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The THALES-2 code is an integrated severe accident analysis code developed at the Japan Atomic
Energy Research Institute (JAERI) in order to simulate the accident progression and transport of
radioactive material for probabilistic safety assessment (PSA) of a nuclear power plant. As part of a
level 3 PSA being performed for a l,100MWe BWR-5 with a Mark-II containment, a series of
calculations were performed by THALES-2 to evaluate the source terms for extensive accident
scenarios. This paper presents the methods and insights on the dependency of source terms on the
core damage sequences and the containment function failure scenarios from this analysis.
As for core damage sequences to be analyzed, 5 following representative core damage sequences
were selected from the core damage sequences systematically identified by PSA works at JAERI; (1)
Loss of containment heat removal with high pressure injection available, (2) Loss of containment
heat removal with low pressure injection available, (3) Loss of coolant injection to the core, (4)
Station blackout and (5) Anticipated Transient Without Scram (ATWS) with high pressure injection
available. As for containment function failure scenarios, this analyses covered the following 4
containment function failure scenarios: overpressure in drywell, overpressure in wetwell, controlled
release by unfiltered containment venting and accident termination by drywell spray recovery. All
physically possible combinations (15 scenarios) above core damage sequences and containment
function failure scenarios were analyzed by THALES-2 to determine the source terms.
Results and insights from the analyses were that 1) the calculated release fractions of Csl and
CsOH to the environment were in the range of 0.01 to 0.1 for late containment overpressure failure
cases, and the release fractions for the containment venting cases were one order of magnitude
smaller than that of over-pressure case and those for drywell spray recovery cases where no
containment failure occurred were two orders of magnitude smaller than the containment venting
cases, 2) the governing factors for source terms of Iodine and Cesium are different depending on
whether the containment fails before core melt or not, 3) the containment venting, which is one of
the accident management measures, can be expected to reduce source terms of I and Cs if
suppression pool bypass is avoided.
Keywords: Source Terms, Severe Accident, THALES-2, Level 2 PSA, BWR, Mark-II Containment
* Japan Systems Corporation
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Contents
1. Introduction 1
1.1 Background and Objective 1
1.2 Outline of the Analysis 1
1.3 Composition of the Report 2
2. Plant and Accident Scenarios Analyzed 3
2.1 Plant Description 3
2.2 Accident Scenarios 3
2.2.1 Core Damage Sequences 3
2.2.2 Containment Function Failure Scenarios 6
2.3 Calculation Conditions and Cases 8
3. Calculation Models and Conditions for Analysis 9
3.1 Modeling of Plant and Thermal Hydraulic Phenomena 9
3.1.1 Volume and Connection Models 9
3.1.2 Modeling of Core Cooling and Containment Cooling Systems 10
3.1.3 Modeling of Phenomena under Severe Accident Conditions 11
3.2 FP Release Path and FP Transport Behavior 13
3.2.1 Models of FP Transport 13
3.2.2 Models of Gaseous FP Deposition 16
3.2.3 Models of Aerosol Deposition 17
3.2.4 Models of Aerosol Growth 19
3.2.5 Models of Pool Scrubbing 20
3.2.6 Models of FP Removal by Spray 21
4. Calculation Results for Accident Progression and Thermal Hydraulic Behavior 22
4.1 Loss of Core Cooling Function (TQUV) Sequence 22
4.2 Station Blackout (TB) Sequence 24
4.3 Loss of Containment Heat Removal with a Low Pressure Injection (TQUVl W) Sequence • 25
4.4 Loss of Containment Heat Removal with a High Pressure Injection (TW) Sequence 26
4.5 ATWS with High Pressure Injection Available (TC) Sequence 27
4.6 Governing Factors for Event Time 27
5. Calculation Results for Source Terms 29
5.1 Dependency of Source Terms on Containment Function Failure Scenarios 29
5.1.1 Source Terms of TQUV Sequence 29
5.1.2 Dependency of FP Removal on Size of Spray Droplet 35
5.1.3 Dependency of Source Terms 36
5.2 Dependency of Source Terms on Core Damage Sequences 40
5.2.1 Comparison of Source Terms of Xe(Overpressure Failure Case) 40
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JAERI-Research 2005-021
(3) y-*7-McR\£r&m(p>bm^-®.y-fry*\z.xz>*m)
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tzz\btf±mtemmxb&o z\(D2oco^^cy-fry*<DbhTBy-fry*^ fam
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47
JAERI-Research 2005-021
# n xm
U.S. Nuclear Regulatory Commission,"Severe Accident Risks: An Assessment for Five U.S.
