Professional Documents
Culture Documents
net/publication/359272079
CITATION READS
1 202
2 authors:
Some of the authors of this publication are also working on these related projects:
All content following this page was uploaded by Taco D. Visser on 03 September 2022.
Contents
1. Introduction 275
2. Life and work of Thomas Young 277
3. Young’s interference experiment 286
4. Weak light 289
5. The wave-particle duality for massive particles 296
6. Optical coherence 304
7. Surface plasmons 314
8. Entanglement and duality 324
9. Multi-order interference and exotic paths 327
10. Singular optics 331
11. Conclusions 337
Acknowledgments 337
References 337
1. Introduction
The experiment that is the subject of this review has been referred to as
“the two-pinhole experiment” or “the double-slit experiment” (Young
himself referred to it as both). It has had a tremendous influence on the his-
tory of science, and it continues to inspire and direct modern researchers to
use it, and its modifications, to probe new areas of physics. In this article we
explore the history of Young’s experiment, its implications, and those
discoveries and experiments that have followed in its wake, even up to
the present day.
fencing and dancing. After continuing his education in the German city of
G€ottingen, he obtained the title of Doctor of Physic, Surgery and
Midwifery. But in order to fulfill his plan of practicing medicine in
London, he was required to spend more time at an English university. He thus
went to Cambridge where, in reaction to his wide-ranging knowledge and
talents, his fellow students nicknamed him “phenomenon Young.” In order
to graduate, Young had to publicly subscribe to the Thirty-Nine Articles, the
foundational statement of the established Church of England. This meant a
formal separation from Young’s upbringing as a Quaker.
After completing his studies he moved to London in 1800 to set up a med-
ical practice there. However, Young turned out to be unpopular as a practical
physician. One of his biographers suggests that this may have been due to a
lack of bedside manner (Peacock, 1855a). In any case, he soon changed his
career by accepting a position as Professor of Natural Philosophy in the
Royal Institution in London. The Institution had been recently founded,
in 1799, with the aim to provide access to scientific and technical knowledge
to a lay audience and to promote its practical application. Young was tasked
with giving lectures and demonstrations on a wide range of topics.
It was at the Institution that Young began pondering the possibility of
light being a wave phenomenon. This was a rather radical thought as, nearly
100 years earlier, Newton had seemingly proven that light consists of a
stream of particles. As he had written in his Opticks (Newton, 1704):
The waves on the surface of stagnating water, passing by the sides of a broad
obstacle which stops part of them, bend afterwards and dilate themselves
gradually into the quiet water behind the obstacle. The waves, pulses or vibra-
tions of the air, wherein sounds consist, bend manifestly, though not as much
as the waves of water. For a bell or a cannon may be heard beyond a hill which
interrupts the sight of the sounding body, and sounds are propagated as read-
ily through crooked pipes as straight ones. But light is never known to follow
crooked passages nor to bend into the shadow. For the fixed stars, by the inter-
position of any of the planets, cease to be seen. And so do the parts of the Sun
by the interposition of the Moon, Mercury or Venus.
Young was, of course, very much aware of the weight of Newton’s words
and knew that his results would face a highly critical reception. He hence
began his report very deferentially (Young, 1800):
Young’s interference experiment 279
Ever since the publication of Sir Isaac Newton’s incomparable writings, his doc-
trines of the emanation of particles of light from lucid substances, and of the
formal pre-existence of coloured rays in white light, have been almost univer-
sally admitted in this country, and but little opposed in others.
But he then proceeds to point out a remarkable analogy between light and
acoustic phenomena, effectively using Newton’s own observations against
him:
The phenomena of the colours of thin plates require, in the Newtonian system,
a very complicated supposition, of an ether, anticipating by its motion the
velocity of the corpuscles of light, and thus producing the fits of transmission
and reflection; and even this supposition does not much assist the explanation.
It appears, from the accurate analysis of the phenomena which Newton has
given, and which has by no means been superseded by any later observations,
that the same color recurs whenever the thickness answers to the terms of an
arithmetical progression. Now this is precisely similar to the production of the
same sound, by means of an uniform blast, from organ-pipes which are differ-
ent multiples of the same length.
It was this analogy, between what we nowadays call Newton rings and stand-
ing acoustic waves, that first made Young doubt the corpuscular theory of
light. By assuming that light is indeed a wave phenomenon, and knowing
the speed of light, as first measured in the 17th century by the Danish astron-
omer Ole Rømer, Young went on to determine the wavelength of different
colors from the location of Newton rings produced by thin plates
(Young, 1802b).
By challenging the established particle theory of light, Young was able to
make a number of important discoveries. One major contribution was his sug-
gestion that light undergoes a phase jump when it is reflected from a medium
denser than that in which it is traveling. In Young (1802a) he describes an
experiment in which the refractive index of the medium underneath a thin
plate is varied, and the resulting change in the fringe pattern clearly demon-
strates that such a jump indeed occurs. His next major step toward a convinc-
ing wave theory of light was the recognition, in 1801, of the principle of
interference. As he would recall a few years later (Young, 1804b):
It was in May 1801 that I discovered, by reflecting on the beautiful experiments
of Newton, a law which appears to me to account for a greater variety of inter-
esting phenomena than any other optical principle that has yet been made
known. I shall endeavour to explain this law by a comparison. Suppose a num-
ber of equal waves of water to move upon the surface of a stagnant lake, with a
certain constant velocity, and to enter a narrow channel leading out of the lake.
Suppose then another similar cause to have excited another equal series of
280 Greg Gbur and Taco D. Visser
waves, which arrive at the same channel, with the same velocity, and at the
same time with the first. Neither series of waves will destroy the other, but their
effects will be combined: if they enter the channel in such a manner that the
elevations of one series coincide with those of the other, they must together
produce a series of greater joint elevations; but if the elevations of one series are
so situated as to correspond to the depressions of the other, they must exactly
fill up those depressions, and the surface of the water must remain smooth; at
least I can discover no alternative, either from theory or from experiment. Now, I
maintain that similar effects take place whenever two portions of light are thus
mixed; and this I call the general law of the interference of light.
This advice was not particularly well heeded, to say the least, and an anon-
ymous ad hominem campaign was launched in the Edinburgh Review
(Brougham, 1803). It later turned out that it was Henry Peter Brougham
(an ardent disciple of Newton, who would be made a Fellow of the
Royal Society in 1803) who wrote
As this paper contains nothing which deserves the name, either of experiment
or discovery, and as it is in fact destitute of every species of merit, we should
have allowed it to pass among the multitude of those articles which must
always find admittance into the collections of a Society which is pledged to
publish two or three volumes every year.
and
…it teaches no truth, reconciles no contradictions, arranges no anomalous
facts, suggests no new experiments and leads to new inquiries. It has not even
the pitiful merit of affording an agreeable play to the fancy.
Indeed, after the extremely hostile reception of his wave theory, Young
turned away from optical research for several years. He also gave up his
282 Greg Gbur and Taco D. Visser
position of Professor because his lectures at the Royal Institution were not
very popular. As he would later write about himself (Hilts, 1978),
…his compressed and laconic style being more adapted for the study of a man
of science than for the amusement of a lady of fashion.
This remark was also a jab at his colleague Humphry Davy, who excelled at
entertaining precisely such ladies in the Royal Institution’s audience. As
Young had earned a large inheritance from his supportive uncle, he could
afford to live without a salaried position.
Ironically, even though today the results of Young’s experiment are
often presented as a classical example of a paradigm shift, it was the doubts
of the prominent French scientist Simeon Denis Poisson that led to their
acceptance. Poisson noticed that a consequence of the wave theory, as for-
mulated in mathematical terms by Auguste Fresnel, would be the existence
of a bright spot at the center of the shadow of a circular obstacle. Since this
had never been observed, Poisson thought that this disproved the theory of
Young and Fresnel. François Arago, however, took up the experimental chal-
lenge and in 1818 succeeded in observing the predicted effect (Arago, 1819),
which is now referred to as the Poisson-Arago spot. The wave nature of light
only became widely accepted after Arago published his results confirming
Fresnel’s work.
Despite his professional setbacks, Young did not remain idle. After his
resignation, he spent the next 5 years compiling the 60 lectures he gave dur-
ing his 2-year tenure, and he oversaw their publication under the title
A Course of Lectures on Natural Philosophy and the Mechanical Arts (Young,
1845). This magnum opus, which greatly resembles an encyclopedia, covers
an enormous range of subjects. In Part I the laws of mechanics, the history
of writing techniques, the theory of perspective, the design of bridges, and
various “timekeepers,” i.e., clocks and watches, are among the many topics
that are described in great detail. In Lecture XIII, entitled On passive strength
and friction, Young introduced a measure of elasticity which is still widely
used and today is called Young’s modulus. Part II of his course is concerned
with fluids and treats capillary action, surface tension, contact angles, and
hydraulic machines. It also deals with sound and musical instruments.
Most significantly, it contains some of his aforementioned work on optics.
In this volume Young also introduced the most familiar version of his
famed experiment, using “two very small holes or slits.” Part III deals
with astronomy, the solar system, gravitation, geography, and the tides.
