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By
the density log is an effective tool, and serves recall that atoms with nuclei of the same Z but
as a valuable aid in f'ormation evaluation. different A are forms of the same element and are
called isotopes.
INTRODUCTION
Beta rays (~) are believed to be physically
Gamma ray-density logging has progressed far equivalent to electrons if the beta radiation
since its original experimental stage. Numerous has a negative charge. If the beta rays have a
major oil companies and several service companies positive charge, they are equivalent to positive-
have made significant contributions to its ad- charged electrons and are called positrons. When
vancement. Although the tool was originally con- talking about positrons, the term negatron is
ceived as an al~iliary exploration device, con- usually used instead of electron; negatrons and
tinued research and development has created new electrons are exactly the same. Beta radiations,
and improved equipment and techniques. This positrons, and negatrons all have the same rela-
manner similar to chemical reactions. The state- nuclear disintegration was fully accepted by the
ment must involve at least four terms: target, scientific world, its mathematical development is
(projectile, product) residual. The projectile very simple: It is observed that the1loss in
and product particles are commonly abbreviated. radioactive nuclei (-dN) that occurs during an
A classic example would be that of a lithium 7 interval (Jt) is directly proportional to the
atom* being bombarded with an energetic proton. total number of nuclei (N) that is present after
Since the proton has a positive charge, it will the time (d t ). Thus,
experience an electrostatic repulsion as it ap-
proaches the nucleus of the lithium atom; but if . . . . (1)
the proton is accelerated to a sufficiently high
energy level, it will penetrate inside the nuclear
radius where the strong, short-range attractive where ~ is a proportionality constant. By
forces are at work. At this point, the proton separation of variables,
_~T . . . . (5)
cross sections. The cross section is said to be
large when the probability of a reaction is very I/,'\ ... I
higb, and conversely, the cross section is said T\NoJ = l'-loe
to be low when the probability of a reaction is
remote. Nuclear cross sections vary over a wide Using algebra, Eg. 5 clears to:
range; they are dependent on the type of particles
energy of particles, type of target, and type of
process. The common unit of nuclear cross section
\T = LOSe Z. .... (6)
It took many years to define the nuclear where T is the half-life of the substance. Since
disintegration processes in terms of mathematical N and No are very difficult numbers to measure,
expressions. The first significant conclusion the exponential law is often expressed in terms
was that the amount of radioactivity of a pure of:
substance decreases with time according to some
parabolic or hyperbolic function. It was later
observed that radioactive decay is statistical in
nature, that it could not be predicted when any where R is the disintegration rate or nuclear
given atom would disintegrate, and that some sta- activity of the material. (Halliday28 presents
tistical hypothesis would have to be developed to adequate explanation of this paramet~r.) It
explain the process. 28 ,3 1 Although it was a long will suffice here to say that R- dN or something
time before the contemporary, exponential law of -(ff
proportional to it. The decay period (1l) is
* Superscripts above names of elements are Atomic normally found by plotting Log R vs t. From Eq. 7
Masses and not reference numbers in the it can be seen that ~ is the slope of the straight
Bibliography. line through these data, thereby allowing the
4 GAMMA RAY-DENSITY LOGGING 1253-G
(a) U
"2.40
--. Np
7...'l-C>
N;4\) ~ 9u '?\ r-
is that cosmic rays have a higher frequency and
2 shorter wavelength which consequently explains
(b)
their higher energy level and greater penetrat-
ing power. The only difference between X-rays
(c) PUL'f() ~ U U\, ~ 0<... and gamma rays is that X-rays originate within
Before discussing gamma emission, it can be the radioactive atom, outside the nucleus; where-
pointed out here that nuclei do not change in A as gamma rays always originate from within the
or Z due to gamma radiation; however, there is a nucleus. Gamma rays and X-rays are otherwise
loss of nuclear energy. identical. Although seldom the case, it is pos-
sible to have gamma rays existing at energy
An interesting aspect of the nuclear dis- levels less than the normal X-rays energy level.
integration process is that a great many nuclei The nomenclature of gamma rays and X-rays is
decay by two or more types of radiation. An ex- purely a matter of their atomic origin. These
ample from Fig. 1 will illustrate this phenome- definitions are greatly simplified, but are ade-
non: Ac 224 will decay by alpha emission to Fr 220 quate for the purpose of this paper. Semat's
in X per cent of the disintegrations and by discussion of gamma rays and X-rays offers an
positron decay to Ra22)~ in Y per cent of the academic treatment of the subject matter. Since
disintegrations. X and Yare experimentally there is no difference in the type of inter-
determined; X + y: 100 per cent. By differen- actions that gamma rays and X-rays (of the same
tiation of Eq. 7, rt.(l£) (~~t =- ,and R-' energy level) have with matter, this paper will
use the generic term "photon" to mean either or
both.
