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Welding in the World (2024) 68:247–257

https://doi.org/10.1007/s40194-023-01666-5

RESEARCH PAPER

Properties oriented WAAM—microstructural and geometrical control


in WAAM of low‑alloy steel
Kai Treutler1 · Tobias Gehling1 · Maxim Scheck2 · Andreas Richter2 · Christian Bohn2 · Rüdiger Ehlers3 ·
Christian Rembe2 · Volker Wesling1

Received: 22 August 2023 / Accepted: 13 December 2023 / Published online: 20 December 2023
© The Author(s) 2023

Abstract
Today, arc-based additive manufacturing has great potential for industrial application due to new developments in robotics,
welding technology, and computer-aided manufacturing. Two issues are currently the focus of research. One is the accurate
generation of geometry with respect to the design, e.g., geometry fidelity, defined roughness, and shape deviations within the
tolerances. Here, there are still open questions, particularly with regard to path planning and the dependence of the geometry
on the selected process variables. The second topic is the adjustment or determination of the achievable mechanical and
microstructural properties, as these are of crucial importance for the use of the technology in industry. The combination of
both areas into a geometry- and property-oriented approach to additive manufacturing has been little discussed in the litera-
ture for arc-based welding processes. The correlations between cooling conditions and emerging properties can serve as a
starting point for such a consideration. The temperature history depends on three key factors: the energy input, the interpass
temperature (which in additive manufacturing is determined by the time to over-weld), and the heat transfer conditions, which
are determined by the part geometry. The melt pool size or volume also depends on these three constraints. In this study,
an approach is presented to realize property-oriented additive manufacturing from the interaction of property-oriented path
planning and a melt pool size control system. By controlling the melt pool size, the cooling of the material can be adjusted
within certain limits, and consequently, a local adjustment of the microstructure can be achieved, which greatly influences
the local mechanical properties. This work demonstrates this approach for a low-alloy filler metal (DIN EN ISO 14341-A G
50 7 M21 4Mo/A5.28 ER80S-D2). Gas metal arc welding was carried out using an M21 shielding gas (82% Ar, 18% ­CO2).
Finally, microstructural characterization will show that different microstructural morphologies and properties can be achieved
in a component by combining property-oriented path planning and the use of a control loop to regulate the melt pool size.

Keywords WAAM · Microstructure · Control · Low alloy steel · Weld pool

1 Introduction

Modern additive manufacturing approaches have the poten-


Recommended for publication by Commission IX - Behaviour of tial to add significant flexibility to manufacturing processes.
Metals Subjected to Welding
In additive manufacturing, an object is built up step by step
* Kai Treutler from raw material. While 3D printing is well established for
treutler@isaf.tu-clausthal.de plastics, additive manufacturing is more complex for metals,
* Volker Wesling resulting in a plethora of manufacturing approaches with
office@isaf.tu-clausthal.de different characteristics.
A well-established approach is wire arc additive manu-
1
Clausthal University of Technology, Institute of Welding facturing (WAAM), where a metal object is welded from
and Machining, Clausthal‑Zellerfeld, Germany
scratch onto a metal ground body using wire filler [1]. Using
2
Clausthal University of Technology, Institute for Electrical an industrial welding robot, this approach allows relatively
Information Technology, Clausthal‑Zellerfeld, Germany
large quantities of metal to be processed in a short period
3
Clausthal University of Technology, Institute for Software of time [2–6]. WAAM is based on arc welding, where an
and Systems Engineering, Clausthal‑Zellerfeld, Germany

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248 Welding in the World (2024) 68:247–257