Young’s interference experiment 283
Their discoveries were not at odds with Young’s undulatory theory, but they
could also not be readily explained by it. All this changed in 1816 when Arago
and Gay–Lussac visited Young at his home. The discussion turned to the
recent work by Fresnel by which Young was less than impressed, claiming
that he himself had already done similar work. The visitors did not agree,
and Arago offers us a rare glimpse into Young’s marriage (Arago, 1835):
…Mrs Young rose up suddenly and left the room. We immediately offered our
most urgent apologies to her husband, when Mrs Young returned, with an
enormous quarto under her arm. It was the first volume of the Natural
Philosophy [i.e., Young’s collected lectures] . She placed it on the table, opened
it up without saying a word, at page 787, and pointed with her finger to a
figure where the curved lines of the diffracted bands, on which the discussion
turned, appeared theoretically established. a
During the same visit Arago also described his own experiments in which,
using a two-slit setup, he had found the surprising result that rays of light
polarized in orthogonal planes will not interfere with each other (Arago,
1819; Arago & Fresnel, 1819). This set Young on an entirely new path
of thinking. A few months later he wrote to Arago (Peacock, 1855b) that
his result could be explained by assuming that light waves do not behave
as “the undulations of sound, consisting simply of the direct and retrograde motions
of their particles in the direction of their radius …,” but rather as “a transverse vibra-
tion, …and this is polarization.”
The suggestion that light is a transverse rather than a longitudinal wave
greatly propelled physical optics. It not only explained Arago’s observations,
but it also offered a direct way to derive Malus’ law. It also opened up the
analysis of crystalline structures in terms that present-day readers would be
familiar with, by assuming a refractive index that depends on the plane of
polarization.
Even as he grew older, Young continued to find new topics to research,
and new problems to solve. In England of the Industrial Revolution, mor-
tality rates in the countryside were significantly lower than those in the
crowded cities. Moreover, these rates were changing quickly due to
improved sanitation, the introduction of vaccination, and better access to
clean drinking water. These circumstances made it very difficult for insur-
ance companies to estimate the costs of annuities. In 1824 the Palladium
Insurance Company enlisted Young’s help and appointed him to the
a
The authors first learned of this story from the late Emil Wolf. After telling it he cried out “What a
woman!”
Young’s interference experiment 285
While completing his work on an Egyptian dictionary, the last day of this
most remarkable man came in 1829 when, after a brief illness, he died in
London at the age of 55. A postmortem examination showed extensive
hardening of the aorta. His friend and biographer Hudson Gurney 1831
put this down to Young’s “unwearied and incessant labor of the mind from the
earliest days of infancy.”
François Arago read a eulogy to the French Academie des Sciences, of
which Young was a foreign member. In it Arago referred to Young’s work
on interference as (Arago, 1835)
…that fine discovery which will render his name imperishable…
In the last part of the eulogy Arago laments the hostile reception of Young’s
ideas and describes how discouraging that must have been for him. Noting
that an initial rejection had been the unfortunate fate of many great scientists
who were later vindicated, he ends poetically with this comforting
suggestion:
Let us try to persuade ourselves that in the dungeons of the inquisitors a
friendly voice had caused Galileo to hear some of the delightful expressions
which posterity has kept sacred for his memory.
286 Greg Gbur and Taco D. Visser
Five years after Young’s death a white marble tablet, with a profile medal-
lion, was revealed in the chapel of St Andrew in Westminster Abbey. The
inscription reads:
Sacred to the memory of Thomas Young M.D. Fellow and Foreign Secretary
of the Royal Society Member of the National Institute of France. A man alike
eminent in almost every department of human learning. Who, equally distin-
guished in the most abstruse investigations of letters and of science, first
established the undulatory theory of light and first penetrated the obscurity
which had veiled for ages the hieroglyphicks of Egypt. Endeared to his friends
by his domestic virtues, honoured by the World for his unrivalled acquirements,
he died in the hopes of the Resurrection of the just. Born at Milverton in
Somersetshire June 13th 1773, died in Park Square London May 10th 1829, in
the 56th year of his age.
P
R1
r1
R2
d z
r2
fringes
incident plane wave
screen A screen B
Fig. 1 The geometry of Young’s interference experiment with two pinholes. A mono-
chromatic plane wave is normally incident on screen A that contains two identical pin-
holes. An interference pattern is formed on a second, parallel screen B. For simplicity it is
assumed that the refractive index in between the two screens is unity.
We can simplify this expression by making two assumptions. First, when the
separation Δz between the two screens is much larger than the distance
d between the two pinholes, as is usually the case, then for a point
P close to the z axis we have to a good approximation that
288 Greg Gbur and Taco D. Visser
jK 1 j2 jK 2 j2 K 1 K *2 ¼ K 2 : (5)
Second, we assume that the spectral density of the incident field at the two
pinholes is the same. Since we are dealing with a plane wave, that implies that
4. Weak light
Though Young’s experiment is perhaps most famous for demonstrat-
ing the wave properties of light, it has also played a crucial role in elucidating
the quantum mechanical wave-particle duality of photons and matter.
As the 19th century drew to a close, it seemed that the wave theory of
light was on very solid footing, especially with the recognition of light as an
290 Greg Gbur and Taco D. Visser
Thomson’s model was not particularly well-formed, but the natural impli-
cation of it is that the interference pattern produced in Young’s experiment
comes from the interaction of many of these little pulses of energy. But what
happens when only a very small number of them are interacting with the
two pinholes at a given time? Thomson suggested that the interference pat-
tern must look very different, because there simply are not enough bumps
around to interfere.
The first attempt to explore this question experimentally was through the
use of Young’s experiment again, and was undertaken by Thomson’s student
Taylor. In his “Interference fringes with feeble light” (Taylor, 1909) he
describes the creation of a low intensity source by having a gas flame illumi-
nating a narrow slit and then placing smoked glass screens in the path of the
emanating light. Each individual screen would absorb a significant fraction of
light passing through them, and screens which were more heavily smoked
would absorb significantly more light than those less smoked. By using mul-
tiple screens, an arbitrarily high amount of attenuation could be achieved,
even to the level where only single photons were illuminating a sewing nee-
dle, acting as the Young apparatus, at any time. A photographic image was
taken of the ensuing diffraction pattern.
For the experiment Taylor took five images of these patterns, for various
screens placed behind the slit. He calibrated his experiment first by taking
292 Greg Gbur and Taco D. Visser
photographs of the light source without any screens present, and determined
how much time was needed for the plates to darken by the same amount;
repeating this experiment with the screens present, then, one could see
how Young’s interference pattern changed when the light intensity was
reduced to the level where a only small number of energy “pulses” were
going through at once.
The experiment required quite a lot of patience. In order to get sufficient
development of the photograph of the dimmest light source, Taylor had to
run the exposure for 3 months. But his patience paid off, and he found an
unexpected result; in his own words
In no case was there any diminution in the sharpness of the pattern although
the plates did not all reach the standard blackness of the first photograph.
In other words, the interference pattern remained the same, no matter how
much the light intensity was reduced. Taylor and Thomson seem to have
initially interpreted this result as indicating that they had not used a dim
enough light source, and they estimated the maximum energy of a single
photon from their arrangement. Their estimate, based on an incorrect model
of quantum physics, ended up being much smaller than the true energy of a
photon.
What happens when we ensure that, on average, just a single photon is
present in the setup? It turns out that although the photons are detected as
individual particles that arrive at seemingly random positions on the detector
area, they travel like waves. The latter conclusion follows from two facts: if
one sums over a large number of detection events, the grainy distribution
gradually becomes smoother and eventually evolves into the classical inter-
ference pattern as first observed by Young. Also, if one of the two apertures
is closed and each photon is forced to pass through the other aperture, the
interference pattern does not emerge. In the words of Feynman, Leighton,
and Sands (1963), this is
a phenomenon which is impossible, absolutely impossible, to explain in any
classical way, and which has in it the heart of quantum mechanics.
Fig. 2 The transition from particles to waves visualized. Detection of light diffracted by
a double slit on a photon-by-photon basis using a CCD camera. A single frame shows
an apparently random distribution of photon impact points. Their integration reveals
the classical fringe pattern. Reproduced from Dimitrova, T.L., & Weis, A. (2008). The
wave-particle duality of light: A demonstration experiment. American Journal of Physics,
76(2), 137–142, with the permission of the American Association of Physics Teachers.
294 Greg Gbur and Taco D. Visser
attenuator MZI
stack beam
blocker oscilloscope
1 M
A
2 loud-
laser pointer BS speaker
trigger
A
B
lens PM
M
screen (P1)
BS lens PD
PZT
screen (P2)
lock
PI
off
scan
ramp generator
Fig. 3 Setup for the simultaneous demonstration of the wave and particle nature of
light. The strong beam is indicated by solid lines, the weak beam by dashed lines.
BS, beam splitter; M, mirror; PM, photomultiplier; PD, photodiode; PI, feedback amplifier.
