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WORKSHOP REPORT
CONTACT Christopher M. Sorensen sor@phys.ksu.edu Department of Physics, Kansas State University, Manhattan, KS 66506, USA.
1
Urs Baltensperger, Paul Scherrer Institute, 5232 Villigen, Switzerland; Junji Cao, Chinese Academy of Sciences, Xi’an, 710075, China; Richard Flagan,
Caltech, Pasadena, CA 91125, USA; Y.S. Mayya, Indian Institute of Technology, Mumbai 400 076, India; Yoshio Otani, Kanazawa University, Kanazawa,
Ishikawa 920-1192, Japan; David Pui, Mechanical Engineering, University of Minnesota, Minneapolis, MN 55455, USA; Christopher Sorensen, Kansas State
University, Physics, Manhattan, KS 66506, USA.
2
We thank our very capable note takers Yuli Wang Heinson, William Heinson, and Pai Liu of Washington University, St. Louis.
3
We thank C Y Wu and Pratim Biswas for conceiving this workshop and nurturing its progress. We acknowledge the funding from AAAR.
ß 2019 The Author(s). Published with license by Taylor & Francis Group, LLC.
This is an Open Access article distributed under the terms of the Creative Commons Attribution-NonCommercial-NoDerivatives License (http://creativecommons.org/licenses/by-
nc-nd/4.0/), which permits non-commercial re-use, distribution, and reproduction in any medium, provided the original work is properly cited, and is not altered, transformed,
or built upon in any way.
732 C. M. SORENSEN ET AL.
technology and thereby create a roadmap for future between aerosol properties and the physiological mecha-
research. The grand challenges presented here are nisms that impact human health, extending beyond the
indeed “grand” and represent the most pressing issues commonly used approach of just PM10 or PM2.5 (par-
for both the science and the technology of aerosols. ticulate matter with an aerodynamic diameter smaller
We address both the areas where aerosols are typically than 10 or 2.5 lm, respectively). The community needs
referred to as “bad aerosols” and as “good aerosols”, to develop a methodology that is sufficiently simple and
followed by a summary of the physical, chemical, and cost-effective, including accurate, cost-effective sensors,
biological properties of aerosol that need to be and then realize the potential scientific and societal bene-
addressed to cope with these challenges. fits of networking these sensors and methods.
Measurements are also needed that can evaluate long-
term versus acute health effects in terms of toxicity. All
Environment
of these studies need to be applied to understand the role
The aerosol community needs to develop a quantita- of aerosols on the health of the individual in order to
tive description of aerosols in the present, past, and correlate/associate the links to end points. Finally, the
future, over length scales from indoor and local community must effectively communicate the results of
through the global. This description must deal with these studies to society.
the inherent complexity of aerosols in the environ- The aerosol community needs to develop sound
ment and their multiple and many-dimensional methods to detect and predict the spread of aerosol vec-
impacts, including climate, visibility, ecosystems, as tors of disease. This will enable appropriate agencies to
well as the numerous involved negative and positive take proactive measures to warn or protect the populous.
feedbacks. This requires a better source apportion- To do this, massively distributed, yet affordable, meas-
ment of aerosols, such as discrimination between nat- urement networks based on recent advances in molecu-
ural and anthropogenic aerosols, and quantification of lar assay techniques are needed. Sampling of the ambient
the corresponding radiative forcings via aerosol–radia- aerosols must occur across a wide range of scales and
tion interaction and aerosol–cloud interaction. The environments such as the home, schools, work-place,
latter relates to the number of cloud condensation hospitals, and the surrounding communities.
nuclei and ice nucleating particles (CCN and INP, The aerosol community needs to advance the state-of-
respectively), i.e., particles that are able to form a the-art in sampling, detection, and analysis of exhaled
cloud droplet/ice crystal at the given supersaturation breath biomarkers for disease, to monitor health.
in a cloud. As about 50% of these particles are not
directly emitted but rather formed in the atmosphere
Bioaerosols
from a variety of precursor gases, it is essential to
understand the underlying processes. Research should A grand challenge for the aerosol community is to
give a special focus to the most vulnerable areas, such understand the influence of personal exposure to bioaer-
as the Arctic. osols on long-term health. Important aspects of this chal-
lenge are how to determine personal exposure to
bioaerosols within integrated exposure to indoor and
Health
outdoor agents. We don’t know the dose–response curve
The aerosol community needs to provide mechanistic for various microorganisms in different environments.
links between aerosol chemical and physical properties We also don’t know how modifications in human envi-
with toxicity and biological end points. This will require ronments, such as urban pollution, feedback to alter the
the community to define the most important biological microbes via, for example, evolutionary pressure.
end points. A comprehensive ensemble of measurements Another important question is what role does cumulative
will be required in order to link aerosol properties to exposure to aero-allergens play in chronic inflammation
physiological mechanisms that lead to those end points. leading to other negative health outcomes?
