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Theoretical aspects
The hadrons inside an atomic nucleus interact through the fundamental interac
tions, viz., the strong, the electromagnetic and the weak interactions. The nuclear
structure can be studied using these interactions as probes and the nuclear phenom
ena are essentially the observable response to the probes that act on the nucleus
through these interactions [1]. In gamma-ray spectroscopy, the probes are gen
erally hadrons that interact with the nucleus through strong interaction and the
subsequent gamma decay is a result of electromagnetic interaction that responds
to the electric charges of the hadrons and their electric currents. A large part of
the knowledge of nuclei comes from the study of electromagnetic transitions since
the electromagnetic interaction is well understood compared to the nuclear forces.
Hence using the features of electromagnetic interaction, gamma-ray spectroscopy
has been extensively applied to probe various aspects of nuclear structure, such
as, energy (E), angular momentum (J), parity (zr), lifetime of the nuclear states;
branching ratios and mixing ratios of the transitions; transition probabilities be
tween two nuclear states etc.
The first section of the present chapter deals with the theory of gamma decay.
The second section is a discussion on the Shell Model (one of the successful models
of nuclear structure) that was used to interpret the experimental results obtained
through gamma-ray spectroscopy in the present thesis.
The nucleus may be regarded as made of point nucleons, each carrying a magnetic
dipole moment and in case of protons, a net charge as well [2]. The charge distri-
Chapter 2. Theoretical aspects 15
bution interacts with the radiation field near the nucleus causing “electric” tran
sitions and the intrinsic magnetism of each nucleon together with that generated
by current loops set up by the orbital motion of the protons induce “magnetic”
transitions in nuclei. The interaction between the nuclear currents and charges
with the radiation field is given by the coupling term:
where, j(r,i) and p(r, t) represent the current and charge densities in the nucleus
respectively. A(r, t) and ip(r, t) are the vector and scalar potentials of the radiation
field [3]. The interaction i?e.m. is considered as a perturbation causing transition
between stationary states of the nuclear Hamiltonian.
where <po(r) and </>k(r) are the wave functions of the initial and final states respec
tively and are products of nuclear and electromagnetic parts. p(Ef) is the density
of final states and is a product of the number of nuclear and electromagnetic states
per energy interval at Ef. In order to calculate the transition probability using the
above equation, it is necessary to make a multipole expansion of the perturbation
He rn_. This requires the decomposition of the potentials into electric and magnetic
multipole parts for the fields they describe. This results in the following expression
for the transition probability for multipole A from an initial nuclear state \JiMiQ
to a final nuclear state | [2]
Here k is the wave number and B(X; J*£ —» J/£) is the reduced transition probabil
ity which can be expressed in terms of the reduced matrix element of the multipole
Chapter 2. Theoretical aspects 16
operator for either electric (0\p (EX)) or magnetic (0\p {MX)) transition.
where the summation is taken over all A nucleons. are the spherical harmonics.
e(i) represents the electric charges for proton and neutrons in units of e. The free-
nucleon values are: e(i) = le for proton and 0 for neutron. In a shell model
calculation (Sec. 2.2.9) where some nucleons form a part of an inert core and a few
active nucleons in a truncated active space are used to determine the properties of
the nucleus, the above free-nucleon values cannot be used. Rather effective charges
have to be considered to account for such truncations. For example, the effective
charge of an active proton is taken to be 1.5e and that of an active neutron is taken
to be 0.5e in a typical shell model calculation. The magnetic transition operator
is given by
where gs(i) and gt(i) are the spin and orbital g-factors respectively. The free-
nucleon values are: gs(i) = 5.586/rN for a proton and -3.826/7,w for a neutron; gt(i)
= lpM for a proton and 0 for a neutron.
The transition probability IY(A), is expressed as number of decays per unit
time. When B(EX) is expressed in units of e2/m2A and B(MA) is expressed in
units of p%fm2X~2 the numerical values of W and B{A) are related as
ahcli0mtUTc)2X+lE?+lB(X in e2fm2X)
W(A) =
^c(2^)2lfSriiFl(i)2A+1^A+^(A in nlfm2X~2) ,
where, the relation, e2 = ahc — 1.44 MeVfm has been used, a = is the
fine structure constant, Mp is the mass of proton, pN = eh/2Mpc2 is the nuclear
magneton. Incorporating the numerical values of all the constants in the above
Chapter 2. Theoretical aspects 17
equation, the electromagnetic transition probabilities for the lowest three multi
poles are obtained as
The reduced transition probabilities can be obtained from the experimentally de
termined mean lifetime (r), branching ratio (BR), mixing ratio (5), conversion
coefficient (a) (defined in the following sub-sections) and the gamma-ray energy
(Ery) using the following relations. Here, the reduced transition probabilities for
electric transitions are given in units of e2fm2X and those for magnetic transitions
are in units of p2Nfm2X~2. The gamma-ray energy E7 is in units of MeV.
