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2007
Noel Smyth
University of Edinburgh
Annette L. Worthy
University of Wollongong, annie@uow.edu.au
Publication Details
Minzoni, A., Smyth, N. F. & Worthy, A. L. (2007). Modulation solutions for nematicon propagation in non-local liquid crystals.
Optical Society of America. Journal B: Optical Physics, 24 (7), 1549-1556.
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Modulation solutions for nematicon propagation in non-local liquid
crystals
Abstract
The propagation of solitary waves, so-called nematicons, in a nonlinear nematic liquid crystal is considered in
the nonlocal regime. Approximate modulation equations governing the evolution of input beams into steady
nematicons are derived by using suitable trial functions in a Lagrangian formulation of the equations for a
nematic liquid crystal. The variational equations are then extended to include the effect of diffractive loss as
the beam evolves. It is found that the nonlocal nature of the interaction between the light and the nematic has
a significant effect on the form of this diffractive radiation. Furthermore, it is this shed radiation that allows the
input beam to evolve to a steady nematicon. Finally, excellent agreement is found between solutions of the
modulation equations and numerical solutions of the nematic liquid-crystal equations.
Disciplines
Physical Sciences and Mathematics
Publication Details
Minzoni, A., Smyth, N. F. & Worthy, A. L. (2007). Modulation solutions for nematicon propagation in non-
local liquid crystals. Optical Society of America. Journal B: Optical Physics, 24 (7), 1549-1556.
Received December 21, 2006; revised February 26, 2007; accepted February 27, 2007;
posted March 15, 2007 (Doc. ID 78332); published June 15, 2007
The propagation of solitary waves, so-called nematicons, in a nonlinear nematic liquid crystal is considered in
the nonlocal regime. Approximate modulation equations governing the evolution of input beams into steady
nematicons are derived by using suitable trial functions in a Lagrangian formulation of the equations for a
nematic liquid crystal. The variational equations are then extended to include the effect of diffractive loss as
the beam evolves. It is found that the nonlocal nature of the interaction between the light and the nematic has
a significant effect on the form of this diffractive radiation. Furthermore, it is this shed radiation that allows
the input beam to evolve to a steady nematicon. Finally, excellent agreement is found between solutions of the
modulation equations and numerical solutions of the nematic liquid-crystal equations. © 2007 Optical Society
of America
OCIS codes: 190.5530, 190.5940, 160.3710, 190.4400.
1. INTRODUCTION The purpose of the present work is to fill the gap be-
The possibility of guiding self-supporting, nonlinear tween these abstract and approximate results. To this
beams (solitary waves) of light in the regime of large non- end, the dynamics of nematicon evolution in a liquid crys-
locality in liquid crystals was shown in a remarkable se- tal is studied using an extension of the method of Ref. [6]
ries of experiments by Assanto et al. [1–4]. They named for optical pulse propagation, which is based on a form of
these light solitons, which resulted from the liquid crystal modulation theory that includes the effect of the disper-
actively guiding the light, nematicons. Moreover, they sive radiation shed by a pulse solitary wave during its
also studied nematicon formation theoretically [2,3]. In evolution. This method was further developed to apply to
this work the existence of static solitons was shown by us- soliton propagation in liquid crystals in the local regime
ing an expansion around the center of the beam, which [7,8]. In a similar work, but for one rather than for two
gave a Gaussian beam and a parabolic profile for the op- space dimensions, as in Refs. [7] and [8], a variational
tical axis [2,3]. This local expansion was matched to an method was employed to obtain approximate Gaussian
exponentially decaying solution away from the center of profiles for steady one-dimensional nematicons [9].
the beam. This matching then gave a condition determin- Gaussian profiles were found to be a good approximation
ing the relation between the nematicon’s amplitude and near the peak of a one-dimensional nematicon but de-
the width of its waist. It also showed that the angle (di- cayed too fast in its tail. Lagrangian methods were also
rector) profile is much wider than the waist of the beam. employed to find approximations to the steady two-
The dynamics of a nematicon was studied approximately dimensional solitary wave solutions of a nonlocal nonlin-
by using the Fock–Leontovich equation in the limit of a ear Schrödinger (NLS) equation with a Gaussian kernel
large cell [3]. An expression for the evolution of the waist in the nonlinear, nonlocal term [10]. However, such a
of the beam was then obtained, which showed its oscilla- Gaussian kernel is not applicable to liquid crystals.
