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Progress in Nuclear Energy 82 (2015) 64e68

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Progress in Nuclear Energy


journal homepage: www.elsevier.com/locate/pnucene

Design of J-PARC Transmutation Experimental Facility


Toshinobu Sasa*
Transmutation Section, J-PARC Center, Japan Atomic Energy Agency, 2-4, Shirakata-Shirane, Tokai-mura, Ibaraki 319-1195, Japan

a r t i c l e i n f o a b s t r a c t

Article history: After the Fukushima accident, nuclear transmutation got much interested as an effective option of nu-
Received 12 November 2013 clear waste management. Japan Atomic Energy Agency (JAEA) proposes the transmutation of minor
Received in revised form actinides by accelerator-driven system (ADS) using leadebismuth eutectic alloy (PbeBi) as a spallation
27 June 2014
target and a coolant of subcritical core. Current design of ADS has 800 MWth of rated power, which is
Accepted 24 July 2014
driven by 20 MW proton LINAC, to transmute minor actinides generated from 10 units of standard Light
Available online 10 September 2014
Water Reactors. To obtain the data required for ADS design, JAEA plans to build a Transmutation
Experimental Facility (TEF) in J-PARC. TEF consists of two buildings, one is an ADS target test facility (TEF-
Keywords:
Transmutation
T), which will be installed PbeBi spallation target, and the other is Transmutation Physics Experimental
Accelerator-driven system Facility (TEF-P), which set up a fast critical/subcritical assembly. TEF will be located at the end of 400 MeV
J-PARC LINAC of J-PARC and accepts 250 kW proton beam. The paper describes an outline of TEF and design of
Transmutation Experimental Facility spallation target.
Spallation target © 2014 Elsevier Ltd. All rights reserved.

1. Introduction facilities are connected by proton beam line with low power beam
extraction mechanism using laser beam. TEF-P is a facility with
After the Fukushima accident, the interest to the management of zero-power critical assembly where a low power proton beam is
radioactive wastes and spent nuclear fuels is increased. The Atomic available to study the reactor physics and the controllability of ADS.
Energy Commission of Japan requests a review of current selection It also has an availability to measure the reaction cross sections of
process of waste disposal site to the Science Council of Japan. The MA, structural materials and so on. TEF-T is planned as an irradi-
Council suggests to enhance activities for research and de- ation test facility which can accept a maximum 400 MeV-250 kW
velopments to reduce the radiological burden of high level wastes proton beam into the leadebismuth eutectic alloy (LBE) spallation
by transmutation technology. target. Using these two facilities, basic physical properties of
Japan Atomic Energy Agency (JAEA) precedes R&Ds to reduce subcritical system and engineering tests of spallation target will be
the radiological hazard of high level wastes by Partitioning and studied.
Transmutation technology (Sasa et al., 2004). In the framework of
the J-PARC project (The Joint Project Team of JAERI and KEK, 2000), 2. Outline of Transmutation Experimental Facility
JAEA also promoted to construct the Transmutation Experimental
Facility (TEF) to study the minor actinide (MA) transmutation by 2.1. Outline of TEF-P
not only the accelerator-driven systems (ADS) but also the fast re-
actors. TEF locates at the end of LINAC of J-PARC, which is also Several neutronic experiments for ADS have been performed in
important components to be developed for future ADS, and share both Europe (Soule et al., 2004; Uyttenhove et al., 2011) and Japan.
the proton beam with other experimental facilities used for mate- In Japanese case, subcritical experiments were performed at the
rial science, life science and high energy nuclear physics. Fast Critical Assembly (FCA) in JAEA/Tokai with a 252Cf neutron
TEF, which illustrated in Fig. 1, consists of two buildings; source and a DT neutron source. Subcritical experiments with
Transmutation Physics Experimental Facility (TEF-P) (Oigawa et al., thermal subcritical core driven by 100 MeV protons are performed
2001) and ADS Target Test Facility (TEF-T) (Sasa et al., 2005). Two at Kyoto University Research Reactor Institute. Many experimental
studies also have been performed to the neutronics of the spallation
neutron source with various target materials such as lead, tungsten,
* Tel.: þ81 29 282 6948; fax: þ81 29 282 5671. mercury and uranium. These experiments for spallation target are
E-mail address: sasa.toshinobu@jaea.go.jp. also useful to validate the neutronic characteristics of ADS.

