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What is This?
Abstract
A multiscale modeling approach to analyze filament-wound composite pressure vessels is developed in this article. The
approach, which extends the Nguyen et al. [Prediction of the elastic-plastic stress/strain response for injection-molded
long-fiber thermoplastics. J Compos Mater 2009; 43: 217–246.] model developed for discontinuous fiber composites to
continuous fiber ones, spans three modeling scales. The microscale considers the unidirectional elastic fibers embedded
in an elastic–plastic matrix obeying the Ramberg–Osgood relation and J2 deformation theory of plasticity. The mesoscale
behavior representing the composite lamina is obtained through an incremental Mori–Tanaka [Average stress in matrix
and average elastic energy of materials with misfitting inclusions. Acta Metall 1973; 21: 571–574.] type model and the
Eshelby [The determination of the elastic field of an ellipsoidal inclusion and related problems. Proc R Soc Lond, Ser A 1957;
241: 376–396.] equivalent inclusion method. The implementation of the micro–meso constitutive relations in the
ABAQUSÕ finite element package (via user subroutines) allows the analysis of a filament-wound composite pressure
vessel (macroscale) to be performed. Failure of the composite lamina is predicted by a criterion that accounts for the
strengths of the fibers and of the matrix as well as of their interface. The developed approach is validated in the analysis
of an aluminum liner – T300 carbon/epoxy pressure vessel to predict the burst pressure. The predictions compare
favorably with the numerical and experimental results by Lifshitz and Dayan [Filament-wound pressure vessel with thick
metal liner. Compos Struct 1995; 32: 313–323]. The approach will be further demonstrated in the study of the effects of
the lamina thickness, helical angle, and fiber–matrix material combination on the burst pressure.
Keywords
Filament-wound composite, pressure vessel, multiscale modeling, elastic–plastic, micromechanical modeling, burst pres-
sure, failure
Figure 1. Schematic of the multiscale modeling approach used to analyze filament-wound composite pressure vessels.
with a macroscopic failure criterion.9–13 More recently, The structure of this article is as follows. After
a continuum damage mechanics approach has been ‘Introduction,’ ‘An elastic–plastic failure model for fila-
used by Liu and Zheng14 in a finite element formulation ment-wound composite pressure vessels’ describes the
to predict progressive damage due to different mechan- extension of the Nguyen et al.17 model to filament-
isms that lead to the bursting of a hydrogen storage would fiber composites by developing constitutive rela-
composite vessel. tions that use an incremental EMTA approach and a
In all the above models, the response of the composite failure criterion for filament-wound elastic–plastic com-
vessel is obtained from the constitutive behavior of the posites. Model validation is presented in ‘Results and
unidirectional (UD) composite lamina by means of the discussion’ where results of the current multiscale
classical lamination theory or a finite element method. model for a filament-wound composite are compared
The model developed in this article is different from the with the experimental results by Lifshitz and Dayan.6
current models for pressure vessels in its micro–macro The model is further demonstrated in this section by
approach (Figure 1). It accounts for the fiber and matrix studying the effects of the lamina thickness, helical
constituent properties to build the macroscopic response angles, and fiber–matrix material combination on the
by means of a multiscale modeling approach using an burst pressure. ‘Conclusions’ summarizes the features
incremental Eshelby–Mori–Tanaka (EMTA) homogen- of this multiscale model for analysis and design of fila-
ization method15,16 associated with a finite element for- ment-wound composite pressure vessels.
mulation.17,18 Indeed, our model extends the Nguyen
et al.17 model developed for discontinuous fiber compos- An elastic–plastic failure model for
ites to continuous fiber ones. It considers the elastic– filament-wound composite pressure
plastic behavior of the matrix material that obeys the
vessels
Ramberg–Osgood relation and J2 deformation theory
of plasticity under small strain assumption. Failure is This section describes the extension of the Nguyen
predicted by the Van Hattum–Bernardo19 model that et al.17 model developed for discontinuous fiber poly-
was adapted to the elastic–plastic fiber composite by mer composites processed by injection molding to fila-
Nguyen et al.17 This failure criterion incorporates the ment-wound composites that possess continuously
strengths of the fibers and the matrix as well as the inter- reinforcing fibers. Fiber length and orientation are
facial fiber–matrix strength. Thus, it explicitly accounts given in filament-wound composite laminates unlike
for the properties of the constituent materials that con- injection-molded fiber thermoplastics where the fiber
trol failure of the composite vessel. length and orientation distributions are entirely deter-
The link between this multiscale modeling approach mined by the injection molding process.
