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To cite this article: Ala Abbas , Eyad Masad , Tom Papagiannakis & Aroon Shenoy (2005): Modelling asphalt mastic stiffness
using discrete element analysis and micromechanics-based models, International Journal of Pavement Engineering, 6:2,
137-146
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The International Journal of Pavement Engineering, Vol. 6, No. 2, June 2005, 137–146
†Turner-Fairbank Highway Research Center, 6300 Georgetown Pike, HRDI-11 McLean, VA 22101-2296, USA
‡Department of Civil Engineering, Texas A and M University, 3135 TAMU, College Station, TX 77843-3135, USA
{Department of Civil and Environmental Engineering, Washington State University, Pullman, WA 99164-2910, USA
§Turner-Fairbank Highway Research Center, 6300 Georgetown Pike, HRDI-11, McLean, VA 22101-2296, USA
This study uses the discrete element method (DEM) to simulate the dynamic mechanical behaviour of
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asphalt mastics. Asphalt mastics are defined as dispersions of aggregate fillers within a medium of
asphalt binder. The fillers refer to the fraction of mineral aggregate passing the 200-mesh sieve, (i.e.
smaller than 75 mm). Mastic measurements obtained using the dynamic shear rheometer were
compared to DEM predictions and available micromechanics-based models.
Three asphalt binders (ABD-1, AAM-1 and ABM-1) and four mineral fillers (glacial gravel, granite,
limestone and greywacke) were used to prepare the mastics in this study. The stiffening effect of the
mineral fillers was investigated at different filler volume fractions.
The DEM results captured the stiffening behaviour of asphalt mastics as a function of the volumetric
concentration of mineral fillers. The DEM results exhibited a high rate of stiffening that is typically
observed in experimental measurements of mastics at relatively low volume concentrations of fillers.
Compared to the DEM results, the micromechanics-based models were not sensitive to the dynamic
shear modulus of the asphalt binder, and they underestimated the stiffening effect of the mineral fillers.
contributes to workability. It was presumed that high In summary, two approaches have been used in
percent voids (low free asphalt content) might lead to stiff modelling the dynamic mechanical behaviour of asphalt
mixtures of low workability that are susceptible to mastics namely micromechanics and rheology-based
cracking, and that samples with low percent voids are models. Both approaches have also been extensively
susceptible to bleeding or shoving. used to model multi-phase composite materials such as
Shashidhar and Romero (1998) used a rheology-based metal alloys, fibre-reinforced composites, bitumen-water
model, the Nielsen model, to study the dynamic emulsions, polymer modified asphalts, asphalt mastics and
mechanical behaviour of asphalt mastics. In brief, the even asphalt mixtures. The first was developed to
Nielsen model was fitted to mastic data of different characterize composites of solid phases, while the latter
filler volume concentrations (filler-to-mastic ratio by have been utilized to model composites of solid particles
volume) through calibrating the two model parameters. dispersed in liquids. As reported by Lewis and Nielsen
A comprehensive discussion was presented on the effect (1970), the relative increase in the composite effective
of various filler characteristics such as average modulus with respect to the matrix modulus has
particle size, gradation, particle shape, presence of been shown to be equivalent to the relative increase in
agglomeration, degree of dispersion and asphalt-filler the composite effective viscosity with respect to the
interaction on the model parameters, and consequently the matrix viscosity. Hence, both approaches could
stiffening curve of the asphalt mastic. In an extension to potentially be used to model the asphalt mastic behaviour
this study, Shashidhar et al. (1999) used the Nielsen model over a broad range of temperatures within which the
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to study the same materials used by Harris and material might behave as a solid-like or liquid-like
Stuart (1995). composite.
Chen and Peng (1998) used the direct tension tester In this study, the mechanical behaviour of asphalt
(DTT) to study the effect of mineral fillers on asphalt mastics was simulated using the discrete element method
behaviour at low temperatures. An increase in both tensile (DEM). This was achieved by using different material
strength and tensile strain was noticed. The unexpected properties representing the binders and the fillers used in
increase in tensile strain was rationalized based on the this study. The effect of the volume fraction of the mineral
contribution of the mineral filler towards retarding crack fillers on the stiffness of the mastic was captured by using
propagation. appropriate binder and filler proportions that reflect the
Buttlar et al. (1999) used a generalized-self consistent target volume fraction. Finally, experimental data were
scheme (GSCS) model to characterize the dynamic compared to the DEM simulation results and micro-
mechanical behaviour of the asphalt mastic. Three mechanics models. It is believed that studying the
aggregate-related reinforcement mechanisms resulting in interaction among the mix constituents through DEM
the increased stiffness of bituminous materials were might provide better understanding of the behaviour of
discussed, namely volume-filling, physiochemical and asphalt mastics, and hence their performance.
