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冑
a dephasing is followed by the revival of the coherence. The
celebrated example of the dephasing 共called collapse in the 1
兩共t = 0兲典 = 共␣ⴱ↠+ ␣ⴱ2â†2兲N兩0典, 共1兲
literature兲 followed by the revival of coherence is provided 2NN! 1 1
by the theoretically predicted 关13兴 and then observed 关14兴
long-time resonant interaction of an atom with a coherent where 兩␣1兩2 + 兩␣2兩2 = 1 and operators â†1 and â†2 create atoms in
state of a single mode of electromagnetic field in the cavity. the left and right condensates, respectively.
This old case of revival was hard to observe because of irre- During the evolution some condensed atoms collide with
versible cavity losses. This is a typical situation. Also in the each other and scatter out to the initially empty environment.
collision of the condensates there are losses due to the elastic The details of this process can be easily investigated in the
scattering away of atoms of two condensates. Properties of second quantization formalism. We consider the field opera-
the scattered atoms were extensively studied in a number of tor in the following form:
papers 关15–20兴. Perhaps the most comprehensive study of
this process was recently offered in 关19兴. The atoms are pro-
duced in pairs so they not only display a bunching charac- ⌿̂共r,t兲 = −共r,t兲â1 + +共r,t兲â2 共2兲
teristic of bosons but also an enhanced correlation of atoms
ejected in opposite directions 关18兴. Very little was said so far
1
冑V 兺
˙ı关qr−共q兲t兴
on the loss of coherence of colliding condensates, which is + e ĉq , 共3兲
due to the losses and the competition of this decoherence q
spectively, V is the quantization volume, and −共r , t兲 and Due to the Gaussian shape of the condensates we take into
+共r , t兲 denote the wave functions of the left and the right account also the scattering in momentum modes 兩q兩 ⫽ 兩Q兩.
condensates, respectively. We assume a Gaussian shape of 共d兲 The terms which express a collision of two scattered
both condensates. atoms:
冕
We consider only short time scales so a free evolution of
the Gaussian condensate, following 关20兴, may be written in
兺
˙ ˙
d 3r e−ı关共q1兲+共q2兲−共q3兲−共q4兲兴teı共q1+q2−q3−q4兲rĉq† ĉq† ĉq1ĉq2 .
the form q1,q2
3 4
冉 冊
q3,q4
⫾共r,t兲 = 冑
1
3/2 3 exp ⫾ı̇Qx1 −
ı̇បtQ
2m
2
This phenomenon occurs very rarely, so these terms will be
neglected.
冉 冊
共e兲 The terms which express knocking out of an atom
冤 冥
បQt 2 2 2
x1 ⫿ + x2 + x3 from the condensed phase as a result of a collision with a
m scattered atom with wave vector q:
⫻exp − . 共4兲
冕
22
兺
˙ ˙
d 3r e−ı关共q兲−共q1兲−共q2兲兴teı共q−q1−q2兲r+ĉq† ĉq† ĉqâ1 ,
1 2
Both condensates move along the x axis, but their momenta q,q ,q1 2
have opposite signs. Here Q is the length of the wave vector
where q1 and q2 are momenta of the products of this colli-
of each condensate, m is a mass of every atom, and is an
sion.
average Thomas-Fermi radius of the left and right conden-
There are experiments in which these processes lead to a
sates. In calculations below we use parameters from experi-
collisional avalanche 关21兴. This situation happens at a very
mental works in 关10,11兴, where sodium condensates were
high atomic density or in the presence of strong interactions.
used.
Here we consider experiments in which these terms may be
The free evolution is included in formula 共3兲 so the
neglected:
Hamiltonian has a short form
共a兲 We have also neglected all terms which do not con-
冕
serve momentum.
g After these simplifications the Hamiltonian takes the form
Ĥ = d3r⌿̂†⌿̂†⌿̂⌿̂, 共5兲
2
Ĥ = ĤA + ĤAE , 共6兲
g = 4mប a
2
where and a is the s-wave scattering length. where
After substitution of Eq. 共3兲 into Eq. 共5兲 the Hamiltonian
共b兲 ĤA describes the energy of interaction between atoms
becomes a sum of the following terms.
in the condensates,
共a兲 The energy of interaction between atoms in the left
condensate: ĤA = ប␣共兩␣1兩4â†1â†1â1â1 + 兩␣2兩4â†2â†2â2â2兲
g
2
冕 d3r+ⴱ +ⴱ ++â†1â†1â1â1 =
g
â†â†â1â1
2共2兲3/23 1 1
+ ប兩␣1␣2兩2â†1â1â†2â2 .
