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Article history: In-vessel retention (IVR) of core melt is a key severe accident management strategy adopted by most
Received 23 November 2009 operating nuclear power plants and advanced light water reactors (ALWRs), AP600, AP1000, etc. Exter-
Received in revised form 25 March 2010 nal reactor vessel cooling (ERVC) is a novel severe accident management for IVR analysis. In present
Accepted 13 April 2010
study, IVR analysis code in severe accident (IVRASA) has been developed to evaluate the safety margin
of IVR in AP1000 with anticipative depressurization and reactor cavity flooding in severe accident. For,
IVRASA, the point estimate procedure has been developed for modeling the steady-state endpoint of two
core melt configurations: Configuration I and Configuration II. The results of benchmark calculations of
AP600 by IVRASA were consistent with those of the UCSB and INEEL. Then, IVRASA is used to calculate
the heat transfer process caused by two core melt configurations of AP1000. The results of calculations
of Configuration I indicate that the heat flux remains below the critical heat flux (CHF), however, the
sensitivity calculations show that the heat flux in the metallic layer could exceed the CHF because of the
focusing effect due to the thin metallic layer. On the other hand, the results of calculations of Configu-
ration II suggest that the thermal failure of the lower head at the bottom location is highly unlikely, but
the heat flux in light metallic layer could be higher than that of base case due to the portion of metal
partitioning into the lower head. This work also investigated the effect of the uncertainties of the CHF
correlations on the analysis of IVR.
© 2010 Elsevier B.V. All rights reserved.
1. Introduction from the molten debris in the lower plenum. If the local heat flux
through the vessel wall exceeded the critical heat flux (CHF), vessel
The in-vessel coolability of a core melt is an important issue in failure would be expected.
addressing a postulated inadequate core cooling event in nuclear IVR of molten core debris inside reactor pressure vessel (RPV)
reactors. In such an even, a significant amount of core materials can lower head through external cooling by cavity water has been the
become molten and relocate downward into the lower head of the subject of numerous numerical and experimental investigations
reactor vessel, as happened in the Three Mile Island Unit2 (TMI-2) conducted by Kolev (1993), Theofanous et al. (1994a,b, 1996a,b),
accident. If it is possible to ensure the lower head to remain intact, Asfia and Dhir (1996), Chu et al. (1997), Rempe et al. (1997),
which can retain the relocated core materials, the enhanced safety Loktinonov et al. (1999), Esmaili and Khatib-Rahbar (2004) and
associated with these plants can reduce concerns about contain- Dinh et al. (2004).
ment failure and associated risks. For example, the Westinghouse Henry and Fauske (1993) investigated the capability of the
Advanced 600 MWe PWR (AP600) adopted ERVC with a flooded external cooling of the RPV lower head to prevent the lower head
reactor cavity as the enhanced safety. Subsequent advanced light failure considering the presence of the RPV insulation. Cheung et
water reactors, such as AP1000 and APR14000, also adopted this al. (1997) developed a subscale boundary layer boiling (SBLB) test
enhanced safety. facility to study the boundary layer boiling and critical heat flux
If the reactor cavity is flooded before melt relocated into the phenomena on a downward facing cured heating surface, and to
lower head, the vessel wall would be initially cool and the outer measure the spatial variation of the critical heat flux. Knudson
vessel wall would remain close to the cavity water saturation tem- and Rempe (2002) established IVR model to simulate heat transfer
perature. Boiling crisis is the sufficient and necessary condition for inside the accumulated molten pool, heat transfer from the molten
lower head failure (Theofanous et al., 1996a). Nucleate pool boil- pool to the reactor vessel, and heat transfer from exterior vessel
ing of the cavity water is an efficient mechanism for heat removal surfaces using SCDAP/RELAP5-3D.
Theofanous et al. (1996a) and Rempe et al. (1997) used one-
dimensional mathematical model to calculate the thermal response
∗ Corresponding author. Tel.: +86 29 82665607; fax: +86 29 82665607. of the lower head. They also provided a summary of the various
E-mail address: szqiu@mail.xjtu.edu.cn (S.Z. Qiu). heat transfer correlations for the ceramic pool and the stratified
0029-5493/$ – see front matter © 2010 Elsevier B.V. All rights reserved.
