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PHYSICAL REVIEW B 78, 184520 共2008兲

Vortex-dynamics approach to the Nernst effect in extreme type-II superconductors


dominated by phase fluctuations
S. Raghu,1 D. Podolsky,2,3 A. Vishwanath,2 and David A. Huse4
1
Department of Physics, Stanford University, Stanford, California 94305, USA
2
Department of Physics, University of California, Berkeley, California 94720, USA
3Department of Physics, University of Toronto, Toronto, Ontario, Canada M5R 1A7
4Department of Physics, Princeton University, Princeton, New Jersey 08544, USA

共Received 20 October 2008; published 26 November 2008兲


We present a method to study the Nernst effect and diamagnetism of an extreme type-II superconductor
dominated by phase fluctuations. We work directly with vortex variables and our method allows us to tune
vortex parameters 共e.g., core energy and number of vortex species兲. We find that diamagnetic response and
transverse thermoelectric conductivity 共␣xy兲 persist well above the Kosterlitz-Thouless transition temperature,
and become more pronounced as the vortex core energy is increased. However, they weaken as the number of
internal vortex states is increased. We find that ␣xy closely tracks the magnetization 共−M / T兲 over a wide range
of parameters.

DOI: 10.1103/PhysRevB.78.184520 PACS number共s兲: 74.25.Fy, 74.20.De, 74.40.⫹k, 74.72.⫺h

A number of experimental observations in superfluidity derstood in terms of a dilute fluid of vortices, but so far this
and superconductivity are best explained in terms of the sta- appealing picture6,7 has not lead to a complete understanding
tistical mechanics and dynamics of vortices. Examples in- of the Nernst effect.
clude the Kosterlitz-Thouless 共KT兲 transition in superfluid There are special challenges involved in constructing a
films and the “flux-flow” contribution to electrical resistivity vortex-based theory of thermoelectric transport that is con-
in type-II superconductors. A natural extension of this para- sistent with the basic principles of statistical mechanics. In
digm involves the use of thermoelectric and thermal trans- contrast to thermodynamics, and even electrical transport,
port experiments as a probe of vortex dynamics. This is es- where a theory of vortices interacting via a long-range po-
pecially pressing given the Nernst effect experiments in the tential can be used, a thermal transport calculation requires a
cuprates.1 The Nernst effect is the appearance of a steady- purely local formulation where no such long-range forces are
state electric field 共Ey兲 when a system is placed in a perpen- explicitly present. In this paper, we present such a local for-
dicular thermal gradient 共ⵜxT兲 and magnetic field 共Hz兲 under mulation and use it to study thermoelectric transport directly
open-circuit conditions. In the cuprate superconductors, a in the vortex language. An advantage of our method is that
large Nernst signal and diamagnetism persists well above Tc, vortex parameters, such as core energy or number of vortex
the superconducting transition temperature, and are espe- species, can be tuned independently of other properties, and
cially enhanced in the underdoped regime of hole-doped ma- their impact on the Nernst signal and magnetization can be
terials. systematically studied. Moreover, it is possible to use our
To explain these results, it has been argued that vortices method to study the Coulomb gas efficiently even in the
are responsible for the large Nernst signal:1 as a vortex drifts high-density limit, where the number of pairwise Coulomb
down the temperature gradient, it generates a transverse elec- interactions is large.
tric field. A vortex description above Tc is useful when Tc Previous theoretical work on the Nernst effect includes
marks the loss of macroscopic phase coherence, while the the time-dependent Ginzburg-Landau theory,8,9 which in-
amplitude of the order parameter remains large below a cludes fluctuations in the amplitude of the order parameter.
higher “mean-field” temperature scale TMFc ⬎ Tc. This idea is
2 The Nernst effect near a quantum critical point has been
most likely to hold true in the underdoped regime of the studied in Ref. 10. A heuristic treatment of the Nernst effect
hole-doped cuprates, where the reduced superfluid stiffness in a vortex liquid has been presented in Refs. 11. In earlier
enables phase fluctuations to suppress Tc below the mean- work, three of us have studied the Nernst effect in an XY
field transition temperature. Prior to the experiments de- model,12 which should be relevant for the underdoped cu-
scribed in Ref. 1, optical conductivity measurements3 prates. Our present results approaching from the vortex
showed that superconducting correlations persist above Tc at viewpoint are consistent with this work. Remarkably, we find
short distance and time scales in BSCCO films. Recently, that the close quantitative connection between the Nernst
current-voltage measurements in YBCO films have also re- effect and diamagnetism observed previously holds in the
vealed a relatively wide zero-field regime where supercon- present study too, even when vortex properties are drastically
ducting fluctuations are likely to persist.4 However, the dia- modified. The effect of vortex core energy on thermody-
magnetism and Nernst measurements1 have exposed a namic properties was studied in Ref. 13.
greater fluctuation regime since the normal state contribu- Method: Consider a two-dimensional 共2D兲 supercon-
tions to these experiments are far smaller than in electrical ductor in the extreme type-II limit, in which the supercur-
transport measurements. Over a range of fields, this “vortex- rents are too feeble to modify the external field. We restrict
liquid regime” Tc ⬍ T ⬍ TMF c 共Ref. 5兲 can be intuitively un- the order parameter to live on the sites n of a square lattice