The energy of interaction in the right condensate is analo- ĤAE = 兺 q,k␣1␣2â1â2ĉ†qĉ†k + H.c.
q,k
gous.
共b兲 The energy of interaction between atoms from differ- Note that the decoherence is caused by the ĤAE only as all
ent condensates: other terms do not change the number of atoms in the con-
densates.
g
2
冕 d3r+ⴱ −ⴱ +−â†1â1â†2â2
III. RATE OF DECAY OF THE NUMBER OF PARTICLES
g −共2/2兲共បQt2/m兲 †
= 3/2 3 e â1â1â†2â2 Most theoretical papers devoted to the dynamical problem
2共2兲 studied here were focused on the properties of scattered at-
ប † † oms. To complement these papers we concentrate here on the
¬ â â1â â2 . fate of the condensates themselves. Our tool is a master
4 1 2
equation for the reduced density matrix of condensed atoms.
共c兲 The terms which express the elastic scattering of two Its derivation follows the scheme described, for instance, in
condensed atoms: 关22兴. We base our derivation on the experimental data from
043628-2
DECOHERENCE IN THE COLLISION OF TWO BOSE-… PHYSICAL REVIEW A 79, 043628 共2009兲
ˆ 共t兲 = Ae−t
2
冑 1
2
冋 冉 冊册
0 − ˆ 1 + Erf
0 − 21 ˆ
冑 , 共8兲
k,l ª 冓 N
2
N
− k − l, + k − l ˆ BEC
2
N
2
冏 冏 N
− k − l, + k − l ,
2
冔
A = 1 ប3233 冑 mប , 1 / 冑 = បQm is the characteristic time of
兩␣ ␣ 兩2mg2冑
where k varies between − N2 and N2 , and l is an integer from
overlapping of the two condensates, ប0 is the average ki- the interval 关0 , min兵 N2 − k , N2 + k其兴. Then the equations for the
netic energy of an atom in the condensate, and ˆ = 关共␣ diagonal terms of ˆ BEC have the form
冉 冊冉 冊
+ 兲N̂ − 兴 is an operator characterizing interaction inside the
dk,l N N
condensates, depending linearly on the number of condensed = 2 −k−l+1 + k − l + 1 k,l−1
atoms. dt 2 2
First, we calculate the average number of particles which
remain in the condensates. It is quite complicated to deal
with the general initial state given by Eq. 共1兲, so we only
− 2 冉 N
2
−k−l 冊冉 N
2
冊
+ k − l k,l . 共10兲
冉 冊
for the simplified model. Furthermore we compare it with the
evolution of a very simple case, namely, a Fock state 1 N
兩典共0兲 = 兩N / 2 , N / 2典. All evolutions are summarized in Fig. 1. Pk共x,0兲 = N ␦„x − 共N/2 − k兲….
2 N/2 − k
Thus, the decay of the number of condensed atoms practi-
cally does not depend on the entanglement of the initial state. In this approximation the average number of particles can be
The average number of particles as a function of time can calculated as the sum
冕
be calculated as the following sum:
具â†1â1共t兲典 ⬇ 兺 dxPk共x,t兲x.
具â†1â1共t兲典 = Tr兵ˆ BECâ†1â1其 = 兺 kBEC
k,l,k,l
共t兲. 共9兲 k
k,l
Equation 共11兲 with this initial condition has the exact solu-
Due to the symmetry we introduce the following notation: tion, which gives
043628-3
KRZYSZTOF PAWŁOWSKI AND KAZIMIERZ RZĄŻEWSKI PHYSICAL REVIEW A 79, 043628 共2009兲
N/2
2k共N − k + 1兲 In the experimental situation time t is so small that Nt Ⰶ 1.
具â†1â1共t兲典 = e−2t 兺
k=−N/2 共N + k + 1兲e
4kt
− Nk − 1
− 1. The largest terms in the sum above are those with k ⬍ 冑N. It
justifies the further approximation e4kt ⬇ 1 + 4kt. Then Eq.
