03857
140.000 28520.6 602.8 602.8 137.932 87.86 1 17.07 117.07 1 .00000 1695 2.03023
145.000 28265.6 1187.8 1187.8 142.036 87.29 1 16.82 116.82 1 .00000 1669 2.02212
150.000 28016.2 1771.6 1771.6 145.992 86.78 1 16.61 116.61 1 .00000 1644 2.01402
155.000 27772.2 2354.7 2354.7 149.812 86.34 1
'6.48 116.48 .99998 1519 2.00592
160.000 27532.9 2937.3 2937.3 153.507 85.99 .42 116.42 .99994 1594 1.99783
165.000 27298.0 3519.8 3519.8 157.089 85.71 1 10.44 116.44 .99986 1569 1.98975
170.000 27067.1 4102.5 4102.5 160.565 85.51 1 16.54 116.54 .99975 1544 1.98167
nS.OOO 26839.7 4686.0 4686.0 163.945 85.40 1 16.72 115.72 .99959 1520 1.97359
180.000 26615.3 5270.5 5270.5 167.237 85.37 1 16.99 116.99 .99935 1495 1 .96551
185.000 26393.4 5856.5 5856.5 170.447 85.42 1 17.34 117.34 .99902 1470 1 .95742
190.000 26173.7 6444.4 6444,5 173.582 85.56 1 17.77 117.77 .99858 1445 1.94932
195.000 25955.7 7034.6 7034.8 176.549 85.77 118.28 118.28 .99799 1420 1.94122
200.000 25738.9 7627.6 7627.7 179.652 86.05 1 18.88 118.88 .99722 1 395 1.93310
205.000 25522.8 8223.6 8223.9 182.596 86.41 119.54 119.55 .99636 1359 1.92496
210.000 25307.0 8823.1 8823.4 185.486 86.84 120.29 120.29 .99521 1344 1.91680
215.000 25091.1 9426.5 9427.0 188.326 87.33 121.10 121.11 .99392 1319 1.90862
220.000 24874.5 10033.9 10034.6 191.120 87.88 121.98 121 .99 .99228 1294 1.90041
225.000 24656.8 10646.0 10646.9 193.872 88.48 122.92 122.94 .99045 1268 1.89216
230.000 24437.6 11262.7 11264.0 196.584 89.13 123.92 123.95 .98826 1 243 1.88388
235.000 24216.2 11884.7 11886.4 199.260 89.84 124.98 125.02 .98581 1218 1.87556
240.000 23992.3 12512.1 12514.3 201.902 90.58 126.10 126.14 .98298 1 921 1.85719
245.000 23765.3 13145.3 13148.1 204.513 91.37 127.26 127.32 .9 /yo5 115/ 1.85877
250.000 23534.8 13784.4 13788.0 207.096 92.19 128.48 128.55 .y / 034 114
1 1 >i 1
1 1.85030
1 £
255.000 23300.2 14429.8 14434.4 209.652 93.05 129.74 129.83 .9 1.14 /
1
1
1
1 16 1.84177
260.000 23061.1 15081.7 15087.5 212.183 93.93 131.05 131.16 1uyu 1.83315
nc: T co
265.000 22816.8 15740.5 15747.6 214.692 94.85 132.40 132.53 1065 1.82449
270.000 22566.9 16406.1 16415.0 217.180 95.78 133.79 133.96 .y5o /2 1039 1.81574
272.638 22432.6 16760.3 16770.1 218.485 96.29 134.54 134.73 .95595 1026 1 .81 106
280.000 22047.9 17759.4 17772.4 222.098 97.73 135.70 136.95 .94773 988 1.79796
285.000 21777.7 18447.2 18462.9 224.532 98.73 138.22 138.51 .94 165 962 1.78893
290.000 21499.5 19142.8 19161.5 226.950 99.75 139.78 140.13 .93523 936 1.77978
