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Composites Science and Technology 135 (2016) 106e115

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Composites Science and Technology


journal homepage: http://www.elsevier.com/locate/compscitech

Effect of strain rate and fibre rotation on the in-plane shear response
of ±45 laminates in tension and compression tests
Hao Cui a, *, Daniel Thomson a, Antonio Pellegrino a, Jens Wiegand b, Nik Petrinic a
a
Department of Engineering Science, University of Oxford, Parks Road, Oxford, OX1 3PJ, UK
b
COMPACT Composite Impact Engineering LTD, Manchester, UK

a r t i c l e i n f o a b s t r a c t

Article history: This work focuses on the effect of strain rate and fibre rotation on the in-plane shear properties of
Received 28 June 2016 composite laminates. The effect of fibre rotation on the measured shear properties, was for the first time
Received in revised form experimentally quantified with the comparison between compression and tension tests of the ±45
5 September 2016
laminate samples. Significant increase of shear strength and decrease of final failure strain was observed
Accepted 19 September 2016
Available online 20 September 2016
with the increase in strain rate from 5e-4 1/s to 1300 1/s. The nonlinear shear model was developed to
simulate the large deformation process, in which the fibre orientation was updated as a function of the
in-plane shear strain. The results of this investigation should motivate the updating of procedures for
Keywords:
In-plane shear
experimental characterization as well as analytical and numerical modelling of in-plane shear response
Fibre rotation of laminates.
Rate-dependent © 2016 Elsevier Ltd. All rights reserved.
Hopkinson bar
±45 laminate

1. Introduction once damage has initiated [1,2]. The ±45 laminates yield quite
uniform shear stress distribution over the whole gauge area [7], and
Carbon fibre composite laminates feature high stiffness and provide stable damage evolution for large deformation. However,
strength in fibre orientation, while their elastic moduli as well as the tension test of ±45 exhibit significant fibre rotation [8]. The
strength in transverse direction are relatively weak. Inter-fibre reinforcement fibres get more aligned with the loading axis as the
failure is one of the dominating failure modes for composite lam- shear strain increases during tests, resulting in the overestimation
inates, and significant nonlinearities may occur prior to fracture in of the shear stress, as confirmed with analytical and numerical
composite structures. Considerable nonlinearity of in-plane work [9,10]. The opposite trend may be observed when the
behaviour has been observed in off-axis compression tests of uni- compression loading is applied, and this can be used in comparison
directional laminates, and it has been found to be dependent on the with tension tests to evaluate the influence of fibre rotation on
strain rate [1,2]. The shear properties of laminated composites are measured shear response.
very important for predicting permanent deformation and damage, This paper aims to study the rate-dependence in in-plane
and several models have been developed [3e6]. In this study, the shear, and to reveal the effect of fibre rotation on the laminate
rate dependent in-plane shear properties were characterized using response in both experiments and modelling. The experimental
±45 laminates, in order to gain deeper understanding of their setups and related data processing methods are introduced in
nonlinear deformation behaviour, and to support the development Section 2. The corresponding numerical models of the specimens
of constitutive models for simulation of composites subjected to and the developed constitutive model used to simulate the con-
impact loading. ducted experiments are outlined in Section 3. All results and
The in-plane shear response can be obtained from off-axis discussions are presented in Section 4, followed by concluding
compression/tension tests. Achieving large deformations poses remarks in Section 5.
several challenges, as the deformation process becomes unstable

* Corresponding author.
E-mail address: hao.cui@eng.ox.ac.uk (H. Cui).

http://dx.doi.org/10.1016/j.compscitech.2016.09.016
0266-3538/© 2016 Elsevier Ltd. All rights reserved.
H. Cui et al. / Composites Science and Technology 135 (2016) 106e115 107