\ tv) :: - (~:)y R- \ . Also, ' \6t- ... '<) = \l)() ~ \l\')
Interaction of Photons with Matter
. • . . (8)
According to Fan0 22 , there are four kinds
of interaction between photons and atomic par-
where ~(x), ,\(y) 'and Y\h+ y ) are the diSintegration ticles: (1) basic interaction with atomic
constants for 0<. decay, f3 decay, and the combined electrons, (2) basic interaction with particles
decay. From the given data: within the nucleus, (3) interaction with electric
1253-G ALBIN J. ZAK AND JOE ED SMITH 5
field surrounding charged particles, and (4) in- I 1.022 Mev before pair-production can occur since
teraction with meson field surrounding the nu- I this amount of energy is needed to supply the rest
cleus. It is further observed that each of these I energy. For large values of E., Ee- is
four kinds of interaction may produce three dif- I
ferent effects: photon absorption, elastic i essentially equal to E_
e +· For the values of
scattering of photon, and inelastic scattering of !
photon. Referring to the basic definition of I, Eyemmitted by Co "0 Er -Z>'Y\c2.may be shared
,
scattering, the process is called elastic if the
projectile acts upon the target as a whole, in any proportions between E e 1- and E e -. Ac-
whereas the process is termed inelastic if the cording to Halliday, the positron usually receives
projectile acts upon and produces some effect on more energy since it is accelerated by the nucleus
a constituent part of the target. There are whereas the negatron is restrained by the nucleus.
twelve possible interaction processes between The positron will eventually combine with an
0:-;~g~~ -;: :h~- p:otoelec::~c effect, the photons (-dP) that is absorbed or scattered away
photon expells an atomic electron from the K- in an additional absorber thickness (dx) is pro-
shell. In the pair-production process, the portional to P and to (dx). Therefore,
I gamma quantum vanishes, and an electron-positron
pair is produced. The photon is scattered by an - dP: k Pdx . . (n)
electron in the Compton process; the photon loses
some of its energy, and the electron is recoiled
from the atomic radius. Also, note that there is
a case where the photon passes through the atom
without having any kind of interaction. In fact,
or
I <I; --\,. ~ clx
The integration yields:
. . . . • . (12)
P'"
!!good geometry!! previously mentioned is necessary -:-pel(
in actually making these experiments. It is fur-
D
1-0 e . . . (16)
ther necessary that the incident photons be mono-
energetic and collimated into narrow beams. P and P~ are normally expressed in units of Mev;
/ in cm /gmj e in gm/cm 3 , and x in cm. Numerous
The value of P will depend on the values of narrow-beam attenuation experiments have verified
Po and x. If an additional absorber thickness Eq. 16, and have measured values of~ .10,18,21,
(dx) is added, P will decrease by (-dP). If stil 29,37
another absorber thickness (dx) is added, (P-dP)
will decrease by (-dP). Thus, there is a definitE Separate theories have been worked out for
mathematical pattern observed: each of the three absorption processes. Remember
tha~ is the attenuation constant for the
P C( Pc.lX .(lOa combined effects of photoelectric absorption,
pair-production, Compton scattering, and such that:
-~~ C{ ~ .I
d)(. . (lOb)
manner:
I . . . (23)
I
~
of scattered photons is quite large for energetic
Note that: hQ.'::: r}b .:: NA · (19) photons and large scattering angles. Fig. 5 is a
V\/ graph showing the results of calculations made
and nc.. =c Z-NA ~ .(20) with Eq. 24 for gamma ray energies up to 10 Mev
vV and scattering angles from 50 to 1200 . Naturally,
where NA is the number of molecules in a mole of
if -e- -= 0) E/ = E Klien and
Y
the absorber substance, ~ is the mass density,
and W the atomic weight. This definition of at- Nishima used a quantum mechanics approach to cal-
tenuation coefficient is essentially the same as culate the nuclear cross section per electron for
that previously presented. the Compton process. 33 Their basic assumption is:
the gamma ray energy is so great that all elec-
In gamma ray-density logging, the radio- trons can be considered free. The Klien-Nishima
active source emits photons with energies in the formula has been well proven by numerous experi-
order of 1.0 to 1.5 Mev. Most of the atoms that ments in this field.
constitute reservoir rocks and interstitial
fluids have nuclei of low A values; hydrogen, 'I'he theory of Compton scattering is of pri-
carbon, oxygen, silicon, calcium, magnesium, mary importance in the density log, and will be
sodium, chlorine, sulfur, etc. Hence, the most used throughout the remaining discussion. By ju-
predominent process active during a gamma-gamma dicious choice of gamma ray source and carefully
log-run is Compton scattering. Since the varia- engineered source-detector arrangement, the
tion in~is directly proportional to variations response of the gamma ray-density logging tool can
in A, P is very nearly an exponential function of be made to depend primarily on the density of the
~. (Refer to Eq. 16). The reader should note formation rock and interstitial fluids.
