Professional Documents
Culture Documents
380-383 (2011)
ARTICLE
Measurement of environmental gamma-ray dose rate around
the Nuclear Fuel Cycle Engineering Laboratories, JAEA
Tomoko MIZUTANI1, Toshimitsu ONUMA1, Masamitsu SUGAI2, Hajime WATANABE2,
Masato MORISAWA1, Masanori TAKEYASU1, Shuichi SUMIYA1
1
Japan Atomic Energy Agency, Tokai-mura, Ibaraki, Japan
2
Joyo Industry Co. Ltd, Tokai-mura, Ibaraki, Japan
The Nuclear Fuel Cycle Engineering Laboratories (NCL), JAEA operates the Tokai Reprocessing Plant (TRP),
plutonium fuel fabrication facilities and the supplemental facilities. In the terrestrial environment, environmental
gamma-ray dose rate was measured continuously using an energy-thermo-compensation-type NaI(Tl) scintillation
detector. The data of environmental dose rate measured in 5 monitoring stations and 8 monitoring posts were
collected and analyzed to monitor on real-time. This paper summarizes the monitoring data of environmental dose
rate around the NCL during the past 10 year (fiscal 1998-2007). The averages of the environmental dose rate for all
monitoring stations and posts were in the range of 32-45 nGy h-1. The long-term variation in the environmental dose
rate was not found. The cases of the short-term increases occurred by the operations of the facilities in the NCL were
concluded to the discharges of 85Kr from the TRP, transportation of MOX fuels or radioactive solid wastes, X-ray
generator to calibrate the radiation monitoring instruments. The other cases to affect the change of the environmental
dose rate were the scavenging of the airborne natural radionuclides, a patient cured by the radiation therapy and the
shield effect by cars.
KEYWORDS: Tokai Reprocessing Plant (TRP), environmental gamma-ray dose rate, long-term variation,
short-term variation, krypton-85 (85Kr), external effective dose, cloud gamma, energy index
380
Measurement of environmental gamma-ray dose rate around the Nuclear Fuel Cycle Engineering Laboratories, JAEA 381
were replaced from a mainframe to a workstation in 1997. during the snowfall or the rainfall event. These values were
Then the differential values of dose rate could easily monitor about 1.8-2.4 times higher than average values. Takeyasu et
and analyze real-time by using the personal computer. The al. reported that the increases of the environmental dose
index of the incidence energy (energy index; a ratio of rate by the scavenging the short-lived Radon-progenies
gamma-ray counts these passed the energy during the rainfall event were observed when the air mass
4)
-compensation-circuit later and former) was used for the came from the Eurasia. The trajectory analysis of the air
analysis. In some locations, the monitoring installations had mass using the METEX5) resulted that the air mass caused
renewed to the devises with a multi channel analyzer, but the the snowfall or the rainfall event in both days were pass
method of the analysis was uniformly using the energy index through the Eurasia.
for all monitoring locations. (2) 85Kr discharged from the TRP
The TRP has released the radionuclides into the
III. Results and discussions atmosphere via three 90-m-high stacks by its operation of the
1. Long-term variation fuel reprocessing. Almost all the noble-gases were
The environmental dose rate during the past 10 year was discharged in the nuclear fuel shearing and dissolution
shown in Table 1, except the value influenced by the processes. Figure 2 shows the variations of the
criticality accident at the JCO in 19992). The averages of the environmental dose rate (10-minute value) observed on
environmental dose rate for all locations were in the range of October 20-23, 2003. The sharp peaks of the environmental
32-45 nGy h-1. The maximum 1-hour values were dose rate were observed at the ST or P located in the
accompanied by the rainfall or the snowfall event. The level direction of leeward, when the large amount of 85Kr
of these monitoring data was similar to the terrestrial gamma exceeded 10 TBq h-1 was dischargedin the shearing process
radiation level in Japan reported by Furukawa.3) The and the forepart of the dissolution process. The TRP
differences of the annual average of the environmental dose 㩿㪜㪥㪜㪀 㩿㪥㪀 㩿㪥㪥㪜→㪥㪜㪀 㩿㪥㪜㪀 㩷㪮㫀㫅㪻㩷㩷㪻㫀㫉㪼㪺㫋㫀㫆㫅 㩿㪥㪥㪮㪀
rate compared with the previous year were r 3% for each 㪎㪇
㪪㪫㪌
㪩㪸㫀㫅
location regardless of the operation of the TRP, except for
㪍㪇
the cases of the renewed of the instrument.