1098-0121/2008/78共18兲/184520共5兲 184520-1 ©2008 The American Physical Society


RAGHU et al. PHYSICAL REVIEW B 78, 184520 共2008兲

added to it. Such an update is purely transverse and is not


accompanied by vortex creation. During a charge update, a
lattice bond is chosen at random, and a vortex/antivortex pair
is added on the two sites connected to this bond. The electric
fluxes are updated locally near the charges to satisfy Gauss’
law. The result of such an update is either the creation of a
vortex/antivortex pair or the motion of a pre-existing vortex
to a neighboring site. We note that while such moves can
change the total number of vortices, the net vorticity does not
change in a system with periodic boundary conditions. Each
move is accepted with probability 1 / 关1 + exp共⌬U / T兲兴, where
+

_
⌬U is the change in energy associated with the move and T
is the local temperature at the center of the plaquette or bond
for that move. By varying the relative frequency of each type
of trial, we have control over Dph, the phase diffusivity, rela-
tive to the vortex diffusivity Dv. In what follows, we work in
the physically reasonable limit Dph Ⰷ Dv 共in practice we set
Dph = 25Dv兲. After an attempt is made to update each bond
FIG. 1. 共Color online兲 Charge updates 共left兲 and curl updates and plaquette, a unit of Monte Carlo time elapses. A related
共right兲 sample the longitudinal and transverse degrees of freedom, method has been used in Ref. 14 to study charged polymers.
respectively, of the dual electric field. When a charge move is attempted, the simplest way to
satisfy Gauss’ law is to add an electric flux e = 2␲r̂ to the link
and assume that all fluctuations arise from the phase: ␺n共t兲 r̂ connecting the positive to the negative charge. However,
= 兩␺0兩ei␪n共t兲. We map to the vortex representation by defining such single bond updates are rarely accepted, resulting in too
a dual electric field e = 共exi , eiy兲 on the bonds 共i , i + x̂兲 and little vortex motion below a temperature scale T ⬃ ␲ / 2 Ⰷ ␳s0;
共i , i + ŷ兲 of a dual lattice, orthogonal to the original lattice to avoid this artificial vortex pinning, we use an update that
ជ ␪ ⫻ ẑ, where ⌬
ជ is a lattice derivative. Here the spreads the electric flux over several bonds. A simple ex-
bonds, via e = ⌬ ample of such an update is shown in Fig. 1. The added flux is
lattice spacing is taken to be the size of a vortex core. The made curl free, and the move we actually use involves a
local field e is related to the local supercurrents via J = ␳s0ẑ patch of 12 plaquettes that is one plaquette larger in all di-
⫻ e, where ␳s0 is the bare superfluid density. Vortices may rections than indicated in Fig. 1. We have explicitly com-
live at the sites i of this dual lattice, and the integer vortex puted the vortex mobility from the voltage autocorrelation
charge ni satisfies Gauss’ law ⌬ ជ · e = 2␲n . We then obtain a function and have seen its enhancement at lower tempera-
i
completely local Hamiltonian for the vortex fluid that retains tures with the use of such updates. As the size of the patch
all phase and vortex degrees of freedom, over which the updates are made is increased, the problems
associated with fictitious vortex pinning are eliminated.
1
H= 兺 e2 + ⑀ci苸sites
4␲ i苸links i
兺 n2i , 共1兲
However, when the charge updates are made over the entire
system, the curl updates are no longer necessary as the exci-
tations of the transverse component of the electric fields be-
where ⑀c is the vortex core energy and we use units where come instantaneous, making the model unsuitable for study-
␳s0 = 1 / 2␲. The dual electric fields can be decomposed into ing thermal transport. Therefore, the charge updates must be
longitudinal and transverse components representing the vor- made over a region whose size is larger than the lattice spac-
tex and supercurrent fluctuations, respectively. When the ing but much smaller than the entire system size. In our
transverse electric fields are integrated out, the model re- simulations, the charge updates are made over a region of 12
duces to the static 2D Coulomb gas. While the static Cou- plaquettes that is one plaquette larger in all directions than
lomb gas model is adequate for studying the equilibrium indicated in Fig. 1. We have found that these moves elimi-
properties of a vortex fluid, we stress that one must include nate the artificial pinning of vortices and allow us to access
both local supercurrents and vortices when dealing with ther- the dynamics down to TKT but are still sufficiently local to
mal transport so as to define a local energy density. The permit the study of thermal transport.
interaction between the vortices is mediated by the supercur- Thermodynamics: We have studied the KT transition of
rents, and this maps simply to the interaction between the the neutral 2D Coulomb gas by tracking the dielectric re-
charges being mediated by the dual electric field in our sponse function
model.
The model is given a Monte Carlo dynamics that captures
the effect of random thermal fluctuations. Two distinct types ⑀ −1
=1−
具共兺 e 兲 典 .
i i
2

