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Article history: The building sector represents nearly one third of the global greenhouse gas (GHG) emissions, in which
Received 14 July 2018 the embodied carbon of reinforced concrete is recognized as a significant source of the GHG emissions.
Received in revised form Developing low carbon reinforced concrete buildings is an important strategy to achieve the long term
26 April 2019
sustainability in urban cities. However, the large variability and the combined effect of different rein-
Accepted 3 May 2019
Available online 6 May 2019
forced concrete design parameters during the production stage presents considerable effects on the total
embodied carbon of buildings, which were not fully explored in literature. Thus, this study aims to
develop a systematic approach to quantify the detailed relationship between different concrete design
Keywords:
Building design
parameters and their combined effects, thereby helping mitigate the building GHG emissions. The
Combined effect proposed approach takes into account the parameters that have significant effects on the embodied
Carbon footprint carbon of reinforced concrete, and studies different variations of reinforced concrete designs to minimize
Greenhouse gas the carbon emissions. The results of this study serve as a decision support basis for improving the
Material production building design in regard to carbon reduction. In an illustrative example, the proposed approach is
Reinforced concrete examined to compare the embodied carbon for different material design scenarios and to suggest the
material choice for a lower embodied carbon in concrete buildings.
© 2019 Elsevier Ltd. All rights reserved.
https://doi.org/10.1016/j.jclepro.2019.05.035
0959-6526/© 2019 Elsevier Ltd. All rights reserved.
V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597 583
Hammond and Jones, 2008; O'Brien et al., 2009; Van den Heede Therefore, the objective of this study is to develop a systematic
and De Belie, 2012). Zhang et al. (2014) evaluated a general value approach to quantify the detailed relationship between different
of embodied carbon (425 kg CO2-e/m3) for the production of plain variations of reinforced concrete designs and building embodied
concrete (without steel reinforcement). Harrison et al. (2010) used carbon as well as the combined effect of concrete design parame-
0.13 kg CO2-e/kg to interpret plain concrete and presented 0.24 kg ters, thereby providing a basis to mitigate the carbon emissions in
CO2-e/kg for additional carbon emissions of 2% steel reinforcement. the built environment. The proposed method takes into account a
Flower and Sanjayan (2007) evaluated the relationship between theoretical mix design process to determine the concrete mix
embodied carbon (225e322 kg CO2-e/m3) and characteristic proportions and to quantify the carbon emissions of different
compressive strength (25e32 MPa) of plain concretes. Miller et al. constituent materials for analyzing the per-unit carbon footprint of
(2015) evaluated the embodied carbon (150e520 kg CO2-e/m3) of various concrete products. The approach considers the indepen-
reinforced concrete as a function of mix proportions, geometry of dent parameters that have significant effects on the embodied
building element, and design age. Similarly, Purnell (2013) gave a carbon of reinforced concrete - namely characteristic strength, use
range of embodied carbon values to reinforced concrete, depending of SCMs, cement type, aggregate size, and recycled steel scrap -
on concrete strength grade, geometry of building element, and therefore can analyze the effects due to the variability in reinforced
loading capacity. concrete designs. It will also investigate the combined effects of
Although the embodied carbon of reinforced concrete has large various reinforced concrete designs on the embodied carbon
variations (due to mix proportions, etc.), the major sources of car- mitigation in buildings, by varying the influential parameters. The
bon emissions were identified as ordinary Portland cement (OPC) embodied carbon is quantified within the cradle-to-site system
(Flower and Sanjayan, 2007; Zhang et al., 2014) and steel rein- boundary, considering the detailed carbon emissions from all the
forcement (Gan et al., 2017b; Yan et al., 2010). Therefore, the pri- stages of production and transportation of reinforced concrete. As
mary option for reducing the embodied carbon of reinforced manufacturers and designers seek to mitigate the carbon emissions
concrete is to replace as much OPC and steel reinforcement as of concrete, the proposed approach provides a basis to better
possible by recycled materials (Meyer, 2009) or to minimize the identify the major environmental burdens of concrete production
volume of materials needed (Liu et al., 2011). García-Segura et al. and to improve the design of reinforced concrete for a lower
(2014) and Purnell and Black (2012) compared the embodied car- embodied carbon in buildings.
