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The concept of topological phases is a powerful framework for characterizing ground SSH model for hard-core bosons
states of quantum many-body systems that goes beyond the paradigm of symmetry The SSH model is formulated on a one-dimensional
breaking. Topological phases can appear in condensed-matter systems naturally, whereas lattice with an even number of sites N and stag-
the implementation and study of such quantum many-body ground states in artificial gered hopping of particles (Fig. 1A). It is conve-
matter require careful engineering. Here, we report the experimental realization of a nient to divide the lattice into two sublattices:
T
Hamiltonian is
he concept of symmetry breaking can be perimental studies of topological phenomena at X
H¼ Jij ½b†i bj þ b†j bi ð1Þ
used to characterize a variety of quantum the single-particle level in classical systems such
i∈A;j∈B
phases. Topological quantum phases, how- as coupled mechanical oscillators (7, 8), radio-
ever, do not fit into this paradigm. The frequency circuits (9), optical devices (10–13), b†i
with (bi ) being the creation (annihilation)
most prominent example of a topological and plasmonic systems (14, 15). Similar studies operator of a particle on site i. In the original
phase is the integer quantum Hall state with its were conducted also in quantum systems such formulation of the SSH model, the particles
robust edge states, giving rise to a quantized as ultracold atoms (16–22), where atomic inter- are noninteracting fermions. Here we con-
Hall conductance (1). The prediction of topo- actions were either negligible (16–21) or used sider hard-core bosons for which the operators
logical insulators (2) revealed another class of only to fill up Bloch bands (22), but the observed b†i (bi ) satisfy bosonic commutation relations
topological states of matter, denoted as symmetry- physics could be explained by a noninteract- on different sites i ≠ j, and additionally the
protected topological phases (SPTs). They occur in ing model. hard-core constraint ðb†i Þ2 ¼ 0, as two bosons
systems that display an excitation gap in the bulk By contrast, the ground state of noninteract- cannot occupy the same site i. In our realization,
(i.e., bulk insulators) and are invariant under a ing bosons is a Bose-Einstein condensate. There- the nearest-neighbor hoppings are dominating—
global symmetry. Their defining property is that fore, bosonic SPT phases only appear in systems with J denoting the strong link and J′ the weak
the ground state at zero temperature cannot be with interactions between the particles. Their link, i.e., jJ′j < jJj (Fig. 1, C and D)—and are
transformed into a conventional insulating state classification requires the analysis of the quan- sufficient to describe the qualitative behavior of
upon deformations of the system that do not close tum many-body ground state and is based on the model. For quantitative comparison between
the excitation gap or violate the symmetry. In group cohomology (23, 24). A notable example theory and experiment, we do not restrict our
particular, the zero-energy edge states are ro- is the Haldane phase of the antiferromagnetic system to the nearest-neigbor approximation.
bust to any perturbation commuting with the spin-1 chain (25), which has been experimentally At the single-particle level, the spectrum of
symmetry operators. observed in some solid-state materials (26, 27). In the Hamiltonian in Eq. 1, shown in Fig. 2A, is
SPT phases were first predicted and observed the context of artificial matter, interactions have obtained by diagonalizing the coupling matrix
in materials in which the interaction between been introduced between bosonic particles in a Jij . It displays two bands separated by a spec-
electrons can be effectively neglected (3, 4). In system with a topological band structure (28, 29), tral gap 2ðjJj jJ′jÞ; depending on the end
this specific case of noninteracting fermions, but studies were restricted to the two-body limit, links of the chain, there may or may not be in-
SPT phases can be classified based on the action still far from the many-body regime. gap localized zero-energy edge modes. There are
of the Hamiltonian on a single particle (5, 6). Here, we report the realization of a many- two such modes for a chain ending with weak
Thus, the appearance of robust edge states is body SPT phase of interacting bosonic particles links J′ (topological configuration, Fig. 1C) and
fully understood from the single-particle eigen- in an artificial system. Our setup is based on none if the chain ends with strong links J
states. This notable simplification motivated ex- a staggered one-dimensional chain of Rydberg (trivial configuration, Fig. 1D). The topology
atoms, each restricted to a two-level system, res- of the bands emerges from the sublattice (or
1
Laboratoire Charles Fabry, Institut d’Optique Graduate onantly coupled together by the dipolar interac- chiral) symmetry of the SSH Hamiltonian (5, 6),
School, CNRS, Université Paris-Saclay, 91127 Palaiseau Cedex, tion (30). We use this system to encode hard-core which notably constrains the hopping matrix
France. 2Institute for Theoretical Physics III and Center for bosons—i.e., bosonic particles with infinite on- Jij to connect only sites of different sublattices—
Integrated Quantum Science and Technology, University
site interaction energy–coherently hopping along e.g., next–nearest-neighbor hoppings Ji;iþ2 ¼ J″
of Stuttgart, 70550 Stuttgart, Germany.