共12兲 共12兲 takes the form
具â†1â1共t兲典 ⬇
冉
关共N + 2兲t + 1兴 2F1 − N,− N −
1
2t
− 1;− N −
1
2t
;− 1
−
1
− 1,
冊 共13兲
共2N+1t兲关2共N + 1兲t + 1兴 2t
where 2F1 is the hypergeometric function 关24兴. It allows us that both models do not include the bosonic enhancement.
to predict the short-time evolution of the average number of For longer time the evolution of the average number of par-
particles even for a large system. ticles is driven by the overlap of both condensates.
We compare our approximate result with the quantum Until this point our numerical and analytical estimations
model for small particle numbers in Fig. 2, getting very good were limited to the case = const. However, the parameter
2
agreement. It is also worth to notice that the dominant terms given by Eq. 共8兲 may be approximated with 0e−2t 共the
in sum 共12兲 are near k = 0. Neglecting all terms except k = 0 is factor of 2 in the exponent appears, because we present result
equivalent to replacing the initial state with the Fock state in the laboratory, and not the center-of-momentum, frame兲,
兩N / 2 , N / 2典. The time scale for a decay of 具â†1â1典 of the Fock where 0 = const. This approximation works well for the ex-
state is proportional to the inverse of the initial number of periments with a weak interaction between condensed atoms
particles, 共in our language it means ␣0 Ⰶ 1 and N␣0 Ⰶ 1兲. As a conse-
quence we are able to describe the full evolution using the
previous results and transforming the time:
N/2
具â†1â1共t兲典Fock ⬇ , 共14兲
Nt + 1
冑 Erf共冑2t兲
t哫 . 共15兲
which is a good approximation also for the correlated state 2冑2
共Fig. 3兲. This observation confirms then the result of 关25兴,
where the efficiency of the Fock ansatz was investigated. The
estimated rate of losses as a function of the initial number of In Fig. 4 we present the numerical result of the average num-
particles is also in good agreement with 关16兴. We consider ber of particles in one drop driven by Eq. 共7兲 and compare it
only very short time scales. In this regime one can approxi- with analytic expression 共13兲 calculated for the transformed
mate the average number of particles in the condensates with time. The evolution of the average number of particles in one
a linear function of time, which corroborates 关16,19,20兴. For drop, 具â†1â1典, is similar for the correlated and the Fock states.
longer time our result agrees only with 关16兴. The reason is Thus, to a good approximation, which gets better for the
average number of particles in one drop
400
2
time of decay 20% particles (s)
quantum model
continuous approximation numerical results
300 fitted curve
1.5
200
1
100
0.5
0
0 0.05 0.1 0.15 0.2 0.25
t (s) 0
0 100 200 300 400 500
N
FIG. 2. 共Color online兲 Average number of particles as a function
of time t. Solid black lines are results of the discrete quantum model FIG. 3. Time at which 20% of particles have been scattered out
for 100 and 400 particles in each drop. The dashed red curves are versus the initial number of particles N. Dashed curve, fitted rela-
the results of our continuous approximation. tion 1 / N 共 = 0.01兲.
043628-4
DECOHERENCE IN THE COLLISION OF TWO BOSE-… PHYSICAL REVIEW A 79, 043628 共2009兲
500 1
numerical result
499.9 analytical result
499.8 0.995
N 1
499.7 g +
0.99 numerical result N=500
499.6
numerical result N=300
numerical result N=100
499.5 fitted curve
0 100 200 300 400 500
t (µs) 0.985
0 0.1 0.2 0.3 0.4 0.5
043628-5
KRZYSZTOF PAWŁOWSKI AND KAZIMIERZ RZĄŻEWSKI PHYSICAL REVIEW A 79, 043628 共2009兲
1.25 1.01
400 atoms
200 atoms
1 100 atoms
numerical results 1.005
fitted curve
1/t (s )
0.75
-2
2
g 11
1
2
0.5
0.995
0.25
0 0.99
0 100 200 300 400 500 600 0 0.05 0.1 0.15 0.2 0.25
N (a) t (s)
0.996
These functions do not change much during the process. In 2
Fig. 7 one can see a decrease in g112
below 1 共antibunching兲 g 12
and an increase in g12 ⬎ 1 共bunching兲—basing on the defini-
2 0.994
tions from 关26兴 for the case = const. In a single act of scat-
tering, occurring at random times, two atoms from different 0.992
condensates collide elastically and scatter out. This random-
ness is the source of the bunching. For the case of time-
0.99
dependent the change in the second-order correlations 0 0.05 0.1 0.15 0.2 0.25
function is even smaller than in Fig. 7 and it would be ex- (b) t (s)
tremely difficult to detect.