bon of OPC concrete with equivalent mix designs containing SCMs,
i.e., fly ash (FA) and ground granulated blast-furnace slag (GGBS). 2. Methodology
Around 20e30% of the emissions in plain concrete can be reduced
with replacement of the FA and GGBS. Habert et al. (2011) and The proposed approach has been devised with reference to
Turner and Collins (2013) compared plain concrete containing 100% carbon accounting guidelines. The approach can compare the
OPC with other comparable mix design containing geo-polymers. embodied carbon of a particular structure due to the use of various
The results indicated that changing to geo-polymers (320 kg CO2- reinforced concrete products. The concrete mix proportions are
e/m3) produces 8% less emissions than conventional OPC concrete derived from theoretical mix design methods or concrete standards
(354 kg CO2-e/m3) (Turner and Collins, 2013). Gan et al. (2015) (BSI, 2006; Teychenne et al., 1997) used by the industry. Section 2.1
evaluated the effect of large-sized aggregates and eco-cement describes the detailed manufacturing process for each composition
(produced from municipal solid wastes) on minimizing the OPC in reinforced concrete as well as the cradle-to-site system boundary
volume, both have over 17% savings on the embodied carbon of for evaluation. A series of procedures for quantifying and mitigating
concrete. Yan et al. (2010) quantified the carbon emission reduction the carbon emissions over the defined system boundary are pre-
in a reinforced concrete building due to the use of recycled steel. sented in Section 2.2.
The results indicated that using recycled steel in a concrete building
reduces over 30% of the embodied carbon as compared to con- 2.1. Manufacturing processes and system boundary
ventional primary steel.
Even though previous studies have evaluated different aspects Fig. 1 shows the manufacturing processes for the key compo-
(like building design and construction planning) to reduce the nents in reinforced concrete and the system boundary. The raw
embodied carbon, there is still a lack of systematic details to materials used in plain concrete production include OPC, aggregate,
demonstrate how changing various (reinforced) concrete designs at water, SCMs, and chemical admixtures. The raw materials are
the production stage would affect the total amount of embodied produced outside a concrete batching plant and delivered to the
carbon in buildings. For example, manufacturers may choose to plant in appropriate modes. OPC and SCMs are transferred pneu-
produce concrete with less carbon footprint, but low carbon con- matically to storage silos while aggregate is delivered by belt con-
crete may have weaker material properties (like strength) and veyers to storage bins. The raw materials of plain concrete are
require more to provide the same building performance (Habert proportioned prior to blending in order to ensure that all the
and Roussel, 2009), and eventually the total embodied carbon in designed mechanical properties are achieved. Based on the mix
the whole building may not be less. As such, it is essential to proportions specified by the concrete engineers, the raw materials
develop a holistic framework that can quantify the relationship are fed to a weight hopper for mixing and blending. The blended
between the variability of material production/design and the total concrete mixtures are loaded onto mixer trucks and transported to
embodied carbon in buildings (Gursel et al., 2014). The proposed construction sites. Steel reinforcement is another important con-
approach will provide material manufacturers and building de- stituent in reinforced concrete. The production of steel reinforce-
signers a more systematic view on how the embodied carbon in ment starts from the processing of pig iron, which is delivered to
buildings is affected by different variations of reinforced concrete at the basic oxygen furnace (BOF) or electric arc furnace (EAF) for
the production stage. In addition, there has been an increasing melting. Steel scrap can be added to BOF and EAF by different
focus on the effects of independent mix design variables (such as amounts to reduce the use of pig iron. Generally, the BOF process
cement strength and SCMs) on carbon emissions of concrete. But contains around 30% of steel scrap whereas the EAF can contain up
the combined effects due to different material design parameters to 100% (WSA, 2014). The pig iron and steel scrap are melted and
on the embodied carbon reduction in buildings have not been refined for producing the desirable grade of steel reinforcement.
studied thoroughly in literature. The system boundary for the quantification of embodied carbon is
584 V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597
cradle-to-site, which includes the carbon emissions from plain 2.2.1. Concrete characteristic strength
concrete and steel reinforcement productions, via all detailed The first step in designing concrete mix proportions is to deter-
manufacturing processes above-mentioned, until the materials are mine the characteristic strength, followed by the determination of
transported to construction sites. the water to binder (w/b) ratio, cementing binder amount and other
constituents. Therefore, any change of strength can result in signif-
2.2. Proposed approach for embodied carbon mitigation icant changes to the subsequent mix proportioning processes and
the carbon emissions of the concrete. The choices of the w/b ratio
Based on the predefined system boundary, a holistic approach is and binder content should guarantee a desirable strength and
proposed to evaluate and mitigate the embodied carbon of rein- workability. In order to assure desirable strength and durability,
forced concrete buildings. Reinforced concrete comprises contri- concrete specifications worldwide require a minimum cement con-
butions from various concrete compositions and steel tent for a selected characteristic strength, e.g., the British Standard
reinforcement which are often combined in a wide variety of pro- (BSI, 2006) proposes 280 kg cement for one m3 of C35 concrete.
