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Monitoring radiation levels in the Pacific Northwest

The Fukushima Nuclear Crisis:Separating Fact from Fiction

Simon Fraser University

April 11, 2011

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 1 / 22
The nuclei

The nuclear chart


Number of protons Z

Number of neutrons N

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 2 / 22
Nuclear decay

Nuclear decay half-life

0 1 2 3 4
T1/2 T1/2 T1/2 T1/2

131
I 8 days
137
Cs 30 years
239
Pu 24100 years
Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 3 / 22
Nuclear fission

Nuclear fission

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 4 / 22
Nuclear fission

Fission fragments

239
Pu
Number of protons Z

235
U
238
U
232
Th

Number of neutrons N

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 5 / 22
Nuclear fission

The nuclear chart


Number of protons Z

Number of neutrons N

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 6 / 22
Fuel release

Fresh and spent nuclear fuel

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 7 / 22
Fuel release

Nuclear chain reaction

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 8 / 22
Fuel release

Plutonium

Plutonium (Pu) is a man made, radioactive, heavy element containing


94 protons.
239
Pu is produced in fuel containing 238 U.
239
Pu is the material of choice for nuclear weapons.

Mixed Oxide nuclear fuel used in one of the Fukushima reactors


contains Pu/U mixture.

The element of Pu is highly toxic when inhaled, (less toxic when


ingested).

Animal studies found that an accumulated dose of a few milligram of


plutonium per kilogram of tissue is lethal.

Traces of Pu were reported to be found at the Fukushima site (but not


talked about recently).
Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 9 / 22
Fission fragments release

Radio-iodine 131 I

131
I is a man made radioactive isotope of Iodine.
131
I has a half life of 8 days.
131
I is an abundant fission fragment.
131
I is used in radiotherapy of cancer.
131
I is not found in the atmosphere in normal conditions .
131
I is a good indicator of radioactivity release in reactor accidents,
the signal is not obstructed by background.

Iodine accumulates in the thyroid, thus large scale exposure to 131 I is


a potential health hazard.

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 10 / 22
Fission fragments release

Radioactive 137 Cs

137
Cs is a man made radioactive isotope of Cesium.
137
Cs has a half life of 30 years.
137
Cs is an abundant fission fragment.
137
Cs is used in radiotherapy of cancer and in food irradiation.
137
Cs was not present in the environment before 1940’s when fission
started to be used for nuclear power releases.
137
Cs background from nuclear weapon tests and previous nuclear
accidents obscures the signal from Fukushima.

Contamination with 137 Cs is long lasting.

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 11 / 22
Fission fragments release

Nuclear weapon tests

∼2000 reported tests ∼550 atmospheric explosions

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 12 / 22
Fission fragments release

Fission fragments release

Release depends critically on the accident scenario.

Fission fragments which exists as gases, vapours, or aerosols are


released first.

The Three Mile Island accident released gases only, including 131 I.

The explosions and fires following the Chernobyl accident resulted in


a release of 6 tons of fragmented fuel along with radioactive gases.

The release of 131 I from the Chernobyl was 2.4 million times larger
than from the Three Mile Island accident.

The crisis management at Fukushima successfully prevented


large-scale radioactivity release in the past month, however, the
cooling operates under emergency conditions.

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 13 / 22
Radiation detection

Characteristic decay spectra


137
Blue: Cs Red:60 Co

2000

1000

500

200
Counts per Channel

100

50

20

10

200 600 1000 1400 1800


Energy [arb.]

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 14 / 22
Radiation detection

GEARS: Germanium detector


for Elemental Analysis and Radioactivity Studies

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 15 / 22
Radiation detection

Background suppression

Blue: shielded Red: unshielded

1460
352
293

609

911
10 4

1121
511

2611
970

1764
728

1237

1376
Counts per Channel

2202
1508

1726
10 3

2103
1847
182
236
91

2444
10 2

10 1

200 600 1000 1400 1800 2200 2600


Energy (keV)

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 16 / 22
Monitoring of Fukushima releases

131
I signature in the SFU rainwater

511
250 March 18

352
Counts

365
150

50

511
250 March 20
352
Counts

365

150

50

511
250 March 29
352
Counts

365

150

50

340 380 420 460 500 540


Energy [keV]

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 17 / 22
Monitoring of Fukushima releases

Time profile of the 131 I signature in Burnaby rainwater


Specific activity of 131I in Burnaby rainwater
Specific activity [Bq/l]

16

14

12

10

0
03/11 03/18 03/25 04/01 04/08
Date

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 18 / 22
Monitoring of Fukushima releases

131
I sampling in seaweed

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 19 / 22
Monitoring of Fukushima releases

131
I signature in the North Vancouver seaweed

Blue: March 15 Red: March 22

511
250

352
Counts

150

50

511
250
365
352
Counts

150

50

340 380 420 460 500 540


Energy [keV]

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 20 / 22
Monitoring of Fukushima releases

Time profile of the 131 I signature in seaweed


Specific activity of 131I in seaweed
500
Specific activity [Bq/kg]

SFU North Vancouver

Bamfield Marine Science Center


400

300

200

100

0
03/11 03/18 03/25 04/01 04/08
Date

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 21 / 22
Monitoring of Fukushima releases

Time profile of the 131 I signature


Specific activity of 131I
25
Specific activity [arbitrary]

rainwater
seaweed NV
20 seaweed BMSC

15

10

0
03/11 03/18 03/25 04/01 04/08
Date

Krzysztof Starosta (SFU) The Fukushima Nuclear Crisis April 11, 2011 22 / 22

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