2. Experimentation performance on condition that the dynamic equilibrium and strain


homogeneity along the sample gauge section are both established
2.1. Material and specimen during the tests [12,13]. A 0.5 mm-thick cardboard was used to
shape the loading pulse in the dynamic compression test thus
A 2 mm-thick laminate ([0º/90 ]4s) was made of HexPly® IM7/ filtering out undesirable high frequency response of the loading
8552 carbon-epoxy prepreg, a material extensively used in both system to the impact loading imposed by the striker. The relatively
industry and academic research. The laminate has been inspected long tension samples required a considerably longer time than the
using ultra-sound scan to ensure that no large defects or voids were compression samples to reach dynamic equilibrium conditions. For
present. The specimens for tension and compression tests were all that reason, a 3 mm-thick rubber sheet was used as pulse shaper to
manufactured by cutting this laminate at 45 with a water-cooled more gradually ramp up the force applied on samples.
diamond saw. The gauge section of the dog-bone tension samples The samples were coated with a black speckle pattern on a
was shaped and surface finished using a surface-grinding machine. white background, which enabled displacement and strain mea-
The geometry of these samples is shown in Fig. 1, with the same surement across the whole sample surface using digital image
gauge section of 5 mm by 8 mm in both tension and compression correlation (DIC) methodology (in-house [14] and commercial
tests. The tension samples were bonded using 3M Scotch-Weld software GOM Aramis were used). Quasi-static tests were recorded
DP490 adhesive into impedance matched, metallic, threaded end- with a camera at frame rate of 2 FPS. The ultra-high speed camera
sleeves for gripping into the loading rigs. SI-Kirana was used in dynamic tests.
The matrix material of the laminates, 8552 epoxy, was tested in The quasi-static compression tests of 8552 epoxy was done with
compression at different strain rates in this study. The cylindrical the Zwick/Roell Z250 machine at two different loading rate:
samples were cut from the epoxy cast with diameter of 4 mm, and 0.001 mm/s and 0.1 mm/s. Dynamic tests were carried out on the
their thickness was 2 mm. split Hopkinson compression bar with striker velocity of 3e8 m/s.

2.2. Test setup

The Zwick/Roell Z250 screw driven testing machine with 20 KN 2.3. In-plane shear data processing
loading cell was used in quasi-static tests. The displacement
controlled loading rate was 0.01 mm/s. An in-house built Split- The displacement (extension and contraction) across the lami-
Hopkinson-Tension and Compression Bar systems [11] were used nate specimens gauge section and the corresponding strain can be
for dynamic tests (Fig. 2). The striker velocity was approximately evaluated from the images taken during tests by means of the DIC
5 m/s in compression tests, and 11 m/s in tension tests. Strain method. The strain distribution within gauge area is reasonably
gauges were used to acquire the strain history on the split Hop- uniform over the gauge section. The average normal strains in both
kinson bars, from which the force histories applied upon all sam- x and y directions were calculated from the changing of edge length
ples were calculated. These dynamic experiments are considered of the gauge area as:
valid for the purpose of classical characterisation of mechanical
εxx ¼ Dlx =l
x (1)
εyy ¼ Dly ly

where Dlx and Dly are the elongations, while lx and ly are the length
and width of the gauge area in the direction of parallel and
perpendicular to the loading direction. The shear strain is then
calculated as:

g12 ¼ εxx  εyy (2)


This equation is strictly valid only for fibre angles of ±45 ,
and
increasing error is involved with the rotation of fibres in shear
deformation.
The shear stress was calculated considering the change in cross-
section:

F
t12 ¼ ð1 þ εxx Þ (3)
2A

2.4. Correction for fibre rotation

The calculation of the shear stress with Eq (3) is accurate for


small strain conditions, while the fibre rotation gets pronounced
when the strains get large. There is an analytical solution for linear-
elastic materials to estimate the ratio between the shear stress txy
at small strains calculated with Eq (3) and the true shear stress txy
Fig. 1. (a) the geometry and (b) the samples for experiments. [10]:
108 H. Cui et al. / Composites Science and Technology 135 (2016) 106e115

Fig. 2. Hopkinson bar systems for dynamic tests.

  transverse properties were not possible to be evaluated accurately,


t12 ð1  bÞ2 Q11 Q22  Q12
2 þ 4bQ66 ðQ11 þ Q22 þ 2Q12 Þ and were not considered in this study.
f ¼ ¼ Considering each point of the nonlinear portion of the true shear
t12 4mnð1 þ bÞQ66 ½bQ11 þ Q22 þ ð1 þ bÞQ12 
stress-strain curve as fictitiously “linear elastic”, the reduced shear
(4) modulus Q66 decreases with shear strain and is calculated as
follows:
where
.
m ¼ cos q (5a) Q66;i ¼ t12;i g12;i (8)

