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Atmospheric Environment: X 2 (2019) 100014

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Atmospheric Environment: X
journal homepage: www.journals.elsevier.com/atmospheric-environment-x

Road dust load dynamics and influencing factors for six winter seasons in T
Stockholm, Sweden
Mats Gustafssona,∗, Göran Blomqvista, Ida Järlskoga, Joacim Lundberga, Sara Janhällb,
Max Elmgrenc, Christer Johanssonc,d, Michael Normanc, Sanna Silvergrenc
a
Swedish National Road and Transport Research Institute (VTI), Linköping, SE, 581 95, Sweden
b
Research Institutes of Sweden (RISE), Box 857, Borås, SE, 501 15, Sweden
c
SLB-analys, Box 8136, Stockholm, SE, 104 20, Sweden
d
Department of Environmental Science and Analytical Chemistry (ACES), Stockholm University, Stockholm, SE, 106 91, Sweden

H I GH L IG H T S

• There is a seasonal dependency in road dust loads in Stockholm.


• The lateral road dust load variation is high.
• Road dust load is depending on road surface properties.
• Repaving of a street resulted in markedly increased dust loads.
• The wet dust sampler (WDS) is a useful tool for total dust load follow-up studies.

A R T I C LE I N FO A B S T R A C T

Keywords: Traffic related non-exhaust particulate sources and road dust are an increasingly important source for PM10 air
Non-exhaust pollution as exhaust sources are decreasing due to regulations. In the Nordic countries, the road dust problem is
sampling enhanced by use of studded tyres, causing increased road wear and winter road maintenance including gritting.
Spatial variation Efforts to reduce road dust emissions requires knowledge on temporal and spatial road dust load dynamics. The
Temporal variation
city of Stockholm, Sweden, has therefore financed seasonal (October to May) road dust sampling to be able to
Macro texture
optimize their winter and spring time street operation measures for reduced road dust emissions. This work
PM10
describes the outcome of six seasons (2011/2012–2016/2017) of road dust sampling in five central streets using
the VTI wet dust sampler (WDS).The results show that road dust load, expressed as DL180 (dust load smaller
than 180 μm) has a seasonal variation with the highest loads (up to 200 g/m2) in late winter and early spring and
a minimum (down to about 15 g/m2) in early autumn and late spring. The dust load varies between streets and is
depending on pavement surface properties. On a smaller scale the dust load has a high variability across streets
due to differences in rates of suspension from different parts of the road surface, with low amounts in wheel
tracks and higher in-between and outside the tracks. Between 2 and 30% of the DL180 is smaller than 10 μm and
could directly contribute to PM10 emissions. In general, higher road surface texture leads to higher dust loads,
but the condition of the pavement (e.g. cracks, aggregate loss) might also have an effect. A new, wear resistant
pavement accumulated markedly higher road dust amounts than a several years old pavement. This paper closes
with a discussion on the complex relation between road dust load and PM10 concentrations and a discussion on
the challenges and comparability of road dust sampling techniques and measures.

1. Background pavement wear, are subject to few international regulations (Amato


et al., 2014b; Denier van der Gon et al., 2012). Non-exhaust emissions
Non-exhaust particles from road traffic have been noticed as an will also be important in the future even if the vehicle fleet would be
increasingly important source to air pollution, since traffic globally is completely electrified (Timmers and Achten, 2016). Except from being
increasing and emissions from non-exhaust sources, like tyre, break and emitted directly to the air, non-exhaust particles deposit and


Corresponding author. , VTI, Linköping, SE, 581 95, Sweden.
E-mail address: mats.gustafsson@vti.se (M. Gustafsson).

https://doi.org/10.1016/j.aeaoa.2019.100014
Received 18 September 2018; Received in revised form 18 January 2019; Accepted 21 January 2019
Available online 30 January 2019
2590-1621/ © 2019 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY license
(http://creativecommons.org/licenses/BY/4.0/).
M. Gustafsson et al. Atmospheric Environment: X 2 (2019) 100014