portions in accordance with the design requirements. Incorpo- Minimum cement content is a theoretically reasonable value that
rating variations of all mix proportion parameters may complicate guarantees the minimum strength and durability of concrete, while
the approach, but provide only a small improvement in the effi- minimizing the cement usage and the carbon emissions of concrete.
ciency of embodied carbon mitigation. Therefore, the proposed Due to these reasons, the proposed approach adopts the minimum
approach focuses on the variations of the most influential param- cement content for each characteristic strength in the concrete mix
eters that have substantial impacts on the embodied carbon of proportioning and embodied carbon mitigation.
reinforced concrete. Based on the literature review and our previ-
ous sensitivity analyses (Gan et al., 2015, 2017a), the influential 2.2.2. Supplementary cementitious materials (SCMs)
parameters on the embodied carbon of reinforced concrete were SCMs are alternative cementing materials for the substitution of
identified as (1) concrete characteristic strength, (2) SCMs, (3) type OPC in concrete production. The OPC substitution rates for SCMs
of cement, (4) maximum size of aggregate, and (5) recycled steel are different, depending on their strength gain mechanisms and
scrap. These five parameters can substantially affect the amounts of chemical compositions. Low calcium fly ash (FA) (<15% CaO by
OPC and steel reinforcement, thereby imposing large uncertainties weight) contains high proportions of SiO2 and Al2O3. In the pres-
on the carbon emissions of reinforced concrete. Other mix ence of water, SiO2 and Al2O3 can react with the calcium hydrate
proportioning parameters have also been evaluated in literature, released by cement hydration, which gradually improves the
but were found to make relatively less contributions to the strength of concrete. However, concrete containing a large amount
embodied carbon of reinforced concrete e for example, cement of low calcium FA may require a longer period to exceed the 28-day
strengths (2012), aggregate types (e.g., natural and recycled ag- target strength. High calcium FA and GGBS are more reactive SCMs,
gregates e see Appendix 1), and chemical admixtures (Flower and containing large amounts of CaO (>20% by weight) and displaying
Sanjayan, 2007; Van den Heede and De Belie, 2012). As such, the good cementitious behavior by reacting with water to improve the
proposed approach will investigate different variations of rein- mechanical strength of concrete. Therefore, the proposed approach
forced concrete by changing the five influential parameters in order focuses mainly on the high calcium FA and GGBS, and considers
to minimize the embodied carbon value. Details about the five their usual substitution rates in the analysis, which are 25e35% for
influential parameters are discussed in the following paragraphs. FA and 25e75% for GGBS (HKBD, 2013).
V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597 585
2.2.3. Type of cement concrete. Then, the content of the fine aggregate can be estimated,
Cement is a highly carbon intensive material and accounts for depending on the maximum aggregate size, w/b ratio, slump value
70%e90% of carbon emissions for concrete (Flower and Sanjayan, and grading of the fine aggregate. The coarse aggregate content can
2007). Different kinds of cement require different production be obtained by deducting the proportion of fine aggregate from the
technologies and may contribute various amounts of carbon total aggregate demand. The fourth step is to decide on the type
emissions in concrete. OPC has a high carbon emission factor and content of SCMs in the concrete production as well as the type
(1.005 kg CO2-e/kg) because of the high energy consumption in of steel reinforcement and recycled scrap content (based on the
cement kilns and in the calcination of limestone. Eco-cement pro- steel manufacturing process selected).
vides similar mechanical properties, but it can contain up to 50% of The properties of concrete and steel reinforcement, as deter-
municipal solid waste incineration ash and reduce the consump- mined from Steps 1e4, are used to design the structural compo-
tion of limestone and energy. Due to these reasons, the carbon nents in buildings and to evaluate the material structural
emission factors for eco-cement manufacture are dramatically performance. In Step 5, structural analysis is conducted to deter-
decreased, to around 0.699 kg CO2-e/kg (Taiheiyo, 2012). It can be mine the building element sizes (e.g., width and height) and check
seen that different types of cement contribute different amounts of the material structural behavior. If the materials selected can meet
carbon and have a large impact on the final results. Thus, the type the criteria in building design codes, the amounts of concrete and
and carbon emission factor of cement should be clearly specified in steel reinforcement required for construction can then be quanti-
an assessment. fied for the quantification of embodied carbon in Step 6. On the
other hand, the relative proportion and specification of each con-
2.2.4. Maximum aggregate size crete constituent material can help measure the per-unit carbon
The maximum size of aggregate refers to the largest sieve size emissions of concrete. Provided the material amount and per-unit
used in the mix proportioning, through which all the aggregate can carbon emissions, the total embodied carbon of reinforced con-
pass. The maximum aggregate size significantly impacts the cement crete in a building can be quantified accordingly. Embodied carbon
content and carbon emissions of concrete. First, the size of aggregate quantification consists of two parts: (a) the cradle-to-gate emis-
affects the cement content and concrete workability by changing the sions from the production of plain concrete and steel reinforce-
particle surface area. For a given weight, a large-sized aggregate has a ment, and (b) the gate-to-site emissions from the transportation of
lower surface area contacting the cement paste. As a result, the need materials to sites.