㪜㫅㫍㫀㫉㫆㫅㫄㪼㫅㫋㪸㫃㩷㪻㫆㫊㪼㩷㫉㪸㫋㪼㩷㩿㫅㪞㫐㩷㪿 㪀
㪧㪋 㪧㪍
㪄㪈
㪛㫀㫊㪺㪿㪸㫉㪾㪼㩷㫉㪸㫋㪼㩷㫆㪽㩷㪏㪌㪢㫉㩷㩿㪫㪙㫈㩷㪿㪄㪈㪀
㪧㪋
2. Short-term variations 㪌㪇
The short-term increases of the environmental dose rate
were observed mainly due to the scavenging of the airborne 㪋㪇
natural radionuclides. The cases of the short-term increases 㪪㪫㪊
occurred by the operations of the facilities in the NCL were 㪊㪇
㪪㪿㪼㪸㫉㫀㫅㪾㩷㪧㫉㫆㪺㪼㫊㫊
according to the discharges of 85Kr from the TRP,
㪉㪇
transportation of MOX fuels or radioactive solid wastes, 㪛㫀㫊㫊㫆㫃㫌㫋㫀㫆㫅㩷㪧㫉㫆㪺㪼㫊㫊
㪏㪌
X-ray generator to calibrate the radiation monitoring 㪈㪇
㪢㫉
instruments. The other cases to affect the change of the
environmental dose rate were assumed to a patient cured by 㪇
㪈㪍㪑㪇㪇
㪈㪍㪑㪇㪇
㪈㪉㪑㪇㪇
㪈㪍㪑㪇㪇
㪉㪇㪑㪇㪇
㪇㪑㪇㪇
㪋㪑㪇㪇
㪏㪑㪇㪇
㪈㪉㪑㪇㪇
㪉㪇㪑㪇㪇
㪇㪑㪇㪇
㪋㪑㪇㪇
㪏㪑㪇㪇
㪈㪉㪑㪇㪇
㪉㪇㪑㪇㪇
㪇㪑㪇㪇
㪋㪑㪇㪇
㪏㪑㪇㪇
㪜㫅㫍㫀㫉㫆㫅㫄㪼㫅㫋㪸㫃㩷㪻㫆㫊㪼㩷㫉㪸㫋㪼㩷㩿㫅㪞㫐㩷㪿 㪀
r㪉㩷㪔㩷㪇㪅㪐㪋㪎㪋㩷
㪄㪈
㪏 㪏
㪠㫅㪻㪼㫏㩷㫆㪽㩷㫋㪿㪼㩷㫀㫅㪺㫀㪻㪼㫅㪺㪼㩷㪼㫅㪼㫉㪾㫐㩷㩿㩼㪀
㪉㪅㪇㪜㪄㪇㪋㪄㪋
㪉㪅㪇㬍㪈㪇
㪏㪇 㪇
㪻㫆㫊㪼㩷㫇㫆㫀㫅㫋㩷䋨㫄㪪㫍㩷㫐 䋩
㪄㪈
㪍 㪍
㪎㪇 㪇
㪈㪅㪌㪜㪄㪇㪋㪄㪋
㪈㪅㪌㬍㪈㪇
㪍㪇 㪋㪇 㪋
㪄㪋
㪈㪅㪇㪜㪄㪇㪋
㪈㪅㪇㬍㪈㪇 㪌㪇 㪇
㪉 㪉
㪋㪇 㪇
㪌㪅㪇㪜㪄㪇㪌㪄㪌
㪌㪅㪇㬍㪈㪇
㪇 㪇
㪊㪇 㪇
㪇㪅㪇㪜㪂㪇㪇 㪉㪇 㪄㪉㪇 㪄㪉
㪈㪋㪑㪇㪇
㪈㪋㪑㪊㪇
㪈㪌㪑㪇㪇
㪈㪌㪑㪊㪇
㪈㪍㪑㪇㪇
㪇 㪇
㪈㪌㪑㪇㪇
㪈㪊㪑㪊㪇
㪈㪋㪑㪇㪇
㪈㪋㪑㪊㪇
㪈㪊㪑㪇㪇
㪇㪅㪉 㪇㪅㪋 㪇㪅㪍 㪇㪅㪏
㪘㫄㫆㫌㫅㫋㩷㫆㪽㩷㫊㫇㪼㫅㫋㩷㪽㫌㪼㫃㩷㫉㪼㫇㫉㫆㪺㪼㫊㫊㪼㪻㩷䋨㪞㪮㪸㩷㫐㪄㪈 䋩
Fig. 3 Correlation with the external effective doses calculated (b) 㪈㪇㪇 㪈㪇
for the cloud gamma by the mathematical model and the
㪐㪇 㪏
㪜㫅㫍㫀㫉㫆㫅㫄㪼㫅㫋㪸㫃㩷㪻㫆㫊㪼㩷㫉㪸㫋㪼㩷㩿㫅㪞㫐㩷㪿 㪀
amount of spent fuel reprocessedin the TRP
㪠㫅㪻㪼㫏㩷㫆㪽㩷㫋㪿㪼㩷㫀㫅㪺㫀㪻㪼㫅㪺㪼㩷㪼㫅㪼㫉㪾㫐㩷㩿㩼㪀
㪄㪈
㪏㪇
conducted that the nuclear fuel shearing and dissolution 㪍
processes in batch mode, the pattern of such a temporary 㪎㪇
㪋
increase of the environmental dose rate along the discharge 㪍㪇 㪯㪄㫉㪸㫐㩷㫀㫉㫉㪸㪻㫀㪸㫋㫀㫆㫅
amount of 85Kr was due to the operating mode of the TRP. 㪉
By the way, because the level of the additional dose rate 㪌㪇
㪈㪌㪑㪇㪇
㪈㪌㪑㪊㪇
discharge data and mathematical models.6) The maximum 㪈㪋㪑㪊㪇
㪈㪍㪑㪇㪇
dose point outside the periphery monitoring area of the NCL
(c) 㪈㪇
was evaluated in the vicinity of the site boundary of 500 m in
the southwest direction except for fiscal 1999. Because of 㪈㪊㪇 㪏
the maintenance of the exhaust equipment of the TRP in
㪜㫅㫍㫀㫉㫆㫅㫄㪼㫅㫋㪸㫃㩷㪻㫆㫊㪼㩷㫉㪸㫋㪼㩷㩿㫅㪞㫐㩷㪿 㪀
㪠㫅㪻㪼㫏㩷㫆㪽㩷㫋㪿㪼㩷㫀㫅㪺㫀㪻㪼㫅㪺㪼㩷㪼㫅㪼㫉㪾㫐㩷㩿㩼㪀
㪄㪈
㪏㪑㪊㪇
㪐㪑㪇㪇
㪐㪑㪊㪇
㪈㪇㪑㪇㪇
㪈㪇㪑㪊㪇
㪈㪈㪑㪇㪇
㪜㫅㫍㫀㫉㫆㫅㫄㪼㫅㫋㪸㫃㩷㪻㫆㫊㪼㩷㫉㪸㫋㪼㩷㩿㫅㪞㫐㩷㪿 㪀
The NCL installed in X-ray generator to calibrate the 㪧㪊
㪄㪈
㪌㪇
㪇㪑㪇㪇
㪇㪑㪇㪇
㪇㪑㪇㪇