electric current induces the heat necessary to melt both the


wire and the surface to which the wire material is attached.
Various shielding gases are used to protect the weld from
interaction with the air. In addition to solid wires, cored
wires are also increasingly used in wire-based additive man-
ufacturing [7–9]. A typical manufacturing system is shown
in Fig. 1.
Arc-based additive manufacturing offers great potential
for industrial applications today due to new developments
in the fields of robotics, welding technology, and computer-
assisted manufacturing [6, 11–13]. Two core topics are cur-
rently the focus of research, in addition to others. One is the
production of geometry, geometry errors, etc. There are still
open questions here, particularly with regard to path plan-
Fig. 2  WAAM part idea of different localized properties
ning and the dependence of the geometry on the selected
process variables. The second issue is the adjustment or
determination of the achievable properties, as these are for low-alloy steels, which have an allotropic phase transfor-
crucial for the use of the technology in industry. For low- mation, the course of the temperature history is of decisive
alloy steels in particular, the mechanical properties that can importance for the properties generated in the component.
be achieved depend on the thermal history of the material The temperature history is dependent on three central fac-
[14–18]. tors: the energy input, the interlayer temperature (in additive
The combination of both areas into a geometry and prop- manufacturing determined by the time until over-welding),
erty-oriented additive manufacturing has so far been little and the heat conduction conditions, which are determined by
discussed in the literature for arc-based welding processes. the component geometry. The melt pool size or the melt pool
Some work has been done by Chaurasia et al. [19–21], Rich- volume also depends on these three boundary conditions.
ter et al. [22–24], and others [25] on the usage of camera sys- In the presented work, an approach is presented to realize
tems for tracking the temperature field of the weld pool. The property-oriented additive manufacturing from the interac-
main outcome of these works is that tracking the temperature tion of property-oriented path planning and a system for
field can lead to increased geometrical and microstructural controlling the melt pool size. By controlling the weld pool
homogeneity. size, the cooling of the material can be adjusted within cer-
The correlations between cooling conditions and emerg- tain limits and a local adjustment of the microstructure, and
ing properties can serve as a starting point for such a con- the mechanical properties can be achieved.
sideration, and therefore, the production of components with The first part of the work will briefly describe a new
locally adjusted properties, such as strength and toughness, approach to realizing property-oriented path planning,
is the overreaching goal Fig. 2. Fig. 3. This is based on a rudimentary thermodynamic
The correlation between the material properties and the simulation of the build-up process, which has been kept
selected energy input and the number of thermal cycles is simple enough to allow an execution in a very short time,
already known for a number of materials [26]. In particular, to obtain a path planning via an adapted SAT solver,

Fig. 1  Welding robot system at


Clausthal University of Tech-
nology [10]

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Welding in the World (2024) 68:247–257 249

Fig. 3  Schematic of the process


steps that need to be taken to
realize property-oriented control
in WAAM

which takes into account defined cooling conditions in 1.2 Microstructure and thermal history
certain component areas [10]. In this publication, the
results of the system identification are used for inves- Understanding the microstructure evolution during additive
tigations of the material properties. The changes in the manufacturing is key to realizing certain material proper-
microstructure that result, in a first approach, from the ties. In the case of continuous cooling or heating, the cor-
step changes in the process parameters. responding CCT or CHT diagram describes the metastable
Finally, a microstructural characterization will show microstructure formation. In general, however, these data
that different microstructure morphologies and properties cannot be directly extrapolated to additive manufacturing
can be realized in a component by combining property- conditions due to the, in many cases, different cooling condi-
oriented path planning and the use of a control loop to tions between WAAM, multilayer welding, and the condi-
regulate the melt pool size. tions under which the CCT/CHT diagrams are generated.
Repeated thermal cycling around certain temperatures will
result in a different microstructure.
1.1 Property‑oriented path planning method The influence of a cyclical temperature evolution on
microstructure formation during welding was analyzed by
One method for the realization of material property-ori- Samardžić et al. [27] and Huang et al. [26] using a weld-
ented path planning was suggested by Ehlers et al. [10]. ing simulator and a quenching and forming dilatometer,
In that paper, it was shown how to search for welding respectively. These physical simulators allow the applica-
paths with a satisfiability solver (SAT). The basic idea tion of transient, particularly cyclic, temperature profiles.
is to discretize the object to be manufactured into blocks The resulting dynamic transformation temperatures for mul-
and represent the connections between these blocks in the tiple temperature cycles can be determined. Microstructural
form of a graph. Two blocks that can be produced con- investigations and hardness measurements were also carried
secutively are connected by an edge in the graph. For their out. Celin et al. [28] investigated the microstructure devel-
initial study of planning welding paths under cooling time opment in different areas of the heat-affected zone during
constraints in 3D, the discretization of the object parts the multipass welding of a fillet weld for a high-strength
into cubes was performed, but the approach presented is fine-grained structural steel. The multipass welding pro-
not restricted to cubes. A search was then performed in cess results in thermal cycles corresponding to those of the
the graph for a fragmented Hamiltonian path, i.e., one WAAM process. The microstructure during the actual weld-
consisting of several independent paths that together visit ing process was compared with that obtained from dilatom-
all vertexes. Additional constraints on the paths encode eter simulations using a temperature profile similar to that
the process-related requirements. The approach was to during the welding process. It was concluded that dilatom-
check whether the planned fragmented path satisfied the eter studies are well suited to simulate the microstructure
required ­t8/5-times after finding a satisfactory assignment evolution in the heat-affected zone under cyclic tempera-
to all variables. The cooling conditions were calculated ture conditions. Several working groups have investigated
by a simplified simulator. Figure 4 shows a visualization microstructure evolution during the WAAM process. Some
of the simulator state in the middle of a welding process results are published in [16, 29–35]. For low-alloy steels,
of a simple geometry. in general, they showed that at least four different types of