0.629
BR 52
B(E1) =
r(l +1a) 1 + S2 ’
816 BR 62
"^ t(1 + a) 1 + 52’
1760 BR 52
B{E3) = (r is in units of ps),
' E1r r(l +1a) 1 + S2 ’
56.8 BR 1
B(M1) (r is in units of fs),
"^ r(l +1a) 1 + S2 ’
74.1 BR 1
- ^ r(l +1a) 1 + S2 ’
0.1585 BR 1
B(M3) , (r is in units of s). (2.8)
E1 t(1 + a) 1 + 52
Weisskopf estimates
Electromagnetic interaction operators have well known structure and only weakly
perturb the strong nuclear interaction. Hence it is possible to compare experi
mentally determined 7-ray transition probabilities between nuclear states with the
theoretical prediction of nuclear models. Considering the extreme independent
Chapter 2. Theoretical aspects 18
particle model of nuclear structure (discussed in the next section) and considering
the nuclear transitions to be taking place by a nucleon moving from one single
particle orbit to another without affecting the rest of the nucleons in the nucleus,
the “Weisskopf single-particle estimates” for the EX and MX reduced transition
probabilities are given by
The angular momentum selection rule for the A-th multipole electromagnetic tran
sition from an initial state i to a final state / is given by
2.1.3 Lifetime
The lifetime or mean life of an excited nuclear state is the average amount of
time it takes for a radioactive nucleus to decay. It is connected to the transition
probability and the half-life by the relation:
1 _ h/2
(2.13)
W ~ 0.693
W = Y,W{i) . (2.14)
i
Chapter 2. Theoretical aspects 20
The relation between the half-life ti/2 and the partial half-lives ti/2(i) = In2/W(i)
is given by the relation:
—=Y 1 (2.15)
*1/2 i *1/2(1)
W(i)
Branching ratio — (2.16)
W
W{E2) S2
b(E 2) (2.19)
W(M1) + W(E2) “ 1 + 82
W(M 1) 1
b(Ml) (2.20)
W(M1) + W(E2) ~ 1 + 82
definite direction. An, oriented nuclei can be produced either as a result of nuclear
reaction or by a Coulomb excitation process or by a low-temperature orientation
technique. In the first two cases, the orientation-axis “z” is the beam direction.
In the latter case, the orientation-axis “z” is determined by the orienting external
fields. An oriented state can also be realized if the nuclei decay through successive
emission of two radiations 71 and j2 (Fig. 2.1). The observation of ji in a fixed
direction kx selects an ensemble of nuclei that has a non-isotropic distribution
of spin orientations. The succeeding radiation 72 then shows a definite angular
correlation with respect to ki [5]. In 7-7 directional correlation measurements only
the directions of the two radiations 71 and 72 are observed. This gives information
on the angular momenta carried away by the radiation, that is they yield spins of
nuclear levels. However they do not yield parities which can be determined from
polarization measurements.
The directional correlation function between 71 and 72 with multipolarities
Li + L[ and L2 + L2 emitted by a nucleus decaying through the cascade J—> J—> Jf
(Fig. 2.1) is given by
where 9 is the angle between ki and k2 and Pk(cos9) are Legendre polynomials [5].
------J,
, -,+^)
7 0
'___ J
72(L2+l!2)
■—~ Jf
Figure 2.1: A nucleus decaying through the cascade of two gamma transitions, 71 and
72 with multipolarities L% + l!l and L2 + l!2 from state to J/ via the intermediate
state J.
Dividing each coefficient A'kk by and expanding Eq. (2.21), one obtains
Here Akk are normalised coefficients which can be broken into two similar factors,
each factor depending on only one transition of the cascade. Thus for the general
case of mixed transitions,
where,
4 /T tr 7 t\ Fk(L1L1Ja)+2S1Fk(L1L[ja)+5fFk(L'1L,lJiJ)
= --------------------------- v", --------------------------- (2.26)
1 + Of
Here is the mixing ratio of 71 and Fk are the generalised F-coefficients when
the initial state is randomly oriented. A similar expression can be written for
AkiL2L2JfJ). The tables of the generalised F-coefficients can be found in Ref. [5,
6] and references therein. The generalised F-coefficients for mixed transitions
satisfy:
Fq(LL' JiJ) = 8ll> . (2.27)
It is assumed L' = L + 1. Theoretical values of only A22 and A44 are important
since usually only these can be observed experimentally.
In fusion-evaporation reactions (employed in the present thesis work), the initial
state (state J, in Fig. 2.1) is oriented, with the beam-direction as the orientation
axis. The projectile brings in orbital angular momentum in the m = 0 substate
with respect to the beam direction as the axis of quantization. The compound
nucleus formed in such reactions is strongly aligned with respect to the beam
axis. The orientation of an axially symmetric state is described by orientation
parameters B\ [7, 6] which are defined with respect to the orientation (symmetry)
axis. The index A refers to the tensor rank of the radiation field and its observation
Chapter 2. Theoretical aspects 23
/
/
/
Figure 2.2: The angles in a directional correlation of two successive radiations 71 and
72 emitted from an axial symmetric oriented source “S”.