Personal exposure must be differentiated from total inte- The aerosol community needs to understand the
grated ambient concentrations, and dose from exposure. roles of bioaerosols in the environment: the hydro-
Measurements—both indoor and outdoor—need to pro- logic cycle, cloud condensation and ice nucleation,
vide sufficient spatial and temporal resolution to quantify and impacts on ecosystems such as crops, grasslands,
exposure. These should include long-term measurements and forests.
that can be used in connection with epidemiology stud- The aerosol community must seize the future and
ies, and that provide the data needed to establish links prepare for changes in biodiversity due to climate
AEROSOL SCIENCE AND TECHNOLOGY 733
change and evolution of microorganisms. It must Making a desirable material at the lab bench is just
anticipate its primary role for understanding and con- the beginning; the challenge is then the scale-up to
trolling bioaerosols in space vehicles, and lunar or yield commercially significant products. Here the
planetary installations. community must address a key tool that is presently
lacking—the ability to measure aerosol properties,
such as size distribution and temperature, space and
Control technology time resolved, within the production reactor. This
People spend most of their time indoors, and indoor daunting challenge must often contend with high tem-
air pollution is shortening lives world-wide. The aero- perature, chemically reactive, and often corrosive
sol community must provide the means to protect the flows, and mass loadings as high as 10%. Such data
public and ensure that people breathe healthy air. are essential for process control, addressing scale-up
This challenge has multiple dimensions which should challenges, and for computational-fluid-dynamics-
be pursued in parallel. reaction-aerosol coupled modeling for process
Filtration is the dominant method of removing par- optimization.
ticles from indoor air. It is a mature technology, but Finally, we must not forget that the aerosol com-
there are opportunities for improved filters through the munity must be responsible for their science. Hence
use of new materials, and integration into filtration sys- life-cycle analysis, toxicity, and environmental impact
tems of additional functions such as gaseous and bio- analysis of new materials must be performed.
logical pollutant removal. The aerosol community must
explore these opportunities to produce breakthroughs Physics and chemistry
using nontraditional technologies.
The aerosol community must bring together physical
The design of indoor environmental space typically
and chemical experiment and modeling to better
follows slowly-developed codes and practices that do
understand a broad variety of fundamental issues. It is
not incorporate the latest human health studies, or the
important to stress that communication between mod-
latest knowledge on the patterns of indoor and outdoor
elers and experimentalists is essential for rapid and
pollutant sources. Narrowing the gap between engineer-
relevant progress.
ing practice, cutting edge technology, and aerosol sci-
There is a significant need to develop a viable
ence to make smart building engineering and controls a
description of light scattering and absorption by par-
standard practice is a grand challenge in itself.
ticles of any size, shape, and composition. This need
Building occupants have a large degree of control
arises because many ambient aerosols, as well as
over their indoor environment, but because the effects aerosols found in materials manufacturing processes
of air pollution are typically subtle and even imper- are non-spherical and can have complex, heteroge-
ceptible to most occupants, indoor air quality has a neous morphologies, and can even contain multiple
lower priority than it deserves. The aerosol commu- phases. Perhaps the most significant use of such
nity must accept the challenge to create innovative knowledge is to quantify the impacts of aerosols on
programs in education to enhance public awareness. the radiation budget of the Earth and, thereby, deter-
mine aerosol impacts on global warming. This need
Materials applies to other applications including optical remote
sensing of ambient aerosols, especially via satellites,
The aerosol community should aspire to be able to and calculation of atmospheric visibility and visibility
make any material at any scale. A simply stated but impairment. In the manufacturing realm another
daunting goal is to create materials of arbitrary com- important application is for real time, in situ meas-
plexity with tailored properties of composition, size urements of aerosols in process flow streams during
and shape. The ability to tailor, to control, to predict materials production. In this regard, as highlighted in
the results will need the combined efforts of labora- the Materials section of this report, the problem of
tory experimentation and theoretical modeling. The optical diagnostics of aerosols with high mass load-
community should explore and take advantage of ing, on the order of 10%, where multiple scattering
developing artificial intelligence methods for mining leads to confusion, is an important impediment that
the vast parameter space for product synthesis and needs to be overcome.
process development. We should aspire to make stuff Another grand challenge is the need to develop a
that our predecessors never dreamed of. viable understanding of particle nucleation and
734 C. M. SORENSEN ET AL.