accumulate, together with dust from other sources, on road surfaces to concentrations in short term studies. Combined with water flushing,
form road dust. The dust is suspended by traffic and/or wind and sweeping has a better reduction potential. The few studies on using dust
contributes to air pollution. The sources to road dust differ widely both binding agents on paved roads generally showed a high potential for
geographically and temporally (Amato et al., 2012, 2014a, 2014b; Chen short term PM10 reduction. Especially in cool climates, dust binding
et al., 2012; Etyemezian et al., 2003; Fujiwara et al., 2011; Kuhns et al., seems to be effective. For instance, Norman and Johansson (2006)
2005; Pirjola et al., 2010; Zhu et al., 2008). Common traffic generated showed that PM10 in a Stockholm street could be decreased by up to
sources are, as mentioned, brake and tyre wear particles (Denier van 35% using CMA (calcium magnesium acetate). Gustafsson et al. (2010)
der Gon et al., 2012; Garg et al., 2000; Gietl et al., 2010; Grigoratos and showed similar results also for MgCl2, CaCl2 and sugar solutions.
Martini, 2014; Hulskotte et al., 2007; Lee et al., 2013; Panko et al., Amato et al. (2014c), on the other hand, showed that dust binding of
2013; Sanders et al., 2003). Road operation measures (traction sanding, paved roads in warm climates, are not effective. In the study made in
salting) and pavement wear from studded tyres are also common Barcelona, neither CMA nor MgCl2, could be shown to have a sig-
sources and in some Northern countries during the winter season nificant effect. The authors concluded that the rapid drying-up of che-
(Gustafsson et al., 2009; Kupiainen and Tervahattu, 2004; Kupiainen mical dust binders in high temperatures and the low amounts of road
et al., 2016; Kupiainen and Pirjola, 2011). . Traction sanding can dust accumulated were important factor influencing the results.
contribute both by containing and being ground into fine, suspendible The city of Stockholm has the most abundant PM10 problems
dust, but also through contribution to pavement wear through a among Swedish cities and there is epidemiological evidence that
grinding effect on pavements. This is referred to as the sand paper effect especially the coarse fraction of PM10 is significantly associated with
(Kupiainen et al., 2003). Dust from surrounding areas, like farm land, both mortality and morbidity of the population (Meister et al., 2012). In
deserts, building sites and gravel roads all differ widely depending on 2005, an abatement plan to reach the EU limit values was adopted that
geography, climate and time of year. included specific abatement measures (Länsstyrelsen i Stockholms län,
Since road dust accumulates on the road surface, the surface prop- 2004) against road dust and its’ suspension. Use of CMA as dust binder
erties are important for subsequent emissions. Road dust accumulation and extra sweeping with a special vacuum sweeper operating without
depends mainly on surface macro texture (commonly Mean Texture water application are the main road dust mitigation measures together
Depth, MTD, or Mean Profile Depth, MPD) that affects both the amount with a ban of studded tyres on certain streets (Norman and Johansson,
of dust accumulated and how available this dust is for suspension by 2006; Norman et al., 2016). To follow up the effects of the Stockholm
traffic. Studies by China and James (2012) and Blomqvist et al. (2013) dust mitigation measures, the changes in road dust load during the
show that for the same dust load and suspension force, a coarser macro winter season have been studied. This paper summarises the results and
texture (expressed as MTD) will emit lower amounts of suspended experiences during the first five seasons of this work.
particles. Studying the total amount of accumulated dust below 180 μm
(DL180) in the surface texture, Blomqvist et al. (2013), showed that, in 2. Methodology
real city street environments (in Stockholm, Sweden), DL180 generally
increased with increasing macro texture. In a real road environment, 2.1. Site description
the volume, composition and speed of the traffic, as well as meteor-
ological factors, will influence the accumulation and suspension (Denby Stockholm is situated close to the Swedish Baltic coast where the
et al., 2013a; Denby et al., 2013b; Norman et al., 2016). Simulta- lake Mälaren connects to the Baltic sea (59°19′46″N 18°4′7″E). It has a
neously, these factors will also influence the source strength of non- humid continental climate with distinct seasons, including cold, snowy
exhaust, as well as exhaust, particles, and the resulting dust load will be periods in winter. The number of inhabitants is about 950 000
the result from a balance between accumulation and suspension. A (Stockholms stad, 2017).
crucial meteorological factor is road surface moisture, which has been Road dust load was sampled at, or in close proximity to air quality
proven to strongly affect the emission of dust (Denby et al., 2013a; monitoring stations in the Stockholm city centre (Fig. 1). The streets
Johansson et al., 2007). In Stockholm, Sweden, where PM10 levels are have different characteristics (Table 1); Hornsgatan, Sveavägen, Folk-
strongly influenced by road dust emissions, an almost perfect anti- ungagatan and Odengatan have four lanes (two in each direction),
correlation can be seen with road surface moisture (Norman and Fleminggatan two lanes (one in each direction), Norrlandsgatan two
Johansson, 2006). Suspension of dust is strongly reduced on moist lanes in the same direction. The traffic amounts were 5467–23 800
streets. In the NORTRIP (NOn-exhaust Road Traffic Induced Particle) vehicles per day and the pavements are stone mastic asphalts (SMA)
emission model, developed as a physically based non-exhaust particle with generally wear resistant rocks such as quartzite, granite and por-
emission model, special efforts have therefore been made to describe phyry, with varying maximum aggregate sizes (11–16 mm). Four sites
and account for road surface moisture (Denby et al., 2013a). (Sveavägen 59, Hornsgatan, Folkungagatan and Norrlandsgatan) were
In Sweden, road dust related PM10 is an important cause for ex- used during all years, Sveavägen 83 from spring 2013, Fleminggatan in