*These authors contributed equally to this work. the chain. The system then realizes a bosonic are forbidden (see below for the experimental
†Corresponding author. Email: sylvain.leseleuc@institutoptique.fr version of the Su-Schrieffer-Heeger (SSH) model realization). The existence and degeneracy of
edge modes are topologically protected from of individually trapped 87Rb atoms (37–39) Rydberg p-level is lost from the structure. The
any perturbation that does not break the sub- (Fig. 1, C and D). The motion of the atoms is detection errors are at the few percent level (35).
lattice symmetry. These single-particle proper- frozen during our experiment, occurring in a For each experimental run, we thus obtain the
ties of the coupling matrix Jij defining the SSH few microseconds. Coupling between the atoms occupancy of each site, which is then averaged
model have been observed in many platforms, is achieved, despite the large interatomic distance by repeating the experiment every ~0.3 s.
such as ultracold atoms (32, 33), polaritons in an (~10 µm), by preparing the atoms in Rydberg To implement the sub-lattice symmetry, we use
array of micropillars (14), or mechanical gran- states for which the dipole-dipole coupling is en- the angular dependence of the dipolar coupling
ular chains (34). hanced to a few megahertz (30, 40). Jij ¼ d 2 ð3cos2 qij 1Þ=R3ij with d the transition
We now turn to the properties of the quan- We first prepare each atom in a Rydberg s-level, dipole moment between the two Rydberg lev-
tum many-body ground state corresponding to j60S1=2 ; mJ ¼ 1=2i , using a two-photon stimu- els. The hopping depends on the separation
a bulk–half-filled chain. For noninteracting fer- lated Raman adiabatic passage (STIRAP) with an Rij , as well as the angle qij with respect to the
mions, the properties of the SSH chain follow efficiency of 95% (35). From there, the atom can quantization axis defined by the magnetic field
from the Fermi sea picture based on the single- be coherently transferred to a Rydberg p-level, Bz ≃ 50 G. In Fig. 1A, we show the measured
particle eigenstates: In the trivial configuration j60P1=2 ; mJ ¼ 1=2i, by using a microwave field angular dependence, p vanishing
ffiffiffi at the “magic
one obtains a single insulating ground state, tuned to the transition between the two Rydberg angle” qm ¼ arccosð1= 3Þ ≈ 54:7°, which allows
whereas in the topological configuration, (i) an levels (E0 =h ∼ 16:7 GHz). The detuning from the us to suppress the hopping along this direction.
