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To cite this article: Mindi Xu, Klaus Willeke, Pratim Biswas & Sotiris E. Pratsinis (1993)
Impaction and Rebound of Particles at Acute Incident Angles, Aerosol Science and Technology,
18:2, 143-155, DOI: 10.1080/02786829308959590
Pratim Biswas
Department of Civil and Environmental Engineering, University of Cincinnati, Cincinnati, OH
45221-0071
Sotiris E. Pratsinis
Department of Chemical Engineering, University of Cincinnati, Cincinnati, OH 45221-0171
- - -
When a particle impacts on a surface at an angle < 90", with the model for conditions used in published experi-
only the normal component of the impact velocity is ments compare well with the data and explain observed
usually considered to contribute to deformation. A new dependencies. I t was found that the rebound velocity
model has been developed in which the impact velocity and also the critical velocity, at which rebound starts,
tangential to the surface contributes towards lateral are strongly dependent on the incident impact angle.
rotation during impact, and the remaining tangential Aspects of the new model have been used to calculate
kinetic energy and the stored elastic deformation energy and explain the performance of a newly developed
provide the energy for particle rebound. Calculations particle bounce monitor.
on the impact surface. Wang and John the particle is rotated by the tangential
(1988a) found that the critical velocity of velocity component (Figure 1-11). After
an impacting particle also depends on the time At the particle center has moved
incident angle. Ammonium fluorescein parallel to the target surface by a distance
particles of 6.86 p m impacting on a stain- I/,.,At. During rotation, some of the parti-
less steel cylinder at a velocity of 0.42 m/s cle's kinetic energy is expended towards
stayed on the cylinder when impacted at lifting part of its surface from contact with
90" to the surface, but rebounded when the target surface. This adhesion energy
the angle was decreased to 75" or less. in the tangential direction is labeled E , ,
Wang and John (1988a) attributed this in Figure 1-111.
phenomenon to the change in adhesion The model developed in this study for
energy between the contact surface and acute-angle impaction is an extension of a
the particle. Subsequently, Wang (1990) model developed for 90" impaction (Xu
found that particle lift-up from a surface and Willeke, 1992a). The elastic deforma-
is angle dependent. tion of the original particle material is
In this study a theoretical model is referred to as "primary" elastic deforrna-
developed to determine particle rebound tion, to distinguish it from other elastic
characteristics for impaction at incident deformations that may occur subse-
angles between 0 and 90". The impact quently. Thus, E,,, represents the energy
velocity is resolved into normal and tan- stored in primary elastic deformation of
gential components. The normal compo- the original particle material when
nent results in particle movement towards deformed over an area of radius R,
the impact surface leading to elastic and (Figure 1-111).
plastic deformation in the particle-surface When the elastic stress limit of the
system. The tangential velocity compo- particle material is exceeded, an amount
nent and the energy in elastic deforma- of energy E, is lost in plastic deformation.
tion determine the degree of particle The region above the plastically hardened
rebound. Calculations with the new model zone of radius R , also stores elastic
are compared to several experimental ,
energy, E , (Figure 1-IV). The plastically
measurements. deformed layer hardens and attains a new
stress limit which may be considerably
higher than that of the original material.
PARTICLE-SURFACE INTERACTION Secondary elastic deformation energy in
MODEL the plastically deformed layer, E,, ,, has
Figure 1 is a representation of the distinct been found to be as much as 50% of the
stages of particle impaction and rebound, normal component of E , , , and has,
as we have incorporated them into our therefore, been incorporated into the
model. A particle of radius R and mass rn right-angle impaction model (Xu and
approaches the target surface with veloc- Willeke, 1992a). Removal of the particle
ity Vl and impacts onto the surface at in the normal direction has to overcome
angle ai with impact kinetic energy the adhesion energy in that direction E,, ,.
Ek, = mu2/2, as shown in Figure 1-1. In order to simplify the acute angle model,
Impact velocity V, is resolved into its nor- it is assumed that no horizontal move-
mal component, V,,,, and its tangential ment occurs during plastic deformation by
component, y,,. the normal velocity component.
