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Electrohydrodynamic Drying—A Concise Overview


Tirtha R. Bajgaia; G. S. Vijaya Raghavana; Fumio Hashinagab; Michael O. Ngadia
a
Department of Bioresource Engineering, McGill University, Ste. Anne-de-Bellevue, PQ, Canada b
Kagoshima Women's Junior College, Kagoshima, Japan

To cite this Article Bajgai, Tirtha R. , Raghavan, G. S. Vijaya , Hashinaga, Fumio and Ngadi, Michael O.(2006)
'Electrohydrodynamic Drying—A Concise Overview', Drying Technology, 24: 7, 905 — 910
To link to this Article: DOI: 10.1080/07373930600734091
URL: http://dx.doi.org/10.1080/07373930600734091

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Drying Technology, 24: 905–910, 2006
Copyright # 2006 Taylor & Francis Group, LLC
ISSN: 0737-3937 print/1532-2300 online
DOI: 10.1080/07373930600734091

Electrohydrodynamic Drying—A Concise Overview


Tirtha R. Bajgai,1 G. S. Vijaya Raghavan,1 Fumio Hashinaga,2 and Michael O. Ngadi1
1
Department of Bioresource Engineering, McGill University, Ste. Anne-de-Bellevue, PQ, Canada
2
Kagoshima Women’s Junior College, Kagoshima, Japan

foods is performed at lower temperatures and basically


Electrohydrodynamic (EHD) drying is a novel method of non- low-energy consumption, but drying times are very long.
thermal processing. The drying can be carried out using either AC Reduction of energy usage in drying of biological mate-
or DC high voltages. The thermodynamic considerations regarding rials is a major concern among environmentalists in terms
the lowering of temperature under EHD drying include rapid rates of reducing greenhouse gas (GHG) emissions.[7,8] As these
of evaporation and exothermic interaction of the electric field with a
dielectric material. Multi-point and plate electrode systems are emissions are directly related to combustion of fossil fuels
efficient in accelerating drying of agricultural materials. Compared to heat the drying air, the evaluation of energy perform-
to hot air (convective) drying systems, EHD drying systems offer ance of existing dryers, and analyzing the options of reduc-
lower food production costs along with superior quality in terms ing energy consumption either by modifications to the
of physiochemical properties such as color, shrinkage, flavor, and dryers design or dryer operation are of prime interest.[9]
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nutrient content. Compared to convective and freeze-drying, EHD


drying systems, given their simpler design and lesser energy con- Another option is a research toward technologies that are
sumption, show great potential for bulk and industrial drying based on electricity, especially when electric current can
applications. be produced from clean energy sources such as wind or
hydro-power.
Keywords Air ions; Corona current; Drying rate; Non-thermal Aside from energy aspects, consumers demand superior
drying; Rehydration; Shrinkage quality products with natural color and a full complement
of flavors and nutrients. This is particularly the case for
INTRODUCTION high-value foods for the outdoors, instant meals, neutra-
ceuticals, baby foods, and seasonal and perishable foods
Conventional drying techniques are associated with con-
and herbs.[10] Developing an alternative method of drying
vective, conductive, radiative, and dielectric heating, as
such foods with a minimum adverse effect on indigenous
well as drying in superheated steam and lyophilization
quality is one of the major concerns of the modern food
either alone or in various combinations. These artificial
industry.
drying methods are all based on hot air drying, which is
Electrohydrodynamic (EHD) drying appears to comply
an energy-intensive process.[1] The use of higher drying
with both issues, namely low energy consumption and high
temperature produces drastic changes in the physical,
product quality, even though it is not a profoundly explored
chemical, and biological properties of food.[2] Loss of tex-
method of drying. In EHD-drying, electric fields of high
ture, color, and volatiles occurs during thermal drying of
intensity and standard industrial=domestic frequency (50
foods. Freeze-drying produces dehydrated products of
or 60 Hz) are applied so as to generate ionized forms of
superior sensory quality but is often prohibitively expens-
air-constituents within the foodstuff.[11] The ionized air is
ive at the commercial scale.[3,4] Energy losses in freeze-
a cluster of molecules bound together by the Coulomb
drying include loss of radiant energy to dryer walls, energy
force associated with an excess or deficiency of electrons.
losses within the existing product, energy dissipation in
The movement of the air ions in a strong electric field gen-
vacuum pumps, and energy released to the environment
erates an ionic wind. Loss of water vapor takes place as the
from freezers and freeze dryer units.[5] Microwave drying
water molecules orient themselves in the direction of an
also generates heat during drying.[6] Osmotic drying of
electric field. During this process, a lowering of entropy
occurs, which in turn lowers the temperature of the
Correspondence: G. S. Vijaya Raghavan, James McGill
Professor, Department of Bioresource Engineering, McGill material being dried. The thermodynamic factors involved
University, Macdonald Campus, 21,111 Lakeshore Rd., Ste. in the drop in temperature which occurs under EHD
Anne-de-Bellevue, Quebec, H9X 3V9, Canada; E-mail: vijaya. include the rapid rate of evaporation and the exothermic
raghavan@mcgill.ca