Fig. 4  Temperature field in a


fast temperature simulation of a
simple WAAM part [10]

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250 Welding in the World (2024) 68:247–257

microstructures could occur. In the top layers, a microstruc- selected wavelengths, the emissivity need not be considered
ture comparable to single run weld metal is present. Beneath [36]. In our solution, two narrowband optical filters (central
the microstructure changes and is comparable to multi run wavelength of the narrowband filters: 680 nm and 860 nm)
welds. Due to the extensive reheating beneath this zone, the are used in front of the cameras to block out the arc. The
microstructure changes again and forms a microstructure spectrum of a low alloy steel with the corresponding filter
comparable to a normalized steel sheet. The fourth zone is wavelength is shown in Fig. 5. The selection of the correct
the transition area between the weld metal and the substrate. filter must be material-dependent due to the different emitted
Here, again, a microstructure comparable to multilayer wavelengths of each material in metal vapor–based plasma.
welded joints occurs. The underlying relationships need to The basic radiation of the argon plasma stays the same, but
be understood and are the basis of a local adjustment of in GMA welding, the metal vapor is dominant.
material properties. Afterwards, the temperature field distri- The emitted wavelengths of the metal vapor plasma
bution can be controlled to achieve certain material proper- depend on its composition. In GMA welding, this in itself
ties. In the following, the realization of a measurement and depends to a large extent on the filler metal used. These
control system is presented, and the first results for local filters are matched to the emission spectrum of the plasma
adjusted material properties are presented. generated by the arc and define the support points. This ena-
bles optical temperature measurements of the molten pool.
The jitter of the two triggered digital camera images used to
2 Materials and methods determine the surface temperature is much smaller than the
exposure time of the images. Therefore, with the temporal
2.1 Experimental setup resolution of the camera's exposure time, the synchronized
cameras capture the same instant. The general setup of the
The experimental setup consists of three core components, measurement system is shown in Fig. 6. The data process-
the welding robot, the visual detection of the melt pool size ing is described in [22–24]. The results are gray images of
and temperature, and the control system. These are presented the weld pool and derived temperature field images, Fig. 7.
individually below, except for the welding robot (a common In combination with the solidification temperature, the melt
kuka robot). pool area can also be derived from the images.

2.1.1 Visual detection of the melt pool size 2.1.2 Control of the weld pool area
and temperature
Fig. 8 shows the experimental setup and the list of compo-
The determination of the melt pool expansion and the tem- nents and used process variables. A hollow cylinder with a
perature is the basis for a local adjustment of the mechanical diameter of 120 mm was manufactured for the initial study.
properties. Only on this basis is it possible to develop a con- The process variables were chosen to give the control system
trol system for specific heat input as a function of heat dis- a sufficiently wide range of possible adjustments. In addition
sipation. The system presented below is based on work that to the melt pool, the temperature in front of the weld pool and
has already been published [22–24]. A two-color pyrometer the interpass temperature were measured using a conventional
measures the temperature of an object via the ratio of the pyrometer. In this way, rising interpass temperatures can be
light emission of several wavelength ranges. These wave- compensated or the process can be set on hold when the inter-
lengths are used as reference points. Under the condition pass temperature exceeds certain limits to assure a stable and
that the object behaves like a black or gray radiator at the controllable process. The mechanism for interpass control is

Fig. 5  Result of the measure-


ment of the spectrum from
530 to 1000 nm with possible
wavelengths λ1 and λ2 for the
ratio pyrometer [22]

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Welding in the World (2024) 68:247–257 251