doi:10.1016/j.nucengdes.2010.04.020
2024 Y.P. Zhang et al. / Nuclear Engineering and Design 240 (2010) 2023–2033
Nomenclature
ıcr,t oxide crust thickness of the top of the oxide pool, m
A coefficient for estimating heat transfer from the sur- ıw thickness of the vessel wall, m
face of the melt pool, W/m2 K4 ε emissivity
Gr Grashoff number, =gˇTmax H3 / 2 ε1 emissivity of the top light metallic layer
g gravity acceleration, m/s2 angle from the bottom center of the lower head,
H height of the metallic layer, vertical size of the cav- degree
ity, m h maximum angle of the heavy metallic layer, degree
H depth of oxide pool, m kinematic viscosity, m2 s
k thermal conductivity, W/(mK) Stefan–Boltzmann constant (5.67 × 10−8 W/m2 K4 )
Nu Nusselt number, =(q H )/kTmax Tmax maximum bulk-wall temperature difference, K
Pr Prandtl number, =/˛
Q̇ volumetric heat generation rate, W/m3 Subscript
q average heat flux at pool boundaries, W/(m2 ) CHF critical heat flux
qh,b heat flux from the bottom of heavy metallic layer, cr ceramic crust
W/(m2 ) dn downward (over the hemispherical boundary)
ql,b heat flux from the top oxidic pool crust into the top h heavy metallic layer
l light metallic layer
light metal layer, W/(m2 )
o oxide pool
ql,t heat flux from the top light metallic layer into the
s upper plenum structures
internal atmosphere of the reactor, W/(m2 ) side the side of the oxide pool
ql,w heat flux from the top metallic layer into the vessel up upward (over the flat boundary of the oxidic pool)
wall, W/(m2 ) w vessel wall
qo,dn heat flux towards the bottom of oxidic pool, W/(m2 )
qo,h heat flux from the ceramic pool to the heavy metallic
layer, W/(m2 ) light molten metallic layer. Khatib-Rahber et al. (1996) adopted a
qo,up heat flux towards the top of oxidic pool, W/(m2 ) two-dimensional model. The comparison of the one-dimensional
qves heat flux from the outer surface of the vessel to and two-dimensional models showed that a one dimensional heat
water, W/(m2 ) transfer model of the lower head performed adequately. Esmaili
R reactor vessel, hemisphere radius, m and Khatib-Rahbar (2004, 2005) established a one-dimensional
R ratio of the Nusselt number model to assess the thermal response of the AP1000 lower head
Ra Rayleigh number (metallic layer), = based on two bounding melt configurations (Configuration I and
(gˇTmax H 3 )/(˛) Configuration II). Theofanous et al. (2004) analyzed the thermal
Ra Rayleigh number (oxide pool), = (gˇQ̇ H 5 )/(k˛) margins of AP1000 and provided experimental data to show that
S area of the melt pool, m2 it was reasonable to allow the robust extension of the AP600 IVR
Sdn area of the bottom of the oxide pool, m2 strategy for severe accident management to higher power reac-
Sh,b area of the bottom of the heavy metallic layer, m2 tors, and in particular, to the AP1000 advanced passive design. So
S1,b area of the bottom of the light metallic layer, m2 far, numerical investigations on IVR of AP1000 are few, and this is a
S1,t area of the top of the light metallic layer, m2 necessary part of the analysis in severe accident. Therefore, IVRASA
Sside area of the side of the oxide pool, m2 code was developed to analyze the safety margin of AP1000 during
Sup area of the top of the oxide pool, m2 severe accident in this work.
T temperature, K This paper consists of two main technical parts. The first part
Tbh bulk temperature of the heavy metallic layer, K (Section 2) presents the simple point estimate procedure (IVRASA)
Tbl bulk temperature of the light metallic layer, K based on the existing constitutive relations, originally developed
T1,b temperature of the bottom of light metallic layer, K for AP600 (Theofanous et al., 1996a; Rempe et al., 1997), and com-
T1,t temperature of the top of light metallic layer, K pare the results calculated by IVRASA with those of the University of
To,m melt temperature of oxide pool California–Stanta Barbara (UCSB) (Theofanous et al., 1996a) and the
Tw,m melt temperature of vessel wall Idaho National Engineering and Environmental Laboratory (INEEL)
Ts,i inner surface temperature of the internal structure, (Rempe et al., 1997). The second part (Section 3) applies IVRASA
K to calculate two core melt configurations of AP1000. And more
Ts,o outer surface temperature of the internal structure, details are conducted on the thermal margins of the AP1000 for
K Configuration II.
