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To cite this article: Magdy A. Ezzat, Ahmed S. El-Karamany & Mohsen A. Fayik (2012): Fractional Ultrafast Laser–Induced
Thermo-Elastic Behavior In Metal Films, Journal of Thermal Stresses, 35:7, 637-651
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Journal of Thermal Stresses, 35: 637–651, 2012
Copyright © Taylor & Francis Group, LLC
ISSN: 0149-5739 print/1521-074X online
DOI: 10.1080/01495739.2012.688662
3
Department of Mathematics, Faculty of Education, Alexandria University,
Alexandria, Egypt
Keywords: Femtosecond laser; Fractional calculus; Laplace transform; Metal film; Modified
fractional heat conduction; Numerical results; Thermoelasticity
INTRODUCTION
The so-called ultra-short lasers are those with pulse duration ranging from
nanoseconds to femtoseconds in general. In the case of ultra-short-pulsed laser
heating, the high-intensity energy flux and ultra-short duration laser beam, have
introduced situations where very large thermal gradients or an ultra-high heating
speed may exist on the boundaries. In such cases, as pointed out by many
investigators, the classical Fourier model, which leads to an infinite propagation
speed of the thermal energy, is no longer valid [1–4]. Researchers have proposed
several models to describe the mechanism of heat conduction during short-pulse
laser heating are useful for thin films [5].
When a metal film is heated by a laser pulse, a thermoelastic wave is
generated due to thermal expansion near the surface. This wave propagates into the
637
638 M. A. EZZAT ET AL.
film [3]. The thermoelastic coupling problem associated with this has been studied
extensively; for example, McDonald [6] has studied the importance of thermal
diffusion in thermoelastic wave generation. Wang and Xu [3] have studied the stress
wave induced by Pico and femtosecond laser pulses in a semi-infinite metal by
expressing the laser pulse energy as a Fourier series. Chen et al. [7] have investigated
the deformation in metal films subjected to ultrafast laser heating by considering the
dual-hyperbolic two temperatures and hot-electron blast models, and found that the
non-thermal damage could be the dominant mechanism in ultra-short laser-material
ablation.
Differential equations of fractional order have been the focus of many
studies due to their frequent appearance in various applications in fluid mechanics,
viscoelasticity, biology, physics and engineering. The most important advantage of
using fractional differential equations in these and other applications is their non-
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local property. It is well known that the integer order differential operator is a local
operator but the fractional order differential operator is non-local. This means that
the next state of a system depends not only upon its current state but also upon
all of its historical states. This is more realistic and it is one reason why fractional
calculus has become more and more popular [8–10].
Although the tools of fractional calculus were available and applicable to
various fields of study, the investigation of the theory of fractional differential
equations are started quite recently by Caputo [8]. The differential equations
involving Riemann–Liouville differential operators of fractional order 0 < < 1,
appear to be important in modeling several physical phenomena [9] and therefore
seem to deserve an independent study of their theory parallel to the well-known
theory of ordinary differential equations.
Fractional calculus has been used successfully to modify many existing models
of physical processes. One can state that the whole theory of fractional derivatives
and integrals was established in the second half of the 19th century. The first
application of fractional derivatives was given by Abel who applied fractional
calculus in the solution of an integral equation that arises in the formulation of the
Tautochrone problem. The generalization of the concept of derivative and integral
to a non-integer order has been subjected to several approaches and some various
alternative definitions of fractional derivatives appeared in [11–15].
In the last few years, fractional calculus was applied successfully in various
areas to modify many existing models of physical processes, e.g., chemistry, biology,
modeling and identification, electronics, wave propagation and viscoelasticity
[16–19]. Fractional order models often work well, particularly for dielectrics and
viscoelastic materials over extended ranges of time and frequency [20, 21]. In heat
transfer and electrochemistry, for example, the half order fractional integral is the
natural integral operator connecting the applied gradients (thermal or material) with
the diffusion of ions of heat [20]. One can refer to Podlubny [9] for a survey of
applications of fractional calculus.
A quasi-static uncoupled theory of thermoelasticity based on fractional heat
conduction equation was put forward by Povstenko [24]. The theory of thermal
stresses based on the heat conduction equation with the Caputo time-fractional
derivative, is used by Povstenko [25] to investigate thermal stresses in an infinite
body with a circular cylindrical hole. Povstenko [34] considered the generalized
Cattaneo-type equations with time-fractional derivatives, the proposed theory
LASER–INDUCED THERMO-ELASTIC BEHAVIOR IN METAL FILMS 639
1
eij = u + uji
(3)
2 ij
where i j = 1 2 3 refer to general coordinates.
640 M. A. EZZAT ET AL.
4. The equation of energy when the heat source is taken into account is:
T ˙ = −qjj + Q (4)
qi x t +
0
= −i (6)
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D f x̄ t
= t −
− d ∈ 0 1 (9)
1 −
0
7. The temporal profile of the laser pulse is non-Gaussian and given by the
following:
Jt t
J t
= 02 exp − (10)
tp tp
where J0 the intensity which is defined as the total energy carried by the pulse
per unit cross-section of the beam, For gold, this time constant is 0.75 ps [37].