particle interaction. It was suggested that while the first is
evident in asphalt mastics, the last reinforcement
mechanism is more pronounced in asphalt mixtures, 2. Objectives
where aggregates form a stone skeleton through which
stresses are transferred. The main two objectives of this study are, to:
Kim et al. (2003) tested sand particles mixed with plain (1) Develop a methodology to capture the dynamic
asphalt binders and asphalt mastics. An increase in fatigue mechanical behaviour of asphalt mastics using the discrete
life was noticed due to the use of mineral fillers. More element technique and compare simulation results to
significant effect was reported for hydrated lime compared experimental mastic data.
with limestone. (2) Study the sensitivity of different micromechanics-
Kim and Little (2004) studied the suitability of different based models, available in the literature, to the dynamic
micromechanics and rheology-based models in character- shear modulus of the asphalt binder, and compare the
izing the dynamic mechanical behaviour of asphalt model predictions to DEM results and mastic data.
mastics. The elastic-viscoelastic correspondence principle
was used to translate the elastic micromechanics models
into viscoelastic models that account for the time and 3. Experimental data
temperature dependency of the asphalt mastics. It was
concluded that micromechanics models provided a good Three asphalt binders (ABD-1, AAM-1 and ABM-1) and
fit to mastic data at low filler volume fractions, while four aggregates (glacial gravel, granite, limestone and
rheology-based models could capture the stiffening effect greywacke referred to as RF, RA, RD and RH,
of limestone fillers up to a volume fraction of 25%. It was respectively) were used in this study. Binders and
suggested that the behaviour of asphalt mastics containing aggregates were obtained from the SHRP materials
hydrated lime is controlled by physiochemical interaction, reference library. Aggregates were ground and the
and thus the effect of hydrated lime is highly binder material passing sieve No. 200 was used as mineral
dependent. fillers. Asphalt mastic specimens were fabricated by
Modelling asphalt mastic stiffness 139
Table 1. Rheological properties of the unaged plain asphalt binders rheometer (BBR) at low temperatures. All tests were
measured using the DSR at a radial frequency of 10rad/sec. performed within the linear viscoelastic range.
Experimental measurements of the dynamic shear
Temperature 258C
modulus, jG*j, and the phase angle, d, were recorded for
Dynamic shear modulus, jG*j Phase angle, d all binders and mastics at a radial frequency of 10rad/s.
Binder type (MPa) (degrees) Rheological measurements of the unaged plain asphalt
ABD-1 2.049 77.1 binders are presented in table 1. The highest coefficient of
AAM-1 1.039 61.5 variation (standard deviation/average) of 5.1% for jG*j
ABM-1 2.804 76.6
was obtained for ABD-1 binder, and the highest
All measurements are based on four replicates. coefficient of variation of 0.4% for d was obtained for
AAM-1 binder. The reader is referred to references
(Shashidhar et al. 1999, Shashidhar and Shenoy 2002) for
mixing each binder type with all four mineral fillers, further details on the specimen fabrication and testing.
resulting in 12 asphalt-filler combinations. The amount of Images of the fillers were captured using a scanning
fillers to be added to the binder was controlled in order to electron microscope (SEM). Example images are
attain nine filler volume fractions: 0, 6, 11, 17, 21, 25, 27, presented in figure 1. Shape and texture varied from
29 and 31%. To produce representative specimens, the particle to particle within the same filler sample. Based on
asphalt binder, in its unaged state, and the mineral fillers scanning a large number of particles, it was noticed that
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were both heated to a temperature of 1658C, followed by the granite has relatively flat surfaces with sharp edges,
mixing and stirring as the blend cooled down. The greywacke tends to be present in agglomerates of
resulting asphalt mastic was then poured into silicone relatively small-size particles, and glacial gravel particles
rubber moulds to make pellets for testing in the dynamic are somewhat round-shaped.
shear rheometer (DSR). Strain sweep data was obtained Figures 2 –4 present the stiffening curves for all asphalt-
using a Rheometrics RDA II DSR at a temperature of 258C filler combinations. It can be seen that the rate of increase
using plates of 8 mm diameter. Testing was limited to the in the mastic modulus increases with the increase in the
intermediate temperature of 258C in order to avoid settling filler volume fraction, and that different fillers result in
of aggregate fillers while testing, as is the case in the different stiffening curves. Higher variations among the
rotational viscometer (RV) run at high temperatures, and fillers are noticed at high filler volume fractions.
while moulding, as is the case in the bending beam Relatively speaking, greywacke has the highest stiffening
Figure 1. Particle shape of the mineral fillers tested in this study (a) granite—RA (b) limestone—RD (c) glacial gravel—RF (d) greywacke—RH.