for cement and water to bind the aggregate particles is reduced. In
contrast, a small-sized aggregate requires greater amounts of cement Cradle-to-gate emissions
and water to bind the aggregate particles and maintain good cohe-
siveness of the concrete mixture. According to BS 8500 (BSI, 2006), The present study includes a theoretical mix design process to
the cement content for 10 mm-sized aggregate can be 18% higher determine the concrete mix proportions and to quantify the per-
than the cement content for 40 mm aggregate. This change can unit carbon emissions from the production of concrete. Eq. (1)
significantly affect the concrete mixture and carbon emissions. Due calculates the carbon emissions of concrete as the product of its
to these reasons, the proposed approach considers the different constituent materials and the corresponding carbon emission
maximum aggregate sizes that are used in concrete production. factors:
" #
2.2.5. Recycled steel scrap X
M X
N
Steel reinforcement production consists of crude steel CEcon ¼ Qm EFmn GWPn K 1 (1)
manufacturing and steel finishing (WSA, 2014). As discussed pre- m¼1 n¼1
Figure 2. Methodology framework for mitigation of embodied carbon in reinforced concrete buildings.
concrete and steel reinforcement. Specifically, the unit carbon CEsteel (in kg CO2-e/kg) are obtained from Table 2 ai stands for the
emissions of concrete CEcon (in kg CO2-e/m3) can be obtained from material waste ratios during construction, which are 6.8% for plain
Eq. (1), whereas the unit carbon emissions for steel reinforcement concrete and 5.1% for steel reinforcement, respectively (Shen et al.,
2002). A refers to the total floor area of the building (in m2).
Raw materials EFmn GWPn (kg CO2-e/kg) In this study, transportation carbon emissions are evaluated
Ordinary Portland cement 1.005 a using either the fuel-based method (that depends on the specific
Eco-cement 0.699b type and amount of fossil fuel consumed) or the freight-distance
Coarse natural aggregate 0.003c method (that depends on the transportation distance and the
Fine natural aggregate 0.003c cargo weight), as follows:
Recycled aggregate 0.002c
Water 0.001d " #
FA 0.008d X
I X
R
GGBS 0.083d EGS ¼ ECi;r FEFr A1 (3a)
a i¼1 r¼1
Zhang et al. (2014).
b
Taiheiyo (2012).
c
Gan et al. (2016).
d
Hammond and Jones (2008).
V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597 587
Table 4
Material designs for each scenario in this study.
Scenarios Concrete strength Content of SCMs/Eco-cement Aggregate size Content of steel scrap
Scenario 1 is the baseline, wherein the core walls and perimeter BOF process with 30% steel scrap and the EAF process with 100%
columns are constructed of C40 concrete (fcu ¼ 40 MPa) whereas steel scrap, respectively (WSA, 2014).
the beams and floor slabs use C30 concrete (fcu ¼ 30 MPa). The Scenario 10 evaluates the combined effects due to different
concrete uses 100% OPC and 10 mm aggregate, and the steel design parameters. The concrete to be used is C80 with 40 mm
reinforcement does not contain any recycled steel scrap. aggregate, containing 75% GGBS and 25% eco-cement as well as
In Scenarios 2 and 3, the compressive strength of concrete in- 100% steel scrap.
creases from C40 to C60 (fcu ¼ 60 MPa) and C80 (fcu ¼ 80 MPa),
respectively. High strength concrete will be used for only col- The concrete is assumed to be produced locally and delivered by
umns and core walls, as they need to withstand heavier loads (it mixer trucks with a transportation distance of 15 km. Steel rein-
is uncommon to use high strength concrete for the floor framing forcement is imported from manufacturers by ship, covering a
elements like floor slabs and beams). All the designs are checked distance of 800 km. With the assumptions aforementioned, the
in structural analysis software to ensure that design codes are embodied carbon are quantified and presented in Section 4.
met (HKBD, 2013).
Scenarios 4 and 5 assume that 35% FA and 75% GGBS are used in
concrete production in order to compare the effects of different 4. Results and discussion
SCMs on embodied carbon mitigation.