excitation gap appears in the bulk, and (ii) the transition is denoted Dmw , and the Rabi frequency By arranging the atoms in two subchains aligned
ground state is fourfold degenerate as the two is Wmw =ð2pÞ ∼ 0:1 to 20 MHz. We denote the state along the magic angle, we satisfy the sublattice
zero-energy edge modes can be either empty or with all Rydberg atoms in the s-level as the symmetry. The measured nearest-neighbor
occupied. For interacting bosons, the descrip- “vacuum” j 0i of the many-body system, whereas couplings are J=h ¼ 2:42ð2Þ MHz and J 0 =h ¼
tion of the many-body ground state is much a Rydberg atom at site i excited in a p-level is 0:92ð2Þ MHz, in full agreement with numer-
more challenging. In the special case with only described as a bosonic particle, b†i j0i. Because ical determination of the pair potential (41). The
nearest-neighbor hoppings J and J′, the bosonic each Rydberg atom can only be excited once to dipolar interaction also gives rise to longer-range
The single-particle spectrum is probed by mi- For any finite chain, the left and right edge logical configuration exhibits four degenerate
crowave spectroscopy (Fig. 2A). Initializing the modes hybridize to form symmetric and anti- ground states corresponding to the bulk half-
vacuum state j0i with all Rydberg atoms in the symmetric states with an energy difference filled, and which are characterized by zero, one,
s-level, a weak microwave probe with a Rabi Ehyb º J′jJ′=JjN , which breaks the degeneracy or two additional particles mainly residing at
frequency Wmw =ð2pÞ ¼ 0:2 MHz applied for a of the edge modes but decreases exponentially the edges. To prepare the ground state, we per-
time t ¼ 0:75 ms can lead to the coherent cre- with the chain length N . This remains negli- form a microwave adiabatic sweep (Fig. 3A),
ation of a particle only if an eigenstate energy gible compared to our experimental time scale where the final detuning Df plays the role of a
matches the microwave detuning Dmw and if for a long chain of 14 sites (Ehyb ≃ h 20 kHz), chemical potential, tuning the number of par-
this state is coupled to j0i by the microwave but the hybridization is observable for smaller ticles loaded in the chain. From a theoretical
field. We show in Fig. 2B the site-resolved chains. Notably, it gives rise to a coherent trans- analysis simulating the full time-evolution, we
probability of finding a particle on a given site fer of a particle between the two boundaries expect that our ramping procedure ending at
for the two different chain configurations. In without involving the bulk modes, as sketched a final detuning jℏDf j < jJj jJ′j prepares the
both cases, we observe a clear signal for ℏDmw < in Fig. 2D. To observe this, we prepare a par- ground state with high fidelity (35).
jJ′j jJj from lower band modes delocalized ticle on the leftmost site using a combination We present in Fig. 3, D and E, the depen-
along the chain. States in the upper band are of an addressing beam and microwaves sweeps dence of the local density of particles on Df : The
not observed as the microwave coupling from (42), and then let the system evolve freely. We bulk sites’ occupancy (blue symbols) exhibits
j0i to these states is very small. Only in the topo- show in Fig. 2E the experimental results for a characteristic plateau at half-filling within
logical configuration do we observe an addi- three chains of four, six, and eight sites. The the single-particle gap. The fluctuations of the
tional signal localized at the boundaries around energy Ehyb is determined from the frequency number of particles in the bulk are strongly
zero energy, corresponding to the two edge of transfer and exhibits the expected exponen- reduced with a measured probability of 48%
modes. The finite width of the signal is caused tial scaling (Fig. 2F), in excellent agreement to find exactly six particles on the 12 bulk sites
by microwave power broadening (35). In Fig. with theoretical calculations, including the full [mainly decreased from 100% by detection er-
2C, we quantitatively show the localization of hopping matrix Jij (35). rors (35)]. The local bulk properties are inde-
A B C
D E F
Fig. 2. Single-particle properties. (A) Single-particle spectrum for the edges. The dashed line indicates the 2% noise level caused by preparation
trivial and the topological configuration probed by microwave spectroscopy. and detection errors. (D) Particle transfer between the two edges. A particle
Right: A selection of single-particle wave functions. (B) Experimental on the left edge is essentially a superposition of the symmetric and
site-resolved spectra showing the averaged occupancy of each site as a antisymmetric zero-energy modes, split in energy by Ehyb owing to the
function of Dmw . The lower-band bulk states are always observed, whereas hybridization for finite chains. (E) Observation of the transfer for chains of
states in the upper band are not visible as their microwave coupling to j 0i is N = 4, 6, and 8 sites after injecting a particle on the leftmost site. (F) From the
either weak or completely inhibited. Edge states at zero energy appear only transfer frequency, we obtain the hybridization energy Ehyb (red circles)
for the topological configuration. The white dashed lines indicate the and compare it to calculations, keeping only nearest-neighbor hoppings
calculated gap. (C) Spatial distribution of the edge states, observed (red bars) (dashed line) and including the full dipolar interaction (solid line).