tion. It was further shown that steady solitons with no An initial beam evolves into a nematicon by undergoing
waist oscillation are recovered for specific values of the in- a breathing motion accompanied by the shedding of linear
put power. The effect of diffractive loss by the soliton as it diffractive radiation. The modulation equations for the
evolves was not considered. beam evolution are obtained by using a suitable trial
On the more abstract side, it is known, since the nem- function in an averaged Lagrangian for the nematicon
aticon equations (1) and (2) below are the same as those equations. These modulation equations have a family of
for a thermoelastic waveguide, that the soliton solution is fixed points that are the steady nematicon solutions, with
stable [5]. However, no results for the dynamics of the conservation of energy selecting the final steady state. It
evolution of a beam-type boundary condition can be ob- is shown how the modulation equations, coupled with loss
tained using the Lyapunov function discussed in Ref. [5]. due to shed diffractive radiation, explain and reproduce
3. APPROXIMATE EQUATIONS
To derive the approximate equations describing the evo-
lution of a nematicon, the Lagrangian for the nematicon
equations (3) is taken in polar coordinates:
冕冕
Z ⬁
Fig. 1. (Color online) Schematic diagram of a liquid-crystal cell L= 关ir共E*Ez − EEz*兲 − r兩Er兩2 + 4r兩E兩2 − r2r
with a propagating polarized light beam. 0 0
冕 冕
⬁ ⬁
E 1 r r
i + ⵜ2E + 2E = 0, ⵜ2 − 2q = − 2兩E兩2 , 共3兲 4r兩E兩2dr = 4␣a2 r sech2 sech2 dr. 共6兲
z 2 0 0
 w
which are the same equations as for the thermoelastic This integral cannot be evaluated exactly unless  = w.
waveguide [5]. As the parameter increases, the response To obtain useful, explicit approximate equations, the con-
of the liquid crystal becomes more nonlocal, and the width cept of equivalent functions is now used [8]. The func-
of the optical axis becomes wider than the waist of the tion sech2共r / 兲 is then replaced by the Gaussian
light beam. Note that in the local limit → 0, the system exp共−r2 / 共A兲2兲, and sech2共r / w兲 is replaced by the Gauss-
(3) can be reduced to the two-dimensional NLS equation, ian exp共−r2 / 共Bw兲2兲, so that the integral (6) can now be ex-
which predicts collapse of an input beam at a finite propa- plicitly evaluated. With this replacement, we have
Minzoni et al. Vol. 24, No. 7 / July 2007 / J. Opt. Soc. Am. B 1551
冕 冕 冕
⬁ ⬁ ⬁
2共1/共A兲2+1/共Bw兲2兲 2 1
4r兩E兩2dr = 4␣a2 r e−r dr I42 = x sech4 x tanh2 x dx = ln 2 + , 共12兲
0 0 0
15 60
2 ␣ a 2A 2B 2w 2 2
冕
⬁
= . 共7兲 2 1
A 2 2 + B 2w 2 I4 = x sech4 x dx = ln 2 − ,
0
3 6
The new coefficients A and B are now determined by
matching the Taylor series of the integral (6) with the hy- where C is the Catalan constant C = 0.915965594. . . [11].
perbolic secants to the result [Eq. (7)] using Gaussians to Taking variations of the averaged Lagrangian (10) with
two terms in the limit w Ⰶ , which is the limit of interest respect to the parameters a, w, ␣, , , and g results in
in the nonlocal regime. This results in the variational equations
d
A = 2I2/冑Ix32, B = 冑2I2 , 共8兲 共I2a2w2 + ⌳g2兲 = 0, 共13兲
dz
where
d
冕
⬁
d
2
共I1aw2兲 = ⌳g , 共14兲
I2 = x sech x dx = ln 2, dz dz
0
dg I22a A2B4␣aw22
冕
⬁ I1 = − , 共15兲
Ix32 = x3 sech2 xdx = 1.352301002 . . . . 共9兲 dz 2w2 共A22 + B2w2兲2
0
d I22 A2B2␣2共A22 + 2B2w2兲
The error in this Taylor-series matching is O共共w / 兲3兲. For I2 =− + , 共16兲
the comparison example of Fig. 3, the steady-state values dz w2 共A22 + B2w2兲2
of w and  are w0 = 1.6768 and 0 = 3.9647, giving an error plus the algebraic equations
in matching of O共8 ⫻ 10−2兲. In general, the larger is, the
smaller 共w / 兲3 is. A 2B 2 2w 2a 2
It might be thought that, since the hyperbolic secants ␣= , 共17兲
2共A22 + B2w2兲共2I42 + qI42兲
of the trial functions have been replaced by equivalent
Gaussians to evaluate the cross integral, it might have
been better to use Gaussians for the trial functions [Eqs. A 2B 4w 4a 2
␣= .