㪇㪑㪇㪇
㪇㪑㪇㪇
㪇㪑㪇㪇
㪇㪑㪇㪇
㪇㪑㪇㪇
㪇㪑㪇㪇
㪇㪑㪇㪇
㪏㪆㪈㪋
㪇㪑㪇㪇
㪇㪑㪇㪇
㪏㪆㪌
㪏㪆㪎
㪏㪆㪈㪇
㪏㪆㪈㪈
㪏㪆㪈㪉
㪏㪆㪈㪊
㪏㪆㪈㪌
㪏㪆㪍
㪏㪆㪏
㪏㪆㪐
㪏㪆㪋
corresponded to 120-150 keV and agreed well with the mean
energy of 122 keV evaluated by the gain of the X-ray Fig. 5 Variations of the environmental dose rate in case of the
generator. shield effect by carsduring August 4-15, 2007
(5) Patient cured by the radiation therapy
In ST5 and P6, the 1-minute values of the environmental TRP was not found. The external effective doses calculated
dose rate were increased in 61 and 90 nGy h-1 by turns (see for the cloud gamma by using the discharged data and the
Fig. 4(c)). Both ST5 and P6 were away at about 1 km and mathematical model were on the order of 10-4 mSv y-1 in
their locations were adjacently the material place of the case of the TRP reprocessed the nuclear fuels. The cloud
private company in ST5 and the general road in P6. The gamma dose from the TRP estimated to be 2.8 u 10-4 mSv
energy index had decreased from 8% to 3.7% in ST5 and GWa-1. The short-term variations of the environmental dose
from 9% to 2.7% in P6. The gamma-ray energy that rate caused by the 85Kr discharged from the TRP, the
contributed to the increase of the environmental dose rate transportation of nuclear materials, X-ray irradiation, a
corresponded to 100-120 keV. The result of the spectrum patient cured by the radiation therapy could presume the
analysis with the multi channel analyzer installed in ST5 causes by using the data of the energy index and
found the peak of the energy range from 50 to 150 keV meteorological observation data.
apparently, and supported the result of the energy index
analysis. Recently, the radioactive medicine such as 99mTc Acknowledgment
and 67Ga emitting the mean gamma-ray energy of 141 keV The authors would like to thank K. Shiba, T. Yoshida and
and 160 keV, respectively, are generally used. Therefore, it Y. Ito of Japan Atomic Energy Agency.
was assumed that the traffic of the patient cured by the
radiation therapy became the cause of the increases of the References
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(6) Shield effect by cars Weighting Function Method for Environmental Radiation
The decline of the environmental dose rate was observed Measurements, JAERI-M 7066, Japan Atomic Energy Research