At each data point i of the small-strain based shear stress-strain


n ¼ sin q (5b)
response. The corrected shear stress comprising fibre rotation is
. then calculated as follows:
b ¼ n2 m2 (5c)
t12 ¼ t12 =f ðQ66 ; qÞ (9)
and q is the fibre orientation. The fibre orientation changes with
shear strain, and is calculated here as:

q ¼ p=4 þ lg12 =2 (6) 3. Numerical modelling

where l is equal to 1 for compression tests and 1 for tension tests. 3.1. Laminate model
The stiffness constants Qij are calculated from material proper-
ties of unidirectional laminates: The tension and compression experiments were simulated
numerically using the finite element method as illustrated in Fig. 3.
Q11 ¼ E11 =ð1  v12 v21 Þ The experimentally acquired boundary conditions were used as
Q12 ¼ Q21 ¼ E11 v21 =ð1  v12 v21 Þ (7) input data for modelling. The laminates were modelled with three
Q22 ¼ E22 =ð1  v12 v21 Þ dimensional 8 node reduced integration solid ‘brick’ element
The material constants in Eq (7) are listed in Table 1. (C3D8R) in Abaqus 6.14, material properties are listed in Table 1.
During large in-plane shear deformation, the moduli in trans- Due to large in-plane shear, the inter-laminar shear stress txz
verse direction, E22, also get degraded. However, the degraded and tyz may also exceed its yielding limit in ±45 laminates,
whereby this transverse shear deformation concentrates at the
resin-rich interface between two layers. To avoid large distortion of
Table 1 bulk elements, the cohesive zone model was used to simulate the
Elastic properties of IM7/8552 laminate [15].
nonlinear deformation in XeZ and YeZ directions. The imple-
E11 162095 MPa mented (as user-defined in Abaqus/Explicit) cohesive law features
E22 9721 MPa very high initial stiffness (1e5MPa/mm) before exceeding its
E33 9721 MPa
reversible limit, to avoid non-physical contribution to the out-of-
G12 4688 MPa
G13 4688 MPa plane deformation. The inter-laminar cohesive stress after
G23 5000 MPa yielding is determined using experimentally determined in-plane
v12 0.362 shear behaviour.
v13 0.362 All simulations were done using Abaqus/Explicit. The quasi-
v23 0.3
static simulation was carried out using the true density for a long
H. Cui et al. / Composites Science and Technology 135 (2016) 106e115 109

verify this functionality in commercial software package Abaqus


6.14. As sketched in Fig. 4, the local material orientation was not
updated for the shear deformation modes A and C, although these
modes dominate in off-axis loaded laminates, with one of them
prevailing depending on the alignment of the element topology
with respect to the fibre orientation. As a result, in this study, the
fibre rotation due to shear deformation was taken into account
within the constitutive model, in order to simulate accurately the
conducted experiments. A user defined material model was
developed to account for the change of fibre rotation due to shear
deformation. A user subroutine VUMAT was written, allowing for
the continuous calculation of the fibre orientation during simula-
tion. The fibre orientation is calculated as follows:

1  εxx
q ¼ arctan (10)
1  εyy

where εxx is the strain along loading axis and εyy is the strain
normal to the loading axis this equation provided very close esti-
Fig. 3. Numerical models for (a) compression tests and (b) tension tests. mation of fibre rotation in comparison to the Eq (6) used in pro-
cessing experimental results.
Within the VUMAT, the strain tensor in global coordinates ~ε was
time to avoid any inertia effect generated during rapid fracture updated first. The following equation was used to compute the
processes. strain in local material coordinates

3.2. Constitutive model


ε ¼ RðqÞ$~ε (11)
T
The local material coordinates should be updated during anal- where ε ¼ ½ε11 ; ε22 ; ε33 ; ε12 ; ε23 ; ε13  is the strain tensor in local
ysis in order to account for the rotation of fibres due to shear material system, and ~ε is the strain in the global system. The rota-
deformation. A single element benchmark study was carried out to tion matrix RðqÞ is