Nuclear Power Plants", NUREG-1150,Vol.2, Appendix C,1990.
(MM^TJ^m&mmn," y<;^ 2PSA W © M t e g f l ^ 5 M # = B W R fryyb
=",INS/M99-17, 2000.
(MM^ts^mmmmm," y^v 2PSA ^mcommim-y §fR^#=BWR fry y b ©
7 - x y — i»=",INS/M01-14, 2002.
(Wi)m^7j^m^mmm:y-<7V 2PSA ¥ & © M t e § 8 - f 5 f g ^ # = B W R 7 * 7 ^ h-
=",INS/M02-11,2003.
M. Kajimoto et al., "Development of THALES-2, A Computer Code for Coupled Thermal
Hydraulics and Fission Product Transport Analysis for Severe Accident at LWRs and Its
Application to Analysis of Fission Product Revaporization Phenomena", Proc. of Int. Mtg.
on Safety of Thermal Reactors, Portland. 584,1991.
K. Abe, et al. , "Overview of Development and Application of THALES Code system for
Analyzing Progression of Core Meltdown Accident of LWRs, Proc. of 2nd Int. Symp. on
Nuclear Power Plant Thermal Hydraulics and Operations", Tokyo. 6.49K,1986.
tt&te {fomft^yp^fr/vfrj y b PSA © » ^ £ ( f f l ) " , f ? 4 m PSA teH-f§H
ft v'^/tf ^ 7 A f&3d|,IAE-R8903,1989.
mm myp'bmm^-^comm^mr^m^", mswipsAim^y&mftyytfv?
1* tm ;£^,IAE-R9006,1990.
N. Watanabe, et al.,"Categorization of Core-Damage Sequences by Containment Event Tree
Analysis for Boiling Water Reactor with Mark-II Containment",3rd International Conference
on Containment Design and Operation,Toronto,1994.
(MM^mm&wmm m^jj^Mtifm," ^7WPSA¥&©Mtep-r 5$R£r»
=BWR7°7>- h=",INS/M97-14,1997.
R. S. Denning et al., "Radionuclide Release Calculations for Selected Severe Accident
Scenarios", report for the U.S. Nuclear Regulatory Commission, NUREG/CR-4624,
BMI-2139, Volumes I-V, July, 1986.
M.Matsumoto,et al., "Preliminary Results of Steel Containment Vessel Model Test",
Transaction of SMiRT-14,H03/2,1997.
Luk,et al.,"Steel Containment Vessel Model Test: Results and Evaluation", Transaction of
SMiRT-15,H06/5,1999.
U.S. Nuclear Regulatory Commission, "Design, Instrumentaion, and Testing of a Steel
Containment Vessel Model",NUREG/CR-5679,SAND98-2701,1999.
L. Baker and C. Just, "Studies of Metal-Water Reactions at High Temperatures III.
Experimental and Theoretical Studies of the Zirconium-Water Reaction", ANL-6548
Argonne National Laboratory, May 1962.
M. Kajimoto, et al., "The validation of the ART Code Through Comparison with NSPP
Experiments in the STEAM-AIR Atmosphere", Workshop on Thermal Hydraulics and
Aerosol Behavior in Containment, Phontna-aux-Roses, France, CSNI Report No. 176, 1990.
^ # %§m, "p>bmm&£t FP mimmmvr^- K ART © { £ / W § I # " , JAERI-M
88-093,1988.
A. Hidaka, et al., "Comparative Study of FP Deposition in Wind Project by ART and
VICTORIA", International Conference on Probabilistic Safety Assessment Methodology and
Applications, PSA'95, Korea, 1995.
M.R.Kuhlman, D.J.Lehmicke, R.O.Meyer, "CORSOR User's Manual", NUREG/CR -4173 ,
BMI-2122, May 1985.
U.S. Nuclear Regulatory Commission,"Technical Bases for Estimating Fission Product
Behavior during LWR Accidents", NUREG-0772, 1981.