that P is an indication of the average density
along the traversed path, not the density at the INSTRUMENTATION OF LOGGING DEVICES
point from which the photons are scattered. If
it were not for the small amount of photoelectric Gamma Ray Detection
absorption and pair-production, a plot of Loge P
vs f would be a straight line, with (~x) as the Radiation detectors that have been used to
slope of the line. date in the gamma ray-density log are of three
general types: (1) ionization chambers; (2)
The first attempt to describe the Compton Geiger-Muller tubes; and (3) scintillation count-
effect was done with the classic diagram shown ers. Each type has its own particular advantages
on Fig. 4*. By using the relativistic laws for and disadvantages. The following discussion will
conservation of momentum and total energy, an present a very brief statement as to the princi-
equation has been derived that predicts the ples of operation of each, will highlight the
change in quantum wavelength of the photon per operational characteristics of each, and show how
Compton collision: 18 ,2l,2b they are adapted to the problem of gamma-gamma
A'_A=~(I-Cos~)
logging.
..... (2l)
The theory and operation of ionization cham-
*See A. H. Compton, Bulletin of National Research bers is adequately covered in the literature cited.
Council, Vol. ~, No. 20 (1922). 24,48,54,64 Basically, this instrument consists
1-------
8 GAMMA RAY-DENSITY LOGGING
~--~-----"-='------'1
1253-G
of a chamber containing an inert gas. Two I thin wire replaces the small tube or cylinder used
electrodes, usually in the form of concentric in the ionization chamber as an anode. Again, the
cylinders, are placed within the sealed chamber. counter chamber is filled with an inert gas but at
As photons penetrate the wall of the chamber, the much less pressure (in the order of one atmosphere
gas molecules will ionize into charged atoms. or less). There is also an electrical field set-
If an electric field is set up in the vessel, the! up across the electrodes of the Geiger counter,
ions will move toward the electrodes and cause an but the field strength is much greater than that
electric current to flow that is proportional to of the ionization chamber. As in the ionization
the degree of ionization produced by the radia- chamber, the photons that enter the chamber will
tion entering the chamber. The negative ions ionize gas molecules, but since the electric field
move toward the positive electrode, and con- is very strong, the ions are greatly accelerated
versely, positive ions toward the negative elec- as they move toward the electrodes. These highly
The photo-multiplier has a series of thin,~ight- 'I Large volumes of literature have been writte
sensitive plates mounted in a vacuum. The plates, I that explain how these three basic gamma ray de-
or stages, of the photo-multiplier tube are nega- i tectors are adapted to practical well logging
tively charged. As a flash of light strikes the ' tools. (Refs. 38, 39, 48, 50, 52, 56, 66, and
first stage, electrons are liberated from the 68.) There is an even larger volume of informa-
metal plate. These electrons are expelled at high tion that deals with the calibration, interpreta-
velocities because of the negative charge of the tion, and application of these gamma ray logging
plate. The parabolic shape of the plate and high tools. (Refs. 40, 42, 44, 45, 51, 57, 58, 59,
kinetic energy of the electrons cause the elec- 60, 61, 63, 65, and 70.) The remaining portion
trons to strike the plate of the second stage; but of this discussion will review the specific prob-
they are immediately repelled and, in so doing, lems of adapting gamma ray detectors to gamma-
cause more electrons to be expelled from the gamma logging, the calibration of these instru-
second stage. This routine is repeated for each ments, and the interpretation of the curves re-
A brief note on statistical error, sensitiv- Estimation of Porosity from Formation Density
ity, time-constant, and logging speed is in order
A very comprehensive analysis of these parameters The density log measures the average or
is presented in literature published by Lane- composite density of the formation near the bore-
Wells Co.56 Any geologist or engineer confronted hole walls. Therefore, the fluids filling the
with the analysis of radioactivity logs should pore spaces are averaged into the value of forma-
I
~--~~
14.
Addison-Wesley and Co., cambri~::::~. ANDI3:~E :lm~::.
ZAK
Blatt, S. M., and Weisskopf, V. F.: Theo-,
T.: "Graphs of the Compton fuer~:
Angle Relationships and the Klein-Nishina
retical Nuclear Physics, (1952) John Wiley Formula from 10 Kev to 500 Mev", National
and Sons, New York, N. Y. I Bureau of Standards Circular No. 542 (1953)
15· Caldwell, Richard L.: "Gamma Radiation from U. S. Dept. of Commerce, Washington, D. C.
