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The International Journal of Life Cycle Assessment (2020) 25:2050–2062

https://doi.org/10.1007/s11367-020-01815-8

LIFE CYCLE SUSTAINABILITY ASSESSMENT

Could the recycled yarns substitute for the virgin cotton yarns:
a comparative LCA
Yun Liu 1,2 & Haihong Huang 1,2 & Libin Zhu 1,2 & Cheng Zhang 3 & Feiyue Ren 1,2 & Zhifeng Liu 1,2

Received: 18 January 2020 / Accepted: 17 August 2020 / Published online: 28 August 2020
# Springer-Verlag GmbH Germany, part of Springer Nature 2020

Abstract
Purpose Cotton yarns spun from natural fibers are widely used in the apparel industry. Most of waste cotton goods are now
disposed by incineration or landfill, which brings resource and environmental challenges to the society. Using the waste cotton to
spin yarns is an alternative way to forward a more sustainable future. In this research, two scenarios for the environmental impacts
of yarns spun from corresponding fibers are investigated, including recycled cotton fibers and virgin cotton fibers.
Methods The life cycle assessment (LCA) has been conducted according to the collected data from on-site investigation of
typical production factories. The life cycle for the recycled cotton yarn production is divided into five stages, i.e., raw material
acquisition, transportation, breaking, mixing, and spinning. The life cycle of virgin cotton yarn production is been divided into
four stages, i.e., raw material acquisition, transportation, mixing, and spinning. The functional unit is 1000 kg produced yarns
which are used for weaving into the fabrics. Notable impacts on climate change, fossil depletion, water depletion, and human
toxicity were observed.
Results The life cycle impact assessment (LCIA) results show that environmental impacts of recycled cotton yarns are far less
than those of virgin cotton yarns, except for climate change and water depletion. The reason is that the land occupation and
irrigation water have great impact on environmental impacts of cotton cultivation. In spinning, the electricity is the key factor
whose environmental impacts account for the most in the virgin cotton yarn scenario, while the electricity and water consump-
tions are the key factors for the recycled cotton yarn scenario in the life cycle of yarn production. The sensitivity analysis indicates
that improving energy efficiency can significantly reduce environmental burdens for both the two scenarios. The uncertainty
distribution of water depletion, human toxicity, fossil depletion, and climate change of the two scenarios were determined with a
90% confidence interval.
Conclusions The LCIA results reveal recycled cotton yarn is a viable alternative to relieve resource and environmental pressure.
About 0.5 ha of agricultural land can be saved, 6600 kg CO2 eq can be reduced, and 2783 m3 irrigation water can be saved by
using 1000 kg of the recycled cotton yarns. It can be concluded that the recycled cotton fibers can be served as a substitute for
virgin cotton fibers to reduce agricultural land and avoid environmental impacts generated from the cotton planting.

Keywords Life cycle assessment . Environmental impact . Virgin cotton yarns . Recycled cotton yarns . Spinning

1 Introduction
Responsible editor: Zuoren Nie
Cotton is one of the most important crops in the world and it
* Haihong Huang plays a vital role in national economic growth. Cotton fibers, a
huanghaihong@hfut.edu.cn type of natural fibers, are widely used in apparel industry. In
2015, 5.6 × 109 kg cotton fibers were produced and more than
1
School of Mechanical Engineering, Hefei University of Technology, 3.5 × 106 ha agricultural land were used for cotton planting in
193 Tunxi Road, Hefei 230009, People’s Republic of China China (National Bureau of Statistics 2017). The large-scale
2
Key Laboratory of Green Design and Manufacturing of Mechanical consumption of cotton in China has become a non-
Industry, Hefei University of Technology, 193 Tunxi Road, negligible challenge to agricultural land occupation.
Hefei 230009, People’s Republic of China
Moreover, a large number of cotton fibers are consumed in
3
School of Mechanical Engineering, Nantong University, 9 Seyuan the apparel industry each year, which results in considerable
Road, Nantong 226019, People’s Republic of China
Int J Life Cycle Assess (2020) 25:2050–2062 2051