Institute, (1977), [in Japanese].
in P2 faced to the parking area of the employee in the NCL.
2) K. Shinohara, et al., The Results of the Environmental
As shown in Fig. 5, the levels of the environmental dose rate Monitoring Related to the Criticality Accident in JCO,
in the daytime of work day clearly declined about 4 nGy h-1 JNC-TN8440 2001-004, Japan Nuclear Cycle Development
in P2. This amount of the decline of the environmental dose Institute, (2001), [in Japanese].
rate was larger than the range of the day cycle due to the 3) M. Furukawa, “Data synthesis for terrestrial gamma radiation
diffusion of the Radon-progenies. The variation of the level measured on the Japanese Islands and their adjacent ocean
environmental dose rate at night and holiday was comparable floor”, Proc. Int. Conf. on Isotopes in Environmental Studies -
as P3 where no traffic and parking of cars. Sakaue et al. Aquatic Forum 2004, Monaco, Oct. 25-29, 2004, p.248 (2004). G
reported that the environmental dose rate measured by the 4) M. Takeyasu, T. Iida, M. Takeishi, “Analysis of Rn-222
NaI(Tl) scintillation detector fixed on the roof of a car Concentration in the upper Atmosphere during Rainfall Using the
declined 20% by the shield effect of the car compared with Wet Scavenging Model for its Decay Products”, Proceedings of
AOCRP-2, Beijing, China, Oct. 9-13, 2006, p.752 (2006).
the case where there was no car.7) Thus, it was concluded
5) Y. Fujimura,Data Analysis and Graphic Display System for
that the decline of the environmental dose rate was caused by Atmospheric Research Using PC, CGER-M-14-2003, National
the shield effect by cars in the location of adjoining the Institute for Environmental Studies, Japan (2003).
parking area. 6) K. Shinohara, T. Asano, “Environmental dose assessment for
low-level radioactive effluents discharged from Tokai reprocessing
IV. Conclusions plant”, Health Physics, 62 [1], 58 (1992).
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New Carborne Radiation Monitoring System”, Annual Report of the
measured around the NCL. At the fiscal period from 1998 to
Niigata Prefectural Radiation Monitoring Center [5], p.45, Niigata
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