Reproduced from Dimitrova, T.L., & Weis, A. (2008). The wave-particle duality of light: A
demonstration experiment. American Journal of Physics, 76(2), 137–142, with the permis-
sion of the American Association of Physics Teachers.
photomultiplier
single sweep
4 averages
16 averages
64 averages
128 averages
A photodiode
B
PM
pi B
ez PD
o
Fig. 4 Simultaneous demonstration of the wave and particle aspects of light. The bot-
tom trace shows the wave-like intensity distribution recorded by the photodiode. The
top trace shows the photon counts of the photomultiplier. By averaging many traces,
the signal from the photomultiplier gradually becomes smoother and approaches that
of the photodiode. Reproduced from Dimitrova, T. L., & Weis, A. (2008). The wave-particle
duality of light: A demonstration experiment. American Journal of Physics, 76(2), 137–142,
with the permission of the American Association of Physics Teachers.
Because the interference was between light beams from independent lasers,
the result seemed to imply that, contrary to Dirac’s view, different photons
can interfere with each other. This was not the end of the investigation,
however. In 1967, Pfleegor and Mandel repeated the experiment with single
photons (Pfleegor & Mandel, 1967). Even though only one photon was pre-
sent in the apparatus at any time with high probability, with the source of the
photon unknown, the interference pattern could still be created. They
concluded
Surprising as it might seem, the statement of Dirac quoted in the introduction
appears to be as appropriate in the context of this experiment as under the
more usual conditions of interferometry.
hν ¼ mc 2 : (17)
Here h denotes Planck’s constant, and c is the speed of light. The first con-
firmation of de Broglie’s conjecture was obtained by Davisson and Germer
in 1927 (Davisson & Gerner, 1927). In their experiments a beam of electrons
was scattered off a Ni crystal. It was known that a plot of the intensity of
X-rays reflected by a crystal in a fixed direction as a function of 1/λ should
show a series of equally spaced peaks. Each peak corresponds to a solution of
the Bragg condition for constructive interference. Davisson and Germer
found that the intensity of reflected electrons, as a function of the root of
their bombarding potential (i.e., their speed), shows a quite similar behavior.
This result indicated that the electrons are indeed wavelike, with a wave-
length, in agreement with Eq. (17), that is inversely proportional to their
velocity.
In the same year, the wave nature of electrons was verified independently
by G.P. Thomson and A. Reid (Thomson & Reid, 1927). G.P. Thomson
was the son of J.J. Thomson, the man who discovered the electron in 1897:
in essence, the father proved the particle properties of the electron, and the
son proved the wave properties of the electron. Passing a narrow beam of
electrons through a thin celluloid film and using a photographic plate as a
detector, Thomson and Reid observed a central spot (formed by undeflected
electrons) surrounded by a series of concentric rings. This clearly demon-
strated electron diffraction.
298 Greg Gbur and Taco D. Visser
The same group later showed the wave character of C70 molecules with a
wavelength of 2 to 5 pm (Brezger et al., 2002). Exploring the wave-particle
duality for even larger molecules could in principle be done at lower tem-
peratures, thereby reducing the molecules’ speed and increasing their de
Broglie wavelength (Arnd, Aspelmeyer, & Zeilinger, 2002). It has even been
suggested that one day the wave character of bacteria and viruses might be
demonstrated (Geyer et al., 2016). In an impressive technical feat, a beam
consisting of a mixture of high-mass (>10,000 atomic mass units) molecular
compounds was studied in Fein et al. (2019). Using a mass spectrometer to
separate different kinds of molecules, the wave nature of molecules con-
sisting of 810 atoms, with a total of some 5000 protons, neutrons, and elec-
trons, was observed. The internal complexity, the number of vibrational
modes, and also the internal energy of each of these particles clearly distin-
guish them from the much simpler quantum objects that were used in earlier
matter wave experiments. In a follow-up study (Eibenberger, Gerlich,
Arndt, Mayor, & T€ uxen, 2019) molecules with a mass of 25,000 amu, con-
sisting of up to 2000 atoms, were shown to have a de Broglie wavelength of
53 fm, i.e., five orders of magnitude smaller than the diameter of the mol-
ecules themselves.
An intriguing version of the double-slit experiment on a molecular scale
was reported in Zhou, Perreault, Mukherjee, and Zare (2021). Deuterium
(D2) molecules were prepared in a quantum superposition of two orthogo-
nal orientations. When helium atoms scatter off such molecules, they expe-
rience both orientations at once. As a result, the scattered intensity is due to a
coherent sum of two processes. Whereas in the classic double-slit experi-
ment the particles pass through both slits in a superposition of trajectories,
here, in contrast, one might think of the D2 molecules as a single slit that
itself is in a superposition of positions. The observed angular scattering
counts were in good agreement with the theoretical prediction.
302 Greg Gbur and Taco D. Visser
D1
Path 2
mirror
D2
BSout
Single-photon
input pulse
BSin Path 1 Φ
mirror
Fig. 6 Sketch of Wheeler’s delayed-choice experiment. The moveable mirror in Path 1
introduces a variable phase difference Φ between the two arms. The second beam split-
ter, BSout, can either be present or absent from the setup.
Young’s interference experiment 303
Fig. 7 Results of the delayed-choice experiment. (A) when the beam splitter BSout is pre-
sent, the photon counts of D1 (blue) and D2 (red) vary harmonically with the phase dif-
ference Φ. When the beamsplitter BSout is not present, no interference is observed and
an equal probability of detection at the two detectors is measured. Reproduced from
Jacques, V., et al., (2007). Experimental realization of Wheeler’s delayed-choice Gedanken
experiment. Science, 315, 966–968.
6. Optical coherence
Though optical science often applies simple models of monochro-
matic planar light waves to explain physical phenomena, all real sources
of light possess inherent random fluctuations. This randomness has observ-
able effects on the behavior of emitted light, affecting the spectrum, polar-
ization, directionality, and interference-causing capabilities of the light
wave. Optical coherence theory was developed to characterize the random-
ness of light and its effects on the measurable behavior of light, and also use
that randomness to improve existing optical applications and develop new
ones (Korotkova & Gbur, 2020). Young’s experiment has played a pivotal
role in understanding and measuring optical coherence properties.
Young’s interference experiment 305
The first person to ponder the subject of optical coherence was the
mile Verdet. As he notes in his textbook (Verdet, 1869)
French scientist E
…interfering rays always have a common source: this is a necessary condition
because with two distinct radiating sources the interference fringes disappear
completely.
Although Verdet did not use the term, one would nowadays say that is due
to the fact that the two sources are uncorrelated. He then goes on to explain
that the superposition, at a particular frequency, of two completely unrelated
point sources (“molecules”) radiating with the same amplitude will vary rap-
idly between constructive and destructive interference. On average the
superposition will have the value between that of a bright fringe and a dark
fringe. Furthermore, he argues that there exists a duration of time and a spa-
tial area over which the light emitted by the two sources may be considered
to vibrate in unison. It is the concordance of these vibrations that is necessary
to produce interference fringes. All these considerations make Verdet the
founding father of optical coherence theory. The random changes of phase
and amplitude that occur in optical wavefields play out at such short time-
scales that they cannot be observed directly. Even an ultra-fast detector pro-
vides only a time-averaged value of these quantities. One of the attractive
points of coherence theory, as we shall see, is that it is formulated in terms
of observable quantities that can be determined with the help of Young’s
experiment.
In the modern approach, as formulated by Wolf, the statistical properties
of a stochastic wavefield are characterized by correlation functions (Wolf,
2007b). If the field is stationary, at least in the wide sense, then its temporal
correlations at two moments t1 and t2 depend only on the time difference
τ ¼ t2 t1. For such a field, represented by an analytic signal V (r, t)
(Mandel & Wolf, 1995), its mutual coherence function is defined as
Here the angular brackets indicate a time average. The average intensity at a
position r is defined as the mutual coherence function evaluated at τ ¼ 0, i.e.,
A normalized version of Γ(r1, r2, τ), called the complex degree of coherence,
is obtained by defining
306 Greg Gbur and Taco D. Visser
Γðr1 , r2 , τÞ
γðr1 , r2 , τÞ ¼ : (21)
½Iðr1 ÞIðr2 Þ1=2
It can be shown that this function is bounded, namely
It can be shown (Mandel & Wolf, 1995) that W(r1, r2, ω) can also be rep-
resented as a correlation function. More specifically,
W ðr1 , r2 , ωÞ
μðr1 , r2 , ωÞ ¼ : (26)
½Sðr1 , ωÞSðr2 , ωÞ1=2
Just like the complex degree of coherence, the magnitude of this quantity is
bounded. One finds that
jK 1 j2 jK 2 j2 jK 1 K 2 j ¼ K 2 : (32)
308 Greg Gbur and Taco D. Visser
g:
IðPÞ ¼ 2jKj2 I f1 + jγðr1 , r2 , τÞj cos ½a12 ðτÞ ωτ (36)
It follows from general considerations of the analytic signal representation
of narrow-band signals (Mandel & Wolf, 1995) that in Eq. (36) both
jγðr1 , r2 , τÞj and a12(τ) vary much slower with τ than the term cos ðωτÞ.
From Eq. (9) we have that
R1 R 2 xd
τ¼ ¼ : (37)
c cΔz
Hence, moving the observation point P along the x direction (i.e., the ver-
tical direction in Fig. 1) results in a change of the time delay τ that is pro-
portional to the displacement of P. This means that the intensity near the
observation point consists of a constant background (the first term within
the curly brackets of Eq. (36)) with a cosine-like term superposed. Thus
the maximum and minimum intensity in the vicinity of P are given by
I max I min
V≡ ¼ jγðr1 , r2 , τÞj: (40)
I max + I min
Eq. (40) states that, unlike the optical field itself that oscillates too rapidly to
be observed, the modulus of the complex degree of coherence can be
directly established from intensity measurements in Young’s experiment.