waste cotton goods are produced. As the largest producer and textile wastes (Esteve-Turrillas and De 2017). The recycled
exporter of textiles in the world, 3.4 × 1010 kg of yarns and 8.9 cotton fibers refrain from generating high amounts of waste-
× 109 meters of fabrics were produced in China in 2014 water in dyeing plants (Roos and Peters 2015). As the
(National Bureau of Statistics 2019) and there was a little recycled cotton yarn is dyed before recycling, there is savings
utilization rate of recycled cotton fibers. About 87% of the in water, energy, dyes and auxiliaries, and effluent treatment
waste cotton fabrics were treated by incineration or landfill cost (Niinimäki and Hassi 2011). The recycled cotton fiber
(Chinese Academy of Engineering. 2018). Thus, development was extracted from the denim cut waste by mechanical means
of waste cotton fibers has great significance for improving and blended with virgin cotton to produce recycled cotton
environmental performance, and the way that how to treat yarns using different blend ratios (Radhakrishnan and
waste cotton goods becomes an environmental challenge to Kumar 2018). This method of recycling denim cut waste is
the society. In the context of economic issues and environ- adopted by some clothing companies, such as H&M, Adidas,
mental protection, it is necessary to seek a substitute for the M&S. Thus, in terms of environmental impacts, the recycled
cotton fibers in the apparel industry to mitigate environmental cotton certainly deserves more research attention for being
burdens. The recycled cotton fibers have attracted much atten- used as a feedstock in the apparel industry.
tion because of their economic value and environmental Due to the diversity of cotton textile products, it is difficult
performance. to evaluate the environmental performance of per textile prod-
Many researchers focused on the application of waste cot- ucts (Liu et al. 2020). The environmental impacts of these
ton products and addition economic value. The textile waste products can be evaluated by considering that of the compo-
primarily can be recycled in the form of reuse and conversion sition of the products. These products are made up of the
into low-value or value-added products. Some innovative fabrics and the fabrics are woven of yarns, and the yarns are
products are developed from recycled fibers, like insulation spun from the fibers. Moreover, the mechanical properties of
materials for acoustics, recycled polyester fabrics for uni- recycled cotton yarns are weaker than virgin cotton yarns
forms, and heavy-duty canvas material (Ahmad et al. 2016). since the second use of the recycled cotton fibers. The
Wanassi et al. (2016) have reported that waste yarns can pro- recycled cotton fibers are uniformly mixed with virgin fibers
duce a new low-cost yarn that has similar physical and me- in a certain proportion and spin to yarns (shown in Fig. 1).
chanical properties comparing with 100% cotton yarn. Yarns are spun from different proportions of different fibers
According to the research of Pegoretti et al. (2014), the that have different energy and resource consumptions.
recycled cotton fibers were applied to acoustic automotive Therefore, it is necessary to assess the environmental impacts
components in the Brazilian automotive sector. Wang et al. of yarns considering the recycled and virgin cotton fibers.
(2017) confirmed that the high-value cellulose nanocrystals Summarized above, although the application of recycled
obtained from waste cotton cloth exhibited a high crystallinity textile products has been investigated, the environmental per-
index. The cotton waste was also utilized to make building formance of virgin and recycled yarns, which can be woven
materials, which helps in solid waste management and gener- into varieties of textile products, has not been well studied so
ates additional revenue (Rajput et al. 2012). Therefore, far. Therefore, the paper focuses on evaluating the environ-
the recycled cotton can be applied to various products because mental impacts of yarns spun from recycled cotton fibers and
of certain addition economic value. virgin cotton fibers by using LCA methodologies. The LCA
The environmental performance of recycled cotton fibers for these yarns has great significance on evaluating the envi-
has also attracted much attention. Sandin and Peters (2018) ronmental impacts of recycled yarn products and identifying
provide strong support for claims that textile reuse and the opportunities to reduce their environmental impacts from
recycling reduce environmental impact compared with incin- the beginning of product design. It can provide the quantita-
eration and landfilling, which based on a summary of forty- tive value to support the popularization of recycled cotton and
one studies. Since there is no textile recycling plant in help to reduce the overall environmental impact in the apparel
Sweden, Zamani et al. (2014) have explored that the potential industry.
environmental benefits of various textile recycling techniques
and it can save 1.0 × 104 kg CO2 eq and 169 GJ of primary
energy through the integration of these recycling technologies. 2 Methods
A comparative life cycle assessment of recycled cotton has
been made by Esteve-Turrillas and De (2017); the results The study uses the “cradle-to-gate” approach to analyze envi-
show that high-quality textiles have advantages over environ- ronmental impacts of the virgin cotton yarns and the recycled
mental impacts and electricity consumption when the recycled cotton yarns. The life cycle for the recycled cotton yarn pro-
cotton is applied to their production. The environmental im- duction has been divided into five stages, i.e., raw material
pacts associated with cotton cultivation and fibers dyeing are acquisition, transportation, breaking, mixing, and spinning.
avoided when recycled cotton fibers are obtained from cutting The life cycle of virgin cotton yarn production has been
2052 Int J Life Cycle Assess (2020) 25:2050–2062