J. A Gieseke, P. Cybulskis, R. S. Denning, M. R. Kuhlman and K. W. Lee, "Radionuclide
Release Under Specific LWR Accident Conditions", Report for the U.S. Nuclear Regulatory
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[3-38] W.E.Ranz,W.R.Marshall, "Evaporation from Drops Part I", Prog.Nucl.Eng. 48,3, PP.141-146,
Mar.1952.
[3-39] W.E.Ranz,W.R.Marshall,"Evaporation from Drops Part II", Prog. NUcl.Eng. 48,4,
pp. 173-180, Apr. 1952.
[3-40] D.R.Grist, "Spray Removal of Fission Products in PWR Containments", Report SRDR267,
Safety and Reliability Directorate, UKAEA, England, 1982.
[3-41] A.K.Postma, et al., "Models for Predicting the Removal of Airborne Contaminants by
Reactor Containment Systems", BNWL-B-417, 1975.
[3-42] I.Langmuir, J.Meteor., "The Production of Rain by a Chain Reaction in Cumulus Clouds at
Temperatures above Freezing.", J. Meteor., 5, 175-192,1948.
[5-1] M. Tanaka, et al., Performance of Containment Sprays for Light Water Reactors and
Evaluation of the Heat Transfer, Nuclear Technology, Vol.54, 1981
[6-i] #w &.% m,"m7Kp^ry^y°7y b<&£#&##wy tttt-tz&m&wmm
",JAERI-Research 2000-060,2000.
[6-2] T. Homma, Y. Inoue and K. Tomita, "OSCAAR Caluculations for the Hanford Dose
Reconstruction Scenario of BIOMASS Theme 2", JAERI-Research 2000-049,2000.
-50-
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Table 2. 3. 2 f&8x0kW
Wti mn THALES-2 M^f AzCDfcfe
fryyb&£: BWR(Type-5, Mark-II)
pmtj fitti/J 3300MWt (110 75 kWe B.)
K7-T <7^7V(DAV)te, '<7!s\#;l>QfflUft&&^'&fc
m 5400m* b L tz0 7^7 b7^/HWW)fc, W®U#
tmm%&w m 4100 mSbmmWf-^M 3400 m.s bLtz0 Jfc^yb
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(7ft2)£{£ffl
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JAERI-Research 2005-021
Table 3. 1. 2 X^ftjS^fitOSS;^
T.^m^±mm W^MSL «
m^pmmmifcMZk 140 t/hr RCIC tfyfrCOfefa®t;
(RCIC) (38.89kg/s)
Mfrp'b*fryy 1580 t/h MB* frv4 TK yfr®mcoMA®m^ i)
(HPCS) (438.89 kg/s)
i&j±p<b&7y& 1690 t/hr/iS a^mi^*^^7°^*
(LPCI) (469.44 kg/s/t?)
\&frp'b*fryy%k 1440 t/hr/i§? ^f^^^T^l;^"
(LPCS) (400 kg/s/t?)
MS^/WI -DAV*7°WSEfl: -gS@fUSfc£#l'7 p <7);£*fc$l: 1690 t/hr
95%flt(444kg/s) -DAV^7V-Tf-i N ^ ^ ^ * 0 95%
-WAV*7V^Mfi - W A V ^ 7 V - ( « , g f e t i © 5%
5%16(25kg/s)
nmm$k:m&#m 4610 kcal/s £*&B£$I*
D/W:Ky-ry^/K wmfr^y by^^
£ 1 : #$P#fT*fiI£/B LX^ft^
Table 3. 2. 2 x 7 o '//V§tfi^ 7 *
ft^7y i 7 a y ^ f l ^ 7 7
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mi) (£1)
14 13
I 1.2566X10" 1.0053X10" 0.1 0.2
2 1.0053X10"13 8. 0425X10"13 0.2 0.4
3 8. 0425X10"13 6. 4340X10"12 0.4 0.8
4 6. 4340X10"12 5. 1472X10-11 0.8 1.6
5 5. 1472X10"11 4. 1177X10'10 1.6 3.2
6 4. 1177X10"10 3. 2942X10"09 3.2 6.4
7 3. 2942 X 10"09 2. 6354X10"08 6.4 12.8
8 2. 6354X10"08 2. 1083X10"07 12.8 25.6
9 2. 1083 X 10"07 1.6866X10"06 25.6 51.2
10 1.6866X10"06 1. 3493X10"05 51.2 102.4
£ 1 : x.7v//us&&& 3.0[g/cm3]LfcS^©ffl(^ig|4, l U ^ O S C T ^ - b\hXl\9-&*i%)
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0 200 400 600 800 1000 1200 1400 1600 1800 2000
H#*J[#]
Fig. 5.1.3 7^yb7=^7Vp%C0 Xe <7}^R)(TQUVi \fr-*)
I s/p|r3fn
<S io"
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10"
10"4 1 — I — I — I — I — I — I — I — I — I — I — I — I — I — I — [ — - I — I — I -
0 200 400 600 800 1000 1200 1400 1600 1800 2000
mmm
Fig. 5.1.4 K7^f!>x;H^©Xe comW) (TQUV mfrM^fr—*)
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0 200 400 600 800 1000 1200 1400 1600 1800 2000
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- \ — ■ — i — ■ — i — ■ — r ^ — i — ■ — i — ■ — r
0 200 400 600 800 1000 1200 1400 1600 1800 2000
- I — I — I — I — I — I — 1 — — 1 — I — I — I — I — I — I — I — I -
0 200 400 600 800 1000 1200 1400 1600 1800 2000
mum
Fig. 5.1.8 y~^yb7^ftco Csl CO^Wl (TQUV T&fr$l£kfr—s\)
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10° T
101
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0 200 400 600 800 1000 1200 1400 1600 1800 2000