From the bounds of jγðr1 , r2 , τÞj , given by Eq. (22), it follows that the
visibility can only attain its maximum value of unity when the field at the
two pinholes is fully coherent. This is illustrated in Fig. 8 where the normal-
ized intensity is plotted as a function of position x of the point of observation
for three different values of the modulus of the complex degree of coher-
ence. Complete destructive and constructive interference, i.e., V ¼ 1, occurs
when jγðr1 ,r2 ,τÞj ¼ 1(green curve). The other extreme, V ¼ 0, correspond-
ing to uncorrelated light with jγðr1 , r2 , τÞj ¼ 0 , gives rise to a constant
intensity distribution (red curve). An example of partially coherent light,
with jγðr1 , r2 , τÞj ¼ 0:5, is given by the dashed blue curve.
The phase of the complex degree of coherence can be determined by
comparing the fringe pattern with the fringes that are produced when the
two pinholes are illuminated by fully coherent and cophasal light, i.e., with
γ(r1, r2, τ) ¼ 1. This procedure is outlined in Section 10.4.1 of Born and
Wolf (1999).
I(x)
x [a.u]
Fig. 8 The normalized intensity pattern that is formed in Young’s experiment for three
selected values of the modulus of the complex degree of coherence. Green curve:
jγðr1 , r2 , τÞj ¼ 1, dashed blue curve: jγðr1 , r2 , τÞj ¼ 0:5, and red curve: jγðr1 , r2 , τÞj ¼ 0.
310 Greg Gbur and Taco D. Visser
P
F1 R1
r1
R2
d z
r2
F2
fringes
incident partially
coherent wave
screen A screen B
Fig. 9 Young’s interference experiment with the pinholes covered by two identical
narrow-band frequency filters F1 and F2.
In the often-encountered situation that the spectral densities at the two pin-
holes are the same, i.e.,
Sðr1 , ωÞ ¼ Sðr2 , ωÞ ¼ SðωÞ, (44)
and again making the assumption described by Eq. (32), we find that
n o
SðP, ωÞ ¼ 2K 2 SðωÞ 1 + Re μðr1 , r2 , ωÞei½kðR1 R2 Þ (45)
¼ 2K 2 SðωÞf1 + jμðr1 , r2 , ωÞj cos ½kðR1 R2 Þ +δg, (46)
where
δ ¼ arg½μðr1 , r2 , ωÞ: (47)
Young’s interference experiment 311
Two of the roots of this equation are μ0 ¼ 1; the third root is μ0 ¼ 1/2.
This theoretical prediction was soon verified using both acoustics
(Basano & Ottonello, 2005) and visible light (Ambrosini, Gori, &
Paoletti, 2005). More recent work has studied the problem of coherence
and destructive interference more generally, looking at multiple pinholes
(Gan & Gbur, 2007) as well as the case when the degree of coherence is dif-
ferent for different pinhole pairs (Rosenbury, Gu, & Gbur, 2012). For the
case of N pinholes, with the same degree of coherence μ0 between the pin-
holes, the nontrivial degree of coherence that produces destructive interfer-
ence is μ0 ¼ 1/(N 1).
Even with two pinholes, Young’s experiment has revealed unexpected
behavior. In 2003, Schouten et al. demonstrated that there are always pairs of
points in the superposition region of Young’s experiment where the field is
fully coherent, regardless of the state of coherence of the light at the pinholes
(Schouten, Visser, & Wolf, 2003).
When nontrivial polarization is added to Young’s experiment, even
richer coherence properties are exhibited. Traditionally, the statistical prop-
erties of the state of polarization have been treated separately from the sta-
tistical properties of the complex wavefield. The polarization was studied at
one point in space, often described by the so-called coherency matrix (Wolf,
1959),
" #
hE*x ðr, tÞE x ðr, tÞi hE *x ðr, tÞE y ðr, tÞi
J≡ , (52)
hE*y ðr, tÞE x ðr, tÞi hE *y ðr, tÞE y ðr, tÞi
where i, j ¼ {x, y}. This matrix can be used to determine the coherence and
polarization properties of the field and interrelations between them.
A degree of coherence for this general case can readily be determined by
returning to Young’s experiment, but now evaluated with fluctuating elec-
tric fields. Again working with a frequency-filtered version of Young’s
experiment, we have
Young’s interference experiment 313
of polarization (Agarwal, Dogariu, Visser, & Wolf, 2005); this work general-
ized the aforementioned work by Schouten et al. for scalar fields (Schouten,
Visser, & Wolf, 2003). Gori et al. interpreted the output of Young’s exper-
iment using a vector mode theory (Gori, Santarsiero, & Borghi, 2006). Also in
2006, Set€al€a, Tervo, and Friberg (2006 a, 2006 b) derived spectral interference
laws for the Stokes parameters in Young’s experiment.
In concluding this section on coherence, we note that Young’s exper-
iment can not only be used to analyze the statistical properties of light,
but also synthesize light with tailored coherence properties. In 2021, Lv
et al. (2021) showed that Young’s experiment can be used to generate non-
uniformly correlated fields, i.e., fields that possess a spatially varying, non-
homogeneous, degree of coherence.
7. Surface plasmons
In 1957, a novel type of electromagnetic guided mode was discovered
by Ritchie in experiments studying electron transmission through thick
metallic foils (Ritchie, 1957). These modes are known as surface plasma
polaritons, often simply called surface plasmons (SPs) (Raether, 1988). At
optical frequencies, they propagate along the interface between a dielectric
and a metal. As is characteristic for surface waves, their maximum intensity is
at the interface, and the fields decay exponentially away from it. The prop-
agation of SPs includes a longitudinal density fluctuation of surface electrons.
Owing to the strong localization of intensity, SPs are routinely employed
in surface-enhanced Raman scattering (SERS) and second harmonic gener-
ation (SHG). Whereas optical communication speeds are limited by the
conversion of light waves into electronic signals for purposes of routing, sig-
nal processing, and amplification, the use of SPs in so-called all-optical net-
works might one day make this electronic bottleneck obsolete. For our
present discussion, we are interested in the role that SPs play in optical trans-
mission through small apertures in metal films. As we will discuss, the total
transmission, the state of coherence, and the state of polarization are all
strongly affected by SPs, and these effects can be demonstrated using
Young’s experiment. A simple intuitive model can explain the mechanism
behind these phenomena.
The diffraction of light by an aperture in an opaque screen can often be
adequately described with classical scalar theory. The main formulas that are
commonly used are one by Kirchhoff, and two expressions due to Rayleigh
and Sommerfeld (Goodman, 1996). One feature these approaches have in
Young’s interference experiment 315
common is the assumption that the field in the aperture is identical to the
incident field, i.e., the field in the absence of the screen, which is often taken
to be a normally incident plane wave. In reality, the actual field will differ
from the incident field because of scattering caused by the screen. In spite of
this approximation, when the aperture is much larger than the wavelength,
the predictions of the three formulas that were just mentioned are very sim-
ilar and quite accurate.
A theoretical model of the behavior of light transmission through a sub-
wavelength hole in an infinitely thin, perfectly conducting screen was intro-
duced by Bethe in 1944 (Bethe, 1944). Bethe predicted the transmission
efficiency to scale as (r/λ)4, where r is the radius of the hole. For holes sig-
nificantly smaller than the wavelength, it was therefore typically assumed
that almost no light would be transmitted.
When dealing with subwavelength apertures in metal films with a finite
thickness and conductivity, a scalar approach no longer suffices and, follow-
ing Bethe, Maxwell’s equations must be used. An example is presented in
Fig. 10 where the time-averaged Poynting vector near a narrow slit in thin
metal film is plotted. The result is seen to be quite intricate and contains
structures like vortices and saddle points. This field structure is not only very
sensitive to the wavelength and polarization of the incident field, but also to
the slit width, the thickness of the film, and its conductivity.
a b
c d
100 nm 0 1
Fig. 10 Time-averaged Poynting vector near a 200-nm wide slit in a 100-nm thick silver
plate. Plane wave light, with a wavelength λ ¼ 500 nm, is incident below. Left-handed (A
and D) and right-handed (B and C) optical vortices are visible, just as two saddle points (E
and F). The color coding indicates the modulus of the normalized Poynting vector.
Reproduced from Schouten, H. F., Visser, T. D., Lenstra, D., & Blok, H. (2003). Light transmis-
sion through a sub-wavelength slit: Waveguiding and optical vortices. Physical Review E, 67,
036608.
316 Greg Gbur and Taco D. Visser
metal
z
SP SP dielectric
x d
U (in) (r1 ) U (in) (r2 )
Fig. 11 A metal film with two identical subwavelength parallel slits is embedded in a
dielectric. The film is illuminated from below (blue arrows). At each side of the metal film
and at each slit SPs are launched both to the left and to the right (red arrows). Cylindrical
waves (blue) emanate from the slits. The distance between the two slits is d.
transmission process; and is illustrated in Fig. 11. Moreover, this model also
adequately describes changes in coherence and polarization.