Fig. 1 The process of the fabrics


production that using virgin fibers
and recycled fibers

divided into four stages, i.e., raw material acquisition, trans- are uniformly mixed with other type fibers in a certain propor-
portation, mixing, and spinning. tion and spun to yarns. Since in this paper the dyeing process
is not included in the life cycle stages of recycled cotton yarns,
2.1 Goal of study the process is not considered in virgin cotton yarn scenario
accordingly. Fig. 2 describes the system boundaries of the two
The goal of the study focuses on evaluating and comparing the scenarios.
environmental impacts of the yarns spun from virgin cotton The production flow of the virgin cotton yarn scenario
fibers and the yarns spun from recycled cotton fibers. The includes two main stages:
improvement opportunities from the manufacturer’s perspec-
tive are identified to support the popularization of recycled & The virgin cotton fibers are uniformly mixed. Considering
cotton fibers. Fashion designers can then take environmental the environmental performance of cotton products, the
performance into consideration when determining the material BCI (Better Cotton Initiative) cotton and organic cotton
design schemes during their works. may be adopted for decreasing the environmental impacts.
& The mixed fibers are finally spun into cotton yarns
2.2 Functional unit through 10 processes in the spinning phase, including
picking, carding, combing, drawing, roving, spinning,
The functional unit (FU) of the product provides a quantified winding, packaging, dust elimination, and air condition.
reference for all relevant inputs and outputs in the LCA anal-
ysis. In this study, the FU is 1000 kg produced yarns which are The production flow of the recycled cotton yarn scenario
used for weaving into the fabrics. It provides the counting base contains three main stages:
of all the process flows as the two systems consider yarn
production with the same use. & The recycled cotton fabrics or yarns are broken through
The mechanical properties of recycled cotton fibers are five processes, i.e., washing, breaking, separating, open-
weaker than virgin cotton fibers since the second use of the ing, and packaging.
recycled cotton fibers. Generally, the recycled cotton fibers & Recycled cotton fibers are uniformly mixed.
are uniformly mixed with virgin fibers in a certain proportion & The mixed recycled fibers are finally spun into recycled
and spun to yarns. In the context of small proportion of cotton yarns through 10 processes that same as virgin
recycled fibers which are mixed with virgin fibers for the cotton yarn production.
functional unit, the environmental impacts of fabrics can be
calculated by summing the environmental impacts of yarns
spun from different fibers.
2.4 Life cycle inventory
2.3 System boundaries
The LCA for yarns spun from virgin cotton fibers and
Those system boundaries are established by the general pro- recycled cotton fibers are performed to evaluate environmen-
cess of material inputs and pollution emissions to the environ- tal impacts on these yarns. The life cycle inventory (LCI) data
ment. Note that the dyeing process is not included in recycled for the two scenarios are shown in Table 1. All the inputs and
cotton yarn scenarios because the colors of recycled cotton outputs of the two scenarios are revealed in LCI table. The
fibers are determined by the waste cotton products. inventory data are collected by on-site investigation of typical
Moreover, in the related factories, the recycled cotton fibers production factories.
Int J Life Cycle Assess (2020) 25:2050–2062 2053

Fig. 2 System boundaries: a virgin cotton yarn scenario, b recycled cotton yarn scenario

2.4.1 Cotton cultivation model for calculating ammonia emissions and nitrous oxide
after the application of mineral fertilizers is incorporated in the
In the cotton cultivation stage, the survey on 10 farmers is following equation:
performed to collect the annual yield of cotton fibers, as well M
as the consumption of fertilizers and pesticides. The result N H 3 ¼ ð17=14Þ  ∑ ðEFam  p  N min þ EFbm  ð1−pÞ  N min Þ
m¼1
shows that generally, 8–10 kg of the urea, 35–40 kg of com-
pound fertilizer, 0.8–1 kg of the pesticides, and 1.8–2.0 L of ð1Þ
fuel oil are required for gaining 100 kg of cotton fibers. The where NH3 is ammonia emission after mineral fertilizer
compound fertilizer includes pure nitrogen, phosphorus pent- application (kg NH3), m is the fertilizer type, M is the
oxide, and potassium oxide. The pesticides are used and number of fertilizer types, EFam is an emission factor
sprayed 4 times in the growth life of cotton. on soils with pH < = 7 (kg NH3-N/kg N), EFbm is an
Because of the residual effect after fertilizers and pesticides emission factor on soils with pH > 7 (kg NH3-N/kg N),
used, the ammonia (NH3), nitrous oxide (N2O), and heavy p is fraction of soils with pH < = 7 (%/100), and Nmin
metal emissions are considered. According to the research of is a mineral fertilizer application (kg N).
Nemecek et al. (2014) and Khoshnevisan et al. (2018), the
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Table 1 Life cycle inventories of