Tw,i inner surface temperature of the vessel wall, K
Tw,o outer surface temperature of the vessel wall, K 2. IVRASA and verification calculations
V volume of the melt pool, m3
IVRASA model is based on DOE/ID-10460 that the Department
Greek characters of Energy (DOE) contracted the UCSB to produce to support the
˛ thermal diffusivity, m2 /s Westinghouse position on AP600 IVR (Theofanous et al., 1996a)
ˇ thermal expansion coefficient, K−1 and the technical evaluation of AP600 IVR by INEEL (Rempe et al.,
ı the thickness, m 1997). The latter was developed by INEEL independently to verify
ıcr oxide crust thickness of the side of the oxide pool, the results of UCSB.
m The UCSB study regarded Configuration I (Fig. 1a) as the final
ıcr,b oxide crust thickness of the bottom of the oxide pool, steady state, their postulated FInal Bounding State (FIBS). A key
m assumption in the UCSB study was their assumed debris configura-
tion. And the UCSB study argued that their FIBS bounded thermal
Y.P. Zhang et al. / Nuclear Engineering and Design 240 (2010) 2023–2033 2025
Fig. 1. Alternate debris configurations evaluated for AP1000 (a) Configuration I and (b) Configuration II.
loads from any other configurations. However, INEEL’s review sug- equations (equation A-106) has been shown as follow:
gested that the UCSB FIBS did not involve several possible thermal
Q̇o ı2cr () qo,dn () Q̇o ıw ()
challenges from other debris configurations. So, INEEL gave Config- + ıcr () +
uration II as the final steady state (Fig. 1b). And INEEL recommended 2kcr kcr 2kw
Configuration II as assumed FIBS, which could contain other core
qo,dn ()ıw ()
melt configurations. − To,m + + Tw,o = 0 (5)
Configuration I assumes a molten ceramic pool of UO2 –ZrO2 kw
lying beneath a metallic layer of Fe–Zr, and Configuration II rep-
resents a case where sufficient uranium dissolves into unoxidized Tw,m − Tw,o
zirconium to form a heavier metallic layer of Fe–U–Zr in the bottom ıw () = kw (6)
qo,dn () + Q̇o ıcr ()
and a light metallic layer of Fe–Zr on the top with a molten ceramic
pool between the two metallic layers.
qves () = qo,dn () + Q̇ ıcr () (7)
2.1. IVRASA methodology Eqs. (5) and (6) were solved iteratively to get the value of the
thickness of the ceramic crust, then the heat flux to the water of
IVRASA is a point estimate procedure that is similar to the model the outer surface of the vessel could be obtained.
used in the UCSB report, and IVRASA contains equations similar to Light metallic layer:
the equations reported in the UCSB study. The governing equations
of the IVRASA model can be seen as follows, and more details about Q̇l Vl + ql,b Sl,b = ql,t Sl,t + ql,w Sl,w (8)
the property equations can be seen in UCSB report (Theofanous
kcr Q̇o ıcr,t
et al., 1996a). However, IVRASA was developed in a more general ql,b = (To,m − Tbl ) + (9)
manner so that it could calculate Configuration I and Configuration ıcr,t 2
II, besides Configuration I assumed as UCSB FIBS, and some modifi-
cations of the Rempe model equations have been shown here. The
melt pool Configuration II more bounded thermal loads from other
configurations (Rempe et al., 1997). So, the schematic of the melt
pool Configuration II is shown in Fig. 2, and the schematic of the
melt pool Configuration I is similar with the schematic of the melt
pool Configuration II.
As discussed above, the governing equations of the three lay-
ers are shown as follows (these equations are also suitable for the
Configuration I).
Oxidic pool:
Q̇o Vo
qo,dn = (2)
Sside + Sdn + Sup R
Nuup
R = (3)
Nudn
4 − T4 ]
[Tl,t Table 1
s,i
ql,t = (10) Comparison of IVRASA with UCSB FIBS.
(1/εl ) + ((1 − εs )Sl,t /εs Ss )
IVRASA UCSB
kw
ql,w = (Tw,m − Tw,o ) (11) Configuration I and Configuration II Configuration I assumed FIBS
ıw Portion of the decay heat in the All the decay heat resides in the
4 − T4 ) metallic layer ceramic pool
ıs (Tl,t s,i Emissivity from the metallic layer Emissivity from the metallic layer
Ts,o = Ts,i − (12)
ks (Ss /εl Sl,t ) + (1 − εs /εs ) may be represented by a point may be represented by a point
value of 0.29a value of 0.45
ks 0.25 Some additional heat sources due to No additional heat sources exist
4
Tw = Ts,o − Ts,i − Ts,o (13) oxidation or steel activations exist in the metallic layer
ıs εs in the metallic layerb
Table 2
Heat transfer correlations used in different models.
Ceramic pool
Top:
Theofanous et al. (1996b) ACOPO (1/2 scale):
Nuup =1.95Ra 0.18
for 1010 < Ra <3 × 106 .