ceedances of the EU limit values (Areskoug et al., 2001). Mainly, con- spring 2013 and from autumn 2015 to spring 2017 and finally Oden-
fined city streets with high traffic amounts have had problems reducing gatan from autumn 2013 to spring 2015. All sites have 4–5 story
the PM10 concentrations. As a result of these findings, research was buildings on both sides of the road but have different street canyon
directed towards understanding the emission processes and how to widths.
abate them. In laboratory experiments, Gustafsson et al. (2009) con-
cluded that studded tyres produced tens of times higher PM10 emis- 2.2. Road dust load sampling and analyses
sions than non-studded winter tyres. In parallel, research in Norway
and Finland pointed out studded tyres and winter sanding as important Road dust load was sampled using the VTI Wet Dust Sampler (WDS,
sources (Kupiainen, 2007; Snilsberg, 2008). As a result of this scientific Fig. 2, Jonsson et al., 2008; Lundberg et al., 2019), which is a sampler
evidence, abatement measures in the Nordic countries have been using high pressurized water to clean a small circular road surface area
focussing on how to reduce PM10 emissions from road dust. These in- during a specified time and compressed air to move the sample from the
clude e.g. reduced use of studded tyres, reduced speed, improved road washing unit to a sample bottle. Each washing is referred to as a “shot”.
sweeping and dust binding. The washing unit uses a spray nozzle with a filled cone spray pattern to
Few studies have investigated the influence of road operational thoroughly clean the surface. Two sampling strategies were used: either
measures on PM10 emissions. Amato et al. (2010) made a review of the six “shots” were collected in one large bottle as one sample to even out
effects of sweeping and concluded that, even though literature was variation at short distances of the road, or each “shot” was collected
scarse, road sweeping alone had not been shown to reduce PM10 individually. The six-shot samples were collected three after one

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Fig. 1. Central Stockholm with investigated streets. White dots indicate positions of air quality monitoring stations.

Table 1 from streets including road dust and other non-exhaust particles, road
Description of the measurement sites. dust load is defined as road dust finer than 200 μm, i.e. close to the
Street Traffic # of Textureb Direction Pavement type
180 μm chosen for sample sieving. The samples were then filtered using
(ADT)a lanes (MTD, mm) (main) Buchner funnels with Munktell 00H filter paper. The filters were burned
at 550 °C and the inorganic amount of the sample determined. The dust
Hornsgatan 23 800 4 1.5/2 E-W SMA16 load is called DL180, being the inorganic fraction of dust smaller than
Sveavägen 59 23 400 4 1.3/1.1 NeS SMA11
180 μm. One of three bottles sampled between wheel tracks were used
Sveavägen 83 18 068 4 – NeS SMA11
Folkungagatan 15 100 4 1.7/1 E-W SMA11 for out-takes to size distribution analyses using a laser granulometer
Fleminggatan 19 100 2 – E-W SMA (Between, 2011 and 2014 a CILAS and between 2014 and 2017 a
Norrlandsgatan 7600 2 1.2/0.9 NeS SMA Malvern Mastersizer 2000). From the cumulative size distribution, the
Odengatan 5467 4 – E-W SMA
fraction of DL180 being smaller than 10 μm can be calculated (DL10).
a DL10 might be of closer interest when comparing dust load to PM10
Vehicles per day, Data from 2014.
b
Wheel track/between wheel tracks. concentrations.
Sampling in and between wheel tracks was performed at 6–8 oc-
another at two distances from the road side, in the left wheel track (WT) casions each winter season, normally between October and May, when
and between wheel tracks (BWT), see Fig. 3. This strategy was com- the extra PM10 road operations were in practise. Transects of single
bined with sampling individual “shots” to get a picture of the lateral shots was performed occasionally during the measurement period.
distribution of road dust, consisting of a transect of single shot samples
from the curb across the parking area or cycle path and across the
2.3. Macro texture – sand patch
rightmost driving lane (Fig. 3).
The WDS has been used in several Swedish national research pro-
The road surface macro texture, as an indication of the road surface
jects, mainly for investigating the influence on different street and road
ability to store dust, was measured using the volumetric, contact
operation measures against road dust emissions (Gustafsson et al.,
method commonly known as the sand patch method (EN
2011, 2012, 2014, 2015, 2016, 2017; Janhäll et al., 2016; Järlskog
13036–1:2010). A pre-defined amount of fine glass beads (90% be-
et al., 2017), and has recently been exported to Finland and Norway
tween 180 and 250 μm according to ISO565) is placed in the middle of
which will increase the availability of comparative studies.
the surface of interest and spread out into a circle shape using a hard
Even though the WDS sampler has a theoretical maximum cut-off at
rubber puck until it cannot be further spread. The diameter of the circle
5 mm, which is the diameter of the outlet from the sampling chamber,
is measured in four equally spaced directions and a mean value cal-
particles of that size on the road surface are not directly relevant for air
culated and used to further calculate the mean texture depth (MTD).
quality. From standard sieving methods the mesh of 180 μm was chosen
The method is operator sensitive. For this reason, the same person
for analysis as it removes the larger particles from the sample reducing
performed all measurements.
variability due to few large particles that is large enough not to be
MTD was measured in left wheel track and between wheel tracks on
emitted to the air, but still include most particles that would affect air
the four streets Hornsgatan, Folkungagatan, Sveavägen and
quality even at shorter distances from the road. The NORTRIP-model
Norrlandsgatan in spring 2012. This is the period in Sweden when
(Denby et al., 2013a,b), developed to calculate the PM10 contribution
macro texture is normally highest, after the winter when studded tyres

