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INSTITUTE OF PHYSICS PUBLISHING PLASMA SOURCES SCIENCE AND TECHNOLOGY

Plasma Sources Sci. Technol. 15 (2006) 845–848 doi:10.1088/0963-0252/15/4/030

Influence of wire mesh electrodes on


dielectric barrier discharge
Xinxin Wang, Haiyun Luo, Zhuo Liang, Ting Mao and Ruili Ma
Department of Electrical Engineering, Tsinghua University, Beijing 100084, People’s Republic of China
E-mail: wangxx@ tsinghua.edu.cn

Received 6 February 2006, in final form 10 August 2006


Published 26 September 2006
Online at stacks.iop.org/PSST/15/845

Abstract
A dielectric barrier discharge in a 2 mm air gap was studied. The experiments show that the
mesh electrode and PET film really make the discharge looking homogeneous. The breakdown
onset voltage in the case of a mesh electrode and PET film is 6.4 kV, considerably lower than
8 kV, the breakdown voltage in the usual case using two spherical electrodes. The field
calculations show that even with this much lower voltage the gap field in the region very close
to the PET film is enhanced to a value near the breakdown field in the usual case. It may be this
field enhancement that initiates a corona discharge which provides seed electrons, leading to the
breakdown of the whole air gap at a lower voltage. A lower voltage applied to the gap means a
lower averaged field over the gap. Because the development of an electron avalanche is very
sensitive to the electric field, a small decrease in the field will depress the avalanche
significantly, preventing a homogeneous discharge from transiting to filament discharge. This
may be the reason why a mesh electrode and PET film make the discharge look homogeneous.
(Some figures in this article are in colour only in the electronic version)

1. Introduction plates made from different materials he got all the homoge-
neous discharges in air. It seems the mesh electrode plays
Plasma surface modification has many advantages over tra- a more important role in obtaining a homogeneous discharge
ditional chemical methods [1] and a homogeneous discharge than the dielectric plate. The role of the mesh was not yet fully
at atmospheric pressure is the most desirable plasma source. understood. While Buchta believed that the higher electrical
However, the difficulties in realizing a homogeneous discharge resistance of the mesh compared with the electrode may play
rather than a filamentary discharge in atmospheric air have seri- an important role [5], Fang proposed that the corona discharge
ously hindered plasma surface modification from its industrial around the wire mesh before breakdown of the gap is impor-
applications. In order to realize a homogeneous discharge, tant [4]. In this paper the influence of wire mesh electrodes on
people have tried to use many methods in which there is one DBD in air at atmospheric pressure is studied.
thing in common: that is, at least one electrode is covered with
a dielectric plate. This dielectric was introduced to limit dis- 2. Experimental set-up
charge current and the gas discharge with such a dielectric is
called a dielectric barrier discharge (DBD). Except for current The experimental set-up is shown in figure 1 and is similar
limitation, other possible influences of the dielectric barrier on to that used by Fang [3]. The air gap was kept at 2 mm and
gas discharge have been suggested. Okazaki found that when powered by a high voltage ac source of 50 Hz. For comparison
two metal wire meshes are used as electrodes that are covered two kinds of dielectric barrier electrodes were used. The first
by a polyethylene terephthalate (PET) plate and powered by a one was a plane electrode covered by a quartz plate (plane elec-
50 Hz line power source, a stable homogeneous discharge in trode and quartz) and the second one was a wire mesh electrode
argon, air or nitrogen is always observed, and he believed this covered by a PET plate (mesh electrode and PET). The plane
homogeneous discharge to be an atmospheric pressure glow electrode and quartz is a traditional dielectric barrier electrode.
discharge (APGD) [2]. He did not give any explanation why The electrode is 50 mm in diameter and made from aluminium.
it makes a homogeneous discharge in air possible. Using the The quartz plate is 90 mm in diameter and 1 mm in thickness.
same mesh electrodes as Okazaki, Fang tried to use dielectric As for the mesh electrode and PET, all parameters are the same
plates 0.1 mm in thickness and made from ceramic [3], PET as that in Fang’s experiments. The mesh electrode is 50 mm
and PTFE (polytetrafluoroethylene) [4]. With these dielectric in diameter and made from a #325 wire mesh with the wire

0963-0252/06/040845+04$30.00 © 2006 IOP Publishing Ltd Printed in the UK 845


X Wang et al

(a)

Figure 1. Schematic diagram of the experimental set-up.