Fig. 4. Fibre rotation during shear deformation of unidirectional laminate: the patterns indicate fibre orientation, and the 1e2 axis is the local material coordinate system used FEM.
110 H. Cui et al. / Composites Science and Technology 135 (2016) 106e115

2 3
c2 s2 0 2s1 c1 0 0
6 s2 c2 0 2s1 c1 0 07
6 7
6 0 0 1 0 0 07
RðqÞ ¼ 6
6 s1 c1
7 (12)
6 s1 c 1 0 c 2  s2 0 07 7
4 0 0 0 0 c1 s1 5
0 0 0 0 s1 c1

where c2 ¼ c21 , s2 ¼ s21 , s1¼sin(q), c1¼cos(q). The normal stress in the


local material system is then updated as follows

sij ¼ Cij εij ði ¼ 1; 2; 3; j ¼ 1; 2; 3Þ (13)

where Cij is the stiffness tensor calculated as follows

c ¼ E11E22  E11 E33v223 .2E22 E33 v13 v23  E22 E33 v213
C11 ¼ E22  E33 v223 E11 2
c
C12 ¼ C21 ¼ ðE22 v12 þ E33 v13 v23 ÞE11 E22 =c
C13 ¼ C
31 ¼ ðv12 v23 þ v13.ÞE11 E22 E33 =c (14)
C22 ¼ E11  E33 v213 E22 2
c
C23 ¼ C
32 ¼ ðE v
11 23 þ E v
22 12.v13 ÞE22 E33 =c
C33 ¼ E11  E22 v212 E22 E33 c

The shear stresses t23 and t13 were updated as follows

t23 ¼ G23 g23


(15)
t13 ¼ G13 g13
The in plane shear stress t12 was controlled by the master
curves obtained from tension/compression tests at different
loading rates. These master curves were read into the VUMAT at the
beginning of the computation, and the exact shear stress was
determined by interpolation between two neighbouring data
points of the curve.
After update of the stress state in the local coordinates system,
Fig. 5. (a) Failure process in quasi-static tension tests; (b) failure process in quasi-static
the stress in the global coordinates can then be calculated as
compression; (c) load-displacement curves.
follows

~ ¼ RðqÞ$s
s (16) the dynamic tests produced similar macroscopic failure pattern as
that in quasi-static tests. Detailed investigation on the failure
mechanisms in tension tests will be presented in Section 4.5. The
cross-section of compression samples in quasi-static tests was
4. Results and discussions analysed and illustrated in Fig. 7. Although the delamination
seemed to trigger the final failure of the ±45 laminates in both
4.1. Force-displacement tension and compression load, the number of delamination planes
in compression tests was much less than that in tension tests. Be-
The edge surface of the specimens was monitored in quasi-static sides, the number of in-plane cracks in compression tests was
tests, and the representative damage evolution processes were considerably smaller than in tension. This could be due to the fact
depicted in Fig. 5 at each stage of the load-displacement curves. In that the high hydro-static stress in compression experiments might
tension tests, there is no visible damage occurring at the moment of have prevented the opening of cracks and growth of voids within
yielding. The load dropped slightly after yielding, and micro cracks the epoxy matrix.
started to emerge at displacement of 0.6 mm. The load carried by In the dynamic tests, the force at both ends of the sample,
the specimen then kept growing causing an increasing number of calculated from the signal on the input bar and output bar [13], are
micro cracks in each ply to appear. There were no delamination plotted in Fig. 8. The force on one end of the specimen is very
cracks observed until the extension of about 1.5 mm was reached, similar to that on the other, showing that dynamic equilibrium
which was followed by catastrophic failure. In compression testing, conditions were achieved from the early stage during experiments.
the stiffness appears higher because of the shorter length of the After an initial ramp-up period where the strain rate rapidly in-
sample. There were not many visible cracks on the edge of creases, a constant strain rate is reached long before failure. Hence,
compression samples, until the contraction of 0.9 mm was reached the sample and test setup produced valid measurement of the
when delamination between layers appeared. nonlinear deformation response.
Samples after tension and compression tests in different loading
rates are all presented in Fig. 6. The delamination between plies of
different angles has resulted in the complete break of tension, and
H. Cui et al. / Composites Science and Technology 135 (2016) 106e115 111

Fig. 6. Samples after tests (a) quasi-static tension; (b) quasi-static compression; (c) dynamic tension; (d) dynamic compression.

