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1. Introduction
A non-Newtonian fluid is a fluid whose flow properties differ in many ways from those of
Newtonian fluids. Most commonly the viscosity of non-Newtonian fluids is not independent
of shear rate or shear rate history. In practice, many fluid materials exhibits non-Newtonian
fluid behavior such as: salt solutions, molten, ketchup, custard, toothpaste, starch suspensions,
paint, blood, and shampoo etc. In a Newtonian fluid, the relation between the shear stress and
the shear rate is linear, passing through the origin, the constant of proportionality being the
coefficient of viscosity. In a non-Newtonian fluid, the relation between the shear stress and the
shear rate is different, and can even be time-dependent. Therefore a constant coefficient of
viscosity cannot be defined. In the previous parts of this book, the mechanics of Newtonian
fluid have been mentioned. In this chapter, the common rheological models of non-Newtonian
fluids are introduced and several approaches concerned with non-Newtonian fluid flows are
( considered. In addition, the solution of common non-Newtonian fluid flows in a circular pipe,
annular and rectangular duct are presented.
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Incompressible Non-Newtonian Fluid Flows 55
3. Rabinowitsch-Mooney equation
Consider a one-directional flow of fluid through a circular tube with radius R, Figure 2. The
volumetric flow rate through an annular element of area perpendicular to the flow and of
width Br is given by
(11)
Q (12)
(13)
Provided there is no slip at the tube wall, the first term in equation (13) vanishes. Equation
(13) then can be written as
Q = 7rfr2(-Y)dr (14)
o
If the fluid is time-independent and homogeneous, the shear stress is a function of shear rate
only. The inverse is that the shear rate y, is a function of shear stress 'rx only and the
variation of 'rx with r is known from the following well-known equation:
r
(15)
R
(16)
_Ri-
.. _._._._._._
~vx
x
dr®J
Fig. 2. Geometric presentation of MR fluid in 0 circular tube
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56 Continuum Mechanics - Progress in Fundamentals and Engineering Applications
SU 4Q 4 'w
-
D
= -
JrR3
= -J'
,3
2 .
(-y)d, (17)
W 0
where u is the average velocity of the fluid flow and D is the diameter of the tube. For flow
in a pipe or tube the shear rate is negative so the integral in equation (17) is positive. For a
given relationship between , and y , the value of the integral depends only on the value of
'w. Thus, for a non-Newtonian fluid, as well as for a Newtonian fluid, the flow
characteristic 8u/D is a unique function of the wall shear stress 'w.
The shear rate y can be extracted from equation (17) by differentiating with respect to ,.
Moreover, if a definite integral is differentiated w.r.t. the upper limit ( 'w)' the result is the
integrand evaluated at the upper limit. It is convenient first to multiply equation (17) by ':u
throughout, then differentiating w.r.t. 'w gives
2 Su 3 d(Su / D) - 4 2 ( .)
(IS)
3 'w- +'w - 'w -y lo
D d,lO
_.
Yw
= Su
D
[~+4
1 'lo
4 (Su / D)
d(Su / D)]
d,w
(19)
Making use of the relationship dX/l: = dlnx, equation (19) can be written as
_y
W
= Su
D
[~+
4
1 d In(Su / D)]
4 d In,w
(20)
As the wall shear rate YlON for a Newtonian fluid in laminar flow is equal to (-8u/D),
equation (20) can be expressed as
. _. [~+
yw - YwN 4
1 d In(Su / D)]
4 dIn, lO
(21)
Equations (20) and (21) are forms of the Rabinowitsch-Mooney equation. It shows that the
wall shear rate for a non-Newtonian fluid can be calculated from the value for a Newtonian
fluid having the same flow rate in the same pipe, the correction factor being the quantity in
the square brackets. The derivative can be estimated by plotting [n(8ujD) against In 'wand
measuring the gradient. Alternatively the gradient may be calculated from the (finite)
differences between values of In(8du/D) and In 'w . Thus the flow curve 'w against Yw can
be determined. The measurements required and the calculation procedure are as follows.
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Incompressible Non-Newtonian Fluid Flows 57
3. Plot In(8du / D) against In 'wand measure the gradient at various points on the curve.
Alternatively, calculate the gradient from the differences between the successive values
of these quantities.
4. Calculate the true wall shear rate from equation (20) with the derivative determined in
'w
step 3. In general, the plot of In(8du / D) against In will not be a straight line and the
gradient must be evaluated at the appropriate points on the curve.
Example 1
The flow rate-pressure drop measurements shown in Table 3 were made in a horizontal
tube having an internal diameter 0 = 6 mm, the pressure drop being measured between two
tapings 2.0m apart. The density of the fluid, p, was 870 kg/m3. Determine the wall shear
stress-flow characteristic curve and the shear stress-true shear rate curve for this material.
