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T [N]
gle and bilayer sheets of graphene result in variations
1 M50
in friction [13]. Furthermore, friction was probed in ex- 10
periments on multi-walled carbon nanotubes and boron
nitride nanotubes [14–16]. In such investigations, the
inner tubes could be slid out of the outer tube reveal- −1
10
ing vanishingly-small molecular friction for carbon, and
50 150 250
a much stronger, area-dependent, molecular friction for d [mm]
boron nitride [16]. Clearly, such works reveal drastic de-
partures from the simple AC laws, as one approaches the
FIG. 2. Measured total traction force as a function of
nanoscale. Moreover, friction can be further complicated separation distance for various numbers of sheets. The
by a stick-slip response, as seen in many cases [17, 18], number of sheets for each of the two identical books is 2M ,
including layers of paper [19, 20]. Remarkably, although where M = 12, 16, 23, 27, 50, 75, and 100, with M increasing
these complex non-linear phenomena may be observed at as indicated by the arrow. The left inset shows a zoomed re-
micrometric scales, it is often the case on larger length gion for M = 50 highlighting stick-slip friction. The right
scales that the simple AC laws with which we are so fa- inset shows three experiments with M = 50, and varying ini-
tial separation distances d0 = 11, 14.5, and 22 mm (vertical
miliar are valid (see reviews [8, 10, 18, 21, 22]).
arrows).
In this Letter, we focus on the following stubborn pop-
ular enigma. As shown in Fig. 1(a), an entire car can be
lifted using a coupling element prepared from two inter-
leaved phonebooks [1]. In order to investigate this strik- number of sheets (e.g. M = 12 and M = 100) induces a
ing observation, we developed a well-controlled system of four orders of magnitude increase in the traction force. In
two identical books, both made up of 2M 1 identical the left inset of Fig. 2, we can see clear evidence of stick-
sheets of paper with width w = 12 cm, length L = 25 cm, slip [19, 20] for an experiment with M = 50. However,
and thickness = 0.10 mm. The two books are perfectly the difference between the local maxima and minima,
interleaved sheet-by-sheet and are then separated in a which results from the difference between the coefficients
vertical orientation, while the total traction force T is of static and kinetic friction, is negligible in comparison
measured (see Fig. 1(b)). The length of overlap between to the global amplitude in T . We can thus neglect this
the two books is denoted by L − d, where d is the separa- effect, as well as the difference in the coefficients of static
tion distance from the clamp of each book to the contact and kinetic friction. Furthermore, in the right inset of
zone (see Fig. 1(c)). Consistent with the actual experi- Fig. 2, we see that the experiments are reproducible and
mental parameters, we make the simplifying assumption independent of the initial separation distance d0 .
that d is large compared to the total thickness 2M of These results can be explained using simple geometri-
one book, so that the angle θn made by the nth sheet as cal and mechanical arguments, for which Fig. 1(c) pro-
it traverses from the clamp to the contact zone is small. vides detailed notations. Each sheet of a given book is
Therefore, L − d is nearly identical for all sheets. Finally, indexed by n ranging from n = 1 in the middle of the
the books are separated at constant velocity (typically book to n = M at one extremity. The problem is sym-
1 mm/min) and we have found, in accordance with the metric with respect to the central line of the book. We
AC laws, that the velocity does not significantly affect define Hn ≡ hn /d = n/d, where hn is the shift in posi-
the results. tion of the nth sheet in the contact zone with respect to
As the books are pulled apart, an initial maximum its position of clamping. As a consequence,pthe tilt angle
th
traction force is first reached before they start to slide θn of the np sheet satisfies sin θn = Hn / 1 + Hn2 and
with respect to each other. In Fig. 2, we show the raw cos θn = 1/ 1 + Hn2 . Essentially, the tilting of each in-
total traction force T , measured during constant-velocity dividual sheet n in the intermediate region between the
sliding, as a function of the distance d, for seven experi- clamping and contact zones converts part of the local
ments with M ranging from 12 to 100. As observed, the traction Tn exerted on it by the operator (at point A) into
smaller d or the larger M , the larger the traction, and a supplementary local normal force Tn tan θn = Hn Tn
those dependences are highly nonlinear. Furthermore, exerted on the stack below it (at point B). Therefore,
the amplification of friction is far from being a small ef- according to AC laws, this leads to a self-induced addi-
fect: a single experiment spans over three decades in the tional inner friction force that resists the traction: the
traction force. Additionally, a tenfold increase in the more the operator pulls, the higher the frictional resis-
3
T [Ν ]
1
2 10
where µ is the coefficient of kinetic friction, and the two 0
10
factors of 2 come from the identical contributions of the 1.5
50 100 150
µ
d [ mm ]
two books and the two pages of one sheet. Finally, the
boundary condition is given by TM = T ∗ , where T ∗ is 1
the unknown traction exerted on the outer Psheet, and
M 0.5
the total traction force is defined by T = 2 k=1 Tk .
