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To cite this article: Yan Jin & Xiao Dong Chen (2009) A Three-Dimensional Numerical Study of the Gas/Particle Interactions
in an Industrial-Scale Spray Dryer for Milk Powder Production, Drying Technology: An International Journal, 27:10, 1018-1027,
DOI: 10.1080/07373930903203588
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Drying Technology, 27: 1018–1027, 2009
Copyright # 2009 Taylor & Francis Group, LLC
ISSN: 0737-3937 print=1532-2300 online
DOI: 10.1080/07373930903203588
powder degradation, etc. In the present study, the three-dimensional (FLOW3DTM) and found that the air flow patterns were
(3-D) transient multiphase flow in an industrial-scale spray dryer sensitive to the values of the turbulence parameters selected
has been investigated using the CFD package FLUENT. The
Eulerian–Lagrangian approach and two-way coupling method were at the annular air inlet. Oakley and Bahu[3] predicted the
used in the simulations. The reaction engineering approach (REA low-frequency oscillations of the central jet, which were
model) for milk particles has been implemented. Some new also observed in the experiments. Guo et al.[4] investigated
characteristics of the gas flow pattern and the particle behavior the swinging and swirling oscillations of the central jet at
(e.g., temperature–time profiles) were identified from the numerical low frequency, which they found even without inlet swirl.
results; for example, the milk particles flow in such a way that
makes the central jet oscillation more nonlinear. The discrete phase Stafford et al.[5] and Kieviet et al.[6] found the instabilities
enhances the turbulence near the air/droplet inlet but damps it down- in the slow recirculation zones near the walls.
stream. The transient turbulent flow causes significant uncertainties The transient air flow and the particle dynamics in spray
in the particle tracking, which presented some challenges in simula- dryers are very complicated, and the interactions of the air
tions. The study has highlighted the importance in performing 3-D and the particles make the problem even more difficult to
transient simulations in order to understand the industrial-scale
dryers. be solved computationally. Langrish and Fletcher[7] sum-
marized the work on applications of CFD in spray drying
Keywords Computational fluid dynamics; Fluent; Gas=particle
before 2001 and stated that one of objectives of the numer-
interaction; Industrial-scale spray dryer; Multiphase ical simulations is to reduce wall depositions rates by mod-
flow; REA drying kinetics model ifying the air flow patterns in the chamber through small
changes in the air inlet geometry for existing dryers. Huang
INTRODUCTION et al.[8,9] and Huang and Mujumdar[10–12] performed a vari-
Spray dryers are widely used in the dairy industry to ety of 2-D=3-D simulations of spray dryers with the com-
produce dry powders from liquids. The capacity of spray mercial CFD package FLUENT.[13] The numerical
dryers in dairy industry is from one ton to some 20 tons results showed the effect of drying air temperature, spray
of dry powder produced per hour. Therefore, spray dryers rate, air flow rate, atomizers, etc., on the performance of
are in general extremely energy hungry. Design of the spray dryers. It has been argued that the drying cham-
high-performance spray dryers that are more energy effi- ber geometry is very important in the dryer design and the
cient and yet can maintain high quality is difficult because dryer’s performance. The incorporation of a fluid bed can
of the complex nature of turbulent flow, the strong air– significantly improve the overall drying performance.
particle interactions, and the process–product quality Fletcher et al.[14] indicate the three-dimensional character-
interactions in the dryers. istics of transient flow in spray dryers. Kota and
Computational fluid dynamics (CFD) packages provide Langrish[15] predicted the deposition patterns by solving
good tools to understand the detailed flow fields in the unsteady Navier-Stokes equations. One-way droplet=air
dryers. Crowe[1] simulated the flow field in a spray coupling was employed in the simulation, which assumed
that the droplets had no effect on the continuous phase.