Let U(in)(ri), with i ¼ 1 or 2, denote the monochromatic incident field at
slit i at frequency ω, and U(out)(ri) the transmitted field. When the incident
field is TE polarized (along the y direction) part of it will be reflected, and a
fraction, α say, will be directly transmitted, i.e.,
where Em and Ed are the relative complex dielectric constants of the metal and
the dielectric, respectively, and k0 ¼ 2π/λ0 is the free-space wavenumber.
The SP wavelength is related to the real part of ksp by λsp ¼ 2π/Re(ksp).
The amplitude decay length is given by 1/Im(ksp). It is seen from
Eqs. (60) and (61) that the SP-mediated amplitude interferes with the ampli-
tude of the light that is directly transmitted by each slit. When the slit widths
are subwavelength these two contributions are of comparable magnitude.
From now on we concentrate on TM polarization and consider the case
of a normally incident, monochromatic plane wave, and hence
This result implies that, depending on the slit separation d, the SPs can either
help or hinder the transmission process. Notice that the intensity modulation
varies with the SP wavenumber ksp, rather than the free-space wavenumber
k0. Even though this intuitive model contains three unknown complex con-
stants, namely the transmission coefficients α and β and the scattering coef-
ficient γ, it provides a clear physical insight into the mechanism that
underlies EOT.
A rigorous numerical analysis presented in Schouten et al. (2005), based
on a Green’s tensor scattering formalism, showed the SPs form a standing
wave pattern between the two slits, as seen in Fig. 12. When the slit sepa-
ration is such that the antinodes coincide with the slit positions the transmis-
sion reaches a maximum, when the nodes of the standing-wave pattern are
at the slits, the transmission is suppressed. In the same study, an experimental
verification using a tunable laser was reported. As shown in Fig. 13, the
predicted modulation of the detected transmitted field (integrated over
many diffraction orders) with frequency, and hence with ksp, was only
observed for TM illumination. This is evidence that SPs indeed play a
pivotal role in the transmission process of light through nanoapertures.
Young’s interference experiment 319
We next turn our attention to the case that the field that is incident on the
slits is not fully coherent, as was assumed so far, but is spatially partially
coherent. Surface plasmons traveling between the slits are then found to
modify the state of coherence as well. Since many properties of a light
field—such as its spectrum, polarization, and directionality—may change
on propagation and are dependent on the spatial coherence of the (second-
ary) source, this suggest that the use of surface plasmons provides a new way
to alter or even tailor the statistical properties of a light field. We recall
(cf. Eq. (26) of Section 6) that the spectral degree of coherence of the
incident field is defined as
and, in strict analogy, the spectral degree of the transmitted field is given by
the expression
320 Greg Gbur and Taco D. Visser
Fig. 13 The top frame shows Young’s interference pattern as observed with a CCD. The
other frames show diffraction-order-integrated transmission spectra for TM illumina-
tion, for selected values of the slit separation d. In the bottom frame results for TE illu-
mination are also included (open squares). The vertical axis on the right corresponds to
this choice of polarization. Reproduced from Schouten, H. F., Kuzmin, N., Dubois, G.,
Visser, T. D., Gbur, G., Alkemade, P. F. A., …Eliel, E. R. (2005). Plasmon-assisted two-slit trans-
mission: Young’s experiment revisited. Physical Review Letters, 94, 053901.
Using the definition (64) for the spectral density of the transmitted field now
gives
h i
ðinÞ
SðoutÞ ðr1 Þ ¼ SðinÞ jβj2 + jγj2 + 2Re γβ* μ12 eiksp d , (68)
h i
ðinÞ*
SðoutÞ ðr2 Þ ¼ SðinÞ jβj2 + jγj2 + 2Re γβ* μ12 eiksp d , (69)
which leads to
ðinÞ ðinÞ*
|μ12(ω)|
μ
|μ12(ω)|
Fig. 14 The absolute value of the spectral degree of coherence of the transmitted field
as a function of the slit separation d, for selected values of the spectral degree of coher-
ence of the incident field. In (A) the slit width w ¼ 100 nm, in (b) w ¼ 100 nm.
Reproduced from Gan, C. H., Gbur, G., & Visser, T. D. (2007). Surface plasmons modulate
the spatial coherence of light. Physical Review Letters, 98, 043908.
film, was analyzed numerically in Gan, Gu, Visser, and Gbur (2012). In such a
setup there is no direct relation between the visibility of the interference pat-
tern produced by the transmitted field and an overall degree of coherence.
Nevertheless, the coherence of neighboring pairs of apertures can be studied.
It was found that this depended strongly on the separation of the holes and
their light-to-SP scattering strength. A further study into the effects of array
Young’s interference experiment 323
geometry, lattice constant, and hole size on coherence conversion was pres-
ented in Gbur and Smith (2021). The same authors had previously discovered
the existence of so-called coherence bandgaps in plasmonic hole arrays
(Smith & Gbur, 2019). In Saastamoinen and Lajunen (2013) a subwavelength
metallic grating with an incident Gaussian Schell-model beam was investi-
gated numerically. The authors introduced a global degree of coherence, as
an intensity-weighted average of the spectral degree of coherence of the
diffracted field. They observed that, for certain grating parameters, this quan-
tity can be enhanced significantly.
A third form of modulation of the diffracted field caused by SPs is that of
the state of polarization (SOP). This effect was examined by Leinonen et al.
(2021). The electric field at the exit plane z ¼ h of the metallic film can be
propagated to an arbitrary plane z > h using the angular spectrum technique
(Mandel & Wolf, 1995). In such an approach each electric field component
is written as an integral of plane waves, i.e.,
Z ∞
E j ðx, zÞ ¼ Aj ðkx Þ exp ½iðkx x + kz ΔzÞ dkx , ðj ¼ x, yÞ, (72)
∞
where Δz ¼ z h,
Z
1 ∞
Aj ðkx Þ ¼ E ðx, tÞ exp ðikx xÞ dx, ðj ¼ x, yÞ, (73)
2π ∞ j
and
8 qffiffiffiffiffiffiffiffiffiffiffiffiffiffi
>
< k20 k2x when jkx j < k0 ,
kz ¼ qffiffiffiffiffiffiffiffiffiffiffiffiffiffi (74)
>
: i k2 k2
x 0 when jkx j < k0 ,
This gives
Ax ðkx Þ ¼ ½α + γ exp ðiksp dÞ cos ðdkx =2Þ, (77)
Ay ðkx Þ ¼ β cos ðdkx =2Þ: (78)
With this formalism the SP-modulated State of Polarization (SOP) of the
transmitted field can be calculated. In Leinonen et al. (2021), the phenom-
enological model that we just described was validated. With the help of a
rigorous Fourier Modal Method it was shown that the values of the three
parameters α, β, and γ remain fairly constant over a range of configuration
parameters such as the slit separation distance. It was shown that not just the
far-zone SOP can be controlled by varying the slit separation, but also the
degree of polarization can be manipulated. In particular, it was shown
numerically that a linearly partially polarized field can, under suitable con-
ditions, be rendered completely unpolarized by the action of surface
plasmons.
The interference of SPs, i.e., without the usual back conversion into light,
has been studied in which was called an SP analog to Young’s double-slit
experiment (Zia & Brongersma, 2007). Two narrow metallic stripes that sup-
port plasmons play the same role as the traditional slits. At the end of the slits
the SPs enter a broad Au film where their interference can be observed with a
photon scanning tunneling microscope.
jI A I B j
D ¼ jP A P B j ¼ : (81)
IA + IB
This quantity is also called “predictability” by Jaeger, Horne, and Shimoney
(1993). It is considered as a marker of the amount of “particleness.” Similarly,
a measure of the amount of “waveness” is provided by the visibility, or fringe
contrast V, which was introduced in Section 6. The usual view is that com-
plete which-way information, i.e., D ¼ 1, rules out the formation of inter-
ference fringes, implying that V ¼ 0. Which-way information can be
obtained, for example, by placing orthogonal polarizers behind each of the
two slits and thus tagging the photons. Remarkably, this information is not
absolute, in the sense that it can be erased to restore the formation of inter-
ference fringes (Scully, Englert, & Walther, 1991; Walborn, Cunha,
Pádua, & Monken, 2002). Conversely, perfectly sharp fringes with V ¼ 1
can only be formed when the intensity from both apertures is equal, i.e., when
D ¼ 0 (Brezger et al., 2002).
In Wootters and Zurek (1979) it was pointed out that duality need not
represent an absolute incompatibility. In fact, in Young-type scenarios an
amount of particleness can be given up for an increase in waveness, and vice
versa. This implies a sort of duality balance between wave and particle
interpretations. More precisely, one can show that (for a list of the many dif-
ferent derivations of this result, see Ref. 6 in Eberly, Qian, and Vamivakas
(2017))
V 2 + D2 1: (82)
326 Greg Gbur and Taco D. Visser
In Qian, Vamivakas, and Eberly (2018) it was argued that this picture cannot
tell the whole story. For example, if the contributions from A and B are
equally strong, then the distinguishability D ¼ 0. If these two fields are also
orthogonally polarized, then no fringes will be produced and the visibility
V ¼ 0. A nonzero signal must be characterized by something more than
V ¼ D ¼ 0, a clear indication that something is absent from this picture.