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58 Continuum Mechanics - Progress in Fundamentals and Engineering Applications
pilot scale pipeline, direct scale-up can be done as described in Section 5. When the data are
in the form of shear stress-shear rate values (tabular or graphical), the flow rate can be
calculated directly using equation (17), where D is the diameter of the pipe to be used and
'w is the wall shear stress corresponding to the specified pressure gradient. Whether
obtained with a rotational instrument or with a tubular viscometer, the data provide the
relationship between , and f . Numerical evaluation of the integral in equation (17) can be
done using selected pairs of values of , and f ranging from 0 to 'w .
If the r - f , relationship can be accurately represented by a simple algebraic expression,
such as the power law, over the required range then this may be used to substitute for f, in
equation (17), allowing the integral to be evaluated analytically. Both these methods are
illustrated in the following example.
Example 2
Using the viscometric data given in Table 5 calculate the average velocity for the material
flowing through a pipe of diameter 37mrn when the pressure gradient is 1.lkPa/m.
Table 5.
Calculations
The wall shear stress is given by
8u 4 2 .
-
o
= 3
'zu
fr
'111
0
(-rfir
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Incompressible Non-Newtonian Fluid Flows 59
1: (Pa) y ,2 Y
0.00 0.0 0.00 (Centerline)
1.70 3.91 11.24
3.39 12.41 142.8
5.09 24.38 631.0
6.78 39.39 1812
8.48 57.14 4108
10.18 77.43 8016 (pipe wall)
Table 6.
By Simpson's rule
10.18
f ,2 yd, "'"10.18/6 [0+8016+4(11.24+613+4108)+2(142.8+ 1812)]= 17490 Pa3s-1
° 3
From equation (17)
U=
The above is the general method but in this case the visco metric data can be well
represented by, = 0.749yo.60 Pa, thus y = 1.62,16675-1. This allows the integral in equation
(17) to be evaluated analytically.
10.18
f f
T"
° °
This agrees with the value found by numerical integration and would give the same value
for u.
Note that the values of the apparent viscosity flo were not used; they were provided to
show that the fluid is strongly shear thinning. If the data were available as values of flo at
corresponding values of y, then , should be calculated as their product. The table of
values of ,2y (Table 6) illustrates the fact that flow in the centre makes a small contribution
to the total flow: flow in the outer parts of the pipe is most significant.
As mentioned previously, the minus sign in equation (17) reflects the fact that the shear rate
is negative for flow in a pipe. In the above calculations, the absolute values of y, and ,
have been used and the minus sign has therefore been dropped.
5. Wall shear stress-flow characteristic curves and scale-up for laminar flow
When data are available in the form of the flow rate-pressure gradient relationship obtained
in a small diameter tube, direct scale-up for flow in larger pipes can be done. It is not
necessary to determine the ,- y curve with the true value of y calculated from the
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BSL Transport Phenomena 2e Revised: Chapter 2 - Problem 2B.7 Page 1 of 7
Problem 2B.7
Annular flow with inner cylinder moving axially (see Fig. 2B.7). A cylindrical rod of
radius J<i,R moves axially with velocity Vz = Va along the axis of a cylindrical cavity of radius R as
seen in the figure. The pressure at both ends of the cavity is the same, so that the fluid moves
through the annular region solely because of the rod motion.
Cylinder of inside
Fluid at modified radius R Fluid at modified
pressure gpo '--! \ ~ pressure gpo
(b) Find the mass rate of flow through the annular region.
(c) 0btain the viscous force acting on the rod over the length L.
(d) Show that the result in (c) can be written as a "plane slit" formula multiplied by a
"curvature correction." Problems of this kind arise in studying the performance of
wire-coating dies.1
Vz In(r / R)
Answers: (a) - = ---
Va In J<i,
(b) w = 7rR2vap [(1 - J<i,2) _ 2J<i,2]
2 In(l/ J<i,)
(c) Fz = -27rLfLVa/ln(1/J<i,)
(d) Fz = -27r LfLVa (1 - ~E - ~E2 + ... ) where E = 1- J<i, (see Problem 2B.5)
E 2 12
Solution
Unlike the previous problem, the fluid here is flowing horizontally, so gravity will not influence its
velocity. If we assume no-slip boundary conditions, then the fluid velocity at the cylindrical rod
r = K,R is Va and the fluid velocity at the outer wall r = R is O.
Part (a)
Choose a cylindrical coordinate system with the positive z-axis pointing to the right, the direction
the inner cylinder is moving in. Then the fluid flows in the z-direction and varies as a function of
radius from the cylinder's axis.
