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Construction and Building Materials 119 (2016) 370–384

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Construction and Building Materials


journal homepage: www.elsevier.com/locate/conbuildmat

Environmental life cycle assessment of lightweight concrete to support


recycled materials selection for sustainable design
Loredana Napolano a,b,⇑, Costantino Menna b, Sossio Fabio Graziano c, Domenico Asprone b,
Marco D’Amore c, Roberto de Gennaro d, Michele Dondi e
a
STRESS scarl, Sviluppo di Tecnologie e Ricerca per l’Edilizia sismicamente Sicura ed EcoSostenibile, Vico II San Nicola alla Dogana 9, 80133 Naples, Italy
b
Department of Structures for Engineering and Architecture, University of Naples Federico II, Via Claudio 21, 80125 Naples, Italy
c
Department of Earth Science, Environment and Resources, University of Naples Federico II, Via Mezzocannone 8, 80134 Naples, Italy
d
CISAG, University of Naples Federico II, Via Mezzocannone 8, 80134 Naples, Italy
e
ISTEC-CNR, Via Granarolo, 64, 48018 Faenza, Italy

h i g h l i g h t s

 A LCA is performed for artificial lightweight aggregates produced from waste sources.
 The environmental impacts of different types of lightweight concrete are investigated.
 Artificial aggregates produced from natural raw materials determine the highest environmental impact in concrete material.
 Lightweight aggregates produced from industrial waste raw materials provide environmental benefits due to the avoided impacts.

a r t i c l e i n f o a b s t r a c t

Article history: The constant increase in consumption of aggregates for concrete production represents a major environ-
Received 18 January 2016 mental issue in the construction industry. Recycled wastes might be used as raw materials in the
Received in revised form 2 May 2016 manufacturing of artificial LightWeight Aggregates (LWAs) in substitution and/or in combination with
Accepted 3 May 2016
aggregates produced using natural sources for several end-uses, thus saving non-renewable resources.
Available online 27 May 2016
In this study, a Life Cycle Assessment (LCA) is performed for different LWAs manufactured with raw
materials supplied by nature or waste. Then, the LCA is conducted on different concretes made of the
Keywords:
different LWAs.
Lightweight concrete
Lightweight aggregates
Ó 2016 Elsevier Ltd. All rights reserved.
Expanded clay
Sustainability

1. Introduction environmental issues related to the depletion of natural resources


and, consequently, to the availability of aggregates.
Concrete is the most consumed material in the construction In the last decades, waste reuse/recycling has been considered
sector and the second most consumed substance on Earth after as a valuable option to substitute the conventional aggregates in
water. The estimated worldwide concrete consumption was 32 mil- concrete production as well as to reduce waste generation. Con-
lion m3 in 2013 [1]. Consequently, the consumption of aggregates, struction and Demolition waste (C&D) recycling, for example, has
which represent the major component in concrete mixes, is con- the potential to reduce the amount of waste disposed in landfills
stantly and rapidly increasing with the rise in concrete production and to preserve natural resources by avoiding new raw material
and utilization. For example, it was estimated that 150 million tons production; this practice has been successfully used in ordinary
of aggregates were produced in 2013 in the countries of European concrete production [2–7].
Union [1]. Inevitably, these considerations give rise to common The environmental comparison between normal/conventional
and recycled concrete (produced using waste as raw materials)
has been performed in several studies [8–16] and the results
⇑ Corresponding author at: STRESS scarl, Sviluppo di Tecnologie e Ricerca per showed clear environmental benefits for all recycled concrete
l’Edilizia sismicamente Sicura ed EcoSostenibile, Vico II San Nicola alla Dogana 9, options, mainly due to the avoided impacts associated with the
80133 Naples, Italy. avoided disposal of waste. For instance, some studies have clearly
E-mail address: loredana.napolano@unina.it (L. Napolano).

http://dx.doi.org/10.1016/j.conbuildmat.2016.05.042
0950-0618/Ó 2016 Elsevier Ltd. All rights reserved.
L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384 371

showed the environmental benefits related to the uses of glasses 2. Materials


and plastic waste as raw materials for aggregates production in
Four artificial LightWeight Aggregates (LWAs) (Type A, Type B, Type C and Type
ordinary concrete [17–21].
NA) are investigated from an environmental point of view. The main difference
It has been also reported that cement is the largest contributor among these LWAs is the raw material used for their production; indeed, three
to the overall life cycle environmental burden of all concrete types LWA types (Type A, B and C) are produced using industrial waste as raw materials
(conventional and recycled ones). This evidence has forced the (LWAs_R indicates recycled sources for raw materials), and one LWA type (Type NA)
using clay as raw material (LWA_N indicates a natural source for raw material).
research community to develop proper environmental friendly
Additional details of all artificial aggregate types are provided in the following
solutions and new low-CO2 binders capable of reducing the envi- sub-sections.
ronmental impacts associated with the cement industry [22–25].
Besides cement component, aggregates are typically the second
largest contributors in normal concrete production [11,14,15] 2.1. LWA_R
while transport phase influences the overall environmental profile
Raw materials (recycled wastes) used to produce LWA_R and afterwards used in
of concretes depending on the transport distances and transport RLAC mixes are the following:
vehicle type [10].
As far as LightWeight Aggregates (LWAs) are concerned, they 1) Mud deriving from the processing (cutting and sawing) of commercial ‘‘ze-
are usually produced starting from minerals, including natural rock olitite” (rocks with zeolite content higher than 50 wt.%), coming from a
quarry site located near Comiziano, Naples-Italy (Campanian Ignimbrite,
materials such as shale, clay, or slate. These raw materials are ther- hereafter referred to as Cab70);
mally expanded to about twice the original volume to get final 2) Mud deriving from the processing (cutting and sawing) of Serizzo (a gran-
aggregate density. The resulting material has properties similar itoid orthogneiss, hereafter referred to as SER), from the Verbania-Cusio-
to natural (bulk) aggregates, but is less dense and consequently Ossola district (Verbania, Italy);
3) Mud resulting from polishing porcelain tiles (Dry Powder Mud, hereafter
yields a lighter concrete product. Indeed, the main difference
referred to as DPM), from the Sassuolo industrial district (Modena, Italy).
between ordinary and lightweight concrete is the bulk density. In
the former, this value usually ranges between 2200 and 2600 kg/ Further information about chemical, mineralogical and technological character-
m3, while in the latter it ranges between 300 and 2000 kg/m3 ization of each industrial waste can be found in [31–33].
[26]. This difference results in the reduction of dead weights on The production process adopted to obtain LWA_R from the above described
structure, and also provides a better thermal and acoustic insula- waste materials is composed of three main steps [31–33]:
1- Mixing of secondary materials: The raw materials require to be properly mixed
tion. Several research activities have investigated the possibility
(in terms of % w/w) in order to achieve the final physical and mechanical properties
of replacing LWAs manufactured with natural raw materials with of the LWA_R. Moreover, the use of DPM and/or Cab70 waste material is needed in
recycled ones for the production of lightweight concretes. How- each LWA_R mix to guarantee a proper expansion process during thermal treat-
ever, the authors of most of these studies focus intensely on the ment. The resulting mixes of raw materials (% w/w) which are used to produce
LWA_R in the RLAC (reported in the subsequent sections) are reported in Table 1
chemical, physical, and mechanical properties/performances of
[31–33] and are named as ‘‘Type” as follows:
new Recycled Lightweight Aggregate Concretes (RLACs) whereas
their environmental performance is usually not considered, even - Type A indicates LWA_R composed of 100% of Cab70 secondary material;
though they investigate the possibility of using waste products - Type B indicates LWA_R composed of 70% and 30% of Cab70 and DPM secondary
deriving from industrial processes [27–33]. Several experimental materials, respectively;
- Type C indicates LWA_R composed of 50% of SER and 50% of DPM secondary
studies [31–33] have also showed opportunities for the reuse of materials.
industrial wastes, such as muds coming from both ornamental
stone (granite sludge from sawing and polishing operations) and 2- Compaction and granulation: Compaction and granulation of secondary
materials and their mix (Table 1) are obtained by means of dry granulation
ceramic production (porcelain stoneware tile polishing sludge); using a compactor apparatus and a briquettes breaker mill according to the fol-
starting from these wastes, the manufacturing of LWAs was lowing procedure. The powder material is moistened by adding 3% water by
demonstrated to be suitable for constituents of structural and/or weight and poured into a feed screw hopper, where it is continuously conveyed
thermo-insulating lightweight concretes. to the compactor which generates the briquettes (Fig. 1a). These are further
granulated and divided in order to obtain a grain size fraction ranging between
On the basis of the results reported in [31–33], the present
3 and 8 mm.
study aims to investigate the environmental footprint of different 3- Thermal treatment: dynamic firing (rotative kiln). The materials coming from
lightweight concretes made of different LWAs by means of a Life the compaction and granulation phase are thermally treated in dynamic condi-
Cycle Assessment (LCA) methodology [34,35]. In detail, the present tions by a rotative kiln at the temperatures and for a duration reported in
paper is organized as follows: Table 1. During this thermal treatment, the compacted DPM raw material
expands thanks to the presence of small amounts (about 3% in weight) of an
abrasive substance, i.e. Silicon Carbide (SiC) contained in the mud coming from
1) The environmental performance of LightWeight Aggregates ceramic tile production; SiC is released at high temperatures from compacted
(LWAs) produced from natural and industrial waste raw material, producing CO2 gas [31–33]. On the contrary, in the case of Cab70,
materials is first calculated and compared. The LWAs manu- the expansion of the compacted material is driven by the gas (H2O steam) which
is incorporated in the material itself. In Fig. 1b, the recycled LWAs are shown
factured with industrial waste raw materials are obtained
after the production steps.
starting from the following waste: Campanian Ignimbrite
(Cab70), Dry Powder Mud (DPM), and granitoid orthogneiss
SERizzo (SER); instead, the LWAs produced by natural raw 2.2. LWA_N
materials are made of (expanded) clay.
Raw material used to produce artificial LWA_N is natural clay (Table 1).
2) Then, the environmental footprint of the Natural Light-
The production process used to obtain LWA_N is composed of three steps [36]:
weight Aggregate Concrete (NLAC) and Recycled Lightweight Mixing process, Thermal treatment and Expansion process. The mined clay is mixed
Aggregate Concrete (RLAC) made with the above mentioned with water, ground and sometimes granulated (mixing process) and then burned
lightweight inert options are assessed and the results are at reverse flow in a rotary furnace at 1200 °C (Thermal treatment). The material
compared. The proposed lightweight concrete mixes have burns and expands with the help of heavy fuel oil (Expansion process). The pellets
are rounded in shape and fall from the kiln in a grade of approximately 0–32 mm
been selected from previous works of the authors [31–33] with an average dry bulk density of approximately 600 kg/m3. The crushing
considering the hypothesis that those mixes should have resistance value is approximately 1.3 MPa (Table 1) [36] according to [37].
the same physical and mechanical performances (for LCA Table 1 reports the composition and the principal properties of LWA_N (named
comparative purposes). as Type NA).
372 L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384

