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Article history: The continuous soil gas radon monitoring is carried out at Palampur and the daily monitoring of radon
Received 2 April 2009 concentration in water is carried out at Dharamshala region of Kangra valley of North West Himalayas,
Received in revised form India, a seismic zone V, to study the correlation of radon anomalies in relation to seismic activities. In
19 May 2009
this study, radon monitoring in soil was carried out by using barasol probe manufactured by Algade
Accepted 25 May 2009
France, whereas the radon content in water was recorded using RAD 7 radon monitoring system of
Durridge Company USA. The effect of meteorological parameters viz. temperature, pressure, wind
Keywords: velocity, rainfall, and humidity on radon emission has been studied. The seasonal average value and
Radon in water standard deviation of radon in soil and water is calculated to find the radon anomaly to minimize the
Radon in soil
effect of meteorological parameters on radon emission. The radon anomalies observed in the region
NW Himalayas
have been correlated with the seismic events of MZ2 reported by Wadia Institute of Himalayas Geology
Earthquake precursor
Dehradoon and Indian Meteorological Department, New Delhi in NW Himalayas within 250 km distance
from the monitoring stations.
& 2009 Elsevier Ltd. All rights reserved.
0969-8043/$ - see front matter & 2009 Elsevier Ltd. All rights reserved.
doi:10.1016/j.apradiso.2009.05.016
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A. Kumar et al. / Applied Radiation and Isotopes 67 (2009) 1904–1911 1905
that the gas easily escapes from water and therefore has to be
Dharamshala
done without any aeration which might lead to out gassing. So the
32 Palampur water sample was collected in such a way that there was no
bubbling.
Fig. 2. Sketch of BMC2 radon probe and view of installed probe at monitoring station.
200
Radon (kBq/m3)
100
7
7
07
7
07
07
7
l-0
-0
-0
-0
-0
-0
-0
-0
-0
n-
n-
b-
ct
r
ar
ov
ec
ay
Ju
Ap
Ja
Ju
Au
Se
Fe
O
M
D
M
Date
Temperature (°C)
30
20
10
910
Pressure (mbar)
885
860
11.0
Avg. Wind Speed
(km/h)
7.0
3.0
80.0
Rainfall (mm)
40.0
0.0
100
Humidity (%)
60
20
Fig. 4. Daily variation of radon concentration in soil along with meteorological parameters viz. temperature, pressure, wind velocity, rainfall, and humidity at Palampur
from 01/01/07 to 31/12/07.
Table 1
Correlation coefficient of radon concentration in soil gas with different meteorological parameters at Palampur from 01/01/07 to 31/12/07.
Parameters Average (Avg.) Standard deviation (Std.) % Variation coefficient (Std./Avg.) Correlation coefficient
Radon (kBq/m3) 56 42 74 –
Temperature (1C) 19 5 26 0.5
Pressure (mbar) 873 5 0.6 0.3
Humidity (%) 53 21 40 0.5
Rainfall (mm) 5 11 220 0.001
Wind velocity (km/h) 6 1 17 0.5
soil gas at Palampur are shown in Table 3. Eight positive event of 2.2 M (31.21N, 77.21E) about a week prior to the event i.e.
anomalies and two negative anomalies were recorded. The first 12/03/07. Second anomaly was observed on 15/03/07 followed by
radon anomaly was recorded on 04/03/07 which was followed by event 3.2 M (31.11N, 78.21E) 12 days before the event which
ARTICLE IN PRESS
1908 A. Kumar et al. / Applied Radiation and Isotopes 67 (2009) 1904–1911
80
Radon (kBq/m3)
40
0
Jan-08 Feb-08 Mar-08 Apr-08 May-08
Date
25
Temperature (°C)
20
15
10
890
Pressure (mbar)
875
860
Fig. 5. Daily variation of radon concentration in soil along with meteorological parameters viz. temperature and pressure at Palampur from 01/01/08 to 14/06/08.