7-rays are defined with respect to the orientation axis (chosen as the z-axis of the
reference system) (Fig. 2.2). The DCO function is then defined as (from Ref. [6]):
where,
A/ 4tt
HXlxxA91*2®) £ ^TT(Ai°Ag|A2g)yA(?(0i,O)r;2?(02,$) (2.29)
9i, 02 and $ are defined in the Fig. 2.2. BXl(Ji) are the orientation parameters
of the state Ji defined with respect to the orientation axis (z-axis). The indices
Ax and A2 are the tensor ranks of the statistical tensors that describe states Ji
Chapter 2. Theoretical aspects 24
and J. Since only directional correlations are considered and polarization is not
detected, Ai and A2 are even integers. The numerical values of the Clebsch-Gordan
coefficients (AiOAg|A2g) are given in [6]. A^2Al (71) are the generalized distribution
coefficient for 71 that connects two oriented states with orientation tensors of rank
Ai and A2.
FtAl (LihJJj) + + SjFf'
4!,a,(7i) = (2.30)
1 + i?
The tables of the above ^-coefficients is given in Ref. [6]. When the initial state
is random (Ai = 0), the Aa2Ai(7i) coefficients are given by Eq. (2.26) and the
i?AiAA2($i$2<h) reduces to ordinary Legendre Polynomial. Eq. (2.28) then represents
the ordinary directional correlation function given by Eq. (2.24).
The Ax2{rf2) are the ordinary directional distribution coefficients for 72. The
ordinary directional distribution coefficients for a transition from a state Ji to a
state Jj and with multipolarity L+L' is given by
where B* are orientation tensors describing the degree of orientation of the parent
nucleus and UA are deorientation coefficients. PA are the ordinary Legendre poly
nomials and P*2 are the unnormalized associated Legendre polynomials. Ax are
angular distribution coefficients which depend on the spin of the initial and final
Chapter 2. Theoretical aspects 25
state and the multipolarity of the 7-transition. The coefficients Aa,2 depend on
the electric/magnetic character of the radiation [8]. 0 is the angle that the emitted
quanta makes with the orientation axis whereas ip is the angle between the electric
vector E of the emitted quanta and the reaction plane (the reaction plane being
defined as the plane containing the orientation axis of the parent nuclear ensemble
and the direction of the primary radiation) [8].
The degree of linear polarization P(i9) of a 7 ray is defined as the difference
between the intensities of the radiations presenting an electric vector parallel to
the reaction plane (ip — 0°) and those with an electric vector perpendicular to that
plane (ip = 90°) [8, 11, 12}:
„ __ _ Amax
0,2 — CX.2A2 , (2.35)
a4 = a4A™ax . (2.36)
Chapter 2. Theoretical aspects 26
The attenuation coefficients depend on J, and the distribution of the nuclear state
over its m substates. According to Yamazaki [8], it is experimentally justifiable to
assume that partial alignment may be represented by a Gaussian distribution of
m-states characterized by a parameter a which is the half-width of the assumed
Gaussian distribution; in particular, the m-state population parameter is given by,
With this assumption otk are expressed as a function of J and a/J and are listed
by der Mateosian and Sunyar [14].
H2 and H4 are called linear-polarization mixing coefficients. They depend on
the initial and final spin and the mixing ratio (5) [15]. They can be derived for
mixed dipole-quadrupole (L = 1, L' = 2) and mixed quadrupole-octupole (L = 2,
L' = 3) transitions using the formalism given in Ref. [15, 10].
F2(ll) - (2/3)AF2(12) + 52F2(22}
H2(L — 1, L — 2) — (2.38)
F2(ll) + 28F2{12) + 52F2(22) ’
H4(L = 1, l/ = 2) = —1/6 . (2.39)
F2(22) - 6F2(23) + (2/3)52F2(33)
H2(L = 2,L — 3) = - (2.40)
F2{22) + 25F2(23) + <52F2(33)
5F4(22) - 28F4{23) + 208F4(33)
H4(L = 2, L' = 3) = (2.41)
30(F4(22) + 28F4(23) + 52F4{33)) '
One attempts to reproduce all the observable physical quantities of the nuclei
discussed in this section through mathematical models. A nuclear model is simply
a way of looking at the nucleus that gives a physical insight into as wide a range of
its properties as possible. The three important models are the liquid-drop model
that treats the nucleus as a macroscopic droplet of water, the shell model that
emphasizes the orbits of individual nucleons in the nucleus and the collective model
which complements the shell model by including the motions of entire nucleus. The
next section discusses the shell model that was used in the present thesis work.
a function of atomic number A. The short range and saturation property of the
9
0*
Mean binding energy per nucleon (MeV)
-4 T
w
wo>
y*
Figure 2.3: Binding energy per nucleon. (The figure is taken from the Internet).
nuclear force can be deduced from the behaviour of the binding energy curve. If a
nucleon were to interact with every other nucleon then the binding energy should
have roughly increased as A(A — l)/2 and consequently the density of the nucleus
should have increased. But the binding energy is almost independent of A (~8.5
MeV/nucleon for A>12) and the electron scattering measurements indicate the
nuclear density to be fairly constant. This implies that a nucleon interacts with
only its nearest neighbours, and it follows that the nuclear force must be short-
ranged and therefore becomes saturated. The saturation of the binding energy
prompted the assumption of localised interactions. Also in spite of the Coulomb
repulsive force the existence of the nucleus consisting of positively charged protons
and neutral neutrons indicate that the nuclear force is much stronger than the
Coulomb force and is also attractive for all nucleons at least in the range of the
nuclear diameter. Coulomb repulsion becomes important for heavier nuclei. The
nuclear force saturates but not the Coulomb force, so there is a slight decrease in
binding energy at higher A. The binding energy curve at low mass region where it
Chapter 2. Theoretical aspects 28
increases with increase in A shows several kinks which correspond to sudden rise in
binding energy per nucleon at certain numbers of neutron and/or protons, called
“magic numbers”. It was observed that nuclei with magic number of nucleons
(N = 8,20,28,50,82,126) of protons and/or neutrons (N = 126 is experimentally
established magic number for neutrons only) exhibit the following properties:
The shell model was successful in explaining these magic numbers in terms of shell
structure in analogy with the atomic shell model and derives its name from this.