http://dx.doi.org/10.1016/j.pnucene.2014.07.031
0149-1970/© 2014 Elsevier Ltd. All rights reserved.
T. Sasa / Progress in Nuclear Energy 82 (2015) 64e68 65

Fig. 2. Prototype design of TEF-T spallation target.

Fig. 1. Transmutation Experimental Facility. neutrons is discussed within a user community of TEF-T. Various
research purpose using spallation neutrons, such as nuclear physics
using ISOL or ultra cold neutron, medical application and engi-
There have been, however, no subcritical experiments combined neering tests of semiconductor, are proposed. A floor plan to accept
with a spallation source installed inside the subcritical fast-neutron proposals as much as possible is underway.
core. The purpose of the TEF-P is divided roughly into three sub-
jects; (1) Reactor physics aspects of the subcritical core driven by a 3. Design of spallation target for TEF-T
spallation source, (2) Demonstration of the controllability of the
subcritical core including a power control by the proton beam 3.1. Proton beam profile
power adjustment, and (3) Investigation of the transmutation
performance of the subcritical core using certain amount of MA and The condition of the proton beam profile is Gaussian profile that
LLFP. Following section describes the detail of these experimental originally determined by proton LINAC. Four types of beam profile
items. are considered for the analysis as summarized in Table 1. The heat
Because we already have experiences and experimental data at power density distributions in the beam window was analyzed by
existing facility FCA, TEF-P is designed with referring to FCA, a PHITS code (Niita et al., 2010) with different beam profiles and
critical assembly for fast reactor systems with layered structure of summarized in Fig. 3. The Gaussian beam profile of case 1 was set to
rectangular lattice matrix. In this concept, the plate-type fuel for the reference case in the JAEA's beam window studies (Sugawara
FCA with various simulation materials such as lead and sodium for et al., 2008).
coolant, tungsten for solid target, ZrH for moderator, B4C for
absorber, and AlN for simulating nitride fuel, can be commonly 3.1.1. Analysis method and conditions
used at TEF-P. Therefore, the correlation of previous experiments To establish the spallation target for TEF-T, the temperature
can be kept with TEF-P experiments. The proton beam will be profile of structural materials and LBE and the thermal stress in the
introduced horizontally at the center of the assembly and various beam window were calculated by the thermal-fluid analysis and
kinds of spallation targets can be installed at various axial position structural analysis. Using these analyses, operative condition of
of the radial center of the subcritical core. TEF-T target system is determined.
Installation of a partial mock-up region of MA-bearing fuel with The thermal-fluid behavior of LBE in TEF-T target was calculated
air-cooling is considered to measure the physics parameters of the by the STAR-CD (CD-Adapco) with a detailed three-dimensional
transmutation system. The central rectangular region model. The tetra metric type is applied and the divided face was
(28 cm  28 cm  60 cmL) will be replaced with a special subas- set a reflected image condition in the Computational Fluid Dy-
sembly, which can install the pin-type MA fuel around the spall- namics (CFD) analysis. At first, LBE flowed through the annular
ation target. region and it joined at the center of the beam window and turned
over and flowed in the inner tube after having passed a rectification
2.2. Outline of TEF-T lattice and an irradiation sample. In a default condition, the flow
rate in the inlet of annulus region was set to 1 litter/sec. The inlet
For the JAEA-proposed ADS, LBE is a primary candidate of velocity was set in a uniform velocity condition. LBE flow is easy to
coolant and spallation target. To solve technical difficulties for LBE form a complicated turbulent flow to have a particular physical
utilization, construction of TEF-T is planned to complete the data property. Therefore, the k-ε model for high Re number was used for
sets, which is required for the design of ADS. The experiments to a turbulence model. The heat power density shown in previous
obtain the material irradiation data for beam window are the most paragraph was used for CFD analysis. The internal pressure to the
important mission of TEF-T. inside of the beam window was set to 0.3 MPa in consideration of
A high power spallation target, which will be mainly used for
material irradiation of candidate materials for a beam window of
Table 1
full-scale ADS, is an essential issue to realize a TEF-T. To set up the
Conditions of proton beam profile.
beam parameters, future ADS concepts are taken into account. In
the reference case of the target, proton beam current density of Item Unit Parameters