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Fig. 2. The VTI wet dust sampler (WDS II). Front view (left) and sampling in a city street (right).

During each winter season (September–May) the pattern is similar


on all streets; low road dust loads in the beginning and at the end of the
season and obvious peaks from midwinter to early spring. Maximum
values of DL180 on different streets vary between 15 and around 200 g/
m2. The difference between WT and BWT differs between streets. On
Hornsgatan, Sveavägen and Fleminggatan, DL180 is generally lower in
WT than between, while Norrlandsgatan and Odengatan have very si-
milar dust loads in both surfaces. Folkungagatan has similar dust loads
some seasons and tendencies to higher dust load in WT in other seasons.
The difference in dust load in WT in Folkungagatan between the
first season and the following seasons is due to the above-mentioned
change in sampling area. Another feature at Folkungagatan is the
marked increase in DL180 during the last season (2016–2017). This is
due to repaving the street with a wear resistant stone mastic asphalt
containing porphyry rock aggregates, but also with a coarse macro
texture (determined by visual inspection) with high capacity to store
dust.
Fig. 3. Used WDS sampling alternatives. Sampling three large bottles in left Long term trends in the data differ from street to street, but the
wheel track (WT1–3) and in-between wheel tracks (BWT1–3) and a profile from Sveavägen sites and Hornsgatan seem to have increasing dust amounts
the kerb over the first driving lane (bottom line of dots). since 2014. Both Sveavägen sites show increasing dust amounts in both
WT and BWT. In Hornsgatan, WT seems unaffected, while BWT in-
are used. During summer and early autumn, texture decreases as non- creases. In Norrlandsgatan, the trend is less obvious.
studded tyres polish the surface (Jacobson, 2005). Data is lacking from A statistical view of the data (Fig. 6) from each surface reveal that
Fleminggatan, Odengatan and from the new pavement laid on Folk- WT of Fleminggatan, Norrlandsgatan and Sveavägen, together with
ungagatan in 2016. BWT on Norrlandsgatan have similarly low dust loads, with small
variation, while WT on Hornsgatan as well as BWT on Fleminggatan
and Hornsgatan stands out with high dust loads and large variability.
3. Results Folkungagatan DL180 data must be separated in time, since the sam-
pling site was changed, and a new pavement was built in summer 2016
3.1. Road dust annual cycle and variation between streets on the site as mentioned above (Fig. 6).

Road dust load (DL180) is highly variable in time and space. In


Fig. 4, the mean values of seven locations in WT and BWT during six 3.2. Small scale spatial road dust variability
winter seasons are shown. DL180 is generally highest from mid-winter
to early spring and lowest in early autumn and late spring. Separated Not only does the dust load vary between streets and during the
into street locations and seasons (Fig. 5), the highest dust loads were season, the small-scale variation across a street can also be very high. In
measured between wheel tracks on Hornsgatan and in wheel track on Fig. 7, ten WDS transects, sampled 2 h and about 20 cm apart at Fle-
Folkungagatan during the first season of measurements (2011–2012). minggatan, have been used to illustrate the variation in dust load. In the
Comparing the pavements revealed that these specific surfaces were driving lane the wheel tracks are easily identified as even surfaces with
more damaged (mainly cracks and aggregate losses) than other sur- low dust load (below 50 g/m2). Between wheel tracks and between the
faces. Therefore, the tests were moved to undamaged parts of the same lanes are areas with higher dust loads, about 50–100 g/m2. Outside the
pavements the following seasons. lane, towards the kerb, the gradient is steep to high dust loads in the

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Fig. 4. Mean road dust load (DL180) in WT and BTW for seven locations in central Stockholm between 2011 and 2017. Error bars are standards deviations.

bicycle lane and parking area, up to about 300 g/m2. The large varia- has a seasonal pattern with lower amounts in early autumn and late
tion in the x direction outside the driving lane can both relate to tem- spring and a maximum in midwinter and early spring and range from
poral variation and to small-scale differences between the transects. about 20 mg/m2 in the generally low dust load in September to almost
Since WDS cleans each sampling surface, the exact same surface cannot 90 g/m2 during the dustiest period in March.
be re-used in the following transect but have been moved up-stream to
the traffic, not to be affected by water smearing by traffic. 3.3.1. Macro texture influence on dust load
In Fig. 10, macro texture (MTD) in and between wheel tracks on
3.3. Size distributions and amount of dust < 10 μm four streets have been plotted to road dust load (DL180) for six winter
seasons from 2011 to 2017. Even though other factors affect the dust
The fraction of road dust being smaller than 10 μm (DL10) is of load, like traffic amount, speed and composition, meteorology and
interest since it can be expected to contribute directly to airborne PM10 different suspension in and between wheel tracks, there is a clear ten-
through suspension. In Fig. 8, cumulative size distributions of DL180 dency that coarser texture is related to higher dust load. Except for the
sampled on 2017-02-02 is shown. These distributions are typical for the exceptionally coarse macro texture in the Folkungagatan wheel track
high road dust load season and the shape is generally similar between (over 2 mm), the macro texture in wheel tracks are lower than between
streets. Nevertheless, the percentage smaller than 10 μm can be quite wheel tracks. Within each functional section (in and between wheel
different. In Table 2, the percentage for the streets in Fig. 8 is shown tracks) there is also a trend with higher dust load at coarser macro
and range from 14 to 18% of DL180. In all BTW samples during the six texture. The new pavement at Folkungagatan (from mid-2016) is not
seasons, the percentage range from 2 to 30%, with a mean value of included in the figure due to lack of macro texture data. Visually, it has
14%. The percentage of DL10 is generally higher in winter and early a high texture, which also is reflected in high dust loads (see Fig. 5).
spring. One should keep in mind that texture was only measured once at each
Mean values of DL10 in BWT between the seasons 2011–2017 is site. Therefore, the variation along the MTD axis in Fig. 10 would likely
shown in Fig. 9. Similar to the DL180 load, the DL10 fraction generally be higher if texture was available for each measurement occasion.