140 A. Abbas et al.
K s 2ð1 2 np Þ
a¼ ¼ : ð3Þ
Kn ð2 2 np Þ
Figure 5. Example of a DEM mastic model consisting of 52% fillers by
volume. Where np was assumed to be 0.15 for the filler particles
(a ¼ 0.92), and 0.45 for the binder particles (a ¼ 0.71).
the need to conduct the analysis in a reasonable length of The filler contact stiffness parameters were determined by
time (i.e. 3 –4 h). developing a model consisting of only filler particles, and
The effect of the filler volume fraction was incorporated varying the K s and K n values until a filler-only shear
through the use of appropriate binder and filler proportions modulus of about 25 GPa, a typical value for the filler
that reflect the target volume fraction, which was calculated shear modulus (Zhou et al. 1995, Kim and Little 2004),
by dividing the filler volume by the total volume (i.e. binder, was obtained. It is worth mentioning however, that
fillers and voids). Concentrations ranging from 0 to 52% were varying the filler shear modulus within the range 15–
considered in the analysis. Care was taken to ensure the 30 GPa was found to have insignificant effect on the
randomness of the filler phase within the assembly. computed effective modulus of the asphalt mastic. The
same procedure was followed to determine the binder K s
4.2 Contact material property and K n values. In this case, the target binder-only shear
modulus values were varied from lower than 1.0 MPa to
Contact models in PFC2D are activated whenever the higher than 2.8 MPa to encompass the range of measured
distance between the centroids of two adjacent particles is binder stiffnesses (table 1). Table 2 presents the contact
less than or equal to the sum of their radii (i.e. the two stiffness parameters used in the simulation. Model
particles overlap). The linear contact model is used to calibration was necessary to account for the differences
simulate the interaction among particles. This model is between the actual material response and the DEM model
defined by two stiffness parameters for each particle in the prior to simulating the mastic behaviour. The DEM model
normal and tangential directions. The former is referred to was two-dimensional and hence, did not include one out-
as the normal stiffness, which relates the normal force to of-plane translational and two out-of-plane rotational
the normal displacement, and the latter is referred to as the degrees of freedom. The model calibration was also used
shear stiffness, which relates the shear force to the shear to reduce the influence of the particle shape and size on the
displacement. For each contact, an effective normal and model predictions, and to inherently account for the effect
shear contact stiffness is calculated from the particles’ of frequency through matching elastic model predictions
stiffnesses assuming that they act in series: to viscoelastic material stiffnesses measured at a particular
frequency.
K ½1 ½2
n Kn In this study, the influence of fillers was accounted for
Kn ¼ ð1Þ
K n þ K ½2
½1
n by changing the stiffness of the elastic contacts. This can
only be done if there is a negligible difference in the phase
angle of the asphalt binders and those of the corresponding
K ½1 ½2
s Ks mastics. It has been shown that most fillers affect the
Ks ¼ : ð2Þ
K ½1
s þ Ks
½2
stiffness of the binder (the magnitude of the dynamic
modulus) rather than its phase angle (Buttlar et al. 1999,
Where K n and K s ¼ effective normal and shear Kim and Little 2004). This finding was confirmed in
contact stiffnesses, respectively; K ½1 ½2
n and K n ¼ normal the experimental measurements used in this study as
142 A. Abbas et al.
Table 2. Filler and binder stiffness parameters and dem shear modulus predictions.
Particle type Shear particle stiffness Ks (N/m) Normal particle stiffness Kn (N/m) Predicted shear modulus G (MPa)
11 11
Aggregate 1.92 £ 10 2.08 £ 10 25636.17
Binder 1.66 £ 109 2.34 £ 109 276.71
1.66 £ 108 2.34 £ 108 36.58
1.66 £ 107 2.34 £ 107 4.71
1.66 £ 106 2.34 £ 106 0.81
the mastics had phase angles that were less than those of an analysis time step of unity (i.e. 1 s), equation (4).
the asphalt binders by only a maximum of 5%. As opposed to the gravitational mass that is equal to the
actual mass of the particle and contributes to the body
forces in the law of motion, the inertial mass contributes
4.3 Boundary and loading conditions to the inertia forces. In the absence of differential
density scaling, the inertial mass is equal to the
Four walls were used to load the asphalt mastic model.
gravitational mass.
This was achieved in two stages, namely the compaction
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Figure 6. Asphalt mastic stiffness ratios predicted using the discrete element method.
inability of describing this high rate stiffening has been the high filler volume concentrations using the DEM, similar
major limitation of the micromechanics models (Masad to that reported by Shashidhar and Shenoy (2002) and
and Niranjanan 2002). justified through using the Percolation theory.
