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Abstract— Integrating electronics into the body of complex layer extrusion of melted thermoplastics, was one of the earli-
structural parts through 3-D printing is one of the most promising est 3-D printing technologies [9] and remains one of the most
new technologies in additive manufacturing, giving the potential widely used due to its low-cost equipment and materials [10].
of lighter weight and smaller electronic systems. Although fused
filament fabrication (FFF) is one of the cheapest and most FFF printers, such as the Makerbot, are common in schools
widely available 3-D printing approaches available, FFF has and universities [11] and have been a major factor in bringing
lagged behind alternatives, such as direct write printing for 3-D printing to the homes of hobbyists worldwide [12].
incorporating electronics into 3-D printed parts. In this article, As with other 3-D printing technologies, there has been
complex structural electronics are demonstrated using FFF. interest in adding electrical functionality to FFF printed parts.
Numerous surface-mount components are integrated into the
printing process for 3-D structures, and electrical contact is made While early FFF printing was based on thermoplastics such
using conductive thermoplastic filament with and without copper as acrylonitrile butadiene styrene (ABS) and polylactic acid
electroplating for improved conductivity. The electrical contact (PLA), demand for improved material properties and new
characteristics and bridging behavior of several commercially functionality has led to widespread printing of thermoplastic
available filaments are investigated. A circuit demonstrator, composite materials [13]. Adding metal or carbon particles
a 555-timer oscillator circuit, is then printed using the process.
to a thermoplastic filament creates a conductive compos-
Index Terms— 3-D printing, additive manufacturing, conduc- ite that can be extruded through a standard heated nozzle,
tive composites, fused filament fabrication (FFF), structural allowing printing of electrical traces and sensors within a
electronics.
printed part without modification of the FFF printer [14].
I. I NTRODUCTION A number of conductive thermoplastic composite filaments are
now commercially available [15], and the technology has been
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1966 IEEE TRANSACTIONS ON COMPONENTS, PACKAGING AND MANUFACTURING TECHNOLOGY, VOL. 10, NO. 12, DECEMBER 2020
Fig. 1. (a) Part alignment and (b) making electrical contact with conductive filament and (c) and (d) example print, a pyramid with four surface-mount
components (two red LEDs and two resistors), with LEDs lit.
electroplated copper layers on printed parts [21], [25], but II. FABRICATION
this approach is manual and soldering smaller surface-mount
components is challenging. A. 3-D Printing
For finer pitch surface-mount components, most demonstra- Two different conductive thermoplastic filaments were
tions instead rely on silver-loaded inks [26] or pastes [23], [21] investigated for component embedding, Protopasta Conductive
for mounting and electrical contact. This hybrid approach PLA, and Multi3D Electrifi. The Conductive PLA consists
requires either manual addition of the ink/paste by hand or use of PLA, a dispersant, and conductive carbon black parti-
of a direct-ink-writing print head within the process, limiting cles [27], whereas Electrifi is based on copper particles within
the value of using the conductive filaments for the conductors. a biodegradable polyester thermoplastic [24]. Each has respec-
Recently, however, there was a limited demonstration that tive advantages; the Conductive PLA is relatively rigid and
suggests it is potentially possible to print directly over a prints at similar temperatures to PLA and ABS (from 190 ◦ C
surface-mount component and make electrical contact. In [19], to 230 ◦ C), typically allowing easier printing, but is relatively
a single large surface-mount LED (5050 package size, with resistive (15 · cm in filament form). [15], [19]. Electrifi
widely spaced contacts) was printed over with the high- is the most conductive thermoplastic filament commercially
performance conductive thermoplastic filament, Electrifi, using available (resistivity of 0.006 · cm in filament form) [24]
an FFF printer, and shown to light successfully with an applied but prints at lower temperatures (130 ◦ C–160 ◦ C) [19] and
voltage. is substantially softer, both of which can make it more
In this work, for the first time, we demonstrate the integra- challenging to integrate into a standard FFF printing process.
