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Received 16 December 1999; received in revised form 24 September 2002; accepted 7 November 2002
Abstract
A small-size spouted bed with a porous draft tube was employed to obtain hydrodynamic data of binary mixtures of glass beads for a
range of operating conditions and design factors. In this case, a small amount of finer particles was added mostly to the large majority of
coarser particles. Under this condition, minimum spouting velocity, bed pressure drop, hold-up of solid particles within a draft tube, gas flow
rate through the annulus and solids circulation rate were determined by changing the total gas flow rate and the mass fraction of finer particles
as operating parameters, and by changing the height of the entrainment zone and the draft tube diameter as geometric parameters. The results
show that the gas flow rate through the annulus increases by increasing the distance between the gas inlet nozzle and the bottom of the draft
tube, that is, the height of the entrainment zone, but decreases with increasing draft tube diameter and mass fraction of finer particles. The
porous draft tube shows a higher gas flow rate through the annulus than the non-porous draft tube, particularly in the case of the low height of
the entrainment zone. The solids circulation rate increases with increasing gas velocity, the height of the entrainment zone and the porous
draft tube diameter. Moreover, the porous draft tube leads to a higher solids circulation rate than the non-porous draft tube.
D 2002 Elsevier Science B.V. All rights reserved.
Keywords: Spouted beds; Porous draft tube; Binary particle mixtures; Minimum spouting velocity; Annulus gas flow rate; Solids circulation rate
0032-5910/02/$ - see front matter D 2002 Elsevier Science B.V. All rights reserved.
doi:10.1016/S0032-5910(02)00321-2
T. Ishikura et al. / Powder Technology 131 (2003) 56–65 57
For these applications as shown in Table 1, a binary Fig. 2 shows the experimental apparatus for a batch
particles system is of practical importance. For conventional system under steady state conditions, and Table 2 indicates
spouted beds of binary mixtures of particles, Ishikura et al. the experimental conditions and particle properties. The
[27], Uemaki et al. [28] and Anabtawi [29] determined the bed consists of a 0.10-m ID acrylic column DT with a
Table 1
Characteristics for a spouted bed without and with a draft tube
Type of bed Design parameters Advantages Limitations Application
[1] Conventional spouted . Diameter of column DT . Simple grid design . Limitation on geometry . Drying of grains and
bed without a draft tube . Diameter of nozzle DO . Regular solids circulation and operation suspensions
. Cone angle h . Good solids mixing for . Limitation of bed height . Coating of particles
. Spout diameter DS coarse solids . Somewhat narrower . Granulation of particles
. Maximum spouted . Low pressure drop particle size . Gas cleaning
bed height Hm . Good fluidization for sticky . Poor spouting for fine particle . Coal gasification
or lumpy solids . Chemical products
[2A] Spouted bed with a . Diameter of draft . No limitation of bed height and . Complex design . Drying of grains and
non-porous (impermeable) tube DD particle size uniformity . Reduced mixing suspensions
draft tube . Entrainment zone . Greater operation flexibility . Plugging of draft tube . Coating of particles
(Draft tube clearance) . Lower gas flow and pressure drop . Reduced contact between . Granulation of particles
HD . Narrower spread of solid RTD gas and solids . Coal gasification
. More control of solid circulation . Lower heat and mass transfer . Combustion
. Pyrolysis hydrocarbon
. Pneumatic conveying
[2B] Spouted bed with a . Diameter of draft . Advantages of (2A) are retained . More complex design . Drying of grains and
porous (permeable) tube DD . More control of gas percolation . Plugging of draft of tube chemical products
draft tube . Entrainment zone HD through annulus . Thermal disinfestation
. Opening ratio of . Higher heat and mass transfer process
porous draft tube b
58 T. Ishikura et al. / Powder Technology 131 (2003) 56–65
Fig. 2, pressure taps are attached for measuring the total bed
pressure drop DPS, the total pressure drop within the draft
tube DPD, and the pressure drop of the annulus DPA,
respectively. Longitudinal pressure distributions PA and
PD were measured at intervals of 0.02 m by inserting a
pressure probe into the annulus or the draft tube. Here the
pressure drop of the annulus was used to calculate the
superficial gas velocity through the annulus UA. A relation-
ship between the pressure gradient DPA/L and the superficial
gas velocity UA for the annulus was calibrated from the
measurements taken under the state of the loosely packed
bed for each of the mass fraction of finer glass beads CS.