flp«[#]
Fig. 5.1.11 mi-p^m^co sr comwiftquvmfrifomfr-*)
n—■—i—•—i—'—i—■—i—■—i—■—i—■—r—■—r
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Fig. 5.1.12 7^7b7^7V^(D Sr (D^ib(TQUVmfrMMkfr—*)
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TtWvyKfl&Jft
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n 1 1 1 1 ' r—> 1 1 1 1 1 1 1 1 1 r-
0 200 400 600 800 1000 1200 1400 1600 1800 2000
Wi
ft
- i — i — i — i — i — \ — i — i — i — i — i — i — i — i — i — i — i — r
0 200 400 600 800 1000 1200 1400 1600 1800 2000
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10°
cvOMfcM—|l~~ ^ Hh HI
10"
10-2 ^fx^;i/@i
L1
fin
tt 10"3
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10"
0
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1
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Fig. 5.1.18 ±XC0 F? com^coikm^ (Tquv ^mi&mfr-*)
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rm 10
tt 10
It
T ' r
0 200 400 600 800 1000 1200 1400 1600 1800 2000
B*«[»]
Fig. 5.1.19 W^PftiZmftco Csl comMTQUV ^mmmfr-*)
10u
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10"S
<-p 10"'
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tt io_34-
ft
i— r ~ i -r
0 200 400 600 800 1000 1200 1400 1600 1800 2000
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10° T
TSP'v;/K IhHh
0 200 400 600 800 1000 1200 1400 1600 1800 2000
B#*J[»]
Fig. 5.1.22 w^p^zmftco sr comMTquv ^miktufr-*)
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10°
cvOhttM HI—
10"
2
10
Z io"3
<□
10"5
m
10"6
10" 7 i
10" ^ — i ■ i ' r
J^
0 200 400 600 800 1000 1200 1400 1600 1800 2000
0 200 400 600 800 1000 1200 1400 1600 1800 2000
l«J[#]
Fig. 5.1.24 bfr-fT-^ftco Sr (73^®](TQUV mtktflfr-*)
109-
JAERI-Research 2005-021
m10
ft
0 200 400 600 800 1000 1200 1400 1600 1800 2000
H#«[#]
Fig. 5.1.25 W^P^M^\H(DXeComWi(TqUV-BfW*fry-(mBfr-*)
10u
10"
S 10"2
m
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*F to S » ffl »
10 ~l—■—i—■—i—'—i—■—i—■—i—■—i—■—i—■—i—■—r
0 200 400 600 800 1000 1200 1400 1600 1800 2000
mmim
Fig. 5.1.26 7^.yb^^)v^oo Xe C0^W)(TqUV-D/W *fryAWBfr—*)
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10° 1 z
D/WX^WmiH
£ 10"2
^fx^ji/ii
TSP^^Kfift* as;
It
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3
10~
10"
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Fig. 5.1.27 by^(7^7V^co Xe (7)^a(TQUV-DAV^yu^^l0^-^)
(m ttmxs xefr*fryy7k\^m.fr\z.mMLtzz\b*fF-y
Xe(-) Te(-)
Csl(-) CsOH(-)
Sr(-) Ru(-)
Ce(-)
-| 1 1 1 1 , 1 r f ^ r"-r"~1 T
0 200 400 600 800 1000 1200 1400 1600 1800 2000
B#£i][#]
Fig. 5.1.28 ^m^cotttli\m-&(TQUV-D/W*frUAmmfr-*)
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10° i
I— £wb$lftlHte
-i—i—i—i—i—i—i—i—i—i—i—i—i—r-
0 200 400 600 800 1000 1200 1400 1600 1800 2000
B#£IJ[#]
Fig. 5.1.29 W-^P^M ^\Hco Csl <7)^ft(TQUV-D/W *:/U/f1t 10^r-x)
10° T
10-1 p
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10
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10
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Fig. 5.1.30 7^yb7^ft(D Csl <7)ipfiKTQUV-D/WX7°W^I0'7--x)
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10 u
: TSP^vKfiKli D/WX^WfllS
i—■—T—'—i—■—i—'—i—'—i—■—r
0 200 400 600 800 1000 1200 1400 1600 1800 2000
H#*J[#]
Fig. 5.1.31 bfrA7^7V^co Csl comMTQUV-DW *fruAmmfr-*)
-i—i—■—i—■—i—■—i—■—i—■—i—■—i—■—i—■—r
1100 1120 1140 1160 1180 1200 1220 1240 1260 1280 1300
B#*!l[#]
Fig. 5.1.32 KM^^%bD/W*frUAKX^^^9^(Dm%(TqUV-D/W*fryym\Bfr-*)
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10"
*P'd>jSHtMi& D/WX^U-flftlB
10"
<n 10-3
gas
St*
lb^P#7f
-i 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 r-
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B#*|[fl\l
Fig. 5.1.34 7^yb7^7Vp%<D Sr <D^W)(TqUV-T>W *fryynfr—*)
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10
10"
10"
TSP^yKflftH D/)Ns\Zfis^m\B
<n 10' 4