This missing information can be identified by a recently derived
“polarization coherence theorem” (Eberly et al., 2017), which connects
the degree of polarization P, the ratio of the intensity of the polarized por-
tion of the field, and its total intensity, with the visibility and the distinguish-
ability through the relation
P 2 ¼ V 2 + D2 : (83)
Notice that since the degree of polarization is bounded by zero and unity,
there is no conflict between Eqs. (82) and (83). An experimental verification
of this theorem was reported in Kanseri and Sethuraj (2019). A further ingre-
dient to consider is the degree of entanglement, of which one of the possible
measures is the concurrence C. The concurrence and the degree of polar-
ization are, within the context of Young’s experiment, perfect opposites. By
considering the aforementioned analogy of factorization of classical polari-
zation states and entanglement, it can be derived that (Qian, Malhotra,
Vamivakas, & Eberly, 2016)
P2 ¼ 1 C2: (84)
This expression shows that gaining some of P2 comes at the expense of losing
an equal amount of C2. This result is quite surprising, since P and C have
such different traditional origins and interpretations, entanglement being a
bipartite property, whereas polarization is a single-party property. On mak-
ing use of Eq. (84) in Eq. (83) it immediately follows that
V 2 + D2 + C 2 ¼ 1: (85)
C
13 1
12
11
9 10
8
5
0 7
6
1
D
4
1
V 1 3
2
Fig. 15 Thirteen measurements of (V, D, C), represented by the red dots, are seen to fit
on the surface of one octant of a unit sphere. Reproduced from Qian, X.-F.,
Vamivakas, A. N., & Eberly, J. H. (2018). Entanglement limits duality and vice versa.
Optica, 5, 942–947.
Blocking Mask
Position
60µm
0
600µm
C
1000µm
AC
300µm
AB
100µm
ABC
Fig. 16 The seven different slit arrangements that were used to test Born’s Rule.
Reproduced from Sinha, U., Couteau, C., Jennewein, T., Laflamme, R., & Weihs, G. (2010).
Ruling out multi-order interference in quantum mechanics. Science, 329, 418–421.
Fig. 17 A three-slit configuration showing both a classical path (green) and a non-
classical path (blue). Reproduced from Sawant, R., Samuel, J., Sinha, A., Sinha, S., &
Sinha, U. (2014). Nonclassical paths in quantum interference experiments. Physical
Review Letters, 113, 120406.
via slit B, and emerge again from slit C (blue curve). For a double-slit
arrangement, this means that Eq. (87) would have be altered to a more gen-
eral form, namely (Sawant, Samuel, Sinha, Sinha, & Sinha, 2014)
κ 105 : (96)
To overcome the technical difficulties involved in observing such a very
small nonzero value of κ, Magana-Loaiza et al. (2016) designed a three-slit
setup illuminated with a polarization that allows for the excitation of SPs
traveling between the closely spaced slits. This enhances the near field
and thus increases the contribution of nonclassical paths. In Fig. 18 the
Poynting vector is shown for the case of only the leftmost slit A being illumi-
nated with an x-polarized field. It can be seen that the Poynting vector clearly
exhibits a loop-like behavior. This results in a strongly increased visibility of
the far-field interference pattern as compared to y-polarized illumination that
Young’s interference experiment 331
d A B C
|P| z
0 x
E
Fig. 18 Simulation of the normalized Poynting vector P in the vicinity of three slits. The
illumination assumes an x-polarized illumination that onto slit A. The Poynting vector is
seen to follow a looped trajectory. Reproduced from Magana-Loaiza, O. S., Leon, I. D.,
Mirhosseini, M., Fickler, R., Safari, A., Mick, U., …Boyd, R. W. (2016). Exotic looped trajectories
of photons in three-slit interference. Nature Communications, 13987, 159–162.
does not generate SPs. Using single heralded photons the individual terms of
Eq. (93) were measured. The observed value of κ 0.3, in agreement with
simulations and well above the level of uncertainty, demonstrates that under
certain conditions nonclassical paths do indeed occur.
here γ is the azimuth of the polarization ellipse, and the integral is along a
closed circuit enclosing the beam axis. The far-zone polarization morphol-
ogy was found to be lattice like, with the precise pattern depending on the
index η of the incident beam.
The occurrence of polarization singularities in an N-pinhole inter-
ferometer has been detailed in Schoonover and Visser (2009). For the case
of N ¼ 2 and with the fields at the two apertures assumed to be cophasal,
x
(a) O
(b)
1
z
2 3
Fig. 20 (A) Three pinholes in an opaque screen producing a hexagonal interference pat-
tern. (B) The fields at the bottom two pinholes are horizontally polarized, whereas the
field at the top pinhole is polarized under an angle θ. Pinholes 1 and 3 are fully corre-
lated. Pinhole 2 is partially correlated with the other two pinholes, quantified by the
parameter μ. Reproduced from Pang, X., Gbur, G., & Visser, T. D. (2015). Cycle of phase,
coherence and polarization singularities in Young’s three-pinhole experiment. Optics
Express, 23, 34093–34108.
Young’s interference experiment 335
Fig. 21 Color-coded plot of the spectral density (left), and the phase of Ex(x, y) when
θ ¼ 0 and μ ¼ 1. Reproduced from Pang, X., Gbur, G., & Visser, T. D. (2015). Cycle of phase,
coherence and polarization singularities in Young’s three-pinhole experiment. Optics
Express, 23, 34093–34108.
shown in the left panel of Fig. 21. The phase of Ex(x, y) is plotted on the
right. Several phase singularities, points where the different phase contours
intersect, can be seen. If now the angle θ is increased to a nonzero value, the
highly symmetric field distribution is perturbed, and the central phase sin-
gularity at x ¼ y ¼ 0 decays into a pair of two polarization singularities,
as illustrated in Fig. 22. The orientation of the polarization axis shows the
characteristic pattern of a lemon (top) and a star singularity (bottom). In
the right-hand panel contours of the corresponding normalized Stokes
parameters are plotted. The two C-points are separated by an L-line
(orange). Furthermore, it is seen that the two C-points have opposite hand-
edness, with s3 ¼ +1 and 1, respectively. By further changing the param-
eters θ and μ electromagnetic coherence singularities, zeros of η(r1, r2, ω),
can be created and annihilated in this configuration.
Beams of light can carry both spin and orbital angular momentum. The
spin angular momentum arises from the vectorial, or polarization, nature of
light, while the orbital angular momentum originates from the spatial distri-
bution of the wavefront. Laguerre-Gauss (LG) beams of light carry a well-
defined amount of orbital angular momentum (OAM) that is proportional
to the variation of the phase structure of the beam. An overview of different
methods to detect OAM is presented in Emile, Emile, and Brousseau (2019).
In Young’s double-slit experiment, the presence of OAM in the incident field
profoundly alters the observed interference pattern. This was demonstrated
336 Greg Gbur and Taco D. Visser
(a) (b)
0.01
0.01
y [mm]
y [mm]
0 0
-0.01
-0.01
-0.01 0 0.01 -0.01 0 0.01
x [mm] x [mm]
Fig. 22 (A) The local orientation of the major axis of the polarization ellipse after the
angle of polarization at pinhole 1 has been increased from zero to θ ¼ 0.03. The phase
singularity of Ex at (0, 0) in Fig. 21 has decayed into two polarization singularities: a
lemon (top) and a star (bottom). (B) Selected contours of the normalized Stokes param-
eters for the same region as in the left-hand panel: s1 ¼ 0 (blue), s2 ¼ 0 (green), s3 ¼ 0.998
(red), s3 ¼ 0.998 (black). Points with horizontal polarization (s3 ¼ 0) are represented by
the orange curve. Reproduced from Pang, X., Gbur, G., & Visser, T. D. (2015). Cycle of phase,
coherence and polarization singularities in Young’s three-pinhole experiment. Optics
Express, 23, 34093–34108.
of this “hole wheel” method is that the number of point apertures limits the
upper bound of the topological charge that can be distinguished. This can be
partly remedied by distributing the apertures nonuniformly over a circle, as
was demonstrated numerically in Shi, Tian, and Chen (2012).
11. Conclusions
After conducting an informal poll among physicists, asking them to
name the experiment they thought was the most beautiful, Crease
(Crease, 2003) described the 10 most popular choices in his engaging book
The Prism and the Pendulum. Remarkably, Young’s experiment is listed
twice. The top spot was taken by the double-slit experiment with electrons
carried out by J€onsson (1961), and the original optical experiment, per-
formed by Young himself, ended in fifth place. It goes without saying that
the present authors feel that these accolades are well deserved. Indeed, it is
more than impressive that more than two centuries after its inception
Young’s experiment still plays a fundamental role in the development of
quantum mechanics, coherence theory, singular optics, and plasmonics.
The much maligned Thomas Young has left us a legacy that stands out in
the history of physics.
Acknowledgments
We wish to thank Dr. Hugo Schouten, Prof. Joe Eberly, Prof. Dorinda Outram, Prof. Ari
Friberg, Prof. Pang Xiaoyan, and the late Prof. Emil Wolf for the many discussions that have
helped shape our understanding.