Scenario 6 compares the difference of embodied carbon be- 4.1. Embodied carbon mitigations using different material designs
tween 100% OPC and 100% eco-cement in concrete production,
whereas Scenario 7 compares the difference between using Fig. 4 shows the embodied carbon of the reinforced concrete
more small-sized aggregate (10 mm) and large-sized aggregate building for different material designs, and the percentage reduc-
(40 mm). tion of each scenario (using Scenario 1 as the baseline). The
To investigate the maximum carbon reduction by recycled steel, embodied carbon for the Scenario 1 is 483 kg CO2-e/m2, wherein
Scenarios 8 and 9 consider using steel reinforcement from the plain concrete accounts for 47% and steel reinforcement contributes
53%. The majority of embodied carbon in the reinforced concrete
Figure 4. Embodied carbon of the reinforced concrete building for different material designs.
V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597 589
Figure 5. Percentage contribution of each structural elements to the total embodied carbon of the reinforced concrete building.
building is attributable to the main structural load-bearing ele- considering carbon mitigation measures together does not neces-
ments (such as core walls). Fig. 5 represents the percentage sarily reduce more CO2 emissions. To investigate the combined
contribution of each structural element to the building embodied effects of different design parameters, more sensitivity analyses are
carbon. It can be seen that core walls and columns (including some conducted in the following Sections.
structural beams) consume the majority of the construction ma-
terials and produce more than 66% of the embodied carbon, as they 4.1.1. Combined effects of high strength concrete and steel
are required to carry substantial gravity and lateral loads (like reinforcement
wind) of the entire building. In contrast, the floor framing elements Table 5 shows the effects of high strength concrete on material
(like floor slabs and beams) only need to carry the gravity load of demand and embodied carbon in the building. The compressive
each individual floor, and therefore account for less embodied strength of concrete for the main structural load-bearing elements
carbon (34%) in the building. (i.e., core walls and columns) is increased from C40 to C60 and C80.
Different material designs substantially vary the embodied As the compressive strength increases, the amount of concrete
carbon of the reinforced concrete building. In Scenario 1, the required for the structural elements decreases dramatically from
structural elements are mainly constructed of C40 concrete con- 43,852 m3 to 36,168 m3 and 30,654 m3. The percentage reduction of
taining 100% OPC, 10 mm aggregate, and 100% primary steel rein- concrete approaches as much as 18% and 30% for C60 and C80,
forcement. Scenarios 2e9 investigate the carbon mitigation by respectively. The amount of steel reinforcement also reduces by 15%
improving one of material design parameters. For example, with and 32% in order to maintain an appropriate rebar ratio in the
the use of C60 and C80 high strength concrete (Scenarios 2 and 3), design code. In general, increasing concrete strength by every
the embodied carbon of the reinforced concrete building is reduced 5 MPa can reduce 4.50% of the plain concrete used and 3.75% of the
by 5% and 11% to 457 and 429 kg CO2-e/m2. Besides, employing steel reinforcement. Theoretically, utilizing high strength concrete
SCMs (Scenarios 4e5), eco-cement (Scenario 6), large-sized is beneficial for mitigating the material demand and therefore the
aggregate (Scenario 7) and steel scrap (Scenario 8e9) alone can embodied carbon. However, it should be noted that as higher
also reduce the building embodied carbon by up to 30% (335 kg concrete strength requires more OPC, the per-unit carbon emis-
CO2-e/m2), 13% (417 kg CO2-e/m2), 8% (444 kg CO2-e/m2) and 39% sions of C60 and C80 concrete will increase accordingly. Specifically,
(293 kg CO2-e/m2), respectively. If the carbon mitigation measures the per-unit carbon emissions for C60 and C80 concrete are 15% and
above-mentioned are considered together (such as in Scenario 10), 36% more than that of C40, which may largely offset the carbon
the embodied carbon is reduced by 76%e107 kg CO2-e/m2, which is emission reduction due to the decreased demand for plain concrete
much less than the sum of the individual effect. It means that and steel reinforcement. Table 5 also provides the final carbon
Table 5
Comparison of embodied carbon for columns and core walls between using C40 concrete versus higher strength concrete (C60 and C80).