Inelastic Scattering of 14-Mev Neutrons in 34. Occhialini, G. P. S., and Powell, C. F.:
the Common Earth Elements", Bull., Am. Phy- I "Nuclear Disintegration Produced by Slow
sics Society, Series II (Feb. 24, 1956)}, I Charged Particles of Small Mass", Nature
No.2, 90. (1947) 122, 186-190.
16. Caldwell, Richard L.: "Nuclear Physics in 35. Pocock, B. W.: "An Analysis of Certain
Petroleum Exploration Research", World Pet. Mathematical Assumptions Underlying the De-
(1956) ~, No.4, 59. sign and Operation of Gamma Ray Surface
17· Caldwell, Richard L., and Sippel, Robert F.: DenSity Gages", Michigan State Highway De-
I
69·
70.
Toelke, L. W.: !!Scintillation Spectrometer
Well Logging", AIME Tech. Paper No. 495-G
(Presented in Denver, Colo., May, 1955.).
Vomocil, J. A.: "In Situ Measurement of Soil
I 51.
Quantitative Interpretation of Radioactivity I Bulk Density", Agricultural Engr. (1954) l2.,
Logs", Oil and Gas Jour. (March 24, 1952) I No·9·
188-194. I 71. Youmans, Arthur, and Monaghan, Ralph: "Sta-
52. Guelke, R. J., Heydenrych, C. R., and Ander- bility Requirements for Scintillation Coun-
son, F.: !Measurement of Radioactivity and I ters Used in Radioactivity Logging", Trans.
Temperature in Narrcw Boreholes and the II AIME (1957) 210, 231.
Development 'Jf Instruments for this Purpose!!,
Jour. of Scientific Instruments and Physics GROUP IV
in Industry (1949) 26, 150-153.
1
PAIR -PRODUCTION~
54
PH OT 0 E L E C T RIC .!::E.!:FJ:F:..!E=-,CUT.---~ /
52
~'/'-
( \
(
0
!
~<:~~~f--t\ V ) 1(-
>--
0
~
\~Y ---e-.----- /
-----= ~y'
Particle COMPTON SCATTERING~ 'C---_----. __ ~ __
photon e-'
MASS NUMBER, A e- electron
e+ positron DIAGRAM SHOWING THREE POSSIBLE
FIGURE I n neutron INTERACTIONS .OF GAMMA RADIATION
DISINTEGRATION CHART FOR p+ proton WITH THE SILICON+4 ATOM
THE THORIUM DECAY SERIES FIGURE 2
(AFTER HALLIDAY)
CD y-------.(x\:)
",r In! ~J--
~i- ..
> 9 /
'"
::i<
/
V
>- 8
t9 ~
0:::
W
z 7
!/
/ V
w
],/,0"
/ /'
z
0
I-
0
6
5
/ VV
~/
I
L.----
---
4
/' I---""'
0
W
# /
0:::
w
l-
I-
« 2
3
1// ' -
V
f-.---
I - - _30· -
u
U)
~
I~ V ----- 45·
60· =
-
~ ::-- 12~0
-
~
o 2 3 4 5 6 7 8 9 10
FIGURE 5
FIG URE 6
GRAPH SHOWING ENERGY SCHEMATIC OF TYPE I SONDE
LOSS OF SCATTERED PHOTONS FOR (RADIAL SOURCE AND
GEIGER - MULLER COUNTER)
VARIOUS SCATTERING ANGLES
DETECTOR REGION
REGIO N
b
b and I are known·
, b
'"'b" 2ToST
h"Z TonI
-e- " 21
,-
.! h-----I
SL SOURCE REGION
FIGURE 7
SCHEMATIC OF TYPE n SONDE
(COLLIMATED SOURCE AND
FIGURE 8
SCINTILLATION COUNTER)
GEOMETRY OF TYPE IT SONDE
10.00
FIGURE 10
L EXAMPLE OF DENSITY LOG 9.00
CALIBRATION CURVE FOR
TYPE I SONDE
8.00
V)
w
/ '- 7.00
::r:
<..>
:z
:z
,
WITH 215 STo. SOURC£
--
w
-'
5.00 u...
'\ w
0
I\V
4 00
'"
0
-'
>-
l-
V)
of-- 300 :z
w
0
2.00
NATURAL DENSITY, ~
cc
POROSITY, %
--Pf!!~T.!.I,Q'L I)!T.!_
CORE DATA
o 2 ... ~ e ,0 ,2 14 '6 'EI 20 0 2
TABLE I
FIGURE II
COMPARISON OF CORE ANALYSIS
PO RO SIT Y WITH POROSITY
DERIVED FROM DENSITY LOGS