This model describes the the structure of the nucleus as consisting of energy levels
grouped into shells and filled up by nucleons in order of increasing energy. The
magic numbers are nucleon numbers that correspond to shell closures. The energy
spacing between two shells is larger than that between levels within the same shell.
Although this is in analogy to the structure of the atom there are some some major
differences. In case of the atom the potential is supplied by the external Coulomb
field of the nucleus, in the nuclear case there is no external source, but the mean
field is exclusively due to the nucleon-nucleon interaction. Also there are two kinds
of nucleons giving rise to a new quantum number, isospin. Further, the nucleon-
nucleon interaction is attractive unlike Coulomb interaction and contains a strong
spin-orbit term. However, in spite of these differences the nucleons appear to move
in definite spatial orbits like electrons without collisions due to the weakness of
the nuclear long-range interaction and the Pauli exclusion principle. The Pauli
Chapter 2. Theoretical aspects 29
where the first term represents the kinetic energy of the individual nucleons and
the second term represents the mean field potential. ipTi represents single-particle
wave function and a represents the single-particle energy of the ith particle. The
choice of the mean field or single particle potential is equivalent to requiring that
the potential should be spherically symmetric. It should be relatively constant
inside heavier nuclei as indicated by the constant density observed in such nuclei
and should fall off rapidly outside the nuclear surface. There are several potentials
available to model the nuclear potential, these include the Woods-Saxon poten
tial, the square well potential, and the harmonic oscillator potential. These are
schematically represented in Fig. 2.4. The harmonic oscillator potential is widely
used due to its simplicity and ease of computation. It has the advantage that many
mathematical operations can be performed analytically. This potential has been
used in all shell model calculations in the present work and hence we discuss this
in detail.
Chapter 2. Theoretical aspects 30
Woods-Saxon
•* ---------Square Well
Here, Vo is the well depth, m is the mass of the nucleon, and oo is the oscillator
frequency of the simple harmonic motion of the particle, hu) is approximately
41A-1/3 MeV. The oscillator frequency oo can be written as,
u J™!L (2.44)
\jrnR2 ’
where R is the nuclear radius. Substituting Eqs. (2.43) and (2.44) in Eq. (2.42),
the energy eigenvalues for a three-dimensional harmonic oscillator obtained are
given by
Enl = (N + ^)huo , (2.45)
where,
iV = 2(n-l) + i (2.46)
N labels the oscillator shell, with n = 1,2,3,... and l = 0,1,2, ...n — 1. The l
(orbital angular momentum) values are labeled using the spectroscopic notation
of s,p, d, f for l = 0,1,2,3.... From the above equation one can deduce the levels
belonging to a given oscillator shell. All levels with same value of N (oscillator
Chapter 2. Theoretical aspects 31
shell number) has the same energy given by Eq. (2.45), i.e. they are degenerate
and the degeneracy is given by 2(21 + 1). By Pauli principle, each nl level can
contain 2(21 + 1) particles. The parity is given by
7T = (-1)' . (2.47)
Therefore, one oscillator shell contains only states with the same parity. Total
number of particles for all levels up to AT is l/3(N+l)(N+2)(N+3). However only
first three magic numbers are reproduced correctly this way, as shown to the left
of Fig. 2.5.
The inclusion of a l2 term splits each oscillator level into levels with different
l as seen in the middle portion of Fig. 2.5. The effect of the l2 term increases
with increase in orbital angular momentum. So orbitals with higher values of l are
attracted more and their energies get lowered compared to low l orbits with same
oscillator shell number N. The addition of the l2 term gives a potential intermedi
ate between the harmonic oscillator and the square well since it is equivalent to
a more attractive potential at larger radii and comes closer to the desired effect of
a more constant interior potential [17]. But even with this correction, the magic
numbers are not reproduced correctly.
