Professional Documents
Culture Documents
Abstract
A dielectric barrier discharge in a 2 mm air gap was studied. The experiments show that the
mesh electrode and PET film really make the discharge looking homogeneous. The breakdown
onset voltage in the case of a mesh electrode and PET film is 6.4 kV, considerably lower than
8 kV, the breakdown voltage in the usual case using two spherical electrodes. The field
calculations show that even with this much lower voltage the gap field in the region very close
to the PET film is enhanced to a value near the breakdown field in the usual case. It may be this
field enhancement that initiates a corona discharge which provides seed electrons, leading to the
breakdown of the whole air gap at a lower voltage. A lower voltage applied to the gap means a
lower averaged field over the gap. Because the development of an electron avalanche is very
sensitive to the electric field, a small decrease in the field will depress the avalanche
significantly, preventing a homogeneous discharge from transiting to filament discharge. This
may be the reason why a mesh electrode and PET film make the discharge look homogeneous.
(Some figures in this article are in colour only in the electronic version)
1. Introduction plates made from different materials he got all the homoge-
neous discharges in air. It seems the mesh electrode plays
Plasma surface modification has many advantages over tra- a more important role in obtaining a homogeneous discharge
ditional chemical methods [1] and a homogeneous discharge than the dielectric plate. The role of the mesh was not yet fully
at atmospheric pressure is the most desirable plasma source. understood. While Buchta believed that the higher electrical
However, the difficulties in realizing a homogeneous discharge resistance of the mesh compared with the electrode may play
rather than a filamentary discharge in atmospheric air have seri- an important role [5], Fang proposed that the corona discharge
ously hindered plasma surface modification from its industrial around the wire mesh before breakdown of the gap is impor-
applications. In order to realize a homogeneous discharge, tant [4]. In this paper the influence of wire mesh electrodes on
people have tried to use many methods in which there is one DBD in air at atmospheric pressure is studied.
thing in common: that is, at least one electrode is covered with
a dielectric plate. This dielectric was introduced to limit dis- 2. Experimental set-up
charge current and the gas discharge with such a dielectric is
called a dielectric barrier discharge (DBD). Except for current The experimental set-up is shown in figure 1 and is similar
limitation, other possible influences of the dielectric barrier on to that used by Fang [3]. The air gap was kept at 2 mm and
gas discharge have been suggested. Okazaki found that when powered by a high voltage ac source of 50 Hz. For comparison
two metal wire meshes are used as electrodes that are covered two kinds of dielectric barrier electrodes were used. The first
by a polyethylene terephthalate (PET) plate and powered by a one was a plane electrode covered by a quartz plate (plane elec-
50 Hz line power source, a stable homogeneous discharge in trode and quartz) and the second one was a wire mesh electrode
argon, air or nitrogen is always observed, and he believed this covered by a PET plate (mesh electrode and PET). The plane
homogeneous discharge to be an atmospheric pressure glow electrode and quartz is a traditional dielectric barrier electrode.
discharge (APGD) [2]. He did not give any explanation why The electrode is 50 mm in diameter and made from aluminium.
it makes a homogeneous discharge in air possible. Using the The quartz plate is 90 mm in diameter and 1 mm in thickness.
same mesh electrodes as Okazaki, Fang tried to use dielectric As for the mesh electrode and PET, all parameters are the same
plates 0.1 mm in thickness and made from ceramic [3], PET as that in Fang’s experiments. The mesh electrode is 50 mm
and PTFE (polytetrafluoroethylene) [4]. With these dielectric in diameter and made from a #325 wire mesh with the wire
(a)
(b)
(c)
Figure 2. Mesh electrode together with the PET film stuck on a
quartz plate. Figure 3. DBD in a 2 mm air gap when the discharge begins.
(a) The homogeneous looking discharge, (b) the applied voltage and
discharge current and (c) the Lissajous figure of the discharge.
