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Mehran Ehsani1
Effects of Restitution and Specularity
Salman Movahedirad2
Shahrokh Shahhosseini1 Coefficients on Solid-Liquid Fluidized
Mahshid Ashtiani2
Bed Hydrodynamics
1
Process Simulation and Control
Research Laboratory, School An Eulerian-Eulerian two-fluid model in combination with the kinetic theory of
of Chemical Engineering, Iran granular flow was applied to simulate a solid-liquid fluidized bed filled with stain-
University of Science and less-steel particles. The drag model of Gidaspow used in computational fluid
Technology, Tehran, Iran. dynamics simulations proved to be the appropriate model for predicting the bed
2
School of Chemical hydrodynamics. The effect of the restitution coefficient of the particles on the bed
Engineering, Iran University hydrodynamics was investigated numerically. For the solid phase wall boundary
of Science and Technology, condition according to Johnson and Jackson a specularity coefficient was intro-
Tehran, Iran. duced and evaluated. The change in specularity coefficient did not affect consider-
ably the bed behavior at the middle part, but at the walls it significantly influenced
the granular temperature. For specularity coefficients more than 0.5 the results do
not change noticeably.
1 Introduction fluidized bed behavior, there are only a few published works on
the effect of these parameters on the bed hydrodynamic
Solid-liquid fluidized beds are widely applied in many indus- [14, 15]. In one of the few studies in this area, Li et al. [15] ana-
tries [1]. As the bed hydrodynamics is of great importance in lyzed the impact of the specularity coefficient in a bubbling
design, scale-up, and operation of the solid-liquid fluidized fluidized bed and found a strong effect on the bed voidage
bed, a large number of attempts were made to comprehend it modeling.
theoretically and experimentally [2]. Among many models and In the present study, the Eu-Eu two-fluid model in combina-
software, which are used to simulate and predict fluidized bed tion with KTGF is employed to simulate a solid-liquid fluidized
behavior, computational fluid dynamics (CFD) tools are the bed. Since the effect of the drag coefficient on the fluidized bed
most promising ones to solve conservation and other required behavior is undeniable, two common drag models are applied
equations [3]. In general, there are two approaches to simulate in the simulations. In addition, CFD simulation data of the to-
hydrodynamics of solid-liquid fluidized beds by means of CFD tal bed voidage is compared with the experimental results. The
tools, i.e., Eulerian-Eulerian (Eu-Eu) and Eulerian-Lagrangian impact of restitution and specularity coefficients on the bed
(Eu-La). Most of the fluidized bed simulations use the Eu-Eu hydrodynamics is studied as well as the influence of several
two-fluid model due to its simplicity and short computational model input and solution parameters such as mesh size and
time. For prediction of particulate phase properties, kinetic time step. The effect of liquid superficial velocity on the bed
theory of granular flow (KTGF) is applied in most CFD simu- hydrodynamics is investigated by comparing the results with
lations [4–10]. the experimental values of the present study.
The results of the Eu-Eu two-fluid model depend on many
modeling parameters such as solid-liquid drag model, particle
restitution coefficient, specularity coefficient, boundary condi- 2 Experimental Setup
tions, and others. The effects of most of these parameters were
investigated by several researchers [11–13]. Although restitu- Experiments were performed to assure the accuracy of CFD
tion and specularity coefficients have great influences on the simulations. A schematic diagram of the experimental setup is
presented in Fig. 1. The fluidized bed dimensions are 0.6 and
0.08 m in length and diameter, respectively. Tap water is fed to
– the column bottom with a uniform flow rate of 1.01 ·10–3 m3s–1,
Correspondence: Dr. Salman Movahedirad (movahedirad@iust.ac.ir), measured by a precalibrated flow meter. Spherical stainless-
School of Chemical Engineering, Iran University of Science and Tech- steel particles with narrow size distribution and small diameter
nology, P.O. Box 16765-163, Tehran, Iran. in comparison to the bed diameter are filled into the bed.