20 mA/cm2, which equals to the maximum beam current density of Case 1 Case 2 Case 3 Case 4
JAEA-proposed 800 MWth ADS, was assumed. Detailed analysis for Energy MeV 400 400 400 400
TEF-T spallation target, which is illustrated in Fig. 2, is described in Average beam current mA 625 625 625 625
following section. Beam power kW 250 250 250 250
During the irradiation of spallation target, a fast neutron field is Beam shape Gauss Gauss Gauss Flat
Maximum beam current density mA/cm2 20 40 60 20
formed around the spallation target. Utilization of excess spallation
66 T. Sasa / Progress in Nuclear Energy 82 (2015) 64e68

1200 tendency was observed as for the overall LBE flow; the dead flow
Case 1 region was formed near the inner surface of the central region of
heat generation density [W/cm3]

1000 Case 2 the beam window, and the size of the dead flow region hardly
Case 3 changed even if the inlet flow rate was increased. It is desirable that
800 Case 4
the local velocity conditions of LBE are less than 2 m/s to avoid the
striking erosion for materials. The maximum velocity of LBE flow
600 was observed just after the rectification lattice, and it was
approximately 1.2 m/sec in the case of the inlet flow rate of 1 litter/
400 sec. In the case of 4 litter/sec, this maximum velocity reached
approximately 4.8 m/sec. Because the flowing velocity was too fast
200 in this condition, the vibration of the target vessel by the LBE flow
was concerned about as well as the acceleration of erosion/corro-
0
0 5 sion. A slit was arranged along the side of the rectification lattice;
distance of radial direction [cm] however, the dead region was formed by the velocity difference and
this state suggested that the cooling performance of the sample
Fig. 3. Heat power density profile of incident beam. holder was spoiled. An additional analysis to confirm a gravity ef-
fect was performed and the deflection of LBE flow was not observed
in this condition.
the flowing LBE and the pressure of the cover gas. On the outer wall Examples of the analysis result for temperature profile are
of the beam window and the border of the atmosphere, release of shown in Figs. 5e7. Fig. 5 shows the temperature profile on the
the radiant heat was considered. In this analysis, the embrittlement beam window by changing the thickness of beam window from
of the structural materials by the irradiation was not considered. 2 mm to 3 mm. The flow rate of LBE was 1 litter/sec, and the proton
Based on the results provided by CFD analysis, the analysis to verify beam profile was Case 1. Because the striking corrosion was nor-
the feasibility of the beam window was performed by ABAQUS mally not observed below 500  C, this value is one of the criteria for
code. The operating conditions for the first stage of TEF-T were then the beam window design. The maximum temperature of 554  C
decided by a result of the analysis on each condition. was observed at the center of the outside surface of the beam
window, because of the formation of the dead region of LBE flow in
4. Analytical results the case of 3 mm thick beam window. In the case of 2 mm thick
window, peak temperature reaches 477  C. In this condition, it was
4.1. Velocity profile and temperature profile confirmed that maximum temperature was reduced about 77  C by
decreasing the thickness of the window. The temperature differ-
The thermal-fluid analyses of TEF-T target were performed to ence of the outside and the inside was 65  C and 37  C in the case of
determine the temperature distribution by various beam injection 3 mm window and 2 mm window, respectively. From these results,
condition. In the analysis, the inlet LBE temperature was fixed to it was disclosed that a condition of 2 mm was preferable. Fig. 6
350  C. shows the effect of the peak current density of the proton beam.
The velocity profiles with three different flow rates from 1 to The flow rate was 1 litter/sec, and the thickness of the beam win-
4 litter/sec are summarized in Fig. 4. In each flow rate, a similar dow was 2 mm. In the conditions of Case 2 and Case 3, where the