yarns spun from virgin cotton Processes Categories Unit Virgin cotton fiber Recycled cotton fiber
fiber and recycled cotton fiber
Cotton - Virgin cotton kg 1210 0
Input Planting Cotton seeds kg 4 0
Planting Urea kg 121 0
Planting Compound fertilizer kg 484 0
Planting Pesticides kg 12.1 0
Planting Fuel oil L 22.9 0
- Recycled fabrics/yarns kg 0 1450
Breaking Electricity kWh 0 157
Breaking Industrial water m3 0 13.9
Breaking Cleaning agents kg 0 6
Breaking H2SO4(98%) kg 0 5.1
Breaking FeSO4 kg 0 6
Breaking PAC kg 0 1.29
Breaking PAM kg 0 0.08
Breaking NaClO (10%) kg 0 10.5
Breaking Urea kg 0 0.04
Breaking Scale inhibitor kg 0 0.056
Breaking NaHSO3 kg 0 0.056
Breaking NaOH (98%) kg 0 0.1
Breaking HCl (35%) kg 0 0.33
Mixing Electricity kWh 7 7
Spining Industrial water m3 8.3 8.3
Spining Electricity kWh 3984 3984
Spining Cartons kg 77 77
Spining PE plastic belt kg 2.43 2.43
Output Planting NH3 kg 32.03 0
Planting N2O kg 26.38 0
Planting Heavy metal (total) g 67.27 0
Breaking Solidified sludge kg 0 23.8
Breaking COD g 0 1675.9
Breaking Ammonium g 0 14.4
Breaking Phosphorus g 0 13.7
Breaking Anilines g 0 7.5
Breaking Suspended substance g 0 289.2
Breaking BOD5 g 0 289.2
Breaking Chlorine dioxide g 0 1.04
Breaking AOX g 0 1.96
Breaking Chromium(+VI) g 0 0.11
Breaking Nitrogen g 0 63.6
Breaking Sulfide g 0 1.15
Breaking Antimony g 0 0.01
Product Spining Yarns kg 1000 1000
Spining By-product kg 210 210

*
PAC poly aluminum chloride, PAM polyacrylamide, COD chemical oxygen demand, BOD5 biochemical oxy-
gen demand, AOX absorbable organic halogen

where Mleach,i is agricultural-related heavy metal i emission, m-


N 2 O ¼ ð44=28Þ  ð0:01 ð2Þ
leach,i is average amount of heavy metal emission, and Ai is allo-
 ðN tot þ N cr þ ð14=17Þ  N H 3 þ ð14=16Þ  N O2 Þ cation factor for the share of agricultural inputs in the total inputs
for heavy metal i.
þ 0:0075  ð14=62Þ  N O2 Þ
Moreover, since the agricultural machinery can be used for
where N2O is an emission of N2O (kg N2O ha-1), Ntot is total many times and has very long life, it is excluded in the LCA
nitrogen in mineral and organic fertilizer (kg N ha-1), Ncr is nitro- analysis. The fuel oil consumed is considered in LCI. About 1.8–
gen contained in the crop residues (kg N ha-1), NH3 is the loss of 2.0 L of fuel oil is required for gaining 100 kg of cotton fibers.
nitrogen in the form of ammonia (kg NH3 ha-1), NOx is the loss of
nitrogen in the form of nitrogen oxides (kg NO2 ha-1), and NO3 is
the loss of nitrogen in the form of nitrate (kg NO3 ha-1). 2.4.2 Fabrics/yarns breaking

M leach;i ¼ mleach;i  Ai ð3Þ In the fabrics/yarns breaking stage, these cotton fabrics/yarns
are washed before being broken. Those cotton fabrics/yarns
Int J Life Cycle Assess (2020) 25:2050–2062 2055

are washed by the washing devices XGP-400, drying with 2.5 Data sources
sunshine, and no ironing. The max capacity of washing device
is 400 kg and output power is 11 kW. The liquor-to-fabrics The primary data of the two scenarios are taken from on-site
ratio in washing process is 15:1. investigation of typical production factories. The factories
The washing process is the main contributor to the water were located in Zhejiang province in China and the annual
consumption in this stage, which results in an equal volume of production of cotton yarns was 2.1 × 107 kg in 2017. The
wastewater. The wastewater is treated by the wastewater treat- upstream data (i.e., the raw materials acquisition, transport,
ment system, 36.3% of which is used as recycled water, and and energy generation) are acquired from GABI database.
the remaining is discharged to the municipal sewage treatment The coal-electricity is used for producing the yarns.
plant after satisfying the required quality standards for dis- However, the industrialization production of recycled cotton
charge (GB4287-2012. 2013) in China. yarns has not been formed yet. This technique needs further
decreasing loss rate of the cotton fibers. In this research, the
recycled fibers are obtained by breaking 50% of waste fabrics
2.4.3 Mixing
and 50% of waste yarns. The mass loss rate of the cotton fibers
is nearly 20% after the process of fabrics breaking. The waste
In the mixing stage, two or more kinds of colored fibers were
fabrics are obtained from the enterprise engaged in the recov-
fully mixed. The yarns offer a great variety of colors, and the
ery of waste clothes and the waste yarns are leftover materials
effect of mixing colors is formed by mixing different colored
of the yarn production in the related factories.
fibers. The mixed ratio of colored fibers in melange yarn
products is between 0.5 and 100%. Since the color of recycled
2.6 Assumptions
cotton fibers is not considered when it is used secondly, the
color of virgin cotton fibers is also not considered in this
To facilitate the implementation of the LCA, some assump-
research.
tions are made in this study and listed as follows:
Furthermore, considering the environmental performance
of cotton products, the BCI cotton, organic cotton, and com-
& Human labor, packaging materials, device maintenance,
mon cotton may be adopted for decreasing the environmental
and administration overheads were excluded.
impacts. Moreover, the recovery mode and fiber types have
& The engineering construction and machines are not in-
strong effect on the performance of recycled cotton yarns.
cluded in the LCA system boundary, since the energy
Thus, the cotton fibers are expected to be uniformly mixed
and material data about factory buildings and machines
for improving the performance of the yarns.
are difficult to obtain.
& The distance between the cotton cultivation origin in
2.4.4 Spinning Xinjiang province and the factory in Zhejiang province
is assumed to be 4650 km by truck (Google map). It
In the spinning stage, the yarns are generated by spinning the should be noted that the transportation distance is consid-
fibers after the mixing stage. This stage has the largest energy ered a constant in this research, since the environmental
consumption compared with other phases. Notably, since the impacts generated from the transportation (less 1% of total
two fibers have no effect on the processes and equipment environmental impacts) are small and the contributions of
used, the energy and water consumption are the same in this cotton transportation to all impact categories are not sen-
phase for the two fibers. Water is only consumed by air con- sitive to the transportation distance in the whole life cycle
ditioner which used to adjust humidity and temperature for (Zhang et al. 2015).
ensuring normal operation of the machines. The dust elimina- & The average distance between the factory of yarn manu-
tion devices are adopted for absorbing the dust generated from facturers and the enterprises located in the local or nearby
the picking, carding, and combing, and the dust produced by cities engaged in recovery of waste clothes is assumed to
these processes can be absorbed by the dedusting devices, so be 100 km by truck.
that the PM2.5 or PM10 in the workshop is same as outdoor.
Auxiliary processes are essential to guarantee its regular pro-
duction including lighting, handing, dust elimination, air com- 2.7 Impact assessment
pressor, office, and other processes. In addition, during the
production of per function unit melange yarns, 0.21 t by- ReCiPe is an assessment method that allows performing the
products were produced according to the annual yield of yarns study at an impact (mid-point) or damage (end-point) category
in 2017. The environmental impacts of the by-products are level (Goedkoop et al. 2013). The ReCiPe mid-point (H)
allocated to yarns according to the price of yarns and by- method was used for life cycle impact assessment (LCIA) of
products (Liu et al. 2020). two scenarios. The impact categories (15 categories) were
2056 Int J Life Cycle Assess (2020) 25:2050–2062