tion and electrical contact to numerous small surface-mount Both filaments have higher resistivity as printed compared
components using conductive and nonconductive filaments with their filament resistivity (up to an order of magnitude
within the same print. Printed slots are used to align and or more higher), although the level of increase varies through
position surface-mount components within the FFF prints (see factors such as print settings and orientation; the full resistivity
Fig. 1), with a controlled pause used to allow part insertion behavior for both filaments upon printing has been studied
[see Fig. 1(a)], followed by further printing of the conductive extensively elsewhere (see [15]). After printing, the Protopasta
traces [see Fig. 1(b)] and the remainder of the part. The can be contacted directly by probes to measure or apply a
component embedding behavior of two commercially available voltage; the softer Electrifi requires the addition of silver paste
conductive filaments was characterized. While both were able or use of screw terminals on the contact points to make a
to make electrical contact, the softer Electrifi filament was robust contact.
found to sag more when crossing a gap in the print and there- For the structural layer, two different thermoplastic fil-
fore to more consistently contact an embedded surface-mount aments (Makerbot True Green ABS and Ultimaker Silver
pad. Electroplating of copper was also demonstrated to reduce Metallic PLA) were used depending on the printer involved
the electrical contact resistance to the part. An oscillator circuit (see below). Both tested conductive filaments adhered to either
with a number of small surface-mount components, including of the structural filaments, and with the exception of the
an eight-pin SOIC-8 package 555 timer, is then demonstrated changes in the needed extrusion temperature, the process was
using the process. found to work similarly for both.
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LAZARUS AND TSANG: 3-D PRINTING STRUCTURAL ELECTRONICS WITH CONDUCTIVE FILAMENTS 1967
TABLE I
P RINT S ETTINGS
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1968 IEEE TRANSACTIONS ON COMPONENTS, PACKAGING AND MANUFACTURING TECHNOLOGY, VOL. 10, NO. 12, DECEMBER 2020
Fig. 3. (a) Printed part with embedded LED and vertical Electrifi vias.
(b) With LED turned on. (c) Printed Protopasta Conductive PLA traces to an
LED. (d) After applied voltage.
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LAZARUS AND TSANG: 3-D PRINTING STRUCTURAL ELECTRONICS WITH CONDUCTIVE FILAMENTS 1969
B. Bridging
To understand the reasons for this difference in printing
yield, the bridging behavior of the two filaments was inves-
tigated. For each conductive filament, a part was printed in
ABS with a series of gaps of differing widths and subsequently
bridged with a line of conductive filament eight layers thick Fig. 5. Printed (a) Electrifi and (b) Protopasta Conductive PLA trace (1 mm
wide, eight layers thick) crossing designed gap of 1 mm (scale bar is 1 mm),
and 1 mm wide. Both were capable of bridging a sizeable gap and (c) measured sag depth.
(to at least 2-mm designed spacing, the largest tested). The
Electrifi, however, is a substantially softer filament, with thin
layers less able to support their own weight; the printed trace, not always make a robust contact to an embedded part.
therefore, sags down into the gap, as is clearly evident in the The Electrifi, on the other hand, sags hundreds of micrometers
side view [see Fig. 5(a)]. The Protopasta filament bridges the more for gaps the size of the surface-mount components used,
gap far better, with minimal sag [see Fig. 5(b)]. The degree resulting in the filament conforming well to the top surface of
of sag for each type of filament was characterized optically the part and giving a solid electrical contact.
for a range of different gaps [see Fig. 5(c)], with at least three
gaps measured for each data point, and the average gap width
measured optically for each set of data points; the average C. 555 Timer Circuit
gap was consistently several hundred micrometers narrower Simple oscillators based on the 555 timer IC have been
than designed due to spreading of the thermoplastic upon a common example circuit within the 3-D printing commu-
extrusion. nity [8], [21], [23] since it requires a modest number of com-
The component embedding process here is based on placing ponents and provides a clear visual indication of functionality.