On impacting the surface, the normal Finally, the particle leaves the impact
velocity component elastically deforms the surface with rebound velocity V, and
particle and the target surface, whereas kinetic energy E,,,, if it can overcome the
Impaction and Rebound of Particles
FIGURE 1. Particle-surface
interaction model: I, incident
particle before impact; 11, first
PRIMARY contact; 111, at the time before
ELASTIC plastic deformation starts; IV,
DEFORMATION during plastic deformation; V,
after rebound.
PLASTIC A N D
SECONDARY
ELASTIC
DEFORMATION
sum of energies E,, E,, and E,,,. The plastic deformation starts, the centers of
normal velocity component, V,,,, depends the particle and the target have
on E, and E,,,, and the tangential com- approached each other by distance he
ponent, V,,,, depends on E, ,. In general, (Bitter, 1963; Rogers and Reed, 1984),
the angle of rebound, a,, is, therefore,
different from incident angle, ai.
CONTACT ELASTIC
DEFORMATION
TOP
VIEW
available before plastic deformation starts. contact distance to be the adhesion energy
Upon first contact (top view of Figure of the same contact area.
2-11, the particle starts deforming elasti- During tangential movement dynamic
cally and continues to do so for the entire friction loss of the particle kinetic energy
time interval At (top view of Figure 2-11). is related to several parameters, such as
Estimates with the plastic deformation surface roughness, contact forces, and
equation by Wang and John (1988b) show movement pattern (rolling or sliding). We
that At for primary elastic deformation is assume that the particle is rolling on a
much longer than the plastic deformation smooth surface with an adhesion contact
and outcoming contact duration time. distance of 0.4 nm. Therefore, the dynamic
Therefore, we have simplified the expres- friction loss of the particle kinetic energy
sion for particle rotation by assuming that is negligible.
rotation stops at the onset of plastic
deformation. The contact area between
the two bodies during this tangential Elastic and Plastic Deformation
movement is an isosceles triangle with In the plastically deformed zone the parti-
area A,: cle material hardens to a new elastic stress
limit (Bitter, 1963), which we have defined
as the secondary elastic stress limit, y,.
The energy stored in secondary elastic
The surface adhesion energy overcome deformation is (Xu and Willeke, 1992a)
by the particle's tangential impact kinetic
energy is
where Ay is the surface adhesion energy where P, is the average surface contact
between particle and target per unit area pressure between particle and target,
of contact. An estimate of the latter may which can be calculated (Bitter, 1963;
be calculated from Derjaguin, et al. (1975) Johnson, 1970; Tsai et al., 1990)
and below which only primary elastic is given by the ratio of V,,, to V,,,. The
deformation takes place. kinetic energy at rebound is less than
the kinetic energy upon impact by the
sum of all the energies that need to be
overcome:
where p, is the particle density. E,,i =E,r +'a,, + E a , t + Ep. ( 16)
Compression of the particle above the The rebound velocity is, therefore,
plastically deformed layer results in addi-
tional storage of elastic energy (Rogers
and Reed, 1984)
The ratio of particle rebound velocity to
impact velocity constitutes the coefficient
of restitution, e,
The energy lost in plastic deformation is
(Bitter, 1963) r
e=--= /l-2(~a,n+~a,t+~p)
v, rnK2
(18)
The normal component of the impact The critical velocity, K,, is the maxi-
kinetic energy, E,,i,,, equals the sum of mum impact velocity at which no rebound
all elastic and plastic deformation ener- occurs. The adhesion energy in the nor-
gies mal direction E , , , can be calculated
through the equations for total adhesion
+ E e , l + Ee,2 + E p .
E k , i , n = Ee,o (I4) energy (Wall et al., 1990; Xu and Willeke,
Equation 14 is used in the model to 1992a). From Eq. 17,
calculate the radius of the plastically
deformed layer
\ 1/4
The energy terms in Eq. 19 are a function
of the particle impact velocity, and hence
Eq. 19 is an implicit function of velocity.