(5)]. However, it was found that if this were done the re- qI4共A22 + B2w2兲2
sulting approximate equations would not give solutions in
good agreement with numerical solutions, as was also the These variational equations are the equations governing
case for the nematicon equations in the local regime [8]. the evolution of the nematicon.
Furthermore, it was found that Gaussian initial condi- By Nöther’s theorem, the nematicon equations (3) have
tions have a greater tendency to split into multiple soli- an energy conservation equation that can be obtained
tons at moderate-to-high amplitudes than do hyperbolic from the Lagrangian (4) from invariances in z. The aver-
secant initial conditions. aged form of this energy conservation equation is then
冕
With the equivalent Gaussian approximation for the ⬁
dH d
cross integral, the averaged Lagrangian is = r关兩Er兩2 − 4兩E兩2 + 2r + 2q2兴dr
dz dz 0
L = − 2共a2w2I2 + ⌳g2兲⬘ − 2I1aw2g⬘ + 2I1gw2a⬘ + 4I1awgw⬘
共18兲
Here
Since energy is conserved, this energy conservation equa-
1 2 tion can be used to determine the final steady nematicon
⌳= 2
l 共11兲
state from the input beam.
is the area of the shelf under the beam, modulo 2. The When ␣ is eliminated between the algebraic equations
integrals I22, I1, I42, and I4 are given by (17), the director angle width  can be found as
冕
⬁ is then given by the first of Eqs. (17). The amplitude and
I1 = x sech x dx = 2C, width of the optical axis are therefore given as algebraic
0 functions of the nematicon in the electric field.
1552 J. Opt. Soc. Am. B / Vol. 24, No. 7 / July 2007 Minzoni et al.
ˆ ⬘I12共ŵ2 + 2âŵ⍜兲
⌳=− , 共21兲
Q
and an outer shelf, was also found by Ref. [12] for per- in analogy with the relation between ᐉ and ⌳. Even
turbed vector solitons of the coupled NLS equations de- though these values of and ⌳ ˜ have been found for a spe-
scribing birefringent optical fibers. These two components cific initial condition, they will be found to give good
of the shelf were shown to be due to two distinct types of agreement with numerical solutions for all initial condi-
eigenfunction of the continuous spectrum for the equa- tions.
tions describing the perturbation. The diffractive radiation loss is now added to the modu-
The radius of the outer portion of the shelf under the lation equations (14)–(16), the first of Eqs. (17), and Eqs.
electric field beam can be estimated from the numerical (18) and (19), which results in Eq. (15) being modified to
solution shown in Fig. 2 as approximately = 15. Solu- [7,8]
tions of the modulation equations give that 
= 2.18853. . . at z = 400 for the initial conditions of Fig. 2.
Hence an estimation for the radius of the outer portion of dg I22a A2B4␣aw22
the shelf is = 71/2, so that I1 = − − 2␦g, 共24兲
dz 2w2 共A22 + B2w2兲2
˜ = 1 2 ,
⌳ 共23兲 where the loss coefficient ␦ is
2
冑2I1
冕 兵关
z ˜兲
R共z⬘兲ln共共z − z⬘兲/⌳ dz⬘
␦=− , 共25兲
˜
32eR⌳ 0
1
4
˜兲
ln共共z − z⬘兲/⌳ 兴 2
其
+ 32/16
2
˜ 兲兴2/16 共z − z⬘兲
+ 2关ln共共z − z⬘兲/⌳
1 2
R2 = ˜ g2兴.
关I2a2w2 − I2â2ŵ2 + ⌳ 共26兲 + − 2q = q sin共2兲 − 2q − 2兩E兩2 cos共2兲.
˜
⌳ r 2
r r
共27兲
For the local regime considered by Refs. [7] and [8], ⌳ ˜
= ⌳ as the optical axis and the electric field have the same
The derivatives were calculated using standard second-
width, and the shelf under the electric field beam is the
order finite differences, which gave a tridiagonal system.
usual NLS shelf [6]. The loss coefficient [Eq. (25)] differs
Together with the boundary conditions r = 0 at r = 0 and
from that of García Reimbert et al. [7,8] by the replace-
˜ in the loss coefficient ␦ and R. This is be- → 0 as r → ⬁, the resulting two-point boundary-value
ment of ⌳ by ⌳ problem was solved using a Picard iteration. The modula-
cause ⌳ in these terms comes from the total radius of the tion equations (14), (16), (18), and (24) were solved nu-
shelf under the beam [7]. merically using the standard fourth-order Runge–Kutta
The final modulation equations describing the evolu- scheme.