Table 2
Seasonal average value and standard deviation of radon concentration in soil and water with different meteorological parameters at Palampur and Dharamshala.
Parameter Time period Average Standard Parameter Time period Average Standard
(Avg.) deviation (Avg.) deviation (Std.)
(Std.)
occurred on 27/03/07. The third anomaly was recorded on 09/05/ recorded in the month of October on 02/10/07 and 04/10/07. These
07 followed by event 2.7 M (31.91N, 77.61E) four days before the anomalies are followed by 3.7 M event which occurred on 04/10/
event which occurred on 13/05/07. The fourth anomaly was 07 in NW Himalayas. The seventh positive anomaly was recorded
recorded on 18/06/07 followed by event 2.6 M (31.11N, 78.11E) 11 on 19/01/08 followed by 2.8 M (32.11N, 76.71E) event which
days before the event which occurred on 29/06/07. The first occurred on 24/01/08. The second negative anomaly was recorded
negative anomaly was recorded on 09/07/07. This anomaly is on 23/02/08 which was followed by 2.2 M (31.01N, 78.11E) event a
correlated with Uttarakashi earthquake of 5.0 M which occurred week prior to the event i.e. on 01/03/08. After a gap of four
on 22/07/07 13 days prior to the earthquake. Two anomalies were months last positive radon anomaly was observed on 08/06/08
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A. Kumar et al. / Applied Radiation and Isotopes 67 (2009) 1904–1911 1909
Avg
2.7 M
100
0
Jan-07 Feb-07 Mar-07 Apr-07 May-07 Jun-07 Jul-07 Aug-07 Sep-07 Oct-07 Nov-07 Dec-07
Date
Fig. 6. Daily variation of radon concentration in soil with seismic events correlated at Palampur using BMC2 probe from 01/01/07 to 31/12/07.
80
2.8M Avg ± 2Std 2.2 M
Avg
Radon (kBq/m3)
2.6 M
40
0
Jan-08 Feb-08 Mar-08 Apr-08 May-08
Date
Fig. 7. Daily variation of radon concentration in soil with seismic events correlated at Palampur using BMC2 probe from 01/01/08 to 14/06/08.
Table 3
Correlation of radon anomalies recorded at Palampur in soil gas with seismic event.
Date of Date of Latitude Longitude Depth Magnitude Epicenter distance % Variation from Precursor time
anomaly event (1N) (1E) (km) (km) (Avg726) (days)
a
Negative anomaly.
which was followed by 2.6 M (31.61N, 77.11E) event five days prior which occurred on 12/03/07. This event is also correlated with the
to the event. positive soil gas anomaly observed on 04/03/07. Two negative
The daily variation of radon concentration in groundwater at radon anomalies were recorded on 23 and 28/ 06/07 followed by
Dharamshala from 01/01/07 to 31/12/07 is shown in Fig. 7. The event 2.6 M (31.11N, 78.11E) which occurred on 29/06/07. This
average value of radon for groundwater at Dharamshala for this event is also correlated with the positive soil gas anomaly
time window is reported to be 59 Bq/l with a standard deviation observed on 18/06/07. The first positive radon anomaly was
(Std.) of 33 Bq/l. The percentage variation coefficient (Std./Avg.) of recorded on 19/07/07 which was followed by Uttarakashi
radon is 55%. The daily variation of radon concentration in earthquake of 5.0 M three days prior to the event which
groundwater at Dharamshala from 01/01/08 to 31/07/08 is shown occurred on 22/07/07. This event is also correlated with the soil
in Fig. 7. The average value of radon for groundwater at gas negative anomaly recorded on 09/07/07. Second positive
Dharamshala for this time window is reported to be 20 Bq/l with anomaly was observed on 01/02/08 followed by 2.4 M (31.21N,
a standard deviation (Std.) of 9 Bq/l. The percentage variation 78.01E) event occurred on 07/02/08. The fourth negative radon
coefficient (Std./Avg.) of radon is 45%. Radon anomalies observed anomaly was recorded on 21/02/08 which was followed by 2.2 M
in groundwater at Dharamshala are shown in Table 4. Six positive (31.01N, 78.11E) event which occurred on 01/03/08. This event is
anomalies and five negative anomalies were recorded. The first also correlated with the soil gas negative anomaly recorded on 23/
negative radon anomaly in groundwater was recorded on 09/03/ 02/08. The third positive anomaly was recorded on 21/03/08
07 followed by 2.2 M (31.21N, 77.21E) three days prior to the event followed by 3.2 M (32.81N, 76.21E) event which occurred on
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1910 A. Kumar et al. / Applied Radiation and Isotopes 67 (2009) 1904–1911
Table 4
Correlation of radon anomalies recorded at Dharamshala in ground water with seismic event.