Table 1
Mix composition (% w/w of LWAs) and main properties of LWAs: LWAs_R and LWAs_N [31–33].

Cab70 SER DPM Clay Production conditions Physical and mechanical properties
(% w/w) (% w/w) (% w/w) (% w/w)
Temperature Soaking time at Bulk density H2O absorption after Crushing
(°C) Tmax (min) (g/cm3) 24 h (%) resistance (MPa)
LWA_R Type A 100 1380 5–6 1.01 5.7 0.6
Type B 70 30 1300 5–6 0.81 1.4 2.94
Type C 50 50 1300 5–6 0.68 2.3 1.2
LWA_N Type NA 100 1200 5–6 0.60 2 1.3

Fig. 1. (a) Briquettes and granulate after compaction and granulation; (b) LWAs_R.

Table 2
Lightweight concrete mix designs (NLAC and RLAC) (quantities are referred to 1 m3 of lightweight concrete) [32,39].

Components MIX NA MIX A MIX B MIX C


Mix design LWAs (kg) Expanded clay
(Type NA) 515
Cab70
(Type A) 404
Cab70 + DPM
(Type B) 259
SER + DPM
(Type C) 306
Portland cement Z 42.5 (kg) 330 400 400 350
Water (kg) 181 224 224 175
Silica sand (kg) 675 760 760 500
Superplasticizer (kg) 0.086
Incorporated air (l) 22

2.3. Recycled and natural lightweight concrete (RLAC and NLAC) strength class (i.e. C20/25) [38] and have the same final density (i.e. 1600 kg/m3)
at 28 days. These two hypotheses reflect typical users’ design choices when light-
All types of LWAs (Table 1), described in Sections 2.1 and 2.2, are used as arti- weight concretes are employed in construction operations, i.e. compressive
ficial aggregates for the production of lightweight concretes. The corresponding strength and material density. The details of the concrete mix design of each option
concrete mix designs (Table 2) have been derived from previous works of the investigated are summarized in Table 2 and are related to 1 m3 of lightweight con-
authors [32] and from commercial product datasheets [36]. Moreover, all light- crete material. The different lightweight concrete options are hereafter denoted as
weight concretes chosen for the LCA analysis belong to the same compressive ‘‘MIX” followed by the letter of the LWA type used to produce them. For instance,
L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384 373

MIX A in Table 2 refers to the lightweight concrete obtained with Type A LWAs_R. respectively, 1 m3 of LWAs is chosen as reference flow (to con-
Concrete mix-design includes sometimes incorporated air (approximately 20 l/m3
sider volumetric amounts in concrete mix design). Hence,
for MIX C, Table 2) and chemical additive, i.e. superplasticizer (for MIX NA, Table 2)
(polycarboxylate ether), in order to reduce damage during freezing and to improve
according to the bulk density values reported in
the workability, respectively [32,39]. Table 1 and 1010 kg of Type A, 810 kg of Type B, 680 kg of Type
C are compared with 600 kg of Type NA.
3. Methods
3.2. System boundary
The environmental performances of the different LWAs (LWA_R
and LWA_N) described in the previous section and the correspond- Fig. 2 shows the NLAC and RLAC production system boundary.
ing lightweight concrete mixes (RLAC and NLAC) are evaluated by Both systems include raw materials production (cement, aggre-
means of a LCA approach [34,35]. Following, the conceptual steps gates production and water supply) and generate 1 m3 of light-
of the LCA are schematically reported, including: (1) Goal and weight concrete as a final output product. The other lifecycle
Scope, (2) Life Cycle Inventory (LCI), (3) Life Cycle Impact Assess- phases, such us construction/installation, use and end of life, of
ment (LCIA) and (4) Interpretation: both NLAC and RLAC, are excluded from the analysis because they
represent phases common to all the alternatives and contribute
3.1. Goal and Scope with the same environmental impacts.
The NLAC system boundary includes the LWA_N production
The primary goal of the present study is to define and compare reported in Fig. 2-(i). The schematic production process related to
the environmental impacts associated with the production of differ- this inert type is reported in Fig. 3 and represents the current pro-
ent types of lightweight concretes: i) Natural Lightweight Aggregate duction practice of expanded clay aggregates in Italy.
Concrete (NLAC) made with LWA_N aggregates (natural clay raw The RLAC system boundary includes the LWA_R production
material) and ii) Recycled Lightweight Aggregate Concrete (RLAC) (Fig. 2-(ii)). The different types of LWA_R are produced starting
made with three different LWAs_R (industrial waste raw materials). from different industrial waste secondary materials, according to
Moreover, in order to highlight the potential environmental benefits the weight ratios reported in Table 1. In particular, Fig. 4 shows
and critical production phases related to the aggregates, the LCA is the system boundary and the production process of LWA_R. The
also performed on the LWAs only. For this reason, we report the main differences between LWA_N and LWA_R, as described in
declared unit which is chosen in these two cases as following: the Materials section and illustrated in the Fig. 4, are the raw mate-
rials used and the manufacturing process adopted for the produc-
 Lightweight concrete: the lightweight concrete mixes (Table 2) tion of LWAs.
have been selected from previous works of the authors [31–
33], considering the hypothesis that those mixes have the same 3.3. Allocation
physical and mechanical performances (for LCA comparative
purposes). In particular, C20/25 compressive strength class According to the European Union directive [40], a waste may be
[38] and a final density of 1600 kg/m3 are chosen as reference regarded as a by-product if several requirements are met, such as
mechanical and physical properties, respectively, for the defini- its use in other industrial processes. In this study, the different
tion of the related reference flow, i.e. 1 m3 of lightweight waste flows, used as raw materials for the production of LWA_R,
concrete. are considered as dependent co-products. In order to effectively
 LWAs: for the assessment of the environmental footprint of the quantify the environmental impacts of the investigated co-
different LWAs, produced starting from both industrial waste products and corresponding RLAC mixes, the allocation procedure
and natural raw materials described in Sections 2.1 and 2.2, is taken into account by means of a System Expansion (SE)