The experimental data could be approximated by quadratic
equations. The equations regarding DPA and UA were
determined by the least squares method for the each average
mass fraction of finer particles. For example, for CS = 0.05,
the following equation was used assuming uniform gas flow
in a horizontal plane:
QT ¼ U AT ¼ UA AA þ UD AD ¼ QA þ QD ð2Þ
Fig. 2. Schematic diagram of experimental apparatus and the details of
optical fiber probe. where QT is total gas flow rate through inlet nozzle, U is
superficial gas velocity in column and UD is superficial gas
velocity within draft tube. To a first approximation, the gas
conical base having an included angle h of p/3 radian and
flow into the draft tube QD is calculated by subtracting the
an inlet nozzle diameter DO of 0.012 m. The porous draft
gas flow rate through the annulus QA from the total gas flow
tubes are 0.30 m long with diameters DD in the range of
rate QT.
0.012 – 0.018 m. The height of the entrainment zone HD,
Before a spouted bed with a draft tube can be used as a
which indicates the distance between the gas inlet nozzle
stable efficient solid – gas contacting reactor, the solids
and the bottom of the draft tube, was varied from 0.02 to
circulation rate WS and the hold-up of solid particles within
0.04 m. This range was determined from a viewpoint of the
the draft tube (1 eD) must be known since these two
stability of spouting and the clogging of solid particles in
parameters are closely related to the state of stable spouting.
relation to the diameter of solid particles used [2]. The
WS is calculated from the mass balance of particles in the
porous-wall draft tube is made from sintered metallic filter
annulus as shown in Eq. (3) by using the experimental value
of stainless steel with the pore diameter of 120 Am and the
void fraction of about 40%. Permeability of the sintered Table 2
metallic filter is given experimentally as a function between Experimental conditions
the pressure drop DP and superficial gas velocity Ur through Column
it, that is, DP =0.74Ur + 3.17Ur2. Two different sizes of glass Inside diameter DT [m] 0.10
beads were used. The coarser particles have an arithmetic Nozzle diameter DO [m] 0.012
mean particle diameter of 1351 Am and the finer particle is Cone angle h [rad] p/3
477 Am in size. Therefore, the ratio of the particle diameters
Porous draft tube (sintered metallic filter, material: stainless steel)
is 2.83. About 3 kg of glass beads corresponding to a static Inside diameter DD [m] 0.012, 0.014, 0.018
bed height of 0.30 m were spouted at a given gas velocity. Tube length LD [m] 0.30
The average mass fraction of finer particles CS is 10 kinds as Distance of HD [m] 0.02, 0.03, 0.04
shown in Table 2. However, as mentioned above, CS = 0.05 entrainment zone
was used except for the measurement of minimum spouting
Particle (glass beads)
gas velocity Ums or gas velocity through annulus UA. Diameter DP [Am] 1351 (G1), 477 (G2)
Air was used as the spouting fluid and its flow rate was DPB/DPS = 2.83
measured by using a quadrant nozzle flow rate meter. The Density qP [kg/m3] 2480
superficial gas velocity U based on the cross-sectional area Mass fraction of CS [kg/kg] 0.00, 0.01, 0.03, 0.05, 0.10,
finer particles 0.15, 0.25, 0.50, 0.75, 1.00
of column was varied from 0.10 to 0.90 m/s. As shown in
T. Ishikura et al. / Powder Technology 131 (2003) 56–65 59
where S is the effective distance between light detecting Fig. 3. Typical pressure drop-flow rate curves for fluidization, and spouting
fibers and sm is the average lag time calculated by FFT without and with a draft tube (FB: fluidized bed; CSB: conventional
analyzer for the data of about 10 second periods. S in Eq. (4) spouted bed; S-DSB: spouted bed with a non-porous draft tube; P-DSB:
was calibrated as S = 1.016 mm. The hold-up of solid spouted bed with a porous draft tube).