and the classical lamination approach resides in the
lamina behavior. In this approach, the lamina behavior
is built through a numerical homogenization based on
Constitutive relations
micromechanics and continuum mechanics, while in the Nguyen et al.17 applied an incremental EMTA to com-
classical lamination theory, it is given in advance based pute the elastic–plastic stress–strain response of a UD
on experimental measurement and simplified approxi- fiber composite. The fibers are assumed to be elastic
mations. Multiscale modeling presented in this article while the matrix is elastic–plastic and obeys the
offers an efficient way to obtain the lamina behavior in Ramberg–Osgood relation under small strain assump-
complex laminated composite structures such as fila- tion. For a filament-wound composite, the fiber aspect
ment-wound pressure vessels. ratio is extremely large (l=d ! 1Þ; the current stiffness
tensor of this composite according to the Mori–Tanaka induces the strain increments in the fiber and matrix
mean field approach is given by phases
1
with T ¼ ½I þ S : H1 m : ðHf Hm Þ , where S is the The overall strain increment and the strain incre-
Eshelby tensor and I the fourth-order identity tensor. ments in the fiber and matrix phases represent the
Assuming proportional loading, the Ramberg–Osgood volume average strain quantities at the scale of the
relation20 is used to describe the elastic–plastic behavior RVE. However, at the macroscale of the composite
of the matrix in terms of the total matrix equivalent vessel, they represent the local overall strain increment,
stress ( m ) and strain ("m ) and the local microscopic fiber strain and matrix strain
n increments, respectively. These concepts are equally
m 0 m applied to the corresponding stress quantities asso-
"m ¼ "em þ "pm ¼ þ ð3Þ
Em Em 0 ciated with the as-defined strain quantities.
Next, the matrix stress increment is then
where 0 and n are material coefficients and are defined computed by
as the reference stress and the power-law exponent. Em,
"em , and "pm are the matrix elastic modulus, equivalent ijm ¼ Hm m
ijkl "kl ð11Þ
elastic strain, and equivalent plastic strain, respectively.
The tangent elastic modulus of the matrix material where the matrix tangent stiffness, Hm
ijkl , is calculated by
determined from equation (3) is used to compute Hm equations (5) to (7) using the matrix tangent modulus
Etm given by equation (4). The computation of the
Em matrix stress increment allows the matrix stress to be
Etm ¼ ð4Þ
nEm updated, and therefore, the matrix equivalent stress can
1þ
kð"pm Þ1n=n be determined using the J2 deformation theory of
plasticity
where k ¼ ð1=hÞ1=n with h ¼ 01n =Em : The non-zero
rffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
components of the symmetric tangent stiffness tensor 3 0m 0m
Hm(Hm,ij ¼ Hm,ji ) for a general three-dimensional m ¼ ð12Þ
2 ij ij
stress state are given by
0
where ijm is the matrix deviatoric stress tensor. The
ð1 m ÞEtm computation of m allows the current matrix equivalent
Hm,11 ¼ Hm,22 ¼ Hm,33 ¼ ð5Þ
ð1 þ m Þð1 2m Þ strain and plastic strain to be determined using the
Ramberg–Osgood relation (3). These quantities are
m Etm saved to start the next increment of the loading process.
Hm,12 ¼ Hm,13 ¼ Hm,23 ¼ ð6Þ Finally, to update the overall stress of the composite at
ð1 þ m Þð1 2m Þ
the end of the current increment, the composite overall
Etm stress increment is computed by
Hm,44 ¼ Hm,55 ¼ Hm,66 ¼ ð7Þ
2ð1 þ m Þ
ij ¼ Hijkl "kl ð13Þ
where Etm is given by equation (4) and m the Poisson’s
ratio of the matrix material. For computational effi- where the tangent stiffness tensor of the composite Hijkl
ciency and stability of the algorithm, the variation of is determined by equation (1).
the Poisson’s ratio with the deformation state is neg-
lected. The elastic Poisson’s ratio is then used in equa-
Failure prediction
tions (5) to (7).
The overall strain increment e applied to the rep- At each load increment, failure is predicted using the
resentative volume element (RVE) of the composite Van Hattum–Bernardo19 model that was adapted to
plastic strain. The initial yield stress Y , hardening coef- Table 2. Constituent strengths for the UD T300/epoxy lamina
ficient H, and power-law exponent m of the 6061-T6
Strength (MPa)
material used in the computation are Y ¼168 MPa,
H ¼ 465 MPa, and m ¼ 0.26, respectively. T300 fibera 3530
The T300 carbon/epoxy overwrap has reinforcement Epoxy 83
consisting of helical and hoop winding, with the helical Fiber–matrix interface 48
angles of 20 between the fiber direction and the lon- a
gitudinal axis of the vessel. The experimental design has ToraycaÕ technical data sheet.
two helical units, each of 0.8 mm thickness, and the
hoop layers of 3.8 mm total thickness. The elastic prop- interfacial strength is assumed to be equal to the
erties of the T300/epoxy lamina given in Lifshitz and shear strength of the matrix material.