Cement production Cement


(i) 1 m3 NLAC

Additive production Additives


Transport

Water supply Tap water (ii) 1 m3 RLAC


CONCRETE
PRODUCTION
i)LWAs_N
(exploded system in fig. 3)
Aggregate production ii) LWAs_R Production
Landfill
(exploded system in fig. 4) waste

Energy

Fig. 2. System boundary, NLAC and RLAC production (1 m3, C20/25 compressive strength class, final density of 1600 kg/m3).
374 L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384

Heavy fuel oil

Natural Raw
material
Clay

Expansion
Transport

Heating
LWAs_N

Mixing
Water

Electricity/
Diesel Production process

Fig. 3. System boundary of LWA_N production process (1 m3).

Finishing porcelain
stoneware les
Product A2

Recycling
Raw porcelain

Process A2
stoneware

Polishing

waste materials

DPM

Compacon and
Raw materials for LWAs

granulaon
Transport
Waste materials

Heang
Mixing
LWAs_R
Process A1
Mining of

Cab70, SER
stones

Sawing

waste materials

Producon process
Process I
Polishing
Grinding

Final natural stone


product
Product A1

Fig. 4. System boundary of LWAs_R production process (1 m3).

approach according to [34–35,41–42]. This approach enables to environmental benefits related to their secondary use. Moreover,
expand the product system and include the additional functions/ it should be pointed out that, for the cases investigated, a pure
uses associated with the by-products [41–42]. Several studies have physical allocation method (e.g. mass allocation) was not applied,
dealt with the evaluation of the environmental impact of the waste since the ratio between product and by-product cannot be varied
sources used as raw materials in the production of aggregates for without changing the inputs and outputs volumes [41]; in addi-
normal concrete; these studies usually implement mass and/or tion, although the economic allocation might be applied, this rule
economic allocation approaches [43–48]. According to the mass was not selected as proper allocation method since the economic
and economic allocation approaches, the inputs and the outputs value of secondary materials herein investigated couldn’t be accu-
of a system (i.e. a production process of a product including by- rately attributed.
products) should be allocated between the products/by-products The resulting SE allows the quantification of the environmental
according to physical (e.g. mass) or economic (e.g. cost) relation- impacts of LWA_R when a by-product is used, taking into account
ships between them, respectively. the avoided raw material supply (e.g. clay extraction and trans-
Although the quantification of the environmental impacts of co- port) and production process of LWA_N, as showed in Fig. 5. In par-
products should be made using the SE approach, (i.e. avoiding the ticular, the allocation scenario herein adopted follows the
allocation of input and output between the products in favor of hypothesis that the LWAs are fully utilized (demand higher that
expanding the product system) little research has been conducted supply [41]) on the basis of the information of annual production
using this approach for the environmental impacts assessment of rate of both aggregates and wastes [51–53].
aggregates made of recycled raw materials [16,49–50]. Within this The expanded product system related to the RLAC production
context, the present study investigates the environmental footprint consists of (Fig. 5) the environmental burden of determining pro-
of LWAs_R, using the SE method considering all processes related duct (Products A1, A2, Fig. 4) for the co-producing processes (i.e.
to the production and treatment of the wastes as well as the waste materials). In detail [41]:
L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384 375

Determining Product: Determining Product:


Mining and sawing of stone Natural stone product Porcelain stoneware les
Product A1 Raw porcelain stoneware and polishing
Process A1 Process A2 Product A2

Dependent Co-Product (Waste materials): Dependent Co-Product (Waste materials):


Cab70 and SER DPM

Transport Transport

Intermien reatment of secondary materials Intermien reatment of secondary materials


Process I1 (compacon, granulaon) Process I1 (compacon, granulaon)

Intermien reatment Process I2 (Heang )


LWAs (Type A, Type B, Type C)

Avoided impact Process D: Process B:


Natural clay extracon and manufacturing process of Recycled Lightweight
LWA_N concrete Producon

Fig. 5. Expanded product system related to RLAC production.

 With regard to the use of Cab70 and SER waste materials, Pro- production site is taken into account for NLAC and RLAC mixes. It is
duct A1 (in the expanded system) is composed by: Process A1 - pointed out that, as hypothesis of the study (that reflects national
+ Process I Process D, where Process A1 includes the mining, current practice in lightweight concrete industry) either industrial
sawing and transportation of natural stones; waste materials and natural clay processing occur in the same
 With regard to the use of DPM waste material, Product A2 (in the plant where lightweight concrete is produced. It is also assumed
expanded system) is composed by: Process A2 + Process I Pro- that all other components of concrete mix-design (cement, fine
cess D, where Process A2 includes raw material extraction for aggregates, etc.), from extraction to production phases, are manu-
porcelain stoneware, transportation and polishing processes; factured in the same plant of the lightweight concrete material.
Three different transport scenarios are considered for the LWAs,
For all the investigated waste materials: corresponding to the relative location of the collecting site of the
waste materials, Cab70 and DPM. This choice is related to the fol-
 Process I (intermittent) includes compaction and granulation lowing consideration: as reported in Table 1, the Cab70 and DPM
(Process I1 Fig. 5), and heating treatment (Process I2 Fig. 5), are always used in the LWAs_R mixes along with other waste
including transportation; materials (e.g. SER). In the transport Scenario 1, it is assumed that
 Process D is the avoided raw materials supply (i.e. natural clay the lightweight concrete plant is located in Naples (Italy), corre-
extraction and transport- from clay extraction plant to aggre- sponding to the area where Cab70 waste material is collected. In
gate manufacturing plant) and the production process of the transport Scenario 2 it is assumed that the plant is located in
LWA_N (Section 2.2) [41]. Modena (Italy), corresponding to the collecting area of DPM waste
material, whereas in the Scenario 3 the transport phase is com-
Given these considerations, the LWAs_R imply 100% of the bur- pletely omitted from the LCA system boundary (for all analyzed
den of Process A, and Process I, including transportation, and cred- cases). Within the latter hypothesis, the location of the i) collecting
its from Process D (Fig. 5); while, RLAC receives 100% of the burden site of the waste materials, ii) the aggregate manufacturing plant
of process B and process D (Fig. 5), where Process B represents the and iii) lightweight concrete plant correspond to the same place
lightweight concrete production process [41]. for all the considered alternatives. Although it represents a not
Although avoiding allocation (in favor of expanding the product very realistic situation, Scenario 3 allows a better focusing on
system) can be regarded as the preferable option (all processes raw materials production and processing, trying to investigate
related to production treatment Process and credit of secondary the environmental impact of LWAs, RLAC and NLAC when the
materials - Process A, I and D, respectively – are included in the impact of the transport is not included. Table 3 shows the input
system boundary), a sensitivity analysis has been also performed data for the transport phase (one way) for all cases of LWAs.
including a different allocation rule, as discussed in the Section 5.
In particular, the LCA results calculated with SE of by-products
3.5. Inventory data, cut off rules and data quality requirements
are then compared with the results obtained by the application
of cut-off allocation criteria, i.e. by associating the environmental
Primary data concerning the amount of raw materials, energy
impact of LWAs only to the intermittent process I1,2 (Fig. 5) includ-
consumption, machineries, emissions, waste materials have been
ing transportation [54].
directly collected from Italian suppliers and manufacturers. Where
the data have been missing, the study has been completed on the
3.4. Transport scenarios basis of information obtained from databases available in the
SimaPro 7.3 LCA software package. These secondary data have
Only the transport of raw materials (industrial waste materials been retrieved from the Ecoinvent 2.2 database [55]. In this specific
and natural clay for LWAs production) to the lightweight concrete case, in order to guarantee data quality requirements, including
376 L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384

Table 3
Transport scenarios.