J=l + s. (2.48)
A single nucleon has s = ±|, so the possible values of the total angular momentum
are j = l±\ (except for Z = 0, in which case only j = \ is allowed). The spin-orbit
Chapter 2. Theoretical aspects 32
•3d 3/2
\ _--------------------------,4c
-4s - -------------------------------- in
\___________________________ .'**^870
-3d-
........... "-3Jm
-2g- -< -.v _______________ "^lSfl
‘tx-T.______________ lill/2
N=5 82 'Ztm
—lh
{70 } ___________"lhna
1m ______ ---------------------------- 2d 3/2
****** y— —3s • -•" ''3sl/2
----- 2d
✓ *8 7/2
N=4 ____ ° 5/2
—Ig- < 50
hm
; 40; ------------------------ ig9/2
-----------------------2p1/2
I&G) : 8 : 8
‘P 1/2
N=1 -lp-
lp 3/2
■: 2 ;
Harmonic spin-orbit
l2 term +
oscillator term (l.s)
Figure 2.5: Single-particle energies for a simple harmonic oscillator, a modified harmonic
oscillator with l2 term, and a realistic shell model potential with l2 and spin orbit (l ■ s)
terms. Here N labels the oscillator shell
Chapter 2. Theoretical aspects 33
interaction is written as
Here V(r) is the central potential and Vis is a strength constant. The (l • s) term
causes the degenerate levels with same l to split into j = l± | levels with degeneracy
(2j + 1) which is the number of the magnetic substates for a given j. Hence by
Pauli principle the maximum number of nucleons that can be accommodated in
each orbit is 2j + 1. For example the 2p orbit splits into 2p3/2 and 2pi/2 (since
/ = 1 in this case). The maximum number of nucleons allowed in the 2p3/2 level is
2 x | + 1 = 4 and in 2pi/2 level is 2 x | + 1 = 2.
The expectation value of the operator l- s for states with definite l, s, j is given
by
= forj = l + 7,
= ^(J + l)*2, forj = l~\- (2-50)
For any pair of states with l > 0, the energy difference between the states is given
by:
<r-^,+i-(f-fUrs(2'+1)s2' (2-51)
The sign of the radial part of the spin-orbit potential is chosen to be negative so
that the member of the pair with larger j is pushed downward as observed exper
imentally. The right part of Fig. 2.5 shows the effect of the spin-orbit coupling on
the level system. Now the shell closures appear at the observed magic numbers.
The real shells are thus not necessarily comprised of the levels comprising a har
monic oscillator shell, particularly at higher levels. The parity of a wave function
is given by (—l)i as mentioned in Eq. (2.47). With only the harmonic oscillator
shell. Thus a real shell bounded by magic numbers contains a majority of levels
of one parity called normal parity orbits and one level of opposite parity called
non-normal or unique parity or intruder orbit (originating from the next major
harmonic oscillator shell).
• The nucleons in the nucleus are assumed to move in a common (mean) po
tential.
• Most of the nucleons are paired so that a pair of nucleons contribute zero
spin and zero magnetic moment.
• The paired nucleons thus form an inert core, and therefore the predicted spin
and magnetic moment of even-even nuclei is zero.
• In the case of odd-A nuclei the properties of the nucleus are characterised by
the unpaired nucleon.
• For odd-odd nuclei, the properties of the nucleus are characterised by the
unpaired proton and neutron.
From this one can see that all the protons are paired to give total angular momen
tum zero and hence according to the model, should not affect the ground-state spin
of the nucleus. The neutrons are paired up to lpi/2 orbital with one odd neutron
in ld^/2 orbital. Thus the theory predicts the ground state spin-parity as 5/2+ and
experimentally it was found to be the same. If there are three particles in a j shell
then two of them can couple to zero angular momentum and the resultant spin is
j due to the unpaired nucleon. This J — 0 coupling of pairs of identical nucleons
in same orbit can be used to predict spin-parity of excited states formed by elevat
ing one particle to higher energy orbits. However there are discrepancies observed
between prediction and observation when the prediction is based only on the rules
mentioned above. As an example, 33AS42 is considered where the neutrons are all
paired and the proton configuration is:
(lsi/2)21 (IP3/2)4 (lpi/2)21 (lcfe/2)6 (2si/2,)2ld3/21 (I/7/2)81 (2P3/2)4 (I/5/2)1 •
From the Single-particle shell model or the Independent particle model, the pre
dicted ground state spin of 33A.S42 should be § . But experimentally the ground
state is |~. This required a modification in the rule which states that if a high
spin orbital (in this case I/5/2) comes after a low spin orbital (2p3/2 in this case),
the high-spin orbital fills faster, pairing its particles before the low-spin orbital can
be filled completely. Following this rule the ground-state configuration of 33A.S42
becomes:
(l^X/2)21 (I-P3/2)4 (lPl/2)21 (1^5/2)6 (2Si(/2)2ld|^21 (I/7/2)81 (2p3/2)3 (1/5/2)2-
This modification in the model is put in the form of pairing potential, which gives
paired nucleons a lower energy than unpaired ones, and which increases with in
crease in l [16]. The pairing interaction is a “residual interaction” not envisaged
within the central potential.
2.2.4 Isospin
The proton and the neutron are regarded as two different charge states of the same
particle, the nucleon, which are indistinguishable under the strong interactions. In
analogy with intrinsic spin, each nucleon is assigned an isospin T — 1/2. Protons
Chapter 2. Theoretical aspects 36
= X+< = - 2) (2.53)
and
(2.54)
n~z<t<a.
(2.55)
2 ~ “ 2
A given T has projection quantum numbers, Tz = T,T — 1,.. . — T, for example,
if T = 1, then Tz = 1,0, —1. T can never be less than its projection, i.e., T > Tz.