Fig. 6  Optical setup of the ratio


pyrometer. The two beams in
blue and red represent the imag-
ing paths of two points in the
weld pool on the cameras [22]

Fig. 7  Captured gray images,


resulting temperature field and
measured weld pool area [22]

Fig. 8  Experimental setup [38]

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described in further detail in [37]. The limits of the manu-


facturing process must be taken into account as additional
nonlinearities. It is possible to reduce the energy input over
a sufficiently large range without reaching the process limit
and without introducing nonlinearity. The fabrication of the
cylinder was chosen to have a stable observation on one point,
without any influences of changing the direction of welding
and/or observation. This allows a longer welding time without
additional ignition processes. Interruptions in the production
process led to the complex interrelationships of material and
energy input already mentioned and are therefore avoided. A
detailed description of the possibilities and the operation of
the system is given in [38].
The melt pool area can be used as the controlled variable.
The aim of the control system developed is to keep the melt Fig. 9  Typical weld metal microstructure of the filler (Le Pera etch-
ant) [39, 40]
pool area as constant as possible at a given set point. Initially,
only the wire feed rate was used as a setting variable. In further
work, the system will also take into account other manipulated 5.7s + 1
K(s) = (1)
variables, such as arc voltage correction and welding speed. 1.9s

2.2 Material and initial welding conditions


2.3 Microstructural characterization
A low-alloy filler metal (DIN EN ISO 14341-A G 50 7 M21
4Mo / A5.28 ER80S-D2) using an M21 shielding gas (82% Ar, Following the welding tests, the additively manufactured
18% ­CO2) was selected as the material for the investigations. hollow cylinders are cut, and the cross-section of the small
The chemical composition is shown in Table 1. The substrate and large bead parts is made, Fig. 11. These were then
for the tests was 14-mm-thick plates of S355. embedded in a polymer, abraded, and polished. The final
The typical microstructure in single pass welds of this filler polishing was performed with a grain size of less than 1 μm
consists of acicular ferrite and grain boundary ferrite, Fig. 9 in the lapping suspension. When grinding, care was taken to
[39, 40]. ensure that the area affected by cutting was reliably removed.
In the presented results, the possibility of locally achieving Subsequently, the samples were etched with Nital. The
two different microstructures will be demonstrated by setting microstructure images were taken after preparation of the
two different set points of the wire feed speed. The first one for samples with a Leica CTR-6000 reflected light microscope
a “small” weld bead with a wire feed speed of 4.5 m/min (heat at different magnifications. Hardness testing was performed
input ca. 330 J/mm) and the second one a “large” weld bead in accordance with ISO 6507. A line of microindentations
with a wire feed speed of approximately 5.4 m/min (heat input was made to determine the average hardness distributed over
ca. 400 J/mm). The set points were synchronized with the rota- the cross-section.
tion of the substrate to match the same position in every layer,
Fig. 11. In a second step, the control loop was closed, and the
targeted weld pool area was set to 90 mm². The design and
boundary conditions of the controller have been described in 3 Results
[37, 38]. There, it is shown that the controlled system can be
described as a quasi-linear system with a static nonlinearity Fig. 11 shows one of the sample geometries. The surface is
and can be described using a Hammerstein model. The block uneven, typical of WAAM-made samples. The width of the
diagram of the controlled system is given in Fig. 10. layers between the small and large beads are slightly dif-
The identification and design of the system leads to a ferent. The difference in width deviates between 0.2 and 1
controller variable K of: mm. Especially in the upper layers, the difference between

Table 1  Chemical composition Filler Contents by mass in %


of the filler
DIN ISO 16834- A C Si Mn Cr Ni Mo Cu Ti V

G 50 7 M21 4Mo 0.07 0.59 1.56 0.09 0.06 0.45 0.12 0.001 0.008

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Welding in the World (2024) 68:247–257 253

Fig. 10  Block diagram of the


closed loop control for the
manufacturing process using the
Hammerstein structure [38]