共2兲
of Monte Carlo moves, electric curl and vortex updates, cor- 4␲TL2
responding to the longitudinal and transverse degrees of free-
dom, are introduced 共Fig. 1兲. During a curl update, a At T = TKT, the dielectric response function satisfies the uni-
plaquette is chosen at random and a random electric curl is versal jump criterion15

184520-2
VORTEX-DYNAMICS APPROACH TO THE NERNST… PHYSICAL REVIEW B 78, 184520 共2008兲

1.2 Nernst effect: To determine the Nernst effect, we


1
again make use of cylindrical geometry and apply a tempera-
1 0.8 ture gradient along the cylinder axis. We compute the trans-
0.6 verse thermoelectric conductivity ␣xy defined via 具Jy典 =
0.8 0.4 −␣xy共−ⵜxT兲 and is closely related to the Nernst signal:
0.2 ␣xy / ␴xx. Here, ␴xx is the electrical conductivity and we have
-1

0.6 0 made the approximation of vanishing Hall angle. The expres-


ε

0.1 0.2 0.3 0.4 sions for the transport coefficients are easily found in the
0.4 T dual vortex representation using the relations

0.2
J = ␳s0ẑ ⫻ e,

0 E = ⌽0ẑ ⫻ j, 共6兲
0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8
where upper 共lower兲 case quantities refer to the original
T
共dual兲 representation and j is the vortex current. The first
FIG. 2. Dielectric response of the dual Coulomb gas, computed equation above is the definition of the dual electric field, and
using Eq. 共2兲, and 共inset兲 rescaled for finite-size effects 共Ref. 16兲. the second is the Josephson relation. We observe that in the
We use an L ⫻ L torus with L = 8 , 10, 12, 14, 40 and core energy ⑀c superconductor, the time-reversal operation, which maps
= 0.125. The transition temperature is the location where the res- J → −J, translates to the particle-hole transformation,
caled data intersect the line y = 4T 共dotted line兲. namely, e → −e in the dual vortex representation and vise
versa. The quantity ␣xy is obtained by measuring 具ex典 and