905
906 BAJGAI ET AL.

interaction of electric fields with dielectric materials. The drying. Compared to oven (convective) drying, EHD-
effects of air ions on biological material is the area of inves- drying lowers the cost of drying food and results in
tigation that has gathered the most interest.[12] superior food physiochemical properties such as nutrient
Krueger et al.[13] observed corona effects, namely an content, flavor, shrinkage, and color. Multiple electrode
ionic wind occurring within an electric field, by applying system in EHD drying shows a high potential for industrial
air ions to microorganisms. Evaporation phenomena of drying given their simplicity of design and lesser energy
air ions with various liquid substances such as saline sol- consumption compared to oven (convective) and freeze-
ution, ethyl alcohol, n-heptane, and water have been stud- drying. The non-thermal nature of EHD-drying may
ied by Hart and Bachman.[14] Carlon and Latham[15] present a wide range of applications in industrial drying,
observed that an increase in electric field strength increased given its capacity to produce high-quality processed
the drying rate of paper discs moistened with water. Chen products.[21,22]
and Barthakur[16] and Chen et al.[17] studied drying of In light of above discussion, this article seeks to examine
potato (Solanum tuberosum L.) slabs with air ions using a review the scope and prospects of EHD drying, considering
standard frequency electric field. Shigemitsu et al.[18] the need for new technologies of non-thermal processing of
showed the evaporation rate of distilled water to be directly biological materials.
proportional to the discharge potential. It is postulated
that the large ion current and ionic wind velocity were
responsible for the faster evaporation rate. Barthakur
and Arnold[19] showed the evaporation rate of water due EHD DRYING METHODS
to negative air ions to be greater than that associated with Electrohydrodynamic (EHD) drying consists of a verti-
positive air ions. Xue et al.[20] observed that increasing air cally moveable electrode with a sharply pointed needle pro-
flow during drying of radish (Raphanus sativus L.) slices in jected to a fixed horizontal grounded metallic plate on
a corona discharge decreased the drying rate. Isobe et al.[2] which the material to be dried is placed. The point elec-
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observed accelerated drying and enhanced sublimation of trode is connected to an AC or DC high-voltage trans-
agar gel under a DC-powered electric field–generating sys- former. The DC high-voltage transformer supplies either
tem. The evaporative effects of an electric field of standard negative or positive high-voltage. In order to set the desired
frequency (60 Hz) were found to be directly proportional to high-voltage parameters for EHD drying, the transformer
the electric field strength and to the duration of its appli- is connected to a voltage regulator. The input to the volt-
cation, but inversely proportional to the electrode gap. A age regulator is supplied from a 60-Hz, 110-V, AC source.
two-point electrode under an optimized electrode gap The electrode gap can be adjusted to the desired distance
allowed faster drying of an apple (Malus domestica Borkh. by moving the pointed electrode up and down (Fig. 1)[21].
cv. Fuji) slice than did a single-point electrode system.[11] The greater the voltage applied under EHD drying, the
Drying rates obtained for radish and spinach (Spinacia greater the drying rate; however, the voltage is maintained
oleracea L.) under a multi-needle emitting electrode system until the occurrence of sparkover. Optimum electrode gap
were as high as those achieved by oven drying.[21,22] How- and sharpness of the corona-generating needles are impor-
ever, the chlorophyll and ascorbic acid contents of the tant in achieving faster drying.
EHD-dried spinach were greater than those of oven-dried
spinach. The EHD-dried radish slices also showed better
color, greater subsequent water reabsorption, less shrink-
age, and less loss of solids in rehydration than oven-dried
radish slices.
Single and multiple needle EHD configurations enhanced
drying compared to convective drying. The resulting negative
or positive corona-associated winds vary linearly with the
applied electric field strength.[23–26]. In further studies on
EHD-drying, Jumah et al.[27] demonstrated the effectiveness
of electro-osmosis under an AC current for dewatering of
tomato paste. Energy losses from coronal discharge during
the drying of agricultural materials was found to be lesser
than under conventional drying techniques.[20,23,28]
In EHD drying, either AC or DC high voltage of ordi-
nary frequency (60 Hz) can be used. Multiple point-to-plate
electrode systems are efficient in accelerating drying of fruit
and vegetables and present significant prospects for bulk FIG. 1. Diagram of electrohydrodynamic (EHD) drying.
ELECTROHYDRODYNAMIC DRYING—AN OVERVIEW 907