0.03 mm in diameter. The PET plate is of a thickness of 0.1 mm
and an area of 64 mm ×64 mm. In order for the soft mesh elec-
(0.5 s exposure time) from SONY. It can be seen on the image
trodes to be in good contact with the PET plate and to be well
that the discharge is radially homogeneous and covers the entire
parallel with each other, the mesh electrode together with the
surface of the electrode. Figures 3(b) and (c) are the current
PET plate was stuck on the quartz plate, as shown in figure 2.
trace together with the applied voltage and Lissajous figure,
The voltage applied to the electrodes was measured with
respectively. As Va rose up a little bit, the discharge noise got
a voltage divider which is composed of two resistors of
louder and the discharge light a little bit more intensive. Many
75 M(R1 ) and 59 k(R2 ). The discharge current and its
discharge filaments could be clearly observed in the gap and
transported charge were measured by placing a 50 resistor (r)
and a 47.5 nF capacitor (C0 ) between the bottom electrode and more current pulses were recorded as shown in figure 4.
ground, respectively. The waveforms of the applied voltage As is known, DBD is often composed of many discharge
and discharge current were recorded with a digital oscilloscope filaments whose development occurs in some tens of nanosec-
TDS-3034B (300 MHz, 2.5 GS s−1 ) from Tektronix. The onds; the best way to be sure that they do not develop is to take a
Lissajous figure was obtained by plotting the applied voltage picture with 10 ns exposure time [6]. There is another method
over time on the x-axis versus the transported charge on of distinguishing between filamentary discharge and homoge-
the Y -axis on the screen of a digital oscilloscope HP54512B neous discharge, by using two figures [2]: the Lissajous figure
(100 MHz, 1 GS s−1 ) from Hewlett Packard. of voltage-charges and the current pulse shapes. While a fila-
mentary discharge is composed of a number of current pulses
per half-voltage cycle and its Lissajous figure is drawn as a par-
3. Results and discussions allelogram, a homogeneous discharge is characterized by a sin-
gle current pulse per half-voltage cycle and its Lissajous figure
3.1. Discharge mode
appears as only two voltage lines, the top line and the bottom
In our experiment the voltage applied to the mesh electrode line of the parallelogram, because the traces of the two vertical
and PET film was manually increased very slowly. When the charges lines jump back and forth within so short a time of only
applied voltage Va rose to 6.6 kV (peak value), discharge began one current pulse that they can hardly be observed. Although
and some noise could be heard, but the intensity of the light the discharge shown in figure 3(a) looks homogeneous, it is
emitted from the discharge gap was so weak that it could be a filamentary discharge rather than a real homogeneous dis-
observed by naked eyes only in a dark room. Figure 3(a) is charge according to the Lissajous figure shown in figure 3(c)
the image of discharge taken with a CCD camera DSC-F707 and the current pulse shapes shown in figure 3(b).
846
Influence of wire mesh electrodes on dielectric barrier discharge
847
X Wang et al
45
non-homogeneous discharge.
30
4. Conclusion
15 The mesh electrode and PET film really make discharge
in a 2 mm air gap look homogeneous. The breakdown
0 onset voltage in case of a mesh electrode and PET film is
0.00 0.05 0.10 0.15 0.20 6.4 kV, considerably lower than 8 kV, the breakdown voltage
Z (mm) in the usual case using two spherical electrodes. The field
calculations show that even with this much lower voltage the
Figure 5. The electric field in a 2 mm air gap. gap field in the region very close to the PET film is enhanced
to a value near the breakdown field in the usual case. It may
in the central part of the air gap. Figure 5 is the field distribution be this field enhancement that initiates a corona discharge
along the Z-axis, the axis of the electrodes. For comparison, which provides seed electrons, leading to the breakdown of
the field in the case of a plane electrode and 0.1 mm PET film the whole air gap at a lower voltage. A lower voltage applied
was also calculated and plotted in figure 5. to the gap means a lower averaged field over the gap. Since
Z = 0 and Z = 0.1 mm are the electrode–PET interface the development of an electron avalanche is very sensitive to
and PET–air gap interface, respectively. In contrast to the the electric field a small decrease in the field will depress the
uniform field in the case without using a mesh electrode, the avalanche significantly, preventing a homogeneous discharge
field in the case using a mesh electrode is distorted. In the air from transiting to filament discharge. This may be the reason
gap (Z 0.1 mm), the field in the region very close to the PET why a mesh electrode and PET film make the discharge look
film is enhanced to 37.5 kV cm−1 . It is important to note that homogeneous.