⑀−1 = 再 0,

4TKT , T = TKT
+
T = TKT
冎 . 共3兲
using the relation ␣xy = ␳s0具ex典 / ⵜxT. While ␣xy is an off-
diagonal transport coefficient when written in terms of elec-
trical currents, it is a diagonal response function in the vor-
tex representation: it is simply the vortex thermopower. We
Figure 2 shows the results of the helicity modulus calculation
have verified that the net vortex motion vanishes once the
using various system sizes and a core energy ⑀c = 0.125. We
steady state in the thermal gradient is reached, as is required
use finite-size scaling16 to identify TKT = 0.22; the naive free-
0 in a thermopower measurement. The quantity ␣xy has the
energy estimate is TKT = 0.25 in our units. In the remainder of
0 advantage that, unlike the Nernst signal, it does not have any
this paper, we cite all temperatures in units of TKT .
explicit dependence on Monte Carlo time tMC, as can be seen
Diamagnetism: When a magnetic field is applied, the re-
from the Kubo formula for ␣xy and dimensional analysis.12
sulting imbalance of vorticity leads us to consider a plasma
Also, in our model, the diagonal thermoelectric coefficient
of vortices in a static neutralizing background 共charge den-
␣xx = 具Jx典 / 共−ⵜxT兲 = 具ey典 / 共ⵜxT兲 maps onto a transverse ther-
sity nb = −B / ⌽0, where ⌽0 = 2␲ is the flux quantum in our
mopower of vortices. It vanishes by symmetry in our model
units兲. To study diamagnetism we permit vortices to enter
since the vortices can travel perpendicular to the thermal
and leave the sample by employing cylindrical geometry
gradient only if a Magnus force is present. However, a Mag-
with open boundaries. Current flow near the boundaries is
nus force can be nonzero only if particle-hole symmetry is
measured, which arises due to a surface depletion of vorticity
broken in the superconductor 共i.e., if the Hall angle is non-
that lowers the free energy relative to a perfectly neutral
vanishing兲.
system. Deep inside the cylinder, beyond some distance x0
Figure 3 shows the simulation results for ␣xy and M 关inset
from the edge, the supercurrents vanish in equilibrium. The
共b兲兴 for applied fields up to B0 = ⌽0 / 共2␲a2兲, where a is the
magnetization can be obtained by inverting the relation
lattice spacing, comparable to the zero-temperature coher-
J = ⵱ ⫻ M on a cylinder whose axis is along the x direction.
ence length ␰0. Both ␣xy and −M / T are expressed in units of
For physical clarity we present continuum formulas below;
the 2D “quantum of thermoelectric conductance,” 2ekB / h.
these can be readily transcribed into the appropriate lattice
We show data for T ⱖ TKT 0 0
; below TKT , our simulations en-
versions,
counter difficulties due to impaired vortex mobility. Fortu-

冕 冕 nately, T ⱖ TKT
x0 x0 0
is a regime of interest since the Nernst signal
M= dx具Jy共x,y兲典 = ␳s dx具ex典. 共4兲 persists well above Tc in the experiments of Wang, et al.1
0 0
The results presented here are in quantitative agreement with
Thus, M is directly proportional to the work function of the earlier computations involving the 2D XY model with Lange-
dual Coulomb gas 共energy cost of removing a vortex from vin dynamics:12 in particular, both models have the feature
the bulk of the system兲. Using Gauss’ law we can also obtain that in the small magnetic field limit, 共a兲 ␣xy and M diverge
logarithmically as B → 0 for T ⱕ TKT and 共b兲 they increase
M = 2␲␳s 冕 0
x0
dx x共具n共x兲典 − B/⌽0兲. 共5兲
linearly with B at small B when T ⬎ TKT.17 Moreover, both
␣xy and M are detectable at temperatures as high as 2TKT in
our model, as well as in the 2D XY model.12 For T Ⰷ TKT, the
Thus, M is also the total edge polarization per unit length. 2D XY model predicts that ␣xy and M / T decay sharply as a
The polarization fields are nonzero only in the charge deple- power law in temperature. Here, the magnetization decreases
tion region near the cylinder’s edge. even more rapidly at high temperatures: a calculation based

184520-3
RAGHU et al. PHYSICAL REVIEW B 78, 184520 共2008兲

1
index.18,19 Such an extension is readily incorporated in our
αxy, -M/T 0.9 (b)
formalism; the Gauss law is now ⵜ · e = 2␲兺␣N=1 v n , where ␣
0.8 i␣
0.6
0.6 is the flavor index. Our data show a systematic dependence

-M/T
0.3 (a) 0.4 on the number of internal flavors. We find that both 兩M兩 and
0
0 3 6 9 0.2 ␣xy of single-flavor vortices 共solid curves in Fig. 3兲 are sys-
εc/TKT0
αxy (2ekB/h)