FIG. 7. 共Color online兲 Second-order correlation functions for
different initial numbers of particles: 共a兲 g211; 共b兲 g212.
V. CONCLUSIONS
The main result of our work is the master equation for step we transform the density matrix and Hamiltonian 共6兲 to
colliding, interacting Bose condensates. We conclude that the the interaction picture
evolutions of the average number of particles for full and ˙ ˙
simplified models are very similar. We investigated analyti- H̃AE = eıHAt/បĤAEe−ıHAt/ប ,
cally a simple case—the dynamics of two correlated and
equal-size droplets of BEC, which gives a good insight into ˙ ˙
˜ = eıHAt/បˆ e−ıHAt/ប .
the dynamics of the system. We obtained the analytical for-
mula for the evolution of the average number of particles. We write H̃AE in the following form:
Using numerics we found that the decoherence is faster than
the decay of the population, but for the experimental param-
eters this decay is relatively small. The process is faster for a
H̃AE = 兺
q,k,i苸兵1,2其
共i兲
Vq,k 共i兲
共t兲Bq,k 共t兲 + H.c.,
larger number of particles. Furthermore we are also able to
共1兲 ˙ ˙
calculate higher-order correlation functions. The results were where ⌬ = 20 − 共q兲 − 共k兲, Vq,k 共t兲 = q,k共t兲e−ı⌬teı共␣+兲N̂t/ប
obtained for short time only but the extension to longer times ˙
−ıt/ប 共1兲 共2兲 共1兲
⫻e ␣1␣2â1â2, Vq,k共t兲 = 关Vq,k共t兲兴†, and Bq,k 共t兲 = ĉ†qĉ†k
is possible. 共2兲
= 关Bq,k共t兲兴 .
†
Using the von Neumann equation one can easily write the
ACKNOWLEDGMENTS first two terms of the perturbation series of the formal solu-
tion for the density matrix 共Born approximation兲,
We thank P. Ziń and P. Deuar for useful discussions. The
冕
work was supported by Polish Government research funds
for 2006–2009. d˜ 1 t
ı̇
= d†H̃AE共t兲,关H̃AE共兲,˜共兲兴‡ − 关H̃AE共t兲,˜共0兲兴.
dt ប2 0 ប
APPENDIX: MASTER EQUATION 共A1兲
We present a derivation of a master equation for the re- We compute the trace of both sides of Eq. 共A1兲 with respect
duced density matrix. To this end we follow 关22兴. In the first to the environment and get the following equation:
043628-6
DECOHERENCE IN THE COLLISION OF TWO BOSE-… PHYSICAL REVIEW A 79, 043628 共2009兲
d˜BEC
dt
1
=− 2
ប
冕 t
0
d TrE兵†H̃AE共t兲关H̃AE共兲,˜共兲兴‡其
The standard approximation extends the limit of integra-
tion from t to ⬁, which makes the calculation shorter and
does not change significantly the value of the integral,
冕 冕
ı̇ t ⬁
− TrE兵关H̃AE共t兲,˜tot共0兲兴其. 共A2兲 ˙ ˙ 2 ˙ ˙ 2
ប deı⌬·e−ıˆ e− ⬇ deı⌬e−ıˆ e−
0 0
冑冋 冉 冊册
We assume that initially the density operator is a product of
the density operator of the condensates BEC and the density 1 2 ⌬ − ˆ
= e−共⌬ − ˆ 兲 /4 1 + ı̇ Erfi .