Correspondence: Xiao Dong Chen, Biotechnology and Food Mezhericher et al.[16,17] simulated droplet drying in spray
Engineering Group, Department of Chemical Engineering, chambers using 2-D and 3-D CFD methods. The results
Monash University, Clayton Campus, Victoria 3800, Australia;
E-mail: dong.chen@eng.monash.edu.au
show the three-dimensionality and asymmetry of the flow
1018
GAS=PARTICLE INTERACTIONS IN MILK POWDER PRODUCTION 1019
dmp
¼ hm Ap ðqn;s qn;b Þ ð1Þ
dt
where Uwater is the local mole fraction of water, p is the local the particle temperature Tp because the Biot number is
absolute pressure, and Tb is the local bulk temperature in the small enough.[25] Then the energy equation of the particles
gas. hm in Eq. (1) is calculated from the Sherwood number can be written as follows:
correlation of the Ranz and Marshall type:[21,22]
dTp dmp
mp cp ¼ hc ðT Tp ÞAp þ hfg ð8Þ
hm dp 1=2 dt dt
ShAB ¼ ¼ 2:0 þ 0:6Red Sc1=3 ð3Þ
Dv;air
where cp, hfg, and hc are the heat capacity, the latent heat,
where dp is the particle diameter, Dv,air is the diffusivity of and the heat transfer coefficient of the milk particles.
qd ju uj
vapor in air, Red ¼ p lp is the Reynolds number, and The multiphase flow was solved with FLUENT 6.3.26
l and the REA drying model was implemented in the
Sc ¼ qDv;air is the Schmidt number. l, q, and u are the dynamic
viscosity, density, and velocity of the gas phase, and up is the FLUENT package through the user-defined function
particle velocity. (UDF).
qv,s is an empirical parameter for solute=solids contain-
ing particles, which is time dependent during the drying DESCRIPTION OF THE TEST CASE
process as a result of the increasing solid content at the sur- The structure of the spray dryer simulated in this study
face. The REA approach[19,23,24] is used to calculate qv,s: is shown in Fig. 1. The dryer, which is 15 m tall and 8 m
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TABLE 1
Dryer operating parameters
Case 1 Case 2 Case 3 Case 4
Droplet inlet Flow rate (ton=h) 18 10.8 3.6 0
Solid mass fraction (%) 48%
Temperature ( C) 78
Air inlet Air flow rate (m3=min) 1650
Air temperature ( C) 210
Absolute humidity kg H2O=(kg dry air) 0.01
Fluidized bed inlet Air flow rate (m3=min) 480
Air temperature ( C) 90
Absolute humidity kg H2O=(kg dry air) 0.01
Air outlet pipe Ambient pressure (Pa) 3210
direction and 65 grid points are given in the circumferential The chamber wall is assumed to be adiabatic. The angle
Downloaded by [University of Regina] at 03:46 25 August 2014
direction. The grid points in the radial direction are distrib- between the velocity of the inlet hot air and the vertical axis
uted differently at different cross sections. Seven grid is 20 . The magnitude of the swirling velocity is 15% of that
points in the radial direction are given at the air inlet, of the axial velocity. k and e at the air inlet are 0.03 m2=s2
and 20 grid points in the radial direction are given in the and 0.2 m2=s3. The numerical results show that the influ-
spray chamber. The mesh resolution is the highest near ence of the air inlet turbulence is quite small. The gravity
the air=droplet inlet, whose mesh spacing is roughly is 9.81 m2=s, which is in the vertical axial direction. The
0.04 m. The sensitivity of the mesh resolution was studied droplet–droplet interaction is not considered in the present
by Jin and Chen[27] that indicates the independency of the study. The DRW stochastic tracking model is utilized to
numerical results on the mesh resolution. The same mesh consider the effect of the turbulent flow on the particles.
resolution is used in the present study. It can also be seen The time scale constant in the model is set to be 0.15, which
from the present numerical results that the mesh resolution is recommended by the FLUENT 6.3 User’s Guide.[13]
is high enough to capture the main vortical structures in the The second-order up-wind scheme is used in space dis-
chamber. The characteristics of the flow field, such as the cretization. First-order implicit solver is used in time
oscillation of the central jet, were also captured success- discretization.