MODEL APPLICATION TO
( 15) PUBLISHED DATA
Since E , , depends on R,, Eq. 15 is solved Calculations with the new model have
by iteration (Xu and Willeke, 1992a). been performed on the experimental data
of Tabakoff and Malak (1987) who used
laser-Doppler anemometry to measure the
Critical and Rebound Velocity impact and rebound velocities of flyash
When a particle impacts a target in the particles impinging on a stainless steel
normal direction, the stored elastic ener- plate that was positioned at incident
gies are the only energy sources for parti- angles of 15" and 75". The flyash was
cle rebound. When the particle impacts polydisperse with a mass median diameter
on a target at an acute angle, the tangen- of 15 pm. The measured impact velocity
tial component of the particle's impact near the impact surface was 98 m/s for
velocity also contributes towards removal all angles. The experimental measure-
of the particle. The angle of rebound, a,, ments are presented in Figure 3 for each
Impaction and Rebound of Particles
BOUNCE SINK
SURFACE
---- D212 ----t
ter. If no air is withdrawn laterally in the the particle concentration in the extracted
x-direction, few of the particles in the center flow is a measure of particle
inlet reach the bounce surface. However, bounce.
when a flow equal to or larger than the The amount of bounce also depends on
center extraction flow is withdrawn later- the angle of inclination of the bounce
ally, the downward particle velocity is sig- surface. Three angles have been studied:
nificantly increased and particles will 8, = 180" (flat), 120°, and 60°, as shown in
reach the bounce surface. If the particles Figure 6. The particle impact velocities
are liquid, they are removed by that sur- were numerically calculated by assuming
face. If they are solid and bouncy, most of potential flow and a point sink for the
them will bounce into the center flow and center extraction flow (Tietjens, 1934;
significantly increase the particle number Dunnett and Ingham, 1986). The dimen-
concentration measured in that flow. Thus, sionless equations for particle motion
Ipl::k
p m ammonium sulfate [(NH4),S04] par-
ticles are shown in Figure 7 as a function
of the calculated particle impact kinetic
energies. The initial particle velocities in (NH4)2S.04 PARTICLES
the inlet of the PBM ranged from 5 to 20
0 1000 2000 3000 4000 5 0 0 0
m/s.
As expected, only a few of the small IMPACT KINETIC ENERGY, Ek,i . 10-'ergs
particles with low impact velocity (smal- FIGURE 7. Dependence of the bounced particle
lest Ek,i)rebound, while the fraction of concentration on impact kinetic energy.
rebounded larger particles (high Ek,i) is
high. The best-fit lines are approximately
linear over the indicated range of impact nate rebound at small incident angles,
kinetic energies. The coefficients for the while the mechanisms associated with the
lines, C,,/Co = A + B E , , , are given in normal kinetic energy dominate rebound
Figure 7. For a given impact kinetic at large incident angles. Figure 8 shows
energy, the 8, = 60" bounce surface results that for the geometry of the PBM the
in a higher fraction of bounced particles tangential impact velocities are indeed
than the other two surfaces. As a, is highest for 0, = 60". The normal impact
lower for 60" than for 120" and 180°, the velocity dominates at 8, = 180". The cal-
critical velocity for rebounding the parti- culations are shown for the range of radial
cle is lowest for 60". This effect has been positions over which particle impact
predicted, as shown in Figure 4, and has occurs.
now been verified by the experimental
data of Figure 7.
In the discussion of Figure 4 it was Particle Rebound Velocity
argued that the mechanisms associated When the critical velocity is exceeded and
with the tangential kinetic energy domi- the particle rebounds, one may ask how
Impaction and Rebound of Particles
INCIDENT
ANGLE, a i
I 1 1 0 1 1 3 1 1 1 !
5 10 15 20 25 30 i
IMPACT VELOCIN, Vi, rn/s
approach the surface at an angle which and a high tangential component, and will,
may result in bounce away from the pri- therefore, rebound more readily.
mary deposition region. The secondary
deposit region may be some distance away The financial support of Mindi Xu by the University of
with little or no particles collected in Cincinnati through a graduate rcsearch assistantship is
gratefully acknowledged.
between.
CONCLUSIONS
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