The p-p, n-n and p-n systems have:
Figure 2.6 shows the level occupation and the spin-directions for the above three
systems. The n-n and p-p systems are allowed to exist only in S = 0 (anti-parallel
spin orientation) state by the Pauli principle. Tz calculated from the definition
given above comes out to be 1 and -1 respectively and hence T = 1 for these
two systems. The n-p system has Tz = 0. Experimentally the n-n, p-p and n-p
interactions are found to be identical (charge independence of the nuclear force).
Therefore the S = 0 state for the n-p system must be identical to the n-n and p-p
systems and hence T = 1 in this case. But the Pauli principle allows n—p system to
exist also with parallel spins (5 = 1). This state then must have T — 0 since if the
only substate of a spin-like quantum number has a value zero, then the spin itself
has that value. In nature the p-p and n-n systems are unbound but the deuteron
which is a n-p system has one bound state with spin-parity 1+. Experimental
observations reveal the bound state wave function to be in predominantly 3 Si
Chapter 2. Theoretical aspects 37
Figure 2.6: Illustration of level occupation and and spin directions for the 2 nucleon
system. Protons are indicated by filled circles, neutrons by open circles. The total spin
and isospin quantum number are given on the left [17].
state with a small admixture of 3Di. Thus the only bound state of deuteron has
S = 1 and is therefore an isospin singlet state (Tz = 0, T = 0). This can also
be deduced from the fact that the p-p and n-n systems with T = 1 are unbound
and hence the identical n-p configuration with 5 = 0 and T = 1 in deuteron is
also unbound. The concept of isospin can be extended to heavier systems which
have several n-n, p-p, n-p pairs, by studying the properties of the isobaric or the
isospin multiplets, i.e., nuclei with same number of nucleons (same A), and the
same isospin, but different z-components of isospin (Tz). From the case of the
deuteron and isospin triplets the following observations can be made:
1. The charge independence of the nuclear force, i.e., the equivalence of n-p,
p-p and n-n forces applies specifically and only to the T = 1 coupling for the
p-n system.
2. Different spin couplings (isospins) have different energies, and the strength
of the interaction of two unlike nucleons in a T = 0 state is stronger (more
attractive) than for a T = 1 state.
3. Different isospins represent different spin couplings and can also represent
states in which nucleons occupy different orbits. Within the same nucleus
Tz remains the same but T can be different and such states with different T
Chapter 2. Theoretical aspects 38
differ in the orbits occupied by the protons and the neutrons or in the spin
couplings.
4. States in different nuclei of an isospin multiplet with same T are called iso-
baric analogue states. Such states differ in interchange of protons into neu
trons and vice-versa. The absolute binding energies of these states are identi
cal once they are corrected for Coulomb energies and the n-p mass difference.
The excitation energy and other properties such as spectroscopic factors and
electromagnetic transition strengths of these states are also similar.
5. In isobaric multiplets (in light nuclei where Coulomb effects are small) the
highest orbit symmetry and the lowest total energy occurs for the smallest
Tz nucleus of the multiplet. N = Z nuclei have the lowest Tz and hence
are most stable. That is why the valley of stability has N ~ Z nuclei until
a mass A ~ 30-40 where Coulomb effect shifts it to the neutron-rich side.
Generally, states of lowest isospin lie lowest and are most proton-neutron
symmetric states in the space and spin coordinates: that is, Pauli principle
favours low T.
in the nucleus.
The basic assumption in shell model of the existence of a central potential in
the nucleus under which nucleons orbit as independent particles is a good approxi
mation of the actual motion. But in reality, there is no pure central potential. The
actual Hamiltonian consists of kinetic-energy terms Ylk T(fc) and the two particle
interaction ^2k<lW(k,l). Schrodinger equation (Eq. (2.42)) now reads [3]:
'a a
zm+ £ iv(k,i) *(1,2, ...A) = £4(1,2, ...A) . (2.56)
Here the eigenvalue ea represents the single-particle energy with a labeling the
single-particle state \nljm). Any product of A single-particle wave functions <f>W
= ))—.<paA(f'(A)) satisfies the Schrodinger equation
and
Et = 40) + £r} , (2-62)
where |$[X) and E^ represent the supposedly small changes in the wave function
and the energy of the unperturbed state. Substitution of Eq. (2.57), (2.61) and
(2.62) in Eq. (2.56) yields
Disregarding the second-order quantities and separating the zeroth- and fist- order
quantities one gets:
if(0)|40)> = 40)|40}) , (2.64)
Multiplying Eq. (2.65) by (4°^l on the left and using Eq. (2.59) one obtains:
This is the energy shift in presence of residual interaction HW from the degenerate
case. The energy of the state |44 is given by:
where,
+(40>(1,2)|V(1,2)|4°>(1,2)) . (2.73)
Here the first term is the binding energy of the core. The second term expresses the
single particle energies of the two extra-core particles and the third term expresses
the two-body matrix elements of the residual interaction. For more than two
particles outside the inert core the multiparticle interaction can be expressed in
terms of the two-body matrix elements.