(b)

(c)
Figure 2. Mesh electrode together with the PET film stuck on a
quartz plate. Figure 3. DBD in a 2 mm air gap when the discharge begins.
(a) The homogeneous looking discharge, (b) the applied voltage and
discharge current and (c) the Lissajous figure of the discharge.
0.03 mm in diameter. The PET plate is of a thickness of 0.1 mm
and an area of 64 mm ×64 mm. In order for the soft mesh elec-
(0.5 s exposure time) from SONY. It can be seen on the image
trodes to be in good contact with the PET plate and to be well
that the discharge is radially homogeneous and covers the entire
parallel with each other, the mesh electrode together with the
surface of the electrode. Figures 3(b) and (c) are the current
PET plate was stuck on the quartz plate, as shown in figure 2.
trace together with the applied voltage and Lissajous figure,
The voltage applied to the electrodes was measured with
respectively. As Va rose up a little bit, the discharge noise got
a voltage divider which is composed of two resistors of
louder and the discharge light a little bit more intensive. Many
75 M(R1 ) and 59 k(R2 ). The discharge current and its
discharge filaments could be clearly observed in the gap and
transported charge were measured by placing a 50  resistor (r)
and a 47.5 nF capacitor (C0 ) between the bottom electrode and more current pulses were recorded as shown in figure 4.
ground, respectively. The waveforms of the applied voltage As is known, DBD is often composed of many discharge
and discharge current were recorded with a digital oscilloscope filaments whose development occurs in some tens of nanosec-
TDS-3034B (300 MHz, 2.5 GS s−1 ) from Tektronix. The onds; the best way to be sure that they do not develop is to take a
Lissajous figure was obtained by plotting the applied voltage picture with 10 ns exposure time [6]. There is another method
over time on the x-axis versus the transported charge on of distinguishing between filamentary discharge and homoge-
the Y -axis on the screen of a digital oscilloscope HP54512B neous discharge, by using two figures [2]: the Lissajous figure
(100 MHz, 1 GS s−1 ) from Hewlett Packard. of voltage-charges and the current pulse shapes. While a fila-
mentary discharge is composed of a number of current pulses
per half-voltage cycle and its Lissajous figure is drawn as a par-
3. Results and discussions allelogram, a homogeneous discharge is characterized by a sin-
gle current pulse per half-voltage cycle and its Lissajous figure
3.1. Discharge mode
appears as only two voltage lines, the top line and the bottom
In our experiment the voltage applied to the mesh electrode line of the parallelogram, because the traces of the two vertical
and PET film was manually increased very slowly. When the charges lines jump back and forth within so short a time of only
applied voltage Va rose to 6.6 kV (peak value), discharge began one current pulse that they can hardly be observed. Although
and some noise could be heard, but the intensity of the light the discharge shown in figure 3(a) looks homogeneous, it is
emitted from the discharge gap was so weak that it could be a filamentary discharge rather than a real homogeneous dis-
observed by naked eyes only in a dark room. Figure 3(a) is charge according to the Lissajous figure shown in figure 3(c)
the image of discharge taken with a CCD camera DSC-F707 and the current pulse shapes shown in figure 3(b).

846
Influence of wire mesh electrodes on dielectric barrier discharge

where t0 is the moment of the initial breakdown; Cd and Cg


are the equivalent capacitors of the dielectric and gas gap,
respectively. In our experiments, Cg equals 8.7 pF for a 2 mm
air gap; Cd is 33.6 pF for two 1 mm quartz plates (εr = 3.87)
and 328 pF for two 0.1 mm PET plates (εr = 3.77).
For a homogeneous discharge, Vg could be calculated with
the formula

Vg (t) = Va (t) − Vd (t) = Va (t) − Qd (t)/Cd , (3)