Waste materials Distance (one way) (km) Distance** Equipment Data Database
Scenario 1 DPM 626 Sassuolo-Naples Lorry Transport lorry 16 t, fleet average Ecoinvent 2.2
Cab70 40 Comiziano-Naples Lorry
SER 881 Verbania-Naples Lorry
Natural clay 775 Milano-Naples Lorry
Scenario 2 DPM 19 Sassuolo-Modena Lorry
Cab70 610 Comiziano-Modena Lorry
SER 284 Verbania-Modena Lorry
Natural clay 179 Milano-Modena Lorry
**
Distance from extraction/production to finishing plant.

time-related, geographical and technological representativeness, and the production process of LWAs_N (Process D) as reported in
LCI Ecoinvent data have been suitably modified on the basis of the expanded system boundary in Fig. 5.
the information and practices of local (Italian) ceramic tile, tuff
stones and aggregate suppliers and manufacturers. In case of insuf- 3.10. LCIA methodology
ficient data, materials or processes that contribute with less than
1% to the total mass or the energy flows or the energy use of pro- The IMPACT 2002+ [56] methodology is used for the impact
duct system have been omitted in the calculations; according to assessment phase. This method is composed of 14 midpoint indica-
[55] the excluded data include: embodied energy and emissions tors and four damage (endpoint) indicators: Human health (DALY),
associated with construction of R/NLAC plant equipment and Ecosystem quality (pdf*m2*yr), Climate change (kg CO2 eq), and
buildings, heating and cooling of such infrastructures, workers Resources (MJ Primary). In this study, only a damage oriented
transportation, accelerator admixtures for concrete, residual wash- method is employed to achieve environmental impact results,
ing water fresh R/NLAC production and environmental burdens because, while the midpoint method provides quantitative results,
caused by the work force. The following sections describe the main the former may offer results which are easily interpreted by the
assumption adopted in the inventory analysis: readers.

3.6. Cutting energy data for LWAs_R 4. Results and discussion

The process A1 (Fig. 5) includes the sawing of stones that As mentioned in the introduction section (Section 1), the first
requires a different amount of energy depending on the hardness part of the LCA analysis involves the comparison of the environ-
of the stone itself. The values of cutting energy are calculated on mental performance of LWAs_R and LWAs_N. Then, the NLAC
the basis of the hardness index of the starting materials used to and RLAC environmental performances are compared (Section 4.2).
produce the waste materials (Cab70 and SER) and are reported in
Table 4. 4.1. LWAs_R and LWAs_N

3.7. Heating treatment energy 4.1.1. Transport scenario 1


With regard to transport scenario 1 (Fig. 6a), the results of the
The same energy input data, referring to the Italian electricity LCA reveal that:
mix, retrieved from Ecoinvent database [55], is also used to model Two LWAs_R types (Type A and Type B) show negative environ-
the heating treatment (i.e. thermal treatment by means of dynamic mental impacts in all the damage categories. It clearly appears that
firing through a rotative kiln) for each LWA production process. the avoided processes (clay extraction, clay transport – 775 km,
Table 3 - and production process of LWAs_N), provide environmen-
3.8. Energy for LWA expansion tal benefits. Indeed, these avoided processes are able to maximize
the overall life cycle environmental performance of these types of
While LWA_N production includes clay extraction and mechan- lightweight aggregate in all the LCA categories. With regard to
ical mixing, thermal and expansion treatments, the LWAs_ R pro- these aggregates (Type A and Type B), the environmental credit
duction do not include this expansion phase, as explained in of the avoided processes (Process D) are higher than the impact
Section 2.1. Indeed, the expansion of LWAs_R is initiated by chem- related to the production process of the waste materials (Process
ical compounds contained in waste materials (SiC and H2O steam). A1 and A2) and the treatment of LWAs including transportation
On the contrary, the heavy fuel oil, at industrial furnace [50] is used (Process I1,2) (Table 5). In addition, by analyzing the environmental
to model the expansion process in the case of LWAs_N. benefits of Process D (Section 4.2), it clearly appears that the
avoided transport of natural clay (avoided 775 km) along with
3.9. Avoided impact the avoided manufacturing phase of Type NA, provide greater envi-
ronmental benefit than those coming from the avoided raw mate-
Avoided environmental impacts for the modeling of LWAs_R rial extraction (Table 5).
concern the raw material extraction, (i.e. natural clay), the trans- In detail:
port from clay extraction plant to aggregate manufacturing plant
- Type A LWAs, made of 100% of Cab70 waste material (Table 1),
presents the lowest environmental impact in all the categories.
Table 4
Indeed, it shows the highest negative environmental
Cutting energy values.
impact ranging between 27% and 77% in all the LCA cate-
Waste materials Cutting energy values (kWh/kg) gories; these results are mainly due to the avoided processes
Cab70 0.196 (Process D) and the shorter transport distance of Cab70, as
SER 0.99 showed in Table 3.
L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384 377

100%
80%
60%
40%

(a) Scenario 1
20%
0%
-20%
-40%
-60%
-80%
-100%
Human health Ecosystem quality Climate change Resources

100%

90%

80%

70%
(b) Scenario 2

60%

50%

40%

30%

20%

10%

0%
Human health Ecosystem quality Climate change Resources

90%

70%
(c) Scenario 3

50%

30%

10%

-10%
Human health Ecosystem quality Climate change Resources

Type A_SE Type B_SE Type C_SE Type NA

Fig. 6. LCA results of LWAs_R and LWAs_N; (a) Transport Scenario 1; (b) Transport Scenario 2; (c) Transport Scenario 3 (reference flow 1 m3).

- Also Type B LWAs, made of 70% of Cab70 and 30% of DPM waste - Type C LWAs exhibits an environmental performance of 48%
materials (Table 1), presents a negative environmental impact, lower than Type NA in all the environmental categories but this
lower than Type A, ranging between 3% and46% in all the aggregate type (differently from the other LWAs_R) does not
LCA categories; as discussed for the Type A, these results are present negative environmental burden. The environmental
mainly due to environmental benefits linked to the avoided performance of Type C LWAs is influenced by the production
processes (Process D). process of SER and DPM waste materials (Process A1,2, Fig. 5).
378 L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384

Table 5
Type A (1 m3), Impacts related to production process – Transport Scenario 1.