References
Agarwal, G. S., Dogariu, A., Visser, T. D., & Wolf, E. (2005). Generation of complete coher-
ence in Young’s interference experiment with random mutually uncorrelated electro-
magnetic beams. Optics Letters, 30, 120–122.
Aharonov, Y., & Bohm, D. (1959). Significance of electromagnetic potentials in the quan-
tum theory. Physical Review, 115, 485–491.
Ambrosini, D., Gori, F., & Paoletti, D. (2005). Destructive interference from three partially
coherent point sources. Optics Communications, 254(1), 30–39.
Angelsky, O. V. (2007). Optical correlation: Techniques and applications. Bellingham,
Washington: SPIE.
Arago, F. (1819). Rapport fait par M. Arago. Annales de Chimie et de Physique, 11, 5–30.
Arago, F. (1835). Biographical memoir of Dr Thomas Young. The Edinburgh New
Philosophical Journal, 20, 213–240.
Arago, F., & Fresnel, A. J. (1819). L’action que les rayons de lumière polarisee exercent les uns
sur les autres. Annales de Chimie et de Physique, 10, 288–300.
Arnd, M., Aspelmeyer, M., & Zeilinger, A. (2002). How to extend quantum experiments.
Fortschritte der Physik, 57, 1153–1162.
338 Greg Gbur and Taco D. Visser
Arndt, M., Nairz, O., Vos-Andreae, J., Keller, C., van der Zouw, G., & Zeilinger, A. (1999).
Wave–particle duality of C60 molecules. Nature, 401, 680–682.
Bach, R., Pope, D., Liou, S. H., & Batelaan, H. (2013). Controlled double-slit electron dif-
fraction. New Journal of Physics, 15, 033018.
Basano, L., & Ottonello, P. (2005). Complete destructive interference of partially coherent
sources of acoustic waves. Physical Review Letters, 94(17), 173901.
Berkhout, G. C. G., & Beijersbergen, M. W. (2008). Method for probing the orbital angular
momentum of optical vortices in electromagnetic waves from astronomical objects.
Physical Review Letters, 101, 100801.
Berry, M. V. (1984). Quantal phase factors accompanying adiabatic changes. Proceedings of the
Royal Society of London. Series A, Mathematical and Physical Sciences, 392, 45–57.
Berry, M. V., & Dennis, M. R. (2001). Polarization singularities in isotropic random vector
waves. Proceedings of The Royal Society A Mathematical Physical and Engineering Sciences, 457,
141–155.
Bethe, H. A. (1944). Theory of diffraction by small holes. The Physical Review, 66, 163–182.
Born, M., & Wolf, E. (1999). Principles of Optics. Cambridge: Cambridge University Press.
Brandt, D., & Hirschi, S. (1974). Electron diffraction at multiple slits. American Journal of
Physics, 42, 4–11.
Brezger, B., Hackerm€ uller, L., Uttenthaler, S., Petschinka, J., Arndt, M., &
Zeilinger, A. (2002). Matter-wave interferometer for large molecules. Physical Review
Letters, 88, 100404.
Brosseau, C. (1998). Fundamentals of polarized light. New York: John Wiley and Sons.
Brougham, H. P. (1803). Art. XVI. The Edinburgh Review, 1, 450–460.
Cao, Q., & Lalanne, P. (2002). Negative role of surface plasmons in the transmission of metal-
lic gratings with very narrow slits. Physical Review Letters, 88, 057403.
Carnal, O., & Mlynek, J. (1991). Young’s double-slit experiment with atoms: A simple atom
interferometer. Physical Review Letters, 66, 2689–2692.
Chambers, R. G. (1960). Shift of an electron interference pattern by enclosed magnetic flux.
Physical Review Letters, 5, 3–5.
Chapman, M. S., Ekstrom, C. R., Hammond, T. D., Rubenstein, R. A., Schmiedmayer, J.,
Wehinger, S., & Pritchard, D. E. (1995). Optics and interferometry with Na2 molecules.
Physical Review Letters, 74, 4783–4786.
Crease, R. P. (2003). The Prism and the Pendulum. New York: Random House.
Davisson, C. J. (1928). Are electrons waves? Journal of the Franklin Institute, 206, 597–623.
Davisson, C. J., & Gerner, L. H. (1927). The scattering of electrons by a single crystal of
Nickel. Nature, 119, 558–560.
de Broglie, L.-V. (2004). On the theory of quanta. Privately published translation by A.F.
Kracklauer.
Dennis, M. R., O’Holleran, K., & Padgett, M. J. (2009). Singular optics: Optical vortices and
polarization singularities. In E. Wolf (Ed.), Progress in optics: Vol. 53 (pp. 293–363).
Amsterdam: Elsevier.
Dimitrova, T. L., & Weis, A. (2008). The wave-particle duality of light: A demonstration
experiment. American Journal of Physics, 76, 137–142.
Divitt, S., Frimmer, M., Visser, T. D., & Novotny, L. (2016). Modulation of optical spatial
coherence by surface plasmon polaritons. Optics Letters, 41, 3094–3097.
Ebbesen, T. W., Lezec, H. J., Ghaemi, H. F., Thio, T., & Wolff, P. A. (1998). Extraordinary
optical transmission through sub-wavelength hole arrays. Nature, 391, 667–669.
Eberly, J. H., Qian, X.-F., & Vamivakas, A. N. (2017). Polarization coherence theorem.
Optica, 4, 1113–1114.
Eckert, M. (2012). Max von Laue and the discovery of X-ray diffraction in 1912. Annalen der
Physik, 524, A83–A85.
Young’s interference experiment 339
Eibenberger, S., Gerlich, S., Arndt, M., Mayor, M., & T€ uxen, J. (2019). Matter-wave inter-
ference of particles selected from a molecular library with masses exceeding 10, 000 amu.
Physical Chemistry Chemical Physics, 15, 14696.
€
Einstein, A. (1905). Uber einen die Erzeugung und Verwandlung des Lichtes betreffenden
heuristischen Gesichtspunkt. Annalen der Physik, 17, 132–148.
Emile, O., Emile, J., & Brousseau, C. (2019). Detection of the orbital angular momentum in optics.
U. Rennes.
Emile, O., Emile, J., de Lesegno, B. V., Pruvost, L., & Brousseau, C. (2015). Analysis of the
topological charge of vortex beams using a hole wheel. EPL, 111, 34001.
Estermann, I., & Stern, O. (1930). Beugung von Molekularstrahlen. Zeitschrift f€ ur Physik, 61,
95–125.
Fein, Y. Y., Geyer, P., Zwick, P., Kialka, F., Pedalino, S., Mayor, M., … Arndt, M. (2019).
Quantum superposition of molecules beyond 25 kDa. Nature Physics, 15, 1242–1245.
Feynman, R., Leighton, R., & Sands, M. (1963). Vol. I. The feynman lectures on physics.
Reading Mass: Addison-Wesley.
Flossmann, F., Schwarz, U. T., Maier, M., & Dennis, M. R. (2005). Polarization singularities
from unfolding an optical vortex through a birefringent crystal. Physical Review Letters,
95, 253901.
Forbes, A., Aiello, A., & Ndagano, B. (2019). Classically entangled light. In T. D. Visser
(Ed.), Vol. 64. Progress in optics (pp. 99–153).
Friedrich, W., Knipping, P., & von Laue, M. (1912). Diffraction. Sber. Bayer. Akad. Wiss.,
524, 303–304.
Gan, C. H., & Gbur, G. (2007). Phase and coherence singularities generated by the interfer-
ence of partially coherent fields. Optics Communications, 280(2), 249–255.
Gan, C. H., & Gbur, G. (2008). Spatial coherence conversion with surface plasmons using a
three-slit interferometer. Plasmonics, 3, 111.
Gan, C. H., Gbur, G., & Visser, T. D. (2007). Surface plasmons modulate the spatial coher-
ence of light. Physical Review Letters, 98, 043908.
Gan, C. H., Gu, Y., Visser, T. D., & Gbur, G. (2012). Coherence converting plasmonic hole
arrays. Plasmonics, 7, 313–322.
Garcia-Vidal, F. J., Martin-Moreno, L., Ebbesen, T. W., & Kuipers, L. (2010). Light passing
through subwavelength apertures. Reviews of Modern Physics, 82, 729–787.
Gbur, G., & Smith, M. (2021). Controlled coherence plasmonic light sources. Photonics,
8, 268.
Gbur, G., Visser, T. D., & Wolf, E. (2004a). Complete destructive interference of partially
coherent fields. Optics Communications, 239(1), 15–23.
Gbur, G., Visser, T. D., & Wolf, E. (2004b). Hidden singularities in partially coherent
wavefields. Journal of Optics A Pure and Applied Optics, 6, S239–S242.
Gbur, G. J. (2017). Singular Optics. Boca Raton: CRC Press.
Genet, C., & Ebbesen, T. W. (2007). Light in tiny holes. Nature, 445, 39–46.
Geyer, P., Sezer, U., Rodewald, J., Mairhofer, L., D€ orre, N., Haslinger, P., …
Arndt, M. (2016). Perspectives for quantum interference with biomolecules and biomo-
lecular clusters. Physica Scripta, 91, 063007.