where Vd and Qd are the voltage applied to Cd and the


(a) transported charge from the discharge, respectively. Qd could
be obtained by integration of the measured current over time [6]
or directly measured with C0 as shown in figure 1 [7]. Vb could
be easily determined by the abruptly falling point on the curve
of the obtained Vg (t). The Lissajous figure could also be used
(b) to determine Vb if it is a homogeneous discharge because the
breakdown points are very easy to find in the figure.
Figure 4. DBD in a 2 mm air gap when Va is a little bit higher than
It is impossible to determine a breakdown voltage Vb
6.6 kV. (a) The applied voltage and discharge current and
(b) filamentary discharge. for the whole gas gap in our experiments since it is a
filamentary discharge and the breakdown of the gas gap
happens localizedly, randomly and independently. In this case,
If the mesh electrode and PET film were replaced by
only Vb0 for the initial breakdown could be determined.
a plane electrode and quartz, the discharge behaviour was
It is important to find that Vb0 for a 2 mm air gap, in the
different. First, a higher applied voltage, as high as 9.7 kV,
case of a mesh electrode and PET film, is 6.4 kV, considerably
was needed to ignite the discharge. Second, more current
lower than that in the usual case. According to the IEC standard
pulses with a little bit lower amplitude were recorded. At
of discharge gap issued in 1960 [8], the breakdown voltage of
the same time, more filaments in the gap were observed. In
a 2 mm air gap in between two spherical electrodes 50 mm
order to figure out the role of the PET film, more experiments
in diameter is 8 kV for ac, dc and negative impulse voltage.
were conducted in which mesh electrodes and quartz and a
It is also important to notice that Vb0 for a 2 mm air gap in
plane electrode and PET film were used. The results were
very similar to that obtained with a plane electrode and quartz. case of plane electrode and quartz is 7.7 kV, much higher
In summary, the mesh electrode and PET film really make than that in the case of a mesh electrode and PET film and
discharge look homogeneous if the applied voltage does not very close to that in the usual case. We believe that it is
significantly exceed the initial breakdown voltage. However, this lowering of Vb0 in the case of the mesh electrode and
this homogeneous looking discharge is still a filamentary PET film that makes the discharge more homogeneous. As
discharge. This result is different from that of Okazaki and is well known [9], the development of an electron avalanche
Fang who obtained a homogeneous discharge under the same in a uniform electric field could be quantified by exp(αd),
experimental conditions as ours. The reason for the difference where α is the coefficient of electron impact ionization and d
is not yet known and maybe there exists some imperfections is the gap distance. Furthermore, α increases exponentially
in our mesh electrode and PET film. with the electric field. Thus, the development of an electron
avalanche is very sensitive to the electric field and a small
decrease in the field will depress the avalanche significantly,
3.2. Breakdown voltage of the gas gap preventing a homogeneous discharge from transiting to a
In the case of a DBD, the discharge is in repetitive mode, filament discharge. The lower the Vb0 , the lower the electric
and the residualy charged particles and metastable atoms or field in which electron avalanches develop, and the more
molecules from the previous discharge will influence the next homogeneous is the discharge. The experimental results from
breakdown. So, we define here two breakdown voltages. The Fang support this conclusion. When a homogeneous discharge
first one is the breakdown onset voltage Vb0 for the initial was obtained in Fang’s experiment using a mesh electrode and
breakdown of the gas gap and the second one is the breakdown PET film, the minimum voltage applied to a 2 mm air gap
voltage Vb for the repetitive discharge mode. In order to is 6.1 kV, lower than that (6.6 kV) in our experiment when
determine the breakdown voltage of a gas gap, it is necessary filamentary discharge was obtained.
to know Vg , the voltage applied to this gap. Although Vg could
not be directly measured, it may be deduced. 3.3. Electric field calculation
Before the initial breakdown, Vg and Vb0 could be
determined by using the following formulae In order to explain why Vb0 is lowered in the case of a mesh
electrode and PET film, the electric field in a 2 mm air gap
Cd was calculated with an applied voltage of 6.6 kV, equal to the
Vg (t) = Va (t), (1)
Cd + C g value corresponding to the initial breakdown. The field was
calculated using the MAXWELL 3D software from ANSOFT
Cd by carefully considering the fine structure of the wire mesh.
Vb0 = Vg (t)|t=t0 = Va (t)|t=t0 , (2)
Cd + C g The results show that the field is almost uniformly distributed

847
X Wang et al

75 plate covering the mesh electrode used in all experiments is


plane plate electrode + 0.1 mm PET film 0.1 mm in thickness, no matter if it is PET or ceramic. As
-------wire mesh electrode + 0.1 mm PET film for the mesh, the sparser the mesh and thinner the wire of
60 the mesh, the higher the field enhancement. However, if the
mesh is too sparse or the wire of the mesh too thin, the electric
field in the air gap will not be radially uniform and leads to a
E ( kV/cm )

45
non-homogeneous discharge.

30
4. Conclusion
15 The mesh electrode and PET film really make discharge
in a 2 mm air gap look homogeneous. The breakdown
0 onset voltage in case of a mesh electrode and PET film is
0.00 0.05 0.10 0.15 0.20 6.4 kV, considerably lower than 8 kV, the breakdown voltage
Z (mm) in the usual case using two spherical electrodes. The field
calculations show that even with this much lower voltage the
Figure 5. The electric field in a 2 mm air gap. gap field in the region very close to the PET film is enhanced
to a value near the breakdown field in the usual case. It may
in the central part of the air gap. Figure 5 is the field distribution be this field enhancement that initiates a corona discharge
along the Z-axis, the axis of the electrodes. For comparison, which provides seed electrons, leading to the breakdown of
the field in the case of a plane electrode and 0.1 mm PET film the whole air gap at a lower voltage. A lower voltage applied
was also calculated and plotted in figure 5. to the gap means a lower averaged field over the gap. Since
Z = 0 and Z = 0.1 mm are the electrode–PET interface the development of an electron avalanche is very sensitive to
and PET–air gap interface, respectively. In contrast to the the electric field a small decrease in the field will depress the
uniform field in the case without using a mesh electrode, the avalanche significantly, preventing a homogeneous discharge
field in the case using a mesh electrode is distorted. In the air from transiting to filament discharge. This may be the reason
gap (Z  0.1 mm), the field in the region very close to the PET why a mesh electrode and PET film make the discharge look
film is enhanced to 37.5 kV cm−1 . It is important to note that homogeneous.
37.5 kV cm−1 is close to 40 kV cm−1 , the breakdown field of
the 2 mm air gap in the usual case where the breakdown voltage
is 8 kV as mentioned above. It may be this field enhancement Acknowledgment
that first initiates a corona discharge in this region and then the
corona discharge provides seed electrons for the breakdown of This work was supported by the National Natural Science
the whole air gap. As we know [9], a self-sustained discharge Foundation of China under contract 50537020.
is formed under condition of γ [exp(αd) − 1] = 1, that is
also the breakdown condition for a homogeneous discharge
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