Type A aggregate – Scenario 1


Category Unit Cab70 Waste material Production process Avoided processes Total
(Process A1) (Process I(1,2)) (Process D)
Clay extraction Transport Production process LWA_N
Human health DALY 1.70E 04 1.79E 05 3.25E 06 1.36E 04 1.37E 04 8.92E 05
Ecosystem quality PDF*m2*yr 2.06E+01 3.35E+00 2.17E 01 4.35E+01 1.14E+01 3.12E+01
Climate change kg CO2 eq 1.57E+02 3.15E+01 1.62E+00 1.22E+02 1.82E+02 1.16E+02
Resources MJ primary 2.31E+03 4.59E+02 2.44E+01 1.78E+03 2.72E+03 1.76E+03

The major contributors to its impact are the cutting energy in 4.2. Avoided impacts and I1,2 intermittent process of LWAs_R
the SER production (Table 4) and the amount of DPM waste
material used in this aggregate type (Table 1). Clay extraction and transport operations along with the manu-
facturing phase (clay burning and expansion with heavy fuel oil)
are major contributors to the environmental impact of Type NA
4.1.2. Transport scenario 2
LWAs, which represent the avoided impacts (Process D, Fig. 5)
In transport scenario 2 (Fig. 6b) the environmental impacts of
for the LWAs_R. The related benefits are especially exploited in
almost all LWAs_R (Type A and Type B) are influenced by the trans-
the scenario 1 (Fig. 6a) along with the ‘‘avoided” transport distance
port of Cab70 waste material due to the increased distance from
of natural clay which is larger than the distance in the other sce-
the collecting site. This circumstance causes a global increase of
narios investigated (Table 3).
the impacts with respect to scenario 1. In addition, considering
In order to estimate the avoided impact for the LWAs_R system
the avoided processes, the main difference between scenario 1
boundary, as a representative example, the environmental profile
and scenario 2 is the transport (in terms of distance) of natural
of the Type A LWAs, for Scenario 1, 2 and 3, is reported in Tables
clay; in the former, the transport distance of natural clay is
5–7, respectively, in terms of quantitative environmental data
775 km while in the latter is 179 km (Table 3). Given these consid-
and considering all the lifecycle manufacturing Processes (Process
erations, it can be observed that the transport scenario 2 reduces
A1, Process I1,2 and avoided Process D, Fig. 6).
the environmental benefits linked to the use of waste materials
The avoided processes related to Type A include the avoided
compared to the results of transport scenario 1. The impact of Type
impact of clay extraction, its transport and the production process
C LWAs rises by 5–20% in the scenario 2 with respect to scenario 1
of LWAs_N (process D, Fig. 5). The quantitative environmental data,
while Type A and Type B LWAs no longer present negative environ-
reported in Tables 5–7, demonstrate that the avoided processes
mental impacts.
provide several environmental benefits. In particular, the major
In detail:
benefits come from the avoided production process of LWAs_N, fol-
lowed by the avoided natural clay transport and extraction.
- Type A, in the Ecosystem Quality category, presents an environ-
Process I, which includes the transport of Cab70 from waste
mental loads higher than all LWAs (LWAs_R and LWAs_N),
materials production plant (i.e. Comiziano) to the aggregate man-
mainly due to a larger transport distance of waste material
ufacturing plant, has a minor impact when transport is excluded
(Cab70, Table 3).
from the analysis (Scenario 3, Table 7) whereas it has major impact
- The environmental impact of Type C in the Human Health, Cli-
when the distance of the aggregate manufacturing plant is the lar-
mate Change and Resources categories is highest than all
gest considered (Scenario 1, Table 5).
LWAs_R (but lowest than Type NA), due to the energy con-
Table 8 reports the quantitative environmental data concerning
sumption related to the production process of waste materials
the manufacturing processes of all LWAs (process I). The manufac-
(SER and DPM); in the Ecosystem Quality damage category,
turing process of LWAs_N (Type NA), as expected, is approximately
instead, its impact is lower than all LWAs_R alternatives due
one order of magnitude larger than the corresponding values of
to a shorter transport distance of waste materials (Table 3).
LWAs_R (e.g. 3.67E + 02 MJ Primary in the Type A and 2.74E
+ 03 MJ Primary in the Type NA, for the Resources damage category).
4.1.3. Transport scenario 3 As already mentioned, this aspect is due to heavy fuel oil used for
In this scenario, the transport of raw materials (industrial waste expansion process of LWAs_N that determines an environmental
and natural clay) and the avoided transport of natural clay are not impact 90% larger than the impact of LWAS_R production process.
included in the Process I and Process D, respectively. All LWAs_R
show an environmental impact lower than the impact of Type 4.3. Recycled and natural lightweight concrete
NA in all damage categories (Fig. 6c). Also in this scenario, Type C
is responsible for the major impact among LWAs_R in almost all This section deals with the environmental burdens computed
damage categories, due to the production process of the waste for 1 m3 of NLAC and RLAC produced starting from the mix designs
materials (SER and DPM). Instead, the environmental profile of reported in Table 2. As it can be observed in Fig. 7, the NLAC (MIX
other LWAs_R is very low (Human Health and Climate Change cat- NA) exhibits the largest environmental impact in all the damage
egories for Type A and Type B) and also negative in the case of Type categories and for each transport scenario herein considered. In
A in Resources category. As already mentioned, it is mainly due to addition, MIX C in the transport scenario 1, MIX A and MIX C in
the environmental benefits related to the Process D which are the transport scenario 2 and 3, present an environmental burden
higher than the impacts of the Process A1,2 and Process I1,2. As greater than MIX B. In detail:
reported in Fig. 6c, the negative environmental profile of the
LWAs_R are substantially limited in the case of scenario 3, since, - Transport scenario 1. The environmental profile of MIX C is
as above mentioned, in the process D the (avoided) transport of mainly related to the production process and transport of waste
natural clay is excluded, resulting in a lower negative environmen- materials used to produce Type C aggregates (SER and DPM), as
tal ‘‘values” for all LWAs_R. seen also in Section 4.1 in the LWAs comparison.
L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384 379

Table 6
Type A (1 m3), Impacts related to production process – Transport Scenario 2.

Type A aggregate – Scenario 2


Category Unit Cab70 Waste material Production process Avoided processes Total
(Process A1) (Process I(1,2)) (Process D)
Clay extraction Transport Production process LWA_N
Human health DALY 1.70E 04 1.18E 04 3.25E 06 3.15E 05 1.37E 04 1.16E 04
Ecosystem quality PDF*m2*yr 2.06E+01 3.53E+01 2.17E 01 1.00E+01 1.14E+01 3.42E+01
Climate change kg CO2 eq 1.57E+02 1.21E+02 1.62E+00 2.82E+01 1.82E+02 6.70E+01
Resources MJ primary 2.31E+03 1.77E+03 2.44E+01 4.12E+02 2.72E+03 9.23E+02

Table 7
Type A (1 m3), Impacts related to production process – Transport Scenario 3.

Type A aggregate – Scenario 3


Category Unit Cab70 Waste material Production process Avoided processes Total
(Process A1) (Process I(1,2)) (Process D)
Clay extraction Transport Production process LWA_N
Human health DALY 1.70E 04 1.09E–05 3.25E 06 0.00E+00 1.37E 04 4.01E 05
Ecosystem quality PDF*m2*yr 2.06E+01 1.10E+00 2.17E 01 0.00E+00 1.14E+01 1.00E+01
Climate change kg CO2 eq 1.57E+02 2.52E+01 1.62E+00 0.00E+00 1.82E+02 8.12E 01
Resources MJ primary 2.31E+03 3.67E+02 2.44E+01 0.00E+00 2.72E+03 6.88E+01