Goodman, J. W. (1996). Introduction to Fourier Optics. New York: McGraw-Hill.
Gori, F., Santarsiero, M., & Borghi, R. (2006). Vector mode analysis of a Young interfer-
ometer. Optics Letters, 31(7), 858–860.
Gori, F., Santarsiero, M., Borghi, R., & Wolf, E. (2006). Effects of coherence on the degree
of polarization in a Young interference pattern. Optics Letters, 31(6), 688–690.
Gurney, H. (1831). Memories of the life of Thomas Young. London: John and Arthur.
Hannonen, A., Partanen, H., Tervo, J., Set€al€a, T., & Friberg, A. T. (2019).
Pancharatnam-Berry phase in electromagnetic double-pinhole interference. Physical
Review A, 99, 053826.
340 Greg Gbur and Taco D. Visser
Nairz, J., Arndt, M., & Zeilinger, A. (2002). Quantum interference experiments with large
molecules. American Journal of Physics, 71, 319–325.
Newton, I. (1704). Opticks. London: Smith and Walford.
Pang, X., Gbur, G., & Visser, T. D. (2015). Cycle of phase, coherence and polari-
zation singularities in Young’s three-pinhole experiment. Optics Express, 23,
34093–34108.
Parker, S. (1971). A single-photon double-slit interference experiment. American Journal of
Physics, 39(4), 420–424.
Peacock, G. (1855). Life of Thomas Young. London: J. Muray.
Peacock, G. (Ed.). (1855). Miscellaneous works of the late Thomas Young. London: J. Murray.
Pfleegor, R. L., & Mandel, L. (1967). Interference of independent photon beams. The
Physical Review, 159, 1084–1088.
Pu, J., Cai, C., & Nemoto, S. (2004). Spectral anomalies in Young’s double-slit interference
experiment. Optics Express, 12, 5131–5139.
Qian, X.-F., Malhotra, T., Vamivakas, A. N., & Eberly, J. H. (2016). Coherence constraints
and the last hidden optical coherence. Physical Review Letters, 117, 153901.
Qian, X.-F., Vamivakas, A. N., & Eberly, J. H. (2018). Entanglement limits duality and vice
versa. Optica, 5, 942–947.
Raedt, H. D., Michielsen, K., & Hess, K. (2012). Analysis of multipath interference in
three-slit experiments. Physical Review A, 85, 012101.
Raether, H. (1988). Surface plasmons on smooth and rough surfaces and on gratings. Berlin:
Springer.
Raghunathan, S. B., Schouten, H. F., & Visser, T. D. (2012). Correlation singularities in
partially coherent electromagnetic beams. Optics Letters, 37, 4179–4181.
Raghunathan, S. B., Schouten, H. F., & Visser, T. D. (2013). Topological reactions of
correlation functions in partially coherent electromagnetic beams. Journal of the Optical
Society of America, 30, 582–588.
Ritchie, R. H. (1957). Plasma losses by fast electrons in thin films. The Physical Review, 106,
874–881.
Robinson, A. (2005). The last man who knew everything. New York: Pi Press.
Rosenbury, C., Gu, Y., & Gbur, G. (2012). Phase singularities, correlation singularities, and
conditions for complete destructive interference. Journal of the Optical Society of America A,
29(4), 410–416.
Rueckner, W., & Titcomb, P. (1996). A lecture demonstration of single photon interference.
American Journal of Physics, 64(2), 184–188.
Saastamoinen, T., & Lajunen, H. (2013). Increase of spatial coherence by subwavelength
metallic gratings. Optics Letters, 38, 5000–5003.
Sala, S., Ariga, A., Ereditato, A., Ferragut, R., Giammarchi, M., Leone, M., …
Scampoli, P. (2019). First demonstration of antimatter wave interferometry. Science
Advances, 5, eaav7610.
Santarsiero, M., & Gori, F. (1992). Spectral changes in a Young interference pattern. Physics
Letters A, 167, 123–128.
Sawant, R., Samuel, J., Sinha, A., Sinha, S., & Sinha, U. (2014). Nonclassical paths in quan-
tum interference experiments. Physical Review Letters, 113, 120406.
Sch€ollkopf, W., & Toennies, J. P. (1994). Non-destructive mass selection of small van der
Waals clusters. Science, 266, 1345–1348.
Schoonover, R. W., & Visser, T. D. (2009). Creating polarization singularities with an
N-pinhole interferometer. Physical Review A, 79, 043809.
Schouten, H. F., Gbur, G., & Wolf, T. D. V. E. (2003). Phase singularities of the coherence
functions in Young’s interference pattern. Optics Letters, 28, 968–970.
Schouten, H. F., Kuzmin, N., Dubois, G., Visser, T. D., Gbur, G., Alkemade, P. F. A., …
Eliel, E. R. (2005). Plasmon-assisted two-slit transmission: Young’s experiment
revisited. Physical Review Letters, 94, 053901.
342 Greg Gbur and Taco D. Visser
Schouten, H. F., Visser, T. D., & Wolf, E. (2003). New effects in Young’s interference
experiment with partially coherent light. Optics Letters, 28(14), 1182–1184.
Scully, M. O., Englert, B.-G., & Walther, H. (1991). Quantum optical tests of complemen-
tarity. Nature, 351, 111–116.
Set€al€a, T., Tervo, J., & Friberg, A. T. (2006a). Contrasts of Stokes parameters in Young’s
interference experiment and electromagnetic degree of coherence. Optics Letterrs,
31(18), 2669–2671.
Set€al€a, T., Tervo, J., & Friberg, A. T. (2006b). Stokes parameters and polarization contrasts in
Young’s interference experiment. Optics Letters, 31(14), 2208–2210.
Shapere, A., & Wilczek, F. (1989). Geometric phases in physics. Singapore: World Scientific.
Shi, L., Tian, L., & Chen, X. (2012). Characterizing topological charge of optical vortex
using non-uniformly distributed multi-pinhole plate. Chinese Optics Letters, 10, 120501.
Sinha, U., Couteau, C., Jennewein, T., Laflamme, R., & Weihs, G. (2010). Ruling out
multi-order interference in quantum mechanics. Science, 329, 418–421.
Smith, M., & Gbur, G. (2019). Coherence resonances and band gaps in plasmonic hole arrays.
Physical Review A, 99, 023812.
Sorkin, R. D. (1994). Quantum mechanics as quantum measure theory. Modern Physics Letters
A, 33, 3119–3127.
Soskin, M. S., & Vasnetsov, M. V. (2001). Singular optics. In E. Wolf (Ed.), Progress in optics:
Vol. 42 (p. p. 219). Amsterdam: Elsevier.
Spreeuw, R. J. C. (1998). A classical analogy of entanglement. Foundations of Physics, 28,
361–374.
Sztul, H. I., & Alfano, R. R. (2006). Double-slit interference with Laguerre-Gaussian beams.
Optics Letters, 31, 999–1001.
Taylor, G. I. (1909). Interference fringes with weak light. Proceedings—Cambridge Philosophical
Society, 15, 114–115.
Tervo, J., Set€al€a, T., & Friberg, A. T. (2003). Degree of coherence for electromagnetic fields.
Optics Express, 11(10), 1137–1143.
Thomson, G. P., & Reid, A. (1927). Diffraction of cathode rays by a thin film. Nature,
119, 890.
Thomson, J. J. (1906-1908). On the ionization of gases by ultra-violet light and on the evi-
dence as to the structure of light afforded by its electrical effects. Proceedings of the
Cambridge Philosophical Society, 14, 417–424.
Tonomura, A., Endo, J., Matsuda, T., Kawasaki, T., & Ezawa, H. (1989). Demonstration of
single-electron buildup of an interference pattern. American Journal of Physics, 57,
117–120.
Tonomura, A., Osakabe, N., Matsuda, T., Kawasaki, T., Endo, J., Yano, S., &
Yamada, H. (1986). Evidence for Aharonov-Bohm effect with magnetic field
completely shielded from electron wave. Physical Review Letters, 56, 792–801.
Verdet, E. (1869). Leçons d’Optique Physique. Paris: G. Masson.
Visser, T. D., & Schoonover, R. W. (2008). A cascade of singular field patterns in Young’s
interference experiment. Optics Communications, 281, 1–6.
von Bergmann, J., & von Bergmann, H. (2007). Foucault pendulum through basic geometry.
American Journal of Physics, 75, 888–892.
Walborn, S. P., Cunha, M. O. T., Pádua, S., & Monken, C. H. (2002). Double-slit quantum
eraser. Physical Review A, 65, 033818.
Weis, A., & Wynands, R. (2003). Three demonstration experiments on the wave and particle
nature of light. Physik und Didaktik in Schule und Hochschule, I,II, 67–73.
Wheeler, J. A., & Zurek, W. H. (Eds.). (1983). Quantum theory and measurement. Princeton:
Princeton University Press.
Whittaker, E. T. (1951). A history of the theories of aether and electricity, 2 Vols. London: Nelson.
Wolf, E. (1954). Optics in terms of observable quantities. Nuovo Cimento, 12, 884–888.
Young’s interference experiment 343