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Fig. 5. Road dust load (DL180) variation during September to May between 2011 and 2017 in seven locations on Stockholm streets.

Measurements in wheel track on roads with similar pavement but Dry road dust sampling methods have shown an inverse relationship
higher speeds indicate that macro texture might vary with about 10% between macro texture (MTD) and suspendible dust load (Blomqvist
over a year, with the highest values after the studded tyre season and et al., 2013; China and James, 2012; Panko et al., 2013; Padoan et al.,
the lowest just before (Lundberg, 2012). Pavements at the measurement 2018) which is a result of a higher capacity to store and retain dust at
sites were not changed during these years, though, why texture values coarser macro textures. Even though only visual observations are
are likely to be representative. available for the texture of the new pavement on Folkungagatan, the
obvious increase in dust load has been followed by a likewise obvious
drop in PM10 concentrations at the site. This indicates a reduced sus-
4. Discussion
pendible road dust emission, even though traffic increased during the
same period. On the other hand, the mean speed in the lane decreased
Based on available literature, the data set on both annual cycles of
by 7 km/h due to a new bus stop (Elmgren, 2018). A high dust load can
road dust load and the road dust cross-sections presented in this work
reflect strong sources, which is likely not the case with the wear re-
are unique data sets. The annual cycle is a result of growing dust
sistant porphyry pavement on Folkungagatan, but also low suspension,
sources as well as increasing dust retention processes during autumn
which is promoted by coarse texture and low suspension forces. In
and winter. In spring the opposite circumstances reduce the dust load.
Folkungagatan, dust sources should be comparably weak, while texture
Generally, dust load is higher between wheel tracks, than in wheel
is deep and the suspension likely to be lower due to lower traffic speed
track, which is a result of the suspension caused by passing wheels. This
than before the traffic shift. Weak sources causing slow accumulation in
difference is especially obvious in Fleminggatan, due to track bound
a rough texture with low suspension from traffic could therefore be
traffic in one single narrow lane with a no-crossing line to the left and a
hypothesized to explain the combination of high dust load and low
bicycle lane to the right. Remaining streets have two lanes in each di-
PM10 on Folkungagatan. Of the total dust load sampled, the fixed dust
rection, resulting in more lane shifting that will affect the distribution
load is high, while the suspendible load is low.
of dust across the street. Norrlandsgatan is the street with least differ-
The WDS sampling in this study samples both suspendible and fixed
ences in and between wheel tracks, probably resulting from being a
dust load, i.e. the total dust load. At a certain location with a site-
short link were cars often shift lanes at low speeds before a crossing
specific pavement surface macro texture and traffic conditions, the
with traffic lights. The size distribution of DL180 is generally rather
fixed load is likely to have a small variation, which was shown by China
similar between streets. Therefore, DL180 dust load is reflected in the
and James (2012). The results of this study, showing that the total dust
DL10 dust load.
load increases with coarser macro texture, could be explained by as-
The influence of macro texture of the pavement on road dust load is
suming that of the dust supplied to the surface, a higher proportion will
obvious, with generally higher dust loads with coarser macro texture.

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Fig. 6. Statistics for each surface 2011–2017. Plots show median, lower quartile, upper quartile, maximum and minimum values. The three rightmost bars in each
figure show statistics for surfaces on Folkungagatan, where the sampling site and the pavement have been changed. In 2011–2012, the WT site was damaged with lost
aggregates and cracks, in 2012–2016 both surfaces were in good condition and in 2016–2017 the street got a new pavement with higher macro texture.

become fixed with increasing texture depth. The suspendible dust load conditions is mostly direct wear from pavement and tyres. Dust accu-
is influenced by direct action and turbulence from wheels and vehicles. mulation will occur when wheel tracks are humid (Amato et al., 2012)
The traffic characteristics (speed, amount, composition) in a street is and will result in suspension of dust at dry-up. In-between wheel tracks
therefore governing the maximum suspension depth. The fixed load is suspension from vehicle turbulence will be the dominant emission
influenced by deposition and compaction and its upper level de- process. The traffic intensity and speed in the street will affect the
termined by the suspension depth. Since turbulent forces decrease ra- amount remaining on the surface. Amato et al. (2017) showed that the
pidly from the surface, the assumption that the proportion of dust that suspendible dust load will decrease with increasing traffic intensity and
is fixed will increase faster is reasonable, but still a speculation. A hy- that the relationship levelled out already at 1500 vehicles per lane and
pothetic model of this reasoning is described in Fig. 11. day. This relation might well be site specific, though, depending on
The cross-street dust load variability described in this work shows road surface and traffic properties.
that wheels, also at rather low speeds (30–50 km/h) in the central city, The dust load is expressed as DL180, meaning the surface con-
are effective dust suspenders. Wheel tracks generally have low dust centration of dust smaller than 180 μm. The only directly comparable
loads. It can be argued that the emission from these surfaces during dry results are from the similar Chinese version of the WDS. This WDS is

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Fig. 7. Road dust load from kerb across parking area and driving lane during 21 h. Built from 10 transects with about 2 h apart.

inspired by the VTI WDS used in this paper but differs in some technical Table 2
dimensions and specifications. In Huang et al. (2017), DL180 of Beijing Percentage of DL180 smaller than 10 μm from sampling
streets vary between 28 and 117 g/m2, which is within the range of the 2017-02-02.
dust loads found in Stockholm. The dust sources are partly different in Street < 10 μm (%)
Beijing and Stockholm and there is no information on the pavement and
traffic properties from the Beijing data. Therefore, further comparison Fleminggatan 17
Folkungagatan 18
is not possible.
Hornsgatan 17
The most commonly used dust load unit for similar studies is silt Norrlandsgatan 13
load (sL), based on the method used in the US EPA emission model AP- Sveavägen 83 15
42 (EPA, 2002). Silt load is defined as particles smaller than 75 μm on Sveavägen 59 14
the road surface. Using the cumulative size distributions of DL180, the

Fig. 8. Examples of cumulative (left) and frequency based (right) mass size distributions in DL180 samples from Stockholm streets in 2017–02-02. Percentage used
for DL10 calculation marked with grey.