Table 8 is approximately 57% of total environmental burden, even higher


Production process of 1 m3 of LWAs_N and LWAs_R. than that of LWAs. Due to the reduced impact of LWAs_R, cement
Damage category Unit Type A Type B Type C Type NA material primary affects the environmental results of MIX B in all
Human health DALY 1.09E 05 8.30E 06 6.46E 06 1.38E 04 LCA categories, accounting for the 70–90% of the total burden.
Ecosystem quality PDF*m2*yr 1.10E+00 8.40E 01 6.54E 01 1.15E+01 The environmental outcomes of aggregates and cement material
Climate change kg CO2 eq 2.52E+01 1.92E+01 1.49E+01 1.83E+02 for both investigated concrete types are also reported in Table 9
Resources MJ primary 3.67E+02 2.80E+02 2.18E+02 2.74E+03 in terms of absolute quantitative amounts for each damage cate-
gory. In particular, the environmental contribution of LWAs_R
(Type B) used to produce 1 m3 of RLAC is reduced by approximately
- Transport scenario 2. The impact of MIX A is influenced by the one half compared to the Type NA LWAs_N in all damage cate-
amount of aggregates used in the mix design (Table 2). This cir- gories. For example, the total energy required to produce 1 m3 of
cumstance mainly affects the Ecosystem Quality category lightweight concrete equals 3900 and 1970 MJ in case of MIX NA
where the impact of MIX A is higher than MIX NA. and MIX B LW concretes, respectively (Table 9), in agreement also
- Transport scenario 2 and scenario 3. The impact of MIX A and with the considerations on avoided energy reported in the previous
MIXC is influenced by the larger amount of LWAs used in these section. It should be also pointed out that, although the cement
two mix designs (Table 2). material is the major contributor to the overall environmental
impact in the MIX B (in terms of percentage, Fig. 8b), its environ-
The RLAC produced with Type B LWAs (MIX B) is the option mental burden (expressed as numerical value, Table 9) roughly
characterized by the lowest environmental impacts in all damage corresponds to the contribution of the cement in the NLAC mix.
categories and in almost each transport scenario herein consid- In particular, the environmental outcomes related to the cement
ered. This result can be attributed to a lower amount of LWAs_R in MIX B result slightly higher than those of the cement in MIX
used in the mix design (Table 2). In order to evaluate the influence NA. This is mainly due to a slightly higher amount of cement used
(from the environmental point of view) of Type B aggregates in the in the MIX B (e.g. 400 kg/m3), as reported in Table 2.
lightweight concrete material, a detailed environmental compar- In light of these considerations, it can be finally remarked that
ison of NLAC (MIX NA) and RLAC (MIX B) is performed and the use of LWAs_R to produce 1 m3 of lightweight concrete of
reported in Fig. 8, considering transport scenario 3. The environ- C20/25 strength class and density of 1600 kg/m3 may significantly
mental contribution of LWAs_N (expanded clay) production in reduce the environmental contribution of artificial LWAs to the
the NLAC (Fig. 9a) accounts for approximately 38–74% of the total total environmental burden in all damage categories.
environmental burden (especially in the Human Health, Ecosystem
Quality and Resources category), whereas the environmental con- 5. Sensitivity analysis
tribution of LWAs_R in MIX B (Fig. 8b) is approximately the 3–21%
of the overall impact among the four damage categories. In detail, In addition to System Expansion (SE [41]) a sensitivity analysis is
for these LCA categories, the environmental impact is mainly due performed on the allocation rules, considering also Cut-Off (CO
to expansion process of clay material (accounting for 2.14 04 [54]), procedure as allocation approach. As discussed in the alloca-
DALY, 12.6 PDF*m2*yr, 1970 MJ primary, respectively- Table 9). tion section, according to SE approach, LWAs_R imply 100% of the
These sources of environmental impacts are substantially limited burden of Process A1,2 and Process I1,2, including transportation
in the case of LWAs_R (see previous section on avoided impact and credits from Process D; while, RLAC receives 100% of the burden
and manufacturing process) and the resulting values for MIX B of process B and process D (Fig. 5). Instead, within the CO approach,
are 2.26E 05 DALY, 2.05 PDF*m2*yr and 207 MJ (Table 9). The LWAs_R receive 100% of the burden of only Process I1,2, including
cement material also affects the environmental results of NLAC transportation, and RLAC receives 100% of the burden of process B
in the Climate Change category; the contribution in this category (Fig. 9). Therefore, LWAs_R bear only the impacts of intermittent
380 L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384

100%

90%

80%

70%
(a) Scenario 1 60%

50%

40%

30%

20%

10%

0%
Human health Ecosystem quality Climate change Resources

100%

90%

80%

70%
(b) Scenario 2

60%

50%

40%

30%

20%

10%

0%
Human health Ecosystem quality Climate change Resources

100%

90%

80%

70%

60%
(c) Scenario 3

50%

40%

30%

20%

10%

0%
Human health Ecosystem quality Climate change Resources

MIX A_SE MIX B-SE MIX C-SE MIX NA

Fig. 7. LCA results of NLAC and RLAC (1 m ); (a) Transport Scenario 1; (b) Transport Scenario 2; (c) Transport Scenario 3 (reference flow 1 m3).
3

treatment of LWAs (Process I1,2) and are free of further burdens previous Sections 4.1 and 4.3, highlighting that the transport sce-
related to the production Process A1,2. The cut-off lines are reported nario 2 reduces the environmental benefits (compared with Type
after process A1,2 and at the end of the activities producing the NA) linked to all waste materials (Fig. 6b) and, consequently, to
recycled material. In addition, they do not receive any credit for their use in RLAC (Fig. 7b).
recycling or re-use of waste (Process D). The results are reported in Figs. 10 and 11 for the different allo-
The sensitivity analysis has been conducted considering the cation methods and for LWAs and Lightweight concretes, respec-
Transport scenario 2; this choice is related to the results of tively. The sensitivity analysis identifies the following points:
L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384 381

Fig. 8. LCA results for 1 m3 of lightweight concrete in transport Scenario 3: (a) MIX NA; (b) MIX B_SE.

Fig. 9. Cut off product system related to RLAC production.

Table 9
MIX NA and MIX B: Cement and aggregates impact in 1 m3 of concrete in Transport Scenario 3.

Category Unit Concrete (total values) LWAs Portland cement


MIX NA MIX B Type NA (515 kg) Type B (259.2 kg) MIX NA (330 kg) MIX B (400 kg)
Human health DALY 2.89E 04 1.10E 04 2.14E 04 2.26E 05 6.15E 05 7.45E 05
Ecosystem quality PDF*m2*yr 2.38E+01 1.51E+01 1.26E+01 2.05E+00 8.29E+00 1.00E+01
Climate change kg CO2 eq 4.64E+02 3.56E+02 1.75E+02 9.60E+00 2.66E+02 3.22E+02
Resources MJ primary 3.90E+03 1.97E+03 2.38E+03 2.07E+02 1.15E+03 1.39E+03

- The environmental impacts of LWAs_R and RLAC vary in all LCA not included in the analysis and then, the environmental results
categories when SE and CO methods are applied (Fig. 10). of RLAC are not affected by the environmental benefits of the
- In almost LCA categories, the environmental impacts of avoided processes.
LWAs_R, when CO is applied, are larger than the impacts of - All LWAs_R, even if CO approach is applied, present a lower
LWAs_R calculated with SE approach (Fig. 10). This is related impact than Type NA, in almost all LCA categories, except for
to the fact that when CO approach is applied, the Process D is Type A in the Ecosystem Quality, as in the SE approach.
382 L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384

Human Health_DALY Ecosystem quality_PDF*m2*yr

Type C_CO 1,56E-04 Type C_CO 1,84E+01

Type C_SE 1,45E-04 Type C_SE 7,93E+00

Type B_CO 6,93E-05 Type B_CO 2,03E+01

Type B_SE 1,06E-04 Type B_SE 1,78E+01

Type A_CO 1,18E-04 Type A_CO 3,53E+01

Type A_SE 1,16E-04 Type A_SE 3,42E+01

Type NA 2,68E-04 Type NA 2,06E+01

(a) (b)
Climate Change_kg eq. CO2
Resources_MJ P
Type C_CO 1,82E+02
Type C_CO 2,68E+03

Type C_SE 1,29E+02 Type C_SE 2,20E+03

Type B_CO 7,38E+01 Type B_CO 1,08E+03

Type B_SE 6,20E+01 Type B_SE 1,11E+03

Type A_CO 1,77E+03


Type A_CO 1,21E+02

Type A_SE 9,23E+02


Type A_SE 6,70E+01
Type NA 3,02E+03
Type NA 2,21E+02

(c) (d)
Fig. 10. Sensitivity analysis for LWAs (1 m3); System Expansion (SE) and Cut Off (CO) in Transport Scenario 2: (a) Human Health; (b) Ecosystem Quality; (c) Climate Change;
(d) Resources.