components roughly at the top surface of a gap and relying The small outline integrated circuit (SOIC) eight-pin surface-
on flow of the extruded filament to conform to the pad and mount version of the 555 timer requires an independent
make a robust contact. FFF typically results in a relatively connection to seven pins without shorting, with a pin pitch of
rough surface finish, up to several hundred micrometers (as only 1.27 mm; note that one of the eight pins of the package is
seen in the cross sections in Fig. 5); this roughness results in not used for the oscillator circuit here. Due to the narrow pin
a similar level of variability in the component position and spacing, the Makerbot was found to be unable to consistently
the height of the gap edges. Since the Protopasta filament avoid shorting, and the Ultimaker 3 with Electrifi was instead
bridges the gaps very well, with vertical sag on the order used. The tendency of Electrifi to conform to the pints of the
of a hundred micrometers, the extruded material likely does embedded part can be seen clearly in Fig. 6(a). Even though
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1970 IEEE TRANSACTIONS ON COMPONENTS, PACKAGING AND MANUFACTURING TECHNOLOGY, VOL. 10, NO. 12, DECEMBER 2020
TABLE II
L ITERATURE S URVEY OF C OMPOSITE F ILAMENT
E LECTRICAL C OMPONENT E MBEDDING
Fig. 6. (a) Side view of embedded SOIC-8 package(scale bar 2 mm) and
SOIC lead. (b) Side view. (c) End-on view CT scans of individual pin interface
(scale bars 500 μm).
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LAZARUS AND TSANG: 3-D PRINTING STRUCTURAL ELECTRONICS WITH CONDUCTIVE FILAMENTS 1971
Our demonstration of an oscillator, including a multipin [5] M. Borges, “Conductive traces on 3D metal parts: Powder coating for
surface-mount IC, is also at a similar or greater level of laser direct structuring applications,” Laser Tech. J., vol. 11, no. 4,
pp. 48–51, 2014, doi: 10.1002/latj.201400039.
complexity to the most advanced systems in the literature for [6] J. A. Paulsen, M. Renn, K. Christenson, and R. Plourde, “Printing
thermoplastic printing, with up to ten components successfully conformal electronics on 3D structures with aerosol jet technology,”
integrated and contacted. Table II shows a survey of notable in Proc. Future Instrum. Int. Workshop (FIIW) Proc., Gatlinburg, TN,
USA, Oct. 2012, pp. 1–4.
examples of electrical part embedding using FFF. Despite its
[7] J. Li et al., “Hybrid additive manufacturing of 3D electronic systems,”
promise in reducing cost and improving accessibility of 3-D J. Micromech. Microeng., vol. 26, no. 10, 2016, Art. no. 105005,
printed structural electronics, component embedding using doi: 10.1088/0960-1317/26/10/105005.
FFF is relatively immature compared with other approaches. [8] G. T. Carranza, U. Robles, C. L. Valle, J. J. Gutierrez, and
R. C. Rumpf, “Design and hybrid additive manufacturing of
Until relatively recently, the focus of most work in the area was 3-D/volumetric electrical circuits,” IEEE Trans. Compon., Packag.,
on filament conductivity and resulting LED demonstrators, and Manuf. Technol., vol. 9, no. 6, pp. 1176–1183, Dec. 2019, doi:
before 2018, the authors were unable to find examples of 10.1109/TCPMT.2019.2892389.
more complex systems using thermoplastic conductors. The [9] R. D. Sochol et al., “3D printed microfluidics and microelec-
tronics,” Microelectron. Eng., vol. 189, pp. 52–68, Apr. 2018,
shift toward more complicated circuits likely resulted from doi: 10.1016/j.mee.2017.12.010.
the increasing availability of higher performance conductors [10] H. Bikas, P. Stavropoulos, and G. Chryssolouris, “Additive manu-
such as Electrifi to the community, and our work is a notable facturing methods and modelling approaches: A critical review,” Int.