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Fig. 9. Mean road dust load (DL10) in BWT for seven locations in central Stockholm between 2011 and 2017. Error bars are standard deviations.

fraction closest to silt load (< 76 μm) can be calculated. Silt load for all will sample the mobile dust that is available for the suction force ap-
streets was calculated from DL180 for the season 2015–2016 and ranges plied, which depends on effect of the vacuum cleaner, the nozzle design
from 2.5 to about 250 g/m2, which can be compared to the re- and how the nozzle is operated. It will also be affected by the humidity
commended default silt loading values for public paved roads of AP-42 of the road surface, which is one of the main reasons why the WDS is
of 0.1–3 g/m2. At industrial facilities, AP-42 suggests silt load up to operating with water. In Sweden, humid, wet or even snowy or icy road
400 g/m2 (EPA, 2006). It should be noted though, that the silt load surfaces are common, and a dry method would be hard to apply in
estimation technique used in the AP-42 method, is based on dry many situations. On the other hand, suspending road dust in water will
brushing and vacuuming of the road surface. This technique might not dissolve some particles that might contribute to airborne PM10 and
be as efficient in removing dust from the surface as the high-pressure affect the size distribution of the dust.
water cleaning used in WDS Therefore, silt loads could be expected to If assuming the dry sampler of Amato et al. (2009) collects all
be lower. Also, a part of the explanation for the large differences, is that available road dust PM10, the dust load smaller than 10 μm (DL10)
the US streets that AP-42 is developed for are very different from calculated in this work can be compared to the PM10 dust load. Amato
Swedish streets in winter and spring, where dust sources are likely to be et al. (2013) found that the PM10 dust load was 2–22 mg/m2 de-
much stronger. pending on location. In our data, DL10 range from 21 to 9000 mg/m2,
A similar dry sampling technique as used in AP-42, which has been indicating that the dustiest street in the study by Amato et al. (2013) is
used rather extensively, is the technique developed by Amato et al. similar in dust load to the cleanest street in the current study. Even
(2009). The dust amount sampled by a dry vacuum cleaning method though streets in Nordic conditions are likely to be much dustier due to

Fig. 10. Influence of road surface texture (MTD) on road dust load (DL180) between 2011 and 2017. Note that the new pavement on Folkungagatan is not included,
due to lack of texture data (see text).

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M. Gustafsson et al. Atmospheric Environment: X 2 (2019) 100014

Fig. 11. Hypothetical model of relation between texture, suspendible and fixed dust load.

studded tyres and winter sanding, this comparison should be made with As obvious in the discussion above, there is a need for harmoniza-
caution, since the aerosol PM10 cut-off is likely not directly comparable tion in road dust sampling techniques, what parameters to study and
to the below 10 μm fraction in a cumulative size distribution in water. more knowledge on their influence on air quality and the road dust
Also, it is likely that this difference is partly a result of the difference in system. Road dust load has an obvious influence on air quality, but the
sampling the suspendible fraction (dry method), and the total dust load processes involved are many and the system complex. The currently
(wet method). A factor complicating the comparison between the most comprehensive road dust emission model, NORTRIP (Denby and
DL180 dust load value and dry vacuuming samplers is that the WDS is Sundvor, 2012), describes many of these processes in detail and has
used in the Nordic countries Sweden, Norway and Finland, with high been shown to describe PM10 emission and concentration with rea-
dust loads, while the dry vacuuming samplers are used in mid and sonable to high accuracy (e.g. Denby et al., 2013a,b; Kauhaniemi et al.,
southern Europe, where the dust load is generally lower. An inter- 2014), taking account for meteorology, traffic, surface moisture, pa-
comparison of different samplers in the same streets should be bene- vement wear and road operation measures.
ficial to better understand the differences. All road dust sampling methods have pros and cons and could
In Stockholm, PM10 is monitored in several places using mainly possibly complete each other. Being a young research area, these issues
TEOM (for details see website of SLB-analys: http://www.slb.nu). One will hopefully be addressed in coming years. Road dust is certainly in
might expect PM10 concentrations in the city to be directly depending many environments an important source for PM10 with a complex
on the dust load, but a number of other factors affect this relationship, dependence on source contributions and meteorology as well as road
as described in Fig. 12. Two main sources contribute to road dust surface and traffic properties, resulting in an array of mitigation pos-
emissions: direct emissions from road surface wear and suspension of sibilities in need of a scientific basis for optimal performance.
accumulated dust. The strength of the dust sources increases in late
autumn, as studded tyre frequency increases as do occasions when sand 5. Conclusions
and salt is used for traction control. Simultaneously, the frequency of
wet or humid road surfaces, binding dust to the surface, increases. The From this work is concluded that:
local contribution to PM10 starts to rise in the autumn but is dampened
by the more frequent wet surfaces. Road dust accumulates during these • There is a seasonal dependency in road dust loads in Stockholm,
conditions but as the frequency of wet road surfaces decrease in spring, with a build-up in autumn, maximum loads in mid-winter to early
the accumulated dust starts to be suspended by traffic, causing high spring and low values in late spring and autumn.
PM10 peaks. As the dust sources decrease and the road dust load is • The road dust load, expressed as DL180, varies from about 15 to
depleted, its contribution to PM10 decreases. 200 g/m2.

Fig. 12. Six seasons in Hornsgatan, Stockholm showing dust load (DL180), local contribution to PM10, studded tyre frequency and road surface wetness.

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M. Gustafsson et al. Atmospheric Environment: X 2 (2019) 100014

• The lateral variation is high with typically large dust loads in be- doi.org/10.5194/acp-14-3533-2014.
Amato, F., Cassee, F.R., Denier van der Gon, H.A.C., Gehrig, R., Gustafsson, M., Hafner,
tween and outside wheel tracks and low in wheel tracks.
• The percentage of DL180 which is below 10 μm (DL10) and there-
W., Harrison, R.M., Jozwicka, M., Kelly, F.J., Moreno, T., Prevot, A.S.H., Schaap, M.,
Sunyer, J., Querol, X., 2014b. Urban air quality: the challenge of traffic non-exhaust
fore directly, through suspension, could contribute to PM10, varies emissions. J. Hazard Mater. 275, 31–36. https://doi.org/10.1016/j.jhazmat.2014.04.
from 2 to 30%, with a mean value of 14%. 053.