1 0 tematically larger than that of vortices with two internal fla-


0 0.2 0.4 0.6 0.8 1
0.8 B/Bo
vors 共dotted lines兲. With multiple vortex species, there is
additional configurational entropy associated with the inter-
0.6 nal degree of freedom. Therefore, the free-energy cost of
0.4 introducing a vortex into the sample is lower, and the system
becomes less diamagnetic. It is more difficult to understand,
0.2
however, why ␣xy decreases as the number of species is in-
0 creased. In phenomenological discussions, the transport co-
0 0.2 0.4 0.6 0.8 1 efficient ␣xy is usually identified with the vortex entropy.20
B/Bo Therefore, one may naively expect ␣xy to increase with the
number of internal vortex flavors. Moreover, ␣xy is equiva-
FIG. 3. 共Color online兲 ␣xy for a system of single-flavor 共solid lent to the vortex thermopower, and if we neglected the loga-
lines兲 and double-flavor 共dotted lines兲 vortices on a 20⫻ 15 cylin- rithmic interactions between vortices, the thermopower is
der, with core energy ⑀c = 0.5TKT 0
. Temperatures shown are 1.0 共top- simply the entropy per particle 共see below兲, which increases
most 2 curves兲, 1.25, 1.5, and 2.0 TKT 0
共bottom two curves兲. Inset
linearly with the number of internal states associated with
共a兲: Core energy dependence of ␣xy 共solid lines兲 and −M / T 共dashed
such particles. Our numerical results however are in sharp
lines兲 in units of 2ekB / h for single-flavor vortices, at T = 2.5TKT
0
and
contrast to such expectations. Instead, our results, which
B = 0.7B0, showing a marked increase in both quantities with core
energy. Inset 共b兲: Diamagnetism −M / T curves for the same tem-
have the opposite trend, point toward a scenario that is far
peratures as the main figure. 共Units of 2ekB / h are used on the ver- more complicated than an ideal gas approximation.
tical axes of both insets.兲 Perhaps the most striking feature of our data is the fact
that ␣xy and −M / T closely track each other. In particular, at
on the dual solid-on-solid model shows that the magnetiza- high temperatures, our results obey the relation ␣xy =
tion of single-flavor vortices decays exponentially as M = −cM / T, where c ⬇ 1, and is difficult to determine accurately
−2T sin共B / B0兲e−2T/␳s, and our numerical results agree with due to noise at large temperatures. Recently, it was shown
this expression. Although we have not succeeded in finding analytically in Ref. 12 that for the 2D XY Hamiltonian with
similar expressions for ␣xy, our numerics indicate that ␣xy overdamped dynamics, c = 1 / 2 at high temperatures. Further-
also decays in this fashion at high temperatures and closely more, one obtains the same relation for Gaussian supercon-
tracks −M / T. ducting fluctuations.21 Here, we have shown that this relation
Vortex core energy dependence: The core energy depen- is even more robust since it hardly depends on the variation
dence of ␣xy and −M / T are shown in Fig. 3 关inset 共a兲兴 at T in the core energy and the number of distinct vortex species
0
= 2.5TKT . So long as ⑀cⰇ ” T, both are found to increase with so long as ⑀c is not much greater than T. This relationship is
⑀c. At this temperature, ␣xy and −M / T track each other indicative of a deep underlying principle that seems to hold
closely. With increasing core energy, ␣xy and −M / T rise from true over a broad range of parameters.
near zero at ⑀c = 0 to O共1兲 at ⑀c = 10TKT
0
, showing that the core Discussion: Thus far, we have focused on the Nernst ef-
energy has a dramatic impact on both of these quantities in fect due to vortices interacting with a logarithmic Coulomb
this regime. The dominant effect of ⑀c is to enhance local interaction. As a point of comparison, we now derive the
superconducting correlations at short distances by increasing Nernst effect of a noninteracting ideal gas of vortices. For
the cost of vortex fluctuations. It enters directly in setting the this case, we will show rigorously that ␣xy is equal to the
“work function” for removing a vortex from the system, thermodynamic entropy per vortex. Then, we will introduce
which is proportional to the magnetization. For ⑀c Ⰷ T, −M interactions through a virial expansion to show the devia-
⬀ ⑀c since more vortices are expelled near the boundaries in tions from this result for interacting vortices.
this limit. We have observed this in our simulations. The As mentioned above, the transverse thermoelectric con-
vortex-free boundary layer grows with ⑀c, and when it be- ductivity ␣xy maps under duality to the thermopower of the
comes comparable to the thickness of the sample this causes vortices, i.e., to the dual electric field created by the vortices
strong finite-size effects. Thus, we have not been able to in response to an applied temperature gradient