Human Health_DALY Ecosystem quality_PDF*m2*yr

MIX C_CO 1,46E-04 MIX C_CO 1,93E+01

MIX C_SE 2,14E-04 MIX C_SE 2,29E+01

MIX B_CO 1,63E-04 MIX B_CO 2,59E+01

MIX B_SE 1,74E-04 MIX B_SE 2,51E+01

MIX A_CO 1,35E-04 MIX A_CO 2,73E+01

MIX A_SE 2,03E-04 MIX A_SE 3,55E+01

MIX NA 3,05E-04 MIX NA 2,89E+01

(a) (b)

Climate Change_kg eq. CO2 Resources_MJ P

MIX C_CO 3,83E+02 MIX C_CO 2,73E+03

MIX C_SE 4,50E+02 MIX C_SE 3,88E+03

MIX B_CO 4,36E+02 MIX B_CO 3,09E+03

MIX B_SE 4,32E+02 MIX B_SE 3,11E+03

MIX A_CO 3,96E+02 MIX A_CO 2,48E+03

MIX A_SE 4,59E+02 MIX A_SE 3,40E+03

MIX NA 4,79E+02 MIX NA 4,11E+03

(c) (d)
Fig. 11. Sensitivity analysis for RLAC, NLAC (1 m3); System Expansion (SE) and Cut Off (CO) in Transport Scenario 2: (a) Human Health; (b) Ecosystem Quality; (c) Climate
Change; (d) Resources.

- The environmental impact of RLAC, when CO is applied is LWAs (Process I1,2) (see Section 3, Allocation); instead, in
approximately 30% lower than the impact of RLAC calculated the CO approach, the environmental results of LWAs_R
with SE approach (Fig. 11). This is due to the fact that the only depend on the intermittent treatment of LWAs (Process
LWAs_R comprises the production process of secondary I1,2), resulting in a lower environmental profile for all
materials (Process A1,2) and the intermittent treatment of LWAs_R.
L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384 383

- By using the CO allocation method, the LCA results reveal that [4] M. Weil, U. Jeske, L. Schebek, Closed-loop recycling of construction and
demolition waste in Germany in view of stricter environmental threshold
the NLAC still exhibits the largest environmental impact in
values, Waste Manage. Res. 24 (3) (2006) 197–206.
almost all the damage categories; [5] A. Rao, K. Jha, S. Misra, Use of aggregates from recycled construction and
- Also when the CO rule is applied as allocation approach, the demolition waste in concrete, Resour. Conserv. Recycl. 50 (1) (2007) 71–81.
RLAC produced with Type B LWAs is still the option character- [6] M. Hiete, J. Stengel, J. Ludwig, F. Schultmann, Matching construction and
demolition waste supply to recycling demand: a regional management chain
ized by the lowest environmental impacts in all damage model, Build Res. Inf. 39 (4) (2011) 333–351.
categories (Fig. 11). [7] R. Woodward, N. Duffy, Cement and concrete flow analysis in a rapidly
expanding economy: Ireland as a case study, Resour. Conserv. Recycl. 55 (4)
(2011) 448–455.
5. Conclusion [8] C. Hoffmann, F. Jacobs, Recyclingbeton aus Beton- und Mischabbruchgranulat
recycling concrete with concrete waste and mixed rubble as aggregates, Mater.
Sci. Tech. (2007).
In the present study, the environmental impacts of the produc- [9] M. Limbachiya, E. Marrocchino, A. Koulouris, Chemical–mineralogical
tion of different types of lightweight concretes, i.e. NLAC and RLAC, characterisation of coarse recycled concrete aggregate, Waste Manage. 27 (2)
made with different artificial LWAs (LWAs_R and LWAs_N), have (2007) 201–208.
[10] S. Marinković, V. Radonjanin, M. Malešev, I. Ignjatović, Comparative
been investigated by means of a LCA approach.
environmental assessment of natural and recycled aggregate concrete,
With regard to the LCA of LWAs, the results obtained by apply- Waste Manage. 30 (11) (2010) 2255–2264.
ing a SE allocation rule reveal that the production of all LWAs_R [11] C. Meyer, The greening of the concrete industry, Cem. Concr. Compos. 31
(2009) 601–605.
(use of industrial waste raw materials) present a significantly
[12] A. Cabral, V. Schalch, D. Molin, J. Ribeiro, Mechanical properties modeling of
lower environmental burden with respect to the production of recycled aggregate concrete, Constr. Build. Mater. 24 (4) (2010) 421–430.
LWAs_N (use of natural raw materials), mainly due to potential [13] N. Fonseca, J. de Brito, L. Evangelista, The influence of curing conditions on the
benefits of avoided impact (raw material supply and production mechanical performance of concrete made with recycled concrete waste, Cem.
Concr. Compos. 33 (6) (2011) 637–643.
process of LWAs_N). In fact, the clay extraction, its transportation [14] P. Van den Heede, N. De Belie, Environmental impact and life cycle assessment
and the production phase (including clay burning and expansion (LCA) of traditional and ‘green’ concretes: literature review and theoretical
with heavy fuel oil), strongly contribute to the environmental calculations, Cem. Concr. Compos. 34 (2012) 431–442.
[15] P. Wu, B. Xia, X. Zhao, The importance of use and end-of-life phases to the life
impacts of LWAs_N. cycle greenhouse gas (GHG) emissions of concrete – a review, Renewable
Among the LWAs_R, the transport scenario affects the relative Sustainable Energy Rev. 37 (2014) 360–369.
efficiency of different mix options, providing a maximum environ- [16] C. Knoeri, E. Sanyé-Mengual, H. Althaus, Comparative LCA of recycled and
conventional concrete for structural applications, Int. J. LCA 18 (909–918) (2013).
mental benefit for all LWA types when the lightweight concrete [17] V. Corinaldesi, G. Gnappi, G. Moriconi, A. Montenero, Reuse of ground waste
plant is located in the area where Cab70 waste material is collected glass as aggregate for mortars, Waste Manage. 25 (2) (2005) 197–201.
(Scenario 1). Indeed, in this scenario, since the avoided transport [18] L. Pezzi, P. De Lice, D. Vuono, F. Chiappetta, A. Nastro, Concrete products with
waste’s material (bottle, glass, plate), Mater. Sci. Forum (2006) 1753–1757.
distance of clay (e.g. 775 km) is higher than other scenarios (e.g.
[19] N. Saikiaa, J. de Brito, Use of plastic waste as aggregate in cement mortar and
175 km in Scenario 2 and no transport in scenario 3), almost all concrete preparation: a review, Constr. Build. Mater. 34 (2012) 385–401.
LWAs_R show a negative environmental impact. [20] L. Pereira-de-Oliveira, J.P. Castro-Gomes, P.M.S. Santos, The potential
pozzolanic activity of glass and red-clay ceramic waste as cement mortars
With reference to 1 m3 of lightweight concrete of C20/25
components, Constr. Build. Mater. 31 (2012) 197–203.
strength class and 1600 kg/m3 of density, it can be pointed out that [21] F. Iucolano, B. Liguori, D. Caputo, F. Colangelo, R. Cioffi, Recycled plastic
the NLAC mix, in all the damage and impact categories presents a aggregate in mortars composition: effect on physical and mechanical
larger impact than all of the RLAC mixes. Furthermore, the environ- properties, Mater. Des. 52 (2013) 916–922.
[22] G. Habert, J. d’Espinose de Lacaillerie, N. Roussel, An environmental evaluation
mental impact of LWAs_N aggregates in the NLAC production of geopolymer based concrete production: reviewing current research trends,
accounts for around 55% of the total environmental burden, J. Cleaner Prod. 19 (11) (2011) 1229–1238.
whereas the environmental impact of LWAs_R in RLAC is almost [23] L. Napolano, C. Menna, D. Asprone, A. Prota, G. Manfredi, Preliminary remarks
on the environmental impact of ordinary and geopolymer concrete, in: First
15% of total environmental burden. These results are confirmed International Conference on Concrete Sustainability, May 27–29, Tokyo, Japan,
also when a CO rule is applied as allocation approach. 2013.
Finally, as far as lightweight concrete is concerned, it appears [24] J.L. Provis, A. Palomo, S. Caijun, Advances in understanding alkali-activated
materials, Cem. Concr. Res. 78 (2015) 110–125.
that the practice of recycling can be successfully implemented in [25] C. Ferone, B. Liguori, I. Capasso, F. Colangelo, R. Cioffi, E. Cappelletto, R. Di
concrete technology, representing an effective way to convert Maggio, Thermally treated clay sediments as geopolymer source material,
industrial waste products (such as ornamental stone and ceramic Appl. Clay Sci. 107 (2015) 195–204.
[26] M. Collepardi, Il Nuovo Calcestruzzo, 2002.
wastes) into raw resources for producing new materials, support-
[27] I. Chiou, K. Wang, C. Chen, Y. Lin, Lightweight aggregate made from sewage
ing construction waste management and construction stakehold- sludge and incinerated ash, Waste Manage. 26 (12) (2006) 1453–1461.
ers’ decisions. [28] D. Kralj, Experimental study of recycling lightweight concrete with aggregates
containing expanded glass, Process Saf. Environ. Prot. 87 (4) (2009) 267–273.
[29] F. Colangelo, F. Messina, R. Cioffi, Recycling of MSWI fly ash by means of
Acknowledgements cementitious double step cold bonding pelletization: technological
assessment for the production of lightweight artificial aggregates, J. Hazard.
Mater. 299 (2015) 181–191.
Thanks are due to Cementir S.p.A and Italiana Zeoliti s.r.l. for [30] C. Ferone, F. Colangelo, F. Messina, F. Iucolano, B. Liguori, R. Cioffi, Coal
technical support on experimental test on concretes and recycled combustion wastes reuse in low energy artificial aggregates manufacturing,
raw materials used to produce LWA, respectively. Materials 6 (2013) 5000–5015.
[31] R. de Gennaro, P. Cappelletti, G. Cerri, M. de’ Gennaro, M. Dondi, S. Graziano, A.
Langella, Campanian ignimbrite as raw material for lightweight aggregates,
References Appl. Clay Sci. 37 (2006) 115–126.
[32] R. de Gennaro, S. Graziano, P. Cappelletti, A. Colella, A. Langella, M. de’
Gennaro, Structural concretes with waste-based lightweight aggregates: from
[1] Federbeton, www.federbeton.it/, La filiera del cemento e del calcestruzzo
landfill to engineered materials, Environ. Sci. Technol. 43 (2009) 7123–7129.
armato nel mondo delle costruzioni, <http://www.federbeton.it/Portals/3/
[33] R. de Gennaro, A. Langella, M. D’Amore, M. Dondi, A. Colella, P. Cappelletti, M.
Documenti/Pubblici/Pubblicazioni/La%20filiera%20del%20cemento%20e%20del
de’ Gennaro, Use of zeolite-rich rocks and waste materials for the production
%20calcestruzzo%20armato%20nel%20mondo%20delle%20costruzioni.pdf>,
of structural lightweight concretes, Appl. Clay Sci. 41 (2008) 61–72.
2014.
[34] ISO:14040, Environmental management – life cycle assessment – principles
[2] N. Lawson, I. Douglas, S. Garvin, C. McGrath, D. Manning, V. Jonathan, Recycling
and framework, ISO – International Organization for Standardization, ISO
construction and demolition wastes—a UK perspective, Environ. Manage.
14000 International Standards Compendium, Switzerland, 2006.
Health 12 (2) (2001) 146–157.
[35] ISO:14044, Environmental management – life cycle assessment – requirements
[3] A. Blum, S. Stutzriemer, Recycled construction minerals for urban
and guidelines, ISO – International Organization for Standardization, ISO 14000
infrastructure in germany: non technical issues, Miner. Energy Raw Mater.
International Standards Compendium, Switzerland, 2006.
Rep. 22 (3–4) (2002) 148–158.
384 L. Napolano et al. / Construction and Building Materials 119 (2016) 370–384