particles within the draft tube (1 eD) was determined from
Eq. (5) based on mass balance of particles within the draft
tube by using both VPS measured by an optical fiber probe spouting velocity Ums of spouting with a draft tube (DSB) is
and WS calculated from Eq. (3). much lower than the others.
For spouting with a porous draft tube, Fig. 4 shows a
ð1 eD Þ ¼ Ws =ðqP AD VPS Þ ð5Þ relationship between the total bed pressure drop DPS and
superficial gas velocity U with the height of the entrainment
zone HD as a parameter for the case where the mass fraction
3. Experimental results and discussion of finer particles is CS = 0.05. This figure shows that DPS
decreases with a decrease in U for the stable spouting
3.1. Spouting characteristics of a binary mixture of fine – region. Furthermore, when the spouting state changes from
coarse particles for porous draft tube stable spouting into fixed bed region, the transitional point
is regarded as minimum spouting velocity Ums. The Ums
A total bed pressure drop DPS is important from a was defined as the velocity at a point where a slight
viewpoint of the stable spouting. In the case of the mass reduction of gas velocity caused solid particles within a
fraction of finer particles CS = 0.05, Fig. 3 shows the porous draft tube to clog and at the same time the pressure
relationship between the typical total bed pressure drop drop rose suddenly. From Fig. 4, it is found that both DPS
DPS and superficial gas velocity U for fluidization (FB), and Ums increase with increasing HD. The reason is that the
and spouting without a draft tube (CSB) and with a non- gas flow through the annulus increases with increasing HD
porous (S-DSB) and a porous (P-DSB) draft tube. As shown as shown in Fig. 10. Also, both DPS and Ums for spouting
in Fig. 3, DPS for spouting with a draft tube (DSB) is lower with a porous draft tube are higher than for spouting with a
than those of others. Therefore, DSB has a considerable non-porous tube, particularly at a lower height of the
advantage from the viewpoint of power consumption. DPS entrainment zone HD. This is due to the decrease of the
for spouting with a porous draft tube (P-DSB) is higher than energy of vertical gas stream entering from bottom of the
for a non-porous draft tube (S-DSB), due to gas percolation porous draft tube by the radial gas percolation through a
from the draft tube to the annulus. Moreover, the minimum porous draft tube.
60 T. Ishikura et al. / Powder Technology 131 (2003) 56–65
3.2. Gas flow rate through the annulus for porous draft tube
The variations of reduced longitudinal pressure with Fig. 6. Effect of average mass fraction of coarser component and HD on
reduced bed level Z/H for the spout and the annulus with minimum spouting velocity for a porous and a non-porous draft tube.
T. Ishikura et al. / Powder Technology 131 (2003) 56–65 61
Fig. 8. Relationship between gas flow rate through annulus and vertical distance as parameters of CS and radial ordinate r for a porous draft tube.
62 T. Ishikura et al. / Powder Technology 131 (2003) 56–65
Fig. 10. Relationship between gas flow rate through annulus and total gas
flow rate as a parameter of HD for a porous draft tube.
Fig. 9. Effect of U on gas velocity through annulus and gas velocity within
draft tube with CS as a parameter for a porous draft tube.
Fig. 12 shows that WS increases with increasing U and
HD. It is considered that as U increases, the entrainment of
the opposite tendency. In this experiment, it is indicated that solid particles in the entrainment zone increases, and there-
UA is lower than minimum gas velocity for fluidization Umf fore WS increases monotonously with U in the same manner
as shown in Fig. 9, and therefore the annulus region is a
stable moving bed.