considered based on LCI results, including climate change, 2 × 103 kg C/ha year. Considering the per FU cotton cultiva-
terrestrial acidification, freshwater eutrophication, marine eu- tion, about 0.58 ha of land was needed to satisfy manufac-
trophication, ozone depletion, water depletion, metal deple- turers’ feedstock demands. Thus, about 1160 kg C are stock-
tion, fossil depletion, freshwater ecotoxicity, marine ing in the soil and the transformed CO2 is 3811 kg.
ecotoxicity, terrestrial ecotoxicity, human ecotoxicity, ioniz- Above all, considering the carbon emissions caused by land
ing radiation, particulate matter formation, and photochemical occupation and the carbon storing in soil, the carbon emissions
oxidant formation. associated with soil is 6.6 × 103 kg CO2 eq. The carbon emis-
sions associated with yarn manufacturing are 4560 kg CO2.
Therefore, the carbon emissions associated with virgin cotton
3 Result yarns are 1.1 × 104 kg CO2 eq, when the carbon emissions
caused by land occupation and the carbon storing in soil are
3.1 LCIA results take into account. However, the environmental impacts of
recycled cotton yarns are not affected by agricultural land due
The environmental impacts of all processes about the two to the use of recycled cotton as raw material, which only emit-
scenarios are calculated. The LCIA results of two scenarios ted 4380 kg CO2 eq in its production.
in all selected categories are presented in Table 2.
The impacts of two scenarios were mainly attributed to 3.1.2 Water use
climate change, fossil depletion, water depletion, and human
toxicity, whereas the remaining categories minimally contrib- Considering the irrigation water during cultivation, the water
uted to the overall environmental burdens. Fig. 3 presents the footprint is introduced for calculating the consumed water of
relative contribution of each different life cycle stage to the cotton cultivation. Green water footprint (WFgreen), blue water
main impact category for the production of the yarn. The footprint (WFblue), and grey water footprint (WFgrey) of global
potential impacts generated from the transportation phase crop production in a spatially explicit way for the period 1996–
and the mixing phase were noted to be insignificant. The spin- 2005 were quantified by Mekonnen and Hoekstra (2011).
ning stage is the dominant contributor towards most of impact Those data are sharing the water footprint website with the form
categories, excepting water depletion. Contributions to the of database (waterfootprint.org). It shows that WFgreen, WFblue,
categories are primarily attributable to the fiber acquisition and WFgrey of 1000 kg cotton fibers are 1400 m3, 250 m3, and
stage, which is the cotton cultivation for the virgin cotton 650 m3 at the national level, respectively. Accordingly, the
scenario, and the fibers recycling for the recycled cotton water required for per FU melange yarns in cotton cultivation
scenario. is 2783 m3 based on the research of Hoekstra. Considering the
water consumed in production, the water consumption of virgin
3.1.1 Carbon emissions cotton fibers is 3514m3. According to the calculation of the
LCA, the category of water depletion associated with recycled
In fact, land use has effect on the ecosystem. Liu et al. (2010) cotton yarn manufacturing stages is 583 m3. It can be seen that,
have developed a model for calculating the carbon emission for the category of water depletion, the recycled cotton scenario
caused by land occupation. For the calculation of land occu- is superior to the virgin cotton scenario because of the irrigation
pation impact, the model with Chinese characterization factors water consumption.
was developed for quantifying the damages to environment by
land use in terms of the change in net primary productivity of 3.1.3 Land occupation
ecosystem. Considering the land type is the semidesert, the
characterization factor of land occupation is 597 g C/m2a. The agricultural land occupation is an important factor for
According to the land occupation of per FU cotton, the carbon evaluating the category of land use. According to the agri-
emissions caused by land occupation are 3462.6 kg C, and it cultural land of cotton and annual harvest yield of Xinjiang
transforms 1.14 × 104 kg CO2 based on its molecular weight. province of China in 2017, about per hectare average output
It is noteworthy that the cultivation land can be stored in of cotton is 2079.3 kg (National Bureau of Statistics. 2017).
soil with the form of soil organic carbon (SOC) because of the It means that 0.58 ha agricultural land is needed to grow
decomposition of humus. The SOC stock changes reflect the cotton.
differences between long-term input of litter (above and below
ground) from trees and decomposition of dissolved organic 3.2 Main contributors
carbon (Jandl et al. 2006; Miegroet and Olsson 2011).
According to research of Khoshnevisan et al. (2018) and To evaluate the key processes of the life cycle for the produc-
IPCC guidelines (Tanabe and Wagner 2003), the rough esti- tion of the yarn in detail, the key processes of the aforemen-
mation showed that the average C sequestration rate was about tioned key impact categories of the two scenarios are
Int J Life Cycle Assess (2020) 25:2050–2062 2057