8. According to Tang and Araki [38], The thermal conduction in the beam can be
modeled as
1−R x
Q x t
= exp − i J t
i = 1 2 3 (11)
x0 x0
2 u 2 u
= + 2
− 3 + 2
T (12)
t2 x2 x
2. The normal stress along the x-axis is given by the constitutive equation:
xx = + 2
exx − 3 + 2
T (13)
u
e = exx = (15)
x
4. According to heat transport in the electron gas which is assumed diffusive
(following modified Fourier’s law) and the neglected effect of conduction through
the metal lattices due to the optical depth (of laser penetration) in metals, the
modification fractional heat transport equation in the context of generalized
thermoelasticity is
2
0 1+ cE T0 1
0
= + + e − 1+ Q (16)
x2 t ! t1+ ! t
Q
ij = ij / + 2
Q = a = C0 0 L x0 = C0 x0 (18)
k2o Co4
Substituting from Eq. (18) into Eqs. (12)–(17) and dropping the primes for
convenience, we obtain the following set of nondimensional equations:
2 u 2 u
2
− = 2 (19)
x x t
2
0 1+ u
0 t t
= + + − 1 1 + exp − − (20)
x2 t ! t1+ x ! t tp2 tp
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u
xx = − (21)
x
2 T0
where = C02 0 k
, 1 = J0 1−R
k0 x0
, = x/x0 .
n−1
LDC g t
= s ḡ s
− g k
0+
s−1−k n − 1 < < n (22)
k=0
and
xx x t
t=0 = 0 (25)
For the boundary conditions, assume that the thin film is attached to a rigid
substrate with constant temperature (namely the ambient temperature). Heat losses
to the front surface is assumed to be negligible during the ultra-short laser heating
process, implying that
= 0 (27)
x x=0
x=a = 0 (28)
u
− =0 (29)
x x=0
and
u x t
x=a = 0 (30)
Hence, we obtain
2 ¯
2
− s 2
ū = (31)
x x
2 u 1
− 1 s ¯ = 1 s − 1 exp −
1 (32)
x2 x 1 + stp
2
ū
xx = − (33)
x
where 1 = 1 + !0 s
.
Eliminating ¯ between Eqs. (31) and (32), we obtain
4 2
D − s + 1 +
s1 D2 + s3 1 ū = 2 exp −
(34)
where D = d/dx, 2 = 1 1
x0 1+tp2 s
2
.
In a similar manner, we can show that ¯ satisfies the equation
4 2
D − s + 1 +
s1 D2 + s3 1 ¯ = −3 exp −
(35)
1−x2 s2
where 3 = x 0 2 .
0
The general solution of Eqs. (34) and (35) for = x/x0 ≥ 0 is
2
ū s
= B1 e−k1 + B2 e−k2 + e− (36)
k12 − 1
k22 − 1
¯ 3 e−
s
= A1 k12 − s2
e−k1 + A2 k22 − s2
e−k2 − (37)
k12 − 1
k22 − 1
Substituting from Eqs. (36) and (37) into Eq. (32), we get
1
A1 = − 1
s k12 − k2
2
(42)
−1
A2 = + 2
s k1 − k2
2 2
where
= s3 k12 − k22
k12 − 1
k22 − 1
(43)
1 = k22 s 1 +
1 − 1 + s − s 1
2 3
(44)
2 = k12 s 1 +
1 − 1 + s2 − s3 1 (45)
Hence,
¯
k12 − s2
e−k1 − k22 − s2
e−k2 1 2
s
= − k1 − s2
1 e−k1 − k22 − s2
2 e−k2
s k1 − k2
2 2
1 − s2
1 e−
− (46)
k12 − 1
k22 − 1
1 1
ū s
= −k1 e−k1 + k2 e−k2 + k1 1 e−k1 − k2 2 e−k2
s k1 − k2
2 2
1
− e− (47)
k12 − 1
k22 − 1
s −k s2
¯ xx s
= e 1 − e−k2 − 1 e−k1 − 2 e−k2
k12 − k2
2
s 1 +
1 − 1 −
− e (48)
k12 − 1
k22 − 1
Limiting Cases
Taking into consideration
f x t
− f x 0
→ 0
f x t
f x t
= I −1 0<<1 (49)
t
t
f x t
= 1
t
where the notion I n is the Riemann–Liouville fractional integral is introduced as a
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= 193 × 103 kg/m3 , T = 142 × 10−6 K−1 , ke = 315 W/m K, Ce = 21 × 104 J/m3 K,
Cl = 25 × 106 J/m3 K, = 13846 GPa, and = 2637 GPa.
Figures 5 and 6 describe the variations of the normal displacement on the front
surfaces for metal of 0.21 m thickness verses , such that when the value of the
fractional order decrease, the peak of the displacement increase the magnitude of
the displacement, as first increase very rapidly with distance attains maximum value
and then gradually decrease to zero.
From the above discussions, the presence of both the relaxation time and the
fractional order parameter has significant effect on the different field variables
of the medium, which has in some particle application can easily be taken under
consideration and accurately assessed.
CONCLUSION
The main goal of this work is to introduce a new mathematical model of
heat conduction with time fractional order for fixed thermal relaxation (taking
the memory effect into our account) for isotropic material as a new improvement
and progress in the field of thermoelasticity. The reason for this development is that
a fractional model could describe simply and elegantly the complex characteristics
of a thermoelastic material. According to this theory, we have to construct a new
LASER–INDUCED THERMO-ELASTIC BEHAVIOR IN METAL FILMS 649
NOMENCLATURE
eij Cauchy strain tensor
x one-dimensional space variable
t the physical time
S the energy source of the laser pulse
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Greek Symbols
the Lamé constants
order of the fractional derivative between 0 and 1
T the thermal expansion coefficient
mass density
o relaxation time
temperature deviation from T0
ij components of stress tensor
2
= C 2T0 k
0 0
Subscript
p pulse
0 room temperature (300 K) or reference state
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