Bottom:
Mayinger et al. (1975):
Nudn = 0.55Ra 0.22
Fig. 3. Comparison of IVRASA heat flux with UCSB (DOE/ID-10460) and INEEL heat for 7×106 < Ra <5 × 1014
fluxes assuming UCSB FIBS and input.
2. Constitutive correlation set used by UCSB in a steady state (Theofanous
et al., 1996a)
Metal
Side wall:
Churchill and Chu (1975):
Nu = 0.076Ra1/3 .
Ceramic pool
Top:
Theofanous et al. (1996b) Mini-ACOPO (1/8 scale):
Nuup = 0.345Ra 0.233
for 1012 < Ra < 3 × 1014 and 2.6 < Pr < 10.8
Bottom:
Theofanous et al. (1996b) Mini-ACOPO:
Nudn = 0.0038Ra 0.35
for 1012 < Ra < 3 × 1014 and 2.6 < Pr < 10.8
12
for 0.1 < Ra < 10 and any Pr.
Ceramic pool
Top:
Theofanous et al. (1996b) ACOPO (1/2 scale):
Nuup = 2.4415Ra 0.1722
Bottom:
Theofanous et al. (1996b) ACOPO (1/2 scale):
H 0.25
Nudn = 0.1857Ra 0.2304 R
for 1010 < Ra <3 × 1016
Table 4
Fractions of Zr oxidation and UO2 relocation calculated by MELCOR and MAAP.
Table 3
Relocation time and decay power calculated by MELCOR and MAAP.
Table 5
Mass of corium inventories for base case.
Fig. 10. IVRASA and Esmaili predictions for vessel wall thickness.
Fig. 9. IVRASA and Esmaili CHF ratios. Fig. 11. IVRASA and Esmaili oxide crust thickness.
2030 Y.P. Zhang et al. / Nuclear Engineering and Design 240 (2010) 2023–2033
results from each analysis are discussed below. The results of the 3.3. Results of melt Configuration II
two conditions are shown in Figs. 12 and 13.
Fig. 12 represents the condition of reduced metallic melt mass The formation of the heavy metallic layer in the lower head
that affects the height of the metallic layer. Because the metal- was proposed to analyze the vessel integrity of AP600 by INEEL in
lic layer has a higher thermal conductivity, the mass of metals 1997. From then on, numerous numerical and experimental inves-
assumed in the metallic layer significantly affects the estimated tigations have been conducted on modeling of the molten pool
magnitude of the heat fluxes focused toward the adjacent vessel structure and the thermal and physicochemical processes occurring
sidewall. If metallic melt mass is reduced, the excess of energy at the interaction of oxidic and metallic melt materials.
which come from the oxide pool and cannot be removed by Experiments performed at OECD MASCA facility (Asmolov et
radiation is focused through the vessel wall causing considerable al., 2004, 2007; Gusarov et al., 2006, 2007; Smirnov et al., 2007;
thermal attack of the vessel. This is so-called focusing effect. This Kiselev et al., 2007), ISTC CORPHAD facility (Bechta et al., 2006a,c,
focusing effect may be a challenge to the integrity of the vessel. 2007a,b) and METCOR facility (Bechta et al., 2004, 2006b) have
For point estimate calculations, IVRASA, respectively, assumed shown the potential for partitioning of the major constituents (U,
the metallic layer contains approximately 37,376 (base case), Zr, Fe) between suboxidized corium melt and steel in the IVR con-
20,000, 15,000 and 3000 kg of AP1000 vessel internal structure ditions. These tests show that the formation of the heavy metallic
steel. layer in the bottom of the vessel head due to component partition-
It can be seen from Fig. 12 that reductions in the steel relo- ing between suboxidized corium melt and steel. This stratification
cation mass only affect metallic layer results, because oxide pool is caused by the increased density of the metallic layer attributed to
heat fluxes are independent of metallic layer mass assumptions. As a transfer of uranium metal that was reduced from uranium oxide
shown in Fig. 12, CHF ratios at vessel locations in contact with the by interaction with Zirconium. Guéneau et al. (1998), Cheynet et al.
metallic layer approach unity for steel masses equal to 15,000 kg. (2002), Almyashev et al. (2002), Mazurin and Gusarov (2002) and
When the steel masses are below this value, CHF ratios are greater Smirnov et al. (2007) have conducted on the thermal and physico-
than unity. This may cause the vessel failure. Particularly, when the chemical processes during the molten pool formation in numerical
steel mass equals to 3000 kg that was the minimum steel mass cal- way. Seiler et al. (2007) proposed a methodology to assess corium
mass inventories and calculate the mass of steel in heavy metallic
layer with different fraction of Zr oxidation for a 1000 MW PWR.