Scenario Strength Plain concrete Steel reinforcement Embodied carbon (kg CO2-e/m2)
Quantity (m3) Emission factor (kg CO2-e/m3) Quantity (tonne) Emission factor (kg CO2-e/kg) Main load-bearing elements Whole building
Figure 6. Carbon emissions of plain concrete against different strength classes (the values are taken as the average of 10 mm and 40 mm aggregates with various SCMs).
calculation results, taking account of both factors. Considering only cement kilns. Compared to OPC, the contributions of SCMs (i.e., FA
the main structural load-bearing elements (i.e., core walls and and GGBS), aggregates and other compositions are not significant,
columns), the embodied carbon drops from 305 kg CO2-e/m2 to 279 although they account for more than 80% of the concrete bulk.
and 251 kg CO2-e/m2, respectively. Increasing concrete strength by However, it should be noted that using different types of SCMs and
every 5 MPa reduces around 2.25% of the embodied carbon for the aggregates substantially affects the OPC content, leading to around
structural elements. The total embodied carbon for the whole 30% uncertainty on the per-unit carbon emissions of concrete. In
building constructed from C40 concrete is 483 kg CO2-e/m2. If C60 general, increasing the compressive strength of concrete by 5 MPa
and C80 concrete are utilized, the embodied carbon drops moder- requires 20 kg more OPC, therefore the per-unit carbon emissions
ately by 5% (457 kg CO2-e/m2) and by 11% (429 kg CO2-e/m2). Even of concrete grow by around 4% (i.e., 20 kg CO2-e/m3) for every
though the embodied carbon is reduced by using high-strength 5 MPa. Since the more OPC content required for higher concrete
concrete, the more OPC content required for higher concrete strength can offset the embodied carbon reduction, special atten-
strength has already offset the carbon reduction. tions are required for material selection at the early stage of
Fig. 6 compares the carbon emissions of OPC concrete and its building design.
compositions against different strength classes (see Appendices 2
and 3 for detailed results). OPC is found to be the largest contrib-
4.1.2. Combined effects of SCMs and eco-cement
utor and accounts for over 90% of the carbon emissions for plain
Fig. 7 shows the per-unit carbon emissions of concrete, taking
concrete, due to its limestone calcination and fossil fuel usage in
into consideration the combined effect of SCMs and eco-cement.
Figure 7. Carbon emissions of concrete considering the combined effects of SCMs and eco-cement (the values are taken as the average of 10 mm and 40 mm aggregates).
V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597 591
Figure 8. Carbon emissions of plain concrete with different strength classes, amounts of SCMs, types of cement, and aggregate sizes.
Three typical concrete strength classes (i.e., C80, C55 and C30) are 4.1.3. Combined effects of concrete strength, SCMs, cement type,
selected for the comparison. As Fig. 7 shows, the embodied carbon and aggregate size
emissions for concrete containing SCMs and/or eco-cement is 30%e This section investigates the minimum carbon emissions of
60% less than that for 100% OPC concrete. Specifically, utilizing 1% of concrete due to the combined effects of the four plain concrete
eco-cement in concrete can reduce 0.95 kg CO2-e/m3 of the carbon design parameters. The relationship between different concrete
emissions in concrete. FA is the most efficient recycled cementi- design parameters is mathematically formulated in Fig. 8. Concrete
tious material, as replacing 1% of OPC in concrete with FA can containing 100% OPC corresponds to the upper bound of the carbon
reduce the carbon emissions of plain concrete by 3.09 kg CO2-e/m3. emissions for each strength class. Mixed-use of 75% GGBS and 25%
A less apparent carbon reduction of 2.86 kg CO2-e/m3 can be ach- eco-cement represents the lower bound carbon emissions for all
ieved by employing 1% of GGBS in concrete. This is because GGBS concrete mix proportions. Since the carbon emissions of concrete
has a larger unit emission factor and produces slightly more carbon vary between the upper and lower bounds, manufacturers can
emissions than FA. When substitution rates of FA and GGBS are simply choose the concrete mix proportions from Fig. 8 that
equal, the carbon emissions of GGBS concrete are more than that of correspond to the minimum possible carbon emission.
FA concrete. The advantage of GGBS is the high substitution rate, For 100% OPC concrete, increasing the compressive strength by
replacing up to 75% of OPC to achieve a dramatic carbon reduction 5 MPa produces 20 kg CO2-e/m3 more carbon emissions. In addi-
in plain concrete by over 60%. tion, increasing the maximum aggregate size to 40 mm can reduce
As discussed previously, OPC accounts for over 90% of the carbon 12% of the OPC content in concrete and 60 kg CO2-e/m3 of the
emissions in plain concrete. If a large amount of GGBS is utilized, carbon emissions. For example, at least 340 kg/m3 of OPC is needed
OPC contributes less to the carbon emissions (67%) of concrete for C40 concrete containing 10 mm aggregate. If the maximum
whereas the percentage contribution of GGBS is gradually aggregate size increases to 40 mm, only 280 kg OPC is needed to
increased to 18% (see Appendix 4). It should be noted that when coat the aggregate particle surface area. As a result of the reduced
large amounts of SCMs are used in concrete, the proportion of OPC cement content, the carbon emissions of concrete become lower. A
decreases to a relatively low level and using eco-cement for carbon similar comparison has been carried out for FA and GGBS concrete.