w
&
It 10"5
i—'—i—r—i—■—i—'—i—'—i—'—i—■—r
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B#*JKH
Fig. 5.1.35 by^7^7V? \(D Sr <7^®)(TQUV-D/Wx:/.W^|07r-X)
10"
StattftCm]
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30 40 50
oc7'n)//>ilL#[/xm]
Fig. 5.1.37 *yw.c«fc5l&sfe$:£(£;ic? !5')
■ 4.0E3
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A 7.0E4
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4tf
40 50 60 70 80
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JAERI-Research 2005-021
m±mm)M- A • 1
mssmwM- 4 • 1
wmm- ▲ 1l 1
D/WJUmR- A 1 1
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1 0 * 10" 10" 10" 10" 5 10" 4 10" 3 10" 2 10" 1
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i
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tsfcta * ' A •■
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K
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-Te
TQUV1W -<- -Ru
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10"9 10"8 10"7 10"6 10"5 10~4 10"3 10"2 10"1 10° 101
Fig.5.2.2 T&fr$i&fr—si\z.$5tfZy—x
? —J»
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i?i£(RCS)
a*(RCS)
j?3S(DRYW)
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Fig. 5.2.3 TQUV i i f f M ^ - * CO Xe Wm
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a#(Rcs)
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0 200 400 600 800 1000 1200 1400 1600 1800 2000 2200 2400
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0 200 400 600 800 1000 1200 1400 1600 1800 2000
H#*U[#]
Fig. 5.2.5 TQUVIW MfrM&fr—x CO Xe COmW]
2000 2200 2400 2600 2800 3000 3200 3400 3600 3800 4000
BS*J[#]
Fig. 5.2.6 TW T&frffi&fr-X CO Xe (D^Wl
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10'
j?jS(RCS) 8t*(RCS)
j?iS(DRYW) jJt.t(DRYW)
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10"
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10"
200 400 600 800 1000 1200 1400 1600 1800 2000
B#£IJ[#]
Fig. 5.2.7 TQUV$ifrnfr—XGO Csl £#SJ
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»j»(RB) * £fc*(RB)
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T 10°
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10"
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—i—'—r
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B#*|[#]
Fig. 5.2.8 TB i |7r—y^(D C s l » ^
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10*
j?ifi(RCS) ftSCRCS)
J¥&(DRYW) ■ ;A*(DRYW)
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; x x x x x
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— —
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H#*|[#]
Fig. 5.2.10 TWMfrWfr—y-CO Csl comwi
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10" 1 T
■MB irr 5
10
ttl
-i—|—i—|—i—I-H—riH—i a
r i—i—i 'i^'i—i—|—n—i—■—i—■—r
0 200 400 600 800 1000 1200 1400 1600 1800 2000 2200 2400
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0 200 400 600 800 1000 1200 1400 1600 1800 2000
B#*J[#]
Fig. 5.2.13 TQUVIW ^frM^fr—*CO Sr co^W]
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2
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A 3*3f(WETW)
o »itt(RB)
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10"7 =
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2000 2200 2400 2600 2800 3000 3200 3400 3600 3800 4000
B#*][#]
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The THALES-2 codeclJ'[2I'[3]'[41 is an integrated severe accident analysis code developed at the
Japan Atomic Energy Research Institute in order to simulate the accident progression and
transport of radioactive material for probabilistic safety assessment (PSA) of a nuclear power
plant. As part of a level 3 PSA being performed at JAERI for a l,100MWe BWR-5 with a
Mark-II containment, a series of calculations were performed by THALES-2 to evaluate the