J. Adv. Manuf. Technol., vol. 83, nos. 1–4, pp. 389–405, Mar. 2016,
milestone toward achieving true structural electronics using doi: 10.1007/s00170-015-7576-2.
this approach. [11] T. Barrett et al., “A review of university maker spaces,” in Proc. ASEE
Annu. Conf. Expo. Proc., Seattle, WA, USA, 2015, pp. 1–5.
[12] I. Mohomed and P. Dutta, “THE age of DIY and dawn of the maker
V. C ONCLUSION movement,” GetMobile: Mobile Comput. Commun., vol. 18, no. 4,
pp. 41–43, Jan. 2015.
FFF is one of the most widely used 3-D printing tech-
[13] X. Wang, M. Jiang, Z. Zhou, J. Gou, and D. Hui, “3D printing of
nologies, and the low cost and accessibility of FFF make polymer matrix composites: A review and prospective,” Compos. B,
it common in the consumer and hobbyist markets. This Eng., vol. 110, pp. 442–458, Feb. 2017, doi: 10.1016/j.compositesb.
work demonstrates for the first time the ability to integrate 2016.11.034.
[14] S. J. Leigh, R. J. Bradley, C. P. Purssell, D. R. Billson, and
numerous surface-mount components directly into the printing D. A. Hutchins, “A simple, low-cost conductive composite material for
process for filament-based printing. The process was both 3D printing of electronic sensors,” PLoS ONE, vol. 7, no. 11, Nov. 2012,
characterized, and an oscillator circuit was demonstrated as Art. no. e49365, doi: 10.1371/journal.pone.0049365.
a representative complex circuit possible in the technology. [15] H. Watschke, K. Hilbig, and T. Vietor, “Design and characteriza-
tion of electrically conductive structures additively manufactured by
Enabling the hobbyists to easily add complex electronics to 3- material extrusion,” Appl. Sci., vol. 9, no. 4, p. 779, Feb. 2019,
D printed parts, a technology previously limited to those with doi: 10.3390/app9040779.
access to specialized printers, could be revolutionary. It is now [16] M. Sajid, J. Z. Gul, S. W. Kim, H. B. Kim, K. H. Na, and
K. H. Choi, “Development of 3D-printed embedded temperature sen-
feasible for even a nonspecialist to print structural electronics sor for both terrestrial and aquatic environmental monitoring robots,”
in a university makerspace or potentially even in the comfort 3D Printing Additive Manuf., vol. 5, no. 2, pp. 160–169, Jun. 2018,
of their own home. doi: 10.1089/3dp.2017.0092.
We envision the use of this manufacturing technology to [17] S. Lathers, M. Mousa, and J. La Belle, “Additive manufacturing
fused filament fabrication three-dimensional printed pressure sensor
enable more complex circuits to be implemented in FFF. for prosthetics with low elastic modulus and high filler ratio filament
Filament-based electronics is still a relatively new technology, composites,” 3D Printing Additive Manuf., vol. 4, no. 1, pp. 30–40,
and there remains a significant need to better understand the Mar. 2017, doi: 10.1089/3dp.2016.0051.
[18] S. B. Walker and J. A. Lewis, “Reactive silver inks for patterning
resulting circuit performance. For future work, we therefore high-conductivity features at mild temperatures,” J. Amer. Chem. Soc.,
suggest that there would be significant impact for follow vol. 134, no. 3, pp. 1419–1421, Jan. 2012, doi: 10.1021/ja209267c.
on investigations on functional circuit behavior for circuits [19] P. F. Flowers, C. Reyes, S. Ye, M. J. Kim, and B. J. Wiley, “3D
printed using conductive thermoplastics. Possible studies could printing electronic components and circuits with conductive thermo-
plastic filament,” Additive Manuf., vol. 18, pp. 156–163, Dec. 2017,
include noise analysis, thermal performance, reliability, current doi: 10.1016/j.addma.2017.10.002.
carrying capacity, and RF characteristics. [20] K. Angel, H. H. Tsang, S. S. Bedair, G. L. Smith, and N. Lazarus,
“Selective electroplating of 3D printed parts,” Additive Manuf., vol. 20,
pp. 164–172, Mar. 2018, doi: 10.1016/j.addma.2018.01.006.
