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Quantum Dots
J. R. Petta et al.
Science 309, 2180 (2005);
DOI: 10.1126/science.1116955
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RESEARCH ARTICLES the surface, with density È2 1011 cmj2.
Coherent Manipulation of When biased with negative voltages, the
patterned gates create a double-well potential
(Fig. 1A). Tunnel barriers [controlled by
Coupled Electron Spins in voltages VL and VR (L, left; R, right)] connect
each dot to adjacent reservoirs, allowing
Semiconductor Quantum Dots electrons to be transferred into the dots.
Interdot tunneling (at a rate set by voltage
J. R. Petta,1 A. C. Johnson,1 J. M. Taylor,1 E. A. Laird,1 A. Yacoby,2 VT) allows electrons to be moved between
M. D. Lukin,1 C. M. Marcus,1 M. P. Hanson,3 A. C. Gossard3 dots when the detuning parameter e º VR –
VL is adjusted. Measurements are performed
We demonstrated coherent control of a quantum two-level system based on in a dilution refrigerator with electron tem-
two-electron spin states in a double quantum dot, allowing state preparation, perature Te È 135 mK, determined from
coherent manipulation, and projective readout. These techniques are based on Coulomb blockade peak widths. Gates L and
rapid electrical control of the exchange interaction. Separating and later R are connected via low-temperature bias tees
recombining a singlet spin state provided a measurement of the spin to high-bandwidth coaxial lines, allowing
Fig. 3. (A) Pulse sequence used to measure T2*. The system is initialized into a function of tS at 100 mT (black curve) and 0 mT (red curve). For tS ¡ T2*,
(0,2)S and transferred by rapid adiabatic passage to the spatially separated S the singlet state does not have ample time to dephase, and PS È 1. For tS d
state. With TT separated by a Zeeman field, S and T0 mix at large detuning T2*, PS È 0.7 at 100 mT and PS È 0.5 at 0 mT. A semiclassical model of
(light blue region), where hyperfine fields drive rotations about the x axis in dephasing due to hyperfine coupling (23) predicts PS È 1/2 at high field and
the Bloch sphere. After a separation time tS, the state is projected onto (0,2)S. PS È 1/3 at zero field. Fits to the model (solid curves), including a parameter
(B) Singlet probability PS measured using the calibrated QPC charge sensor, as adjusting measurement contrast, give T2* 0 10 ns and Bnuc 0 2.3 mT.
Fig. 4. (A) Pulse sequence demonstrating exchange control. After initializing in oscillations in PS as a function of both e and tE. (Inset) Model of PS using
into (0,2)S, detuning e is swept adiabatically with respect to tunnel J(e) extracted from S-Tþ resonance condition, assuming g* 0 –0.44 and ideal
coupling through the S-Tþ resonance (quickly relative to S-Tþ mixing), measurement contrast (from 0 to 1). (C) Rabi oscillations measured in PS at
followed by a slow ramp (tA È 1 ms) to large detuning, loading the system in four values of detuning indicated by the dashed lines in (B). Fits to an
the ground state of the nuclear fields kj,À. An exchange pulse of duration tE exponentially damped cosine function, with amplitude, phase, and decay
rotates the system about the z axis in the Bloch sphere from kj,À to k,jÀ. time as free parameters (solid curves), are shown. Curves are offset by 0.3 for
Reversing the slow adiabatic passage allows the projection onto (0,2)S to clarity. (D) Faster Rabi oscillations are obtained by increasing tunnel coupling
distinguish states kj,À and k,jÀ after time tE. Typically, tS 0 tS¶ 0 50 ns. (B) PS and by increasing detuning to positive values, resulting in a p-pulse time of
as a function of detuning and tE. The z-axis rotation angle f 0 J(e)tE/I results È350 ps.
References and Notes 19. K. Ono, D. G. Austing, Y. Tokura, Science 297, 1313 32. We have verified that the system is in the ground
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cond-mat/0412048 (2004). 29. The separation detuning can be changed by keeping pulse Zoller. Funding was provided through the Army
13. A. C. Johnson et al., Nature 435, 925 (2005). displacements fixed and sweeping the measurement Research Office under grants DAAD55-98-1-0270
14. J. Levy, Phys. Rev. Lett. 89, 147902 (2002). point detuning using dc gates, or by keeping the and DAAD19-02-1-0070; the Defense Advanced
15. Except where noted, a Tektronix AWG520 pulse measurement point fixed and changing pulse parameters. Research Projects Agency–Quantum Information
generator with a 1-ns minimum pulse width was 30. J. M. Taylor et al., in preparation. Science and Technology program; NSF under grant
used for fast gate control. The sample response to 31. The semiclassicalmodel developed in (23, 30) yields DMR-0072777; the NSF Career Program; the Harvard
fast pulses was checked by measuring gs with pulses 2
PS ðtS Þ 0 1 j C21 1 j ejðtS =T2 Þ for B d B nuc and Center for Nanoscale Systems; and the Sloan and
applied individually to gates L and R. A doubling of n 2
n Packard Foundations.
PS ðt S Þ 0 1j 34 C2 1j 19 1 j 2ej2ðt S =T2 Þ ðt S =T2 Þ2 j
1
the charge stability diagram was observed for pulse
widths down to 1 ns (12).
o2
16. J. R. Petta, A. C. Johnson, C. M. Marcus, Phys. Rev. 5 July 2005; accepted 22 August 2005
1 for B ¡ Bnuc. A fit to the 100-mT data gives
Lett. 93, 186802 (2004). Published online 1 September 2005;
17. M. Field et al., Phys. Rev. Lett. 70, 1311 (1993). C1 0 0.62 T 0.01 and T2* 0 10 T 1 ns. A fit to the B 0 0 10.1126/science.1116955
18. J. M. Elzerman et al., Phys. Rev. B 67, 161308 (2003). data with T2* 0 10 ns fixed gives C2 0 0.74 T 0.01. Include this information when citing this paper.