source terms for extensive accident scenarios. This paper presents the insights from the
analyses.
2. FP RELEASE SCENARIOS
In this paper, the FP release scenarios are defined by combinations of a core damages
sequence scenario and a containment function failure scenario. The core damage sequence
means a combination of success/failure of safety systems and operations for prevention of core
damage. The containment function failure scenario means a combination of the containment
failure modes which define the reason of containment failure such as overpressure,
overtemperature, accident management measures taken for mitigation and the location of
containment failure. As for the energetic events such as steam explosion which cannot be
simulated by THALES-2, these scenarios are out of the calculation case.
3. MODELING BY THALES-2
The THALES-2 BWR version, used in this study, simulates the thermal-hydraulic transient in
the reactor cooling system of a BWR and its containment and reactor buildings with
consideration of the operation of emergency core cooling systems (ECCS) and other engineered
safety systems together with their control logics.
The thermal hydraulics model of the code is based on a volume-and-j unction concept.
Parameters such as mass of fluid, pressure, mixture level, void fraction, and temperatures of
fluid (gas and liquid) and wall are calculated in each volume. The core region is divided by axial
and radial nodes. The temperatures of fuel and cladding in each node are calculated with
consideration of the relocation of molten-fuel to lower region. Severe accident phenomena
considered in the code include the hydrogen generation by the metal-water reaction, reactor
vessel lower head failure, hydrogen burning in the containment and generation of
non-condensable gases by the molten-core/concrete interaction.
The models for the FP release and transport are based on those of the ART code'51 and they
cover the release of FPs from fuel and the transport of FPs in the form of gas, aerosol, deposit
on structure walls and floors, and solution in water. THALES-2 solves the governing equations
for multi-component aerosol, taking into account the particle size distribution by a sectional
method. The aerosol model considers the size growth by agglomeration and
condensation/evaporation, chemical adsorption of the gas species at structure surfaces,
deposition of aerosol to walls and floors, removal by sprays and filters, scrubbing by water
pools, and convection by liquid as well as gas flow. The aerosol removal by pool scrubbing in
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the suppression pool is calculated by the Kaneko's model[6] based on experiments by the
Japanese utilities.
In THALES-2, radionuclides including components of fuel and structure materials are
classified into 10 groups in terms of chemical properties. Seven representative chemical species
or elements, i.e., Xe, Csl, CsOH, Te, Sr, Ru and Ce, were considered in this study.
The control volumes for representing the BWR in the present analysis is shown in Fig. 1. The
reactor cooling system was divided into seven volumes, the reactor core, upper plenum, steam
dome, down comer, lower plenum and recirculation loops A and B. Moreover, the containment
was divided into drywell, wetwell, pedestal, and vent pipe that connects the drywell and wetwell.
The environment was modeled by hypothetical volumes connected with the containment or the
reactor building by junctions representing the leaks or piping for containment venting. Other
models used in this analysis include: the filtration of FPs by the stand-by gas treatment
system(SGTS), feedwater system, reactor core isolation cooling system(RCIC), high pressure
core spray system(HPCS) and low pressure injection system(LPCI) that takes suction from the
condensate storage tank or suppression pool.