Fig. 7. Failure of compression samples in quasi-static tests.

4.2. In-plane shear response

The original shear stress, calculated directly with Eq (3) is


plotted in Fig. 9 as a function of shear strain. In the quasi-static
tests, the shear stress increased with rising tangential shear stiff-
ness after yielding, similar to tests reported in literature [8,9,16,17].
Both tension and compression tests produce quite similar shear
response at small strain stage, although the shear stress from
compression tests appears slightly higher than that in tension. The
shear stress obtained from dynamic tests exhibits a certain degree
of softening process after the elastic phase and then the stress
plateaued in compression tests and increased slightly in tension
tests. It is interesting to identify that the results from tension and
compression start to deviate from each other after shear strain
larger than 10% (see the arrows in Fig. 9). Considering the fact that
the fibres rotate in opposite directions between compression and
tension tests, this study indicate that the shear stress are reason-
ably accurate for strain smaller than 10%. This observation corre-
lated nicely with the studies on V-notched cross-ply specimens
[18].

Fig. 8. The equilibrium and shear strain in (a) dynamic compression and (b) dynamic
4.3. Rate dependence of corrected shear response tension tests.

The analytical solution for estimating the effect of fibre rotation


was used in this study to approximate the true in-plane shear and compression tests. The final failure strain in dynamic tests is
behaviour from the original data. The shear stresses look consid- smaller than that in quasi-static ones. The shear stress obtained
erably different from the apparent ones after the correction. In from compression tests is slightly higher than that from tension
particular there was no significant strain hardening beyond the tests. This may indicate the dependence of in-plane shear response
yield, as shown in Fig. 10. The shear strength increased significantly upon hydrostatic pressure [19,20] and thus caused different
with the strain rate, with similar trends observable in both tension deformation and failure mechanisms, as discussed in Section4.1.
112 H. Cui et al. / Composites Science and Technology 135 (2016) 106e115

Fig. 9. The original stress from tension and compression tests in (a) quasi-static and Fig. 10. Corrected shear from (a) tension tests and (b) compression tests.
(b) dynamic rate.

enforcement mechanisms for the avoidance of unphysical defor-


4.4. Evaluation of experimental results with FEM mation between neighbouring elements along fibre direction. Both
factors tend to trigger concentration of plastic softening deforma-
In-plane shear model at different strain rate for each test tion, and caused premature dropping of the loading capacity.
configuration was generated by averaging the experimental results. The simulation without updating fibre orientation, using small-
All tests were simulated with both the small-strain based and strain based shear stress, was also evaluated in this study. It pro-
corrected shear properties within updating of fibre orientation vided good prediction in quasi-static compression tests. However,
during computation. The fibre orientation does change with in- noticeable deviation from experimental results was shown in all
plane shear deformation and can be determined kinematically tension simulations. This deviation may be induced by several
regardless of the material constitutive behaviour. For the purpose of factors not accounted for, such as the nonlinearity in transverse
representing existing modelling methods, the small-strain based direction and rotation of fibre. Not taking into account the fibre
shear stress calculation model was also employed to simulate all orientation in constitutive models may compensate the fact that
these tests without updating fibre orientation. the contribution from fibre rotation has been included in the
All predicted force-displacement curves were compared with original shear response, making these simulations more accurate
experiments in Fig. 11. When the fibre orientation was updated than above mentioned ones.
during simulation, the original shear stress resulted in significant For the simulations with corrected shear properties and upda-
overestimation of the load in large strain stage. For tension tests, ted fibre orientation during computation, excellent correlations
the load from simulations was higher than experimental value even were achieved between simulations and experiments. This study
at the small displacement stage. The fibre rotation has contributed did show that taking into account the fibre rotation is necessary to
to the originally determined shear properties, and the updating of characterise experimentally more closely the true in-plane shear
material orientation may bring in additional fibre rotation, result- behaviour from uniaxial loading the ±45 laminated samples, as
ing in predicted load higher than the experimental value. Signifi- well as that updating of fibre orientation during simulation would
cant oscillations were observed in dynamic compression improve the accuracy of numerical models. Further improvement is
simulations with updating fibre orientation. Because the fibre achievable by relaxing the assumption adopted in this study that
rotation in compression decreased the element stiffness in global the transverse properties of the laminates remain undamaged.
coordinates at the early stage of deformation. Besides, current When comparing the results against constitutive models readily
commercial finite element codes are not provided with available in commercial simulation packages, it is clear that not
H. Cui et al. / Composites Science and Technology 135 (2016) 106e115 113