R EFERENCES [21] N. Lazarus, S. S. Bedair, S. H. Hawasli, M. J. Kim, B. J. Wiley,
and G. L. Smith, “Selective electroplating for 3D-printed electronics,”
[1] E. MacDonald et al., “3D printing for the rapid prototyping of Adv. Mater. Technol., vol. 4, no. 8, Aug. 2019, Art. no. 1900126,
structural electronics,” IEEE Access, vol. 2, pp. 234–242, 2014, doi: 10.1002/admt.201900126.
doi: 10.1109/ACCESS.2014.2311810.
[22] E. Vaneckova et al., “Copper electroplating of 3D printed composite
[2] A. Joe Lopes, E. MacDonald, and R. B. Wicker, “Integrating stereolitho-
graphy and direct print technologies for 3D structural electronics fabri- electrodes,” J. Electroanal. Chem., vol. 858, Feb. 2020, Art. no. 113763,
cation,” Rapid Prototyping J., vol. 18, no. 2, pp. 129–143, Mar. 2012, doi: 10.1016/j.jelechem.2019.113763.
doi: 10.1108/13552541211212113. [23] J. Li, Y. Wang, G. Xiang, H. Liu, and J. He, “Hybrid additive man-
[3] H. Ota et al., “3D printed ‘Earable’ smart devices for real-time detection ufacturing method for selective plating of freeform circuitry on 3D
of core body temperature,” ACS Sensors, vol. 2, no. 7, pp. 990–997, printed plastic structure,” Adv. Mater. Technol., vol. 4, no. 2, Feb. 2019,
Jul. 2017, doi: 10.1021/acssensors.7b00247. Art. no. 1800529, doi: 10.1002/admt.201800529.
[4] J. P. Swensen, L. U. Odhner, B. Araki, and A. M. Dollar, “Printing [24] (2019). Electrifi FAQs. [Online]. Available: https://Multi3Dllc.com/faqs
three-dimensional electrical traces in additive manufactured parts for [25] M. J. Kim et al., “One-step electrodeposition of copper on conductive
injection of low melting temperature metals,” J. Mech. Robot., vol. 7, 3D printed objects,” Additive Manuf., vol. 27, pp. 318–326, May 2019,
no. 2, pp. 021004-1–021004-10, May 2015, doi: 10.1115/1.4029435. doi: 10.1016/j.addma.2019.03.016.
Authorized licensed use limited to: ETH BIBLIOTHEK ZURICH. Downloaded on December 13,2023 at 23:35:39 UTC from IEEE Xplore. Restrictions apply.
1972 IEEE TRANSACTIONS ON COMPONENTS, PACKAGING AND MANUFACTURING TECHNOLOGY, VOL. 10, NO. 12, DECEMBER 2020
[26] C. Cao et al., “Methodology for the additive manufacture of embedded Nathan Lazarus received the B.S. degree in electri-
conductive paths connecting microelectromechanical sensors using con- cal engineering from the University of Pennsylvania,
ductive and flexible filaments with extrusion devices,” Rapid Prototyping Philadelphia, PA, USA, in 2007, and the M.S. and
J., vol. 26, no. 2, pp. 349–359, Oct. 2019, doi: 10.1108/RPJ-03-2019- Ph.D. degrees in electrical and computer engineering
0058. from Carnegie Mellon University, Pittsburgh, PA,
[27] M. Ibrahim, Y. Mogan, S. N. S. Jamry, and R. Periyasamy, “Resistivity in 2010 and 2012, respectively.