• In average, DL10 follows the same seasonal cycle as DL180 with


Amato, F., Karanasiou, A., Cordoba, P., Alastuey, A., Moreno, T., Lucarelli, F., Nava, S.,
Calzolai, G., Querol, X., 2014c. Effects of road dust suppressants on PM levels in a
high loads in mid-winter to early spring and low values in late spring mediterranean urban area. Environ. Sci. Technol. 48, 8069–8077. https://doi.org/10.
and autumn. The DL10 percentage of DL180 is generally highest in 1021/es502496s.
Amato, F., Bedogni, M., Padoan, E., Querol, X., Ealo, M., Rivas, I., 2017. Characterization
midwinter and early spring and lower in autumn and late spring. of road dust emissions in Milan: impact of vehicle fleet speed. Aerosol and Air Quality
• Road dust load is depending on road surface properties, where Research 17, 2438–2449. https://doi.org/10.4209/aaqr.2017.01.0017.
higher macro texture increases dust loads. Areskoug, H., Alesand, T., Hansson, H.-C., Hedberg, E., Johansson, C., Vesely, V.,

• Repaving of one of the streets resulted in markedly increased dust Widequist, U., Ekengren, T., 2001. Kartläggning av inandningsbara partiklar i
svenska tätorter och identifikation av de viktigaste källorna, ITM, Luftlaboratoriet.
loads, but also reduced PM10 concentrations, indicating a growth of Stockholm University (in Swedish).
the fixed dust load but a reduction in suspendible dust load due to Blomqvist, G., Gustafsson, M., Lundberg, T., 2013. Road surface dust load is dependent on
high macro texture. road surface macro texture. In: European Aerosol Conference, Prague, Czech


Republic.
A comparison between DL180 and silt load results in that the Chen, J., Wang, W., Liu, H., Ren, L., 2012. Determination of road dust loadings and
Stockholm streets have silt loads comparable to values suggested for chemical characteristics using resuspension. Environ. Monit. Assess. 184, 1693–1709.
industrial sites in AP-42, which is likely a result of more effective https://doi.org/10.1007/s10661-011-2071-1.
China, S., James, D.E., 2012. Influence of pavement macrotexture on PM 10 emissions
sampling using the WDS technique compared to the whisk broom from paved roads: a controlled study. Atmos. Environ. 63, 313–326. https://doi.org/
and dustpan used for silt load sampling as well as a result of large 10.1016/j.atmosenv.2012.09.018.
differences between Swedish and north American dust sources and Denby, B.R., Sundvor, I., 2012. NORTRIP Model Development and Documentation, NILU
Scientific Report OR23.
road conditions. Denby, B.R., Sundvor, I., Johansson, C., Pirjola, L., Ketzel, M., Norman, M., Kupiainen, K.,
• Road dust load is an important source for high PM10 concentrations, Gustafsson, M., Blomqvist, G., Kauhaniemi, M., Omstedt, G., 2013a. A coupled road
dust and surface moisture model to predict non-exhaust road traffic induced particle
but the relation is affected by many factors, the main one being road
emissions (NORTRIP). Part 2: surface moisture and salt impact modelling. Atmos.
surface humidity. The highest PM10 concentrations appear at high Environ. 81, 485–503. https://doi.org/10.1016/j.atmosenv.2013.09.003.
dust loads and dry roads in late winter and early spring. Denby, B.R., Sundvor, I., Johansson, C., Pirjola, L., Ketzel, M., Norman, M., Kupiainen, K.,
• The wet dust sampler (WDS) is a useful tool for total dust load Gustafsson, M., Blomqvist, G., Omstedt, G., 2013b. A coupled road dust and surface
moisture model to predict non-exhaust road traffic induced particle emissions
follow-up studies in most climates and weather conditions and
(NORTRIP). Part 1: road dust loading and suspension modelling. Atmos. Environ. 77,
opens up for a range of sample analyses connected to sources and 283–300. https://doi.org/10.1016/j.atmosenv.2013.04.069.
road operation activities. Sampling of the suspendible fraction re- Denier van der Gon, H., Gerlofs-Nijland, M.E., Gehrig, R., Gustafsson, M., Janssen, N.,
quires other techniques, though. Harrison, R.M., Hulskotte, J., Johansson, C., Jozwicka, M., Keuken, M., Krijgsheld, K.,
Ntziachristos, L., Riediker, M., Cassee, F.R., 2012. The policy relevance of wear
emissions from road Transport, now and in the future - an international workshop
Declaration of interests report and consensus statement. J. Air Waste Manag. Assoc. 63, 136–149. https://doi.
org/10.1080/10962247.2012.741055.
Elmgren, M., 2018. Trafikomläggning Och Ny Hårdare Asfalt På Folkungagatan,
None. Stockholm Mätningar Och Beräkningar Av NO2 Och PM10, SLB 4:2018, SLB-Analys.
http://slb.nu/slb/rapporter/pdf8/slb2018_004.pdf (in Swedish).
Acknowledgements EPA, 2002. AP-42, Fifth Edition, Volume I, Chapter 13: Miscellaneous Sources.
EPA, 2006. AP42 Section 13.2.1 Paved Roads - Update November 2006.
Etyemezian, V., Kuhns, H., Gillies, J., Chow, J., Hendrickson, K., McGown, M., Pitchford,
This work was financed by the Traffic Office of the city of M., 2003. Vehicle-based road dust emission measurement (III): effect of speed, traffic
Stockholm. Development of the WDS was financed by the Swedish volume, location, and season on PM10 road dust emissions in the Treasure Valley, ID.
Atmos. Environ. 37, 4583–4593. https://doi.org/10.1016/S1352-2310(03)00530-2.
Transport Administration and Sweden's innovation agency (VINNOVA).
Fujiwara, F., Rebagliati, R.J., Dawidowski, L., Gómez, D., Polla, G., Pereyra, V.,
The authors would like to acknowledge the PM10-group in Stockholm Smichowski, P., 2011. Spatial and chemical patterns of size fractionated road dust
(Peter Ringkrans, Susanne Pettersson, Tomas Nitzelius and Emma collected in a megacitiy. Atmos. Environ. 45, 1497–1505. https://doi.org/10.1016/j.
atmosenv.2010.12.053.
Nordling) for fruitful discussions and support. We would also like to
Garg, B.D., Cadle, S.H., Mulawa, P.A., Groblicki, P.J., Laroo, C., Parr, G.A., 2000. Brake
thank Håkan Wilhelmsson, Håkan Arvidsson and Tomas Halldin at VTI wear particulate matter emissions. Environ. Sci. Technol. 34, 4463–4469. https://doi.
and Billy Sjövall at SLB-analys for technical and laboratory support as org/10.1021/es001108h.
well as the PEAB staff keeping us safe in the night-time streets of Gietl, J.K., Lawrence, R., Thorpe, A.J., Harrison, R.M., 2010. Identification of brake wear
particles and derivation of a quantitative tracer for brake dust at a major road. Atmos.
Stockholm. Environ. 44, 141–146. https://doi.org/10.1016/j.atmosenv.2009.10.016.
Grigoratos, T., Martini, G., 2014. Non - Exhaust Traffic Related Emissions. Brake and Tyre
References Wear PM. Literature Survey. JRC Science and Policy Reports.
Gustafsson, M., Blomqvist, G., Gudmundsson, A., Dahl, A., Jonsson, P., Swietlicki, E.,
2009. Factors influencing PM10 emissions from road pavement wear. Atmos.
Amato, F., Pandolfi, M., Viana, M., Querol, X., Alastuey, A., Moreno, T., 2009. Spatial and Environ. 43, 4699–4702. https://doi.org/10.1016/j.atmosenv.2008.04.028.
chemical patterns of PM10 in road dust deposited in urban environment. Atmos. Gustafsson, M., Blomqvist, G., Jonsson, P., Ferm, M., 2010. Effekter Av Dammbindning
Environ. 43, 1650–1659. https://doi.org/10.1016/j.atmosenv.2008.12.009. Av Belagda Vägar, VTI Rapport 666. Swedish National Road and Transport Research
Amato, F., Querol, X., Johansson, C., Nagl, C., Alastuey, A., 2010. A review on the ef- Institute (in Swedish). http://urn.kb.se/resolve?urn=urn:nbn:se:vti:diva-6527.
fectiveness of street sweeping, washing and dust suppressants as urban PM control Gustafsson, M., Blomqvist, G., Jonsson, P., 2011. Damningsminimerad Vinter- Och
methods. Sci. Total Environ. 408, 3070–3084. https://doi.org/10.1016/j.scitotenv. Barmarksdrift. Mått, Medel Och Strategier, VTI Rapport 701. Swedish National Road
2010.04.025. and Transport Research Institute (in Swedish). http://urn.kb.se/resolve?urn=
Amato, F., Schaap, M., Denier van der Gon, H.A.C., Pandolfi, M., Alastuey, A., Keuken, urn:nbn:se:vti:diva-1785.
M., Querol, X., 2012. Effect of rain events on the mobility of road dust load in two Gustafsson, M., Blomqvist, G., Johansson, C., Norman, M., 2012. Driftåtgärder Mot PM10
Dutch and Spanish roads. Atmos. Environ. 62, 352–358. https://doi.org/10.1016/j. På Hornsgatan Och Sveavägen I Stockholm - Utvärdering Av Vintersäsongen 2011-
atmosenv.2012.08.042. 2012, VTI Rapport 767. Swedish National Road and Transport Research Institute (in
Amato, F., Schaap, M., Denier van der Gon, H.A.C., Pandolfi, M., Alastuey, A., Keuken, Swedish). http://urn.kb.se/resolve?urn=urn:nbn:se:vti:diva-1847.
M., Querol, X., 2013. Short-term variability of mineral dust, metals and carbon Gustafsson, M., Blomqvist, G., Janhäll, S., Johansson, C., Norman, M., 2014. Driftåtgärder
emission from road dust resuspension. Atmospheric Environment 74, 134–140. Mot PM10 I Stockholm: Utvärdering Av Vintersäsongen 2012–2013, 0347-6030, VTI.
https://doi.org/10.1016/j.atmosenv.2013.03.037. (in Swedish). http://urn.kb.se/resolve?urn=urn:nbn:se:vti:diva-6858.
Amato, F., Alastuey, A., de la Rosa, J., Gonzalez Castanedo, Y., Sánchez de la Campa, Gustafsson, M., Blomqvist, G., Janhäll, S., Johansson, C., Norman, M., 2015. Driftåtgärder
A.M., Pandolfi, M., Lozano, A., Contreras González, J., Querol, X., 2014a. Trends of Mot PM10 I Stockholm: Utvärdering Av Vintersäsongen 2013–2014, 847. Swedish
road dust emissions contributions on ambient air particulate levels at rural, urban National Road and Transport Research Institute (in Swedish). http://urn.kb.se/
and industrial sites in southern Spain. Atmos. Chem. Phys. 14, 3533–3544. https:// resolve?urn=urn:nbn:se:vti:diva-7799.