295.000 21212.8 19846.3 19868.5 229.353 100.78 141 .38 141 .80 .92843 9 1 1.77052
300.000 20916.9 20557.9 20584.2 231.744 101.83 143.02 143.53 .92130 834 1 .761 13
305.000 20611.0 21277.7 21308.6 234.122 102.89 144.71 145.31 .91379 858 1.75160
310.000 20294.4 22005.9 22042.0 236.490 103.95 146.44 147.15 .90593 832 1.74192
315.000 19966.5 22742.6 22784.6 238.847 105.04 148.22 149.06 .89772 805 1.73208
320.000 19626.4 23488.1 23536.8 241.196 106.13 150.05 151.04 .88919 780 1.72206
325.000 19273.1 24242.7 24298.8 243.536 107.22 151 .94 153. 10 .88035 754 1 .71 184
330.000 18905.8 25006.4 25070.9 245.870 108.31 153.88 155.24 .87120 727 1.70142
335.000 18523.4 25779.6 25853.6 248.198 109.40 155.87 157.48 .851 75 700 1.69076
340.000 18124.8 26562.7 26647.1 250.521 110.48 157.94 159.83 .85204 574 1.67986
345.000 17708.7 27356.0 27452.0 252.842 111.55 150.08 162.31 .84207 547 1.66867
350.000 17273.6 28159.9 28268.8 255.160 112.60 152.29 154.92 .83 187 519 1.65717
355.000 16817.9 28975.0 29098.2 257.478 113.62 164.61 167.71 .82147 592 1.54533
360.000 16339.6 29801.5 29940.7 259.797 114.62 167.03 170.71 .81085 564 1.63310
365.000 15836.5 30640.3 30797.2 262.119 115.57 159.58 173.97 .80007 536 1.62044
370.000 15305.8 31491.9 31668.4 264.446 115.46 172.29 177.56 .7891 508 1.60727
375.000 14744.1 32357.3 32555.6 266.779 117.30 175.21 181 .58 .77799 479 1.59353
380.000 14147.3 33237.3 33460.0 269.122 118.05 178.40 186.17 .75672 450 1.57912
385.000 13509.7 34133.4 34383.3 271.479 118.70 181 .96 191.57 .75532 420 1.56392
390.000 12824.0 35047.2 35327.6 273.854 119.23 186.05 198.14 .74375 389 1.54774
395.000 12079.8 35981.2 36296.3 275.254 119.60 190.91 206.50 .73200 358 1.53036
400.000 11262.1 36939.3 37293.9 278.689 119.75 196.99 217.75 .72005 325 1.51143
405.000 10346.6 37927.9 38328.4 281.178 119.57 205. 10 234.17 .70785 292 1,49041
410.000 9291.7 38959.2 39414.3 283.753 118.84 217.06 261.09 .69533 257 1.45636
415.000 8012.0 40060.4 40583.6 286.487 116.84 237.72 314.81 .63240 219 1.43739
420.000 6273.2 41315.5 41932.6 289.504 110.53 287.81 479.31 .66883 181 1.39841
425.160 0.0 44431.5 45399.9 297.647 .65361 0 1.26583
135
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192
NBS-n4A IREV. 2-8C)
U.S. DEPT. OF COMM. 1. PUBLiCATION OR 2. Performing Organ. Report No, 3. PubM cation D ate
REPORT NO.
BIBLIOGRAPHIC DATA
NBS Monogr. 169 April 1982
SHEET (See instructions)
4. TITLE AND SUBTITLE
THERMO PHYSICAL PROPERTIES OF NORMAL BUTANE FROM 135 TO 700 K AT