Chem. Eng. Technol. 2015, 38, No. 10, 1827–1836 ª 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim www.cet-journal.com
1828 Research Article
The initial particle velocity was set to zero and the initial parti-
cle volume fraction (ep)1) was considered to be 0.6 according to
Figure 1. Schematic representation of the experimental setup. the experimental data. At the bottom inlet, water flows into the
bed with a specific velocity and exits the bed under atmospher-
Pressure transducers are placed at the top and bottom of the ic pressure. For the liquid and particulate phases, no slip wall
bed. The particles are initially packed in the bed up to 40 % of and partially slip wall conditions were considered, respectively,
the bed height with the initial bed viodage of 0.4. All experi- as proposed by Johnson and Jackson [24]:
ments were done at a constant temperature of 25 C. Details of
the experimental fluidized bed are listed in Tab. 1. ¶up;w
up;w ¼ A (18)
¶n
Table 1. Experimental conditions.
where A is the slip coefficient which depends on the specularity
Bed diameter [m] 0.08 coefficient and is defined as:
Bed height [m] 0.6 6mp ep; max
A ¼ pffiffiffiffiffi (19)
Particle material Stainless steel 3qpfp ep rp go
Particle diameter [m] 0.003
In the above equations, ep and ep,max denote the particulate
Particle density [kg m–3] 8030 volume fraction and its maximum value, respectively. q is the
granular temperature, which represents the particle collision
intensity. fp and tp,w are the specularity coefficient and partic-
3 Numerical Simulations ulate velocity, respectively. rp and mp signify the particulate
density and viscosity, respectively. In order to examine the
The Eu-Eu approach is applied for simulations and the kinetic effect of slip condition, different values of the specularity coeffi-
theory of granular flow is used to model the particle flow. It is cient are used in this study.
presumed that the particles are spherical in shape and have a
uniform size. The liquid phase is assumed to be incompressible
and its other physical properties are considered to be constant. 3.2 Solution Procedure and Method: Investigation
The detailed equations of momentum and mass conservation of Modeling Parameters
for each phase and other effective equations are summarized in
Tab. 2. Conservations of mass and momentum for both phases The effective equations, mentioned in the previous sections,
were solved during the simulations, see Eqs. (1)–(4) in Tab. 2. were solved under appropriate boundary conditions by means
Kinetic theory of granular flow provides a model for simulation of CFD techniques. The simulations were run for 30 s in un-
of the particles in Eqs. (11)–(15) in Tab. 2. steady state mode and time-averaged quantities were reported
To obtain the kinetic part of granular viscosity and conduc- for the last 25 s for reducing start-up effects. A first-order im-
tivity, the equation proposed by Syamlal et al. [16] was em- plicit upwind scheme was used for discretization of momen-
ployed. Eqs. (16) and (17) from Tab. 2 were used for momen- tum, granular temperature, and energy equations. The phase-
tum exchange between the liquid and solid phases. Therefore, coupled SIMPLE algorithm, which is a multiphase flow model,
two different drag models, i.e., from Wen and Yu [17] and is taken for pressure-velocity coupling. The focus of this section
Gidaspow [18], were applied. The particulate phase pressure
according to Eq. (5) from Tab. 2 was embedded into the mo- –
mentum conservation equation for the solid phase. Granular 1) List of symbols at the end of the paper.