Table 2 The LCIA results of the


virgin cotton yarn production and Impact category Unit Virgin cotton Recycled cotton
recycled cotton yarn production.
Values are presented per FU Climate change kg CO2 eq 11000 4380
Terrestrial acidification kg SO2 eq 5.84 5.62
Freshwater eutrophication 10-3 kg P eq 2.8 19.8
Ozone depletion 10-8CFC-11 eq 2.47 4.35
Fossil depletion kg oil eq 1240 1100
Freshwater ecotoxicity kg 1,4-DB eq 0.29 0.45
Human toxicity kg 1,4-DB eq 68.8 69.2
Ionizing radiation kg U235 eq 25.2 75.7
Marine ecotoxicity kg 1,4-DB eq 0.127 0.247
Marine eutrophication kg N eq 2.06 2.04
Metal depletion kg Fe eq 139 44.2
Particulate matter formation kg PM10 eq 1.93 1.82
Photochemical oxidant formation kg NMVOC 5.55 5.42
Terrestrial ecotoxicity kg 1,4-DB eq 0.0358 2.29
Water depletion m3 3514 583
Land occupation ha 0.58 0

described in Fig. 3. For both scenarios, the electricity For the virgin cotton yarn scenario, the environmental im-
was most significant contributor to the impact on the pact is concentrated in the cotton cultivation and fibers spin-
main categories. The top three contributors to climate ning stages. The category of climate change is dominated by
change were fiber acquisition, electricity, and tap water. the land occupation. The other categories of environmental
The environmental impacts generated from the waste impacts in this stage are dominated by fertilizers and urea
discharge are smaller than other processes because consumption in the cotton cultivation stage. It should be men-
wastewater treatment system is established for reducing tioned that 79.1% of contribution to the category of water
water consumption. depletion is attributable to the cotton cultivation, which shows