fully. The global mesh and the mesh near the air inlet are Four cases were simulated to understand the effect of
shown in Fig. 1b. the milk droplet feeding rate. The gas phase is two-way
Although the present study focuses on the multiphase coupled with the discrete phase in the first three cases.
flow in the spray dryer, the fluidized bed was also added The pure gas phase flow was simulated in the fourth case.
to the computational domain so that a more realistic The flow field is distributed uniformly before the beginning
velocity profile can be given at the bottom of the spray of the simulation, where the initial temperature, pressure,
dryer. Figure 1c shows the streamlines of the gas phase velocity, and absolute humidity are 20 C, 0 Pa, 0 m=s,
from the fluidized bed inlet, which are colored with the and 0.01 kg H2O=(kg dry air). The time step used in the
streamline ID. The figure indicates the necessity of includ- simulation is 0.01 s, which is verified to be small enough
ing the fluidized bed into the computational domain. It can according to the numerical results. The maximum number
be noticed that the streamlines that are released from the of subiterations is 20. The subiterations are skipped when
inlet of the fluidized bed usually direct to the wall before the solution is converged. The convergence is decided if
entering the spray dryer. Some small vortical structure the residues are smaller than 0.001.
can be found at the corner. The flow field near the dryer
bottom is so complicated that it is almost impossible to
address the inlet profile without simulating the dryer and RESULTS AND DISCUSSION
the fluidized bed as one entity. Thus, the fluidized bed Some numerical results in Case 1 was compared with the
and the spray dryer were simulated together in the present experimental data, which are reliable results taken from
study. The mass flow rate, temperature, and humidity of plant trials by the research group led by Chen. The pre-
the fluidizing air are given in Table 1. The air velocity is dicted exhaust air temperature is 73 C, which is close to
normal to the fluidized bed inlet. The inlet area for fluid- the plant data. Figure 2 shows the agreement of the aver-
ized bed is 18 m2. The detailed porous structure of the fluid- aged wall temperature predicted by the simulation and
ized bed inlet was neglected in the present study. the experimental data by Chen et al.[28] The experimental
1022 JIN AND CHEN
FIG. 7. Oscillation of the air-phase flow field. (a) Mass center history,
(b) pattern of the mass center positioning (section x ¼ 2 m, air=particle If the section is far away from the air=droplet inlet
two-way coupling, Case 4).
(Fig. 8b), the turbulent kinetic energy k is clearly decayed
due to the presence of the particles. There are two peaks
of k in Cases 3 and 4, whereas only one remains in
Figure 8 shows the turbulent kinetic k distribution at the Cases 1 and 2. Moreover, the turbulence near the side wall
line x ¼ 2 m, y ¼ 0 m and x ¼ 10 m, y ¼ 0 m, which are is enhanced by the particles in Case 1.
obtained at 190 s. Two peak values of the turbulent kinetic The dispersion of particles due to the turbulent flow is
energy k, as a result of the shear layer produced by the cen- considered using the stochastic tracking model. Figure 9
tral jet, can be found at the points r 0.8 m and indicates the importance of this turbulence effect.
r 1.1 m. The interesting discovery of the present study Figures 9a and 9c are from the numerical simulations with
is that there is another peak of k near the jet center. The the stochastic tracking model, whereas Figs. 9b and 9d are
values of the central peak in Cases 1–4 are 17.0, 14.2, without the stochastic tracking model. The particles were
1.6, and 4.0 (m2s2), respectively. This means that the colored with their residence time in the dryer. The red
turbulence near the jet center can be strengthened by the particles have the longest residence time and the blue
particles if the inlet droplet flow rate is high, whereas it particles have the shortest residence time. An ‘‘inverse
can be damped if the inlet liquid feed is small. This mushroom’’-like structure of the particles was generated
phenomenon indicates again the importance of simulating at 1 s (Fig. 9a). Without considering turbulent effect, fewer
industrial-size spray dryers directly, which have much particles are swirled back to the dryer. The particle move-
higher droplet feeding rate than in the small-scale dryers. ment history is significantly influenced by the turbulent
GAS=PARTICLE INTERACTIONS IN MILK POWDER PRODUCTION 1025
index.[7]
It is worth noting that the 3-D simulation predicts much
stronger heat=mass transfer near the droplet inlet than the
1-D model.[31] The difference can be seen from the defini-
qd ju uj
tion of the Reynolds number, Red ¼ p lp , which is used
to compute the heat and mass transfer coefficient. The
cross-section averaged air velocity, u ¼ m _ =ðqAÞ, is used in
the 1-D model, where m _ is the mass flow rate of the hot
air and A is the cross-section area. However, the local air
velocity in 3-D simulation can be much larger than the
average velocity. For example, the inlet air velocity at the
air inlet is about 27 m=s, which is about 10 times the aver-
age velocity. Thus, the 3-D simulation predicts much stron-
ger heat and mass transfer near the air=droplet inlet.