emission reduction may become less efficient. Specifically, using It should be noted that if large amounts of SCMs and/or eco-cement
eco-cement can reduce the carbon emissions of 100% cement are used in concrete, the variation of carbon emissions between
concrete by around 30%, but the percentage decreases to only 20% two consecutive strength classes is reduced to only 5 kg CO2-e/m3.
for the concrete specimen with 75% GGBS. The results indicate that Moreover, the carbon reduction using large-sized aggregates also
increasing the amount of SCMs in concrete could degrade the effect becomes less efficient at only 14 kg CO2-e/m3. It means that
of eco-cement (by one third). This is one of the reasons why CO2 increasing the amount of SCMs/eco-cement in concrete could
emissions reduction considering different carbon mitigation mea- alleviate the effects of high strength concrete and large-sized ag-
sures together (such as Scenario 10 in Fig. 4) is less efficient than gregates. This is another reason why the combined effects of
the sum of the individual effect. different carbon mitigation measures are not as significant as the
sum of the individual effect.
592 V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597
Table 6
Relationship between different material design parameters and the embodied carbon in the building.
Concrete strength [1% (reduce concrete & steel demands, but increase per-unit carbon emissions of Y 0.13 Y Y 1.05 11% (Doubling strength)
concrete) 0.92 (0.22%)
FA [1% (decrease per-unit carbon emissions of concrete) Y 2.12 e Y 2.12 15% (35% FA)
(0.44%)
GGBS Y 1.96 e Y 1.96 30% (75% GGBS)
(0.41%)
Eco-cement (MSWI) Y 0.65 e Y 0.65 13% (100% eco-cement)
(0.13%)
Large-sized [1% (reduce OPC content) Y 0.52 e Y 0.52 8% (40 mm)
aggregates (0.11%)
Steel scrap [1% (decrease per-unit carbon emissions of steel) e Y Y 1.89 40% (100% recycled)
1.89 (0.39%)
V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597 593
reinforcement can achieve a maximum reduction of 10%e40%. If recycled steel scrap in reinforcement reduces the total building
the recommendations above-mentioned are implemented, the embodied carbon by 39%, and therefore should be encouraged.
embodied carbon in the building can be reduced to a very low level Using eco-cement reduces the embodied carbon of a reinforced
(over 70%) with 200 and 150 kg CO2-e/m2 for lower and upper concrete building by 14%, and embodied carbon can be reduced by
floors. 9% with the use of 40 mm aggregate. The findings of this study
The choice of different raw materials affects the thermal resis- serve as a decision support basis for more environmentally sus-
tance (i.e., R-value) of reinforced concrete and hence the heating/ tainable decisions in concrete production and building design. It
cooling requirements of the whole building. As compared to OPC has to be noted that the theoretical improvements are based on the
concrete, the concrete specimens containing recycled SCMs have a particular building used in this study, but the conclusions drawn
lower thermal conductivity and can potentially reduce the carbon here could be extrapolated to other concrete buildings with a
emissions from building energy use. But it is also important to similar configuration (e.g., similar mix proportions or concrete
consider the local weather condition, thermal insulation, and products with the same compressive strength, SCMs, and recycled
building configuration when analyzing the energy use due to scrap content). The actual results may differ for different buildings,
different material options. If the exterior walls comprise a thermal but the same method can be used to quantify the relevant carbon
insulation layer (e.g., polystyrene or mineral wood), the thermal emissions and to generate carbon reduction strategies.
resistance of a building will depend largely on the insulation layer.
Different choices of reinforced concrete may not significantly
Appendix A1. The effect of recycled aggregate on the carbon
impact the heating/cooling requirements. In addition, in subtropi-
emissions of concrete
cal weather where solar radiation accounts for a large proportion of
the cooling load, the thermal conductivity of glass facade plays a
To investigate the effect of recycled aggregate on the overall
more important role in determining the heating/cooling re-
CO2-e of concrete, the C35 concrete with 10 mm aggregate and
quirements. The change of concrete materials may have less sig-
100% OPC is selected as the basic mixture. Two extra mixtures, Mix
nificant effects on the carbon emissions from energy use.