Since the DEM predictions were obtained using
calibrated dynamic shear moduli (table 2) that are
different than those of the plain asphalt binders (table 1), 5. Micromechanics-based models
interpolation was used to predict the stiffening curves of
asphalt binders presented in table 1. Figures 7 –9 present Three micromechanics-based models are presented in this
the quality of fit for the discrete element predictions to section for comparison with the DEM simulation results
asphalt mastic data. A good fit is depicted in figure 7 to and asphalt mastic rheological measurements.
mastic data prepared using unaged ABD-1 binder. DEM
predictions, on the other hand, overestimated the stiffen-
5.1 Lower-bound hashin model
ing of the unaged AAM-1 binder (figure 8) and
underestimated the stiffening of the unaged ABM-1 This model is conceptualized on variational principles
binder (figure 9). In these figures, simulation results are that utilize classical minimum theorems to minimize
presented beyond the available experimental range in the strain energy within a composite in order to
order to demonstrate that a vertical asymptote is reached at estimate bound limits for the effective elastic moduli.
Figure 7. Asphalt mastic stiffness ratios measured using the DSR and predicted using the discrete element method; unaged ABD-1 binder and four
mineral fillers.
144 A. Abbas et al.
Figure 8. Asphalt mastic stiffness ratios measured using the DSR and predicted using the discrete element method; unaged AAM-1 binder and four
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mineral fillers.
A wide range of models belonging to this category is binder; Gf ¼ shear modulus of the aggregate filler;
available in the literature. In this study the lower-bound Km* ¼ dynamic bulk modulus of the asphalt binder;
Hashin model presented by Hashin and Shtrikman ff ¼ filler volume fraction and nm ¼ binder Poisson’s
(1963) is discussed. This model relates the composite ratio.
shear modulus, Gc* ; to the micormechanical material
properties as follows:
5.2 Generalized self-consistent scheme (GSCS) model
ff
Gc* ¼ G*m þ ð5Þ Generalized self-consistent scheme models are based on a
6 K* þ2G *
m m multi-layer spherical composite embedded in an infinite
1
þ ð1 2 ff Þ
Gf 2G*
m 5Gm 3K m þ4G*
* * homogeneous medium of unknown effective properties.
m
The derivation follows from the assumption that the strain
energy of the infinite medium is equal to the strain energy
* ¼ 2ð1 2 nm Þ * of the composite with no inclusion. The first analytical
Km G ð6Þ formulation of such models is credited to Christensen and
3ð1 2 2nm Þ m
Lo (1979, 1986) who derived a self-consistent scheme
where, Gc* ¼ dynamic shear modulus of the asphalt model for two-phase elastic materials. As is the case in the
mastic; G*m ¼ dynamic shear modulus of the asphalt variational models, this model satisfies equilibrium and
Figure 9. Asphalt mastic stiffness ratios measured using the DSR and predicted using the discrete element method; unaged ABM-1 binder and four
mineral fillers.
Modelling asphalt mastic stiffness 145
Figure 10. Effect of the dynamic shear modulus of the asphalt binder on the predictions of three micromechanical-based models; Lower-Bound
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Hashin Model, GSCS Model, and Inverse Rule of Mixtures (Gf ¼ 25 GPa, nf ¼ 0.15, and nm ¼ 0.45).
continuity equations. A rather lengthy set of equations the interaction among the filler particles within the
is used to predict the relative increase in the effective shear composite. The difference between model predictions and
modulus with respect to the dynamic shear modulus of the measurements increased at higher filler volume fractions.
binder: Nevertheless, better estimates were obtained using the
GSCS model than the other two models. Figure 10 also
!2 !
G*c G*c shows that these models tend to be insensitive to the
A þB þC ¼0 ð7Þ changes in the dynamic shear moduli of the asphalt binder
G* m G* m within the ranges used in this study.
Federal Highway Administration (FHWA) throughout his Kim, Y.R., Little, D.N. and Song, I., Effect of mineral fillers on fatigue
resistance and fundamental material characteristics: mechanistic
Eisenhower Graduate Research Fellowship. The authors evaluation. Transport. Res. Rec., 2003, 1832, 1–8.
would like also to thank Mr. Tom Harman from Turner – Kim, Y.R. and Little, D.N., Linear viscoelastic analysis of asphalt
Fairbank Highway Research Center for his valuable mastics. J. Mater. Civil Eng., 2004, 16, 122 –132.
Lewis, T.B. and Nielsen, L.E., Dynamic mechanical properties of
comments and Dr. Clay Ormsby for his help with the particulate-filled composites. J. Appl. Polym. Sci., 1970, 14,
scanning electron microscope. 1449–1471.
Masad, E. and Niranjanan, S., Microstructural finite element analysis of
the influence of localized strain distribution on asphalt mix properties.
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