Fig. 11. Comparison of force-displacement curves from experiments and simulations, (a) quasi-static tension; (b) quasi-static compression; (c) dynamic tension; (d) dynamic
compression.

taking into account the rotation of fibre not only results in an in-
crease in the apparent stress calculated using small strain theory,
but it also causes the apparent reduction in stiffness in the original
fibre orientation and a change in the in-plane distribution of
stresses. With the growing demand for more accurate tools for
predictive modelling of composite systems and structures, the fibre
rotation should be considered both in experiments and in numer-
ical simulations, such that the true in-plane shear properties could
be utilised. Further accounting for nonlinearities in the transverse
direction, should lead to an even more accurate characterisation
and modelling of the intrinsic material behaviour.

4.5. Strain rate effect on failure mechanisms

The uniaxial compression test results on the matrix material are


shown in Fig. 12. It can be observed that the stiffness prior to
yielding and the yielding stress increased considerably with the
strain rate, very similar to the rate-dependence observed in ±45 Fig. 12. True stress-true strain curves from uniaxial compression of 8552 epoxy at
laminates. The failure strain in both pure epoxy samples and the different strain rates.
±45 laminates decreased with the strain rate. Hence, the rate-
dependence in the in-plane shear deformation may be dominated
by the epoxy matrix. Fig. 12.
The post-yielding response was different between the epoxy The complete failure of ±45 laminates was caused by the
matrix and the laminate. The stress increased considerably in the delamination crack between layers on shown on the left side of
plastic deformation stage in the compression tests of matrix; Fig. 13. The delamination fractures initiated as cracks within the
however, the in-plane shear stress in Fig. 10 kept decreasing after epoxy matrix in dynamic tests, and no significant fibre-matrix
yielding. The failure surface of tension samples were investigated interface failure was observed. Shear cusps with orientation
as shown in Fig. 13. The dense distribution of in-plane micro cracks perpendicular to the fibres were observed. Their size varied
was observed on the free surface of the laminates. The initiation considerably, possibly controlled by the volume fraction of the
and growth of the micro cracks decreased the loading capacity of matrix confined by fibres. In quasi-static tests, shear cusps were
epoxy matrix at micro scale, and resulted in the decrease of the in- mainly formed within matrix pockets of sufficient volume.
plane shear stress at homogenized ply level. Noticeable debonding between fibres and matrix was also identi-
Micro cracks at the surface ply took form of shear cusps with fied. The strength of fibre-matrix interface may increase at higher
sharp edges in dynamic tests. The epoxy matrix was more severely loading rates above that of the epoxy matrix, which caused the
distorted before the formation of shear cusps in quasi static tests, migration of failure mechanisms from the interface into the matrix
due to the larger failure strain in lower loading rate as shown in itself.
114 H. Cui et al. / Composites Science and Technology 135 (2016) 106e115

Fig. 13. The deformation and fracture of tension samples from (a) dynamic tests and (b) quasi-static tests.

5. Conclusions Acknowledgements

The in-plane shear behaviour was characterised with ±45 The authors would like to acknowledge Rolls-Royce plc, for their
laminates loaded in both compression and tension at two distinct continuing support through the Solid Mechanics University Tech-
loading rates. The split Hopkinson bar system and high-speed nology Centre at the University of Oxford.
camera enabled the successful measurement of the shear defor-
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