Fig. 4. Velocity profile by changing inlet flow rate.


T. Sasa / Progress in Nuclear Energy 82 (2015) 64e68 67

Fig. 7. Contour plot of the stress strength of the beam window.

analysis, results of the STAR-CD were used for the temperature of


each node. Fig. 7 shows the contour plot of the stress strength
Fig. 5. Temperature profile of beam window by changing thickness.
(Tresca stress) on the cross-section of the beam window along the
direction of beam-axis, which is taken upward in the vertical di-
beam current density was increased, the maximum temperature rection. The stress strength reached the maximum value of 190 MPa
exceeded 500  C. The temperature differences also increased in on the outer surface of the beam window.
either condition. It was, therefore, confirmed that Case 2 and 3 were The stress strength obtained by steady-state analysis was
unacceptable conditions from a viewpoint of the structural divided into the primary general membrane stress (Pm), the pri-
soundness of the beam window. mary bending stress (Pb) and secondary thermal-load stress (Q) to
As one method to realize a uniform exposure dose for each estimate the structural integrity of the beam window. At this time,
specimen, the beam of the flat top type has been considered. In Pm and Pb were calculated only from the internal pressure to the
Case 4, the maximum temperature was 482  C and the temperature inside of the beam window (0.3 MPa). On the other hand,
difference was 38  C with 1 litter/sec LBE flow rate and the 2 mm Pm þ Pb þ Q was calculated from both the internal pressure to the
thick beam window. By the result of flat top type, the temperature inside of the beam window and the temperature distribution of the
incline was extremely large at the position around the beam edge. beam window. Fig. 8 shows the values for Pm þ Pb þ Q by changing
However, the maximum temperature and the temperature differ- the flow rate of LBE and the beam profile. In this figure, the hori-
ence were at the same level as Case 1. We would, therefore, zontal axis represents the temperature at the center of wall thick-
continue this verification because this beam shape had an effective ness of the beam window where the values for Pm þ Pb þ Q was
factor for the test of materials irradiation. maximum, and the dotted line represents the value of 3Sm. When
As a result of these analyses, the following conditions are the Pm þ Pb þ Q is located under the dotted line, the designed beam
acceptable for the TEF operation; (1) the flow rate of LBE is 1 litter/ window can be regarded as feasible. From this figure, it is observed
sec, (2) the thickness of the beam window is 2 mm, and (3) the that the Case 1 and Case 4 is feasible to use and Case 2 may be used
proton beam which has a Gaussian shape with the peak current with high LBE flow late of 4 litter/sec.
density of 20 mA/cm2. We set these conditions as a reference case
for the realization of TEF-T and carried out thermal-stress analysis 5. Conclusion
to verify the soundness of the beam window.
To perform the design study for the transmutation system of
4.2. Thermal stress analysis long-lived nuclides, the construction of TEF, which consist two
buildings, TEF-T and TEF-P, is proposed under the J-PARC Project.
The thermal stress for the steady-state was estimated using According to the current construction schedule, TEF-T will be built
ABAQUS (Dassault Systems) code, the computational code for the
finite element method (FEM). In the ABAQUS code, the beam
window was modeled as the cylinder-slab geometry. The model
consisted of 1896 4-node axial-symmetric elements. For the