We now introduce the variable z = n/M , as well as the 0 −2 −1 0 1
dimensionless amplification parameter α = 2µM 2 /d, 10 10 10 10
and use a continuous description by replacing Tn by T (z), [N]
since M 1. We thus obtain the ODE: FIG. 3. Coefficient of kinetic friction as a function of
0
the average effective load per page. (circles) Values of
T (z) + 2αz T (z) = 0 . (2) µ obtained by fitting each experiment performed on the inter-
leaved books to Eq. (3), as a function of the average effective
Together with the boundary condition T (1) = T ∗ , load hN i defined in text. Since µ is load-dependent, we indi-
we get by integration the local traction force T (z) = cate the traction range over which Eq. (3) was fit to the data
T ∗ exp[α(1 − z 2 )]. Finally, we obtain the total traction by the grey horizontal lines. (squares) Values of µ obtained
R1
force T = 2M 0 dz T (z) in the self-similar form: independently using a tribometer for two sheets of the same
paper. In this case, hN i is simply the externally-applied load,
and the error bars correspond to the standard deviation of the
√
r
T π measurements that have been repeated at least five times. The
= exp(α) erf α . (3)
2M T ∗ 4α inset shows a fit to Eq. (3) (dashed line) of a traction experi-
ment (plain line), for M = 50.
This expression is remarkable fort two reasons. First, it
tends to 1 as α → 0, which means that it represents the
geometrical amplification gain of friction with respect to known to be dependent on the normal load. Specifically,
a simple linear collection of 2M independent flat sheets µ increases with decreasing load and can even be higher
with local friction T ∗ . Secondly, it depends solely and than 1 for small loads, due to adhesion forces [26]. This
almost exponentially on the amplification parameter α, fact is confirmed in Fig. 3, where we plot the coefficient
which thus appears as the central dimensionless param- of kinetic friction obtained from a standard tribology ex-
eter of this study. periment between two sheets of paper, as a function of
We find that the data is well described by Eq. (3), us- the applied normal load (squares). Let us now compare
ing a single value T ∗ = 0.01 N of the microscopic traction this result with the interleaved-book case. As explained
force, and with a single coefficient of kinetic friction fit above, our model is based on the AC laws and considers
freely to each traction experiment. A typical example is a single average µ for each experiment, that is constant
shown in the inset of Fig. 3, for which an excellent fit irrespective of the load. This hypothesis is equivalent to
is obtained over more than two decades in the traction taking a coarse-grained approach, even though the load
force, with a constant value µ = 0.73 ± 0.02. The range increases towards the centre of the books and at small
over which our simple model is applicable, with a con- d. The previous assumption is sufficient to describe the
stant µ, is clear from the fit, and deviations are observed data, as evidenced by the fit in the inset of Fig. 3. Then,
at small overlap between the books. Note that the tiny we define through AC laws an effective load per page,
force T ∗ acting on the outmost sheets is a crucial bound- N = T /(4M µ), which would correspond to the load ap-
ary condition. It is this finite force, corresponding to no plied on each page if the 2M sheets were parallel (i.e.
more than the weight of a butterfly, that is self-amplified all θn = 0). Note that, by defining the microscopic load
by the operator – either in a well-controlled experiment N ∗ ≡ T ∗ /(2µ), Eq. (3) also provides the amplification
as we have carried out here, or when lifting a car with gain N /N ∗ in normal load. The average traction force
phonebooks [1]. In our experiment, the boundary force hT i of a given experiment is calculated over the range
T ∗ originates from the elasticity of the paper: the outer of applicability of the theory, and used to obtain the av-
sheets have a tendency to be flat and resist slightly the erage effective load per page hN i. The result µ(hN i) is
bowing induced in the contact region, thus creating a shown in Fig. 3 (circles), with the ranges of applicabil-
small normal force resulting in a small friction force. ity indicated by the grey horizontal lines. In short, a
The coefficient of kinetic friction is a phenomenological single value of µ could be used to adequately describe
quantity whose value depends on several parameters [23]. each T (d) experiment with the theory, even though the
For metal-on-metal [24] and paper-on-paper [25], µ is load varied over the indicated range. The consistency
4
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279 (2006). Acknowledgments The authors thank the television
[19] N. Garoff, The friction between paper surfaces (PHD thesis) channel France 5 and the 2P2L producing company, for
(Institutionen för pappers- och massateknologi, 2002).
[20] F. Heslot, T. Baumberger, B. Perrin, B. Caroli, and the scientific program “On n’est pas que des cobayes” [1]
C. Caroli, Physical review E 49, 4973 (1994). which stimulated this study through the participation
[21] J. Gao, W. Luedtke, D. Gourdon, M. Ruths, J. Is- of F.R. and C.P., as well as the French ANR (WAFPI
raelachvili, and U. Landman, The Journal of Physical project: ANR-11-BS04-0030) and NSERC of Canada for
Chemistry B 108, 3410 (2004). funding.
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91, 94 (2015). Author Contributions H.A. performed the
[23] O. Ben-David and J. Fineberg, Physical review letters
106, 254301 (2011). interleaved-book experiments; J.F.B. performed the
[24] I. Etsion and M. Amit, Journal of tribology 115, 406 classical paper friction experiments; T.S., E.R. and
(1993). K.D.-V. developed the theoretical model; C.P. and F.R.
[25] http://www.cetr.com/eng/services/paper.html. designed the study; H.A., T.S., E.R., K.D.-V. and F.R.
[26] J. Crassous, L. Bocquet, S. Ciliberto, and C. Laroche, wrote the manuscript; all the authors discussed the
Europhysics Letters 47, 562 (1999). results and the content of the article.