Dayan6 are the data for the homogenized lamina The finite element model for the analysis uses the
(mesoscale), and thus, cannot directly be used in our composite layered shell element of ABAQUS. The
micro–macro modeling approach that requires the internal pressure is applied incrementally, and the
properties for the fiber and matrix materials. action of the dome is replaced by an axial load distri-
Therefore, a kind of ‘reverse engineering’ is necessary bution at one end of the vessel equal to P R2in , where P
to obtain the constituents’ elastic properties. To do so, is the internal pressure and Rin the internal radius of the
some realistic guess values of the carbon fiber and liner. The shell element layup has four layers represent-
epoxy properties as well as of the fiber volume fraction ing the liner, the two helical units, and the hoop unit.
are used in the iterative EMTA elastic properties calcu- The layup is denoted by the layer thickness in milli-
lation. The predicted results are then compared to the meters and ordered as [4.5 0.8 0.8 3.8]. Figures 2 and
T300/epoxy lamina elastic properties given in Lifshitz 3 present the distributions of the failure criterion at the
and Dayan.6 If the agreement between the EMTA pre- onset of failure (corresponding to the applied pressure
dictions and the values in Lifshitz and Dayan6 is within of 83.5 MPa) in the helical and hoop layers, respect-
5%, the reverse engineering procedure stops, and the ively. Failure, as indicated by the value of the criterion
elastic properties of the constituents are then identified. greater than or equal to unity, is predicted to first occur
Table 1 presents the as-identified elastic properties for in the helical layers. Figure 3 shows that the hoop layer
the T300 carbon fiber and epoxy resin. In the same has approached failure at this pressure level (failure
table are also shown the predicted elastic properties criterion close to unity).
(engineering constants) for the T300/epoxy lamina, The predicted evolution of the internal pressure
which are in good agreement with the corresponding versus the laminate hoop strain is illustrated in
values used in Lifshitz and Dayan.6 The percentages Figure 4 that also presents the Lifshitz–Dayan6 experi-
of relative errors are very small and are given in the mental results. The experiment in Lifshitz–Dayan6
same table. Next, adopting the power-law exponent included an initial small gap between the liner and the
n ¼ 4 in the Ramberg–Osgood relation (3) for the composite laminate that resulted when the tank was
epoxy matrix,22 and considering a matrix strength cooled to room temperature. When the vessel was
value in the 80–85 MPa range, a reference stress, 0, loaded for the first time, all the load was supported
of 90 MPa and matrix failure strain of 3.15% are by the liner until the gap was closed. This explains a
obtained for the epoxy material used in the analysis. small but non-zero value of the experimental pressure
Table 2 presents the constituent material strengths in Figure 4 before the composite layers start to deform.
used in the failure criterion (11). The fiber–matrix The prediction has neglected this initial condition and
Figure 2. Contour of the failure criterion value in a helical layer at the onset of failure (corresponding to the applied pressure of 83.5
MPa).
Figure 3. Contour of the failure criterion value in the hoop layer at the onset of failure (corresponding to the applied pressure of
83.5 MPa).
Figure 4. Predicted and experimental pressure vs. hoop strain Figure 5. Predicted liner’s equivalent Mises stress vs. applied
for an aluminum liner - T300 carbon/epoxy pressure vessel: The pressure for the studied aluminum liner - T300 carbon/epoxy
experimental results were extracted from the experimental pressure vessel.
curve reported in Lifshitz and Dayan.6
therefore has assumed that the liner and composite different layers to be closely monitored, and thus, the
layers deform at the same time. This assumption only model offers an efficient way to optimize the compos-
has a minor effect on the predicted pressure versus the ite layup to maximize the burst pressure. The vessel
laminate hoop strain and burst pressure shown in that was built and reported in Lifshitz and Dayan6
Figure 4, which indicates a good agreement between has the liner–helical–hoop layer structure [4.5 0.8 0.8
the predicted and experimental results. The predicted 3.8]. This parametric study keeps the total thickness
results based on the two different finite element meshes and thickness of the liner constant but varies the
(Mesh 1 with 7650 elements and Mesh 2, 30,780 elem- thickness of the helical and hoop layers. The follow-
ents) are practically identical. This indicates that Mesh ing layups are then analyzed in addition to the experi-
1 already has the adequate number of elements used. mental one: [4.5 0.4 0.4 4.6], [4.5 0.6 0.6 4.2], [4.5 1.2
The predicted burst pressure is 84 MPa while the experi- 1.2 3], and [4.5 1 1 3.4]. The experimental layup is used
mental value reported in Lifshitz and Dayan6 was as the reference.