Fig. 6. Temperature profile by changing current density of the proton beam. Fig. 8. Evolution for Pm þ Pb þ Q by changing the flow rate of LBE and the beam profile.
68 T. Sasa / Progress in Nuclear Energy 82 (2015) 64e68

at the first phase and TEF-P will be constructed at the latter phase. installed according to the experimental requirement. It was shown
Licensing procedures for TEF-P construction will be processed that reference case of injected proton beam condition (400 MeV-
simultaneously with TEF-T construction. 250 kW and 20 mA/cm2 of beam current density) was applicable to
TEF-P is a critical assembly, which can accept the 400 MeV- the TEF-T target. Further studies to improve irradiation perfor-
10 W proton beam for the spallation neutron source. The pur- mance will be performed, (a) the optimization of a beam shape and
poses of TEF-P are the experimental validation of the data and the configuration of the flow channel, (b) the inlet LBE condition
method to predict neutronics of the fast subcritical system with including the deflection of LBE flow, and (c) the change of cooling
spallation neutron source, the demonstration of the controlla- performance for the beam window by the additional bypass jet
bility of subcritical system driven by an accelerator, and the basic flow to eliminate the dead flow region.
research of reactor physics for transmutation of MA and LLFP. The
distinguished points of TEF-P in comparison with existing References
experimental facilities can be summarized as follows: (1) both the
high energy proton beam and the nuclear fuel are available, (2) CD-Adapco “STAR-CD”, CFD Commercial Code.
Dassault Systems “ABAQUS”, FEM Commercial Code.
the maximum neutron source intensity of about 1012 n/s is strong Niita, K., et al., 2010. PHITS: Particle and Heavy Ion Transport Code System, Version
enough to perform precise measurements even in the deep 2.23. JAEA-Data/Code 2010-022.
subcritical state (e.g. k-eff ¼ 0.90), and, is low enough to easily Oigawa, H., et al., 2001. Conceptual design of Transmutation Experimental Facility.
In: Proc. Global 2001, Paris, France. CD-ROM.
access to the assembly after the irradiation, (3) wide range of Sasa, T., et al., 2004. Research and development on accelerator-driven trans-
pulse width (1 ns e 0.5 ms) is available by the laser charge ex- mutation system at JAERI. Nucl. Eng. Des. 230, 209e222.
change technique, (4) MA and LLFP can be used as a shape of foil, Sasa, T., et al., 2005. Conceptual Study of Transmutation Experimental Facility (2)
Study on ADS Target Test Facility (in Japanese), JAERI-Tech 2005-021.
sample and fuel by installing an appropriate shielding and remote
Soule, R., et al., 2004. Neutronic studies in support to ADS: the Muse experiments in
handling devises. the MASURCA facility. Nucl. Sci. Eng. 148, 124e152.
TEF-T is a facility to prepare the database for engineering design Sugawara, T., Suzuki, K., Nishihara, K., et al., 2008. Investigation of Beam Window
Structure for Accelerator Driven System e Simplified Overall Integrity Assess-
of ADS using 400 MeV-250 kW proton beam and the PbeBi spall-
ment and Detailed Assessment on Buckling-. JAEA-Research 2008-026. Japan
ation target. The purposes of TEF-T are R&D for the structural Atomic Energy Agency (in Japanese).
strength of the beam window which is irradiated by both high- The Joint Project Team of JAERI and KEK, 2000. The Joint Project for High-Intensity
energy proton and neutron, the compatibility of the structural Proton Accelerators (in Japanese), JAERI-Tech 2000-003.
Uyttenhove, W., et al., 2011. The neutronic design of a critical lead reflected zero-
material with flowing liquid PbeBi and the operation of the high power reference core for on-line subcriticality measurements in accelerator
power spallation target. Several kinds of target head can be driven systems. Annu. Nucl. Energy 38 (7), 1519e1526.

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