2k + 1 r
vk = —-— J V(ri- f2)Pk{cosO)dO (2.75)
yT _ Ej(2J + l){jlj2\V\jlh)jT
(2.76)
juh~ Ej(2/+1)
where, {jij2\V\jij2)JT stands for the matrix element of the two-body interaction
V for a state coupled to angular momentum J and isospin T. The monopole term
is the same for all relative orientations of j\ and j2, that is, all J values. So
it does not contribute to splittings of a multiplet but only gives an overall shift
to the multiplet. It is viewed as the mean energy brought to the nucleus by
the addition of two interacting nucleons irrespective of the relative orientation
of their orbits. The evolution of single-particle levels and subsequently of shell
gaps are to a first order governed by monopole interactions. It is the principal
origin of the mass dependence of relative single-particle energies. In particular, the
monopole p-n interaction leads to the changes in neutron single-particle energies
as a function of proton number and vice-versa. Thus it influences the evolution of
shell closures. The J-dependent part of the two-body matrix elements is contained
in the multipole components. The quadrupole component leads to quadrupole
deformation. The quadrupole moment is found to be sizable, it is strongest at
9 = 0° and 90°. The quadrupole component contributes to the splitting of the
multiplet. The long-range component of the residual interaction which is crucial
in producing the collective properties and non-spherical nuclei is simulated by the
quadrupole interaction. The multipole expansion of any interaction can be used to
estimate the effects of an arbitrary two-body residual interaction between nucleons
in any pair of single particle orbits [17].
Chapter 2. Theoretical aspects 43
This dependence on A is depicted in Fig. 2.7. The spacings get compressed for
heavier nuclei. There is a simultaneous decrease in all energy levels with increase
in A hence this effect does not alter the shell model predicted sequences of the
levels significantly. The other effect on single-particle energies comes from the
residual interactions. This can cause drastic changes in the energy and sequence
of the shell model levels. The residual interaction between closed shells of filled
orbits and a single valence nucleon outside that shell in an orbit j and magnetic
substate m alters the SPE of that orbit. The wave function of a closed shell is
spherically symmetric (J = 0), that is, the closed shell has no preferred direction
in space. Hence its interaction with the valence nucleon is independent of m, i.e.,
independent of direction. This implies that the shift in SPE is exclusively due to
Chapter 2. Theoretical aspects 44
Figure 2.7: Changes of single-particle energies with nucleon number, reflecting the de
pendence of energies of confined particles on the size of the containment volume [17].
Chapter 2. Theoretical aspects 45
the monopole part of the interaction between the closed and open shell nucleons
since that is the only multipole that is 9 independent (Pq[Cos9) = constant).
A major shell consists of orbits of different j values, and each of the j values of a
closed major shell can have a different (spherically symmetric) effect on each of the
valence j orbits, thus shifting them to different extents. Thus the relative single
particle energies in a given major shell depend critically on the specific lower-lying,
filled closed shells. The interaction of a given shell j\ with another shell j2 (closed
or open) depends on the extent of overlap between the two; orbits with same n, l, j
are likely to have higher overlaps. If one of the two interacting shells is closed then
the overlap is radial since as stated above, the interaction in this case in angle
independent.
The filling of neutron (proton) orbits can strongly change the proton (neu
tron) level order due to strong attractive p-n interaction. The proton and neutron
single-particle sequences are slightly different because of Coulomb potential. The
monopole interaction is given by Eq. (2.76). The monopole shift of a certain orbital
jx increases linearly with increasing number of nucleons in the orbital j2. As the
orbit j2 is occupied, the single-particle energy of the orbit ji, is changed by
where nj2 is the occupation number (operator) of orbit j2 [25]. At shell closures, all
other components except the monopole component vanish. The monopole compo
nent governs (spherical) SPEs on top of closed (sub)shells according to the above
equation. In open shell systems, its effects can be viewed through Eq. (2.78) as
effective single-particle energies.
The separation energy of an orbit calculated with the bare SPE of the config
uration space and including the effects of the monopole interaction is called the
effective single-particle energy (ESPE) and depends on the configurations. Thus
the spacing between the ESPEs defines the energies for the excitation of the indi
vidual nucleons, and thus the effective shell gaps [24, 26].
Chapter 2: Theoretical aspects 46
Two particles outside inert core in orbits ja and jb can couple to give total J =
integer values from \ja — jb\ to (ja + jb)- A two-particle wave function (space-spin
part) is given by [3]:
one finds
TYIq 771 b
= (~l)J^jb$JM(jb{l)ja(2)) ■ (2.82)
Chapter 2. Theoretical aspects 47
= (-i)J-2i$jM(i(i)i(2)) = -(-i)j^M(j(i)j(2)),
(2.83)
since 2j is always odd. Thus <hjM is antisymmetric for J even and symmetric
for J odd. Similarly the isospin part of the two-particle wave function is
antisymmetric for T even and symmetric for T odd. Thus the total two-
particle wave function for two nucleons will be antisymmetric if
J + T — odd . (2.84)
Many predictions for \jnJ) configurations are identical to those for \j2J) config
urations if seniority is conserved (where seniority (j/) is defined as the number of
unpaired particles in a state of angular momentum J in the configuration jn, so
that the number of unpaired particles is (n-v)). There are several ways of predict
ing the total angular momentum for a multiparticle configuration. The m-scheme
approach is one such approach that has been employed in the code used in the
shell model calculations in the present work.