11
M. Gustafsson et al. Atmospheric Environment: X 2 (2019) 100014

Gustafsson, M., Blomqvist, G., Janhäll, S., Johansson, C., Norman, M., Silvergren, S., Contribution of mineral dust sources to street side ambient and suspension PM10
2016. Driftåtgärder Mot PM10 I Stockholm: Utvärdering Av Vintersäsongen 2014- samples. Atmos. Environ. 147, 178–189. https://doi.org/10.1016/j.atmosenv.2016.
2015, VTI Rapport 897. Swedish National Road and Transport Research Institute (in 09.059.
Swedish). http://urn.kb.se/resolve?urn=urn:nbn:se:vti:diva-10735. Länsstyrelsen i Stockholms län, 2004. Åtgärdsprogram För Att Klara Miljökvalitetsnormen
Gustafsson, M., Blomqvist, G., Janhäll, S., Johansson, C., Järlskog, I., Lundberg, J., För Partiklar I Stockholms Län: Offprint from Stockholm County Administration's
Norman, M., Silvergren, S., 2017. Driftåtgärder Mot PM10 I Stockholm: Utvärdering Report to the Swedish Government. Regeringsuppdrag Redovisat 2004-01-19, Dnr
Av Vintersäsongen 2015–2016, 03476030 (ISSN). Swedish National Road and 1842-02-87078. Swedish National Road and Transport Research Institute (in
Transport Research Institute (in Swedish). http://urn.kb.se/resolve?urn= Swedish). http://urn.kb.se/resolve?urn=urn:nbn:se:vti:diva-5134.
urn:nbn:se:vti:diva-11889. Lee, S., Kwak, J., Kim, H., Lee, J., 2013. Properties of roadway particles from interaction
Huang, Y., Han, K., Li, D., Chen, L., Ren, B., Qin, J., 2017. Characteristic of remaining dust between the tire and road pavement. Int. J. Automot. Technol. 14, 163–173. https://
and wet road dust on city roads in Beijing. Chinese J. Environ. Eng. 11, 4149–4154. doi.org/10.1007/s12239-013-0018-y.
https://doi.org/10.12030/j.cjee.201605171. Lundberg, T., 2012. Kontrollmetod För Nya Vägbeläggningar; Makrotextur, VTI-Notat 35.
Hulskotte, J.H.J., van der Gon, H.A.C.D., Visschedijk, A.J.H., Schaap, M., 2007. Brake VTI- Swedish National Road and Transport Research Institute (in Swedish). http://
wear from vehicles as an important source of diffuse copper pollution. In: Tanik, A., urn.kb.se/resolve?urn=urn:nbn:se:vti:diva-597.
Ozturk, I., Yazgan, M.S., Heath, R. (Eds.), Water Science Technology, pp. 223–231. Lundberg, J., Blomqvist, G., Gustafsson, M., Janhäll, S., Järlskog, I., 2019. Wet Dust
Jacobson, T., 2005. Polering Av Asfaltbeläggning, VTI Notat 12. Swedish National Road Sampler – a Sampling Method for Road Dust Quantification and Analyses.
and Transport Research Institute (in Swedish). http://urn.kb.se/resolve?urn= (Manuscript).
urn:nbn:se:vti:diva-1537. Meister, K., Johansson, C., Forsberg, B., 2012. Estimated short-term effects of coarse
Janhäll, S., Gustafsson, M., Andersson, K., Järlskog, I., Lindström, T., 2016. Utvärdering particles on daily mortality in Stockholm, Sweden. Environ. Health Perspect. 120,
Av Städmaskiners Förmåga Att Reducera Vägdammsförrådet I Gatu- Och 431–436. https://doi.org/10.1289/ehp.1103995.
Tunnelmiljöer I Trondheim, VTI Rapport 883. Swedish National Road and Transport Norman, M., Johansson, C., 2006. Studies of some measures to reduce road dust emissions
Research Institute (in Swedish). http://urn.kb.se/resolve?urn=urn:nbn:se:vti:diva- from paved roads in Scandinavia. Atmos. Environ. 40, 6154–6164. https://doi.org/
8292. 10.1016/j.atmosenv.2006.05.022.
Järlskog, I., Blomqvist, G., Gustafsson, M., Janhäll, S., 2017. Utvärdering Av Norman, M., Sundvor, I., Denby, B.R., Johansson, C., Gustafsson, M., Blomqvist, G.,
Städmaskiners Förmåga Att Reducera Vägdammsförrådet I Gatu- Och Tunnelmiljöer - Janhäll, S., 2016. Modelling road dust emission abatement measures using the
En Fältstudie I Trondheim 2016. Swedish National Road and Transport Research NORTRIP model: vehicle speed and studded tyre reduction. Atmos. Environ. 134,
Institute (in Swedish). http://urn.kb.se/resolve?urn=urn:nbn:se:vti:diva-8292. 96–108. https://doi.org/10.1016/j.atmosenv.2016.03.035.
Johansson, C., Norman, M., Gidhagen, L., 2007. Spatial & temporal variations of PM10 Padoan, E., Ajmone-Marsan, F., Querol, X., Amato, F., 2018. An empirical model to
and particle number concentrations in urban air. Environ. Monit. Assess. 127, predict road dust emissions based on pavement and traffic characteristics. Environ.
477–487. https://doi.org/10.1007/s10661-006-9296-4. Pollut. 237, 713–720. https://doi.org/10.1016/j.envpol.2017.10.115.
Jonsson, P., Blomqvist, G., Gustafsson, M., 2008. Wet Dust Sampler: Technological Panko, J.M., Chu, J., Kreider, M.L., Unice, K.M., 2013. Measurement of airborne con-
Innovation for Sampling Particles and Salt on Road Surface. Seventh International centrations of tire and road wear particles in urban and rural areas of France, Japan,
Symposium on Snow Removal and Ice Control Technology. Transportation Research and the United States. Atmos. Environ. 72, 192. https://doi.org/10.1016/j.atmosenv.
Circular E-C126, pp. 102–111. 2013.01.040.
Kauhaniemi, M., Stojiljkovic, A., Pirjola, L., Karppinen, A., Härkönen, J., Kupiainen, K., Pirjola, L., Johansson, C., Kupiainen, K., Stojiljkovic, A., Karlsson, H., Hussein, T., 2010.
Kangas, L., Aarnio, M.A., Omstedt, G., Denby, B.R., Kukkonen, J., 2014. Comparison Road dust emissions from paved roads measured using different mobile systems. J.
of the predictions of two road dust emission models with the measurements of a Air Waste Manag. Assoc. 60, 1422–1433. https://doi.org/10.3155/1047-3289.60.12.
mobile van. Atmos. Chem. Phys. 14, 9155–9169. https://doi.org/10.5194/acp-14- 1422.
9155-2014. Sanders, P.G., Xu, N., Dalka, T.M., Maricq, M.M., 2003. Airborne brake wear debris: size
Kuhns, H., Gillies, J., Etyemezian, V., Dubois, D., Ahonen, S., Nikolic, D., Durham, C., distributions, composition, and a comparison of dynamometer and vehicle tests.
2005. Spatial variability of unpaved road dust PM10 emission factors near El Paso, Environ. Sci. Technol. 37, 4060–4069. https://doi.org/10.1021/es034145s.
Texas. J. Air Waste Manag. Assoc. 55, 3–12. Snilsberg, B., 2008. Pavement Wear and Airborne Dust Pollution in Norway;
Kupiainen, K., 2007. Road Dust from Pavement Wear and Traction Sanding. Department Characterization of the Physical and Chemical Properties of Dust Particles. Doctoral
of Biological and Environmental Sciences. University of Helsinki, Faculty of Thesis 2008:133. Dept. of Geology and Mineral Resources Engineering. NTNU,
Biosciences, Helsinki, pp. 50. Trondheim, pp. 110.
Kupiainen, K.J., Pirjola, L., 2011. Vehicle non-exhaust emissions from the tyre-road in- Stockholms stad, 2017. Statistik Om Stockholm, Befolkningsöversikt 2017, Årsrapport.
terface - effect of stud properties, traction sanding and resuspension. Atmos. Environ. accessed in August, 2018 (in Swedish). https://statistik.stockholm.se/attachments/
45, 4141–4146. https://doi.org/10.1016/j.atmosenv.2011.05.027. article/188/BefolkningsÃversikt%202017.pdf.
Kupiainen, K., Tervahattu, H., 2004. The effect of traction sanding on urban suspended Timmers, V.R.J.H., Achten, P.A.J., 2016. Non-exhaust PM emissions from electric ve-
particles in Finland. Environ. Monit. Assess. 93, 287–300. https://doi.org/10.1023/ hicles. Atmos. Environ. 134, 10–17. https://doi.org/10.1016/j.atmosenv.2016.03.
B:EMAS.0000016799.19441.0e. 017.
Kupiainen, K., Tervahattu, H., Räisänen, M., 2003. Experimental studies about the impact Zhu, D., Kuhns, H.D., Brown, S., Gillies, J.A., Etyemezian, V., Gertler, A.W., 2008. Spatial
of traction sand on urban road dust composition. Sci. Total Environ. 308, 175–184. and seasonal emissions of road dust in the Lake Tahoe Basin. In: Proceedings of the
https://doi.org/10.1016/S0048-9697(02)00674-5. Air and Waste Management Association's Annual Conference and Exhibition, AWMA,
Kupiainen, K., Ritola, R., Stojiljkovic, A., Pirjola, L., Malinen, A., Niemi, J., 2016. pp. 3149–3163.

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