A characteristic feature of this plant is that it has the suppression pool under the drywell floor;
therefore, if the drywell floor is penetrated by the molten core, the melt will fall into the
suppression pool and it makes a flow path from the drywell to the containment venting pipe that
bypasses the suppression pool. The suppression pool bypassing is expected to increase the
source terms when containment venting is conducted for preventing the overpressure failure of
the containment.
The source term analyses were performed for the representative sequence of each core damage
sequence group with THALES-2. Considering the various influencing factors on source terms,
the source term analyses were performed for a variety of FP release scenarios. The present
analyses covered the following 3 containment function failure scenarios in the FP release
scenarios: overpressure, controlled release by unfiltered containment venting and accident
termination by drywell spray recovery. Furthermore, as for the over pressure, which was
considered to be more important than the other containment function failure scenarios from the
frequency and consequence point of view, two different failure locations, drywell and wetwell,
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were considered. Thus, the source term analyses were performed with THALES-2 for 15 relase
scenarios except what can't happen from the combination of 20 scenarios given by 4
containment function failure scenarios for each of the 5 core damage accident sequences.
Since it is considered that the radionuclides Xe, Csl and CsOH, which are volatile and have
high release fractions to the environment, should be important for the consequence analysis, this
paper describes the source terms for these radionuclides. The other radionuclides, which have
much lower volatility, have smaller release fractions and relatively lower importance for level 3
PSA. In order to understand governing factors for the source terms of non-volatile species, the
results for Sr, which has relatively high source term among non-volatile radionuclides, are
discussed in this paper as a representative of non-volatile species.
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JAERI-Research 2005-021
release to the environment for other containment function failure scenarios may be determined
as the times of events shown in Fig.2 such as the times of the core support plate failure, reactor
pressure vessel head failure, and melt through of pedestal floor.
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using the calculation results of a core damage sequence TQUV as a representative example.
Figure 4 shows source terms for all containment function failure scenarios, almost 100% of Xe
would be released to the environment except for non-containment failure case (drywell spray
recovery case). And Sr doesn't depend on the containment function failure scenarios.
Source term of Csl tend to becomes small in the order of overpressure failure case,
containment venting case and drywell spray recovery case.
The source term of drywell failure case is slightly larger than that of the wetwell failure case.
This small difference can be explained by the fact that, as was described in section 5.2, the Csl
suspended in RCS is the dominant factor for source terms. This is based on the difference of the
path from RCS to the environment.
The drywell spray recovory case was analyzed with the assumption that the drywell spray and
the residual heat removal system of containment were recovered at 20 hours after accident
initiation. The containment doesn't fail in this case because of the successful removal of decay
heat from the drywell and wetwell. The FP release to environment is only by the small leakage
from the containment. This case has the smallest source terms in all core damage sequences.
As for the containment venting case, the vent valve was assumed to open at the pressure 1.5
times higher than the design pressure of the containment and close at the design pressure. At the
timing of the failure of the pedestal floor, the molten fuel drops into the suppression pool. At the
same time, the drywell pressure increases significantly and the first containment venting occurs.
Figure 5 shows the relative mass for total core inventory of Csl in the plant for containment
venting case of TQUV sequence as an example. Since the depressurization by the containment
venting actuation is smaller than that by the containment overpressure failure, the
depressurization of containment by the venting does not cause the release of large fraction of the
FP suspended in RCS. Thus the dominant factor of this case is not the Csl suspended in RCS but
that suspended in the drywell. Furthermore, it should be noted that the source term of
containment venting case is significantly smaller than that of over pressure failure case. The
reasons for this difference is that (1) the contribution of Csl suspended in RCS is smaller in the
venting case because of lower RCS wall temperature and smaller depressurization of the RCS
and (2) the shorter duration(several minutes in the present calculation) of release in the venting
case allow the more deposition of aerosol in the containment. The present results suggest that
the containment venting, which is one of the accident management measures, can be expected to
reduce source terms. But it has a demerit that the release of FP to the environment occurs at
earlier phase than in the overpressure failure case.