Chapter 2. Theoretical aspects 48
Configuration mixing
Excited states generally do not have pure configurations but are complex linear
combinations of multiparticle wave functions. The residual interaction mixes con
figurations and for a given state the nucleus has only a certain probability to be
Chapter 2. Theoretical aspects 49
on the matrix element. There may be several states with close-lying energies that
can mix to give an observed nuclear state. A series of two-state mixing calcula
tions can however approximate such a situation. Two initial states with energy Ex
and E% and wave functions </>i and 02 with the same spin-parity and isospin are
considered [17]. Under the influence of the residual interaction V they mix to give
the observed nuclear states with energies Ej and Eu and wave functions ipi and
'ipu (Fig. 2.8). The task is to find the appropriate linear combination of (pi and </->2
%
Eii
02 AEs
E,
AE UNP
E,
0i AES
Et
Vi
where a2 + f32 = 1 . The wave functions and final energies are obtained by diago
terms of the unperturbed energies and the mixing matrix element are given by
D= 1 . (2.89)
Eqs. (2.88) and (2.89) are universal expressions completely independent of the
nature of interaction or the initial splitting [17].
chart to another.
The sdpfmw interaction is derived from an effective one body plus two-body Hamil
tonian and is composed of three parts: the USD (2s, Id) interaction, the McGrory
(1/, 2p) interaction and the Millener-Kurath cross-shell interaction [33]. It was
designed to operate in the (2s, ld)A“16"(1/, 2p)n model space with a single-value
of n and was developed to explain the 32 region. The core is assumed to be
160.
In the universal (2s, Id) interaction denoted by USD [34, 27, 28] the parameters
consist of 63 two-body matrix elements and three single-particle energies relative to
the 16 0 core that were determined from a least-squares fit to ~440 binding energies
in A = 18 - 39 nuclei. The McGrory’s interaction [35] consists of 195 TBME and
four SPE relative to 40Ca core. The starting point of the interaction is the (If, 2p)
effective interaction of Kuo and Brown [36]. McGrory performed a least-squares fit
to 29 binding energies in the A = 42 - 44 region with only eight (/7/2/7/2IUI/7/2/7/2)
TBME variable. The Millener-Kurath particle-hole interaction [37] was developed
to describe the non-normal parity states in the A = 16 region. A fairly good fit
was obtained to the T = 0 and 1, lp-lh states of 160 with the parameters of this
interaction.
Warburton et al. [33]: used the Millener-Kurath potential to generate 510 TBME
needed to describe the interaction connecting the (2s, Id) and (If, 2p) shells. Out
of these, selected TBMEs were varied to give a better agreement with the the T =
Chapter 2. Theoretical aspects 53
0 and 1, lp-lh states of 40Ca. For A <40 nuclei the A-0-3 dependence was adopted
for all the three interactions while for .4>40 nuclei the TBME of the Millener-
Kurath and McGrory’s interactions are fixed at their >1=40 values. In calculations
with (2s, ld)A~16~n(lf, 2p)n model space, the TBME of the USD are given an A
dependence appropriate to A — n rather than A. The single-particle energies are
assumed to be independent of A. The SPEs of the ld5/2, ld3/2 and lsi/2 orbits
are those of the USD interaction and SPEs of the four fp orbits are the relative
values of McGrory. The energy gap between (2s, Id) and (1/, 2p) was initially
determined from the difference between the experimental binding energies of41 Ca
and 40Ca. Later, this energy gap was fixed so as to best describe binding energies
of selected levels in the A = 35 - 43 region.
The Nushell@MSU code [30, 31, 32] is an m-scheme code at heart but uses angular
momentum and isospin projection to produce a basis with good J and good T if
desired. A basis state with given value of M does not in general have a definite
value of the total angular momentum J. However the angular momentum projec
tion operator can be used to construct explicit linear combinations of the m-scheme
Slater determinants which have good total angular momentum. The Hamiltonian
is evaluated in the reduced dimension (J,T) basis. This is much smaller than the
m-scheme matrix. This matrix is then diagonalized and the eigenvectors are then
generated in the full m-scheme basis before observables are calculated. The central
potential is a Harmonic oscillator potential. There is a library of model spaces and
interactions. The model space indicates the orbitals and the truncation within that
set of orbitals which is assumed for a given calculation. The basic inputs are the
single-particle matrix elements and the two-body matrix elements. The program
calculates reduced transition probabilities from which the transition probabilities,
lifetimes, branching ratios and mixing ratios can be calculated using Eqs. (2.7),
(2.13), (2.16), (2.17) and (2.18). The sequence of programmes for prediction of
energies of the nuclear states is given below:
Chapter 2. Theoretical aspects 54
1. SHELL makes a batch file that coordinates the program sequence and their
inputs.
2. NUBASIS makes a list of all possible m-scheme basis states for a given model
space together with a given set of restrictions. The single-particle states for
the calculation are contained in a data file, and restrictions can be placed in
both individual J orbits and major shells.
5. NULANCZOS finds the lowest N eigenvalues and eigenvectors for the matrix
by the Lanczos diagonalization method. The output of this program is the
set of eigenvalues and the eigenvectors in the projected basis.
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