冏 冏
reliably determine the bulk behavior for large values of the
vortex core energy ⑀c. We expect ␣xy to saturate at a finite ex
␣xy = ␳s0 ,
value in this limit; when all thermally generated vortex fluc- ⵜ xT j=0
tuations are suppressed, the remaining field-induced vortices
respond to the thermal gradient in a way that is independent where measurement is carried out under open-circuit bound-
of the magnitude of ⑀c. ary conditions for the vortices, j = 0.
Dependence on the number of vortex flavors: Several Consider noninteracting particles, which can be bosonic,
theories of cuprates predict additional degrees of freedom fermionic, or distinguishable 共the result will be independent
associated with vortices that endows them with a flavor of particle statistics兲, in a system with Galilean invariance so

184520-4
VORTEX-DYNAMICS APPROACH TO THE NERNST… PHYSICAL REVIEW B 78, 184520 共2008兲

that the energy of a particle with momentum k is ⑀k that instead of holding the pressure constant as in the case of
= k2 / 2m. The Boltzmann equation for the particle distribu- the ideal gas, we must require quantity P − n2TB2共T兲 to re-
tion g = g共r , k , t兲 is ṙ · ⵜrg = −共g − g0兲 / ␶, where g0 is the par- main constant, where B2 is the second virial coefficient of the
ticle distribution in equilibrium and ␶ is a relaxation time. In system. Therefore,
the Boltzmann equation, we have assumed that no external
forces are present 共however, gradients in chemical potential
and temperature are present兲. Then, the vortex current is
␣xy = − 冉 冊
⳵␮
⳵T P−n2TB2共T兲,N
. 共8兲


In the dilute limit where the interactions are very weak, i.e.,
d dk
j共r兲 = vkg共k,r兲 when B2 Ⰶ P / 共n2T兲,

冉 冊
共2␲兲d

冋冕 册
⳵S ⳵
2␶ d dk k 2 ␣xy = −n 共TB2兲. 共9兲
=− ⵜr g共k,r兲 ⳵N P,T ⳵T
md 共2␲兲d 2m
Thus, when B2 ⬎ 0, which is true in the case of repulsive
2␶ interactions, we see that ␣xy decreases in magnitude and is
=− ⵜr关␳E共r兲兴, no longer simply identified with the entropy per particle.
md
Indeed, our numerical calculations strongly suggest that in-
where ␳E is the energy density of the vortices. Note that, teractions between vortices play an important role in deter-
independently of the particle statistics, the energy density of mining the temperature dependence of ␣xy and invalidate a
an ideal gas is proportional to the pressure P. Therefore, simple identification of ␣xy as the vortex transport entropy.
open-circuit boundary conditions are equivalent to the re- In conclusion, we have presented a method to study the
quirement that the pressure in the system be uniform, ⵜP=. thermodynamic and transport properties of 2D vortex liq-
Therefore, uids. This method enables us to directly observe the effect of

冏 冏 冉 冊 冉 冊
modifying the core energy and the number of vortex species
⳵␮ ⳵␮ ⳵S on diamagnetism and Nernst effect. We have found that both
␣xy = − =− = , 共7兲
⳵T j=0 ⳵T P,N ⳵N P,T quantities persist well above TKT and ␣xy closely tracks
−M / T when TKT ⬍ TⰆ ” ⑀c. We have provided a detailed analy-
where S is the entropy, ␮ the vortex chemical potential, N the sis of the Nernst effect of a vortex liquid that deals directly
vortex number, and where in the last line we have used a with vortex variables. The method presented here can be
Maxwell relation. Thus, ␣xy of an ideal gas of vortices is a generalized to study thermal transport of vortex liquids in
measurement of entropy per vortex. three dimensions 共3D兲 and can be extended to study quantum
Next, we consider the leading correction to ␣xy due to phase fluctuations.
pairwise interactions among the particles. Assuming that the
particles are classical and indistinguishable the interactions We thank P. W. Anderson, S. A. Kivelson, P. A. Lee, and
can be treated perturbatively with a virial expansion. From N. P. Ong for very helpful discussions. This work was sup-
the Boltzmann equation above, it is clear that the open- ported by NSF under Contracts No. DMR-0645691 共A.V.兲
circuit boundary conditions on the particles amount to a con- and No. DMR-0213706 共D.A.H.兲 and by the Stanford Insti-
straint of uniform kinetic energy density. This in turn implies tute for Theoretical Physics 共S.R.兲.

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