Fig. 10 plots the gas flow rate through the annulus QA/QT
and the total gas flow rate QT with HD as a parameter.
QA/QT increases with decreasing QT and with increasing HD
for each of the systems. This is because the gas jet expands
with decreasing QT and with increasing HD. The porous
draft tube provides a higher QA/QT than the non-porous
draft tube, particularly in the narrower HD because of a
considerable decrease in the static pressure for the annulus
zone of cone section as shown in Fig. 7. From the viewpoint
of gas distribution to the annulus, the porous draft tube has
an advantage over the non-porous wall tube in the lower
height of the entrainment zone.
Fig. 11 indicates the effect of the porous draft tube
diameter DD on QA/QT. QA/QT increases with decreases in
DD for each of the systems. From this figure, QA/QT for
spouting with a porous draft tube is higher than for a non-
porous draft tube for every condition.
Fig. 12. Relationship between solids circulation rate and U as a parameter Fig. 13. Relationship between solids circulation rate and U as a parameter
of HD for a porous draft tube. of DD for a porous draft tube.
of finer particles CS = 0.05 and 0. The VPS was measured by with decreasing UD within the stable spouting region. When
an optical fiber probe as shown in Fig. 2. From Fig. 14, VPS the behavior of particles changes from stable spouting to the
increases linearly with increasing UD and VPS is almost the fixed bed, the transition point is regarded as minimum
same for CS = 0.05 and 0, probably due to a small fraction of spouting velocity within the draft tube UDms. UDms is about
finer particles. 83% of the coarser particle terminal velocity UT for both
Fig. 15 shows the effects of both superficial gas velocity CS = 0.05 and CS = 0. This ratio does not change in spite of
within draft tube UD and average mass fraction of finer different geometric and operating conditions as found from
particles CS on total pressure drop within the draft tube DPD past research [25]. UDms depends only on the void fraction
and hold-up of solid particles within the draft tube (1 eD). eD within the draft tube, similar to hindered settling. This
The results show that the behavior of both gas and solid finding is different from the tendency of the minimum
particles within the draft tube is similar to that for vertical spouting velocity Ums as shown in Figs. 4 and 5, which
pneumatic conveying. (1 eD) was calculated from the indicates the index on the beginning points of the whole
mass balance within the draft tube as shown in Eq. (5), spouting system for different geometric and operating con-
using the local velocity of particles VPS as shown in Fig. 14. ditions.
It is shown that DPD and (1 eD) are almost the same for On the other hand, (1 eD) increases gradually as UD de-
CS = 0.05 and CS = 0, probably because of the small mass creases. Furthermore, when (1 eD) reached about 0.06, the
fraction of finer particles. However, minimum spouting behavior of particles within the draft tube could not maintain
velocity Ums and gas velocity through annulus UA are not the stable pneumatic conveying state and a slight reduction of
equivalent for CS = 0.05 and CS = 0, respectively, as shown gas velocity within the draft tube caused solid particles within
in Figs. 6 and 9, due to notable effect of average void the draft tube to clog. Therefore, the pressure drop DPD and
fraction within annular bed flow eA. Also DPD for spouting hold-up of solid particles (1 eD) within the draft tube play
with a porous draft tube is higher than for a non-porous draft important roles in maintaining stable spouting.
tube due to the larger kinetic energy of solid particles within
the porous draft tube. The kinetic energy of particles
decreases with decreasing UD. Therefore, DPD decreases 4. Conclusions
List of symbols
AA cross-sectional area of annulus, ( = p(DT2 DD2)/4),
Fig. 15. Effect of gas velocity within draft tube on both total pressure drop
(m2)
within draft tube and hold-up of solid particles within draft tube as a AD cross-sectional area of draft tube, ( = pDD2/4), (m2)
parameter of CS for a porous draft tube. AT cross-sectional area of bed, ( = pDT2/4), (m2)
T. Ishikura et al. / Powder Technology 131 (2003) 56–65 65