[36] Laterlite SPA ‘‘www.laterlite.com; www.leca.it”. [47] U. Hossain, C.S. Poona, I.M.C. Lo, J.C.P. Cheng, Comparative environmental
[37] EN 13055-1, Lightweight Aggregates – Part 1: Lightweight Aggregates for evaluation of aggregate production from recycled waste materials and virgin
Concrete, Mortar and Grout, 2002. sources by LCA, Resour. Conserv. Recycl. 109 (2016) (2016) 67–77.
[38] EC2 EuroCode 2, Design of Concrete Structures – Part 1-1: General Rules and [48] S. Yin, R. Tuladhar, M. Sheehan, M. Combe, T. Collister, A life cycle assessment
Rules for Buildings, 2004. of recycled polypropylene fibre in concrete footpaths, J. Cleaner Prod. 112
[39] UNI EN 206-1, Concrete - Part 1: Specification, Performance, Production and (2016) 2231–2242.
Conformity, 2006. [49] F. Faleschini, P. De Marzi, D. Pellegrino, Recycled concrete containing EAF slag:
[40] EU, European Union, (2008). European Union. Directive 2008/98/EC of the environmental assessment through LCA, Euro. J. Environ. Civil Eng. 18 (9)
European Parliament and of the Council of 19 November 2008 on waste (2014) 1009–1024.
Eurostat (2009) Generation of waste, total arising and by selected activities for [50] J. Turk, Z. Cotic, A. Mladenovic, A. Šajna, Environmental evaluation of green
2008. concretes versus conventional concrete by means of LCA, Waste Manage. 45
[41] B. Weidema, Avoiding co-product allocation in LCA, J. Ind. Ecol. 4 (3) (2001) (2015) (2015) 194–205.
11–33. [51] R. Virta, Minerals Yearbook. Clay and Shale (Advance Release), 2012.
[42] ISO:14049, Environmental management - Life cycle assessment - Illustrative [52] EXCA (2013), European Expanded Clay Association, ‘‘EXCA’s contribution to
examples on how to apply ISO 14044 to goal and scope definition and the European Commission’s consultation on structural options for the EU
inventory analysis, 2012. Emission Trading System”. Brussels, 28/02/2013.
[43] C. Chen, G. Habert, Y. Bouzidi, A. Jullien, A. Ventura, LCA allocation procedure [53] ISPRA, Istituto Superiore Per La Protezione E La Ricerca Ambientale- Rapporto
used as an incitative method for waste recycling: an application to mineral Rifiuti Speciali, 2014.
additions in concrete, Resour. Conserv. Recycl. 54 (2010) 1231–1240. [54] Ecoinvent 3, database, <http://www.ecoinvent.org/database/ecoinvent-
[44] G. Habert, A method for allocation according to the economic behavior in the version-3/system-models/allocation-cut-off-by-classification/>, 2014.
EU-ETS for by-products used in cement industry, Int. J. Life Cycle Assess. 18 [55] J. Hedemann, U. König, Technical Documentation of the Ecoinvent Database.
(2013) 113–126. Final report ecoinvent data v2.0 No. 4, Swiss Centre for Life Cycle Inventories,
[45] C. Jiménez, M. Barra, A. Josa, S. Valls, LCA of recycled and conventional Dübendorf, CH, 2007.
concretes designed using the equivalent mortar volume and classic methods, [56] O. Jolliet, M. Margni, R. Charles, S. Humbert, J. Payet, G. Rebitzer, R. Rosenbaum,
Constr. Build. Mater. 84 (2015) 245–252. IMPACT 2002+: a new life cycle impact assessment methodology, Int. J. LCA 8
[46] N. Tosic, S. Marinkovic, T. Dasic, M. Stanic, Multicriteria optimization of natural (6) (2003) 324–330.
and recycled aggregate concrete for structural use, J. Cleaner Prod. 87 (2015)
766–776.

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