Fig. 3 Compositions of the key


processes to main categories: A—
virgin cotton yarn scenario, B—
recycled cotton yarn scenario
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that the irrigation water, compound fertilizer, and pesticides explore the influences of parameter uncertainty distribution
are the dominant contributors to the category. on the aforementioned impact categories.
For the recycled cotton yarn scenario, 40.3% of contribu- According to the LCA results, electricity occupies absolute
tion to the category of water depletion is attributable to the share in the spinning stage on each category for both scenar-
recycled cotton fiber acquisition, which demonstrated that the ios. Fertilizer consumption (includes urea and compound fer-
washing process is the dominant contributor to water deple- tilizer) accounts for a critical proportion of water depletion and
tion. Meanwhile, environmental impacts generated from the climate change in the cotton acquisition stage. The consump-
washing of fabrics are mitigated effectively by the use of tion of water for washing is sensitive to the category of water
recycled water. depletion. The electricity, fertilizer, and water are considered
uncertain parameters due to the change of these parameters
3.3 Sensitivity analysis that have strong effects on environmental impacts of two
scenarios.
Sensitivity analysis is a way to predict the relationships be- Determining the distribution of parameters is crucial when
tween input and output variables in a system (Ye et al. 2017). very limited sample data of an uncertain parameter are pro-
Since the production data for yarns may be have uncertainties, vided; the triangular distribution is used (Liu et al. 2012).
sensitivity analysis was conducted to examine the effects of Therefore, considering the sample data are finite, it assumed
changed several production data. In this analysis, 5% of fer- that these parameters follow the triangular distribution, as
tilizer consumption is reduced in cotton cultivation stage for shown in Table 3.
the virgin cotton yarn scenario, 5% of water consumption is The results show the probability density distribution histo-
decreased in the washing process for the recycled cotton yarn grams of water depletion, human toxicity, fossil depletion, and
scenario, and 5% of total electricity consumption for both climate change for both scenarios with a 90% confidence in-
scenarios is decreased. Each parameter was changed indepen- terval (Fig. 5).
dently from all others so that the magnitude of its effect on the Thus, for water depletion, the range of virgin cotton yarns
base scenarios could be assessed. It should be noted that the is from 3489 to 3551 m3 and the range of recycled cotton
transportation distance is considered a constant in this re- yarns is from 554 to 606 m3. For human toxicity, the range
search, since the environmental impacts generated from the of virgin cotton yarns is from 63.7 to 70.5 kg 1,4-DB eq, and
transportation (less 1% of total environmental impacts) are the range of recycled cotton yarns is from 64.4 to 71.0 kg 1,4-
small and the contributions of cotton transportation to all im- DB eq. For fossil depletion, the range of virgin cotton yarns is
pact categories are not sensitive to transportation distance in from 1131 to 1252 kg oil eq and the range of recycled cotton
the whole life cycle (Zhang et al. 2015). yarns is from 1033 to 1149 kg oil eq. For climate change, the
Fig. 4 demonstrates the results of a 5% variation to prom- range of virgin cotton yarns is from 10643 to 11456 kg CO2 eq
inent processes on the aforementioned impact categories. and the range of recycled cotton yarns is from 4078 to 4544 kg
Obviously, the decreasing of electricity consumption mainly CO2 eq.
affects the contribution of the presented stages in the life cycle
of yarns on the aforementioned categories, especially on cli-
mate change and fossil depletion. It indicates that improving 4 Discussions
energy efficiency can significantly reduce environmental bur-
dens. Additionally, the decrease in electricity consumption In this paper, the LCA for recycled cotton yarns and virgin
has a significant influence on human toxicity because of the cotton yarns are established to investigate their environmental
combustion of fossil fuels, and water consumption in the impacts. It can provide quantitative value to support the pop-
washing process has little effect on human toxicity due to ularization of recycled cotton and help to reduce the overall
the use of recycled water. Furthermore, irrigation water and environmental impact in the apparel industry. Fig. 3 exhibits
fertilizer consumption in cotton cultivation stage have a great- that electricity consumption is the key process in the life cycle
er impact on water depletion. of both the two scenarios. The results show that environmental
impacts of recycled cotton yarns are far less than those of
3.4 Uncertainty analysis virgin cotton yarns, except for climate change and water de-
pletion. The reason is that the land occupation and irrigation
The varying life cycle boundaries, technology levels in differ- water have great impact on environmental impacts of cotton
ent countries and regions, lead to the different parameters and cultivation. It can be observed that recycled cotton yarn is a
calculation results (Jiao et al. 2019). The LCIA results are viable alternative to relieve resource and environmental
questionable and non-satisfactory for the interpretation phase pressure.
without uncertainty analysis in LCA (Bicer and Dincer 2018). Thus, it can be considered that the recycled fibers can be
Therefore, a Monte Carlo simulation method is used to effectively avoiding environmental impacts generated from
Int J Life Cycle Assess (2020) 25:2050–2062 2059