Vz = vz(r)
1 J. B. Paton, P. H. Squires, vv. H. Darnell, F. M. Cash, and J. F. Carley, Processing of Thermoplastic Materials,
E. C. Bernhardt (ed.), Reinhold, New York (1959), Chapter 4.
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BSL Transport Phenomena 2e Revised: Chapter 2 - Problem 2B.7 Page 2 of 7
p=Jp(z)
Because Vz = vz(r), only rPTZ (the z-momentum in the positive r-direction) and rPzz (the
z-momentum in the positive z-direction) contribute to the momentum balance.
z+L
/ rP=:::.I.:+L
/
i
------I---r
rPr:::. I,.;, / \
- z J
~ I
\
\
I
\
\
I
/
\
I
_____ \ __ \..~_J
,
'"
L
Figure 1: This is the shell over which the momentum balance is made for flow in a horizontally
oriented annulus.
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BSL Transport Phenomena 2e Revised: Chapter 2 - Problem 2B.7 Page 3 of 7
-1'~+~-yt;-~-!!_(1'T )=0
L dr rz
So we have
d
d1' (TTrz) = O.
dvz
-fJ1'- = C1
d1'
Cl
vz(1') = --lnr+C2
fJ
C1
vz(r;,R) = --In(r;,R) + C2 = Va
fJ
C1
vz(R) = --In R + C2 = 0
fJ
(
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BSL Transport Phenomena 2e Revised: Chapter 2 - Problem 2B.7 Page 4 of 7
= ~ln!_
In I'\: R
Therefore,
Vz In(r / R)
Va In I'\:
Part (b)
dm d(pV) dV
w- - - -- -p-
- dt - dt - dt'
The volumetric flow rate dV / dt is average velocity times cross-sectional area.
w = p(vz)A
The average velocity is obtained by integrating the velocity over the area the fluid is flowing
through and then dividing by that area.
w = 27rp
}
t Ivan
K I'\:
(Ru) In u(R du)
')
~7rPVoR211 I d
= I u nu u
n I'\: K
2 2
27r pvaR2 (u-- u
+ -lnu ) 11
In I'\: 4 2 K
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BSL Transport Phenomena 2e Revised: Chapter 2 - Problem 2B.7 Page 5 of 7
Therefore,
Part (c)
The viscous stress Trz physically represents the force in the z-direction on a unit area
perpendicular to the r-direction. By evaluating Tn at r = r;,R and multiplying it by the surface
area of the inner cylinder, we obtain the viscous force acting on it over its length. The final point
to note is that because the fluid is acting from a larger radius r on the inner cylinder, which has a
smaller radius r;,R, we place a minus sign in front of Trz.
dvz
Trz = -/.LTr
= -/.L.!!:._ ( Vo In!:_)
dr lnr;, R
Vo J{ 1
= -/.L--'-
lnr;, r J{
/.Lvo 1
In r;, r
Fz = - (- /.LVo . ~) I ·27r(r;,R)L
In r;, r T=~R
27rAAL/.Lvo 1
In r;, AA
27r L/.Lvo
In r;,
27r L/.Lvo
-lnr;,
Therefore,
F __ 27rL/.Lvo
z- In(l/r;,)'
The minus sign here makes sense because the viscous (frictional) force of the fluid opposes the
motion of the cylinder, which is moving in the positive z-direction.
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BSL Transport Phenomena 2e Revised: Chapter 2 - Problem 2B.7 Page 6 of 7
Part (d)
To make the annulus a plane slit, we let the radius of the inner cylinder tend towards the radius
of the outer cylinder; that is, K, is very slightly less than 1.
F, = 27T Lj..lvo
- In K,
27T Lj..lvo
In(l - c.:)
c.:2 c.:3
In(l - c.:) = -c.: - - - - - ...
2 3
Substitute this formula into Fz.
c.: c.:2
1-----···
2 12
1+ Oc.: + Oc.:2
c.: c.:2
(- ) 1+-+-+···
2 3
€ ~2
-2" -"3 - ...
c.: c.:2
(- ) - - - - - 2c.:5 - ..•
2 4
Therefore,
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BSL Transport Phenomena 2e Revised: Chapter 2 - Problem 2B.7 Page 7 of 7
If we orient the slit horizontally so that pressure and gravity do not influence the fluid flow as is
the case in this problem, then Txz simplifies.
J Direction of
gravitational force
Figure 2: This is Couette flow in a horizontal slit with one moving wall at x = B.
p'Vo
Txz = - 2B
The viscous force acting on the moving wall is Fz = +T xz Ix=B . TlV L. There is no minus sign here
because the fluid acting on the wall has a lower x-coordinate than the moving wall at x = B.
Fz = (- p,Vo ) I . WL
2B x=B
WLp,vo
2B
Comparing this formula with the boxed result, we see that they are equivalent if E = 2B, the slit
width, and W = 27r. TlV should be a distance, but it's only an angle; thus, the fraction in the
boxed result is not truly a plane slit formula. The remaining series in parentheses then must be a
curvature correction.
E
'-._..-'
"plane slit" formula curvature correction
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