tion of the nematicon are then Eqs. (14) and (16), the first The first comparison between the numerical solution
of Eqs. (17), (18)–(19), and (24). The solution of these and the solution of the approximate equations is shown in
modulation equations will be compared with full numeri- Fig. 3, for which the initial conditions are that a = 0.5 and
cal solutions of the nematicon equations (1) and (2) in Sec- w = 4 at z = 0 with q = 2 and = 10. It can be seen that there
tion 5. is excellent agreement in both the mean and the envelope
of the amplitude oscillation, with the approximate mean,
being the amplitude of the final steady nematicon, being
5. RESULTS slightly higher than the numerical mean. The agreement
In this section, full numerical solutions of the nematicon between the period of the solution of the modulation equa-
equations (1) and (2) will be compared with solutions of tions and that of the full numerical solution is excellent.
the approximate equations (14) and (16), the first of Eqs. This agreement is remarkable, given that the amplitude
(17), (18)–(19), and (24). The numerical method used to of the beam doubles over the initial amplitude during the
solve the nematicon equations (1) and (2) is the same as oscillations and that the frequency of the modulation
that of Ref. [8], so only a brief description of the method equations’ solution was obtained by linearizing about the
will be given here. The electric field equation (1) was fixed point and then assuming that this result holds away
solved using a pseudospectral method [13]. The main dif- from the fixed point. In the derivation of the modulation
ference with the method described in Ref. [13] is that the equations, it was assumed that for large the director re-
stepping in the z direction is performed in Fourier space sponse is small. While the electric field amplitude a has
using a fourth-order Runge–Kutta method rather than in a large amplitude oscillation, numerical solutions of the
physical space using a leap-frog scheme. The r derivatives full nematicon equations (1) and (2) show that the direc-
are calculated using fast Fourier transforms. To numeri- tor angle has a small oscillation amplitude of ␣ = O共0.2兲.
cally solve the optical axis equation (2), it was rewritten The reason that the electric field response is so large is
in the form that two-dimensional solitary waves for nonlocal NLS-
1554 J. Opt. Soc. Am. B / Vol. 24, No. 7 / July 2007 Minzoni et al.
where
6. CONCLUSIONS
The evolution of beamlike initial conditions into steady 2I22D2â − A2B2Dˆ 2ŵ2â共2␣ˆ + ⌫1â兲
⍜= ,
nematicons has been studied for the regime of strongly
A2B2ˆ ŵâ2共2A2␣ˆ ˆ 3 + ⌫2Dˆ ŵ + 2B2⌫3␣ˆ ŵ3兲
nonlocal nematic liquid crystals. Modulation equations
for the evolution of the beam were derived by using suit-
able trial functions in a Lagrangian formulation of the I22
Q = Q1 − 关Q2 + ⍜Q3兴,
nematicon equations. When terms that include the effect 2A2B4␣ˆ ˆ 2ŵ4
of diffractive loss as the beam evolves were added to these
冉 冊
modulation equations, excellent agreement was found be-
I22 2â
tween numerical solutions and solutions of the modula- Q1 = 1− ⍜ , Q2 = ␣ˆ 2ˆ 2ŵ2 + ⌫1ˆ 2ŵ2â,
2
tion equations. In the strongly nonlocal regime studied in 2ŵ ŵ
the present work, the width of the beam in the optical
axis is much larger than that of the electric field. This
Q3 = 2␣ˆ ˆ 2ŵâ + ⌫2ˆ 2ŵ2â + 2⌫3␣ˆ ˆ ŵ2â
larger optical axis width has the effect of increasing the
length of the shelf of linear diffractive radiation under the − 4D−1␣ˆ ˆ 2ŵ2â共A2⌫3ˆ + B2ŵ兲, 共A3兲
electric field beam over that studied in previous works
[6–8]. This, in turn, leads to increased diffractive loss
from the nematicon as it evolves. 2A2B4ŵ4â 4A4B4ˆ ŵ3â2共ˆ − ⌫3ŵ兲
⌫1 = , ⌫2 = ,
The approach of the present work completes that of qI4D2 qI4D3
Conti et al. [3], since the effect of the diffractive radiation
shed as the beam evolves is taken into account. It has
B2ŵ共qI4ˆ 2 + 4I3兲
been shown that the shed radiation acts as a damping ⌫3 = , D = A2ˆ 2 + B2ŵ2 . 共A4兲
that settles the initial condition to the steady nematicon. qI4ˆ 共2A2ˆ 2 − B2ŵ2兲
The evolving beam undergoes a breathing motion in its
waist, in the manner of a damped simple harmonic oscil- As in Ref. [6], the frequency of the simple harmonic mo-
lator. tion equation (A2) is now matched to the steady nemati-
As final comments, some remarks are needed on the con oscillation frequency ˆ ⬘, given by Eq. (16) with a, w,
nature of the approximations made to derive the evolu- , and ␣ replaced by their fixed-point values. This results
tion equations for the nematicon. The trial functions used in the radius ᐉ of the shelf of low-wavenumber diffractive
for the beam electric field and the director angle include radiation under the beam being determined by