Fig. 4 Sensitivity analysis results

the cotton planting. Moreover, the pesticides and fertilizers are practices should be disseminated to textile plants (Hasanbeigi
required in cotton cultivation, which is far to be considered and Price 2012). A spinning quality control model based on
sustainable practice and has deleterious effects on environ- hierarchical multi-process is used to accurately control yarn
ment preservation. quality, improve the fracture strength, and reduce
From the perspective of manufacturers, compared with en- nonconforming ratio of yarns (Shao and Ma 2018). Some
vironmental impacts of virgin cotton yarns, the emitted CO2 measures are adopted for reducing fibers waste percentage,
eq of the recycled cotton yarns can be decreased by 60.18%. such as reasonably setting the top card rack density and inser-
The consumed Oil eq of the life cycle of the recycled cotton tion depth and eliminating embedded fiber in top comb and
yarns can be decreased by 11.3%. The consumed water of the cylinder (Xiao et al. 2016).
recycled cotton yarns can be saved by 79.1%. There was a The government should also strengthen environmental pro-
slight increase (0.58%) for human toxicity (shown in Fig. 6). It tection education and raise the awareness of environmental
reveals that the recycled cotton fibers should be served as a protection as future works which to enable enterprises to re-
substitute for virgin cotton fibers. ceive recycled fibers. Most of the old clothes have not been
According to the annual production of reference factory in reprocessed or harmlessly treated yet. It is reported that about
2019, recycled cotton fibers account for 3% of annual fibers 2.6 × 1010 kg of old clothes is discarded every year. The reuse
and the proportion will be further increased along with the rate of old clothes is less than 1%, and the remaining old
development of recycled process. There is no degradation in clothes are used for incineration and landfill (China
the recycled cotton products’ performance after adding association of circular economy. 2016). For this reason, the
recycled cotton fibers. enterprises should further develop related products about
In China, the cotton cultivation area was 3.2 million ha and recycled cotton fibers so that it will bring huge potential eco-
the per hectare average output of cotton is 1698.6 kg in 2017. nomic benefits.
However, the per hectare output of cotton is 2079.3 kg in However, the recovery mode and fiber types have strong
Xinjiang province since its unique geographical location and effect on the cost of recycled cotton yarns. Considering the
climate (National Bureau of Statistics. 2017). It means that the scattered distribution of recycled cotton fabrics, the diversity
utilization of 1000 kg recycled cotton yarns can save about of cotton fabrics, and the complexity of fibers separation, the
0.5 ha of agricultural land and reduce 6600 kg CO2 eq. Thus, cost of recycled cotton yarns may be higher than that of virgin
agricultural land can be saved by using recycled cotton fibers. cotton yarns, and an important trend in future work is how to
Some feasible improvement opportunities for reducing en- reduce the costs of recycling cotton yarns.
vironmental impacts of the recycled fibers are put forward. The morphology and physical properties of cotton fibers
The energy-saving measures should be adopted for improving are crucial to evaluate the mechanical properties of yarns
the environmental performance in the production, such as the (Memon et al. 2015). Compared with the dyed fibers, the
relevant know-how about energy efficiency technologies and dyestuffs and auxiliaries are not necessary to achieve good

Table 3 Uncertain parameters of


distributions Input parameters Type Distribution parameters Mean value Standard deviation Unit

Fertilizer Triangular 483.4, 605.0, 665.3 584.5 38.1 kg/t


Electricity-virgin Triangular 3543.4, 3991.0, 4223.1 3919.8 141.9 kWh/t
Washing water Triangular 20.0, 22.2, 24.4 22.2 0.9 m3/t
Electricity-recycled Triangular 3756.8, 4148.0, 4427.7 4111.3 138.2 kWh/t
Land occupation Triangular 5626,5800 5974 5800 56 m2/t
2060 Int J Life Cycle Assess (2020) 25:2050–2062

Fig. 5 Probability density of water depletion, human toxicity, fossil depletion, and climate change

colorfastness of the virgin cotton fibers and recycled cotton There are still some limitations in this study and listed as
fibers. Moreover, the mechanical properties of recycled cotton follows:
yarns are weaker than virgin cotton yarns because of the sec-
ond use of the recycled cotton fibers. Generally, the recycled & The cotton cultivation stage is simplified since it is com-
cotton fibers are fully mixed with other type fibers spun to plex and long-time.
yarns in a certain proportion and woven into fabrics. The & One factory production data is collected from the annual
virgin cotton fibers are always mixed with other type fibers production data of melange yarn manufacturer in Zhejiang
spun into yarns when the color scheme of yarns is taken into province in China, and the uncertainties caused by geo-
consideration. graphical differences are existing and need to be further
Since the downstream data of recycled cotton fibers are investigated.
difficult to collect, we tried our best to collect extensive data & There are many recycling methods for the recycled cotton
to quantify the cradle-to-gate life cycle impacts of yarns. fibers which have different environmental impacts.
Int J Life Cycle Assess (2020) 25:2050–2062 2061

Fig. 6 Dominant impact category


of virgin yarns and recycled yarns
(the unit is given in Table 2)

& The differences in production technologies between China Furthermore, the pesticides and fertilizer are required in the
and Europe may bring uncertainties such as fertilizers and cotton cultivation, which is far to be considered sustainable
pesticides based on European situations. practice and has deleterious effects on environment preserva-
& The noise generated in the production plants is ignored tion. Recycled cotton fibers can serve as a substitute for virgin
and this deserves to be further studied. cotton fibers to avoid environmental impacts generated from
the cotton planting and reduce agricultural land occupation.
More methods on recycling cotton fibers should be further
developed to achieve the reuse of waste resources.
5 Conclusions
Funding information This research was financially supported by the
National Natural Science Foundation of China (Grant no. 51722502).
In this work, a cradle-to-gate LCA of virgin cotton yarns and
recycled cotton yarns has performed using on-site investiga-
Compliance with ethical standards
tion data. The LCIA results reveal that environmental impacts
of recycled cotton yarns are far less than those of virgin cotton All the listed authors have confirmed the final version of the manuscript
yarns. Notable impacts on climate change, fossil depletion, and approved it for submission.
water depletion, and human toxicity have been observed. In
cotton cultivation, the land occupation and irrigation water
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