6. CONCLUDING REMARKS
Using the THALES-2 code, a set of source terms were calculated for use in a level 3 PSA of a
BWR with Mark-II type containment, and for obtaining better understanding on the profile of
source terms of severe accident scenarios. Results and insights from the analyses for a
l,100MWe BWR-5 with a Mark-II type containment were that 1) the calculated release
fractions of Csl and CsOH to the environment were in the range of 0.01 to 0.1 for late
containment overpressure failure cases, and the release fractions for the containment venting
cases were one order of magnitude smaller than that of overpressure failure cases and those for
drywell spray recovery cases where no containment failure occurred were two orders of
magnitude smaller than the containment venting cases, 2) the governing factors for source
terms of Iodine and Cesium are different depending on whether the containment fails
before core melt or not, 3) the containment venting, which is one of the accident
management measures, can be expected to reduce source terms if suppression pool
bypass is avoided.
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REFERENCES
[1] Kajimoto, M., et al., "Analysis of Source Term Uncertainty Issues for LWRs", PSAM-II, San
Diego,(1994)
[2] Kajimoto, M. et al. "Development of THALES-2, A Computer Code fort Coupled Thermal
Hydraulics and Fission Product Transport Analysis for Severe Accident at LWRs and Its
Application to Analysis of Fission Product Revaporization Phenomena, Proc. of Int. Mtg. on
Safety of Thermal Reactors, Portland. 584,1991.
[3] Muramatsu, K., et al., "Modeling Improvement and Application of the Intergrated Severe
Accident Analysis Code THALES-2 for Assessment of Accident Management Strategies",
PSA95, Korea, 1995.
[4] Ishikawa, J. et al., "Systematic Source Term Analyses for Level 3 PSA of a BWR with
Mark-II Type Containment with THALES-2 code", 10th International Conference on
Nuclear Engineering, Apr., 2002.
[5] Ishigami, T. et al., "User's Manual of ART Code for Analyzing Fission Product Transport
Behavior during Core Meltdown Accident", JAERI-M 88-093,1988.
[6] Kaneko, I., et al., "Experimental Study on Aerosol Removal Effect by Pool Scrubbing", 22nd
DOE/NRC Nuclear Air Cleaning and Treatment Conference, Aug., 1992.
[7] R. S. Denning et al., "Radionuclide Release Calculations for Selected Severe Accident
Scenarios", report for the U.S. Nuclear Regulatory Commission, NUREG/CR-4624,
BMI-2139, Volumes I-V, July, 1986.
-131-
JAERI-Research 2005-021
Condensate
Environment
Storage Reactor Building -i
Tank Blowout
Containment Pannel
break
Leakage
Containmqrilj
Leak
Emergency
"Gas Treatment
System
t Containment
Venting System
RCIC: Reactor Core Isolation Cooling System, SRV: Safety Relief Valve,
ADS: Automatic Depressurization System, HPCS: High Pressure Core Spray System,
LPCS: Low Pressure Core Spray System, LPCI: Low Pressure Core Injection System
\
\
I
_ 1
\ \ 1
*
1
J r 1
0 500 1000 1500 2000 2500 3000 3500 4000
10"
10"° 10"" 10"' 10"' 10u
Time[min]
Release Fraction[-]
Fig.2 Source terms for core damage sequences calculated by THALES-2
Note: This figure summarizes information in Figs 5.2.1 and 5.2.2
in the main text.
132-
JAERI-Research 2005-021
0 200 400 600 800 1000 1200 1400 1600 1800 2000
T_me[m_n]
Fig. 5 Relative mass of Iodine in the plant
(Containment venting case: TQUV sequence)
-133-
This is a blank page.
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3
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9.80665 1 2.20462 n 0.0980665 1 0.967841 735.559 14.2233
4.44822 0.453592 1 0.101325 1.03323 1 760 14.6959
2 1 3
tt IS 1 Pa-s(N-s/m )=10P( .+:TX')(g.(cm-s)) 1.33322 x 10"' 1.35951 x 10" 1.31579 x 1 0 1 1.93368 xlO" 2
ftttS lm 2 /s=10 , St(x . - 7 x ) ( c m V s ) 6.89476 x 10"3 7.03070 x 10"2 6.80460 x 10"2 51.7149 1
St Bq Ci Gy rad C/kg R Sv
w 1 2.70270 x IO- II
*H 1 100 3876 1 100
M
4
3.7 x 10'° 1 0.01 1 2.58 x 10" 1 0.01 1
(86fp 12 fl 26BSffi)
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