the effect of nonlocality, introducing an additional varia-
ˆ ⬘I12共ŵ2 + 2âŵ⍜兲
tional parameter. To evaluate a coupling integral between ⌳=− . 共A5兲
the electric field and the director angle, equivalent Gaus- Q
1556 J. Opt. Soc. Am. B / Vol. 24, No. 7 / July 2007 Minzoni et al.
The fact that the shelf under the soliton oscillates at 7. C. García Reimbert, A. A. Minzoni, and N. F. Smyth,
the frequency of the soliton was also shown by Yang [12] “Spatial soliton evolution in nematic liquid crystals in the
nonlinear local regime,” J. Opt. Soc. Am. B 23, 294–301
for the vector soliton solutions of the coupled NLS equa- (2006).
tions for a birefringent fiber by examining the eigenfunc- 8. C. García Reimbert, A. A. Minzoni, N. F. Smyth, and A. L.
tions for the equations governing a small perturbation Worthy, “Large-amplitude nematicon propagation in a
from the soliton state. liquid crystal with local response,” J. Opt. Soc. Am. B 23,
2551–2558 (2006).
This research was supported by the Engineering and 9. P. D. Rasmussen, O. Bang, and W. Królikowski, “Theory of
Physical Sciences Research Council under grant EP/ nonlocal soliton interaction in nematic liquid crystals,”
Phys. Rev. E 72, 066611 (2005).
C548612/1. 10. A. I. Yakimenko, V. M. Lashkin, and O. O. Prikhodko,
“Dynamics of two-dimensional coherent structures in
nonlocal nonlinear media,” Phys. Rev. E 73, 066605 (2006).
REFERENCES 11. M. Abramowitz and I. A. Stegun, Handbook of
1. G. Assanto, M. Peccianti, and C. Conti, “Nemations: optical Mathematical Functions with Formulas, Graphs, and
spatial solitons in nematic liquid crystals,” Opt. Photonics Mathematical Tables (Dover, 1972).
News Feb. 2003, pp. 44–48. 12. J. Yang, “Vector solitons and their internal oscillations in
2. C. Conti, M. Peccianti, and G. Assanto, “Route to birefringent nonlinear optical fibers,” Stud. Appl. Math. 98,
nonlocality and observation of accessible solitons,” Phys. 61–97 (1997).
Rev. Lett. 91, 073901 (2003). 13. B. Fornberg and G. B. Whitham, “A numerical and
3. C. Conti, M. Peccianti, and G. Assanto, “Observation of theoretical study of certain nonlinear wave phenomena,”
optical spatial solitons in a highly nonlocal medium,” Phys. Philos. Trans. R. Soc. London, Ser. A 289, 373–403 (1978).
Rev. Lett. 92, 113902 (2004). 14. W. Królikowski, O. Bang, N. I. Nikolov, D. Neshev, J.
4. M. Peccianti, C. Conti, G. Assanto, A. de Luca, and C. Whyller, J. J. Rasmussen, and D. Edmundson, “Modulation
Umeton, “Routing of anisotropic spatial solitons and instability, solitons and beam propagation in spatially
modulational instability in liquid crystals,” Nature 432, nonlocal nonlinear media,” J. Opt. B: Quantum
733–737 (2004). Semiclassical Opt. 6, S288–S294 (2004).
5. E. A. Kuznetsov and A. M. Rubenchik, “Soliton 15. Y. Huang, Q. Guo, and J. Cao, “Optical beams in lossy
stabilization in plasmas and hydrodynamics,” Phys. Rep. non-local Kerr media,” Opt. Commun. 261, 175–180 (2006).
142, 103–165 (1986). 16. M. Peccianti, A. De Rossi, G. Assanto, A. De Luca, C.
6. W. L. Kath and N. F. Smyth, “Soliton evolution and Umeton, and I. C. Khoo, “Electrically assisted self-
radiation loss for the nonlinear Schrödinger equation,” confinement and waveguiding in planar nematic liquid
Phys. Rev. E 51, 1484–1492 (1995). crystal cells,” Appl. Phys. Lett. 77, 7–9 (2000).