study on conductive composite filament for freeform fabrication of In 2012, he joined the U.S. Army Research Lab-
functionality embedded products,” ARPN J. Eng. Appl. Sci., vol. 11, oratory, Adelphi, MD, USA, where he is currently
no. 10, 6525-6530, 2016. a Staff Researcher with the Sensors and Electron
[28] A. D. Valentine et al., “Hybrid 3D printing of soft electron- Devices Directorate. He has also served as a Part-
ics,” Adv. Mater., vol. 29, no. 40, Oct. 2017, Art. no. 1703817, Time Faculty Member for several semesters with
doi: 10.1002/adma.201703817. George Washington University, Washington, DC, USA, lecturing on microme-
[29] N. Grimmelsmann, Y. Martens, P. Schäl, H. Meissner, and A. Ehrmann, chanical systems design. He has authored or coauthored 46 refereed journal
“Mechanical and electrical contacting of electronic components on tex- publications and holds 15 patents received or pending. His research interests
tiles by 3D printing,” Procedia Technol., vol. 26, pp. 66–71, Dec. 2016, include micromechanical power devices, stretchable electronics, and additive
doi: 10.1016/j.protcy.2016.08.010. manufacturing.
[30] S. W. Kwok, K. Goh, Z. Tan, S. Tan, and W. Tjiu, “Electrically Dr. Lazarus’s awards and honors include ARL’s Honorary Award for Engi-
conductive filament for 3D-printed circuits and systems,” Appl. Mater. neering and the Rookie of the Year Excellence in Federal Career Award (Gold)
Today, vol. 9, pp. 167–175, Dec. 2017. from the Baltimore Federal Executive Board. In 2019, he was selected for the
[31] J. O. Thostenson et al., “Integrated flexible conversion circuit between Presidential Early Career Award for Scientists and Engineers (PECASE) and
a flexible photovoltaic and supercapacitors for powering wearable sen- the highest honor given by the U.S. government for researchers beginning
sors,” J. Electrochem. Soc., vol. 165, pp. B3122–B3129, Apr. 2018, their independent research careers.
doi: 10.1149/2.0141808jcs.
[32] Z. Lei et al., “Fabrication of highly electrical conductive composite
filaments for 3D-printing circuits,” J. Mater. Sci., vol. 53, no. 20, Harvey H. Tsang received the B.S. degree in
pp. 14495–14505, Oct. 2018, doi: 10.1007/s10853-018-2645-1. electrical engineering from the University of Texas
[33] B. Podsiadly, A. Skalski, B. Walpuski, P. Walter, and M. Sloma, “Elec- at Arlington, Arlington, TX, USA, in 2009, and the
trically conductive acrylonitrile butadiene styrene (ABS)/copper com- M.S. and Ph.D. degrees in electrical engineering
posite filament for fused deposition modeling,” Proc. SPIE, vol. 10808, from the University of Texas at El Paso, El Paso,
Oct. 2018, Art. no. 1080856, doi: 10.1117/12.2501546. TX, in 2011 and 2016, respectively.
[34] K. Kutuniva, J. Mäkikangas, A. Mustakangas, T. Rautio, J. Kumpula, From 2010 to 2016, he was conducting research
and K. Mäntyjärvi, “DFAM based multi-material 3D printing using con- with 3-D printers for electronics at nScrypt and
ductive and flexible filaments,” Key Eng. Mater., vol. 786, pp. 364–370, Sciperio Inc., Orlando, FL, USA. Since 2016, he
Oct. 2018, doi: 10.4028/www.scientific.net/KEM.786.364. has been an Electronics Engineer with the Army
[35] Z. Lei et al., “Novel electrically conductive composite filaments Research Laboratory, Adelphi, MD, USA, where
based on Ag/saturated polyester/polyvinyl butyral for 3D-printing cir- his research interests include flexible hybrid electronics, 3-D printed radio
cuits,” Composites Sci. Technol., vol. 180, pp. 44–50, Aug. 2019, frequency devices in extreme environments, photonic sintering of conductive
doi: 10.1016/j.compscitech.2019.05.003. composites, and multifunctionalization of 3-D printed materials.
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