This shows, again, the importance of performing 3-D
transient simulation in order to understand the spatial
effect on particles. Even at 3-D, the steady-state simulation
FIG. 9. Effect of the turbulence on the particle behavior in the dryer, can only give one sort of particle history, but the real par-
Case 1.
ticles move in a wide range of possibilities. The statistical
study of the transient simulation is significant to quantify
the particle variables in the dryer.
flow, which is important in studying the particle residence
time, moisture content, and the insolubility index.[7] CONCLUSIONS
Figure 10 displays all the particles having the same Great effort has been done in simulating 2-D=3-D
initial particle diameter (215 mm) and the same initial veloc- transient=steady multiphase flow fields in spray dryers in
ity direction in the dryer at 140 s. The x coordinate is the recent years.[8–12,14,16,17,20] Compared with the previous
instantaneous particle residence time since the particles study, the present article focuses on the air=particle interac-
enter the dryer. Due to the transient gas flow, especially tion in an industrial-scale dryer, on which there is still very
the turbulent effect, the particles travel in quite different few 3-D transient simulations. The REA model has been
routes. The particle velocity can vary between 0 and used in 3-D simulations for the first time. Moreover, a
15 m s1, and the moisture content varies between 0 and reflecting wall boundary condition is used in the simula-
0.18 wt% on dry basis. The average residence time of the tion, which is more accurate in the real plant operation
particles that leave the dryer from the particle exit is about than the escaping wall boundary condition.
51 s. Figure 10d shows the temperature of the particles that From the numerical results, some characteristics that
have the same size (215 mm). Figures 10e and 10f indicate are indicated by previous researchers are also captured,
the particle temperature from 0 to 1 s and from 0 to 0.1 s. such as the low-frequency oscillation of the central jet
Results of two time steps (0.01 and 0.001 s) are compared, and the three-dimensionality of the flow field. Some new
1026 JIN AND CHEN
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FIG. 10. The influence of the turbulent gas flow on the particle variables history (a: time dependent velocity; b: time dependent moisture content;
c: particle mass, d, e, f: particle temperature), Case 1.
characteristics in the spray dryer are argued: It is found in the dryer but can vary in a wide range due to the turbu-
that the particles make the central jet oscillate more nonli- lent effect. A statistical method is necessary in studying
nearly. The second frequency of the oscillation drops with particle behavior because of the uncertainty of the particle
the increasing droplet feeding rate. The turbulence kinetic tracking.
energy can be strengthened by the particles near the air=
liquid inlet for large feeding rate, whereas it is damped in ACKNOWLEDGEMENT
the main dryer chamber. The particle dispersion caused The project is sponsored by the Gardiner Foundation
by the turbulent flow has a rather important effect on the and Dairy Innovation Australia Ltd., Melbourne,
particle behaviors. The particle behavior is not certain Australia. We also thank Dr. Kamlesh Patel in the same
GAS=PARTICLE INTERACTIONS IN MILK POWDER PRODUCTION 1027
research group for his help in discussing the properties of simulations. Chemical Product and Process Modeling 2007, 2 (3),
the drying model and the properties of the milk particles. 1–18.
16. Mezhericher, M.; Levy, A.; Borde, I. Droplet-droplet interactions
in spray drying using 2D computational fluid dynamics. Drying
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