RESULTS AND DISCUSSION carried out by Hashinaga et al.[11] and Bajgai and
Drying rates (moisture loss) under EHD, oven (convec- Hashinaga[21,22] showed the higher drying efficiency of
tive), and ambient air drying methods are shown in Fig. 2. sharp needles. Thus, the intra-electrode separation, elec-
The rate of drying with a five-needle electrode under ambi- trode gap, electric field strength, and electrode sharpness
ent condition (25C and 65% RH) demonstrates the effec- were determinant factors for EHD drying.
tiveness of EHD drying compared to ambient air (25C) More studies on the drying characteristics of wire and
and convective (60C) drying.[21] Lai and Wong[23] needle electrodes in EHD-drying are needed to understand
observed a similar drying rate by corona discharge from their influence on the drying mechanism. Various studies in
a needle electrode under ambient conditions and with air- this area show that both AC and DC currents are
flow. Under ambient conditions, until the occurrence of employed with high voltages. Figure 2 shows the EHD
sparking, as the applied voltage increased the drying due (25C and RH 65%), oven (convective) (60C) and ambient
to the corona effect was enhanced, but at high air flow air (25C) drying pattern of radish slices dried in an ordi-
velocities drying was independent of the applied voltage. nary fluorescent tube lighted chamber. The EHD drying
Barthakur and Arnold[19] showed ionic current and electric was more effective compared to convective and ambient
wind velocities to be greater for negative air ions than for air drying. A good agreement in slope was found between
positive air ions. Under 5.25 kV applied voltage with elec- the EHD and convective drying pattern of radish slice.
trode gaps of 5, 10, and 20 mm, the electric wind velocities However, further studies on AC and DC high-voltage mul-
for negative and positive air ions were 2.5, 1.7, and 0.8 m s 1 tiple needle electrode–to–plate electrode system with air
and 2.1, 1.5, and 0.7 m s 1, respectively. Under identical flow or reduced atmospheric conditions would be required
conditions ionic currents for the negative and positive air to fully assess the superior EHD drying protocol.
ions were 16.2, 7.8, and 2.4 mA and 9.0, 5.0, and 1.9 mA, As consumers prefer foods with greater nutrient content,
respectively. natural color, texture, and flavor, a demand for develop-
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After the introduction of a certain number of pointed ment of new technologies is obvious. Food quality is one
electrodes for a fixed drying area, the rate of drying did of the main preoccupations in food research. To address
not increase with the addition of further pointed electrodes, these issues, the relevant data on the effects of EHD drying
indicating the importance of intra-electrode separation.[21] on food quality were compiled and examined in view of
Hashinaga et al.[11] observed maximum drying under a assessing its future potential from an energy and environ-
13-mm electrode gap. The optimum electric field strengths mental prospective.
they noted for sharp and blunt needles in the experiment Conventional hot air drying of fruits and vegetables
were 4.4  105 and 4.7  05 V m 1, respectively. In previous leads to irreversible textural damage due to high shrinkage
studies on evaporating water and alcohol, Hashinaga which is related to the water volume removed during the
et al.[29] used a wire electrode instead of a needle electrode. process.[30] Figure 3 shows the shrinkage pattern under
Wire electrodes are blunt at their ion emitting ends, EHD (25C) and oven (60C) drying of radish slices. After
whereas needle electrodes are sharper. Further studies 7 h of drying, EHD and oven drying caused 55 and 80%
shrinkage, respectively.[21] These results are comparable

FIG. 2. EHD, oven (convective), and ambient drying pattern of radish FIG. 3. Shrinkage pattern for EHD- and oven (convective)-dried radish
slices. slices.
908 BAJGAI ET AL.