Fig. 9. Typically, this filler forms acicular ferrite with small


amounts of grain boundary ferrite in single pass welds.
Looking at the two heat inputs, there are clear differ-
ences in the microstructure in the top layer with regard to
the amount of grain boundary ferrite and the grain size of
the accicular ferrite. The microstructure from the area with
higher energy input, i.e., the larger the weld pool is, the
coarser the microstructure. This corresponds to the cur-
rent state of knowledge on the behavior of this group of
materials.
The coarser structure due to the increased energy input
also continues in the other two identified microstructural
areas. Below the top layers, the accicular ferrite initially
dissolves, and globular ferrite or bainite is formed. This
dissolution increases towards the bottom layers due to the
Fig. 11  Manufactured cylinder with changing process variables
more frequent reheating, culminating in a ferritic-pearlitic
microstructure in the third zone in the high-energy input
the two parts increases due to the different heat input to heat region with significantly larger grains than the low-energy
dissipation ratios. input, Fig. 13. In the case of a lower energy input, a ferritic-
This change in the geometry leads to the assumption that bainitic microstructure forms, Fig. 14.
a different cooling behavior has been reached and that the In summary, it can be concluded that the formation of the
microstructure should be significantly different. microstructure corresponds to the current state of knowledge
[16, 41–45]. Moreover, the small difference in energy input
3.1 Microstructure leads to significant changes in the microstructure morphol-
ogy. This is especially true in regions with a high number
The microstructure of approx. the 30-mm high hollow cyl- of reheating events.
inder wall structures can be subdivided into four different
zones, Fig. 12. The bottom layer, which is just above the 3.2 Hardness
substrate, will not be discussed in detail in this paper due to
the relatively large heat conduction compared to the wall- Figure 15 shows the distribution of the hardness over the
like structure in higher layers and the dilution with the base cross-section of the additively manufactured material. The
material. A microstructure typical of multilayer welds can different microstructures in the specimen result in different
be seen in the bottom layers. hardnesses of the material. First, a reduction from the top to
Fig. 12 shows an overview of the cross-sections of two the middle of the specimen can be seen. This is due to the
different heat inputs. In addition, Fig. 12 shows an over- dissolution of the ferritic ferrite and the formation of ferritic-
view of the resulting different microstructures of the four perlitic or ferritic-bainitic microstructures. From the middle
zones. In the upper zone, the microstructure is typical for to the bottom, the hardness then increases again due to the
a single-layer weld or cover layer typical of this filler, cf. increased amount of bainite or perlite formed.

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254 Welding in the World (2024) 68:247–257

Fig. 12  Microstructure comparison of three different zones and two heat inputs

Fig. 13  Microstructure comparison of the most reheated region for two heat inputs

Furthermore, due to different heat inputs, on average, the the cross-section of the sample geometry with and without
hardness at the low-energy input side is approx. 20HV0.1 the control loop activated. Due to the closed control loop,
above the high energy input side. This behavior was also a reduction in the surface waviness and a reduction in the
expected and is in line with the current state of research deviation of the width of the specimen can be achieved.
[15, 16]. Furthermore, it can be seen that due to the closed control
loop, the width of the component is almost constant over
3.3 Closed‑loop control the entire height.
Figure 17 shows the area of the weld pool, the welding
By closing the control loop and thereby regulating the melt power used and the interpass temperature during the tests. A
pool size to approx. 90 mm², the effects of an increasing hollow cylinder with 30 layers was produced in each case, and
interpass temperature on the geometry expression could be manufacturing one layer took 40 s The closed-loop controller
significantly reduced. Fig. 16 shows the comparison between with integral behavior reduces the welding power to 5% as the

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Welding in the World (2024) 68:247–257 255

Fig. 14  Microstructure comparison of the most reheated region for two heat inputs, SEM images

Fig. 15  Hardness distribution within the additive-manufactured steel

interpass temperature rises, and after 20 to 25 layers, constant


temperatures are reached. Furthermore, the closed control loop
allows the weld pool area to be kept constant. Without closed-
loop control, this is not the case. To keep the area of the weld
pool constant, the welding power must be reduced. This also
lowers the measured interpass temperature.

4 Summary and outlook

The presented work reviews the first realization of a system


Fig. 16  Sectional view of the manufactured parts with open-loop for property-oriented arc-based additive manufacturing and
(left) and closed-loop (right) control. The red-dashed line shows the
measurement points of the micro-identification to determine the hard- shows the implementation on a first simple example. The
ness distribution [38] implementation of the system includes the following:

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256 Welding in the World (2024) 68:247–257

Fig. 17  Comparison of distur-


bance response for open-loop
(black) and closed-loop (blue)
control [38]

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