and calculated (black crosses), showing an exponential localization on the All theoretical results are obtained by diagonalizing the coupling matrix.
density around Df ¼ 0, even in the trivial con- The picture remains valid even in our regime from the trivial state by a finite value of the string
figuration, is caused by preparation errors cre- where jJj ≃ 2:6jJ′j. We measure a large and neg- order parameters C x and C z (23, 43) with
ative density-density correlation C z ð2i; 2i þ 1Þ ¼
h i
ating lattice defects. A defect gives rise to two
X
N 2
chains, one of which starts with a weak link, and hZ2i Z2iþ1 i ≃ 0:67ð1Þ with Zi ¼ 1 2b†i bi , cor- ip2 Zk
thus supports a zero-energy edge state, which responding to a suppressed probability of finding z
Cstring ¼ Z2 e k¼3 ZN1
gets populated when Df becomes positive. In- two particles on the same dimer. We also access ð3Þ
cluding preparation and detection errors in the the off-diagonal correlations, C x ði; jÞ ¼ hXi Xj i
simulation (solid lines) gives an excellent agree- with Xi ¼ bi þ b†i measuring the coherence be- x
and in analogy for Cstring . Indeed, we measure a
ment with the experimental data (35). tween two sites i and j , by applying a strong finite string order in the topological phase with
We gain more insight into the many-body microwave pulse before the detection, which z
Cstring ¼ 0:11ð2Þ and Cstring
x
¼ 0:05ð2Þ, whereas in
state by analyzing the correlations between par- rotates the local measurement basis around the the trivial phase they are consistent with zero,
ticles, which we can measure because our de- Bloch sphere. We obtainC x ð2i; 2i þ 1Þ ≃ þ0:48ð2Þ, z
e.g., Cstring ¼ 0:02ð3Þ. All measured correlators
tection scheme provides the full site-resolved indicating that a particle is coherently and sym- are in good agreement with simulations.
particle distribution. In the strongly dimerized metrically delocalized on two sites, forming a We now demonstrate the degeneracy of the
regime jJj≫jJ′j, we expect the ∼ N =2 particles in dimer. Furthermore, our detection scheme allows many-body ground state in the topological phase
the bulk to be highly correlated as they can us to determine string order parameters. For our and the bulk excitation gap. We first prepare
minimize their energy by each delocalizing on a experimental implementation, the theory pre- a six-particle many-body ground state with the
dimer (two sites connected by a strong link J ). dicts that we can distinguish the topological state bulk at half-filling but empty edge states by an
Fig. 4. Probing the SPT phase degeneracy and bulk excitation gap. with six particles (solid circle), we can (i) reach one of the other
(A) A microwave sweep ending at Df =ð2pÞ ¼ 1 MHz first prepares the degenerate ground states by adding a particle at the edge for zero energy
many-body ground state with six particles, and we then apply for 2 µs a cost. In addition, we can probe the bulk excitation gap by (ii) adding a
microwave probe with a Rabi frequency Wmw =ð2pÞ ¼ 0:3 MHz and a variable particle to, or (iii) removing a particle from, the bulk. (C) Measured
detuning Dmw . (B) Magnified view of the bottom of the energy spectrum occupancy of bulk (blue circles) and edge sites (green and brown circles)
of a chain in the topological configuration. Starting from the ground state showing the three expected transitions. Error bars are SEMs.
fermionic SSH model and correspondingly Discussion and outlook 29. M. Di Liberto, A. Recati, I. Carusotto, C. Menotti, Phys. Rev. A
94, 062704 (2016).
leads to a splitting of the single-particle edge We prepared quantum many-body states in two 30. A. Browaeys, D. Barredo, T. Lahaye, J. Phys. B 49, 152001
modes. However, such a perturbation commutes topologically different phases and observed (2016).