PRESSURES TO 70 MPa
5. AUTHOR(S)
6. PERFORMING ORGANIZATION (If joint or other than NBS. see instructions) 7. Contract/Grant No.
NATIONAL BUREAU OF STANDARDS

DEPARTMENT OF COMMERCE 8. Type of Report & Period Covered
WASHINGTON, D.C. 20234
Final
9. SPONSORING ORGANIZATION NAME AND COMPLETE ADDRESS (Street. City. State. ZIP)
Same as No. 6
10. SUPPLEMENTARY NOTES
Library of Congress Catalog Card Number: 82-600512
Document describes a computer program; SF-185, FlPS Software Summary, is attached.

11. ABSTRACT (A 200-word or less factual summary of most si gnifi cant information. If document includes a si gnificant
bi bliography or literature survey, mention it here)
Using a modified version of the nonanalytic equation of state, thermophysical

properties of normal butane are derived from physical properties data and are
tabulated at integral temperatures from 135 to 700 K along isobars at pressures to
70 MPa. These isobar tables, along with a table for the saturated liquid, give
values for densities, compressibility factors, internal energies, enthalpies,
entropies, heat capacities, fugacities, sound velocities, dielectric constants, and
isochore and isotherm derivatives. Equations, whose coefficients are determined from
a least squares fit to selected experimental data, are also presented for vapor
pressures, orthobaric liquid and vapor densities, ideal gas properties, second virial
coefficients, dielectric constants, heats of vaporization, melting pressures, and
orthobaric liquid specific heats, enthalpies, and entropies. Comparisons between
experimental and calculated values for all properties considered here are reported in
detail.
12. KEY WORDS (Six to twelve entries; alphabetical order; capjtalize only proper names; and separate key words by semicolon s)
Densities; dielectric constants; enthalpies; entropies; equation of state;
fugacities; internal energies; isobars; isochores; isotherms; Joule-Thomson
inversion; latent heats of vaporization; melting line; normal butane; orthobaric
dens-it ies; spe r.ifir heats; vapor pressure.g; vel or.-j ti es nf snnnd.
13. AVAILABILITY 14. NO. OF
PRINTED PAGES
Unlimited
I I
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Thermophysical Properties of Normal Butane

from 135 to 700 K at Pressures to 70 MPa

William M. Haynes and Robert D. Goodwin

Thermophysical Properties Division

U.S. DEPARTMENT OF COMMERCE, Malcolm Baldrige, Secretary

Issued April 1982

National Bureau of Standards Monograph 169

U.S. GOVERNMENT PRINTING OFFICE

2. Physical Properties and Their Formulation 2

2.1 Fixed-Point Values 2

2.2 Melting Line and Vapor Pressures 3

2.3 The Orthobaric Densities 4

2.4 The Virial Equation 5

2.5 The Equation of State 6

2.6 The Ideal Gas Functions 8

2.7 Thermal Loop Computations 8

2.8 The Heats of Vaporization 9

2.9 Saturated Liquid Enthalpies and Entropies 9

2.10 Dielectric Constants 10

3.1 The Homogeneous Domain 11

3.2 The Saturated Liquid 12

3.3 The Compressed Liquid 13

3.4 Fugacity Coefficients 13

3.5 Simplified Computation 13

4. Tests and Conclusions 13

5. Tables of Physical and Thermodynamic Properties 14

5.1 Calculated P-p-T Isochores and Isotherms 14

5.2 The Joule-Thomson Inversion Locus 14

5.3 Thermophysical Properties of the Saturated Liquid ..... 15

5.4 Thermophysical Properties Along Selected Isobars 15

APPENDIX A. Symbols and Units 23

APPENDIX B. Conversion of Units 25

APPENDIX C. Fixed-Point Values for Normal Butane 26

APPENDIX D. Normal Butane Properties Reference Index 27

APPENDIX E. Computer Program 30

Figure 2. P-T locus of P-p-T data for normal butane 50

Table 1. Comparisons of vapor pressure data with eq (2) 51

Table 2. Comparisons of saturated liquid density data with eq (3) . . 54

Table 3. Comparisons of saturated vapor density data with eq (4) . . 57

Table 4. Comparisons of second virial coefficients with eq (5). . . . 59

Table 5. Behavior of coefficients of equation of state for

Table 7. Comparisons of experimental P-p-T data of normal butane

Table 8. Comparisons of data for ideal gas functions with eq (7). . . 85

Table 10. Comparisons of heat of vaporization data with eq (9) , . . . 87

Table 12. Entropies and specific heats of saturated liquid normal

Table 14. Comparisons with saturated liquid specific heats 95

Table 15. Comparisons with C and C data 96

Table 17. Calculated P(T) isochores of normal butane 98

Using a modified version of the nonanalytic equation of state,

Key words: Densities; dielectric constants; enthalpies; entropies;

300 K at pressures to 35 MPa. As a result of new dielectric constant measure-

modified from earlier versions [26-29], is also currently being employed in

et al . [21]. Many new properties data, especially at low temperatures, have

collection of references for the major physical properties of normal butane,

2. Physical Properties and Their Formulation

state originates on a given liquid-vapor coexistence boundary, the P(T) melting

2.1 Fixed-Point Values

2.2 Melting Line and Vapor Pressures

is obtained, where P^ = 6.7358 x lO"'' MPa, T^ = 134.86 K, P^ = 363.4 MPa, and

et al . [1] from the triple- to the normal boiling-point; the heat of

thermofunctions formulated in section 2.6; the virial equation formulated in

are given by the relation.

where e = 1.85 and, from least squares analysis,

a = - 9.5092 4729 d = 4.8614 7936

f(T) E 1 + a'u^ + b'u + cexp[n(l - 1/u)] ,

P - P^(p) = p^-R-[T - T^(p)] + p^RT^-F(p.T) , (6)