operator of the environment. From the initial conditions 2 2 冑
冕
This is just an analog of the principal-value part in
d˜BEC 1 t
d TrE兵†H̃AE共t兲关H̃AE共兲,˜共兲兴‡其
冕
=− 2 ⬁
dt ប ˙ 1
eı共0−兲 = ␦共0 − 兲 − ı̇P
0
0 共0 − 兲
and can be rewritten as
冕
encountered, for instance, in a study of a spontaneous emis-
d˜BEC 1 t
=− 2 d 兺 V共2兲 共1兲
q 共t兲Vq 共兲˜
BEC − V共1兲 BECV共2兲
q 共t兲˜ q 共兲
sion from a two-level atom 关27兴. In that case the infinite
dt ប 0 q value of this shift is 共after renormalization兲 interpreted as the
Lamb shift and incorporated into the transition frequency of
− V共1兲 BECV共2兲
q 共兲˜ BECV共2兲
q 共t兲 + ˜
共1兲
q 共t兲Vq 共兲. 共A3兲 the atom. In analogy we neglect the corresponding term in
Invoking the Markov approximation we approximate the our derivation. Moreover, the exact value of the eigenvalue
operator BEC共兲 under the integral over with BEC共t兲. After of the Hamiltonian ĤA drops out from further calculations,
eliminating the degrees of freedom of the environment, one
can transform the whole equation back to the Schrödinger 8g2兩␣1␣2兩2冑
冑 V 2 ប 2 兺
2 2 ˙ 2 2
picture. Finally, the master equation takes the form ˆ = e− 共k + q兲 /2eı共ˆ −⌬兲te−t e−共⌬ − ˆ 兲 /4 .
k,q
2 2
dBEC In the Gaussian function e− 共k + q兲 /2 the wave vectors k
= − 关ˆ †â1â2BEC,â†1â†2兴 − 关â1â2, BECâ†1â†2ˆ 兴. and q corresponds to the wave vectors of the scattered atoms.
dt
From the momentum conservation both vectors should have
The operator ˆ is defined as similar lengths to Q ⬇ 3.6⫻ 106 m−1—the length of the wave
vectors of the condensates. The dispersion 1 / has a rela-
ˆ =
16兩␣1␣2兩2g2
V 2ប 2
冕0
t
d 兺 e −
k,q
2共k + q兲2/2 −ı˙⌬共t−兲 ˙ı
e ˆ 共t−兲 −共t2+2兲
e e , tively small value of 2 ⫻ 104 m−1. Thus it is reasonable to do
the following approximation:
ˆ 共t兲 =
8兩␣1␣2兩2g2冑 V2
V2冑ប2 共2兲
6 冕 dqdke−
2共k + q兲2/2 −ı˙⌬·t ˙ı
e ˆ t −t2 −共⌬ − ˆ 兲2/4
e e e
=
16兩␣1␣2兩2g2冑22
共2兲 冑3ប2
6 冕 ˙ ˙ 2
dqe−2ı关0−共q兲兴teıˆ te−t e−关0 − 共q兲 − 共1/2兲ˆ 兴
2/
=
64兩␣1␣2兩2g2冑23
共2兲 冑 ប
6 3 2
4 冕 ˙ ˙ 2
dqqe−2ı关0−共q兲兴teıˆ te−t 共qe−关0 − 共q兲 − 共1/2兲ˆ 兴 /兲.
2
共A4兲
043628-7
KRZYSZTOF PAWŁOWSKI AND KAZIMIERZ RZĄŻEWSKI PHYSICAL REVIEW A 79, 043628 共2009兲
兩␣1␣2兩2g2冑2 −t2
冑 冉 冊
2
The function qe−关0 − 共q兲 − 共1 / 2兲ˆ 兴 / is well localized around 2m 1
ˆ 共t兲 = 2 e 0 − ˆ
ប 冑33
these q, which satisfy a condition ប 2
共q兲 = 0 − 21 ˆ . ⫻ 冕 2
dqqe−关0 − 共q兲 − 共1/2兲ˆ 兴 / .
冋 冉 冊册
justifies further approximation
冕 冑 1 + Erf 0 − 2 ˆ
1
2/ m
dqqe−关0 − 共q兲 − 共1/2兲ˆ 兴 = .
冑
冉 冊
2ប
2/ 1
qe−关0 − 共q兲 − 共1/2兲ˆ 兴 ⬇ ␦ 0 − 共q兲 − ˆ Finally
2
Substituting Eq. 共A5兲 into Eq. 共A4兲 we get which is formula 共8兲 used in the main part of this paper.
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