Date of Date of Latitude Longitude Depth Magnitude Epicenter distance % Variation from Precursor time
anomaly event (1N) (1E) (km) (km) (Avg.726) (days)
a
Negative anomaly.
190 5.0 M
Avg ± 2Std
Avg 2.2 M
2.6 M
Radon (Bq/l)
95
0
Jan-07 Feb-07 Mar-07 Apr-07 May-07 Jun-07 Jul-07 Aug-07 Sep-07 Oct-07 Nov-07 Dec-07
Date
Fig. 8. Daily variation of radon concentration in water with seismic events correlated at Dharamshala using RAD 7 from 01/01/07 to 31/12/07.
2.4 M 3.2 M
2.5M
60
2.2 M Avg ± 2Std
2.2 M
2.4 M Avg
Radon (Bq/l)
30
0
Jan-08 Feb-08 Mar-08 Apr-08 May-08 Jun-08 Jul-08
Date
Fig. 9. Daily variation of radon concentration in water at Dharamshala using RAD 7 from 01/01/08 to 31/07/08.
24/03/08. Two anomalies were recorded in the month of April on spatially and temporally clustered earthquakes, the largest earth-
22 and 24 which was followed by the event 2.2 M which occurred quake is assumed to precede the anomaly (Hartmann and Levy,
on 25/04/08 in NW Himalayas. The fifth positive anomaly was 2005). The area under study reveals seismicity associated with
observed on 17/05/08 followed by 2.5 M (77.11N, 31.31E) event five active faults and folds trending normal or oblique to the
day prior to the event i.e. on 22/05/08. The fifth negative anomaly Himalayan trend which leads to the under thrusting of the blocks.
was recorded on 19/06/08 which was followed by 2.4 M (77.31N, The thrust planes which show regional extensions are frequently
31.41E) event which occurred on the same date in NW Himalayas intersected by transverse lineaments/faults which control the
(Figs. 8 and 9). neo-tectonic activity of the region and have resulted in the
In present studies the seismic events of magnitude r5 within contemporary morphological readjustment including the drai-
the epicenter distance of 250 km from the monitoring site (which nage shifts, recurrence of slope failures along the main structural
is within the radiosensitive range) are correlated. In the case of line and its offshoots, etc. (Dhar et al., 2003). Therefore possibility
ARTICLE IN PRESS
A. Kumar et al. / Applied Radiation and Isotopes 67 (2009) 1904–1911 1911
of minor shocks has the potential to generate anomalies at long Dhar, S., Randhawa, S.S., Sood, R.K., 2003. Lineament control and seismo-tectonic
distances and facilitate the activation/opening of the passageway activity of the area around Dharamsala, Himalayan frontal zone, Himachal
Pradesh, India. In: geohazards in North–West Himalayas, Indian geologists
along the thrusts, lineaments/ faults for the carrier gas. association, Punjab University, Chandigarh, pp. 28–29.
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as well as groundwater anomaly but the time of anomaly is changes associated with the earthquake sequence in June 2000 in the South
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