For point estimate calculations of melt Configuration II, the
masses of the corium inventories for base case calculations as
discussed in the previous sections were adopted in this section
(Table 5). The advantage of IVRASA model is that it is convenient
to change the mass of unoxidized uranium in the bottom layer by
altering the value of the fraction of uranium that is in the oxide
form (fU ). The formation of fU is defined as:
mU 270
fU = 1 − (24)
MUO2 238
where MUO2 is the total mass of UO2 , and mU the mass of uranium
in the bottom layer.
Note that the formulas of the masses of uranium, steel and zir-
conium in the bottom layer remain the same with those given by
Esmaili and Khatib-Rahbar (2005). IVRASA calculation results of
Configuration II are shown as follows under different values of fU .
As discussed in previous sections, the reason for the stratifica-
tion is because the density of the bottom metallic layer composed of
Fig. 13. Comparison of CHF ratios with additional heat sources in the metallic layer. U–Zr–Fe is greater than that of the oxide pool. As shown in Table 6
Y.P. Zhang et al. / Nuclear Engineering and Design 240 (2010) 2023–2033 2031
Table 6
Portion of results of IVRASA calculations for Configuration II.
the bottom of the vessel lower head, and to the increase of the mass
of Zr in the light metallic layer (Fig. 15) that slightly mitigates the
focusing effect on the vessel locations adjacent to the light metallic
layer. The heat flux in light metallic layer is higher than that of base
case (Fig. 9) due to the portion of metal partitioning into the lower
head. It can be seen from Fig. 17 that the heat flux ratio for all the
calculations is well below the unity, so the increased focusing effect
in the light metallic layer due to portion of metal partitioning to the
bottom layer is slightly small.
Although IVRASA predicts that CHF ratios remain below unity
Fig. 14. The variation of density with respect to fU .
for Configuration II under different values of fU , there are poten-
tial factors affecting heat loads in the heavy metallic layer, such as
the inter-metallic reactions, oxidation in the heavy metallic layer.
and Fig. 14, we can see that densities of oxide layer and heavy Chevalier et al. (2004) performed a new thermodynamic modeling
metallic layer calculated by IVRASA are in agreement with these of the O–U–Zr system and suggested that the solubility of the oxy-
calculated by Esmaili, and the density of the bottom layer is greater gen existed in uranium–zirconium liquid. However, there are few
than that of the oxide layer. It can be seen from Fig. 14 that the investigations on the impact of the inter-metallic reactions and the
density of the bottom layer increases with an increase of the value oxidation in the heavy metallic layer. It is hard to determine the
of fU . The density of Zr is great smaller than that of uranium, so this quantifications of the impact of the inter-metallic reactions and the
may be due to the decrease of the mass of Zr in the bottom layer, oxidation in the heavy metallic layer, so the impact of the inter-
as shown in Fig. 15. metallic reactions and the oxidation in the heavy metallic layer
As shown in Figs. 16 and 17, we can see that the heat flux at needs additional experimental and analytic studies.
locations adjacent to the heavy metallic layer increases with an
increase of the value fU , and varies inversely with the value of fU in
3.4. Sensitivity analysis of CHF correlations for IVR analysis
the light metallic layer. It is due to the decrease of the total mass in
the heavy metallic layer (Fig. 15) that slightly focuses heat loads to
ERVC for AP1000 may not be successful without an enhanced
insulation design or other enhanced measures. It can be seen from
Fig. 18 that there is a very small margin of IVR calculation of AP1000
for Configuration I using AP600 CHF correlation (Eq. (22)). However,
if modified CHF correlation for AP1000 is used, there is a large ther-
mal margin of IVR calculation. Therefore, different margins of IVR
calculations could be obtained using different CHF correlations.
Theofanous et al. (2003) observed a strong effect of surface
condition in their experiments at the UPLU-V facility for AP1000.
They used the sand particles to roughen the test section sur-
faces modified the surfaces molecules properties, and found that
the molecular deposition of aluminum could be dissolved by de-
ionized water in some of tests, leading to a significant decrease
in the CHF values in subsequent tests. However, this degradation
effect was not observed in those tests using tap water rather than
de-ionized water. Therefore, there exists a large uncertainty in the
UPLU-V experimental data. Rempe et al. (2008) also suggested that
there was a large uncertainty in the CHF data. Moreover, recent
studies argued that nanofluids could be used to enhance the IVR
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