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Research Article 1829
2
Particulate phase shear stress tp ¼ ep mp ðvp þ vp T Þ þ ep ðlp mp Þvp I – (6)
3
4
mp ¼ ep rp dp g0;pp ð1 þ epp Þ
5 pffiffiffiffiffiffi
rffiffiffi
q ep rp dp qp 2
þ ½1 þ ð1 þ epp Þð3epp 1Þep g0;pp (7)
p 6ð3 þ epp Þ 5
pp sin w
þ pffiffiffiffiffiffiffi
2 I2D
1
Liquid shear stress tl ¼ el ml ðvl þ vl T Þ el ml ðvl ÞI (8)
3
rffiffiffi
4 q
Particle bulk viscosity lp ¼ ep rp dp go;pp ð1 þ epp Þ (9)
5 p
2 !1=3 31
Radial distribution function
ep
g0;pp ¼ 41 5 (10)
ep; max
Granular temperature 3 ¶
e r q þ ep rp vp q ¼ pp I þ tp : vp þ kp q gp þ yp (11)
2 ¶t p p
pffiffiffiffiffiffi
15dp rp ep qp 12 2 16
kp ¼ 1þ h ð4h 3Þep g0;pp þ ð41 33hÞhep g0;pp (12)
4ð41 33hÞ 5 15p
1
h ¼ ð1 þ epp Þ (13)
2
yp ¼ 3kp q (15)
Chem. Eng. Technol. 2015, 38, No. 10, 1827–1836 ª 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim www.cet-journal.com
1830 Research Article
Figure 2. Bed voidage as a function of time in different mesh 4.1 Effect of Drag Coefficient
size at vf = 2.19 ·10–1 m s–1.
In fluidized beds, the drag force between the fluid and particles
has an important impact on the bed hydrodynamic, thus em-
3.2.2 Time Step ploying a proper drag model plays a significant role in simulat-
ing fluidized beds [27]. Two common drag models, which are
Several fixed time steps were used for the prediction of bed voi- widely used in solid-liquid interaction problems, are presented
dage. Fig. 3 shows the overall bed voidage over 30 s for different by Wen and Yu [17] and Gidaspow [18] and either of them is
time steps. As can be seen in Fig. 3 for the selected mesh size, proper for a limited particle fraction [30]. The Wen and Yu
time steps range from 10–3 to 5 ·10–3 and give very similar re- model [17] uses the correlation of Richardson and Zaki [31],
sults under the steady-state condition that are close to the which is valid when the internal forces are negligible [32]. The
experimental value. Obviously, a large time step of 10–2 and Gidaspow drag model [18] is based on the Ergun equation for
even 5 ·10–3 leads to some fluctuations. On the other hand, de- void fractions less than 0.8 and on an empirical correlation for
creasing the time step to 10–3 increases the computational time void fractions more than 0.8. Huilin and Gidaspow [33] pro-
considerably without significant enhancement in the accuracy posed a switch function to consider the continuity of these drag
or precision. correlations from dilute to dense regime.
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Research Article 1831
b)
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1832 Research Article
b)
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Research Article 1833
As in the solid-liquid fluidized bed, for the liquid that is sur- Moreover, it is obvious that the overall bed voidage is higher by
rounding the particles and prevents perfectly elastic particle increasing the fluid velocity, which is consistent with the results
collisions, the restitution coefficients differ from unity. On the of our previous work [40].
other hand, Figs. 5–8 indicate that a restitution coefficient of
0.9 and a specularity coefficient of 0.1 fitted the experimental
results well. 4.5 Distribution of Granular Temperature
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1834 Research Article
Symbols used
CD [–] drag coefficient
d [m] diameter
e [–] restitution coefficient
Figure 10. Time-averaged granular temperature as a function of dimensionless
distance for different (a) restitution coefficients, (b) specularity coefficients at g [m s–2] gravitational acceleration
h/hmax = 0.5 and vf = 2.19 ·10–1 m s–1. g0 [–] radial distribution
coefficient
h [m] expanded bed height
hmax [m] maximum expanded bed height
5 Conclusions I [–] unit tensor
I2D [–] second invariant of the deviatoric stress
An Eu-Eu two-phase model was employed to simulate a solid- tensor
liquid fluidized bed by means of the CFD method. To investi- k [–] diffusion coefficient for granular energy
gate the effect of different modeling parameters on the bed n [–] normal vector
hydrodynamics, different mesh sizes and time steps were eval- p [Pa] pressure
uated. The results showed that the mesh size has a stronger R [m] column radius
influence on the bed hydrodynamics prediction. Moreover, a t [s] time
time step, which could significantly increase the computational v [m s–1] velocity
cost, has no noticeable effect on the overall bed voidage predic- x [m] radial distance
tion. Comparison of the simulation results and the experimen- y [m] mesh size
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Research Article 1835
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