1 and Mix 2, are designed with one being replaced by 20% recycled
coarse aggregate and another replaced by 20% recycled fine
5. Conclusions aggregate. Figure A1 compares the carbon emissions between a
basic mixture using natural aggregate and two alternative mixtures
In this study, a holistic approach is presented to help mitigate using recycled aggregates. The results imply that around half of the
the embodied carbon of reinforce concrete in buildings. The carbon emissions from aggregate extraction can be reduced by
method is used to design various concrete mix proportions and to replacing one kg of recycled aggregate in concrete production. In
evaluate the carbon emissions from each composition in reinforced Mix 1, the percentage contribution of natural and recycled fine
concrete production. The method also provides systematic details aggregate, i.e., 0.64% þ 0.08%, is reduced by 0.08% as compared to
to illustrate the effect of various concrete mix designs on the total the fine fraction in the basic mixture (0.80%). For Mix 2 which ap-
embodied carbon in buildings. The findings reveal more insights plies 20% recycled coarse aggregate, the contribution of the coarse
into the combined effect of various concrete design parameters on fractions, i.e., 0.73% þ 0.09%, is reduced by 0.09%. It is not suggested
the embodied carbon mitigation, which will serve as a basis to help to use recycled aggregate to reduce the CO2-e of concrete as the
optimize the carbon performance of buildings. Increasing concrete reduction is less than 1%. However, using recycled aggregate in
compressive strength by 100% reduces the amount of concrete by concrete production can reduce the demand for natural resources
36% and reduces the embodied carbon by 11%. The results also and C&D wastes disposed of at landfills. This is very important for
show that using SCMs (35% FA or 75% GGBS) reduces the embodied the small cities with local scarcity of resources and landfill spaces.
carbon of a building by 16% or 31%, respectively. Using 100%
Fig. A1. The effect of recycled aggregate on the carbon emissions of concrete.
594 V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597
Table A2.1
Mixture proportions and CO2-e emissions for C40 concrete
Sources of emission Calculated from literature data Using the proposed approach
Mixture from literature (kg/m3) Emissions (kg CO2-e/m3) Trial mixture (kg/m3) Emissions (kg CO2-e/m3)
Table A2.2
Carbon emissions of OPC concrete using 10 mm sized aggregate
Strength SCM substitutions Carbon emission of raw materials (kg CO2-e/m3) Carbon emissions of concretea
Table A2.3
Carbon emissions of OPC concrete using 40 mm sized aggregate
Strength SCM substitutions Carbon emission of raw materials (kg CO2-e/m3) Carbon emissions of concretea
Appendix A3. Concrete batching and transportation of weight materials. An effective carbon reduction approach is to
concrete constituent materials locate the concrete batching plant at a strategic position that can
minimize the transportation distance and time, or to reduce the
Concrete batching contributes 3.36 kg CO2-e/m3, being respon- returned concrete due to the slump loss during transportation.
sible for 1%e3% of the overall carbon emissions. As discussed pre-
viously, the manufacturing processes are primarily powered by
electricity (5.8 kWh/m3), with very small amounts of fossil fuels
used by the mechanical equipment and refrigerants for ice making.
Of the overall electricity consumption, the mixing equipment is the
most significant contributor (2.54 kWh/m3), which accounts for
half of the carbon emissions generated by concrete manufacture.
The remaining electricity consumption is shared by the screening
and belt conveying of aggregate, pneumatic transfer of cement and
SCMs, and other electricity usages such as lighting and air condi-
tioning throughout the manufacturing processes and office space.
The carbon emissions due to the transportation of concrete
constituent materials are estimated according to industrial average
data. The average transportation carbon emissions is estimated to
be 13.62 kg CO2-e/m3. As Figure A2 shows, transportation of OPC
from Japan contributes 43.72% of the carbon emissions associated
with transportation. It is followed by the overseas transportation of
aggregate from China (33.60%) and domestic transport of aggregate
(12.69%) and OPC (5.44%). The carbon emissions due to trans-
portations depend on the vehicle types (i.e., road transport,
waterborne shipment, and rail), transportation distance, and
weight of the cargo. The high proportion of OPC transportation
(from Japan) is related mainly to the long shipment distance, i.e., on
Fig. A2. Carbon emissions due to transportation of concrete constituent materials2
average 2500 km/trip from Japan to Hong Kong. Transportation of
aggregate from China and Hong Kong are the second and the third
largest contributors because aggregate is very bulky and heavy
596 V.J.L. Gan et al. / Journal of Cleaner Production 229 (2019) 582e597
Fig. A3. Breakdown of carbon emissions for typical C50 concrete with various amounts of SCMs (the values are taken as the average of 10 mm and 40 mm aggregates)3
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