37.5 kV cm−1 is close to 40 kV cm−1 , the breakdown field of
the 2 mm air gap in the usual case where the breakdown voltage
is 8 kV as mentioned above. It may be this field enhancement Acknowledgment
that first initiates a corona discharge in this region and then the
corona discharge provides seed electrons for the breakdown of This work was supported by the National Natural Science
the whole air gap. As we know [9], a self-sustained discharge Foundation of China under contract 50537020.
is formed under condition of γ [exp(αd) − 1] = 1, that is
also the breakdown condition for a homogeneous discharge
References
in a gap of uniform field. In usual cases, γ is coefficient of
electron emission from the cathode. In the case of a DBD, [1] Roth J R 1995 Industrial Plasma Engineering (Bristol:
γ is related to the processes of providing seed electrons such Institute of Physics Publishing)
as desorption of electrons from the dielectric barrier [10]. If [2] Okazaki S et al 1993 Appearance of stable glow discharge in
the corona discharge provides additional seed electrons, γ air, argon, oxygen and nitrogen at atmospheric pressure
using a 50 Hz source J. Phys. D: Appl. Phys. 26 889–92
could be qualitatively considered to have increased and the [3] Fang Z et al 2003 Surface modification of
α required for breakdown can be lowered, which means a polytetrafluoroethylene film using the atmospheric pressure
lowered breakdown voltage. glow discharge in air J. Phys. D: Appl. Phys. 36 2980–5
Although Fang and the authors all believe that the role [4] Fang Z 2005 Research on atmospheric pressure glow
of the mesh electrode is to produce corona discharges, it is discharge and its applications to surface modification of
materials PhD Dissertation Xi’an Jiaotong University
different in explanation of the way the mesh plays. While [5] Buchta J et al 2000 Comparison of ozone production in
our explanation is that a corona discharge produced in the air atmospheric pressure glow discharge and silent discharge
gap provides seed electrons, Fang’s explanation [4] is that the Czech. J. Phys. (Suppl. 3) 50 273–6
corona discharge is produced around the fine wire of the mesh [6] Mashines F et al 1998 Experimental and theoretical study of a
electrode, and the PET film covering the mesh is charged from glow discharge at atmospheric pressure controlled by a
dielectric barrier J. Appl. Phys. 83 2950–7
its surface contacting the mesh by the corona discharge, leading [7] Mangolini L et al 2004 Effect of current limitation through the
to the electrons emitting from the other surface of the PET film dielectric in atmospheric pressure glows in helium J. Phys.
into the air gap as seed electrons. D: Appl. Phys. 37 1021–30
The field calculations show that a right choice of mesh [8] Zhang R Y et al 2003 High-voltage Testing Technology
and dielectric plate is important. The dielectric plate should (Beijing: Press of Tsinghua University)
[9] Raizer Y P 1991 Gas Discharge Physics (Berlin: Springer)
not be thicker than 0.1 mm, otherwise the enhancement of gap [10] Golubovskii Y B et al 2002 Influence of interaction between
field in the region close to the dielectric would be too small to particles and dielectric surface over a homogeneous barrier
influence the discharge. That is the reason why the dielectric discharge in nitrogen J. Phys. D: Appl. Phys. 35 751–61
848