860 atm (87 MPa). The results from the simulations are reported in
Figure 5 presents the evolution of equivalent stress Figure 6 that generally shows a significant effect of
in the liner with the applied pressure. The plastic flow in the hoop-to-helical thickness ratio on the burst pres-
the liner allows the pressure to be increased from sure. Figure 6 shows that increasing the thickness of
30 MPa to the burst pressure of 84 MPa with small the helical units from 0.8 to 1.2 mm (decreasing the
increases in the liner equivalent stress. The sudden hoop layer thickness from 3.8 to 3 mm) has a modest
increase in the liner equivalent stress when the internal effect on the burst pressure. The [4.5 1 1 3.4] layup
pressure has exceeded 84 MPa is caused by the total achieves the maximum burst pressure (87 MPa);
failure of the composite layers. however, increasing the thickness of each helical unit
to 1.2 mm and decreasing the hoop layer thickness to
The effect of hoop-to-helical thickness ratio on the 3 mm practically does not affect the burst pressure. On
the other hand, decreasing the thickness of the helical
burst pressure units from 0.8 to 0.4 mm has significantly reduced the
This section applies the developed multiscale model to burst pressure. The [4.5 0.4 0.4 4.6] vessel has the
perform a parametric study to determine the effect of lowest burst pressure (67.5 MPa). These findings
hoop-to-helical thickness ratio on the burst pressure. agree with the numerical results in Lifshitz and
A similar study was conducted in Lifshitz and Dayan.6
Dayan;6 however, the application of the present To understand the reason for the reduction of the
model allows the evolution of the failure criterion in burst pressure with the reduction of the helical layer
Figure 6. Predicted effect of hoop-to-helical thickness ratio on Figure 8. Predicted matrix equivalent stress vs. applied pres-
the burst pressure for a 4.5-mm thick aluminum liner - T300 sure in the [4.5 0.8 0.8 3.8] (reference vessel) and [4.5 0.4 0.4 4.6]
carbon/epoxy pressure vessel. vessels.
Figure 10. The matrix stress components vs. applied pressure Figure 12. Effect of fiber-matrix material combination on the
in the [4.5 0.4 0.4 4.6] vessel. burst pressure.
helical angles with respect to the reference case (ana- by the same amount decreases the burst pressure by
lyzed in the previous section) are allowed to investigate about 3%.
the effect of helical angles on the tank burst pressure.
The reference vessel presents the helical layers oriented
at 20 . From these values, the helical angles of 15
and 25 are considered in this study. Figure 11 shows
The effect of fiber–matrix material combination
the analysis results in terms of the tank pressure versus It has been observed in the previous analyses (Figure 8)
hoop strain. More alignment of the helical layer orien- that when the failure criterion is verified at a given
tation in the axial direction by 5 does practically not pressure, the equivalent stress in the epoxy matrix is
affect the burst pressure, while more deviation of the close to the matrix strength (83 MPa). This would sug-
orientation of these layers from the axial direction gest that using a stiffer and stronger epoxy matrix
would lead to higher burst pressure. To investigate the criterion. Although the use of the current failure criter-
effect of fiber–matrix material combination, this section ion is practical and sufficiently accurate, damage and
considers a significantly stiffer and stronger epoxy failure predictions of filament-wound composite vessels
material having 5 GPa elastic modulus and 90 MPa can be improved by expanding this multiscale modeling
strength. The other parameters (reference stress and approach to incorporate progressive damage mechan-
power-law exponent) of the Ramberg–Osgood relation isms in a local or non-local formulation using con-
are kept constant. The effect of fiber–matrix material tinuum damage mechanics.
combination is presented in Figure 12 that shows a sig-
nificant increase of the burst pressure by the use of a
Funding
stiffer and stronger epoxy (Epoxy 2) compared to the
reference vessel that used the actual epoxy (Epoxy 1). The development of EMTA-NLA was funded by the United
States Department of Energy’s (US DOE) Office of Vehicle
The increase in burst pressure obtained is about 4.8%.
Technologies (Dr Carol Schutte, Team Lead for Materials
Technology). The application of EMTA-NLA to filament-
wound composite pressure vessels has been supported by
the US DOE’s Office of Fuel Cells Technologies (Dr Ned
Conclusions Stetson, Technology Development Manager).
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