FIG. 5. Rehydration ratio for EHD- and oven (convective)-dried radish


 slices at 25C.
FIG. 4. Water absorption of radish slices dried with EHD (25 C) and
oven (convective) (60C).

to those obtained for apple slice shrinkage under EHD dry- Color is an important attribute of dried fruit and vege-
ing.[11] Many dehydrated products in the market with
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tables. Deterioration of color in dried fruits and vegetables


notably shrunken structures are due to the collapse of also indicates loss of nutrients. Carotenoids, and chloro-
capillaries. Such permanent damage brings loss of proto- phylls are among the most widely distributed pigments in
plasmic membrane permeability and loss of turgor pressure fruits and vegetables. Lycopene, carotenoids, and antho-
in the cell of the dried material. Protein denaturation, cyanins have antioxidant properties that may aid in reduc-
starch crystallization, and hydrogen bonding are associated ing the risk of cancer.[34] Table 1 shows the Hunter color
with excessive shrinkage.[31] The lesser shrinkage under ‘‘a’’ values of spinach during 7 h of EHD, oven and ambi-
EHD-drying represents the retention of the natural struc- ent air drying. The alteration of color of the dried spinach
ture of the biological material. after 7 h of drying was highly reduced for EHD drying
Water absorption and rehydration properties of EHD compared to oven (convective) drying, which in turn main-
and oven (convective)-dried radish slices at ambient tem- tained better color than ambient air drying. Total chloro-
perature (25C) are compared in Figs. 4 and 5. EHD dried phyll, chlorophyll a, chlorophyll b, and ascorbic acid
radish slices showed greater water absorption and rehydra- were higher in EHD-dried than oven-dried spinach.[22] In
tion ratios compared to oven-dried slices. High tempera- a different study, EHD-dried radish showed less loss in
ture drying of fruits and vegetables ruptures the subjected solids during soaking, greater water absorption, and better
plant cells, which results in loss of their water absorption color than oven-dried radish.[21] In another study, EHD-
properties. The reduced absorption of water and rehydra- dried apple slices did not show any observable product
tion ratio in oven-dried material is associated with a degradation, important color change, or formation of
collapse in structure and reduction in porosity.[32] Greater foreign substances.[11] An HPLC analysis carried out for
shrinkage also affects aroma retention, caking and sticki- organic acids and sugars in EHD and oven-dried spinach
ness, puffiness, and final moisture content of the samples (Table 2) showed identical peaks for organic acids,
material.[33]

TABLE 1
Hunter color value ‘‘a’’ for EHD (5C), oven (convective) (60C) and ambient air–dried (25C) spinach
Drying time (h)
Drying methods 0 3 5 7
EHD 20.5  1.9 18.5  2.1 17.5  2.1 16.3  2.2
oven (convective) 20.5  1.9 17.2  2.4 14.7  2.2 08.5  2.4
Ambient air 20.5  1.9 18.4  1.7 17.6  2.2 16.1  1.7
ELECTROHYDRODYNAMIC DRYING—AN OVERVIEW 909

TABLE 2
HPLC profile for organic acids and sugar for EHD and oven (convective)-dried spinach samples
Retention time (min) Peak area (relative)
Organic compounds EHD dried Oven (convective) dried EHD dried Oven (convective) dried
a
Organic acids
Citric 13.664 13.624 5472 1479
L:Malic 15.798 15.802 12,322 19,607
Succinic 18.676 18.638 3438 11,449
Fumaric 21.128 21.024 29,672 79,662
Propionic 25.275 25.244 17,671 29,913
Sugarsb
Fructose 6.924 6.806 1,791,548 1,506,103
a
Shimadzu LC-10AS chromatograph equipped with a Shodex SC-125S column, size, 4.6 mm  500 mm; mobile phase, 0.1% H3PO4,
flow rate, 0.3 ml=min; column temperature, 55C; detector, Shimadzu SPD-6A at 210 nm; recorder, Shimadzu Chromatopack C-R4A.
b
Shimadzu SCL-10 chromatograph equipped with a Shim-pack CLC-NH2(M) column; size, 6.0 mm  150 mm; mobile phase, 70%
CH3CN; flow rate, 0.3 ml=min; column temperature, 40C, detector, Shimadzu SPD-6A at 192 nm; recorder, Shimadzu Chromatopack
C-R8A.

indicating that EHD drying did not generate new undesir- of air ions, energy dissipation, post-dried food quality, and
able substances compared to convective drying. scale-up–related problems are needed.
The currents and voltage measured in various EHD dry-
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ing systems designed and employed by Lai and Wong,[23]


Bajgai and Hashinaga,[21,22] Hashinaga et al.,[11,29] Isobe ACKNOWLEDGEMENTS
et al.,[2] Chen and Barthakur,[16] Chen et al.,[17] and The authors gratefully acknowledge the financial sup-
Carlong and Latham[15] showed the existing ionic current port from Natural Sciences and Engineering Research
under EHD drying to be small in magnitude. Although Council (NSERC) and Fonds Québécois de la Recherche
the voltage applied remains high, the small current reduces sur la Nature et les Technologies (FQRNT).
the consumption of electrical energy to fairly low levels
during the drying process. The Townsend effect of second-
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