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1698–1701 (1979).
many-body ground state degeneracy. To check bosons: (i) a ground state degeneracy charac- 32. M. Atala et al., Nat. Phys. 9, 795–800 (2013).
these expectations, we first repeat the spectro- terized by zero-energy edge states, (ii) an exci- 33. E. J. Meier, F. A. An, B. Gadway, Nat. Commun. 7, 13986
scopic measurement in the single-particle regime tation gap in the bulk, (iii) a nonvanishing string (2016).
(applying the microwave probe on an empty order, and (iv) a robustness of these properties 34. R. Chaunsali, E. Kim, A. Thakkar, P. G. Kevrekidis, J. Yang,
chain, as shown in Fig. 2A), and observe a split- against perturbations respecting the protecting Phys. Rev. Lett. 119, 024301 (2017).
35. See supplementary materials.
ting of the edge modes (Fig. 5B). By contrast, the symmetry S B . 36. F. Grusdt, M. Höning, M. Fleischhauer, Phys. Rev. Lett. 110,
spectroscopic measurement for the bosonic many- The symmetry protecting our SPT phase de- 260405 (2013).
body ground state (applying the probe after the fines the symmetry group U ð1Þ ℤT2 , which can 37. H. Kim et al., Nat. Commun. 7, 13317 (2016).
adiabatic preparation reaching half-filling of the also protect the Haldane phase of an antiferro- 38. M. Endres et al., Science 354, 1024–1027 (2016).
bulk, as done in Fig. 4) indeed reveals a quasi- magnetic spin-1 chain (25). We show numerically 39. D. Barredo, S. de Léséleuc, V. Lienhard, T. Lahaye, A. Browaeys,
Science 354, 1021–1023 (2016).
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(35) by using simulations that include van der state, as they can be smoothly connected by 41. S. Weber et al., J. Phys. B 50, 133001 (2017).
Waals interactions. We also checked that when adding hopping terms with complex amplitudes 42. S. de Léséleuc, D. Barredo, V. Lienhard, A. Browaeys,
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jJj jJ′j, the spectroscopic measurement reveals Our work demonstrates that Rydberg plat- 44. S. Weber et al., Quantum Sci. Technol. 3, 044001
a symmetry-protected ground state degeneracy. forms, which combine flexible geometries and (2018).
45. S. de Léséleuc, Replication data and theory code for: QUANTICA and XYLOS) and from the IXCORE-Fondation pour la SUPPLEMENTARY MATERIALS
Experimental realization of a symmetry protected topological Recherche. H.P.B. is supported by the European Union under the science.sciencemag.org/content/365/6455/775/suppl/DC1
phase of interacting bosons with Rydberg atoms. Zenodo ERC consolidator grant SIRPOL (grant no. 681208). Author Supplementary Text
(2019). contributions: S.d.L., V.L., P.S., and D.B. carried out the experimental Figs. S1 to S8
measurements and data analysis; S.W. and N.L. performed the Table S1
ACKN OW LEDG MEN TS theoretical analysis. All work was supervised by H.P.B., T.L., and References (46–71)
Funding: This project has received funding from the European A.B. All authors contributed to the writing of the manuscript.
Union’s Horizon 2020 research and innovation program under Competing interests: The authors declare no competing interests. 31 October 2018; accepted 18 July 2019
grant agreement no. 817842 (PASQuanS), from “Investissements Data and materials availability: The experimental data and theory Published online 1 August 2019
d’Avenir” LabEx PALM (ANR-10-LABX-0039-PALM, projects code of this study are available at (45). 10.1126/science.aav9105